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Chevrel phase: A review of its crystal structure and electrochemical properties

Progress in Natural science:materials International 2023年第1期33卷 8-15页

作者： Meng Liu Guocheng Lv Tianming Liu Hao Liu Lingchang Kong Lintao Tian Wenxiu Rao Yuxin Li Libing Liao Juchen Guo Engineering Research Center of Ministry of Education for Geological Carbon Storage and Low Carbon Utilization of Resources Beijing Key Laboratory of Materials Utilization of Nonmetallic Minerals and Solid Wastes National Laboratory of Mineral Materials School of Materials Science and Technology China University of Geosciences(Beijing) School of Science China University of Geosciences Materials Science and Engineering Program University of California-Riverside Department of Chemical and Environmental Engineering University of California – Riverside

Chevrel phase compounds have attracted increasing attention as electrochemical energy storage materials and electro-catalysts. Benefiting from their unique crystal structure, Chevrel phase compounds can not only function as the host structures for reversible intercalation of a broad range of cations, but also exhibit high catalytic activity in electrochemical reduction reactions. Here we provide an overview of recent progress in the development of Chevrel phase materials including new understanding of structural features, synthetic methods, and electrochemical properties. A brief conclusion and perspectives on the future development of Chevrel phase materials are also provided.

关键词： Chevrel phase Electrochemical properties Energy storage Electro-catalysis

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Enhancing the Performance of Perovskite Light-Emitting Diodes via Synergistic Effect of Defect Passivation and Dielectric Screening

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Nano-Micro Letters 2024年第10期16卷 244-256页

作者： Xuanchi Yu Jia Guo Yulin Mao Chengwei Shan Fengshou Tian Bingheng Meng Zhaojin Wang Tianqi Zhang Aung Ko Ko Kyaw Shuming Chen Xiaowei Sun Kai Wang Rui Chen Guichuan Xing Institute of Applied Physics and Materials Engineering University of MacaoAvenida da UniversidadeTaipaMacao 999078People's Republic of China Department of Electrical and Electronic Engineering Southern University of Science and TechnologyShenzhen 518055People's Republic of China

Metal halide perovskites,particularly the quasi-two-dimensional perovskite subclass,have exhibited considerable potential for next-generation electroluminescent materials for lighting and ***,the presence of defects within these perovskites has a substantial influence on the emission efficiency and durability of the *** this study,we revealed a synergistic passivation mechanism on perovskite films by using a dual-functional compound of potassium *** dual functional potassium bromide on the one hand can passivate the defects of halide vacancies with bromine anions and,on the other hand,can screen the charged defects at the grain boundaries with potassium *** approach effectively reduces the probability of carriers quenching resulting from charged defects capture and consequently enhances the radiative recombination efficiency of perovskite thin films,leading to a significant enhancement of photoluminescence quantum yield to near-unity values(95%).Meanwhile,the potassium bromide treatment promoted the growth of homogeneous and smooth film,facilitating the charge carrier injection in the ***,the perovskite light-emitting diodes based on this strategy achieve a maximum external quantum efficiency of~21%and maximum luminance of~60,000 cd m^(-2).This work provides a deeper insight into the passivation mechanism of ionic compound additives in perovskite with the solution method.

关键词： Synergistic passivation strategy Defects passivation Dielectric screening Perovskite light-emitting diodes

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Realization of a quadrupole topological insulator phase in a gyromagnetic photonic crystal

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National science Review 2024年第11期11卷 47-53页

作者： Peiheng Zhou Gui-Geng Liu Zihao Wang Shuwei Li Qindong Xie Yunpeng Zhang Subhaskar Mandal Xiang Xi Zhen Gao Longjiang Deng Baile Zhang National Engineering Research Center of Electromagnetic Radiation Control Materials Key Laboratory of Multi-spectral Absorbing Materials and Structures of Ministry of EducationUniversity of Electronic Science and Technology of China Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University School of Electrical Engineering and Intelligentization Dongguan University of Technology Department of Electronic and Electrical Engineering Southern University of Science and Technology Centre for Disruptive Photonic Technologies The Photonics InstituteNanyang Technological University

The field of topological photonics was initiated with the realization of a Chern insulator phase in a gyromagnetic photonic crystal(Ph C) with broken time-reversal symmetry(T), hosting chiral edge states that are topologically protected propagating modes. Along a separate line of research, a quadrupole topological insulator was the first higher-order topological phase supporting localized corner states, but has been so far limited to T-invariant systems, as T is a key ingredient in early models. Here we report the realization of a quadrupole topological insulator phase in a gyromagnetic Ph C, as a consequence of topological phase transition from the previously demonstrated Chern insulator phase. The phase transition has been demonstrated with microwave measurements, which characterize the evolution from propagating chiral edge states to localized corner states. We also demonstrate the migration of topological boundary states into the continuum, when the gyromagnetic Ph C is magnetically tuned. These results extend the quadrupole topological insulator phase into T-broken systems, and integrate topologically protected propagating and localized modes in a magnetically tunable photonic crystal platform.

关键词： quadrupole topological insulator time-reversal symmetry breaking corner states topological phase transition

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Correntropy-Based Data Selective Adaptive Filtering

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IEEE Transactions on Circuits and Systems I: Regular Papers 2024年第2期71卷 754-766页

作者： Chien, Ying-Ren Wu, Sheng-Teng Tsao, Hen-Wai Diniz, Paulo S.R. Adaptive and Autonomous Communication Laboratory Department of Electrical Engineering National Ilan University Yilan City260007 Taiwan College of Electrical Engineering and Computer Science Graduate Institute of Communication Engineering National Taiwan University Taipei10617 Taiwan Program of Electrical Engineering Department of Electronics and Computer Engineering COPPE/Poli Universidade Federal do Rio de Janeiro Rio de Janeiro68504 Brazil

Data selection can be used in conjunction with adaptive filtering algorithms to avoid unnecessary weight updating and thereby reduce computational overhead. This paper presents a novel correntropy-based data selection method as an alternative to conventional data selection mechanisms based on squared error values. We developed a variable correntropy sensing algorithm to maximize the instantaneous correntropy function for the Gaussian kernel function to mitigate the impact of impulse noise and other forms of noise that can be disregarded in data selection. The proposed data selection mechanism can be implemented with any adaptive filtering algorithm. In simulations, the proposed method (implemented with the least mean squared algorithm) outperformed comparable error-based data selection schemes in terms of hit rate and miss rate, and the resulting weight updating ratio was close to the expected weight updating ratio. © 2023 IEEE. Personal use is permitted, but republication/redistribution requires IEEE permission.

关键词： Adaptive filters

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Efficient and stable hybrid perovskite-organic light-emitting diodes with external quantum efficiency exceeding 40 per cent

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Light(science & Applications) 2024年第7期13卷 1364-1371页

作者： Lingmei Kong Yun Luo Qianqian Wu Xiangtian Xiao Yuanzhi Wang Guo Chen Jianhua Zhang Kai Wang Wallace CHChoy Yong-Biao Zhao Hongbo Li Takayuki Chiba Junji Kido Xuyong Yang Key Laboratory of Advanced Display and System Applications of Ministry of Education Shanghai UniversityShanghai 200072China. Institute of Nanoscience and Applications Department of Electrical and Electronic EngineeringSouthern University of Science and TechnologyShenzhen 518055China. Department of Electrical and Electronic Engineering The University of Hong KongHong KongChina. Department of Physics and Lakeside AR/VR Laboratory International Joint Research Center for Optoelectronic and Engineering ResearchYunnan UniversityKunming 650091China. Experimental Center of Advanced Materials School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China. Graduate School of Organic Materials Science Frontier Center for Organic MaterialsYamagata University4-3-16 JonanYonezawa 992–8510Japan

Light-emitting diodes(LEDs)based on perovskite semiconductor materials with tunable emission wavelength in visible light range as well as narrow linewidth are potential competitors among current light-emitting display technologies,but still suffer from severe instability driven by electric ***,we develop a stable,efficient and highcolor purity hybrid LED with a tandem structure by combining the perovskite LED and the commercial organic LED technologies to accelerate the practical application of *** LED and organic LED with close photoluminescence peak are selected to maximize photon emission without photon reabsorption and to achieve the narrowed emission *** designing an efficient interconnecting layer with p-type interface doping that provides good opto-electric coupling and reduces Joule heating,the resulting green emitting hybrid LED shows a narrow linewidth of around 30 nm,a peak luminance of over 176,000 cd m^(−2),a maximum external quantum efficiency of over 40%,and an operational half-lifetime of over 42,000 h.

关键词： diodes narrow quantum

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A ShuffleNet Architecture-Based Multi-Layer Feature Scaling and Fusion Approach for Underwater Net Cage Damage Detection in Aquaculture

A ShuffleNet Architecture-Based Multi-Layer Feature Scaling ...

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2024 IEEE International Conference on Consumer Electronics-Asia, ICCE-Asia 2024

作者： Huang, Xiang-Rui Chen, Yi-Cheng Chen, Liang-Bi Hu, Wu-Chih National Penghu University of Science and Technology Master Program in Electrical Engineering and Computer Science Department of Electrical Engineering Penghu Taiwan National Penghu University of Science and Technology Department of Computer Science and Information Engineering Penghu Taiwan

ISBN: (纸本)9798331530839

In offshore aquaculture operations, personnel equipped with diving gear are often necessary to inspect the underwater net cages for damage, particularly on the sea floor. This manual inspection process is time-consuming and complex. To overcome this problem, this paper proposes a computer vision solution for identifying damage in underwater net cages to address the inefficiencies and challenges of traditional manual inspections. The proposed scheme utilizes a high-performance multi-branch computational architecture designed based on ShuffleNet architecture to detect net cage damage more efficiently. Experimental results demonstrate that this work performs well on the ImageNet ILSVRC-2010 dataset and achieves an accuracy of 88.54% in underwater net damage detection. © 2024 IEEE.

关键词： Aquaculture

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Modeling the effects of salt concentration on aqueous and organic electrolytes

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npj Computational materials 2023年第1期9卷 546-552页

作者： Stephanie C.C.van der Lubbe Pieremanuele Canepa Department of Materials Science and Engineering National University of Singapore9 Engineering Drive 1117575 SingaporeSingapore Department of Chemical and Biomolecular Engineering National University of Singapore4 Engineering Drive 4117585 SingaporeSingapore Department of Electrical and Computer Engineering and Texas Center for Superconductivity University of HoustonHoustonTX 77204USA

Understanding the thermodynamic properties of electrolyte solutions is of vital importance for a myriad of physiological and technological *** mean activity coefficientγ±is associated with the deviation of an electrolyte solution from its ideal behavior and may be obtained by combining the Debye-Hückel(DH)and Born(B)***,the DH and B equations depend on the concentration and temperature-dependent static permittivity of the solutionεr(c,T)and the size of the solvated ions ri,whose experimental data is often not ***,we use a combination of molecular dynamics and density functional theory to predictεr(c,T)and ri,which enables us to apply the DH and B equations to any technologically relevant aqueous and nonaqueous electrolyte at any concentration and temperature of interest.

关键词： equations electrolyte apply

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Phase-Field Model of Electronic Antidoping

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Physical Review Letters 2024年第25期132卷 256502-256502页

作者： Yin Shi Guo-Dong Zhao Ismaila Dabo Shriram Ramanathan Long-Qing Chen Department of Materials Science and Engineering Department of Electrical and Computer Engineering

Charge carrier doping usually reduces the resistance of a semiconductor or insulator, but was recently found to dramatically enhance the resistance in certain series of materials. This remarkable antidoping effect has been leveraged to realize synaptic memory trees in nanoscale hydrogenated perovskite nickelates, opening a new direction for neuromorphic computing. To understand these phenomena, we formulate a physical phase-field model of the antidoping effect based on its microscopic mechanism and simulate the voltage-driven resistance change in the prototypical system of hydrogenated perovskite nickelates. Remarkably, the simulations using this model, containing only one adjustable parameter whose magnitude is justified by first-principles calculations, quantitatively reproduce the experimentally observed treelike resistance states, which are shown unambiguously to arise from proton redistribution-induced local band gap enhancement and carrier blockage. Our work lays the foundation for modeling the antidoping phenomenon in strongly correlated materials at the mesoscale, which can provide guidance to the design of novel antidoping-physics-based devices.

关键词： Doping effects Neural basis of learning & memory Strongly correlated systems Phase-field modeling

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Annealing effect on structural, morphological, optical, and electrical properties of spin coated ZnS thin films for photovoltaic application

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Optical and Quantum Electronics 2025年第1期57卷 1-25页

作者： Ali, Md. Hasan Hossain, Md. Faruk Hossain, Md. Mahabub Haque, Md. Dulal Islam, Abu Zafor Md. Touhidul Department of Electronics and Communication Engineering Hajee Mohammad Danesh Science and Technology University Dinajpur5200 Bangladesh Advanced Energy Materials and Solar Cell Research Laboratory Department of Electrical and Electronic Engineering Begum Rokeya University Rangpur Rangpur5400 Bangladesh Department of Electrical and Electronic Engineering Rajshahi University of Engineering and Technology Rajshahi6204 Bangladesh Department of Electrical and Electronic Engineering University of Rajshahi Rajshahi6205 Bangladesh

The conventional cadmium sulfide (CdS) window/buffer layer in photovoltaic cells is environmentally hazardous because of the poisoning of cadmium (Cd). Alternatively, ZnS is more environmentally friendly than CdS and has a larger band gap, which makes it a potential candidate for window/buffer layers. In this study, ZnS thin films were deposited on glass substrates by a spin coating process and annealed at three (250 °C, 350 °C, and 450 °C) different temperatures. The XRD patterns confirmed that all the spin coated films had mixed wurtzite and cubic structures with a preferred orientation along the (111) plane of the predominant cubic phase. The highest crystallite size and lowest dislocation density were found at 350 °C annealing temperature due to the narrow, sharp and high intensity diffraction peak compared with those at 250 °C and 450 °C annealing temperatures. The SEM results indicate that the surface of the ZnS film annealed at 350 °C has a better surface coverage area with good uniformity, and is more homogeneous with a minimum amount of pinholes, voids and cracks than the other samples annealed at 250 °C, and 450 °C. The estimated optical band gap was determined to be between 3.957 and 3.991 eV. The calculated electrical resistivity values are on the order of 104 Ω cm. All the findings revealed that the film annealed at 350 °C presented good material properties for utilizing as buffer layer in thin film solar cells. © The Author(s), under exclusive licence to Springer science+Business Media, LLC, part of Springer Nature 2024.

关键词： Crystallite size

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Simultaneous improving luminescence intensity and stability of CsPbBr_(3):SCN−@Eu/Zr-Uio-66-NH_(2) with tunable emissions from blue to green and applications in indoor photovoltaics

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Nano Research 2024年第8期17卷 6879-6887页

作者： Minze Li Yao Sun Honglai Lu Peifen Zhu Ruihong Wang Guofeng Wang Key Laboratory of Functional Inorganic Material Chemistry Ministry of EducationSchool of Chemistry and Materials ScienceHeilongjiang UniversityHarbin 150080China Department of Electrical Engineering and Computer Science University of MissouriColumbiaMO 65211USA

The construction of stable and efficient materials that emit blue and green light remains a *** the blue light materials reported,metal-organic framework(MOF)materials are rarely reported as blue phosphors due to their weak luminescence *** on the construction of CsPbBr_(3)@MOF(CPB@MOF),an innovative idea was proposed to simultaneously enhance the green luminescence of CPB and the blue luminescence of MOF through the interaction between CPB and MOF for the first *** expected,the blue luminescence from CPB:7%SCN−@0.5%MOF:Eu as well as the green luminescence from 5%CPB:7%SCN−@MOF:Eu was sufficient to construct high-performance light-emitting diode(LED)devices and further excite solar cells to generate stable photoelectric *** white LED(WLED)device with excellent color quality(color rendering index(CRI)=96.2)and correlated color temperature(CCT=9688 K)can be constructed by using the obtained blue-emitting CPB:7%SCN-@0.5%MOF:Eu,green-emitting 5%CPB:7%SCN−@MOF:Eu,and red-emitting PPB:30%Mn^(2+).The density functional theory(DFT)theoretical calculation results indicate that the p orbital of Pb plays the major role in the conduction band,and the p orbital of Br plays the major role in the valance band of CPB and CPB:SCN−.While the p orbital of O plays the major role in both the conduction band and valance band of *** heat capacity of CPB and CPB:SCN−separately reaches the Dulong–Petit limit at 200 and 400 K,indicating that the thermal stability of CsPbBr_(3)increases after SCN−doping.

关键词： CsPbBr_(3):SCN−@Uio-66-NH_(2) composites luminescence stability white light-emitting diodes(WLEDs) indoor photovoltaics density functional theory(DFT)calculation

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