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Journal of Extracellular Biology 2022年第10期1卷 e63页

作者： Paolini, Lucia Monguió-Tortajada, Marta Costa, Marta Antenucci, Fabio Barilani, Mario Clos-Sansalvador, Marta Andrade, André Cronemberger Driedonks, Tom A. P. Giancaterino, Sara Kronstadt, Stephanie M. Mizenko, Rachel R. Nawaz, Muhammad Osteikoetxea, Xabier Pereira, Carla Shrivastava, Surya Boysen, Anders Toftegaard van de Wakker, Simonides Immanuel van Herwijnen, Martijn J. C. Wang, Xiaoqin Watson, Dionysios C. Gimona, Mario Kaparakis-Liaskos, Maria Konstantinov, Konstantin Lim, Sai Kiang Meisner-Kober, Nicole Stork, Michiel Nejsum, Peter Radeghieri, Annalisa Rohde, Eva Touzet, Nicolas Wauben, Marca H. M. Witwer, Kenneth W. Bongiovanni, Antonella Bergese, Paolo Department of Molecular and Translational Medicine University of Brescia Brescia Italy Center for Colloid and Surface Science (CSGI) Department of Chemistry University of Florence Sesto Fiorentino (FI) Italy Department of Medical and Surgical Specialties Radiological Sciences and Public Health University of Brescia Brescia Italy CREC Research Program Health Science Research Institute Germans Trias i Pujol (IGTP) Badalona Spain Heart Institute (iCor) Cardiology Department Germans Trias i Pujol University Hospital Badalona Spain iBET Instituto de Biologia Experimental e Tecnológica Oeiras Portugal Instituto de Tecnologia Química e Biológica António Xavier Universidade Nova de Lisboa Oeiras Portugal Department of Veterinary and Animal Sciences University of Copenhagen Copenhagen Denmark Laboratory of Regenerative Medicine ‒ Cell Factory Department of Transfusion Medicine and Hematology Fondazione IRCCS Ca' Granda Ospedale Maggiore Policlinico Milano Italy REMAR-IGTP Group Germans Trias i Pujol Research Institute (IGTP) & Nephrology Department University Hospital Germans Trias i Pujol (HUGTiP) Catalonia Badalona (Barcelona) Spain Department of Cell Biology Physiology and Immunology Universitat Autònoma de Barcelona (UAB) Bellaterra Spain Experimental and Clinical Cell Therapy Institute (ExCT) Spinal Cord Injury and Tissue Regeneration Center Paracelsus Medical University Salzburg Austria CDL Research University Medical Center Utrecht Utrecht University Utrecht Netherlands Department of Molecular and Comparative Pathology Johns Hopkins School of Medicine Baltimore MD United States Department of Civil Chemical Environmental and Materials Engineering Alma Mater Studiorum University of Bologna Bologna Italy Fischell Department of Bioengineering University of Maryland College Park MD United States Department of Biomedical Engineering University of California Davis CA United States Department of Rheumatology and Inflammation Research Institute of Medicine

Extracellular vesicles (EVs) large-scale production is a crucial point for the translation of EVs from discovery to application of EV-based products. In October 2021, the International Society for Extracellular Vesicles (ISEV), along with support by the FET-OPEN projects, “The Extracellular Vesicle Foundry” (evFOUNDRY) and “Extracellular vesicles from a natural source for tailor-made nanomaterials” (VES4US), organized a workshop entitled “massivEVs” to discuss the potential challenges for translation of EV-based products. This report gives an overview of the topics discussed during “massivEVs”, the most important points raised, and the points of consensus reached after discussion among academia and industry representatives. Overall, the review of the existing EV manufacturing, upscaling challenges and directions for their resolution highlighted in the workshop painted an optimistic future for the expanding EV field. © 2022 The Authors. Journal of Extracellular Biology published by Wiley Periodicals, LLC on behalf of the International Society for Extracellular Vesicles.

关键词： EV-based products extracellular vesicles ISEV workshop large-scale production manufacturing processing regulatory issues

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Detection of the 2021 Outburst of RS Ophiuchi with the LST-1

arXiv

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arXiv 2023年

作者： Kobayashi, Yukiho Aguasca-Cabot, Arnau Martín, María Isabel Bernardos Green, David López-Coto, Rubén Abe, K. Abe, S. Aguasca-Cabot, A. Agudo, I. Alvarez Crespo, N. Antonelli, L.A. Aramo, C. Arbet-Engels, A. Arcaro, C. Artero, M. Asano, K. Aubert, P. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Baxter, J. Becerra González, J. Bernardini, E. Bernardos, M.I. Bernete Medrano, J. Berti, A. Bhattacharjee, P. Biederbeck, N. Bigongiari, C. Bissaldi, E. Blanch, O. Bonnoli, G. Bordas, P. Bulgarelli, A. Burelli, I. Burmistrov, L. Buscemi, M. Cardillo, M. Caroff, S. Carosi, A. Carrasco, M.S. Cassol, F. Cauz, D. Cerasole, D. Ceribella, G. Chai, Y. Cheng, K. Chiavassa, A. Chikawa, M. Chytka, L. Cifuentes, A. Contreras, J.L. Cortina, J. Costantini, H. Dalchenko, M. Dazzi, F. De Angelis, A. de Bony de Lavergne, M. De Lotto, B. De Lucia, M. de Menezes, R. Del Peral, L. Deleglise, G. Delgado, C. Delgado Mengual, J. della Volpe, D. Dellaiera, M. Di Piano, A. Di Pierro, F. Di Pilato, A. Di Tria, R. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Eisenberger, L. Elsässer, D. Emery, G. Escudero, J. Fallah Ramazani, V. Ferrara, G. Ferrarotto, F. Fiasson, A. Foffano, L. Freixas Coromina, L. Fröse, S. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Gasbarra, C. Gasparrini, D. Geyer, D. Giesbrecht Paiva, J. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Grau, R. Green, J. Green, D. Gunji, S. Günther, P. Hackfeld, J. Hadasch, D. Hahn, A. Hashiyama, K. Hassan, T. Hayashi, K. Heckmann, L. Heller, M. Herrera Llorente, J. Hirotani, K. Hoffmann, D. Horns, D. Houles, J. Hrabovsky, M. Hrupec, D. Hui, D. Hütten, M. Iarlori, M. Imazawa, R. Inada, T. Inome, Y. Ioka, K. Iori, M. Ishio, K. Jimenez Martinez, I. Jurysek, J. Kagaya, M. Karas, V. Katagiri, H. Kataoka, J. Kerszberg, D. Kobayashi, Y. Kohri, K. Kong, A. Kubo, H. Kushida, J. Lainez, M. Lamanna, G. Lamastra, A. Le Flour, T. Linhoff, M. Institute for Cosmic Ray Research The University of Tokyo 5-1-5 Kashiwa-no-ha Chiba Kashiwa277-8582 Japan Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Martí i Franquès 1 Barcelona08028 Spain Instituto de Astrofísica de Andalucía-CSIC Glorieta de la Astronomía s/n Granada18008 Spain Max-Planck-Institut für Physik Föhringer Ring 6 München80805 Germany Department of Physics Tokai University Japan Institute for Cosmic Ray Research University of Tokyo Japan Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain Instituto de Astrofísica de Andalucía-CSIC Spain EMFTEL department IPARCOS Universidad Complutense de Madrid Spain INAF - Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy Max-Planck-Institut für Physik Germany INFN Sezione di Padova Università degli Studi di Padova Italy The Barcelona Institute of Science and Technology Spain LAPP Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS-IN2P3 Annecy France Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan Universidad del Azuay Ecuador INAF - Osservatorio di Astrofisica e Scienza dello Spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain CIEMAT Spain Department of Physics TU Dortmund University Germany INFN Sezione di Bari Politecnico di Bari Italy INAF - Osservatorio Astronomico di Brera Italy INFN Sezione di Trieste Università degli Studi di Udine Italy University of Geneva Département de Physique Nucléaire et Corpusculaire Switzerland INFN Sezione di Catania Italy Italy Aix Marseille Univ CNRS IN2P3 CPPM France INFN Sezione di Bari Università di Bari Italy INFN Sezione di Torino Italy Palacky University Olomouc Faculty of Science United States University of Alcalá UAH Spa

Novae are luminous explosions in close binaries which host a white dwarf and a companion donor star. They are triggered by a thermonuclear runaway when the white dwarf accretes a critical amount of matter from the secondary. Though novae are established as high-energy gamma-ray emitters through observations by the Fermi Large Area Telescope (LAT), the origin of the gamma-ray emission, whether it is hadronic or leptonic, had been under intense debate until very recently. RS Ophiuchi (RS Oph) is a well-known recurrent symbiotic nova with a recurrence time scale of 15 years. The most recent outburst of RS Oph in 2021 brought the first detection of very-high-energy (VHE) gamma rays from a nova ever. The first Large-Sized Telescope prototype (LST-1) of the Cherenkov Telescope Array observed this historic event along with H.E.S.S. and MAGIC. The LST-1 observations in the first days after the burst onset show a clear VHE gamma-ray signal from RS Oph. The low energy threshold of LST-1 allows us to reconstruct the RS Oph gamma-ray spectrum down to ∼30 GeV, providing the best connection of the VHE gamma-ray data to the Fermi LAT energy range. The results from the analysis of the LST-1 observations are consistent with those obtained with H.E.S.S. and MAGIC, and also support a hadronic origin for the observed gamma-ray fluxes. In this contribution, we will present the analysis results of the LST-1 observations of the 2021 outburst of RS Oph. © 2023, CC BY.

关键词： Telescopes

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The Mpemba effect in spin glasses is a persistent memory effect

arXiv

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arXiv 2018年

作者： Baity-Jesi, Marco Calore, Enrico Cruz, Andres Fernandez, Luis Antonio Gil-Narvión, José Miguel Gordillo-Guerrero, Antonio Iñiguez, David Lasanta, Antonio Maiorano, Andrea Marinari, Enzo Martin-Mayor, Victor Moreno-Gordo, Javier Sudupe, Antonio Muñoz Navarro, Denis Parisi, Giorgio Perez-Gaviro, Sergio Ricci-Tersenghi, Federico Ruiz-Lorenzo, Juan Jesus Schifano, Sebastiano Fabio Seoane, Beatriz Tarancón, Alfonso Tripiccione, Raffaele Yllanes, David Department of Chemistry Columbia University New YorkNY10027 United States Zaragoza50018 Spain Dipartimento di Fisica e Scienze della Terra Università di Ferrara e INFN Sezione di Ferrara FerraraI-44122 Italy Departamento de Física Teórica Universidad de Zaragoza Zaragoza50009 Spain Departamento de Física Teórica Universidad Complutense Madrid28040 Spain Departamento de Ingeniería Eléctrica Electrónica y Automática U. de Extremadura Cáceres10003 Spain Universidad de Extremadura Badajoz06006 Spain Fundación ARAID Diputación General de Aragón Zaragoza Spain Institute of Fluid Dynamics Nanoscience and Industrial Mathematics Department of Materials Science and Engineering and Chemical Engineering Universidad Carlos III de Madrid Leganés28911 Spain Dipartimento di Fisica Sapienza Università di Roma RomeI-00185 Italy Dipartimento di Fisica Sapienza Università di Roma INFN Sezione di Roma 1 CNR-Nanotec RomeI-00185 Italy Departamento de Ingeniería Electrónica y Comunicaciones and I3A U. de Zaragoza Zaragoza50018 Spain Centro Universitario de la Defensa Carretera de Huesca s/n Zaragoza50090 Spain Departamento de Física Universidad de Extremadura Badajoz06006 Spain Dipartimento di Matematica e Informatica Università di Ferrara e INFN Sezione di Ferrara FerraraI-44122 Italy Sorbonne Universités CNRS IBPS Laboratoire de Biologie Computationnelle et Quantitative - UMR 7238 qSorbonne Universités Institut des Sciences du Calcul et des Données 4 place Jussieu Paris75005 France Department of Physics and Soft and Living Matter Program Syracuse University SyracuseNY13244 Chan Zuckerberg Biohub San FranciscoCA94158 United States

The Mpemba effect occurs when a hot system cools faster than an initially colder one, when both are refrigerated in the same thermal reservoir. Using the custom built supercomputer Janus II, we study the Mpemba effect in spin glasses and show that it is a nonequilibrium process, governed by the coherence length ξ of the system. The effect occurs when the bath temperature lies in the glassy phase, but it is not necessary for the thermal protocol to cross the critical temperature. In fact, the Mpemba effect follows from a strong relationship between the internal energy and ξ that turns out to be a sure-tell sign of being in the glassy phase. Thus, the Mpemba effect presents itself as an intriguing new avenue for the experimental study of the coherence length in supercooled liquids and other glass formers. Copyright © 2018, The Authors. All rights reserved.

关键词： Supercooling

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11th German Conference on Chemoinformatics (GCC 2015) Abstracts

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JOURNAL OF CHEMINFORMATICS 2016年第SUPPL 1期8卷 1-27页

作者： [Anonymous] GDCh-CIC Division Associated Board Member Beilstein-Institut zur Förderung der Chemischen Wissenschaften Trakehner Str. 7-9 60487 Frankfurt Germany. ufechner@beilstein-institut.de. Division Medicinal Chemistry Amsterdam Institute for Molecules Medicines and Systems (AIMMS) VU University Amsterdam The Netherlands. Centre for Bioinformatics Uni Hamburg Bundesstr. 43 20146 Hamburg Germany. Sanofi-Aventis Deutschland GmbH 65926 Frankfurt am Main Germany. stefan.guessregen@***. Sanofi-Aventis Deutschland GmbH 65926 Frankfurt am Main Germany. GlaxoSmithKline Stevenage SG1 2NY UK. nicola.j.richmond@***. Discngine Paris 75011 France. Organisch-Chemisches Institut Westfälische Wilhelms-Universität Münster Germany. marwin.segler@wwu.de. Organisch-Chemisches Institut Westfälische Wilhelms-Universität Münster Germany. Bundeskriminalamt Wiesbaden Central Analytics II 65173 Wiesbaden Germany. Department of Chemistry and Biochemistry University of California Santa Barbara CA 93111 USA. shea@chem.ucsb.edu. Department of Chemistry and Biochemistry University of California Santa Barbara CA 93111 USA. Chemistry Department Ludwig-Maximilians-Universität München Butenandtstr. 7 81377 Munich Germany. Inorganic Chemistry and Center for Nanointegration University of Duisburg-Essen Essen Germany. CAM-D Technologies Essen Germany. Institute for Bioinformatics and Chemoinformatics Westphalian University of Applied Sciences Recklinghausen Germany. Institute for Bioinformatics and Chemoinformatics Westphalian University of Applied Sciences Recklinghausen Germany. achim.zielesny@w-hs.de. Leiden University Leiden Netherlands. j.fraaije@chem.leidenuniv.nl. Culgi BV Berlin Germany. Physikalische Chemie III TU Dortmund 44227 Dortmund Germany. stefan.kast@tu-dortmund.de. Centre for Molecular Informatics Department of Chemistry University of Cambridge Lensfield Road Cambridge CB2 1EW United Kingdom. kcb27@cam.ac.uk. Centre for Molecular Informatics Department of Chemistry

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EMERGING ROLES OF NIH AND EPA IN THE REGULATION OF RDNA TECHNOLOGY

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BIO-TECHNOLOGY 1983年第9期1卷 757-768页

作者： KORWEK, EL Edward L. Korwek Ph.D. J.D. is associated with the law offices of Keller and Heckman 1150 17th St. N.W. Washington D.C. 20036.REFERENCES Committee on Recombinant DNA "Potential Biohazards of Recombinant DNA Molecules" Nature250: 175 (1974) Proc. Nat. Acad. Sci.71: 2593 (1974) Science185: 303 (1974).|Article|Fed. Regist.48: 24556 (1983).Milewski E. Editor's Note. Recombinant DNA Tech. Bull.4: i (1981).Inside EPA 4 1 (1983). EPA has already held a meeting and published a draft report on the subject of its regulation of this area under the TSCA. EPA "Administrator's Toxic Substances Advisory Committee Meeting" Fed. Regist.48: 8342 (1983) Regulation of Genetically Engineered Substances Under TSCA Chemical Control Division Office of Toxic Substances Office of Pesticides and Toxic Substances Environmental Protection Agency Washington D.C. (March 1982). Congress also recently held a hearing on the subject of existing federal authority over the release of R-DNA-containing organisms into environment. M. Sun Science221: 136 (1983).Sects. 2-30 15 U.S. Code sects. 2601-2629 (1976 and Supp. V 1981). Hereinafter all references in the text to TSCA refer to the section numbers as enacted and not to the corresponding U.S. Code sections.The Administrative Procedure Act specifically states that the reviewing court shall "hold unlawful and set aside agency action findings and conclusions found to be hellip in excess of statutory jurisdiction authority or limitations or short of statutory right. hellip " 5 U.S. Code sect. 706(2)(C) (1976).PHS Act 42 U.S. Code sects. 217a and 241 (1976) Charter Recombinant DNA Advisory Committee Department of Health and Human Services (1982).Korwek E. Food Drug and Cosm. L. J.35: 633 (1980) p. 636.Although DHHS has some authority under Section 361 of the PHS Act to regulate R-DNA materials that cause human disease and are communicable most types of experimentation would not fall into this category. Because of this limitation the Sub committee of the Federal

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Cover Picture: Photoelectron Generation by Photosystem II Core Complexes Tethered to Gold Surfaces (ChemSusChem 4/2010)

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ChemSusChem 2010年第4期3卷 393-393页

作者： Michele Vittadello Prof. Maxim Y. Gorbunov Prof. Daniel T. Mastrogiovanni Leszek S. Wielunski Dr. Eric L. Garfunkel Prof. Fernando Guerrero Dr. Diana Kirilovsky Dr. Miwa Sugiura Prof. A. William Rutherford Dr. Ahmad Safari Prof. Paul G. Falkowski Prof. Department of Chemistry and Chemical Biology Rutgers The State University of New Jersey 610 Taylor Road Piscataway NJ 08854 (USA) Fax: (+1) 732-932-4083 PECS Department Medgar Evers College of the City University of New York 1650 Bedford Avenue Brooklyn NY 11225 (USA) Environmental Biophysics and Molecular Ecology Program Institute of Marine and Coastal Sciences Rutgers The State University of New Jersey 71 Dudley Road New Brunswick NJ 08901-8521 (USA) Department of Physics Rutgers The State University of New Jersey 619 Allison Road Piscataway NJ 08854 (USA) Unité de Recherche Associée 2096 Centre National de la Recherche Scientifique Service de Bioénergétique 91191 Gif-sur-Yvette (France) Cell-Free Science and Technology Research Center Ehime University Bunkyo-cho Matsuyama Ehime 790-8577 (Japan) Department of Materials Science and Engineering Rutgers The State University of New Jersey 607 Taylor Road Piscataway NJ 08854-8065 (USA)

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Abstracts from the 2011 Joint Annual Meeting of the Society for Northwestern Vertebrate Biology and Washington Chapter of the Wildlife Society, Held at the Wesley Inn, Gig Harbor, Washington, March 23–25, 2011

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Northwestern Naturalist 2011年第2期92卷 136-166页

作者： Michael J. Adams Christopher A. Pearl Jessica Y. Adkins Daniel D. Roby Ladd Bayliss Peter J. Loschl Donald E. Lyons Yasuko Suzuki Hannah E. Anderson Sarah T. Hamman Keith B. Aubry Catherine M. Raley John J. Rohrer Eric C. Lofroth Scott H. Fitkin Michael L. Best Hartwell H. Welsh Jamie B. Bettaso Don T. Ashton Hartwell H. Welsh Scott McBain Lindsay M. Biga Andrew R. Blaustein Susan F. Brady R. Steven Wagner Daniel J. Selski James E. Johnson R. Bruce Bury Wynn W. Cudmore Hartwell H. Welsh Nathan D. Chelgren Tara Chestnut Chaucney W. Anderson Julie Kirshtein Megan T. Cook Tiffany S. Garcia Stephen Corn Erin Muths Amanda Kissel Rick Scherer Eric Delvin Jonathan D. Bakker Peter W. Dunwiddie Diana L. Dishman Deborah A. Duffield Harriet R. Huber Dyanna M. Lambourn Karen M. Dvornich Greg Falxa Gary M. Fellers Patrick M. Kleeman David Miller Brandon Fessler Jason T. Irwin Daniel D. Beck R. Steven Wagner Marc P. Hayes John A. Frew Christian E. Grue Chris R. Friesen Robert T. Mason Stevan J. Arnold Suzanne Estes Tiffany S. Garcia Katie M. Dugger Josh Johnson Mike Rochelle A. J. Kroll Stephanie S. Gervasi Caren S. Goldberg Dan Davis Erica Bree Rosenblum Bill Bosworth Lisette P. Waits Purnima Govindarajulu Gregory A. Green Steve Negri Jennifer R. Griffiths Daniel E. Schindler Christian E. Grue Karen M. Dvornich Adam G. Hansen David A. Beauchamp Casey M. Baldwin Marc P. Hayes Gretchen Padgett-Flohr Blake R. Hossack Winsor H. Lowe Paul Stephen Corn Aaron N. Johnston Kris Kendell Dave Prescott Scott Stevens Peter M. Kiffney Carol Volk Kerensa A. King Christian E. Grue James M. Grassley Andrew J. Kroll Matt Hane Josh Johnston Mike Rochelle Stuart Farber Niels Leuthold Michael J. Adams John P. Hayes Bo Li Michael T. Brett Kent B. Livezey Ilon E. Logan Teresa J. Lorenz Kimberly A. Sullivan Amanda V. Bakian Deanna Lynch Nancy Thomas Krysten Schuler Steven Jeffries Joshua Malt Kelly R. McAllister Joanne P. Schuett-Hames Aimee P. McIntyre Jay E. Jones Eric M. Lund Frithiof T. Waterstrat Jack N. Giovanini Stephen D. Duke Marc P. Hayes US Forest Service Pacific Northwest Research Station Olympia WA 98512 kaubry@fs.fed.us US Forest Service Okanogan-Wenatchee National Forest Methow Valley Ranger District Winthrop WA 98862 British Columbia Ministry of Environment Victoria BC V8W9M1 Washington Department of Fish and Wildlife Winthrop WA 98862 Humboldt State University 1 Harpst St. Arcata CA 95521 addsmike14@*** US Forest Service Pacific Southwest Research Station 1700 Bayside Dr. Arcata CA 95521 hwelsh@fs.fed.us US Fish and Wildlife Service Arcata Field Office 1655 Heindon Road Arcata CA 95521 jamie_bettaso@fws.gov Redwood Sciences Laboratory US Forest Service1700 Bayview Drive Arcata CA 99521 dashton@fs.fed.us hwelsh@fs.fed.us McBain &amp Trush 980 7th Street Arcata CA 95521 scott@*** Oregon State University Environmental Sciences Graduate Program Corvallis OR 97331 lindsay.biga@science.oregonstate.edu Oregon State University Department of Zoology Corvallis OR 97331 US Geological Survey Forest and Rangeland Ecosystem Science Center 3200 SW Jefferson Way Corvallis OR 97331 buryb@usgs.gov Life Science Department Chemeketa Community College Salem OR 97309 wynn.cudmore@chemeketa.edu US Forest Service Redwood Sciences Laboratory 1700 Bayview Drive Arcata CA 95521 hwelsh@fs.fed.us USGS Oregon Water Science Center 2130 SW 5th Avenue Portland OR 97207 chestnut@usgs.gov USGS Headquarters 12201 Sunrise Valley Drive Reston VA 20192 US Geological Survey Northern Rocky Mountain Science Center Aldo Leopold Wilderness Research Institute 790 E. Beckwith Avenue Missoula MT 59801 scorn@usgs.gov US Geological Survey Fort Collins Science Center 2150 Centre Avenue Building C Fort Collins CO 80526 Department of Biological Sciences Simon Fraser University Burnaby BC V5A 1S6 Colorado State University Department of Fishery and Wildlife Biology Fort Collins CO 80523 The Nature Conservancy 120 Union Ave SE Olympia WA 98501 edelvin@tnc.org School of Forest Resources University of Washington Seattle WA

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Double-Cable Conjugated Polymers with Pendent Near-Infrared Electron Acceptors for Single-Component Organic Solar Cells

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Angewandte Chemie 2022年第35期134卷

作者： Shijie Liang Baiqiao Liu Dr. Safakath Karuthedath Jing Wang Dr. Yakun He Wen Liang Tan Hao Li Prof. Yunhua Xu Prof. Ning Li Prof. Jianhui Hou Prof. Zheng Tang Prof. Frédéric Laquai Prof. Christopher R. McNeill Prof. Christoph J. Brabec Prof. Weiwei Li Beijing Advanced Innovation Center for Soft Matter Science and Engineering & State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical Technology Beijing 100029 China Contribution: Data curation (lead) Formal analysis (lead) Investigation (equal) Writing - original draft (supporting) Writing - review & editing (supporting) Department of Chemistry School of Science Beijing Jiaotong University Beijing 100044 P. R. China KAUST Solar Center (KSC) Physical Sciences and Engineering Division (PSE) Material Science and Engineering Program (MSE) King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Kingdom of Saudi Arabia Contribution: Data curation (supporting) Formal analysis (supporting) Investigation (supporting) Writing - original draft (supporting) Writing - review & editing (supporting) Center for Advanced Low-dimension Materials College of Materials Science and Engineering Donghua University Shanghai 201620 P. R. China Contribution: Data curation (supporting) Formal analysis (supporting) Investigation (supporting) Methodology (supporting) Writing - review & editing (supporting) Institute of Materials for Electronics and Energy Technology (i-MEET) Friedrich-Alexander-Universität Erlangen-Nürnberg Martensstrasse 7 91058 Erlangen Germany Contribution: Data curation (supporting) Formal analysis (supporting) Investigation (supporting) Methodology (supporting) Writing - original draft (supporting) Writing - review & editing (supporting) Department of Materials Science and Engineering Monash University Wellington Road Clayton Victoria 3800 Australia State Key Laboratory of Polymer Physics and Chemistry Beijing National Laboratory for Molecular Sciences Institute of Chemistry Chinese Academy of Sciences Beijing 100190 P. R. China Contribution: Data curation (supporting) Formal analysis (supporting) Writing - review & editing (supporting) Contribution: Funding acquisition (supporting) Writing - review & editing (supportin

Double-cable conjugated polymers with near-infrared (NIR) electron acceptors are synthesized for use in single-component organic solar cells (SCOSCs). Through the development of a judicious synthetic pathway, the highly sensitive nature of the 2-(3-oxo-2,3-dihydroinden-1-ylidene)malononitrile (IC)-based electron acceptors in basic and protonic solvents is overcome. In addition, an asymmetric design motif is adopted to optimize the packing of donor and acceptor segments, enhancing charge separation efficiency. As such, the new double-cable polymers are successfully applied in SCOSCs, providing an efficiency of over 10 % with a broad photo response from 300 to 850 nm and exhibiting excellent thermal/light stability. These results demonstrate the powerful design of NIR-acceptor-based double-cable polymers and will enable SCOSCs to enter a new stage.

关键词： Double-Cable Conjugated Polymers Electron Acceptors Near Infrared Single Component Solar Cells

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NWChem: Past, present, and future

arXiv

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arXiv 2020年

作者： Aprà, E. Bylaska, E.J. de Jong, W.A. Govind, N. Kowalski, K. Straatsma, T.P. Valiev, M. van Dam, H.J.J. Alexeev, Y. Anchell, J. Anisimov, V. Aquino, F.W. Atta-Fynn, R. Autschbach, J. Bauman, N.P. Becca, J.C. Bernholdt, D.E. Bhaskaran-Nair, K. Bogatko, S. Borowski, P. Boschen, J. Brabec, J. Bruner, A. Cauët, E. Chen, Y. Chuev, G.N. Cramer, C.J. Daily, J. Deegan, M.J.O. Dunning, T.H. Dupuis, M. Dyall, K.G. Fann, G.I. Fischer, S.A. Fonari, A. Früchtl, H. Gagliardi, L. Garza, J. Gawande, N. Ghosh, S. Glaesemann, K. Götz, A.W. Hammond, J. Helms, V. Hermes, E.D. Hirao, K. Hirata, S. Jacquelin, M. Jensen, L. Johnson, B.G. Jónsson, H. Kendall, R.A. Klemm, M. Kobayashi, R. Konkov, V. Krishnamoorthy, S. Krishnan, M. Lin, Z. Lins, R.D. Littlefield, R.J. Logsdail, A.J. Lopata, K. Ma, W. Marenich, A.V. Martin del Campo, J. Mejia-Rodriguez, D. Moore, J.E. Mullin, J.M. Nakajima, T. Nascimento, D.R. Nichols, J.A. Nichols, P.J. Nieplocha, J. Otero-de-la-Roza, A. Palmer, B. Panyala, A. Pirojsirikul, T. Peng, B. Peverati, R. Pittner, J. Pollack, L. Richard, R.M. Sadayappan, P. Schatz, G.C. Shelton, W.A. Silverstein, D.W. Smith, D.M.A. Soares, T.A. Song, D. Swart, M. Taylor, H.L. Thomas, G.S. Tipparaju, V. Truhlar, D.G. Tsemekhman, K. van Voorhis, T. Vázquez-Mayagoitia, Á. Verma, P. Villa, O. Vishnu, A. Vogiatzis, K.D. Wang, D. Weare, J.H. Williamson, M.J. Windus, T.L. Woliński, K. Wong, A.T. Wu, Q. Yang, C. Yu, Q. Zacharias, M. Zhang, Z. Zhao, Y. Harrison, R.J. Pacific Northwest National Laboratory RichlandWA99352 United States Lawrence Berkeley National Laboratory BerkeleyCA94720 United States National Center for Computational Sciences Oak Ridge National Laboratory Oak RidgeTN37831 United States Brookhaven National Laboratory UptonNY11973 United States Argonne Leadership Computing Facility Argonne National Laboratory ArgonneIL60439 United States Intel Corporation Santa ClaraCA95054 United States QSimulate CambridgeMA02139 United States Department of Physics University of Texas at Arlington ArlingtonTX76019 United States Department of Chemistry University at Buffalo State University of New York BuffaloNY14260 United States Department of Chemistry Pennsylvania State University University ParkPA16802 United States Oak Ridge National Laboratory Oak RidgeTN37831 United States Washington University St. LouisMO63130 United States 4G Clinical WellesleyMA02481 United States Faculty of Chemistry Maria Curie-Sklodowska University in Lublin Lublin20-031 Poland Department of Chemistry Iowa State University AmesIA50011 United States J. Heyrovský Institute of Physical Chemistry Academy of Sciences of the Czech Republic Prague 818223 Czech Republic Department of Chemistry and Physics University of Tennessee at Martin MartinTN38238 United States Université libre de Bruxelles BrusselsB-1050 Belgium Facebook Menlo ParkCA94025 United States Institute of Theoretical and Experimental Biophysics Russian Academy of Science Pushchino Moscow142290 Russia Department of Chemistry Chemical Theory Center Supercomputing Institute University of Minnesota MinneapolisMN55455 United States SKAO Jodrell Bank Observatory MacclesfieldSK11 9DL United Kingdom Department of Chemistry University of Washington SeattleWA98195 United States Dirac Solutions PortlandOR97229 United States Chemistry Division U. S. Naval Research Laboratory WashingtonDC20375 United States School of Chemistry and Biochemis

Specialized computational chemistry packages have permanently reshaped the landscape of chemical and materials science by providing tools to support and guide experimental efforts and for the prediction of atomistic and electronic properties. In this regard, electronic structure packages have played a special role by using first-principle-driven methodologies to model complex chemical and materials processes. Over the last few decades, the rapid development of computing technologies and the tremendous increase in computational power have offered a unique chance to study complex transformations using sophisticated and predictive many-body techniques that describe correlated behavior of electrons in molecular and condensed phase systems at different levels of theory. In enabling these simulations, novel parallel algorithms have been able to take advantage of computational resources to address the polynomial scaling of electronic structure methods. In this paper, we briefly review the NWChem computational chemistry suite, including its history, design principles, parallel tools, current capabilities, outreach and outlook. Copyright © 2020, The Authors. All rights reserved.

关键词： Computational chemistry

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Publisher Correction: On the issue of transparency and reproducibility in nanomedicine

引用

Nature nanotechnology 2019年第8期14卷 811页

作者： Hon S Leong Kimberly S Butler C Jeffrey Brinker May Azzawi Steve Conlan Christine Dufès Andrew Owen Steve Rannard Chris Scott Chunying Chen Marina A Dobrovolskaia Serguei V Kozlov Adriele Prina-Mello Ruth Schmid Peter Wick Fanny Caputo Patrick Boisseau Rachael M Crist Scott E McNeil Bengt Fadeel Lang Tran Steffen Foss Hansen Nanna B Hartmann Lauge P W Clausen Lars M Skjolding Anders Baun Marlene Ågerstrand Zhen Gu Dimitrios A Lamprou Clare Hoskins Leaf Huang Wantong Song Huiliang Cao Xuanyong Liu Klaus D Jandt Wen Jiang Betty Y S Kim Korin E Wheeler Andrew J Chetwynd Iseult Lynch Sayed Moein Moghimi André Nel Tian Xia Paul S Weiss Bruno Sarmento José das Neves Hélder A Santos Luis Santos Samir Mitragotri Steve Little Dan Peer Mansoor M Amiji Maria José Alonso Alke Petri-Fink Sandor Balog Aaron Lee Barbara Drasler Barbara Rothen-Rutishauser Stefan Wilhelm Handan Acar Roger G Harrison Chuanbin Mao Priyabrata Mukherjee Rajagopal Ramesh Lacey R McNally Sara Busatto Joy Wolfram Paolo Bergese Mauro Ferrari Ronnie H Fang Liangfang Zhang Jie Zheng Chuanqi Peng Bujie Du Mengxiao Yu Danielle M Charron Gang Zheng Chiara Pastore Department of Urology Mayo Clinic Rochester MN USA. Department of Physiology and Biomedical Engineering Mayo Clinic Rochester MN USA. Department of Nanobiology Sandia National Laboratories Albuquerque NM USA. Center for Micro-Engineered Materials University of New Mexico Albuquerque Albuquerque NM USA. Departments of Chemical and Biological Engineering University of New Mexico Albuquerque NM USA. Department of Molecular Genetics and Microbiology University of New Mexico Albuquerque NM USA. UNM Comprehensive Cancer Center University of New Mexico Albuquerque NM USA. Cardiovascular Research Group School of Healthcare Science Manchester Metropolitan University Manchester UK. British Society for Nanomedicine Liverpool UK. Institute of Life Science Swansea University Medical School Swansea University Swansea UK. Strathclyde Institute of Pharmacy and Biomedical Sciences University of Strathclyde Glasgow UK. Department of Molecular and Clinical Pharmacology Institute of Translational Medicine University of Liverpool Liverpool UK. Department of Chemistry School of Physical Sciences University of Liverpool Liverpool UK. Centre for Cancer Research and Cell Biology Queen's University of Belfast Belfast UK. National Center for Nanoscience and Technology of China Beijing China. Cancer Research Technology Program Nanotechnology Characterization Laboratory Frederick National Laboratory for Cancer Research Frederick MD USA. Laboratory of Animal Sciences Program Center for Advanced Preclinical Research Frederick National Laboratory for Cancer Research Frederick National Laboratory for Cancer Research Frederick MD USA. Trinity Translational Medicine Institute Department of Clinical Medicine Trinity College Dublin Dublin Ireland. Laboratory for Biological Characterisation of Advanced Materials Trinity Translational Medicine Institute Trinity College Dublin Dublin Ireland. Nanomedicine Group Advanced Materials and Bioengineering Research (AMBER) centre Centre

An amendment to this paper has been published and can be accessed via a link at the top of the paper.

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