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Patterned graphene oxide via one-step thermal annealing for controlling collective cell migration

Journal of materials Chemistry B 2024年第35期12卷 8733-8745页

作者： Huang, Chien-Yu Chen, Chong-You Wei, Chia-Hung Yang, Jia-Wei Lin, Yu-Chien Kao, Chih-Fei Chung, Johnson H. Y. Chen, Guan-Yu Institute of Biomedical Engineering College of Electrical and Computer Engineering National Yang Ming Chiao Tung University Hsinchu300093 Taiwan Department of Electrical and Computer Engineering College of Electrical and Computer Engineering National Yang Ming Chiao Tung University Hsinchu300093 Taiwan Department of Biological Science and Technology College of Biological Science and Technology National Yang Ming Chiao Tung University Hsinchu300093 Taiwan Intelligent Polymer Research Institute Institute for Innovative Materials University of Wollongong NSW2500 Australia National Yang Ming Chiao Tung University Hsinchu300093 Taiwan

Graphene oxide (GO) is a two-dimensional metastable nanomaterial. Interestingly, GO formed oxygen clusterings in addition to oxidized and graphitic phases during the low-temperature thermal annealing process, which could be further used for biomolecule bonding. By harnessing this property of GO, we created a bio-interface with patterned structures with a common laboratory hot plate that could tune cellular behavior by physical contact. Due to the regional distribution of oxygen clustering at the interface, we refer to it as patterned annealed graphene oxide (paGO). In addition, since the paGO was a heterogeneous interface and bonded biomolecules to varying degrees, arginine-glycine-aspartic acid (RGD) was modified on it and successfully regulated cellular-directed growth and migration. Finally, we investigated the FRET phenomenon of this heterogeneous interface and found that it has potential as a biosensor. The paGO interface has the advantages of easy regulation and fabrication, and the one-step thermal reduction method is suitable for biological applications. We believe that this low-temperature thermal annealing method would make GO interfaces more accessible, especially for the development of nano-interfacial modifications for biological applications, revealing its potential for biomedical applications. © 2024 The Royal Society of Chemistry.

关键词： Biomolecules

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La-substituted W-type barium-nickel ferrites for tunable and high-performance electromagnetic wave absorption

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International Journal of Minerals,Metallurgy and materials 2025年第3期32卷 645-656页

作者： Long Wang Jiurong Liu Shenghui Xie Yanli Deng Zhou Wang Shanyue Hou Shengying Yue Gang Wang Na Wu Zhihui Zeng Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials(Ministry of Education) School of Materials Science and EngineeringShandong UniversityJinan 250061China Electronic Materials Research Laboratory Key Laboratory of the Ministry of Education and International Center for Dielectric ResearchSchool of Electronic Science and EngineeringXi’an Jiaotong UniversityXi’an 710049China Army Engineering University of PLA College of Field Engineering Nanjing 210007China Laboratory for Multiscale Mechanics and Medical Science State Key Laboratory for Strength and Vibration of Mechanical StructuresSchool of AerospaceXi’an Jiaotong UniversityXi’an 710049China Department of Electrical and Computer Engineering Beckman Institute for Advanced Science and TechnologyUniversity of Illinois at Urbana-ChampaignUrbana 61801USA School of Chemistry and Chemical Engineering Shandong UniversityJinan 250100China

W-type barium-nickel ferrite(BaNi_(2)Fe_(16)O_(27))is a highly promising material for electromagnetic wave(EMW)absorption be-cause of its magnetic loss capability for EMW,low cost,large-scale production potential,high-temperature resistance,and excellent chemical ***,the poor dielectric loss of magnetic ferrites hampers their utilization,hindering enhancement in their EMW-absorption *** efficient strategies that improve the EMW-absorption performance of ferrite is highly desired but re-mains ***,an efficient strategy substituting Ba^(2+)with rare earth La^(3+)in W-type ferrite was proposed for the preparation of novel La-substituted ferrites(Ba_(1-x)LaxNi_(2)Fe_(15.4)O_(27)).The influences of La^(3+)substitution on ferrites’EMW-absorption performance and the dissipative mechanism toward EMW were systematically explored and ***^(3+)efficiently induced lattice defects,enhanced defect-induced polarization,and slightly reduced the ferrites’bandgap,enhancing the dielectric properties of the ***^(3+)also enhanced the ferromagnetic resonance loss and strengthened magnetic *** effects considerably improved the EMW-absorption perform-ance of Ba_(1-x)LaxNi_(2)Fe_(15.4)O_(27)compared with pure W-type *** x=0.2,the best EMW-absorption performance was achieved with a minimum reflection loss of-55.6 dB and effective absorption bandwidth(EAB)of 3.44 GHz.

关键词： electromagnetic wave absorption W-type barium ferrite rare earth dielectric

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Computational investigation of the structural and electrolyte properties of the extended family of lithium (thio)boracite materials: Li4B7O12Cl and beyond

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Physical Review materials 2024年第6期8卷 065401-065401页

作者： D. Cory Lynch Yan Li Pieremanuele Canepa N. A. W. Holzwarth Department of Physics Department of Materials Science and Engineering Department of Electrical and Computer Engineering Texas Center for Superconductivity at the

Motivated by previous investigations that showed very promising high ionic conductivities within relatively stable framework structures, we report a systematic first-principles study of the extended family of lithium (thio)boracites, consisting of eight chemical compositions. Three of the compositions—Li4B7O12Cl, Li4Al3B4O12Cl, and Li6B7S13Cl—are comparable to synthesized and analyzed materials reported in the experimental literature. The five additional compositions—Li4B7S12Cl, Li4Al3B4S12Cl, Li6B7O13Cl, Li6Al3B4O13Cl, and Li6Al3B4S13Cl—are predicted from the computational modeling and analysis presented in this paper. For each material, idealized ordered rhombohedral, cubic, or monoclinic ground-state structures are determined. Through various methodologies including thermodynamic, voltage window, and harmonic phonon analyses, stability is assessed for all eight Li (thio)boracite-derived compositions. Based on the dominant energetics of density functional theory, an analysis of the thermodynamically accessible phases predicts stability for Li4B7O12Cl only. The analysis of the voltage windows of these materials suggests that the sulfur materials are much more reactive in contact with lithium metal than their oxygen counterparts. This reactivity problem has been identified in other highly conducting solid electrolytes and various mitigation methods discussed in the literature look promising. Within the harmonic approximation, phonon analysis predicts that all eight materials are dynamically stable in their ground-state structures. Future investigations will focus on the performance of the family of lithium (thio)boracites, including ionic conductivity predictions and ion migration mechanisms.

关键词： Batteries First-principles calculations Ionic transport Structural properties

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Squid-inspired and wirelessly controllable display for active camouflage in aquatic-environment

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npj Flexible Electronics 2024年第1期8卷 900-909页

作者： Doyoung Kim Seung Won Seon Minkyung Shin Jihwan Kim Bogeun Kim Janghoon Joo Sang Uk Park Wooseok Kim Hee Kyu Lee Byeong Woon Lee Se Gi Lee Su Eon Lee Ji-Hun Seo Seung Ho Han Bong Hoon Kim Sang Min Won Department of Electrical and Computer Engineering Sungkyunkwan University2066Seobu-roJangan-guSuwon 16419Republic of Korea Department of Smart Wearable Engineering Soongsil UniversitySeoul 06978Republic of Korea Electronic Convergence Materials and Devices Research Center Korea Electronics Technology Institute(KETI)Seongnam 13509Republic of Korea Department of Materials Science and Engineering Korea UniversitySeoul 02841Republic of Korea Department of Robotics and Mechatronics Engineering DGISTDaegu 42988Republic of Korea

Achieving optimal camouflage in an aquatic environment necessitates the ability to modulate transmittance in response to the surrounding obscurity and potential *** adaptation involves a dynamic transition from transparency to a deep-blue color,especially in low-light or dark *** a strategy promotes a seamless assimilation with the surroundings,enabling the absorption of searchlights and,subsequently,diminishing the risk of detection by ***,the presence of sophisticated mechanisms that facilitates stable and efficient control of transmittance is imperative,enabling smooth transition between transparent and deep-blue hues within the aquatic *** study presents nature-inspired programmable camouflage system that integrates an electrochromic display as the primary transmittance change element and a wireless base module for power and data *** technology offers a robust and flexible construction,ensuring stable operation as demonstrated through mechanical-fatigue experiments and quantitative simulation.A custom circuit and a power-control software package enable active control of multiple electrochromic displays while submerged in water.

关键词： transparency submerged lights

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Boost DC-DC Converter with Non-dissipative Snubber

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IEEJ Transactions on electrical and Electronic engineering 2024年第11期19卷 1858-1878页

作者： Yau, Yeu-Torng Department of Ph.D. Program Prospective Technology of Electrical Engineering and Computer Science National Chin-Yi University of Technology Taichung No.57 Sec. 2 Zhongshan Rd. Taiping Dist Taichung41170 Taiwan

To provide a hold-up time function in DC-DC supplies for cell site stations or data centers, using a boost converter with a bulk output capacitor as a front-end converter stage is a simple and highly cost-effective solution. However, conventional boost converters with a hard-switching operation result in low conversion efficiency and increased electromagnetic interference emissions. In this paper, a boost converter with a new non-dissipative snubber is proposed that only requires two additional diodes, an inductor, and a multilayer ceramic capacitor. The main feature of the proposed snubber is that the components are not located on the main power processing path. This means they only require low ratings, improving cost-effectiveness. A prototype converter is analyzed, realized, and applied to a 300 W redundant DC-DC power supply module for a 5G cell base station. © 2024 The Author(s). IEEJ Transactions on electrical and Electronic engineering published by Institute of electrical Engineers of Japan and Wiley Periodicals LLC. © 2024 The Author(s). IEEJ Transactions on electrical and Electronic engineering published by Institute of electrical Engineers of Japan and Wiley Periodicals LLC.

关键词： Boost converter

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Experimental observation of coherent-perfect-absorber and laser points in anti-PT symmetry

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Physical Review A 2024年第3期110卷 033504页

作者： Minye Yang Qi Zhong Zhilu Ye Şahin K. Özdemir Mohamed Farhat Ramy El-Ganainy Pai-Yen Chen State Key Laboratory for Manufacturing Systems Engineering School of Electronic Science and Engineering Department of Electrical and Computer Engineering Department of Engineering Science and Mechanics The Materials Research Institute Computer Electrical and Mathematical Science and Engineering Division Department of Physics Henes Center for Quantum Phenomena

The coexistence of coherent perfect absorber and laser or amplifier (CPAL) point is a peculiar spectral singularity associated with the scattering matrices of non-Hermitian systems. While the potential of CPAL systems for sensing application has been highlighted recently, the extreme sensitivity of parity-time (PT)-symmetric CPAL devices to the input signal deviations has so far impeded their practical utilization. Here we explore a strategy for implementing CPAL circuits by exploiting another type of non-Hermitian symmetry, namely anti-PT (APT) symmetry. We demonstrate that the condition for building CPAL in our proposed APT-symmetric electronic circuits additionally requires parity symmetry, which simplifies the circuit design and implementation. Additionally, we show that this newly proposed structure is 1.85 times more robust compared to previous CPAL devices studied in the literature.

关键词： Noise Quantum sensing Non-Hermitian systems PT-symmetry

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Separation of Rare Earth Elements from Monazite Via Sulfidation 10th

Separation of Rare Earth Elements from Monazite Via Sulfidat...

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10th Symposium on Rare Metal Technology, held at the TMS Annual Meeting and Exhibition, TMS 2023

作者： Stinn, Caspar Kaker, Vasu Adams, Zachary Kenneth Allanore, Antoine Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA United States Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology CambridgeMA United States

ISBN: (纸本)9783031227608

Rare earth elements are critical for sustainability applications;yet, their extraction, separation, and smelting remain environmentally and economically tedious. Conventional rare earth processing consists of a sequence of physical beneficiation, hydrometallurgical, and metallothermic or electrolytic processes to produce pure metals and alloys. Environmental impacts are concentrated in impurities management and material separation. Recently, sulfide-based separation chemistries have been shown to offer higher separation effectiveness than legacy hydrometallurgical methods at a fraction of the cost and energy usage. However, previous experimental studies have only employed synthetic feedstocks of mixed rare earth oxides or FeNdB magnets. Herein, we consider rare earth element separation from monazite mineral using sulfidation. We explore the use of iron and alkaline-earth compounds as separation additives to enable separation of rare earth elements and sequestration of normally occurring radioactive materials in parallel with de phosphorylation. Preliminary experimental results indicate that the addition of iron during rare earth mineral sulfidation is a promising method to promote selectivity, potentially enabling targeted rare earth element extraction and production. © 2023, The Minerals, Metals & materials Society.

关键词： Rare earths

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Automated classification of big X-ray diffraction data using deep learning models

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npj Computational materials 2023年第1期9卷 169-180页

作者： Jerardo E.Salgado Samuel Lerman Zhaotong Du Chenliang Xu Niaz Abdolrahim Materials Science program University of RochesterRochesterNew York 14627USA Department of Computer Science University of RochesterRochesterNew York 14627USA Department of Mechanical Engineering University of RochesterRochesterNew York 14627USA Laboratory for Laser Energetics University of RochesterRochesterNew York 14627USA

In current in situ X-ray diffraction(XRD)techniques,data generation surpasses human analytical capabilities,potentially leading to the loss of *** techniques require human intervention,and lack the performance and adaptability required for material *** the critical need for high-throughput automated XRD pattern analysis,we present a generalized deep learning model to classify a diverse set of materials’crystal systems and space *** our approach,we generate training data with a holistic representation of patterns that emerge from varying experimental conditions and crystal *** also employ an expedited learning technique to refine our model’s expertise to experimental *** addition,we optimize model architecture to elicit classification based on Bragg’s Law and use evaluation data to interpret our model’s *** evaluate our models using experimental data,materials unseen in training,and altered cubic crystals,where we observe state-of-the-art performance and even greater advances in space group classification.

关键词： Automate classify cubic

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RDP: Ranked Differential Privacy for Facial Feature Protection in Multiscale Sparsified Subspaces

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IEEE Internet of Things Journal 2025年第11期12卷 17333-17348页

作者： Ou, Lu Liao, Shaolin Gao, Shihui Huang, Guandong Qin, Zheng Hunan University School of Journalism and Communication Hunan Changsha410082 China Sun Yat-sen University School of Electronics and Information Technology Guangzhou510275 China Illinois Institute of Technology Department of Electrical and Computer Engineering ChicagoIL60616 United States Purdue University Elmore School of Electrical and Computer Engineering West LafayetteIN47907 United States Hunan University College of Computer Science and Electronic Engineering Hunan Changsha410082 China State Grid Hunan Materials Company Department of Deployment Management Hunan Changsha410118 China

With the widespread sharing of personal face images on the Internet, systems based on face recognition encounter the real threat of being breached by potential adversaries who are able to access individuals’ face images and use them to intrude the systems. In this article, we propose a novel privacy protection method in the sparsified multiscale feature subspaces to protect sensitive facial features, taking care of the influence or weight-ranked subspace coefficients on the privacy budget, named "ranked differential privacy (RDP)." After the multiscale subspaces’ decomposition, the lightweight Laplacian noise is added to the dimension-reduced sparsified subspaces’ coefficients according to the geometric superposition method. Then, we rigorously prove that the RDP satisfies Ε0-differential privacy. After that, the nonlinear Lagrange multiplier method (LM) is formulated for the constraint optimization problem of maximizing the utility of protected face images of high-visualization quality with sanitizing noise, under a given privacy budget Ε0. Then, two methods are proposed to solve the nonlinear Lagrangian multiplier method (LM) problem and obtain the optimal noise scale parameters: 1) the analytical normalization approximation (NA) method with identical average noise scale parameter for real-time online applications and 2) the LM optimization method via gradient descent (LMGD) to obtain the nonlinear solution through iterative updating for more accurate offline applications. Experimental results on two real-world datasets show that our proposed RDP outperforms other state-of-the-art methods: at a privacy budget of Ε0 = 0.2 , the peak signal-to-noise ratio (PSNR) of the optimized RDP is about ~10 dB higher than (10 times as high as) the highest PSNR of all state-of-the-art methods compared. © 2014 IEEE.

关键词： Differential privacy

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Density Functional Theory Study of Surface Stability and Phase Diagram of Orthorhombic CsPbI3

arXiv

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arXiv 2024年

作者： Li, Kejia Wang, Mengen Department of Electrical and Computer Engineering and Materials Science and Engineering Program SUNY BinghamtonNY13902 United States

CsPbI3 has been recognized as a promising candidate for optoelectronic device applications. To further improve the efficiency of the devices, it is imperative to better understand the surface properties of CsPbI3, which affect charge carrier transport and defect formation properties. In this study, we perform density functional theory calculations to explore the stability of the (001), (110), and (100) surfaces of orthorhombic CsPbI3, considering different stoichiometries and surface reconstructions. Our results show that, under the chemical potentials confined by the thermodynamically stable region of bulk CsPbI3, the CsI-terminated surfaces of (001) and (110) and the stoichiometric surface of (100) are stable. Among these three surfaces, the CsI-terminated (110) surface has the lowest surface energy and no mid-gap states, which benefits the transport properties of the material. © 2024, CC BY-NC-SA.

关键词： Stoichiometry

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