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Frontispiz: ABis-(carbone) Pincer Ligand and Its Coordinative Behavior toward Multi-Metallic Configurations

Angewandte Chemie 2022年第24期134卷

作者： Bamlaku Semagne Aweke Dr. Cheng-Han Yu Minna Zhi Dr. Wen-Ching Chen Glenn P. A. Yap Prof. Lili Zhao Prof. Tiow-Gan Ong Institute of Chemistry Academia Sinica Taipei Taiwan ROC Department of Applied Chemistry National Yang Ming Chiao Tung University Hsinchu Taiwan ROC Sustainable Chemical Science and Technology (SCST) Taiwan International Graduate Program (TIGP) Academia Sinica Taipei Taiwan ROC Institute of Advanced Synthesis School of Chemistry and Molecular Engineering Nanjing Tech University Nanjing China Department of Chemistry and Biochemistry University of Delaware Newark DE USA Department of Chemistry National Taiwan University Taipei Taiwan ROC Department of Medicinal and Applied Chemistry Kaohsiung Medical University Kaohsiung Taiwan ROC

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Inside Cover: Diels–Alder Conversion of Acrylic Acid and 2,5-Dimethylfuran topara-Xylene Over Heterogeneous Bi-BTC Metal-Organic Framework Catalysts Under Mild Conditions (Angew. Chem. Int. Ed. 2/2021)

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Angewandte Chemie International Edition 2020年第2期60卷

作者： Jyun-Yi Yeh Season S. Chen Shih-Cheng Li Celine H. Chen Dr. Tetsuya Shishido Dr. Daniel C. W. Tsang Dr. Yusuke Yamauchi Yi-Pei Li Prof. Kevin C.-W. Wu International Graduate Program of Molecular Science and Technology (NTU-MST) National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Taiwan International Graduate Program (TIGP) Academia Sinica No. 128 Sec. 2 Academia Road Taipei 11529 Taiwan Department of Chemical Engineering National (Taiwan) University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan School of Engineering Brown University Providence RI 02912 USA Department of Applied Chemistry for Environment Tokyo Metropolitan University 1-1 Minami-osawa Hachioji Tokyo 192-0397 Japan Department of Civil and Environmental Engineering The Hong Kong Polytechnic University Hung Hom Kowloon Hong Kong China JST-ERATO Yamauchi Materials Space-Tectonics Project Kagami Memorial Research Institute for Materials Science and Technology Waseda University 2-8-26 Nishiwaseda Shinjuku-ku Tokyo 169-0051 Japan Australian Institute for Bioengineering and Nanotechnology (AIBN) School of Chemical Engieering The University of Queensland Brisbane QLD 4072 Australia Center of Atomic Initiative for New Materials National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan

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Front Cover: From Textile Coloring to Light-emitting Electrochemical Devices: Upcycling of the Isoviolanthrone Vat Dye (Chem. Asian J. 6/2023)

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Chemistry – An Asian Journal 2023年第6期18卷

作者： Tatiana Ghanem Kwang Keat Leong Hwandong Jang Alexis Hardouin Dr. Philippe Blanchard Prof. Dominik Lungerich Dr. Pierre Josse Prof. Eunkyoung Kim Dr. Clément Cabanetos University of Angers CNRS MOLTECH-ANJOU SFR MATRIX F-49000 Angers France Department of Chemical and Biomolecular Engineering Yonsei University 50 Yonsei-ro Seodaemun-gu 03722 Seoul South Korea Center for Nanomedicine (CNM) Institute for Basic Science (IBS) IBS Hall 50 Yonsei-ro Seodaemun-gu 03722 Seoul South Korea Graduate Program of Nano Biomedical Engineering (NanoBME) Advanced Science Institute Yonsei University 50 Yonsei-ro Seodaemun-gu 03722 Seoul South Korea Building Blocks for FUture Electronics Laboratory (2BFUEL) IRL2002 CNRS-Yonsei University Seodaemun-gu 03722 Seoul South Korea

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ABis-(carbone) Pincer Ligand and Its Coordinative Behavior toward Multi-Metallic Configurations

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Angewandte Chemie 2022年第24期134卷

Carbones are divalent carbon(0) species that contain two lone pairs of electrons. Herein, we have prepared the first known stable and isolable free bis -(carbone) pincer framework with a well-defined solid-state structure. This bis -(carbone) ligand is an effective scaffold for forming monometallic (Ni and Pd) and trinuclear heterometallic complexes with Au−Pd−Au, Au−Ni−Au, and Cu−Ni−Cu configurations. Sophisticated quantum-theoretical analyses found that the metal–metal interactions are too weak to play a significant role in upholding these multi-metallic configurations; rather, the four lone pairs of electrons within the bis -(carbone) framework are the main contributors to the stability of the complexes.

关键词： Bis-(Carbone) Heterometallic Coordination Metal–Metal Interactions Pincer Ligands

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Diels–Alder Conversion of Acrylic Acid and 2,5-Dimethylfuran topara-Xylene Over Heterogeneous Bi-BTC Metal-Organic Framework Catalysts Under Mild Conditions

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Angewandte Chemie 2020年第2期133卷

The heterogeneous metal-organic framework Bi-BTC successfully catalyzed the synthesis of para -xylene from bio-based 2,5-dimethylfuran and acrylic acid in a promising yield (92 %), under relatively mild conditions (160 °C, 10 bar), and with a low reaction-energy barrier (47.3 kJ mol −1 ). The proposed reaction strategy also demonstrates a remarkable versatility for furan derivatives such as furan and 2-methylfuran.

关键词： 2,5-dimethylfuran acrylic acid Bi-BTC metal-organic frameworks para-xylene

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Self‐Assembly of Wireframe DNA Nanostructures from Junction Motifs

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Angewandte Chemie 2019年第35期131卷

作者： Kai Huang Donglei Yang Zhenyu Tan Silian Chen Ye Xiang Yongli Mi Chengde Mao Bryan Wei School of Life Sciences Tsinghua University-Peking University Center for Life Sciences Center for Synthetic and Systems Biology Tsinghua University Beijing 100084 China School of Chemical Science and Engineering Tongji University Shanghai 200092 China Institute of Molecular Medicine (IMM) Renji Hospital Shanghai Jiao Tong University School of Medicine Shanghai 200127 China Present address: Biophysics Program University of Michigan Ann Arbor MI 48109 USA Center for Infectious Disease Research Collaborative Innovation Center for Diagnosis and Treatment of Infectious Diseases Beijing Advanced Innvation Center for Structural Biology Department of Basic Medical Sciences School of Medicine Tsinghua University Beijing 100084 China School of Life Sciences Peking University Beijing 100084 China Department of Chemical and Biological Engineering Hong Kong University of Science and Technology Kowloon Hong Kong SAR China Department of Chemistry Purdue University West Lafayette IN 47907 USA

Wireframe frameworks have been investigated for the construction of complex nanostructures from a scaffolded DNA origami approach; however, a similar framework is yet to be fully explored in a scaffold‐free “LEGO” approach. Herein, we describe a general design scheme to construct wireframe DNA nanostructures entirely from short synthetic strands. A typical edge of the resulting structures in this study is composed of two parallel duplexes with crossovers on both ends, and three, four, or five edges radiate out from a certain vertex. By using such a self‐assembly scheme, we produced planar lattices and polyhedral objects.

关键词： DNA-Nanostrukturen Drahtgitterstrukturen Selbstorganisation Verzweigungsmotive

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Observation of a μs isomer in In8549134: Proton-neutron coupling “southeast” of Sn8250132

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Physical Review C 2019年第1期100卷 011302(R)-011302(R)页

作者： V. H. Phong G. Lorusso T. Davinson A. Estrade O. Hall J. Liu K. Matsui F. Montes S. Nishimura A. Boso P. H. Regan R. Shearman Z. Y. Xu J. Agramunt J. M. Allmond D. S. Ahn A. Algora H. Baba N. T. Brewer C. G. Bruno R. Caballero-Folch F. Calvino M. Wolińska-Cichocka G. Cortes I. Dillmann C. Domingo-Pardo A. Gargano S. Go C. J. Griffin R. K. Grzywacz L. Harkness-Brennan T. Isobe A. Jungclaus D. Kahl L. H. Khiem G. Kiss A. Korgul S. Kubono K. Miernik A. I. Morales N. Nepal M. Piersa Zs. Podolyák B. C. Rasco K. P. Rykaczewski H. Sakurai Y. Shimizu D. W. Stacener T. Sumikama H. Suzuki H. Takeda J. L. Tain A. Tarifeño-Saldivia A. Tolosa-Delgado V. Vaquero P. J. Woods R. Yokoyama C. Yuan RIKEN Nishina Center RIKEN 2-1 Hirosawa Wako-shi Saitama 351-0198 Japan Faculty of Physics VNU University of Science 334 Nguyen Trai Thanh Xuan 120062 Hanoi Vietnam Chemical Medical and Enviromental Science Division National Physical Laboratory Teddington TW110LW United Kingdom Department of Physics University of Surrey Guildford GU2 7XH United Kingdom School of Physics and Astronomy University of Edinburgh EH9 3FD Edinburgh United Kingdom Department of Physics and Science of Advanced Materials Program Central Michigan University Mount Pleasant Michigan 48859 USA Department of Physics the University of Hong Kong Pokfulam Road Hong Kong Department of Physics University of Tokyo Hongo 7-3-1 Bunkyo-ku 113-0033 Tokyo Japan National Superconducting Cyclotron Laboratory East Lansing Michigan 48824 USA Department of Physics University of Surrey Guildford GU27XH United Kingdom Department of Physics and Astronomy University of Tennessee Knoxville Tennessee 37996 USA Instituto de Física Corpuscular (CSIC-Universitat de Valencia) Apartado Correos 22085 E-46071 Valencia Spain Physics Division Oak Ridge National Laboratory Oak Ridge Tennessee 37831 USA Institute of Nuclear Research MTA ATOMKI Debrecen 4026 Hungary Physics Division Oak Ridge National Laboratory Oak Ridge Tennessee 37830 USA TRIUMF Vancouver British Columbia Canada V6T 2A3 INTE-ETSEIB Universitat Politécnica de Catalunya (UPC) E-08028 Barcelona Spain Heavy Ion Laboratory University of Warsaw PL-02-093 Warsaw Poland Department of Physics and Astronomy University of Victoria Victoria Canada BC V8P 5C2 Istituto Nazionale di Fisica Nucleare Complesso Universitario di Monte S. Angelo I-80126 Napoli Italy Department of Physics University of Liverpool Liverpool L69 7ZE United Kingdom Instituto de Estructura de la Materia CSIC E-28006 Madrid Spain Institute of Physics Vietnam Academy of Science and Technology 10 Dao Tan Ba Dinh 118011 Hanoi Vietnam Graduate University of Science and Techno

We report on the observation of a microsecond isomeric state in the single-proton-hole, three-neutron-particle nucleus In134. The nuclei of interest were produced by in-flight fission of a U238 beam at the Radioactive Isotope Beam Factory at RIKEN. The isomer depopulates through a γ ray of energy 56.7(1) keV and with a half-life of T1/2=3.5(4)μs. Based on the comparison with shell-model calculations, we interpret the isomer as the Iπ=5− member of the π0g9/2−1⊗ν1f7/23 multiplet, decaying to the Iπ=7− ground state with a reduced-transition probability of B(E2;5−→7−)=0.53(6)W.u. Observation of this isomer, and lack of evidence in the current work for a Iπ=5− isomer decay in In132, provides a benchmark of the proton-neutron interaction in the region of the nuclear chart “southeast” of Sn132, where experimental information on excited states is sparse.

关键词： Isomer decays Lifetimes & widths Nuclear structure & decays Rare & new isotopes Shell model 90 ≤ A ≤ 149

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Author Correction: 3D-printed liquid metal polymer composites as NIR-responsive 4D printing soft robot

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Nature communications 2024年第1期15卷 943页

作者： Liwen Zhang Xumin Huang Tim Cole Hongda Lu Jiangyu Hang Weihua Li Shi-Yang Tang Cyrille Boyer Thomas P Davis Ruirui Qiao Australian Institute of Bioengineering & Nanotechnology The University of Queensland Brisbane QLD 4072 Australia. Department of Electronic Electrical and Systems Engineering University of Birmingham Birmingham UK. School of Mechanical Materials Mechatronic and Biomedical Engineering University of Wollongong Wollongong NSW 2522 Australia. School of Electronics and Computer Science University of Southampton Southampton SO17 1BJ UK. shiyang.tang@soton.ac.uk. Cluster for Advanced Macromolecular Design School of Chemical Engineering The University of New South Wales Sydney NSW 2052 Australia. Australian Institute of Bioengineering & Nanotechnology The University of Queensland Brisbane QLD 4072 Australia. t.davis@uq.edu.au. Australian Institute of Bioengineering & Nanotechnology The University of Queensland Brisbane QLD 4072 Australia. r.qiao@uq.edu.au.

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Activatable NIR-II Photothermal Lipid Nanoparticles for Improved Messenger RNA Delivery

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Angewandte Chemie 2023年第25期135卷

作者： Dr. Benhao Li Dr. Mengyao Zhao Weiping Lai Dr. Xuanbo Zhang Bowei Yang Prof. Xiaoyuan Chen Prof. Qianqian Ni Departments of Diagnostic Radiology Surgery Chemical and Biomolecular Engineering and Biomedical Engineering Yong Loo Lin School of Medicine and Faculty of Engineering National University of Singapore Singapore 119074 Singapore Nanomedicine Translational Research Program NUS Centre for Nanomedicine Yong Loo Lin School of Medicine National University of Singapore Singapore 117597 Singapore Contribution: Investigation (lead) Writing - original draft (lead) Contribution: Investigation (supporting) Department of Chemistry State Key Laboratory of Molecular Engineering of Polymers and iChem Shanghai Key Laboratory of Molecular Catalysis and Innovative Material Fudan University Shanghai 200433 China Clinical Imaging Research Centre Centre for Translational Medicine Yong Loo Lin School of Medicine National University of Singapore Singapore 117599 Singapore Institute of Molecular and Cell Biology Agency for Science Technology and Research (A*STAR) Singapore 138673 Singapore Contribution: Funding acquisition (equal) Supervision (equal) Writing - review & editing (equal)

Endosomal escape remains a central issue limiting the high protein expression of mRNA therapeutics. Here, we present second near-infrared (NIR-II) lipid nanoparticles (LNPs) containing pH activatable NIR-II dye conjugated lipid (Cy-lipid) for potentiating mRNA delivery efficiency via a s timulus-responsive p hotothermal-promoted e ndosomal e scape d elivery (SPEED) strategy. In acidic endosomal microenvironment, Cy-lipid is protonated and turns on NIR-II absorption for light-to-heat transduction mediated by 1064 nm laser irradiation. Then, the heat-promoted LNPs morphology change triggers rapid escape of NIR-II LNPs from the endosome, allowing about 3-fold enhancement of enhanced green fluorescent protein (eGFP) encoding mRNA translation capacity compared to the NIR-II light free group. In addition, the bioluminescence intensity induced by delivered luciferase encoding mRNA in the mouse liver region shows positive correlation with incremental radiation dose, indicating the validity of the SPEED strategy.

关键词： Endosomal Escape Lipid Nanoparticle Photothermal Effect Second Near-Infrared Window

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Fungal diversity notes 253-366:taxonomic and phylogenetic contributions to fungal taxa

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Fungal Diversity 2016年第3期78卷 1-237页

作者： Guo Jie Li Kevin D.Hyde Rui Lin Zhao Sinang Hongsanan Faten Awad Abdel-Aziz Mohamed A.Abdel-Wahab Pablo Alvarado Genivaldo Alves-Silva Joseph F.Ammirati Hiran A.Ariyawansa Abhishek Baghela Ali Hassan Bahkali Michael Beug D.Jayarama Bhat Dimitar Bojantchev Thitiya Boonpratuang Timur S.Bulgakov Erio Camporesi Marcela CBoro Oldriska Ceska Dyutiparna Chakraborty Jia Jia Chen K.W.Thilini Chethana Putarak Chomnunti Giovanni Consiglio Bao Kai Cui Dong Qin Dai Yu Cheng Dai Dinushani A.Daranagama Kanad Das Monika C.Dayarathne Eske De Crop Rafael J.V.De Oliveira Carlos Alberto Fragoso de Souza JoséIde Souza Bryn T.M.Dentinger Asha J.Dissanayake Mingkwan Doilom E.Ricardo Drechsler-Santos Masoomeh Ghobad-Nejhad Sean P.Gilmore Aristóteles Góes-Neto MichałGorczak Charles H.Haitjema Kalani Kanchana Hapuarachchi Akira Hashimoto Mao Qiang He John K.Henske Kazuyuki Hirayama Maria J.Iribarren Subashini C.Jayasiri Ruvishika S.Jayawardena Sun Jeong Jeon Gustavo H.Jerônimo Ana L.Jesus E.B.Gareth Jones Ji Chuan Kang Samantha C.Karunarathna Paul M.Kirk Sirinapa Konta Eric Kuhnert Ewald Langer Haeng Sub Lee Hyang Burm Lee Wen Jing Li Xing Hong Li Kare Liimatainen Diogo Xavier Lima Chuan Gen Lin Jian Kui Liu Xings Zhong Liu Zuo Yi Liu J.Jennifer Luangsa-ard Robert Lücking H.Thorsten Lumbsch Saisamorn Lumyong Eduardo M.Leaño Agostina V.Marano Misato Matsumura Eric H.C.McKenzie Suchada Mongkolsamrit Peter E.Mortimer Thi Thuong Thuong Nguyen Tuula Niskanen Chada Norphanphoun Michelle A.O’Malley Sittiporn Parnmen Julia Pawłowska Rekhani H.Perera Rungtiwa Phookamsak Chayanard Phukhamsakda Carmen L.A.Pires-Zottarelli Olivier Raspé Mateus A.Reck Sarah C.O.Rocha AndréL.C.M.Ade Santiago Indunil C.Senanayake Ledo Setti Qiu Ju Shang Sanjay K.Singh Esteban B.Sir Kevin V.Solomon Jie Song Prasert Srikitikulchai Marc Stadler Satinee Suetrong Hayato Takahashi Takumasa Takahashi Kazuaki Tanaka Li Ping Tang Kasun M.Thambugala Donnaya Thanakitpipattana Michael K.Theodorou Benjarong Thongbai Tuksaporn Thummarukcharoen Qing Tian Saowaluck Tibpromma Annemieke State Key Laboratory of Mycology Institute of MicrobiologyChinese Academy of SciencesNo 31st West Beichen RoadChaoyang DistrictBeijing 100101People’s Republic of China Centre of Excellence in Fungal Research and School of Science Mae Fah Luang UniversityChiang Rai 57100Thailand Key Laboratory for Plant Diversity and Biogeography of East Asia Kunming Institute of BotanyChinese Academy of ScienceKunming 650201YunnanPeople’s Republic of China Department of Botany and Microbiology College of ScienceKing Saud UniversityP.O.Box:2455Riyadh 1145Saudi Arabia Department of Botany and Microbiology Faculty of ScienceSohag UniversitySohag 82524Egypt ALVALAB C/La Rochela nº47E-39012 SantanderSpain Micolab Programa de Pós-Graduação em Biologia de FungosAlgas e PlantasDepartamento de BotânicaUniversidade Federal de Santa CatarinaCampus Universitário TrindadeCEP:88040-900 FlorianópolisSanta CatarinaBrazil Department of Biology University of WashingtonBox 351800SeattleWA 98195-1800USA Guizhou Key Laboratory of Agricultural Biotechnology Guizhou Academy of Agricultural SciencesGuiyang 550006GuizhouPeople’s Republic of China National Fungal Culture Collection of India(NFCCI) Biodiversity and Palaeobiology GroupMACS’Agharkar Research InstituteG.G.Agarkar RoadPune 411004India PO Box 116 HusumWA 98623-0116USA Formerly Department of BotanyGoa UniversityGoaIndia No.128/1-J Azad Housing SocietyCurcaP.O.Goa Velha 403108India *** 345 Shipwatch LaneHerculesCA 94547USA Microbe Interaction Laboratory(BMIT) BIOTECNational Science and Technology Development Agency(NSTDA)113 Thailand Science ParkThanon PhahonyothinTombon Khlong NuengAmphoeKhlong LuangPathum Thani 12120Thailand Academy of Biology and Biotechnology Southern Federal UniversityRostov-on-Don 344090Rostov regionRussia A.M.B.Gruppo Micologico Forlivese BAntonio“Cicognani” Via Roma Forlì Italy 18 A.M.B.Circolo Micologico“Giovanni Carini”C.P.314BresciaItaly Societàper gli Studi Naturalistici della Romagna C.P.144Bagnacavallo

Notes on 113 fungal taxa are compiled in this paper,including 11 new genera,89 new species,one new subspecies,three new combinations and seven reference *** geographic and taxonomic range of fungal taxa are *** the Ascomycota the new genera Angustospora(Testudinaceae),Camporesia(Xylariaceae),Clematidis,Crassiparies(Pleosporales genera incertae sedis),Farasanispora,Longiostiolum(Pleosporales genera incertae sedis),Multilocularia(Parabambusicolaceae),Neophaeocryptopus(Dothideaceae),Parameliola(Pleosporales genera incertae sedis),and Towyspora(Lentitheciaceae)are *** introduced species are Angustospora nilensis,Aniptodera aquibella,Annulohypoxylon albidiscum,Astrocystis thailandica,Camporesia sambuci,Clematidis italica,Colletotrichum menispermi,***,Comoclathris pimpinellae,Crassiparies quadrisporus,Cytospora salicicola,Diatrype thailandica,Dothiorella rhamni,Durotheca macrostroma,Farasanispora avicenniae,Halorosellinia rhizophorae,Humicola koreana,Hypoxylon lilloi,Kirschsteiniothelia tectonae,Lindgomyces okinawaensis,Longiostiolum tectonae,Lophiostoma pseudoarmatisporum,Moelleriella phukhiaoensis,***,Mucoharknessia anthoxanthi,Multilocularia bambusae,Multiseptospora thysanolaenae,Neophaeocryptopus cytisi,Ocellularia arachchigei,***,Ochronectria thailandica,Ophiocordyceps karstii,Parameliola acaciae,***,Parastagonospora cumpignensis,Pseudodidymosphaeria phlei,Polyplosphaeria thailandica,Pseudolachnella brevifusiformis,Psiloglonium macrosporum,Rhabdodiscus albodenticulatus,Rosellinia chiangmaiensis,Saccothecium rubi,Seimatosporium pseudocornii,***,Sigarispora ononidis and Towyspora *** combinations are provided for Eutiarosporella dactylidis(sexual morph described and illus trated)and Pseudocamarosporium ***,illustrations and/or reference specimens are designated for Aposphaeria corallinolutea,Cryptovalsa ampelina,Dothiorella vidmadera,Ophiocordyceps formosana,P

关键词： Ascomycota Basidiomycota Neocallimastigomycota Oomycota.Zygomycota Phylogeny Taxonomy New genus New species

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