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Sandwich-Structured Solar Cells with Accelerated Conversion Efficiency by Self-Cooling and Self-Cleaning Design

Journal of Bionic engineering 2024年第6期21卷 2955-2968页

作者： Huide Fu Ben Wang Rui He Yongpu Yang Hongyuan Li Zhiguang Guo College of Chemistry and Environmental Engineering Shenzhen UniversityShenzhen518060China State Key Laboratory for Turbulence and Complex Systems Department of Mechanics and Engineering ScienceBeijing Innovation Center for Engineering Science and Advanced TechnologyCollege of EngineeringPeking UniversityBeijing100871China Hubei Collaborative Innovation Centre for Advanced Organic Chemical Materials and Ministry of Education Key Laboratory for the Green Preparation and Application of Functional Materials Hubei UniversityWuhan430062PR China State Key Laboratory of Solid Lubrication Lanzhou Institute of Chemical PhysicsChinese Academy of ScienceLanzhou730000PR China

Photovoltaic(PV)power generation is highly regarded for its capability to transform solar energy into electrical ***,in real-world applications,PV modules are prone to issues such as increased self-heating and surface dust accumulation,which contribute to a reduction in photoelectric conversion ***,elevated temperatures can adversely affect the components’operational *** augment the efficiency and extend the lifespan of PV modules,it is crucial to implement cooling strategies and periodic surface dust *** this research,we introduce a composite PV module design that amalgamates a hygroscopic hydrogel with self-cleaning *** design incorporates a superhydrophobic polydimethylsiloxane(PDMS)film as its exposed surface layer and employs a PAM-CaCl2-SiC hygroscopic hydrogel for rear *** arrangement is intended to facilitate efficient surface self-cleaning and passive cooling of the composite PV *** studies were conducted to evaluate the performance of this innovative composite PV module design,and the results showed that the composite PV panel had an increase of about 1.39%in power generation compared to an ordinary PV panel in the spring of Shenzhen,China.

关键词： Self-cleaning Solar cell Superhydrophobic Hygroscopic hydrogel Conversion efficiency

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Promotional effect of cobalt doping on catalytic performance of cryptomelane-type manganese oxide in toluene oxidation

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Journal of Environmental Sciences 2023年第4期126卷 263-274页

作者： Ning Dong Mengyue Chen Qing Ye Dan Zhang Hongxing Dai Key Laboratory of Beijing on Regional Air Pollution Control Department of Environmental ScienceSchool of Environmental and Chemical EngineeringFaculty of Environment and LifeBeijing University of TechnologyBeijing 100124China R&D Department of Atmospheric Prevention and Control Technology Guangdong Suncere Technology Co.Ltd.Guangzhou 510220China Beijing Key Laboratory for Green Catalysis and Separation Key Laboratory of Beijing on Regional Air Pollution ControlKey Laboratory of Advanced Functional MaterialsEducation Ministry of Chinaand Laboratory of Catalysis Chemistry and NanoscienceDepartment of Environmental Chemical EngineeringSchool of Environmental and Chemical EngineeringFaculty of Environment and LifeBeijing University of TechnologyBeijing 100124China

The cryptomelane-type manganese oxide (OMS-2)-supported Co (x Co/OMS-2;x=5,10,and15 wt.%) catalysts were prepared via a pre-incorporation *** as-prepared materials were used as catalysts for catalytic oxidation of toluene (2000 ppmV).Physical and chemical properties of the catalysts were measured using the X-ray diffraction (XRD),Fourier transform infrared spectroscopic (FT-IR),scanning electron microscopic (SEM),X-ray photoelectron spectroscopy (XPS),and hydrogen temperature-programmed reduction (H_(2)-TPR)*** all of the catalysts,10Co/OMS-2 performed the best,with the T90%,specific reaction rate at 245℃,and turnover frequency at 245℃ (TOFCo) being 245℃,1.23×10^(-3)moltoluene/(gcat·sec),and 11.58×10^(-3)sec-1for toluene oxidation at a space velocity of 60,000mL/(g·hr),*** excellent catalytic performance of 10Co/OMS-2 were due to more oxygen vacancies,enhanced redox ability and oxygen mobility,and strong synergistic effect between Co species and OMS-2 ***,in the presence of poisoning gases CO_(2),SO_(2)or NH_(3),the activity of 10Co/OMS-2 decreased for the carbonate,sulfate and ammonia species covered the active sites and oxygen vacancies,*** the activation treatment,the catalytic activity was partly *** good low-temperature reducibility of 10Co/OMS-2 could also facilitate the redox process accompanied by the consecutive electron transfer between the adsorbed O_(2)and the cobalt or manganese *** the oxidation process of toluene,the benzoic and aldehydic intermediates werefirst generated,which were further oxidized to the benzoate intermediate that were eventually converted into H_(2)O and CO_(2).

关键词： Cryptomelane-type manganese oxide Cobalt doping Volatile organic compound Toluene oxidation

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Effect of turbulent fluctuation on the ignition of millimeter particle:Experimental studies and numerical modelling with a new correlation of nusselt number Author links open overlay panel

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Particuology 2024年第8期91卷 168-175页

作者： Lele Feng Jie Liu Haihui Xin Liangliang Jiang Yuxin Wu Saeideh Babaee Jiangsu Key Laboratory of Coal-based Greenhouse Gas Control and Utilization China University of Mining and TechnologyXuzhou221008China School of Safety Engineering China University of Mining and TechnologyXuzhou221116China Key Laboratory of Hubei Province for Coal Conversion and New Carbon Materials Wuhan University of Science and TechnologyWuhan430000China Department of Chemical and Petroleum Engineering University of CalgaryCalgaryAlbertaCanada Department of Energy and Power Engineering Tsinghua UniversityBeijing100084China Department of Chemical and Metallurgical Engineering University of the WitwatersrandJohannesburgSouth Africa

Understanding the influencing mechanism of turbulent fluctuation on the ignition characteristics of millimeter coal particles is *** this work,to study the effect of turbulent fluctuation on ignition time,millimeter coal particles are subjected to a specific flow field,generated in a furnace with symmetric fans.A one-dimensional model with the new proposed correlation and the Ranz-Marshall(R-M)correlation for Nu(Nusselt number)is established to simulate the coal ignition *** addition,the effects of fan speed,temperature,particle diameter,particle distance and coal type on the ignition time are *** is found that an increase in fan speed from 0 to 3000 rpm leads to a particle Reynolds number Re_(p)increase from 0 to 22.5,and a turbulent particle Reynolds number Re_(t)*increase from 0 to *** a consideration of the fluctuation effect,the new correlation of Nu gives a better prediction of ignition time compared to the R-M ***,the ignition time is revealed to decrease with an increasing fan speed and an elevating *** the ignition time shows merely an initial boost with enlarging particle distance,it exhibits a linearity with the term of particle diameter dp1.3-1.7 and Reynolds numbers(Nu*/Nu)-0.6(Nu*is turbulent Nusselt number).Based on this relationship,the difference of predicted ignition time is calculated at different Re_(p)and Re_(t)*.It is shown that at low Re_(p)or high Re_(t)*values,the new correlation should substitute for the R-M correlation.

关键词： Turbulent fluctuation Particle heat transfer Empirical correlation Coal ignition

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Mesoporous amorphous FeOOH-encapsulated BiO_(2–x) photocatalyst with harnessing broad spectrum toward activation of persulfate for tetracycline degradation

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Chinese Journal of chemical engineering 2024年第7期71卷 235-248页

作者： Pengfei Wu Zhaolong Liu Li Wu Yingkun Zhang Bing Wang Zhanghao Cheng Wenquan Cui Xiangyang Lv Qingling Liu Tianjin Key Laboratory of Indoor Air Environmental Quality Control School of Environmental Science and EngineeringTianjin UniversityTianjin 300350China Hebei Pollution Control Technology Innovation Center of Steel and Coking Industry Department of Environmental and Chemical EngineeringHebei College of Industry and TechnologyShijiazhuang 050091China Hebei Key Laboratory of Environmental Photocatalytic and Electrocatalytic Materials College of Chemical EngineeringNorth China University of Science and TechnologyTangshan 063210China Hebei Academy of Product Quality Supervision&Inspection Shijiazhuang 050227China

With the growing concern about the water environment,the advanced oxidation process of persulfate activation assisted by photocatalysis has attracted considerable attention to decompose dissolved organic *** this work,to overcome the drawbacks of the photocatalytic activity reduction caused by the photo-corrosion of non-stoichiometric BiO_(2–x),a novel material with amorphous FeOOH in situ grown on layered BiO_(2–x) to form a core-shell structure similar to popcorn chicken-like morphology was produced in two simple and environmentally beneficial *** a series of degradation activity tests of hybrid materials under different conditions,the as-prepared materials exhibited remarkable degradation activity and stability toward tetracycline in the FeOOH@BiO_(2–x)/Vis/PS system due to the synergism of photocatalysis and persulfate *** results of XRD,SEM,TEM,XPS,FTIR,and BET show that the loading of FeOOH increases the specific surface area and active sites appreciably;the heterogeneous structure formed by FeOOH and BiO_(2–x) is more favorable to the effective separation of photogenerated *** optimal degradation conditions were at a catalyst addition of 0.7 g·L^(–1),a persulfate concentration of 1.0 g·L^(–1),and an initial pH of 4.5,at which the degradation rate could reach 94.7%after 90 *** influence of typical inorganic anions on degradation was also *** studies and radical quenching experiments revealed that·OH,SO_(4)^(-)·,and·O_(2)^(-)were the principal active species generated during the degradation of *** results of the 1,10-phenanthroline approach proved that the effect of dissolved iron ions on the tetracycline degradation was limited,and the interfacial reaction that occurs on the active sites on the material's surface was a critical *** work provides a novel method for producing efficient broad-spectrum Bismuth-based composite photocatalysts and photocatalytic-activated persulfate synerg

关键词： Amorphous FeOOH BiO_(2–x) Activated persulfate Photocatalytic Tetracycline degradation

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Towards atom-level understanding of metal oxide catalysts for the oxygen evolution reaction with machine learning

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npj Computational materials 2024年第1期10卷 2430-2440页

作者： Jaclyn R.Lunger Jessica Karaguesian Hoje Chun Jiayu Peng Yitong Tseo Chung Hsuan Shan Byungchan Han Yang Shao-Horn Rafael Gómez-Bombarelli Department of Materials Science and Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA Center for Computational Science and Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA Department of Chemical and Biomolecular Engineering Yonsei UniversitySeoul 03722Republic of Korea Department of Computational and Systems Biology Massachusetts Institute of TechnologyCambridgeMA 02139USA Department of Materials Science and Engineering University of TorontoTorontoON M5SCanada Department of Mechanical Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA Research Laboratory of Electronics Massachusetts Institute of TechnologyCambridgeMA 02139USA

Green hydrogen production is crucial for a sustainable future,but current catalysts for the oxygen evolution reaction(OER)suffer from slow kinetics,despite many efforts to produce optimal designs,particularly through the calculation of descriptors for *** this study,we develop a dataset of density functional theory calculations of bulk and surface perovskite oxides,and adsorption energies of OER intermediates,which includes compositions up to quaternary and facets up to(555).We demonstrate that per-site properties of perovskite oxides such as Bader charge or band center can be tuned through element substitution and faceting,and develop a machine learning model that accurately predicts these properties directly from the local chemical *** leverage these per-site properties to identify promising perovskites with high theoretical OER *** identified design principles and promising materials provide a roadmap for closing the gap between current artificial catalysts and biological enzymes such as photosystem II.

关键词： perovskite oxides kinetics

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Tetris-Style Stacking Process to Tailor the Orientation of Carbon Fiber Scaffolds for Efficient Heat Dissipation

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Nano-Micro Letters 2023年第9期15卷 310-324页

作者： Shida Han Yuan Ji Qi Zhang Hong Wu Shaoyun Guo Jianhui Qiu Fengshun Zhang The State Key Laboratory of Polymer Materials Engineering Sichuan Provincial Engineering Laboratory of Plastic/Rubber Complex Processing TechnologyPolymer Research Institute of Sichuan UniversityChengdu 610065People’s Republic of China Department of Mechanical Engineering Faculty of Systems Science and TechnologyAkita Prefectural University015-0055AkitaJapan Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900People’s Republic of China

As the miniaturization of electronic devices and complication of electronic packaging,there are growing demands for thermal interfacial materials with enhanced thermal conductivity and the capability to direct the heat toward heat sink for highly efficient heat ***-based carbon fiber(CF)with ultrahigh axial thermal conductivity and aspect ratios exhibits great potential for developing thermally conductive composites as ***,it is still hard to fabricate composites with aligned carbon fiber in a general approach to fully utilize its excellent axial thermal conductivity in specific ***,three types of CF scaffolds with different oriented structure were developed via magnetic field-assisted Tetris-style stacking and carbonization *** regulating the magnetic field direction and initial stacking density,the self-supporting CF scaffolds with horizontally aligned(HCS),diagonally aligned and vertically aligned(VCS)fibers were *** embedding the polydimethylsiloxane(PDMS),the three composites exhibited unique heat transfer properties,and the HCS/PDMS and VCS/PDMS composites presented a high thermal conductivity of 42.18 and 45.01 W m^(−1)K^(−1)in fiber alignment direction,respectively,which were about 209 and 224 times higher than that of *** excellent thermal conductivity is mainly ascribed that the oriented CF scaffolds construct effective phonon transport pathway in the *** addition,fishbone-shaped CF scaffold was also produced by multiple stacking and carbonization process,and the prepared composites exhibited a controlled heat transfer path,which can allow more versatility in the design of thermal management system.

关键词： Carbon fiber Magnetic field Thermal management Thermally conductive composites

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Three-dimensional lightweight melamine foams modified by MXene sheets and CoNi alloys towards multifunctional microwave absorption

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Nano Research 2025年第2期18卷 377-389页

作者： Nannan Wu Zhengying Shen Yitao Ma Zhizheng Wu Chuanxin Hou Sijie Guo Jian Tian Jiurong Liu School of Material Science and Engineering Shandong University of Science and TechnologyQingdao 266590China School of Mathematics and Systems Science Shandong University of Science and TechnologyQingdao 266590China School of Environmental and Material Engineering Yantai UniversityYantai 264005China Department of Chemical&Biomolecular Engineering University of TennesseeKnoxvilleTN 37996USA Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials Ministry of Education and School of Materials Science and EngineeringShandong UniversityJinan 250061China

Taking the increasing issue of electromagnetic waves(EMW)pollution and the necessity for applications in extreme environments,there is a pressing requirement to create multifunctional microwave absorption materials(MAMs)to meet the current *** this work,we achieved the successful combination of MXene sheets and metal organic framework(MOFs)derived CoNi@C magnetic alloys onto the three dimensional(3D)melamine foam(MF)skeleton using vacuum impregnation and electrostatic self-assembly *** obtained MF@MXene/CoNi@C composite foams achieved outstanding MA performance,with an optimal reflection loss(RL)value of–24.1 dB and a maximum effective absorption bandwidth(EAB)of 6.88 GHz at a thickness of 1.68 mm,effectively covering the whole Ku *** superior MA performance is ascribed to the composite foams’multi-component architecture,distinctive 3D porous structure,and the synergistic impact of multiple loss ***,the MF@MXene/CoNi@C composite foams demonstrate exceptional photothermal conversion,thermal insulation,and infrared stealth capabilities,effectively coping with the demands of applications in extreme *** work serves as a valuable resource and source of inspiration for the development of lightweight broadband,multifunctional efficient MAMs.

关键词： multifunctional microwave absorption MXene thermal insulation infrared stealth

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Accelerating Factor Xa inhibitor discovery with a de novo drug design pipeline

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Chinese Journal of chemical engineering 2024年第8期72卷 85-94页

作者： Yujing Zhao Qilei Liu Jian Du Qingwei Meng Liang Sun Lei Zhang State Key Laboratory of Fine Chemicals Frontiers Science Center for Smart Materials Oriented Chemical EngineeringInstitute of Chemical Process Systems EngineeringSchool of Chemical EngineeringDalian University of TechnologyDalian 116024China Ningbo Institute of Dalian University of Technology Ningbo 315016China Shenzhen Shuli Tech Co. LtdShenzhen 518126China Department of Physics City University of Hong KongTat Chee AvenueKowloonHong Kong SARChina

Small-molecule drugs are essential for maintaining human health. The objective of this study is to identify a molecule that can inhibit the Factor Xa protein and be easily procured. An optimization-based de novo drug design framework, Drug CAMD, that integrates a deep learning model with a mixed-integer nonlinear programming model is used for designing drug candidates. Within this framework, a virtual chemical library is specifically tailored to inhibit Factor Xa. To further filter and narrow down the lead compounds from the designed compounds, comprehensive approaches involving molecular docking,binding pose metadynamics(BPMD), binding free energy calculations, and enzyme activity inhibition analysis are utilized. To maximize efficiency in terms of time and resources, molecules for in vitro activity testing are initially selected from commercially available portions of customized virtual chemical libraries. In vitro studies assessing inhibitor activities have confirmed that the compound EN300-331859shows potential Factor Xa inhibition, with an IC_(50)value of 34.57 μmol·L^(-1). Through in silico molecular docking and BPMD, the most plausible binding pose for the EN300-331859-Factor Xa complex are identified. The estimated binding free energy values correlate well with the results obtained from biological assays. Consequently, EN300-331859 is identified as a novel and effective sub-micromolar inhibitor of Factor Xa.

关键词： chemical product design Mathematical programming method Deep learning Binding affinity Factor Xa inhibitor

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Towards designing high mechanical performance low-alloyed wrought magnesium alloys via grain boundary segregation strategy:A review

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Journal of Magnesium and Alloys 2024年第5期12卷 1774-1791页

作者： Zhi Zhang Jinshu Xie Jinghuai Zhang Xu-Sheng Yang Ruizhi Wu Key Laboratory of Superlight Material and Surface Technology Ministry of EducationCollege of Materials Science and Chemical EngineeringHarbin Engineering UniversityHarbin 150001China State Key Laboratory of Ultra-Precision Machining Technology Department of Industrial and Systems EngineeringThe Hong Kong Polytechnic UniversityHung HomKowloonHong KongChina Hong Kong Polytechnic University Shenzhen Research Institute Shenzhen 518060China

Low-alloyed magnesium(Mg)alloys have emerged as one of the most promising candidates for lightweight ***,their further application potential has been hampered by limitations such as low strength,poor plasticity at room temperature,and unsatisfactory *** address these challenges,grain refinement and grain structure control have been identified as crucial factors to achieving high performance in low-alloyed Mg *** effective way for regulating grain structure is through grain boundary(GB)*** review presents a comprehensive summary of the distribution criteria of segregated atoms and the effects of solute segregation on grain size and growth in Mg *** analysis encompasses both single element segregation and multi-element co-segregation behavior,considering coherent interfaces and incoherent ***,we introduce the high mechanical performance low-alloyed wrought Mg alloys that utilize GB segregation and analyze the potential impact mechanisms through which GB segregation influences materials *** upon these studies,we propose strategies for the design of high mechanical performance Mg alloys with desirable properties,including high strength,excellent ductility,and good formability,achieved through the implementation of GB *** findings of this review contribute to advancing the understanding of grain boundary engineering in Mg alloys and provide valuable insights for future alloy design and optimization.

关键词： Magnesium alloys Grain boundary segregation High strength High plasticity High formability

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Interface engineering and Anion engineering of Mo-Based Heterogeneous Electrocatalysts for Hydrogen Evolution Reaction

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Energy & Environmental materials 2023年第1期6卷 87-104页

作者： Zehao Yin Xuan Liu Siru Chen Tingli Ma Yanqiang Li State Key Laboratory of Fine Chemicals School of Chemical EngineeringDalian University of TechnologyPanjin CampusPanjin 124221China School of Material and Chemical Engineering Centre for Advanced Materials ResearchZhongyuan University of TechnologyZhengzhou 450007China Department of Materials Science and Engineering China Jiliang UniversityHangzhou 310018China Graduate School of Life Science and Systems Engineering Kyushu Institute of TechnologyKitakyushu Fukuoka 808-0196Japan

Development and utilization of hydrogen energy is an effective way to achieve carbon neutrality,only hydrogen production through electrolytic water splitting meets the goal of zero carbon *** facilitate the large-scale commercialization of water splitting devices,the development of highly efficient and low-cost catalysts to reduce the energy consumption is ***_(2)has been regarded as a promising electrocatalyst to replace platinum in hydrogen evolution reaction due to its low price and unique 2D layered ***,the poor conductivity and inert basal planes of MoS_(2)limited its wide-spread ***,researches have demonstrated that the conductivity and active sites of MoS_(2)can be improved by heteroatoms doping or constructing of heterogeneous *** this review,the recent progress of Mo-based catalysts are summarized centered on MoS_(2)based on interface engineering and anion engineering,including MoS_(2)–MoO_(2),MoS_(2)–Mo_(2)C,MoS_(2)–MoN_(x),MoS_(2)–MoP,and MoS_(2)–MoSe_(2).The preparation method,structure,and performance of the catalysts are introduced and the possible mechanism behind the improved catalytic activity are revealed to give readers an overall comprehension on the progress of the Mo-based electrocatalysts for hydrogen evolution *** addition,an outlook on future opportunities and development directions of Mo-based catalysts are proposed to facilitate the development of Mo-based catalysts for hydrogen production.

关键词： electrocatalysis heterostructure hydrogen evolution reaction Mo-based catalysts

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