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1st International Conference on Smart City Innovation, ICSCI 2018

作者： Nofiana Raharjo, S.H. Istirokhatun, T. Susanto, H. Integrated Laboratory for Research and Services Diponegoro University Semarang Indonesia Master Program of Environmental Science School of Postgraduate Studies Diponegoro University Semarang Indonesia Department of Environmental Engineering Faculty of Engineering Diponegoro University Semarang Indonesia Department of Chemical Engineering Faculty of Engineering Diponegoro University Semarang Indonesia Jl. Prof Soedarto SH Tembalang Semarang Indonesia

Supply of sustainable clean water is an activity that must be carried out towards smart cities. Nevertheless, the availability of water is decreasing both in quality and quantity. Wastewater including domestic wastewater is a potential source that can be reused as clean water supply dealing with water scarcity. This is due to domestic wastewater is produced continuously in large amount. In addition, reuse can reduce the total cost of handling wastewater. One modern technology that can be used for domestic wastewater treatment is membrane technology. Characteristics, various types, advantages, disadvantages, and challenges of membrane technology for domestic wastewater were discussed. This paper presents a review of domestic wastewater reuse by using membrane technology. More specifically this paper discusses domestic wastewater. © 2019 IOP Publishing Ltd. All rights reserved.

关键词： Membrane technology

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Author Correction: Synergistic wall digestion and cuproptosis against fungal infections using lywallzyme-induced self-assembly of metal-phenolic nanoflowers

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Nature communications 2024年第1期15卷 9773页

作者： Fang Liu Yongcheng Chen Yue Huang Yutong Li Zhouyu Lu Haijie Han Xiaohui Song Qiao Jin Jian Ji Eye Center the Second Affiliated Hospital School of Medicine Zhejiang University Hangzhou PR China. MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and Engineering Zhejiang University Hangzhou PR China. Eye Center the Second Affiliated Hospital School of Medicine Zhejiang University Hangzhou PR China. 2317050@***. Eye Center the Second Affiliated Hospital School of Medicine Zhejiang University Hangzhou PR China. jinqiao@***. MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and Engineering Zhejiang University Hangzhou PR China. jinqiao@***. Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030032 P.R. China. jinqiao@***. State Key Laboratory of Transvascular Implantation Devices The Second Affiliated Hospital Zhejiang University School of Medicine Hangzhou PR China.

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Heavy metals concentration in mangrove tissues and associated sediments and seawater from the north coast of Persian Gulf, Iran: Ecological and health risk assessment

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Environmental Nanotechnology, Monitoring and Management 2021年 15卷

作者： Rezaei, Marzieh Kafaei, Raheleh Mahmoodi, Marzieh Sanati, Ali Mohammad Vakilabadi, Dariush Ranjbar Arfaeinia, Hossein Dobaradaran, Sina Sorial, George A. Ramavandi, Bahman Boffito, Daria Camilla Department of Environmental Health Engineering Faculty of Health and Nutrition Bushehr University of Medical Sciences Bushehr Iran Student Research Committee School of Public Health and Safety Shahid Beheshti University of Medical Sciences Tehran Iran Department of Biostatistics Faculty of Health and Nutrition Bushehr University of Medical Sciences Bushehr Iran Department of Environmental Science Persian Gulf Research Institute Persian Gulf University Bushehr Iran Systems Environmental Health and Energy Research Center The Persian Gulf Biomedical Sciences Research Institute Bushehr University of Medical Sciences Bushehr Iran Environmental Engineering Program Department of Chemical and Environmental Engineering College of Engineering and Applied Science University of Cincinnati Cincinnati 45221-0012 OH United States Department of Chemical Engineering Polytechnique Montréal C.P. 6079 Succ CV Montréal H3C3A7 QC Canada

We evaluated the concentration of copper (Cu), zinc (Zn), mercury (Hg), nickel (Ni), chromium (Cr), vanadium (V), and cobalt (Co) in the mangrove tissues (leaf and root) and adjusted sediments, as well as seawater samples in the north coast of the Persian Gulf from three counties (Mahshahr, Bord Khun, Asaluyeh). Assaluyeh and Mahshahr were selected because of their proximity to the oil and petrochemical industries and Bord Khun was considered for being away from pollution sources. The metal detected in highest concentration in mangrove leaves and roots was Cu (Asaluyeh: 1.507 μg/g and 1.198 μg/g, Bord Khun: 1.812 and 1.756 μg/g, and Mahshahr: 0.880 and 1.617 μg/g, for leaves and roots, respectively). For sediments, Cr (among the metals) had the highest concentration (1.325 μg/g) in Asaluyeh, whereas in Bord Khun and Mahshahr Ni was predominant: 2.542 and 2.237 μg/g, respectively. For seawater, Cu was the most abundant metal and Hg was the one with the lowest concentration. The bio-concentration factor for Zn and Cu revealed that mangroves in the study areas have suitable potential for phytoremediation of these two metals. Translocation factors from the roots to leaves also indicated higher transportability for Zn and Cu through the plant tissues, compared to the other metals. Ecological indexes quantified the contamination of sediments and revealed a low level of heavy metal accumulation in sediments of the north of the Persian Gulf. Human risk hazards appeared low in all the areas under study. Gas and petrochemical activities can be considered as a potential source of the discharge of heavy metals into the aquatic environment. © 2021 Elsevier B.V.

关键词： Asaluyeh Bord Khun Heavy metals distribution Mahshahr Mangrove ecosystem Pollution assessment

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Yogurt-inspired hybrid membrane vesicles for the prevention and treatment of Helicobacter pylori infection

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Cell Biomaterials 2025年第4期1卷

作者： Lujie Liu Yiming Guo Baikui Wang Yuanwei Pan Chenchen Zhao Zhiping Xiao Yu Liu Guocan Yu Xiaoyuan Chen Lang Rao Institute of Chemical Biology Shenzhen Bay Laboratory Shenzhen 518132 China Department of Diagnostic Radiology Yong Loo Lin School of Medicine and Faculty of Engineering National University of Singapore Singapore 119074 Singapore College of Animal Science Zhejiang University Hangzhou 310058 China Key Laboratory of Bioorganic Phosphorus Chemistry & Chemical Biology Department of Chemistry Tsinghua University Beijing 100084 China Clinical Imaging Research Centre Centre for Translational Medicine Yong Loo Lin School of Medicine National University of Singapore Singapore 117599 Singapore Nanomedicine Translational Research Program Yong Loo Lin School of Medicine National University of Singapore Singapore 117597 Singapore Theranostics Center of Excellence (TCE) Yong Loo Lin School of Medicine National University of Singapore Singapore 138667 Singapore Institute of Molecular and Cell Biology Agency for Science Technology and Research (A∗STAR) Singapore 138673 Singapore Department of Chemical and Biomolecular Engineering College of Design and Engineering National University of Singapore Singapore 117575 Singapore Department of Biomedical Engineering College of Design and Engineering National University of Singapore Singapore 117575 Singapore Department of Pharmacy and Pharmaceutical Sciences Faculty of Science National University of Singapore Singapore 117544 Singapore

Helicobacter pylori ( H. pylori ) infection is a critical initiating factor in numerous gastrointestinal diseases. Here, we present yogurt-inspired hybrid membrane vesicles (hMVs) engineered by fusing bacterial outer membrane vesicles (OMVs) with modified milk fat globule membrane vesicles (MMVs) to prevent and treat H. pylori infection. The hMVs function as binding site competitors, reducing bacterial adhesion while regulating epithelial integrity and immune responses. This dual mechanism synergistically inhibits H. pylori infection and promotes gastric epithelial repair. In vitro , hMVs demonstrated remarkable efficacy in accelerating scratch-wound healing, enhancing lipid raft formation, increasing tight junction protein ZO-1 expression, and promoting macrophage phagocytosis of apoptotic epithelial cells. In mouse models for both H. pylori prevention and treatment, oral administration of hMVs effectively reduced H. pylori loads by 86% and 66%, respectively. Additionally, this treatment mitigated inflammatory factor secretion, decreased neutrophil recruitment, and preserved the abundance of beneficial probiotics in the stomach.

关键词： Helicobacter pylori infection drug delivery nanomedicine extracellular vesicles nanobiotechnology

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TMIC-79. IDH1-R132H REWIRES AUTOPHAGY IN THE GLIOMA MICROENVIRONMENT TO FACILITATE TUMOR PROGRESSION AND RESPONSE TO RADIATION

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Neuro-Oncology 2024年第SUPPLEMENT_8期26卷 viii316–viii316页

作者： Banerjee, Kaushik Nunez, Felipe Mujeeb, Anzar Mausar, Ava Tronrud, Claire Zhu, Ziwen Taher, Ayman Kadiyala, Padma Carney, Stephen Garcia-Fabiani, Maria Belen Comba, Andrea Alghamri, Mahmoud McClellan, Brandon Faisal, Syed Nwosu, Zeribe Hong, Hanna Qin, Tingting Sartor, Maureen Ljungman, Mats Cheng, Shi-Yuan Appleman, Henry Lowenstein, Pedro Lahann, Joerg Lyssiotis, Costas Castro, Maria Department of Neurosurgery University of Michigan Medical School Ann Arbor USA Department of Cell and Developmental Biology University of Michigan Medical School Ann Arbor USA Departments of Chemical Engineering Material Science and Engineering Biomedical Engineering and Macromolecular Science and Engineering. University of Michigan Ann Arbor USA Rogel Cancer Center University of Michigan Ann Arbor USA Department of Molecular and Integrative Physiology University of Michigan Ann Arbor USA Department of Computational Medicine and Bioinformatics University of Michigan Ann Arbor USA Department of Radiation Oncology University of Michigan Ann Arbor USA Ken & Ruth Davee Department of Neurology Northwestern University Feinberg School of Medicine Chicago USA The Lou and Jean Malnati Brain Tumor Institute The Robert H. Lurie Comprehensive Cancer Center Northwestern University Feinberg School of Medicine Chicago USA Department of pathology University of Michigan Medical School Ann Arbor USA

Gliomas are primary brain tumors with a poor prognosis. IDH1R132Hexhibits a gain of function mutation leading to 2-hydroxyglutarate (2HG) production. We previously demonstrated, 2-HG mediated epigenetic rewiring is associated with better prognosis and its presence impacts several cellular functions including immune responses and enhanced DNA-damage response in IDH1R132Hgliomas harboring p53 and ATRX loss-of-function mutations. Also, IDH1R132Helicits metabolic reprogramming which implies that IDH1R132Hcould modify the energetic state of gliomas with consequences in tumor biology and therapeutic responses. In this study, RNA-seq and ChIP-seq data revealed human and mouse IDH1R132Hgliomas have downmodulated gene ontologies related to mitochondrial metabolism. This was paralleled by a decrease in glycolysis, rendering autophagy as a source of energy for IDH1R132Hglioma cells. We also found that IDH1R132H-neurospheres have decreased levels of oxygen consumption and extracellular acidification rates, characteristic of an autophagic/quiescent state when compared to IDH1WT-neurospheres. Analysis of the autophagy pathway revealed that both human and mouse IDH1R132Hgliomas have increased expression of pULK1-S555, pATG4b-S383, enhanced conversion of LC3I to LC3II, and decreased expression of pULK1-S757, p62 indicating that IDH1R132Hcells have augmented autophagy activity compared to IDH1WTcells. Blocking autophagy selectively impairs the growth of IDH1R132Hglioma cellsin vitro. Targeting autophagy by systemic administration of synthetic protein nanoparticles packaged with siRNA targeting Atg7 sensitized IDH1R132Hglioma cells to radiation-induced cell death, resulting in tumor regression, long-term survival, and immunological memory when used in combination with irradiation. Our results thus indicate that the metabolic changes in IDH1R132Hglioma cells lead to compromised mitochondrial functions and increased autophagic activity which contributes to their radioresistance, repres

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Thermal Contributions to the Local and Long-Range Structural Disorder in CH3NH3PbBr3

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PRX Energy 2023年第3期2卷 033004-033004页

作者： Nicholas J. Weadock Cameron MacKeen Xixi Qin Louis Waquier Yevgeny Rakita Julian A. Vigil Hemamala I. Karunadasa Volker Blum Michael F. Toney Frank Bridges Materials Science and Engineering University of Colorado Boulder Boulder Colorado 80309 USA Department of Chemical and Biological Engineering University of Colorado Boulder Boulder Colorado 80309 USA Physics Department University of California Santa Cruz California 95064 USA Thomas Lord Department of Mechanical Engineering and Materials Science Duke University Durham North Carolina 27708 USA Duke University Program in Materials Science and Engineering Duke University Durham North Carolina 27708 USA SSRL Materials Science Division SLAC National Accelerator Laboratory Menlo Park California 94025 USA Department of Materials Engineering Ben-Gurion University of the Negev Beer-Sheva 84105 Israel Department of Chemical Engineering Stanford University Stanford California 94305 USA Department of Chemistry Stanford University Stanford California 94305 USA Stanford Institute for Materials and Energy Sciences SLAC National Accelerator Laboratory Menlo Park California 94025 USA Department of Chemistry Duke University Durham North Carolina 27708 USA Renewable and Sustainable Energy Institute (RASEI) University of Colorado Boulder Boulder Colorado 80309 USA

The hybrid lead halide perovskite (LHP) family exhibits large structural fluctuations that contribute to the remarkable properties of LHP-based optoelectronic devices. In three-dimensional LHPs such as CH3NH3PbBr3, the structural phase transitions have been well characterized; changes in local structure and origins of structural disorder, however, have received less attention. We investigate the temperature dependence of the Pb—Br bond distribution, effective spring constant, and dynamic correlations with a combined extended x-ray-absorption fine structure (EXAFS), single-crystal x-ray diffraction (SXRD) and ab initio molecular dynamics (AIMD) study. EXAFS provides a snapshot of the local environment around the probe atom, rather than the time- and space-averaged structure obtained from SXRD. Molecular librations are observed below the orthorhombic-tetragonal transition temperature, and across this transition we find an anomalous increase in the Pb-Br effective spring constant. The x-ray absorption near edge structure reveals only subtle changes in the electronic structure; therefore, we propose that the increase in bond strength is the result of a redistribution of the charge density, concomitant with the loss of persistent Br…H bonding. Furthermore, the temperature dependence of the Pb—Br bond asymmetry indicates that the structural disorder in CH3NH3PbBr3 is primarily driven by thermally activated anharmonic dynamics rather than static disorder. Our results describe the local structure responsible for the optoelectronic performance of LHP devices and bring new insights into modifying halide bonding to prevent halide migration.

关键词： First-principles calculations Solar energy harvesting devices Disordered systems Hybrid perovskites X-ray absorption spectroscopy

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Two-dimensional ReS2: Solution to the unresolved queries on its structure and inter-layer coupling leading to potential optical applications

arXiv

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arXiv 2021年

作者： Gadde, Janardhan Rao Karmakar, Anasuya Maji, Tuhin Kumar Mukherjee, Subhrajit Alexander, Rajath Sharma, Anjanashree M.R. Das, Sarthak Mondal, Anirban Dasgupta, Kinshuk Naik, Akshay Majumdar, Kausik Hawaldar, Ranjit Adarsh, K.V. Ray, Samit Kumar Karmakar, Debjani Centre for Materials for Electronic Technology Pune411008 India Indian Institute of Science Education and Research Pune411008 India Department of Chemical Biological and Macromolecular Sciences S.N. Bose National Centre for Basic Sciences Kolkata Salt Lake700106 India Department of Physics Indian Institute of Technology Kharagpur Kharagpur721302 India Advanced Carbon Materials Section Materials Science Group Bhabha Atomic Research Centre Trombay Mumbai400085 India Centre for Nano Science and Engineering Indian Institute of Science Bangalore560012 India Department of Electrical Communication Engineering Indian Institute of Science Bangalore560012 India Department of Physics Indian Institute of Science Education and Research Bhopal462066 India Department of Condensed Matter Physics and Material Science S.N. Bose National Centre for Basic Sciences Kolkata Salt Lake700106 India Technical Physics Division Bhabha Atomic Research Centre Trombay Mumbai400085 India

Over the last few years, ReS2 has generated a myriad of unattended queries regarding its structure, the concomitant thickness dependent electronic properties and its apparently contrasting experimental optical response. In this work, with elaborate first-principles investigations, using density functional theory (DFT) and time-dependent DFT (TDDFT), we identify the structure of ReS2, which is capable of reproducing and analyzing the layer-dependent optical response. The theoretical results are further validated by an in-depth structural, chemical, optical and optoelectronic analysis of the large-area ReS2 thin films, grown by the chemical vapor deposition (CVD) process. Micro-Raman (MR), X-ray photoelectron spectroscopy (XPS), cross-sectional transmission electron microscopy (TEM) and energy-dispersive X-ray analysis (EDAX) have enabled the optimization of the uniform growth of the CVD films. The correlation between the optical and electronic properties was established by static photoluminescence (PL) and excited state transient absorption (TA) measurements. Sulfur vacancy-induced localized mid-gap states render a significantly long life-time of the excitons in these films. The ionic gel top-gated photo-detectors, fabricated from the as-prepared CVD films, exhibit a large photo-response of ~ 5 A/W and a remarkable detectivity of ~ 1011 Jones. The outcome of the present work will be useful in promoting the application of vertically grown large-area films in the field of optics and opto-electronics. © 2021, CC BY.

关键词： Density functional theory

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[email protected] as high-performance and durable electrocatalyst for oxygen reduction reaction in alkaline membrane fuel cells

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Journal of Alloys and Compounds 2023年 938卷

作者： Shaik Gouse Peera Chao Liu Arunchander Asokan Matthew E. Suss Department of Environmental Science Keimyung University 1095 Dalseo-gu Daegu 42601 Republic of Korea Faculty of Materials Metallurgy and Chemistry Jiangxi University of Science and Technology Ganzhou 341000 China Faculty of Mechanical Engineering Technion – Israel Institute of Technology Haifa 320003 Israel Grand Technion Energy Program Technion – Israel Institute of Technology Haifa 3200003 Israel Wolfson Department of Chemical Engineering Technion – Israel Institute of Technology Haifa 3200003 Israel

Discovery of electrocatalysts composed of cheap transition metals are urgent to replace the traditional Pt/C catalyst used for oxygen reduction reaction (ORR). Herein, we synthesized Cu nanoparticles encapsulated with nitrogen-doped carbon ( [email protected] ) as an excellent and durable catalyst for ORR. A systematic evaluation of the effect of Cu content, acid leaching and secondary heat treatment have been established with the help of half-cell studies. The morphological analysis revealed that Cu nanoparticles surrounded by thick nitrogen doped carbon layers and further, the acid leaching and subsequent pyrolysis, boosted the electrocatalytic performance. The optimized [email protected] catalyst showed onset potential (potential corresponding to a current density of 0.10 mA cm −2 ) and half-wave potential of 0.97 V vs. RHE and 0.85 V vs. RHE, surpassing the state-of-the-art Pt/C catalyst. In addition, the [email protected] catalyst exhibited outstanding durability, tolerance to carbon monoxide and methanol molecules. In the alkaline fuel cell, [email protected] catalyst delivered 118 mW cm −2 peak power density in alkaline fuel cell operated with H 2 -O 2 , whereas Pt/C only delivered a peak power density of 97 mW cm −2 under ambient operating conditions. High ORR activity and better stability of [email protected] catalyst could be a potential alternative to Pt/C catalyst in alkaline fuel cells and metal-air cell cathodes.

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Nemato-elasticity of hybrid molecular-colloidal liquid crystals

arXiv

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arXiv 2021年

作者： Senyuk, B. Mundoor, H. Smalyukh, I.I. Wensink, H.H. Department of Physics University of Colorado BoulderCO United States Department of Electrical Computer and Energy Engineering Materials Science and Engineering Program and Soft Materials Research Center University of Colorado BoulderCO United States Chemical Physics Program Departments of Chemistry and Physics University of Colorado BoulderCO United States Renewable and Sustainable Energy Institute National Renewable Energy Laboratory University of Colorado BoulderCO80309 United States Laboratoire de Physique des Solides Université Paris-Saclay CNRS UMR 8502 Orsay91405 France

Colloidal rods immersed in a thermotropic liquid-crystalline solvent are at the basis of so-called hybrid liquid crystals which are characterized by tunable nematic fluidity with symmetries ranging from conventional uniaxial nematic or anti-nematic to orthorhombic [Mundoor et al., science 360, 768 (2018)]. We provide a theoretical analysis of the elastic moduli of such systems by considering interactions between the individual rods with the embedding solvent through surface-anchoring forces, as well as steric and electrostatic interactions between the rods themselves. For uniaxial systems the presence of colloidal rods generates a marked increase of the splay elasticity which we found to be in quantitative agreement with experimental measurements. For orthorhombic hybrid liquid crystals we provide estimates of all twelve elastic moduli and show that only a small subset of those elastic constants play a relevant role in describing the nemato-elastic properties. The complexity and possibilities related to identifying the elastic moduli in experiments are briefly discussed. The results are expected to be helpful in stimulating future studies on defect-dressed "topological" colloids and the analysis of boundary-driven phenomena where the non-trivial director topology generated by biaxial nematics plays a key role. © 2021, CC BY-NC-SA.

关键词： Elasticity

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Photodynamic therapy-triggered on-demand drug release from ROS-responsive core-cross-linked micelles toward synergistic anti-cancer treatment

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Nano Research 2019年第5期12卷 999-1008页

作者： Yongjuan Li Jian Hu Xun Liu Yong Liu Shixian Lv Juanjuan Dang Yong Ji Jinlin He Lichen Yin Institute of Functional Nano and Soft Materials (FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhou 215123China College of Chemistry Chemical Engineering and Materials ScienceSuzhou Key Laboratory of Macromolecular Design and Precision SynthesisJiangsu Key Laboratory of Advanced Functional Polymer Design and ApplicationSoochow UniversitySuzhou 215123China Department of Biomedical Engineering University of Groningen and University Medical Center GroningenAntonius Deusinglaan 19713 AV Groningen The Netherlands Department of Cardiothoracic Surgery Wuxi Peoples Hospital Affiliated to Nanjing Medical UniversityWuxi 214023China

Polymeric micelles have demonstrated wide utility for chemodrug delivery,which however,still suffer from shortcomings such as undesired drug loading,disassembly upon dilution,pre-leakage of drug cargoes during systemic circulation,and lack of cancer-selective drug ***,a poly(ethylene glycol)(PEG)-polyphosphoester-based,reactive oxygen species (ROS)-responsive,core-cross-linked (CCL) micellar system was developed to encapsulate both chemodrug (doxorubicin,Dox) and photosensitizer (chlorin e6,Ce6).The hydrophobic core of the micelles was cross-linked via a thioketal (TK)-containing linker,which notably enhanced the drug loading and micelle *** tumor cells,far-red light irradiation of Ce6 generated ROS to cleave the TK linkers and disrupt the micelle *** such,micelles were destabilized and Dox release was promoted,which thereafter imparted synergistic anti-cancer effect with ROS-mediated photodynamic *** study provides an effective approach to realize the precise control over drug loading,formulation stability,and cancer-selective drug release using polymeric micelles,and would render promising utilities for the programmed anti-cancer combination therapy.

关键词： core-cross-linked micelles on-demand drug release photodynamic therapy reactive oxygen species (ROS) responsiveness synergistic an ti-cancer therapy

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