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Electronic and magnetic properties of perovskite selenite and tellurite compounds: CoSeO3, NiSeO3, CoTeO3, and NiTeO3

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Physical Review B 2020年第4期101卷 045107-045107页

作者： A. Rafi M. Iasir Todd Lombardi Qiangsheng Lu Amir M. Mofrad Mitchel Vaninger Xiaoqian Zhang David J. Singh Nuclear Engineering Program University of Missouri Columbia Missouri 65211 USA Department of Physics and Astronomy University of Missouri Columbia Missouri 65211-7010 USA Department of Biomedical Biological and Chemical Engineering University of Missouri Columbia Missouri 65211 USA Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials Collaborative Innovation Center of Advanced Microstructures School of Electronic Science and Engineering Nanjing University Nanjing 210093 China Department of Chemistry University of Missouri Columbia Missouri 65211 USA

Selenium and tellurium are among the few elements that form ABO3 perovskite structures with a four valent ion in the A site. This leads to highly distorted structures and unusual magnetic behavior. Here we investigate the Co and Ni selenite and tellurite compounds, CoSeO3, CoTeO3, NiSeO3, and NiTeO3, using first principles calculations. We find an interplay of crystal field and Jahn-Teller distortions that underpin the electronic and magnetic properties. While all compounds are predicted to show an insulating G-type antiferromagnetic ground state, there is a considerable difference in the anisotropy of the exchange interactions between the Ni and Co compounds. This is related to the Jahn-Teller distortion. Finally, we observe that these four compounds show characteristics generally associated with Mott insulators, even when described at the level of standard density functional theory. These are then dense bulk insulators that are correctly described as insulators in a standard band structure picture but that satisfy the common experimental criteria to classify them as Mott-type insulators.

关键词： Antiferromagnetism Band gap Exchange interaction Jahn-Teller effect

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Performance of the Large-Sized Telescope prototype of the Cherenkov Telescope Array 38

Performance of the Large-Sized Telescope prototype of the Ch...

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38th International Cosmic Ray Conference, ICRC 2023

作者： Morcuende, D. López-Coto, R. Moralejo, A. Nozaki, S. Vuillaume, T. Abe, K. Abe, S. Aguasca-Cabot, A. Agudo, I. Alvarez Crespo, N. Antonelli, L.A. Aramo, C. Arbet-Engels, A. Arcaro, C. Artero, M. Asano, K. Aubert, P. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Baxter, J. Becerra González, J. Bernardini, E. Bernardos, M.I. Bernete Medrano, J. Berti, A. Bhattacharjee, P. Biederbeck, N. Bigongiari, C. Bissaldi, E. Blanch, O. Bonnoli, G. Bordas, P. Bulgarelli, A. Burelli, I. Burmistrov, L. Buscemi, M. Cardillo, M. Caroff, S. Carosi, A. Carrasco, M.S. Cassol, F. Cauz, D. Cerasole, D. Ceribella, G. Chai, Y. Cheng, K. Chiavassa, A. Chikawa, M. Chytka, L. Cifuentes, A. Contreras, J.L. Cortina, J. Costantini, H. Dalchenko, M. Dazzi, F. De Angelis, A. de Bony de Lavergne, M. De Lotto, B. De Lucia, M. de Menezes, R. Del Peral, L. Deleglise, G. Delgado, C. Delgado Mengual, J. della Volpe, D. Dellaiera, M. Di Piano, A. Di Pierro, F. Di Pilato, A. Di Tria, R. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Eisenberger, L. Elsässer, D. Emery, G. Escudero, J. Fallah Ramazani, V. Ferrara, G. Ferrarotto, F. Fiasson, A. Foffano, L. Freixas Coromina, L. Fröse, S. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Gasbarra, C. Gasparrini, D. Geyer, D. Giesbrecht Paiva, J. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Grau, R. Green, J. Green, D. Gunji, S. Günther, P. Hackfeld, J. Hadasch, D. Hahn, A. Hashiyama, K. Hassan, T. Hayashi, K. Heckmann, L. Heller, M. Herrera Llorente, J. Hirotani, K. Hoffmann, D. Horns, D. Houles, J. Hrabovsky, M. Hrupec, D. Hui, D. Hütten, M. Iarlori, M. Imazawa, R. Inada, T. Inome, Y. Ioka, K. Iori, M. Ishio, K. Jimenez Martinez, I. Jurysek, J. Kagaya, M. Karas, V. Katagiri, H. Kataoka, J. Kerszberg, D. Kobayashi, Y. Kohri, K. Kong, A. Kubo, H. Kushida, J. Lainez, M. Lamanna, G. Lamastra, A. Le Flour, T. Linhoff, M. Longo, F. López-Oramas, A. IPARCOS-UCM Instituto de Física de Partículas y del Cosmos EMFTEL Department Universidad Complutense de Madrid MadridE-28040 Spain Instituto de Astrofísica de Andalucía-CSIC Glorieta de la Astronomía s/n Granada18008 Spain The Barcelona Institute of Science and Technology Campus UAB Bellaterra Barcelona08193 Spain Max-Planck-Institut für Physik Föhringer Ring 6 München80805 Germany Univ. Savoie Mont Blanc CNRS Laboratoire d’Annecy de Physique des Particules IN2P3 Annecy74000 France Department of Physics Tokai University Japan Institute for Cosmic Ray Research University of Tokyo Japan Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain EMFTEL department IPARCOS Universidad Complutense de Madrid Spain INAF Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy INFN Sezione di Padova Università degli Studi di Padova Italy Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan Universidad del Azuay Ecuador INAF Osservatorio di Astrofisica e Scienza dello spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain CIEMAT Spain Department of Physics TU Dortmund University Germany INFN Sezione di Bari Politecnico di Bari Italy INAF Osservatorio Astronomico di Brera Italy INFN Sezione di Trieste Università degli Studi di Udine Italy University of Geneva Département de physique nucléaire et corpusculaire Switzerland INFN Sezione di Catania Italy Italy Aix Marseille Univ CNRS IN2P3 CPPM France INFN Sezione di Bari Università di Bari Italy INFN Sezione di Torino Italy Palacky University Olomouc Faculty of Science Czech Republic University of Alcalá UAH Spain Port d’Informació Científica Spain University of Rijeka Department of Physics Croatia Institute for Theoretical Physics and Astrophysics Universität W

The next-generation ground-based gamma-ray Cherenkov Telescope Array Observatory (CTAO) will consist of imaging atmospheric Cherenkov telescopes (IACTs) of three different sizes distributed in two sites. The Large-Sized Telescopes will cover the low-energy end of the CTA energy range, starting at about 20 GeV. After its first years of operation at the CTA northern site, the Large-Sized Telescope prototype (LST-1) is in the final stage of its commissioning phase, having collected a significant amount of scientific data to date. In this contribution, we present the physics performance of the telescope using low-zenith Crab Nebula observations and Monte Carlo simulations fine-tuned accordingly. We show performance figures of merit such as the energy threshold, effective area, energy and angular resolution, and sensitivity based on the standard Hillas-parameters approach and following the source-independent and dependent analysis methods. The analysis threshold is estimated at 30 GeV. The energy resolution is around 30%, and the angular resolution is 0.3 degrees at 100 GeV. The best integral sensitivity of LST-1 is about 1.1% of the Crab Nebula flux above 250 GeV for 50 hours of observations. We also show the spectral energy distribution and light curve from Crab Nebula observations, which agree with results from other IACTs and link smoothly with Fermi-LAT when considering statistical and systematic uncertainties near the energy threshold. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Shellfish

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The effect of organic acid hydrolysis on the properties of nanocellulose from edamame husk (Glycine max (L.) merill)

Case Studies in Chemical and Environmental Engineering

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Case Studies in chemical and Environmental engineering 2025年 11卷

作者： Wahyudi, Muhammad Sapto Holilah Bahruji, Hasliza Prasetyoko, Didik Asranudin Pratama, Agus Wedi Indriani, Dina Wahyu Suryanegara, Lisman Faradilla, RH Fitri Mahardika, Melbi Wardani, Ratih Kusuma Piluharto, Bambang Knight, Victor Feizal Norrrahim, Mohd Nor Faiz Research Center for Biomass and Bioproducts National Research and Innovation Agency of Indonesia (BRIN) Cibinong Indonesia Research Collaboration Center for Nanocellulose BRIN-Andalas University Padang Indonesia Study Program of Chemistry Faculty of Science and Technology UIN Sunan Kalijaga Yogyakarta Indonesia Centre of Advanced Material and Energy Sciences Universiti Brunei Darussalam Jl. Tungku Link BE 1410 Brunei Darussalam Department of Chemistry Faculty of Science and Data Analytics Institut Teknologi Sepuluh Nopember Surabaya Indonesia Research Center for Applied Microbiology National Research and Innovation Agency (BRIN) Cibinong Indonesia Department of Biosystem Engineering Faculty of Agricultural Technology Universitas Brawijaya Jalan Veteran Malang Indonesia Department of Food Science and Technology Faculty of Agriculture Universitas Halu Oleo Kendari Indonesia Academy Pharmacy of Surabaya Ketintang Gayungan Surabaya 60231 Indonesia Department of Chemistry Faculty of Mathematics and Natural Sciences University of Jember Jember Indonesia Research Center for Chemical Defence Defence Research Institute Universiti Pertahanan Nasional Malaysia Kem Sungai Besi Kuala Lumpur 57000 Malaysia

The increasing demand for sustainable materials has highlighted nanocellulose as a promising candidate due to its exceptional mechanical strength, thermal stability, and superior barrier properties. These attributes enable its application in diverse fields, including packaging, biomedical devices, and nanocomposites. This study investigates the valorization of edamame bean husks, a byproduct of the globally consumed legume snack, as a sustainable feedstock for nanocellulose production. Cellulose was extracted from the husks via delignification and bleaching, followed by a green and facile acid hydrolysis method employing organic acids (maleic acid, lactic acid, citric acid, and formic acid) to produce nanocellulose. The resulting nanocellulose exhibited a fibrillar morphology with particle sizes ranging from 7.59 to 17.51 nm, depending on the acid used. X-ray diffraction analysis revealed a crystallinity index ranging from 63.49 % to 67.24 %. Notably, acid hydrolysis significantly enhanced the thermal stability of the nanocellulose compared to both the raw husk and isolated cellulose. These findings demonstrate the potential of edamame agricultural waste as a valuable resource for sustainable and eco-friendly nanocellulose production, contributing to a circular bioeconomy. © 2025 The Authors

关键词： Characterization Edamame husk waste Green synthesis Nanocellulose Organic acids

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Lotus root-like porous carbon nanofiber anchored with CoP nanoparticles as all-pH hydrogen evolution electrocatalysts

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Nano Research 2018年第3期11卷 1274-1284页

作者： Hengyi Lu Wei Fan Yunpeng Huang Tianxi Liu State Key Laboratory of Molecular Engineering of Polymers Department of Macromolecular Science Fudan University 220 HandanRoad Shanghai 200433 China State Key Laboratory for Modification of Chemical Fibers and Polymer Materials College of Materials Science and Engineering Donghua University 2999 North Renmin Road Shanghai 201620 China

The development of highly active and cost-effective hydrogen evolution reaction （HER） catalysts is of vital importance to addressing global energy issues. Here, a three-dimensional interconnected porous carbon nanofiber （PCNF） membrane has been developed and utilized as a support for active cobalt phosphide （COP） nanoparticles. This rationally designed self-supported HER catalyst has a lotus root-like multichannel structure, which provides several intrinsic advantages over conventional CNFs. The longitudinal channels can store the electrolyte and ensure fast ion and mass transport within the catalysts. Additionally, mesopores on the outer and inner carbon walls enhance ion and mass migration of the electrolyte to HER active CoP nanoparticles, thus shortening the ion transport distance and increasing the contact area between the electrolyte and the CoP nanoparticles. Moreover, the conductive carbon substrate provides fast electron transfer pathways by forming an integrated conductive network, which further ensures fast HER kinetics. As a result, the CoP/PCNF composites exhibit low onset-potentials （-20, -91, and -84 mV in 0.5 M H2SO4, 1 M PBS, and 1 M KOH, respectively）. These findings show that CoP/PCNF composites are promising self-supporting and high-performance all-pH range HER catalysts.

关键词： porous carbon nanofiber cobalt phosphide hydrogen evolutionreaction all-pH range

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Enabling Polymer Single Crystals to Be High-Performance Dielectric

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Angewandte Chemie 2023年第7期136卷

作者： Dr. Min Chen Prof. Wee-Liat Ong Prof. Boyu Peng Dr. Xuyun Guo Dr. Jie Ren Prof. Ye Zhu Prof. Hanying Li MOE Key Laboratory of Macromolecular Synthesis and Functionalization International Research Center for X Polymers Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Department of Polymer Science and Engineering Zhejiang University Hangzhou 310027 P. R. China ZJU-UIUC Institute College of Energy Engineering State Key Laboratory of Clean Energy Utilization Zhejiang University Hangzhou 310027 P. R. China Department of Applied Physics Research Institute for Smart Energy The Hong Kong Polytechnic University 0000 Hong Kong P. R. China

Semicrystalline polymer dielectrics (SPDs) are highly sought-after state-of-the-art dielectric materials. As the disorder in SPDs degrades their electrical properties, homogeneously ordered SPDs are desired. However, complex crystallization behaviors of polymers make such homogeneity elusive. Polymer lamellar single crystals (PLSCs), the most regularly-ordered form of SPDs possible under mild crystallizing conditions, are ideal platforms for understanding and developing high-performance dielectric materials. Here, a typical and widely used SPD, polyethylene (PE) is selected as the model material. We successfully obtained, large, uniform, and high-quality PE PLSCs and devised a non-destructive strategy to construct PE PLSC-based vertical capacitors. These nanometer-thick capacitors exhibit exceptional dielectric properties, with a high breakdown strength of 6.95 MV/cm and a low dielectric constant of 2.14±0.07, that outperform the properties of any existing neat PE. This work provides novel insights into exploring the performance possibility of ordered SPDs and reveals the PLSCs as potential high-performance dielectric materials.

关键词： Dielectrics Nano Capacitor Devices Polyethylene Polymer Single Crystals

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Green synthesis of iron oxide nanoparticles using Cymbopogon citratus extract and sodium carbonate salt: Nanotoxicological considerations for potential environmental applications

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Environmental Nanotechnology, Monitoring and Management 2020年 14卷

作者： Patiño-Ruiz, David Sánchez-Botero, Lina Tejeda-Benitez, Lesly Hinestroza, Juan Herrera, Adriana Engineering Doctorate Program Nanomaterials and Computer-Aided Process Engineering Research Group Universidad de Cartagena Cartagena 130010 Colombia Department of Fiber Science and Apparel Design Cornell University Ithaca United States Chemical Engineering Program Nanomaterials and Computer-Aided Process Engineering Research Group Universidad de Cartagena Cartagena 130010 Colombia

Synthesis of functional and biocompatible nanomaterials, based on the green chemistry paradigm, aims to innovate by using environmentally friendly techniques. Green synthesis using natural extracts instead of chemicals is proving to be an efficient route to prepare metal and metal oxide nanoparticles. In this study, the green synthesis of iron oxide nanoparticles (FeO-NPs) is reported, using a Cymbopogon citratus (C. citratus) extract and sodium carbonate as the reducing and pH stabilizer agents, respectively. FeO-NPs are extensively studied and applied due to the exceptional physicochemical properties, outstanding the superparamagnetism, and the large surface area. These properties are corroborated using different characterization techniques, in which a regular crystal structure and the magnetic response are similar compared with FeO-NPs synthesized via the traditional methods. The presence of magnetite and maghemite (Fe₃O₄ and γ-Fe₂O₃) phases are evidenced. A major composition of Fe₃O₄ allows predominant superparamagnetism. However, surface functionalization reduces the spin coordination avoiding a high saturation magnetization. The presence of phytochemical content in the C. citratus allows the reduction of iron(III) to iron(II) using H⁺ radicals produced from hydroxyl and carbonyl groups, and the in-situ functionalization using these groups. Additionally, the biocompatibility of the FeO-NPs is evaluated performing a nanotoxicological assessment, in which Caenorhabditis elegans nematodes are used as the biological model. The presence of organic molecules on FeO-NPs promotes no toxicity and low effects on the locomotion, growth, and reproduction, suggesting a low risk using these functional nanoparticles for environmental applications, and outstanding the synthesis route with a green approach. © 2020 Elsevier B.V.

关键词： Caenorhabditis elegans Cymbopogon citratus extract Ecotoxicological effects FeO nanoparticles Green synthesis Sodium carbonate

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Author Correction: Nuclear mechanosensing drives chromatin remodelling in persistently activated fibroblasts

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Nature biomedical engineering 2021年第12期5卷 1517-1518页

作者： Cierra J Walker Claudia Crocini Daniel Ramirez Anouk R Killaars Joseph C Grim Brian A Aguado Kyle Clark Mary A Allen Robin D Dowell Leslie A Leinwand Kristi S Anseth Materials Science and Engineering Program University of Colorado Boulder Boulder CO USA. BioFrontiers Institute University of Colorado Boulder Boulder CO USA. Department of Molecular Cellular and Developmental Biology University of Colorado Boulder Boulder CO USA. Department of Chemical and Biological Engineering University of Colorado Boulder Boulder CO USA. BioFrontiers Institute University of Colorado Boulder Boulder CO USA. leslie.leinwand@colorado.edu. Department of Molecular Cellular and Developmental Biology University of Colorado Boulder Boulder CO USA. leslie.leinwand@colorado.edu. BioFrontiers Institute University of Colorado Boulder Boulder CO USA. kristi.anseth@colorado.edu. Department of Chemical and Biological Engineering University of Colorado Boulder Boulder CO USA. kristi.anseth@colorado.edu.

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Cover Feature: LipophilicN-Hydroxyimide Derivatives: Design, Synthesis, and Application to Aerobic Alkane Oxidation Under Neat Conditions (ChemPlusChem 4/2023)

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ChemPlusChem 2023年第4期88卷

作者： Takaya Kaneiwa Kaito Yamada Dr. Ryo Nakano Prof. Makoto Yamashita Department of Molecular and Macromolecular Chemistry Graduate School of Engineering Nagoya University Tokai National Higher Education and Research System Furo-cho Chikusa-ku Nagoya 464-8603 Japan Integrated Research Consortium on Chemical Science (IRCCS) Nagoya University Tokai National Higher Education and Research System Furo-cho Chikusa-ku Nagoya 464-8602 Japan

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Do greenness and landscape indices for greenspace correlate with suicide ratio?

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Landscape and Urban Planning 2024年 242卷

作者： Lee, Hsiao-Yun Chang, Hao-Ting Herianto, Samuel Wu, Chi-Shin Liu, Wan-Yu Yu, Chia-Pin Pan, Wen-Chi Wu, Chih-Da Department of Leisure Industry and Health Promotion National Taipei University of Nursing and Health Sciences Taipei 112 Taiwan Department of Geomatics College of Engineering National Cheng Kung University Tainan 70101 Taiwan Chemical Biology and Molecular Biophysics Program Taiwan International Graduate Program (TIGP) Academia Sinica Taipei 11529 Taiwan Institute of Chemistry Academia Sinica Taipei 11529 Taiwan Department of Chemistry (Chemical Biology Division) College of Science National Taiwan University Taipei 10617 Taiwan National Center for Geriatrics and Welfare Research National Health Research Institutes Zhunan 350 Taiwan Department of Forestry National Chung Hsing University Taichung 402 Taiwan Innovation and Development Center of Sustainable Agriculture National Chung Hsing University Taichung 402 Taiwan School of Forestry and Resource Conservation National Taiwan University Taipei 10617 Taiwan Institute of Environmentaland Occupational Health Sciences National Yang Ming Chiao Tung University Taipei 11221 Taiwan National Institute of Environmental Health Sciences National Health Research Institutes Miaoli 35053 Taiwan Innovation and Development Center of Sustainable Agriculture National Chung Hsing University Taichung City 402 Taiwan

Previous studies have demonstrated the preventive effects of greenness and greenspace using three classes of exposure metrics (greenspace coverage, greenness, and landscape indices for greenspace) on suicide. Nevertheless, most studies were individually employed for each metric using a single-phase method, representing the short-term exposure. We hierarchically investigated the association between three classes of exposure metrics and suicide using long-term data from 2000 to 2018 in Taiwan. Normalized difference vegetation index (NDVI) was used to represent the greenness exposure, while mean patch area (area and edge), area-weighted mean fractal dimension index (shape), and proximity index (proximity) were opted to represent landscape indices for greenspace. Using the generalized additive mixed model, we revealed that the relative risk (95% confidence interval) of greenspace coverage, NDVI, mean patch area, area-weighted mean fractal dimension index, and proximity index was 0.998 (0.997, 0.999), 0.860 (0.811, 0.912), 0.999 (0.999, 0.999), 1.485 (1.056, 2.088), and 0.999 (0.999, 0.999), respectively. This indicates that long-term exposure to both greenspace coverage and greenness is associated with a reduced suicide ratio. Similarly, long-term exposure to greenspace that is greater in size, simpler in shape, and closer in proximity is associated with a decreased suicide risk. For formulating future afforestation policies, the layout and connectivity of greenspaces should be considered besides increasing green areas. This study not only demonstrated the significance of long-term exposure to greenspace for reducing the suicide ratio, but also illustrated a hierarchical approach to examine the effects of greenspace. © 2023

关键词： Greenness Greenspace coverage Landscape indices for greenspace Longitudinal ecological study Suicide

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A new capnellene skeleton from the octocoral Capnella imbricata (Quoy & Gaimard, 1833)

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Journal of Molecular Structure 2023年 1271卷

作者： Wu, I-Ting Fan, Yu-Chen Lin, Guan-Zhou Wang, Yi-Lin Hwang, Tsong-Long Lai, Kuei-Hung Chung, Hsu-Ming Department of Applied Chemistry National Pingtung University Pingtung900391 Taiwan Graduate Institute of Biomedical Sciences Graduate Institute of Natural Products College of Medicine Chang Gung University Taoyuan33305 Taiwan Research Center for Chinese Herbal Medicine Graduate Institute of Healthy Industry Technology College of Human Ecology Chang Gung University of Science and Technology Taoyuan33305 Taiwan Department of Chemical Engineering Ming Chi University of Technology New Taipei City243303 Taiwan Department of Anesthesiology Chang Gung Memorial Hospital Taoyuan333 Taiwan PhD Program in Clinical Drug Development of Herbal Medicine College of Pharmacy Taipei Medical University Taipei11031 Taiwan Graduate Institute of Pharmacognosy College of Pharmacy Taipei Medical University Taipei11031 Taiwan Traditional Herbal Medicine Research Center Taipei Medical University Hospital Taipei11031 Taiwan

chemical investigations on the ethyl acetate extract of the octocoral Capnella imbricata collected from the waters of Taiwan, which led to the isolation of three capnellenes (1–3), including one new metabolite, 9(12)-capnellene-8β,10α,15-triol (1), along with two known metabolites, 9(12)-capnellene-5α,8β,10α-triol (2), and 9(12)-capnellene-8β,10α-diol (3). The structures of the isolated metabolites were elucidated through extensive spectroscopic analyses, while the relative stereochemistry of 3 was confirmed by a single-crystal X-ray diffraction analysis for the first time in this study. Compounds 1–3 were evaluated in terms of their anti-inflammatory activity by examining their inhibitory effects on the generation of superoxide anions and the release of elastase by human neutrophils. © 2022 Elsevier B.V.

关键词： Metabolites

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