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Emerging WS_(2)/WSe_(2)@graphene nanocomposites: synthesis and electrochemical energy storage applications

Rare Metals 2024年第1期43卷 1-19页

作者： Yu-Meng Gao Yong Liu Kai-Jia Feng Jun-Qing Ma Ying-Jie Miao Bin-Rui Xu Kun-Ming Pan Osaka Akiyoshi Guang-Xin Wang Ke-Ke Zhang Qiao-Bao Zhang National Joint Engineering Research Center for Abrasion Control and Molding of Metal Materials Henan Key Laboratory of Non-Ferrous Materials Science and Processing TechnologySchool of Materials Science and EngineeringHenan University of Science and TechnologyLuoyang 471023China Provincial and Ministerial Co-Construction of Collaborative School of Electrical Engineering Henan University of Science and TechnologyLuoyang 471023China Biomaterials Laboratory Faculty of EngineeringOkayama UniversityTsushima-NakeOkayama-Shi 700-8530Japan Department of Materials Science and Engineering College of MaterialsXiamen UniversityXiamen 361005China Fujian Key Laboratory of Surface and Interface Engineering for High Performance Materials Xiamen UniversityXiamen 361005China

In recent years, tungsten disulfide(WS_(2)) and tungsten selenide(WSe_(2)) have emerged as favorable electrode materials because of their high theoretical capacity, large interlayer spacing, and high chemical activity;nevertheless, they have relatively low electronic conductivity and undergo large volume expansion during cycling, which greatly hinder them in practical applications. These drawbacks are addressed by combining a superior type of carbon material, graphene, with WS_(2) and WSe_(2) to form a WS_(2)/WSe_(2)@graphene *** materials have received considerable attention in electro-chemical energy storage applications such as lithium-ion batteries(LIBs), sodium-ion batteries(SIBs),and supercapacitors. Considering the rapidly growing research enthusiasm on this topic over the past several years, here the recent progress of WS_(2)/WSe_(2)@graphene nanocomposites in electrochemical energy storage applications is summarized. Furthermore, various methods for the synthesis of WS_(2)/WSe_(2)@graphene nanocomposites are reported and the relationships among these methods, nano/microstructures, and electrochemical performance are systematically summarized and discussed. In addition, the challenges and prospects for the future study and application of WS_(2)/WSe_(2)@graphene nanocomposites in electrochemical energy storage applications are proposed.

关键词： WS_(2)/WSe_(2)@graphene nanocomposites Liion batteries(LIBs) Na-ion batteries(SIBs) Supercapacitors Electrochemical performance

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Temperature-dependent microstructural evolution in a compositionally complex solid electrolyte:The role of a grain boundary transition

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Journal of Advanced Ceramics 2025年第3期14卷 163-176页

作者： Shu-Ting Ko Chaojie Du Huiming Guo Hasti Vahidi Jenna L.Wardini Tom Lee Yi Liu Jingjing Yang Francisco Guzman Timothy J.Rupert William J.Bowman Shen J.Dillon Xiaoqing Pan Jian Luo Aiiso Yufeng Li Family Department of Chemical and Nano Engineering University of California San DiegoLa JollaCalifornia 92093USA Program in Materials Science and Engineering University of California San DiegoLa JollaCalifornia 92093USA Department of Materials Science and Engineering University of California IrvineIrvineCalifornia 92697USA Department of Physics and Astronomy University of California IrvineIrvineCalifornia 92697USA Irvine Materials Research Institute University of California IrvineIrvineCalifornia 92697USA

Compositionally complex solid electrolyte(Li_(0.375)Sr_(0.4375))(Ta_(0.375)Nb_(0.375)Zr_(0.125)Hf_(0.125))O_(3)(LSTNZH)samples are synthesized using different sintering temperatures,durations,and cooling conditions(furnace cooling(FC)*** quenching(AQ)).The temperature-dependent grain growth has been examined to investigate the microstructural evolution and the origin of exaggerated(abnormal)grain *** moderate temperatures,the grain growth of LSTNZH follows a cubic root growth model with an Arrhenius temperature *** increasing temperature,bimodal microstructures develop,and the Arrhenius temperature dependence breaks ***,increasing the temperature induces increased Nb segregation at general grain boundaries(GBs),in contrast to classical GB segregation models but suggesting premelting-like GB disordering,which can explain the observed abnormal grain growth(AGG).In addition,the large grains become faceted with increasing temperature,which occurs concurrently with the temperature-induced transitions in GB segregation and grain growth,thereby further supporting the occurrence of a GB phase-like(complexion)*** impacts on the densification,ionic conductivity,and hardness are also *** work provides a new insight into the fundamental understanding of the grain growth mechanisms of the emergent class of medium-and high-entropy compositionally complex ceramics(CCCs),which is essential for tailoring microstructures and material properties.

关键词： compositionally complex ceramics(CCCs) solid electrolytes perovskite grain growth grain boundary(GB) electron backscatter diffraction(EBSD)

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Crafting chirality in three dimensions via a novel fabrication technique for bound states in the continuum metasurfaces

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Light(science & Applications) 2024年第3期13卷 390-392页

作者： Zaid Haddadin Anna My Nguyen Lisa V.Poulikakos Department of Electrical&Computer Engineering University of California San DiegoLa JollaCAUSA Department of Mechanical&Aerospace Engineering University of California San DiegoLa JollaCAUSA Program of Materials Science&Engineering University of California San DiegoLa JollaCAUSA

An additional deposition step was added to a multi-step electron beam lithographic fabrication process to unlock the height dimension as an accessible parameter for resonators comprising unit cells of quasi-bound stat... 详细信息

关键词： dimensions dimension intrinsic

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Boost DC-DC converter with regenerative snubber

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Energy Reports 2024年 12卷 798-819页

作者： Yau, Yeu-Torng Department of Ph.D. Program Prospective Technology of Electrical Engineering and Computer Science National Chin-Yi University of Technology Taichung Taiwan Department of Electrical Engineering National Chin-Yi University of Technology Taichung Taiwan

To accommodate the wide range of input voltages supplied by redundant batteries and ensure an adequate hold-up time for communication systems during utility power failures, power supplies used in 5 G base stations typically include a front-end boost converter as the first stage and a second-stage isolated converter. In this paper, a new topology for a regenerative snubber in boost converters is proposed. Compared to traditional active or passive snubber topologies, the proposed snubber offers the advantages of having fewer components and occupying less space. Moreover, it does not require additional active devices and can be driven by widely-used commercial PWM control integrated circuits, achieving a higher level of cost-effectiveness and offering increased industrial applications. The final prototype of a power supply for a networking switch hub (as used in 5 G base stations) is fabricated to demonstrate the feasibility of the proposed method. © 2024 The Authors

关键词： Topology

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Tough Polymeric Hydrogels Based on Amino Acid Derivative Mediated Dynamic Metal Coordination Bonds

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Chinese Journal of Polymer science 2024年第10期42卷 1578-1588,I0014页

作者： Meng Li Meng-Yuan Zhang Wu-Xuan Lei Zhu-Ting Lv Qing-Hua Shang Zheng Zhao Jiang-Tao Li Yi-Long Cheng Engineering Research Center of Energy Storage Materials and Devices Ministry of EducationSchool of ChemistryXi’an Jiaotong UniversityXi’an710049China Polymer Materials&Engineering Department School of Materials Science&Engineering Chang’an UniversityXi’an710064China School of Electrical Engineering Xi’an Jiaotong UniversityXi’an710049China Department of Nuclear Medicine the First Affiliated Hospital of ChinaXi’an Jiaotong UniversityXi’an710049China

Abstract The development of physically crosslinked hydrogels with excellent mechanical and sensing properties is of importance for expanding the practical applications of intelligent soft hydrogel ***,after copolymerization of hydroxyl-containing amino acid derivative N-acryloyl serine(ASer)with acrylamide(AM),we introduce Zr4+through an immersion strategy to construct metal ion-toughened non-covalent crosslinked hydrogels(with tensile strength of up to 5.73 MPa).It is found that the synergistic coordination of hydroxyl and carboxyl groups with Zr^(4+)substantially increases the crosslinking density of the hydrogels,thereby imparting markedly superior mechanical properties compared to hydroxyl-free Zr^(4+)-crosslinked hydrogels,such as N-acryloyl alanine(AAla)copolymerized with AM hydrogels(with tensile strength of 2.98 MPa)Through the adjustment of the composition of the copolymer and the density of coordination bonds,the mechanical properties of the hydrogels can be modulated over a wide ***,due to the introduction of metal ions and the dynamic nature of coordination bonds,the hydrogels also exhibit excellent sensing performance and good self-recovery properties,paving the way for the development of flexible electronic substrates with outstanding comprehensive performances.

关键词： Hydrogel Amino acid Metal coordination Mechanical performance Flexible sensor

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Hardware Implementations of Interleaved Modular Multiplications Over F256 3

Hardware Implementations of Interleaved Modular Multiplicati...

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3rd International Conference on Advancement in electrical and Electronic engineering, ICAEEE 2024

作者： Apon, Imtiaz Ahamed Hasan, Md Ratul Haque, Md. Salman Department of Electrical and Electronic Engineering Saidpur5311 Bangladesh Department of Materials Science and Engineering Khulna9203 Bangladesh Department of Materials and Metallurgical Engineering Dhaka1000 Bangladesh

ISBN: (纸本)9798350388282

Very-large-scale integration (VLSI) of elliptic curve cryptography (ECC) is vital for efficiently securing the digital world. This research demonstrates a description of elliptic curve cryptography (ECC), with a focus on both hardware and software approaches. An effective technique is used to create a modified interleaved modular multiplication architecture that maximizes performance while minimizing hardware use. Almost 532 and 522 slice registers are available for Spartan-6 and others with 4 unique control sets each. ECC processors must carefully balance area, time, and frequency to achieve maximum efficiency, as these factors always involve limitations. In this study, a 256-bit encryption method is used with a modified algorithm for interleaved modular multiplication (IMM) in the prime field. This method requires more resources and time, but it still operates at a satisfactory speed. In addition, a new hardware circuit methodology is introduced and implemented utilizing the Xilinx ISE software on various FPGA platforms, such as Kintex-7, Virtex-5, Virtex-6, and Spartan-6. The proposed 256-bit modular multiplication design occupies only 1478, 1497, 1478 and 1483 look-up tables (LUTs) and attains noteworthy completion with 1.9 μ s, 2.09 μ s, 3.83 μ s, and 2.11 μ s on Kintex-7, Virtex-5, Spartan-6, and Virtex-6, respectively, at maximum frequencies of 134.7 MHz, 77.9 MHz, 67.097 MHz, and 121.527 MHz individually. Taking the National Institute of Standards suggested prime fields into consideration. Rigorous simulation and verification procedures are conducted employing Modelsim and Maple's software to ensure the accuracy and reliability of the obtained results. © 2024 IEEE.

关键词： VLSI circuits

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Dynamical phase-field model of cavity electromagnonic systems

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npj Computational materials 2024年第1期10卷 1263-1273页

作者： Shihao Zhuang Yujie Zhu Changchun Zhong Liang Jiang Xufeng Zhang Jia-Mian Hu Department of Materials Science and Engineering University of Wisconsin-MadisonMadisonWI53706USA Pritzker School of Molecular Engineering The University of ChicagoChicagoIL60637USA Department of Electrical and Computer Engineering Northeastern UniversityBostonMA02115USA Department of Physics Northeastern UniversityBostonMA02115USA

Cavity electromagnonic system,which simultaneously consists of cavities for photons,magnons(quanta of spin waves),and acoustic phonons,provides an exciting platform to achieve coherent energy transduction among different physical systems down to single quantum *** we report a dynamical phase-field model that allows simulating the coupled dynamics of the electromagnetic waves,magnetization,and strain in 3D multiphase *** examples of application,we computationally demonstrate the excitation of hybrid magnon-photon modes(magnon polaritons),Floquet-induced magnonic Aulter-Townes splitting,dynamical energy exchange(Rabi oscillation)and relative phase control(Ramsey interference)between the two magnon polariton *** simulation results are consistent with analytical calculations based on Floquet Hamiltonian *** are also performed to design a cavity electro-magno-mechanical system that enables the triple phononmagnon-photon resonance,where the resonant excitation of a chiral,fundamental(n=1)transverse acoustic phonon mode by magnon polaritons is *** the capability to predict coupling strength,dissipation rates,and temporal evolution of photon/magnon/phonon mode profiles using fundamental materials parameters as the inputs,the present dynamical phase-fieldmodel represents a valuable computational tool to guide the fabrication of the cavity electromagnonic system and the design of operating conditions for applications in quantum sensing,transduction,and communication.

关键词： theory phonon phase

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Electronic structure prediction of multimillion atom systems through uncertainty quantification enabled transfer learning

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npj Computational materials 2024年第1期10卷 1423-1437页

作者： Shashank Pathrudkar Ponkrshnan Thiagarajan Shivang Agarwal Amartya S.Banerjee Susanta Ghosh Department of Mechanical Engineering-Engineering Mechanics Michigan Technological UniversityHoughtonMIUSA Department of Electrical and Computer Engineering University of CaliforniaLos AngelesCA90095USA Department of Materials Science and Engineering University of CaliforniaLos AngelesCA90095USA Faculty member of the Center for Data Sciences Michigan Technological UniversityHoughtonMIUSA

The ground state electron density—obtainable using Kohn-Sham Density Functional Theory(KSDFT)simulations—contains a wealth of material information,making its prediction via machine learning(ML)models ***,the computational expense of KS-DFT scales cubically with system size which tends to stymie training data generation,making it difficult to develop quantifiably accurate ML models that are applicable across many scales and system ***,we address this fundamental challenge by employing transfer learning to leverage the multi-scale nature of the training data,while comprehensively sampling systemconfigurations using *** ML models are less reliant on heuristics,and being based on Bayesian neural networks,enable uncertainty *** show that our models incur significantly lower data generation costs while allowing confident—and when verifiable,accurate—predictions for a wide variety of bulk systems well beyond training,including systems with defects,different alloy compositions,and at multi-million-atom ***,such predictions can be carried out using only modest computational resources.

关键词： alloy prediction transfer

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ESG Investing: A Statistically Valid Approach to Data-Driven Decision Making and the Impact of ESG Factors on Stock Returns and Risk

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IEEE Access 2024年 12卷 69434-69444页

作者： Teja, Kamurthi Ravi Liu, Chuan-Ming National Taipei University of Technology International Program of Electrical Engineering and Computer Science Taipei10608 Taiwan National Taipei University of Technology Department of Computer Science and Information Engineering Taipei10608 Taiwan

This study examines the impact of environmental, social, and governance (ESG) factors on economic investment from a statistical perspective, aiming to develop a tested investment strategy that capitalizes on the connection between ESG factors and financial performance. ESG investing: A statistically valid approach to data-driven decision-making (ESGI-SVADDM) investment strategy is based on a rigorous, statistically valid approach that utilizes data, math, statistics, and data science libraries to drive investment decisions, eliminating the need for personal opinions and subjectivity. The process includes establishing an investment thesis, formulating testable hypotheses (HPS), retrieving and refining relevant data, calculating relevant measures, and testing and validating all hypotheses. The study uses S&P 500 stock data and ESG data from Sustainalytics to test the hypotheses. The empirical tests conducted revealed a negative correlation between ESG risk and expected returns, as well as a positive trend in the relationship between ESG risk and the overall risk of stocks. Moreover, the study found that higher ESG risk scores are associated with lower returns for investors, and that adopting a strategy of investing in stocks with low ESG risk and shorting stocks with high ESG risk yields superior returns compared to the market portfolio. © 2013 IEEE.

关键词： Investments

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TiO_(2)@C catalyzed hydrogen storage performance of Mg-Ni-Y alloy with LPSO and ternary eutectic structure

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Journal of Magnesium and Alloys 2024年第2期12卷 767-778页

作者： Wenjie Song Wenhao Ma Shuai He Wei Chen Jianghua Shen Dalin Sun Qiuming Wei Xuebin Yu College of Mechanical and Electrical Engineering Shaanxi University of Science and TechnologyXi’anShaanxi 710021China Department of Materials Science Fudan UniversityShanghai 200438China School of Aeronautics Northwestern Polytechnical UniversityXi’anShaanxi 710072China Department of Mechanical Engineering&Engineering Science the University of North Carolina at CharlotteCharlotteNorth Carolina 28223United States of America

A designed Mg_(88.7)Ni_(6.3)Y_(5)hydrogen storage alloy containing 14H type LPSO(long-period stacking ordered)and ternary eutectic structure was prepared by regulating the alloy composition and *** hydrogen storage performance of the alloy was improved by adding nano-flower-like TiO_(2)@C *** decomposition of the LPSO structure during hydrogenation led to the formation of plenty of nanocrystals which provided abundant interphase boundaries and activation *** nanoscale TiO_(2)@C catalyst was uniformly dispersed on the surface of alloy particles,and the"hydrogen overflow''effect of TiO_(2)@C accelerated the dissociation and diffusion of hydrogen on the surface of the alloy *** a result,the in-situ endogenous nanocrystals of the LPSO structure decomposition and the externally added flower-like TiO_(2)@C catalyst uniformly dispersed on the surface of the nanoparticles played a synergistic catalytic role in improving the hydrogen storage performance of the Mg-based *** the addition of the TiO_(2)@C catalyst,the beginning hydrogen desorption temperature was reduced to 200℃.Furthermore,the saturated hydrogen absorption capacity of the sample was 5.32 wt.%,and it reached 4.25 wt.%H_(2) in 1 min at 200℃and 30 bar.

关键词： Hydrogen storage Mg LPSO TiO_(2)@C Synergistic catalysis

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