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Designed Fabrication of Multifunctional Magnetic Gold Nanoshells and Their Application to Magnetic Resonance Imaging and Photothermal Therapy†

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Angewandte Chemie 2006年第46期118卷

作者： Jaeyun Kim Sungjin Park Ji Eun Lee Seung Min Jin Jung Hee Lee In Su Lee Ilseung Yang Jun‐Sung Kim Seong Keun Kim Myung‐Haing Cho Taeghwan Hyeon National Creative Research Initiative Center for Oxide Nanocrystalline Materials and School of Chemical and Biological Engineering Seoul National University Seoul 151‐744 Korea Fax: (+82) 2‐886‐8457 Laboratory of Toxicology College of Veterinary Medicine and BK21 Program for Veterinary Science Seoul National University Seoul 151‐744 Korea Fax: (+82) 2‐873‐1268 School of Chemistry Seoul National University Seoul 151‐744 Korea Present address: Advanced Materials Division Korea Research Institute of Chemical Technology Daejeon 305‐343 Korea Department of Radiology Samsung Medical Center School of Medicine Sungkyunkwan University Seoul 137‐200 Korea

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Erratum to: Vol. 35 No. 1 Publisher’s Erratum

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Chinese Journal of Oceanology and Limnology 2017年第2期35卷 466-467页

作者： Shuangyan He Mingxia He Jürgen Fischer Dongliang Yuan Peng Xu Tengfei Xu Xianping Yang Leonid Sokoletsky Xiaodao Wei Fang Shen Juhong Zou Maohua Guo Songxue Cui Wu Zhou Dalu Gao Guangzhen Jin Xianqing Lü Fuwen Qiu Wendong Fang Aijun Pan Jing Cha Shanwu Zhang Jiang Huang Tao Wang Yongzhou Cheng Xiaoyan Chen Zhaopu Liu Xiaohua Long Zhishuai Hou Haishen Wen Jifang Li Feng He Qun Liu Jinhuan Wang Biao Guan Qinglong Wang Md. Shahjahan Md. Farajul Kabir Kizar Ahmed Sumon Lipi Rani Bhowmik Harunur Rashid Shu Li Kefu Yu Jianxin Zhao Yuexing Feng Tianran Chen Shun Zhou Yichao Ren Christopher M. Pearce Shuanglin Dong Xiangli Tian Qinfeng Gao Fang Wang Liming Liu Rongbin Du Xiaoling Zhang Shichun Sun Song Feng Jianing Lin Song Sun Fang Zhang Zhipeng Zhang Xuexi Tang Haitian Tang Jingjing Song Jian Zhou Hongjun Liu Qixiang Wang Kuimei Qian Xia Liu Yuwei Chen Chengjun Sun Fenghua Jiang Wei Gao Xiaoyun Li Yanzhen Yu Xiaofei Yin Yong Wang Haibing Ding Zhongmin Sun Yongqiang Wang Pengcheng Yan Hui Guo Jianting Yao Jiro Tanaka Hiroshi Kawai Na Song Muyan Chen Tianxiang Gao Takashi Yanagimoto Xia Lu Sheng Luan Jie Kong Longyang Hu Yong Mao Shengping Zhong Yan Liu Weihong Zhao Caiyan Li Hui Miao Ocean Remote Sensing Institute Ocean University of China Qingdao China Institute for Space Sciences Freie Universität Berlin Berlin Germany Ocean College Zhejiang University Hangzhou China Key Laboratory of Ocean Circulation and Waves (KLOCAW) Institute of Oceanology Chinese Academy of Sciences Qingdao China Qingdao Collaborative Innovation Center of Marine Science and Technology Qingdao China University of Chinese Academy of Sciences Beijing China First Institute of Oceanography State Oceanic Administration Qingdao China State Key Laboratory of Estuarine and Coastal Research East China Normal University Shanghai China National Satellite Ocean Application Service Beijing China Key Laboratory of Space Ocean Remote Sensing and Application SOA Beijing China Key Laboratory of Physical Oceanography (Ocean University of China) Ministry of Education Qingdao China Key Lab of Marine Science and Numerical Modeling First Institute of Oceanography SOA Qingdao China Third Institute of Oceanography State Oceanic Administration Xiamen China State Key Laboratory of Tropical Oceanography South China Sea Institute of Oceanology Chinese Academy of Sciences Guangzhou China Jiangsu Provincial Key Laboratory of Marine Biology College of Resources and Environmental Sciences Nanjing Agricultural University Nanjing China Fisheries College Ocean University of China Qingdao China Key Laboratory of Mariculture Ministry of Education Ocean University of China Qingdao China Department of Fisheries Management Bangladesh Agricultural University Mymensingh Bangladesh Sado Marine Biological Station Faculty of Science Niigata University Sado Niigata Japan Department of Aquatic Ecology and Water Quality Management Wageningen University Wageningen University and Research Centre Amsterdam The Netherlands Science and Math Program Asian University for Women Chittagong Bangladesh Key laboratory of Marginal Sea Geology South China Sea Institute of Oceanology Chinese Academy of Sciences

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Universal research index: An inclusive metric to quantify scientific research output

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Journal of Academic Librarianship 2023年第3期49卷

作者： Keshavarz-Fathi, Mahsa Yazdanpanah, Niloufar Kolahchi, Sajad Ziaei, Heliya Darmstadt, Gary L. Dorigo, Tommaso Dochy, Filip Levin, Lisa Thongboonkerd, Visith Ogino, Shuji Chen, Wei-Hsin Perc, Matjaz Tremblay, Mark S. Olusanya, Bolajoko O. Rao, Idupulapati M. Hatziargyriou, Nikos Moradi-Lakeh, Maziar Bella, Federico Rosivall, Laszlo Gandomi, Amir H. Sorooshian, Armin Gupta, Manoj Gal, Ciprian Lozano, Andres M. Weaver, Connie Tanzer, Michael Poggi, Alessandro Sepanlou, Sadaf G. Weiskirchen, Ralf Jambrak, Anet Režek Torres, Pedro J. Capanoglu, Esra Barba, Francisco J. Ernest, Chua Kian Jon Sigman, Mariano Pluchino, Stefano Gharehpetian, Gevork B. Fereshtehnejad, Seyed-Mohammad Yang, Muh-Hwa Thomas, Sabu Cai, Wenju Comini, Elisabetta Scolding, Neil J. Myles, Paul S. Nieto, Juan J. Perry, George Sedikides, Constantine Rezaei, Nima School of Medicine Tehran University of Medical Sciences Tehran Iran Universal Scientific Education and Research Network (USERN) Iran Department of Pediatrics Stanford University School of Medicine Stanford CA United States Istituto Nazionale di Fisica Nucleare (INFN) Via Francesco Marzolo Sezione di Padova Italy High Impact Learning Academy Learning and Development Department Brussels Belgium Center for Marine Biodiversity and Conservation Integrative Oceanography Division Scripps Institution of Oceanography University of California San Diego San Diego CA United States Medical Proteomics Unit Office for Research and Development Faculty of Medicine Siriraj Hospital Mahidol University Bangkok Thailand Department of Epidemiology Harvard T.H. Chan School of Public Health Boston MA United States Program in MPE Molecular Pathological Epidemiology Department of Pathology Brigham and Women's Hospital and Harvard Medical School Boston MA United States Broad Institute of MIT and Harvard Cambridge MA United States Department of Aeronautics and Astronautics National Cheng Kung University Tainan Taiwan Research Center for Smart Sustainable Circular Economy Tunghai University Taichung 407 Taiwan Department of Mechanical Engineering National Chin-Yi University of Technology Taichung 411 Taiwan Faculty of Natural Sciences and Mathematics University of Maribor Maribor Slovenia Department of Medical Research China Medical University Hospital China Medical University Taichung Taiwan Complexity Science Hub Vienna Vienna Austria Alma Mater Europaea Maribor Slovenia Children's Hospital of Eastern Ontario Research Institute Department of Pediatrics University of Ottawa Ottawa ON Canada Centre for Healthy Start Initiative Ikoyi Lagos Nigeria Alliance of Bioversity International International Center for Tropical Agriculture Cali Colombia International Centre of Insect Physiology and Ecology (ICIPE) Nairobi Kenya School of Electrical and Computer Engineering Natio

Scientometrics and bibliometrics, the subfields of library and information science, deal with the quantity and quality of research outputs. Currently, various scientometric indices are being used to quantify and compare research outputs. The most widely known is the h-index. However, this index and its derivatives suffer from dependence on the mere count of a scholar's highly cited publications. To remedy this deficiency, we developed a novel index, the Universal Research Index (UR-Index) (https://***/UR-Index/) by which every single publication has its own impact on the total score. We developed this index by surveying international top 1 % cited scientists in various disciplines and included additional component variables such as publication type, leading role of a scholar, co-author count, and source metrics to this scientometric index. We acknowledge that unconscious biases built into the component variables included in the UR-Index might put research from specific groups at a disadvantage, thus continued efforts to improve equitable scholarly impact in science and academia are encouraged. © 2023 Elsevier Inc.

关键词： Citations CiteScore h-index Impact factor Leading author Research impact Scholarly impact Scholarly output Scientometrics UR-Index USERN

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Highly Recyclable and Tough Elastic Vitrimers from a Defined Polydimethylsiloxane Network

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Angewandte Chemie 2023年第47期135卷

作者： Dr. Jiancheng Luo Dr. Xiao Zhao Hao Ju Dr. Xiangjun Chen Dr. Sheng Zhao Dr. Zoriana Demchuk Dr. Bingrui Li Dr. Vera Bocharova Dr. Jan-Michael Y. Carrillo Dr. Jong K. Keum Prof. Sheng Xu Prof. Alexei P. Sokolov Dr. Jiayao Chen Prof. Peng-Fei Cao Chemical Sciences Division Oak Ridge National Laboratory Oak Ridge TN-37830 USA State Key Laboratory of Organic-Inorganic Composites Beijing University of Chemical Technology Beijing 100029 China Materials Science and Engineering Program University of California San Diego La Jolla CA-92093 USA Department of Chemistry University of Tennessee Knoxville TN-37996 USA The Bredesen Center for Interdisciplinary Research and Graduate Education University of Tennessee Knoxville TN-37996 USA Center for Materials Sciences Oak Ridge National Laboratory Oak Ridge TN-37830 USA Neutron Scattering Division Oak Ridge National Laboratory Oak Ridge TN-37830 USA

Despite intensive research on sustainable elastomers, achieving elastic vitrimers with significantly improved mechanical properties and recyclability remains a scientific challenge. Herein, inspired by the classical elasticity theory, we present a design principle for ultra-tough and highly recyclable elastic vitrimers with a defined network constructed by chemically crosslinking the pre-synthesized disulfide-containing polydimethylsiloxane (PDMS) chains with tetra-arm polyethylene glycol (PEG). The defined network is achieved by the reduced dangling short chains and the relatively uniform molecular weight of network strands. Such elastic vitrimers with the defined network, i.e., PDMS-disulfide-D, exhibit significantly improved mechanical performance than random analogous, previously reported PDMS vitrimers, and even commercial silicone-based thermosets. Moreover, unlike the vitrimers with random network that show obvious loss in mechanical properties after recycling, those with the defined network enable excellent thermal recyclability. The PDMS-disulfide-D also deliver comparable electrochemical signals if utilized as substrates for electromyography sensors after the recycling. The multiple relaxation processes are revealed via a unique physical approach. Multiple techniques are also applied to unravel the microscopic mechanism of the excellent mechanical performance and recyclability of such defined network.

关键词： Defined Network Polydimethylsiloxane Recyclable Polymer Tough Elastomer Vitrimers

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Drug Release Kinetics from Polymer Matrix through Fractal Approximation of Motion

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Smart Materials Research 2012年第1期2012卷

作者： S. Băcăiţă C. Urîtu M. Popa A. Uliniuc C. Peptu M. Agop Department of Natural and Synthetic Polymers Faculty of Chemical Engineering and Environmental Protection “Gheorghe Asachi” Technical University Prof. Dr. Docent Dimitrie Mangeron Road No. 73 700050 Iasi Romaniatuiasi.ro Physics Department Faculty of Machine Manufacturing and Industrial Management “Gheorghe Asachi” Technical University Prof. Dr. Docent Dimitrie Mangeron Road No. 59A 700050 Iasi Romaniatuiasi.ro Centre of Advanced Researches for Bionanoconjugates and Biopolymers “Petru Poni” Institute of Macromolecular Chemistry Grigore Ghica Voda Avenue No. 41A 700487 Iasi Romaniaicmpp.ro Lasers Atoms and Molecules Physics Laboratory University of Science and Technology Villeneuve d’Ascq 59655 Lille Franceuniv-lille1.fr

The present paper analyzes the process of drug release from polymer matrix. This process has been considered as fractal polymer process. Since complexity of physical processes is replaced by fractality, the paper studies the process through fractal approach. In drug dynamics, fractal “diffusion” equation can be obtained through fractal approximation of motion. All experimental release curves have been best demonstrated by Weibull relation (which was, in its turn, also demonstrated). Weibull parameters are related to the fractal dimension of drug release kinetics from a polymer matrix. Such a dimension can characterize and measure the complexity of the system. In the above-mentioned context, some experimental results of our researchers are presented and analyzed by comparing them with Peppas relation, a basic law in the description of drug release kinetics. Consequently, experimental data for Weibull relation are better correlated with certain resulting factors. At the same time, some conclusions regarding the phenomena involved in the process are considered as being based on the approach.

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Tumor Targeting: A Strategy for Tumor Targeting by Higher-Order Glycan Pattern Recognition: Synthesis and In Vitro and In Vivo Properties of Glycoalbumins Conjugated with Four DifferentN-Glycan Molecules (Small 46/2020)

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Small 2020年第46期16卷

作者： Ivan Smirnov Regina Sibgatullina Sayaka Urano Tsuyoshi Tahara Peni Ahmadi Yasuyoshi Watanabe Ambara R. Pradipta Almira Kurbangalieva Katsunori Tanaka Biofunctional Chemistry Laboratory Alexander Butlerov Institute of Chemistry Kazan Federal University 18 Kremlyovskaya street Kazan 420008 Russia Biofunctional Synthetic Chemistry Laboratory RIKEN Cluster for Pioneering Research 2-1 Hirosawa Wako Saitama 351-0198 Japan RIKEN Center for Biosystems Dynamics Research 6-7-3 Minatojima-minamimachi Chuo-ku Kobe Hyogo 650-0047 Japan Department of Chemical Science and Engineering School of Materials and Chemical Technology 2-12-1 Ookayama Meguro-ku Tokyo 152-8552 Japan GlycoTargeting Research Laboratory RIKEN Baton Zone Program 2-1 Hirosawa Wako Saitama 351-0198 Japan

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Author Correction: Human and environmental safety of carbon nanotubes across their life cycle

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Nature Reviews Materials 2024年 374页

作者： Mijin Kim Dana Goerzen Prakrit V. Jena Emma Zeng Daniel A. Heller Matteo Pasquali Rachel A. Meidl Molecular Pharmacology Program Memorial Sloan Kettering Cancer Center New York NY USA School of Chemistry and Biochemistry Georgia Institute of Technology Atlanta GA USA Department of Physiology Biophysics and Systems Biology Weill Cornell Medicine Cornell University New York NY USA Department of Pharmacology Weill Cornell Medicine Cornell University New York NY USA Department of Chemical and Biomolecular Engineering Rice University Houston TX USA Carbon Hub Rice University Houston TX USA Department of Chemistry Rice University Houston TX USA Department of Materials Science and NanoEngineering Rice University Houston TX USA Smalley-Curl Institute Rice University Houston TX USA Baker Institute for Public Policy Rice University Houston TX USA

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Centenarian clocks: epigenetic clocks for validating claims of exceptional longevity

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GEROscience 2023年第3期45卷 1817-1835页

作者： Dec, Eric Clement, James Cheng, Kaiyang Church., George M. Fossel., Michael B. Rehkopf, David. H. Rosero-Bixby, Luis Kobor, Michael S. Lin, David TS. Lu, Ake T. Fei, Zhe Guo, Wei Chew, Yap Ching Yang, Xiaojing Putra, Sulistyo E. Dwi Reiner, Alex P. Correa, Adolfo Vilalta, Adrian Pirazzini, Chiara Passarino, Giuseppe Monti, Daniela Arosio, Beatrice Garagnani, Paolo Franceschi, Claudio Horvath, Steve University of California Department of Pediatrics Division of Genetics and Genomic Medicine Irvine USA (GRID:grid.266093.8) (ISNI:0000 0001 0668 7243) Betterhumans Inc. Gainesville USA (GRID:grid.266093.8) University of Ferrara Department of Chemical Pharmaceutical and Agricultural Sciences Ferrara Italy (GRID:grid.8484.0) (ISNI:0000 0004 1757 2064) University of California Los Angeles Medical Informatics David Geffen School of Medicine Los Angeles USA (GRID:grid.19006.3e) (ISNI:0000 0000 9632 6718) Harvard Medical School Department of Genetics Boston USA (GRID:grid.38142.3c) (ISNI:***) Wyss Institute for Biologically Inspired Engineering Harvard University Cambridge USA (GRID:grid.38142.3c) (ISNI:***) Telocyte LLC Grand Rapids USA (GRID:grid.38142.3c) Stanford University Epidemiology & Population Health and Medicine School of Medicine Stanford USA (GRID:grid.168010.e) (ISNI:***) Universidad de Costa Rica Centro Centroamericano de Población San Pedro Costa Rica (GRID:grid.412889.e) (ISNI:0000 0004 1937 0706) University of British Columbia Edwin S.H. Leong Healthy Aging Program Centre for Molecular Medicine and Therapeutics Vancouver Canada (GRID:grid.17091.3e) (ISNI:0000 0001 2288 9830) University of California Los Angeles Dept. of Human Genetics David Geffen School of Medicine Los Angeles USA (GRID:grid.19006.3e) (ISNI:0000 0000 9632 6718) Altos Labs San Diego USA (GRID:grid.518162.9) (ISNI:0000 0005 0774 3285) University of California Los Angeles Dept. of Biostatistics Fielding School of Public Health Los Angeles USA (GRID:grid.19006.3e) (ISNI:0000 0000 9632 6718) Zymo Research Corp Irvine USA (GRID:grid.19006.3e) University of Surabaya Department of Biology Faculty of Biotechnology Surabaya Indonesia (GRID:grid.444430.3) (ISNI:0000 0000 8739 9595) Public Health Sciences Division Fred Hutchinson Cancer Research Center Seattle USA (GRID:grid.270240.3) (ISNI:0000 0001 2180 1622) University of Mississippi Medical Center Medicine and Population Health Science Ja

Claims surrounding exceptional longevity are sometimes disputed or dismissed for lack of credible evidence. Here, we present three DNA methylation-based age estimators (epigenetic clocks) for verifying age claims of centenarians. The three centenarian clocks were developed based on n = 7039 blood and saliva samples from individuals older than 40, including n = 184 samples from centenarians, 122 samples from semi-supercentenarians (aged 105 +), and 25 samples from supercentenarians (aged 110 +). The oldest individual was 115 years old. Our most accurate centenarian clock resulted from applying a neural network model to a training set composed of individuals older than 40. An epigenome-wide association study of age in different age groups revealed that age effects in young individuals (age < 40) are correlated (r = 0.55) with age effects in old individuals (age > 90). We present a chromatin state analysis of age effects in centenarians. The centenarian clocks are expected to be useful for validating claims surrounding exceptional old age.

关键词： Centenarian clocks Epigenetic clocks Longevity

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A LRET Nanoplatform Consisting of Lanthanide and Amorphous Manganese Oxide for NIR-II Luminescence Lifetime Imaging of Tumor Redox Status

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Angewandte Chemie 2022年第47期134卷

作者： Dr. Mengyao Zhao Dr. Hongjun Zhuang Dr. Hongxin Zhang Dr. Benhao Li Jiang Ming Prof. Xiaoyuan Chen Prof. Meiwan Chen State Key Laboratory of Quality Research in Chinese Medicine Institute of Chinese Medical Sciences University of Macau Macau 999078 China Departments of Diagnostic Radiology Surgery Chemical and Biomolecular Engineering and Biomedical Engineering Yong Loo Lin School of Medicine and Faculty of Engineering National University of Singapore Singapore 119074 Singapore Contribution: Conceptualization (lead) Investigation (lead) Writing - original draft (lead) Department of Chemistry State Key Laboratory of Molecular Engineering of Polymers and iChem Shanghai Key Laboratory of Molecular Catalysis and Innovative Material Fudan University Shanghai 200433 China Contribution: Investigation (supporting) Nanomedicine Translational Research Program NUS Center for Nanomedicine Yong Loo Lin School of Medicine National University of Singapore Singapore 117597 Singapore Clinical Imaging Research Centre Centre for Translational Medicine Yong Loo Lin School of Medicine National University of Singapore Singapore 117599 Singapore Institute of Molecular and Cell Biology Agency for Science Technology and Research (A*STAR) Singapore 138673 Singapore Contribution: Funding acquisition (lead) Supervision (lead)

Designing luminescence lifetime sensors in the second near-infrared (NIR-II) window is a great challenge due to the difficult structural construction. Here, we report a tumor redox responsive and easily synthesized material, amorphous manganese oxide (MnO x ) with indirect band gap of 1.02 eV, as an energy acceptor to build a luminescence resonance energy transfer (LRET) toolbox for universally regulating NIR-I to NIR-II luminescence lifetimes of lanthanide nanoparticles, in which energy transfer is based on matched energy gap instead of conventional overlapped spectra. We further utilize ytterbium (Yb 3+ )-doped YbNP@MnO x as an NIR-II luminescence lifetime sensor to realize in vitro quantitative redox visualization with relative errors under 5 % in samples covered with mouse skin. Furthermore, HepG2 cells and tumors with high redox state have been accurately distinguished by NIR-II luminescence lifetime imaging. The quantified intracellular and intratumor glutathione (GSH) levels are highly consistent with the commercial kit results, illustrating the reliable redox visualization ability in biological tissue.

关键词： Amorphous Manganese Oxide Lanthanide Luminescence Lifetime Imaging NIR-II LRET Quantitative Redox Visualization

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Enhancing miso production with optimized puffed-rice koji and its biological function evaluation

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Food Bioscience 2024年 60卷

作者： Lin, Shin-Ping Chou, Yu-Chieh Chen, Chiao-En Lai, Yen-Tso Hsieh, Chen-Che Tsai, Tsung-Yu Lin, Yun-Hsin Santoso, Shella Permatasari Lin, Hui-Wen Cheng, Kuan-Chen School of Food Safety Taipei Medical University 250 Wu-Hsing Street Taipei 11031 Taiwan Research Center of Biomedical Device Taipei Medical University 250 Wu-Hsing Street Taipei 11031 Taiwan TMU Research Center for Digestive Medicine Taipei Medical University 250 Wu-Hsing Street Taipei 11031 Taiwan Ph.D. Program in Drug Discovery and Development Industry College of Pharmacy Taipei Medical University 250 Wu-Hsing Street Taipei 11031 Taiwan Institute of Food Science and Technology National Taiwan University 1 Roosevelt Rd. Sec. 4 Taipei 10617 Taiwan Department of Food and Nutrition Providence University 200 Sec. 7 Taiwan Boulevard Shalu Dist. Taichung 43301 Taiwan Institute of Biotechnology National Taiwan University 1 Roosevelt Rd. Sec. 4 Taipei 10617 Taiwan Department of Food Science Fu Jen Catholic University 510 Zhongzheng Rd. Xinzhuang Dist. New Taipei City 242062 Taiwan Department of Chemical Engineering Widya Mandala Surabaya Catholic University 37 Jl. Kalijudan 37 East Java Surabaya 60114 Indonesia Collaborative Research Center for Zero Waste and Sustainability 37 Jl. Kalijudan East Java Surabaya 60114 Indonesia Department of Optometry Asia University 500 Lioufeng Rd. Wufeng Taichung 41354 Taiwan Department of Medical Research China Medical University Hospital China Medical University 91 Hsueh-Shih Road Taichung 40402 Taiwan

In order to enhance enzyme activities of koji and further improve the health benefits and nutritional value of miso, puffed rice was used to prepare koji with optimization of fermentation utilizing response surface methodology (RSM), and the optimized puffed rice koji was used to produce miso and low-salt miso. Results showed that β-glucosidase activity increased by 1.98-fold after RSM optimization. The optimized puffed rice koji also showed the highest β-amylase and protease activities (237.1 and 968.8 units/g, respectively) compared to rice koji (108.7 and 637.4 units/g, respectively). Moreover, miso made from puffed-rice koji presented a much higher polyphenol content, antioxidant activity, and aglycone conversion. These findings clarified the relationship between changes in enzyme activities in koji and the important components of miso, and also advance solid-state fermentation research and development of functional miso. © 2024

关键词： Aspergillus oryzae Koji Miso Puffed rice Solid-state fermentation β-glucosidase

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