The swift advancement of sustainable energy technologies,coupled with the urgent need to address environmental challenges,has generated considerable interest in the multifaceted applications of biochar materials to pr...
详细信息
The swift advancement of sustainable energy technologies,coupled with the urgent need to address environmental challenges,has generated considerable interest in the multifaceted applications of biochar materials to promote energy,water,and environmental *** comprehensive review examines recent advancements in the production and applications of functionalized biochar materials,emphasizing their pivotal roles in energy conversion and storage,wastewater treatment,CO_(2)reduction,soil amelioration,and the promotion of carbon neutrality within a circular economy *** functionalization of biochar materials involves surface chemistry and porosity modifications,achieved through techniques like templating,chemical activation,metal impregnation,or heteroatom *** modifications substantially enhance the catalytic activity,energy storage capacity,and cycling stability of biochar materials,making them particularly effective in diverse energy applications such as water splitting,fuel cells,and ***,functionalized biochar materials demonstrate remarkable efficacy as catalysts and adsorbents in wastewater treatment,proficiently removing pollutants like heavy metals,organic contaminants,and nutrients,thereby facilitating resource recovery from *** review also underscores the potential of functionalized biochar materials in CO_(2)capture and conversion,exploring innovative strategies to augment their CO_(2)adsorption capacity and state-of-the-art catalytic processes for transforming captured CO_(2)into valuable fuels and *** summary,this review offers valuable insights into the recent advancements in biochar research,underscoring its substantial commercial potential as a versatile material contributing to a cleaner and more sustainable future.
The dielectric environment plays a significant role in the performance of transition metal dichalcogenide FETs. In a previous study, a low mobility of monolayer (ML) MoS2 was extracted when located on an ultrathin die...
详细信息
Purpose: Colour fundus images are widely used in diagnosis treatment decision of several retinal diseases such as diabetic retinopathy (DR), glaucoma and age-related macular degeneration (AMD). These very common condi...
详细信息
The work function, which is the energy barrier for an electron escaping from the surface of a material, is a fundamental material surface property with many applications spanning energy harvesting, heterogeneous catal...
详细信息
The work function, which is the energy barrier for an electron escaping from the surface of a material, is a fundamental material surface property with many applications spanning energy harvesting, heterogeneous catalysis, vacuum electronics, and solid-state electronics. In this review, we define different aspects of the work function through an electrostatic potential treatment. We discuss in detail the role of electric fields, especially the heterogeneous surface patch field, in order to clarify potential points of confusion about work-function measurement and interpretation. We review standard experimental approaches to measure work function and the use of density-functional theory as a computational tool to predict work function. We then discuss the influence of materials chemistry and structure on work-function trends. We also discuss the role of work function in various applications, including a particular focus on relative electron energy-level alignment. Finally, we discuss two common approaches for engineering work-function values for specific applications: tuning the Fermi level and tuning the surface dipole. This review provides guidance for researchers interested in the intersection of work function, surface characterization, surface and interface physics and chemistry, and materials and device design for a wide array of technologically relevant applications.
Quantifying the nucleation processes involved in liquid-vapor phase-change phenomena,while dauntingly challenging,is central in designing energy conversion and thermal management *** technological advances in the deep...
详细信息
Quantifying the nucleation processes involved in liquid-vapor phase-change phenomena,while dauntingly challenging,is central in designing energy conversion and thermal management *** technological advances in the deep learning and computer vision field offer the potential for quantifying such complex two-phase nucleation processes at unprecedented *** leveraging these new technologies,a multiple object tracking framework called“vision inspired online nuclei tracker(VISION-iT)”has been proposed to extract large-scale,physical features residing within boiling and condensation ***,extracting high-quality features that can be integrated with domain knowledge requires detailed discussions that may be field-or case-specific *** this regard,we present a demonstration and discussion of the detailed construction,algorithms,and optimization of individual modules to enable adaptation of the framework to custom *** concepts and procedures outlined in this study are transferable and can benefit broader audiences dealing with similar problems.
We develop convergence acceleration procedures that enable a gradient descent-type iteration method to efficiently simulate Hartree-Fock equations for many particles interacting both with each other and with an extern...
详细信息
We develop convergence acceleration procedures that enable a gradient descent-type iteration method to efficiently simulate Hartree-Fock equations for many particles interacting both with each other and with an external potential. Our development focuses on three aspects: (i) optimization of a parameter in the preconditioning operator; (ii) adoption of a technique that eliminates the slowest-decaying mode to the case of many equations (describing many particles); and (iii) a novel extension of the above technique that allows one to eliminate multiple modes simultaneously. We illustrate performance of the numerical method for the two-dimensional model of the first layer of helium atoms above a graphene sheet. We demonstrate that incorporation of aspects (i) and (ii) above into the “plain” gradient descent method accelerates it by at least two orders of magnitude, and often by much more. Aspect (iii)—the multiple-mode elimination—may bring further improvement to the convergence rate compared to aspect (ii), the single-mode elimination. Both single- and multiple-mode elimination techniques are shown to significantly outperform the well-known Anderson Acceleration. We believe that our acceleration techniques can also be employed by other iterative methods, especially those handling hard-core-type interaction of many particles.
Fantasy Sports has a current market size of ${\$}$27B and is expected to grow more than ${\$}$84B in less than a decade. The intent is to create virtual teams that somehow reflect what would happen if the constituent ...
详细信息
The urgency of reducing pollutants and greenhouse gas emissions while maintaining fuel supply for the development of society remains one of the greatest *** energy,a clean and sustainable energy resource,can be conver...
详细信息
The urgency of reducing pollutants and greenhouse gas emissions while maintaining fuel supply for the development of society remains one of the greatest *** energy,a clean and sustainable energy resource,can be converted into fuels through solar-driven catalysis,and this provides an attractive solution for future energy *** current development of photothermal catalysis(PTC)based on the integration of solar thermal and photochemical contributions is becoming increasingly popular for full spectrum *** combination of the thermochemical and photochemical processes synergistically drives the catalytic reactions efficiently under relatively mild *** this review,the mechanisms of PTC are classified based on driving forces and the benefits of photothermal effects in different PTC reactions are ***,the techniques for differentiating and quantifying the various effects of PTC,including experimental designs,thermometry characterization techniques,and computational studies,are ***,the major determinant properties and architectural designs for efficient photothermal catalysts are ***,applications for fuel generation through water splitting and carbon dioxide reduction are ***,the current challenges and future directions of PTC are *** article aims to provide a comprehensive review of the current advances in PTC along with a guide for understanding the mechanisms and rational material designs to pursue solar fuel that would diversify and increase the sustainability of our energy supply.
Protected surface states arising fromnon-trivial bandstructure topology in semimetals can potentially enable advanced device functionalities in compute,memory,interconnect,sensing,and *** necessitates a fundamental un...
详细信息
Protected surface states arising fromnon-trivial bandstructure topology in semimetals can potentially enable advanced device functionalities in compute,memory,interconnect,sensing,and *** necessitates a fundamental understanding of surface-state transport in nanoscale topological ***,we investigate quantum transport in a prototypical topological semimetal NbAs to evaluate the potential of this class of materials for beyond-Cu interconnects in highly-scaled integrated *** density functional theory(DFT)coupled with non-equilibrium Green’s function(NEGF)calculations,we show that the resistance-areaRAproduct in NbAs films decreases with decreasing thickness at the nanometer scale,in contrast to a nearly constant RA product in ideal Cu *** anomalous scaling originates from the disproportionately large number of surface conduction states which dominate the ballistic conductance by up to 70%in NbAs thin *** also show that this favorable RA scaling persists even in the presence of surface defects,in contrast to RA sharply increasing with reducing thickness for films of conventional metals,such as Cu,in the presence of surface *** results underscore the potential of topological semimetals as future back-end-of-line(BEOL)interconnect metals.
Power densification is making thermal design a key step in the development of future electrical devices. Systems such as data centers and electric vehicles are generating more heat, which requires efficient cooling to...
详细信息
暂无评论