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Future Foods 2025年 11卷

作者： Possari, Laís T. Paula, Marina S. de Nunes, George F. Reis, Iago A. Basaglia, Marcos V. Otoni, Caio G. Bettini, Sílvia H.P. Federal University of São Carlos (UFSCar) Graduate Program in Materials Science and Engineering (PPGCEM) SP São Carlos 13565-905 Brazil Federal University of São Carlos (UFSCar) Department of Materials Engineering (DEMa) SP São Carlos 13565-905 Brazil University of Campinas (UNICAMP) Institute of Chemistry SP Campinas 13083-862 Brazil

Bioplastics have the potential to mitigate the aggravating crisis of plastic pollution. Valorizing agri-food side streams for such a purpose is particularly beneficial as it valorizes massively produced waste, thus contributing to the shift towards circular and regenerative productive chains. In this work, citrus pulp (CP) obtained as a by-product from orange juice production was upcycled into thermoplastic compounds via extrusion-assisted plasticization with glycerol. Compounds with poly(lactic acid) (PLA) were then produced by extrusion melt blending. An experimental 2² factorial design with a central point was performed to evaluate their mechanical, thermal, and biodegradation behavior. The levels for the variables plasticized CP (PCP) and glycerol contents were 30 and 70 % for PCP, and 40 and 60 % for glycerol. Calorimetry showed that PCP increased PLA free volume and chain mobility. Still, the different fractions of PCP and glycerol did not alter the melting behavior of the compounds significantly. PCP led to a progressive toughening effect on PLA. Mass loss after 90 d of soil burial reached 53–64 % for the formulations containing 70 % PCP, and PLA chain scission was accelerated at 30 % PCP with 60 % glycerol, and 70 % PCP with 40 % glycerol. This work opens new pathways to citrus biomass valorization by exploring CP, a scarcely investigated residue, and a novel processing strategy. The produced compounds can be applied as bio-based semi-rigid packaging and utensils. © 2025

关键词： Biodegradable plastic Biomass Citrus sinensis Food waste PLA Upcycling

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Research on Shelf-Life Extension Technologies for Food Sustainability: An Assessment of Scientific Activities and Networks

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Scientific World Journal 2022年第1期2022卷 7120662页

作者： Thavorn, Jakkrit Muangsin, Veera Gowanit, Chupun Muangsin, Nongnuj Technopreneurship and Innovation Management Program Graduate School Chulalongkorn University Bangkok 10330 Thailand Department of Computer Engineering Faculty of Engineering Chulalongkorn University Bangkok 10330 Thailand Department of Chemistry Faculty of Science Chulalongkorn University Bangkok 10330 Thailand

A clearer understanding of research streams and players involved in efforts to address the sustainability of global food and agricultural systems is needed to clarify the current state of scientific knowledge and form collaborations to pursue future research directions. This study presents new insights into this issue through a scientometric process involving a case study of technologies for extending fruit shelf-life. The text mining software was utilized to analyze 3,131 Web of science-indexed articles published between 2000 and 2020 as a means to glean the conceptual structure of current knowledge and conduct a social network analysis to explore scientific and publication activity. The findings were mapped onto a strategic diagram of research productivity and collaboration between players at the national, organizational, and individual levels. This research's main findings highlight that research on shelf-life technology is in continuous development, and academic institutions from China, Spain, and the U.S. are the core national players in this field. The results provide insights for further investigation to strengthen co-research and technological development programs in other fields. Researchers who are exploring networking opportunities can use the model and process presented as a guideline for identifying emerging and future research trends and formulating strategies. © 2022 Jakkrit Thavorn et al.

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Leaky Waves in Flatland

Leaky Waves in Flatland

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European Conference on Antennas and Propagation, EuCAP

作者： Massimo Moccia Giuseppe Castaldi Andrea Alù Vincenzo Galdi Department of Engineering Fields & Waves Lab University of Sannio Benevento Italy Photonics Initiative Advanced Science Research Center City University of New York New York NY USA Department of Electrical Engineering City College of The City University of New York New York NY USA Physics Program Graduate Center City University of New York New York NY USA

We introduce a new in-plane radiation mechanism that can occur in artificial or natural low-dimensional materials, which can be viewed as the "flatland" analog of conventional leaky-wave radiation. We show that this concept can be physically realized in suitably designed planar junctions of purely reactive, isotropic metasurfaces supporting line waves. Our results provide a new tool for manipulating surface waves, which can find interesting applications in the emerging field of van der Waals polaritonics.

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Enhanced electrochemical performance of a LiFePO4 cathode with an environmentally friendly pectin/polyethylene glycol binder

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Journal of Power Sources 2024年 613卷

作者： Chen, Yan-Ruei Chen, Liang-Yu Chung, Chin-Yi Su, Yu-Hsuan Wu, Feng-Yu Hsu, Tsung-Ming Chi, Po-Wei Wu, Phillip M. Chang-Liao, Kuei-Shu Tang, Hong-Yi Wu, Maw-Kuen Institute of Physics Academia Sinica 128 Section 2 Academia Road Taipei11529 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University 128 Section 2 Academia Road Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu300044 Taiwan College of Science National Chung Hsing University 145 Xingda Road South District Taichung402 Taiwan Department of Applied Chemistry National Chi-Nan University 1 University Road Puli Nantou545301 Taiwan

The advancement of lithium-ion battery technology relies on the development of materials that not only improve performance but also align with environmental sustainability. This work presents a novel water-based pectin-PEG binder for LiFePO4 cathodes that combines eco-friendliness with electrochemical innovation. The binder material is made by mixing pectin, a flexible natural substance, with polyethylene glycol through a radical copolymerization process. This combination gives the binder both flexibility and a boost in electrical performance. Our experimental results demonstrate that LFP cathodes with this binder have an intriguing self-healing ability in comparison with the conventional PVDF binder, enhanced charge-discharge capacities, improved cycling stability, and higher ionic conductivity. Specifically, electrodes utilizing the pectin-PEG binder exhibit an impressive retention of discharge capacity. They maintain roughly 150 mAh g−1 after 500 cycles at 1C with 99% retention, and about 141 mAh g−1 with 97% retention at 3C. Cyclic voltammetry (CV) confirms that the PP binder maintains its ionic diffusion properties at high sweep rates, whereas galvanostatic intermittent titration technique reveals a much higher lithium ion diffusion coefficient (DLi+) within the operational voltage range of the LFP-PP250 electrodes. These findings establish an attractive direction for the development of electrodes for high-energy density, sustainable lithium-ion batteries. © 2024 Elsevier B.V.

关键词： Lithium compounds

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Global dispersal and adaptive evolution of domestic cattle:a genomic perspective

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Stress Biology 2023年第1期3卷 98-110页

作者： Xiaoting Xia Kaixing Qu Yan Wang Mikkel-Holger SSinding Fuwen Wang Quratulain Hanif Zulfiqar Ahmed Johannes A.Lenstra Jianlin Han Chuzhao Lei Ningbo Chen Key Laboratory of Animal Genetics Breeding and Reproduction of Shaanxi ProvinceCollege of Animal Science and TechnologyNorthwest A&F UniversityYangling 712100China Academy of Science and Technology Chuxiong Normal UniversityChuxiong 675000China Qingdao Municipal Bureau of Agriculture and Rural Affairs Qingdao 266000China Section for Computational and RNA Biology Department of BiologyUniversity of CopenhagenCopenhagen 1350Denmark National Institute for Biotechnology and Genetic Engineering FaisalabadPakistan Faculty of Veterinary and Animal Sciences University of Poonch RawalakotAzad Jammu and Kashmir 12350Pakistan Faculty of Veterinary Medicine Utrecht UniversityUtrechtThe Netherlands Livestock Genetic Program International Livestock Research Institute(ILRI)Nairobi 00100Kenya CAAS-ILRI Joint Laboratory On Livestock and Forage Genetic Resources Institute of Animal ScienceChinese Academy of Agricultural Sciences(CAAS)Beijing 100193China

Domestic cattle have spread across the globe and inhabit variable and unpredictable *** have been exposed to a plethora of selective pressures and have adapted to a variety of local ecological and management conditions,including UV exposure,diseases,and stall-feeding *** selective pressures have resulted in unique and important phenotypic and genetic differences among modern cattle breeds/*** efforts to sequence the genomes of local and commercial cattle breeds/populations,along with the growing availability of ancient bovid DNA data,have significantly advanced our understanding of the genomic architecture,recent evolution of complex traits,common diseases,and local adaptation in ***,we review the origin and spread of domestic cattle and illustrate the environmental adaptations of local cattle breeds/populations.

关键词： Cattle Origin Domestication Migration route Environmental adaptation Selective pressure

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A Constraint on the Amount of Hydrogen from the CO Chemistry in Debris Disks

arXiv

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arXiv 2023年

作者： Iwasaki, Kazunari Kobayashi, Hiroshi Higuchi, Aya E. Aikawa, Yuri Center for Computational Astrophysics National Astronomical Observatory of Japan Osawa Mitaka Tokyo181-8588 Japan Department of Physics Nagoya University Furo-cho Chikusa-ku Aichi Nagoya464-8602 Japan Division of Science School of Science and Engineering Tokyo Denki University Ishizaka Hatoyama-machi Hiki-gun Saitama350-0394 Japan Department of Astronomy Graduate School of Science The University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo113-0033 Japan

The faint CO gases in debris disks are easily dissolved into C by UV irradiation, while CO can be reformed via reactions with hydrogen. The abundance ratio of C/CO could thus be a probe of the amount of hydrogen in the debris disks. We conduct radiative transfer calculations with chemical reactions for debris disks. For a typical dust-to-gas mass ratio of debris disks, CO formation proceeds without the involvement of H2 because a small amount of dust grains makes H2 formation inefficient. We find that the CO to C number density ratio depends on a combination of nHZ0.4χ−1.1, where nH is the hydrogen nucleus number density, Z is the metallicity, and χ is the FUV flux normalized by the Habing flux. Using an analytic formula for the CO number density, we give constraints on the amount of hydrogen and metallicity for debris disks. CO formation is accelerated by excited H2 either when the dust-to-gas mass ratio is increased or the energy barrier of chemisorption of hydrogen on the dust surface is decreased. This acceleration of CO formation occurs only when the shielding effects of CO are insignificant. In shielded regions, the CO fractions are almost independent of the parameters of dust grains. Copyright © 2023, The Authors. All rights reserved.

关键词： Dust

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Core packing of well-defined x-ray and NMR structures is the same

arXiv

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arXiv 2022年

作者： Grigas, Alex T. Liu, Zhuoyi Regan, Lynne O’Hern, Corey S. Graduate Program in Computational Biology and Bioinformatics Yale University New HavenCT06520 United States Integrated Graduate Program in Physical and Engineering Biology Yale University New HavenCT06520 United States Department of Mechanical Engineering and Materials Science Yale University New HavenCT06520 United States Institute of Quantitative Biology Biochemistry and Biotechnology Centre for Synthetic and Systems Biology School of Biological Sciences University of Edinburgh United Kingdom Department of Physics Yale University New HavenCT06520 United States Department of Applied Physics Yale University New HavenCT06520 United States

Numerous studies have investigated the differences and similarities between protein structures determined by solution NMR spectroscopy and those determined by x-ray crystallography. A fundamental question is whether any observed differences are due to differing methodologies, or to differences in the behavior of proteins in solution versus in the crystalline state. Here, we compare the properties of the hydrophobic cores of high-resolution protein crystal structures and those in NMR structures, determined using increasing numbers and types of restraints. Prior studies have reported that many NMR structures have denser cores compared to those of high-resolution x-ray crystal structures. Our current work investigates this result in more detail, and finds that these NMR structures tend to violate basic features of protein stereochemistry, such as small non-bonded atomic overlaps and few Ramachandran and side chain dihedral angle outliers. We find that NMR structures solved with more restraints, and which do not significantly violate stereochemistry, have hydrophobic cores that have a similar size and packing fraction as their counterparts determined by x-ray crystallography at high-resolution. These results lead us to conclude that, at least regarding the core packing properties, high-quality structures determined by NMR and x-ray crystallography are the same, and the differences reported earlier are most likely a consequence of methodology, rather than fundamental differences between the protein in the two different environments. Significance: Dense packing of hydrophobic residues is key to protein structure and stability. Previously, it has been noted that structures solved by NMR spectroscopy have denser cores than x-ray crystal structures. Here, we calculate the core size and packing fraction of NMR structures with experimental restraints in the PDB. Their cores are typically smaller, but denser. However, NMR structures with accurate stereochemistry possess core pa

关键词： X ray crystallography

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Guiding Brain-to-Vocalization Decoder Design Using Structured Generalization Error

Guiding Brain-to-Vocalization Decoder Design Using Structure...

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Annual International Conference of the IEEE engineering in Medicine and Biology Society (EMBC)

作者： Jingya Huang Pablo Tostado-Marcos Sowmya Manojna Narasimha Aashish N. Patel Ezequiel. M. Arneodo Timothy Q. Gentner Gal Mishne Vikash Gilja Department of Electrical and Computer Engineering University of California San Diego CA Department of Bioengineering University of California San Diego CA Institute for Neural Computation University of California San Diego CA Neuroscience Graduate Program University of California San Diego CA Department of Physics University of California San Diego CA Department of Psychology University of California San Diego CA Halıcıoğlu Data Science Institute University of California San Diego CA

ISBN: (数字)9798350371499

ISBN: (纸本)9798350371505

State-of-the-art intracortical neuroprostheses currently enable communication at 60+ words per minute for anarthric individuals by training on over 10K sentences to account for phoneme variability in different word contexts. There is limited understanding about whether this performance can be maintained in decoding naturalistic speech with 40K+ word vocabularies across elicited, spontaneous, and conversational speech contexts. We introduce a vocal-unit-level generalization test to explicitly evaluate neural decoder performance with an expanded and more diverse behavioral repertoire. Tested on neural decoders modeling zebra finch vocalization, an analog to human vocal production, we compare three decoders with different input types: spike trains, neural factors, and firing rates. The factors and rates are latent neural features inferred using trained Latent Factor Analysis via Dynamical Systems (LFADS) models that capture the population neural dynamics during vocal production. While the conventional random holdout generalization error measure is similar for all three decoders, factor- and rate-based decoders outperform spike-based decoders when testing vocal-unit-holdout generalization error. These results suggest the later models better adapt to flexible vocalization inference when trained with partial observation of data variation, motivating further exploration of decoders incorporating latent neural and vocalization dynamics.

关键词： Training Adaptation models Vocabulary Firing Measurement uncertainty Neuroprostheses Production Decoding engineering in medicine and biology Testing

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Methyl Nitrate as a Byproduct in Advanced Water Treatment Systems: Liquid Chromatographic Determination Method and Cause of Formation

SSRN

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SSRN 2023年

作者： Kodamatani, Hitoshi Sugihara, Kenta Mezyk, Stephen P. Ishida, Kenneth P. Roback, Shannon L. Plumlee, Megan H. Chemistry Program Department of Science Graduate School of Science and Engineering Kagoshima University 1-21-35 Korimoto Kagoshima890-0065 Japan Department of Chemistry and Biochemistry California State University Long BeachCA90840 United States Research and Development Department Orange County Water District Fountain ValleyCA92708 United States Social Ecology University of California IrvineCA92697 United States

Neutral low-molecular-weight organics such as methyl nitrate that can readily pass through reverse osmosis (RO) membranes employed in potable water reuse facilities attract interest owing to public health considerations. In this study, a novel determination method based on high-performance liquid chromatography, online photochemical conversion to peroxynitrite, and luminol chemiluminescence detection was developed for methyl nitrate measurement in treated water. The maximum photochemical conversion efficiency of methyl nitrate to peroxynitrite was found to be 6.5% using a 222-nm excimer lamp. The calibration curve for the developed method was linear between 1.0 × 10−9 and 1.0 × 10−7 M, and the limit of detection was 0.3 nM (0.03 μg/L) given an injection volume of 200 μL. The methyl nitrate concentrations in RO permeate from reclaimed wastewater and product water after subsequent treatment by a UV/H2O2 advanced oxidation process (AOP) were 2.2 and 22.5 nM (0.17 and 1.7 μg/L), respectively. UV irradiation of RO permeate in the laboratory using a low-pressure Hg lamp confirmed the formation of methyl nitrate in the permeate in the absence of H2O2 and residual chloramines. This chemiluminescent detection method for methyl nitrate will promote a greater understanding of the origin and formation of this treatment byproduct in reclaimed wastewater. © 2023, The Authors. All rights reserved.

关键词： Irradiation

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Perturbation theory for evolution of cooperation on networks

arXiv

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arXiv 2022年

作者： Meng, Lingqi Masuda, Naoki Department of Mathematics University at Buffalo State University of New York BuffaloNY14260-2900 United States Computational and Data-Enabled Science and Engineering Program University at Buffalo State University of New York BuffaloNY14260-5030 United States

Network structure is a mechanism for promoting cooperation in social dilemma games. In the present study, we explore graph surgery, i.e., to slightly perturb the given network, towards a network that better fosters cooperation. To this end, we develop a perturbation theory to assess the change in the propensity of cooperation when we add or remove a single edge to/from the given network. Our perturbation theory is for a previously proposed random-walk-based theory that provides the threshold benefit-to-cost ratio, (b/c)∗, which is the value of the benefit-to-cost ratio in the donation game above which the cooperator is more likely to fixate than in a control case, for any finite networks. We find that (b/c)∗ decreases when we remove a single edge in a majority of cases and that our perturbation theory captures at a reasonable accuracy which edge removal makes (b/c)∗ small to facilitate cooperation. In contrast, (b/c)∗ tends to increase when we add an edge, and the perturbation theory is not good at predicting the edge addition that changes (b/c)∗ by a large amount. Our perturbation theory significantly reduces the computational complexity for calculating the outcome of graph *** Codes 91A22, 91D30 Copyright © 2022, The Authors. All rights reserved.

关键词： Surgery

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