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Sequential crystallization during the formation of bulk heterojunction in organic solar cells

science China materials 2025年第5期68卷 1686-1688页

作者： Xiaoxiao Jia Qifeng Zhang Guozhong Cao Department of Materials Science and Engineering University of Washington Department of Electrical and Computer Engineering North Dakota State University

A silicon solar cell with a power conversion efficiency (PCE)of 4% was born in Bell Lab in 1954, seven decades ago. Today,silicon solar cells have reached an efficiency above 25%and achieved pervasive commercial success [1]. In spite of the steady improvement in efficiency, the interest and enthusiasm in search for new materials and innovative device architectures for newgeneration solar cells have never diminished or subsided;

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From light sensing to adaptive learning:hafnium diselenide reconfigurable memcapacitive devices in neuromorphic computing

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Light(science & Applications) 2025年第1期14卷 215-226页

作者： Bashayr Alqahtani Hanrui Li Abdul Momin Syed Nazek El-Atab Electrical and Computer Engineering Program Computer Electrical Mathematical Science and Engineering DivisionKing Abdullah University of Science and Technology(KAUST)ThuwalSaudi Arabia Electrical Engineering Department College of EngineeringPrincess Nourah Bint Abdulrahman University(PNU)RiyadhSaudi Arabia

Advancements in neuromorphic computing have given an impetus to the development of systems with adaptive behavior,dynamic responses,and energy efficiency *** charge-based or emerging memory technologies such as memristors have been developed to emulate synaptic plasticity,replicating the key functionality of neurons—integrating diverse presynaptic inputs to fire electrical impulses—has remained *** this study,we developed reconfigurable metal-oxide-semiconductor capacitors(MOSCaps)based on hafnium diselenide(HfSe2).The proposed devices exhibit(1)optoelectronic synaptic features and perform separate stimulus-associated learning,indicating considerable adaptive neuron emulation,(2)dual light-enabled charge-trapping and memcapacitive behavior within the same MOSCap device,whose threshold voltage and capacitance vary based on the light intensity across the visible spectrum,(3)memcapacitor volatility tuning based on the biasing conditions,enabling the transition from volatile light sensing to non-volatile optical data *** reconfigurability and multifunctionality of MOSCap were used to integrate the device into a leaky integrate-and-fire neuron model within a spiking neural network to dynamically adjust firing patterns based on light stimuli and detect exoplanets through variations in light intensity.

关键词： integrate volatile integrating

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Wide field of view large aperture meta-doublet eyepiece

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Light(science & Applications) 2025年第1期14卷 167-176页

作者： Anna Wirth-Singh Johannes E.Fröch Fan Yang Louis Martin Hanyu Zheng Hualiang Zhang Quentin T.Tanguy Zhihao Zhou Luocheng Huang Demis DJohn Biljana Stamenic Juejun Hu Tian Gu Arka Majumdar Department of Physics University of WashingtonSeattleWAUSA Department of Electrical and Computer Engineering University of WashingtonSeattleWAUSA Department of Materials Science and Engineering Massachusetts Institute of TechnologyCambridgeMAUSA Department of Electrical and Computer Engineering University of MassachusettsLowellMAUSA Department of Electrical and Computer Engineering University of CaliforniaSanta BarbaraCAUSA

Wide field of view and light weight optics are critical for advanced eyewear,with applications in augmented/virtual reality and night *** refractive lenses are often stacked to correct aberrations at a wide field of view,leading to limited performance and increased size and *** particular,simultaneously achieving a wide field of view and large aperture for light collection is desirable but challenging to realize in a compact ***,we demonstrate a wide field of view(greater than 60°)meta-optic doublet eyepiece with an entrance aperture of 2.1 *** the design wavelength of 633 nm,the meta-optic doublet achieves comparable performance to a refractive lens-based eyepiece *** meta-doublet eyepiece illustrates the potential for meta-optics to play an important role in the development of high-quality monochrome near-eye displays and night vision systems.

关键词： optics refractive illustrate

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Polarization-encodable photonic memory cells using nextgeneration 2D phase-change materials

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Nano Research 2025年第3期18卷 510-518页

作者： Amin Shafiee Linhong Chen Mahdi Nikdast Jie Yao Department of Electrical and Computer Engineering Colorado State UniversityFort CollinsCO 80523USA Department of Materials Science and Engineering University of CaliforniaBerkeleyCA 94720USA

Integration of phase-change materials(PCMs)created a unique opportunity to implement reconfigurable photonics devices that their performance can be tuned depending on the target *** PCMs such as Ge-Sb-Te(GST)and Ge-Sb-Se-Te(GSST)rely on melt-quench and high temperature annealing processes to change the organization of the molecules in the materials’*** a reorganization leads to different optical,electrical,and thermal properties which can be exploited to implement photonic memory cells that are able to store the data at different resistance or optical transmission *** the great promise of conventional PCMs for realizing reconfigurable photonic memories,their slow and extremely power-hungry thermal mechanisms make scaling the systems based on such devices *** addition,such materials do not offer a stable multi-level response over a long period of *** address these shortcomings,the research carried out in this study shows the proof of concept to implement next-generation photonic memory cells based on two-dimensional(2D)birefringence PCMs such as SnSe,which offer anisotropic optical properties that can be switched *** demonstrate that by leveraging the ultrafast and low-power crystallographic direction change of the material,the optical polarization state of the input optical signal can be *** enables the implementation of next-generation high-speed polarization-encodable photonic memory cells for future photonic computing *** to the conventional PCMs,the proposed SnSe-based photonic memory cells offer an ultrafast switching and low-loss optical response relying on ferroelectric property of SnSe to encode the data on the polarization state of the input optical *** a polarization encoding scheme also reduces memory read-out errors and alleviates the scalability limitations due to the optical insertion loss often seen in optical transmission encoding.

关键词： ferroelectric materials phase-change materials photonic memory optical storage cells polarization encodable photonic memories optical polarization

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Recent advances in tip-enhanced Raman spectroscopy probe designs

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Nano Research 2023年第4期16卷 5555-5571页

作者： Da Xu Boqun Liang Yaodong Xu Ming Liu Department of Electrical and Computer Engineering University of California-RiversideRiversideCalifornia 92521USA Materials Science and Engineering program University of California-RiversideRiversideCalifornia 92521USA

Tip-enhanced Raman spectroscopy(TERS)imaging is a super-resolution imaging technique that features the merits of both surface-enhanced Raman spectroscopy(SERS)and scanning probe microscopy(SPM),such as the high chemical sensitivity from the former and the nanoscale spatial resolution from the *** advantages make TERS an essential nanospectroscopic characterization technique for chemical analysis,materials science,bio-sensing,*** probes,the most critical factor determining the TERS imaging quality,are expected to provide a highly confined electromagnetic hotspot with a minimized scattering background for the generation of Raman signals with high spatial *** two decades of development,numerous probe design concepts have been proposed and *** review provides a comprehensive overview of the state-of-the-art TERS probe designs,from the working mechanism to the practical *** start with reviewing the recent development of TERS configurations and the corresponding working mechanisms,including the SPM platforms,optical excitation/collection techniques,and probe preparation *** then review the emerging novel TERS probe designs,including the remote-excitation probes,the waveguide-based nanofocusing probes,the metal-coated nanofocusing probes,the nanowire-assisted selective-coupling probes,and the tapered metal-insulator-metal *** discussion focuses on a few critical aspects,including the surface-plasmon-polariton(SPP)hotspot excitation technique,conversion efficiency,working frequency,and *** the end,we review the latest TERS applications and give a perspective on the future of TERS.

关键词： tip-enhanced Raman spectroscopy plasmonics scanning probe microscopy nanoscale imaging nanophotonics nanofocusing

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Surface phase diagram of CsSnI3 from first-principles calculations

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Physical Review materials 2024年第9期8卷 093401页

作者： Kejia Li Chadawan Khamdang Mengen Wang Department of Electrical and Computer Engineering Materials Science and Engineering Program

CsSnI3 is widely studied as an environmentally friendly Pb-free perovskite material for optoelectronic device applications. To further improve material and device performance, it is important to understand the surface structures of CsSnI3. We generate surface structures with various stoichiometries, perform density functional theory calculations to create phase diagrams of the CsSnI3 (001), (110), and (100) surfaces, and determine the most stable surfaces under a wide range of Cs, Sn, and I chemical potentials. Under I-rich conditions, surfaces with Cs vacancies are stable, which lead to partially occupied surface states above the valence band maximum. Under I-poor conditions, we find the stoichiometric (100) surface to be stable under a wide region of the phase diagram, which does not have any surface states and can contribute to long charge-carrier lifetimes. Consequently, the I-poor (Sn-rich) conditions will be more beneficial to improve the device performance.

关键词： Electronic structure Surface reconstruction Surface states Perovskites Semiconductors Density functional theory

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Artificial visual perception neural system using a solution-processable MoS_(2)-based in-memory light sensor

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Light(science & Applications) 2023年第8期12卷 1583-1594页

作者： Dayanand Kumar Lana Joharji Hanrui Li Ayman Rezk Ammar Nayfeh Nazek El-Atab Smart Advanced Memory Devices and Applications(SAMA)LaboratoryElectrical and Computer Engineering ProgramComputer Electrical Mathematical Science and Engineering DivisionKing Abdullah University of Science and Technology(KAUST)Thuwal 23955Kingdom of Saudi Arabia Department of Electrical Engineering and Computer Science Khalifa UniversityAbu Dhabi 127788United Arab Emirates

Optoelectronic devices are advantageous in in-memory light sensing for visual information processing,recognition,and storage in an energy-efficient ***,in-memory light sensors have been proposed to improve the energy,area,and time efficiencies of neuromorphic computing *** study is primarily focused on the development of a single sensing-storage-processing node based on a two-terminal solution-processable MoS2 metal-oxide-semiconductor(MOS)charge-trapping memory structure—the basic structure for charge-coupled devices(CCD)—and showing its suitability for in-memory light sensing and artificial visual *** memory window of the device increased from 2.8 V to more than 6V when the device was irradiated with optical lights of different wavelengths during the program ***,the charge retention capability of the device at a high temperature(100 ℃)was enhanced from 36 to 64%when exposed to a light wavelength of 400 *** larger shift in the threshold voltage with an increasing operating voltage confirmed that more charges were trapped at the Al_(2)O_(3)/MoS_(2) interface and in the MoS_(2) layer.A small convolutional neural network was proposed to measure the optical sensing and electrical programming abilities of the *** array simulation received optical images transmitted using a blue light wavelength and performed inference computation to process and recognize the images with 91%*** study is a significant step toward the development of optoelectronic MOS memory devices for neuromorphic visual perception,adaptive parallel processing networks for in-memory light sensing,and smart CCD cameras with artificial visual perception capabilities.

关键词： visual neural process

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Superior efficiency and stability of YbO_(x)-enhanced perovskite solar cells

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science China materials 2024年第4期67卷 1356-1358页

作者： Qifeng Zhang Guozhong Cao Department of Electrical and Computer Engineering North Dakota State UniversityFargoND 58108-6050USA Department of Materials Science and Engineering University of WashingtonSeattleWA 98195-2120USA

Perovskite solar cells represent a revolutionary class of photovoltaic devices that have gained substantial attention for their exceptional performance and potential to provide an affordable and efficient solution for harnessing solar energy. These cells utilize perovskite-structured materials, typically hybrid organicinorganic lead halide compounds, as the light-absorbing layer.

关键词： energy perovskite stability

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ESG Investing: A Statistically Valid Approach to Data-Driven Decision Making and the Impact of ESG Factors on Stock Returns and Risk

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IEEE Access 2024年 12卷 69434-69444页

作者： Teja, Kamurthi Ravi Liu, Chuan-Ming National Taipei University of Technology International Program of Electrical Engineering and Computer Science Taipei10608 Taiwan National Taipei University of Technology Department of Computer Science and Information Engineering Taipei10608 Taiwan

This study examines the impact of environmental, social, and governance (ESG) factors on economic investment from a statistical perspective, aiming to develop a tested investment strategy that capitalizes on the connection between ESG factors and financial performance. ESG investing: A statistically valid approach to data-driven decision-making (ESGI-SVADDM) investment strategy is based on a rigorous, statistically valid approach that utilizes data, math, statistics, and data science libraries to drive investment decisions, eliminating the need for personal opinions and subjectivity. The process includes establishing an investment thesis, formulating testable hypotheses (HPS), retrieving and refining relevant data, calculating relevant measures, and testing and validating all hypotheses. The study uses S&P 500 stock data and ESG data from Sustainalytics to test the hypotheses. The empirical tests conducted revealed a negative correlation between ESG risk and expected returns, as well as a positive trend in the relationship between ESG risk and the overall risk of stocks. Moreover, the study found that higher ESG risk scores are associated with lower returns for investors, and that adopting a strategy of investing in stocks with low ESG risk and shorting stocks with high ESG risk yields superior returns compared to the market portfolio. © 2013 IEEE.

关键词： Investments

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Thermoelectric infrared detectors:Design,fabrication,and performance assessment

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Journal of Semiconductors 2024年第12期45卷 95-110页

作者： Daryoosh Vashaee Department of Electrical and Computer Engineering North Carolina State UniversityRaleighNC 27606USA Department of Materials Science and Engineering North Carolina State UniversityRaleighNC 27606USA

This study presents a comprehensive optimization and comparative analysis of thermoelectric(TE)infrared(IR)detec-tors using Bi_(2)Te_(3) and Si *** theoretical modeling and numerical simulations,we explored the impact of TE mate-rial properties,device structure,and operating conditions on responsivity,detectivity,noise equivalent temperature difference(NETD),and noise equivalent power(NEP).Our study offers an optimally designed IR detector with responsivity and detectivity approaching 2×10^(5) V/W and 6×10^(9) cm∙Hz^(1/2)/W,*** enhancement is attributed to unique design features,includ-ing raised thermal collectors and long suspended thin thermoelectric wire sensing elements embedded in low thermal conductivity organic materials like ***,we demonstrate the compatibility of Bi_(2)Te_(3)-based detector fabrication pro-cesses with existing MEMS foundry processes,facilitating scalability and ***,for TE IR detectors,zT/κemerges as a critical parameter contrary to conventional TE material selection based solely on zT(where zT is the thermoelec-tric figure of merit andκis the thermal conductivity).

关键词： thermoelectric infrared focal plane arrays micromachining Bi_(2)Te_(3)

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