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arXiv 2023年

作者： Biswas, Abhijit Xu, Rui Alvarez, Gustavo A. Zhang, Jin Christiansen-Salameh, Joyce Puthirath, Anand B. Burns, Kory Hachtel, Jordan A. Li, Tao Iyengar, Sathvik Ajay Gray, Tia Li, Chenxi Zhang, Xiang Kannan, Harikishan Elkins, Jacob Pieshkov, Tymofii S. Vajtai, Robert Birdwell, A. Glen Neupane, Mahesh R. Garratt, Elias J. Ivanov, Tony Pate, Bradford B. Zhao, Yuji Zhu, Hanyu Tian, Zhiting Rubio, Angel Ajayan, Pulickel M. Department of Materials Science and Nanoengineering Rice University HoustonTX77005 United States Sibley School of Mechanical and Aerospace Engineering Cornell University IthacaNY14853 United States Max Planck Institute for the Structure and Dynamics of Matter Center for Free-Electron Laser Science Luruper Chaussee 149 22761 Germany Department of Materials Science & Engineering University of Virginia CharlottesvilleVA22904 United States Center for Nanophase Materials Sciences Oak Ridge National Laboratory Oak RidgeTN37831 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States DEVCOM Army Research Laboratory RF Devices and Circuits AdelphiMD20783 United States Chemistry Division Naval Research Laboratory WashingtonDC20375 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Flatiron Institute New YorkNY10010 United States

Understanding the emergent electronic structure in twisted atomically thin layers has led to the exciting field of twistronics. However, practical applications of such systems are challenging since the specific angular correlations between the layers must be precisely controlled and the layers have to be single crystalline with uniform atomic ordering. Here, we suggest an alternative, simple and scalable approach where nanocrystalline two-dimensional (2D) film on three-dimensional (3D) substrates yield twisted-interface-dependent properties. Ultrawidebandgap hexagonal boron nitride (h-BN) thin films are directly grown on high in-plane lattice mismatched wide-bandgap silicon carbide (4H-SiC) substrates to explore the twist-dependent structure-property correlations. Concurrently, nanocrystalline h-BN thin film shows strong nonlinear second-harmonic generation and ultra-low cross-plane thermal conductivity at room temperature, which are attributed to the twisted domain edges between van der Waals stacked nanocrystals with random in-plane orientations. First-principles calculations based on time-dependent density functional theory manifest strong even-order optical nonlinearity in twisted h-BN layers. Our work unveils that directly deposited 2D nanocrystalline thin film on 3D substrates could provide easily accessible twist-interfaces, therefore enabling a simple and scalable approach to utilize the 2D-twistronics integrated in 3D material devices for next-generation nanotechnology. © 2023, CC BY.

关键词： Harmonic generation

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Lattice dynamics localization in low-angle twisted bilayer graphene

arXiv

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arXiv 2020年

作者： Gadelha, Andreij C. Ohlberg, Douglas A.A. Rabelo, Cassiano Neto, Eliel G.S. Vasconcelos, Thiago L. Campos, João L. Lemos, Jessica S. Ornelas, Vinícius Miranda, Daniel Nadas, Rafael Santana, Fabiano C. Watanabe, Kenji Taniguchi, Takashi van Troeye, Benoit Lamparski, Michael Meunier, Vincent Nguyen, Viet-Hung Paszko, Dawid Charlier, Jean-Christophe Campos, Leonardo C. Cançado, Luiz G. Medeiros-Ribeiro, Gilberto Jorio, Ado Physics Department Electrical Engineering Graduate Program Computer Science Department Universidade Federal de Minas Gerais Belo HorizonteMG31270-901 Brazil Physics Institute Universidade Federal da Bahia Campus Universitário de Ondina Salvador - BA40170-115 Brazil Divisão de Metrologia de Materiais Inmetro Duque de Caxias RJ25250-020 Brazil 1-2-1 Sengen Tsukuba-cityIbaraki305-0047 Japan Physics Applied Physics and Astronomy Jonsson Rowland Science Center Room 1C25 110 8th Street TroyNY12180 United States Louvain-la-Neuve Belgium

A low twist angle between the two stacked crystal networks in bilayer graphene enables self-organized lattice reconstruction with the formation of a periodic domain. This superlattice modulates the vibrational and electronic structures, imposing new rules for electron-phonon coupling and the eventual observation of strong correlation and superconductivity. Direct optical images of the crystal superlattice in reconstructed twisted bilayer graphene are reported here, generated by the inelastic scattering of light in a nano-Raman spectroscope. The observation of the crystallographic structure with visible light is made possible due to lattice dynamics localization, the images resembling spectral variations caused by the presence of strain solitons and topological points. The results are rationalized by a nearly-free-phonon model and electronic calculations that highlight the relevance of solitons and topological points, particularly pronounced for structures with small twist angles. We anticipate our discovery to play a role in understanding Jahn-Teller effects and electronic Cooper pairing, among many other important phonon-related effects, and it may be useful for characterizing devices in the most prominent platform for the field of *** Codes 82D03 Copyright © 2020, The Authors. All rights reserved.

关键词： Electronic structure

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Macroscopically Self-Aligned and Chiralized Carbon Nanotubes: From Filtration to Innovation

arXiv

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arXiv 2023年

作者： Doumani, Jacques Zahn, Keshav Yu, Shengjie Barrios, Gustavo Rodriguez Sasmal, Somesh Kikuchi, Rikuta Kritzell, T. Elijah Xu, Hongjing Baydin, Andrey Kono, Junichiro Department of Electrical and Computer Engineering Rice University 6100 Main Street HoustonTX77005 United States Applied Physics Graduate Program Smalley–Curl Institute Rice University 6100 Main Street HoustonTX77005 United States Carbon Hub Rice University 6100 Main Street HoustonTX77005 United States Smalley–Curl Institute Rice University 6100 Main Street HoustonTX77005 United States Department of Physics and Astronomy Rice University 6100 Main Street HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University 6100 Main Street HoustonTX77005 United States

Because of their natural one-dimensional (1D) structure combined with intricate chiral variations, carbon nanotubes (CNTs) exhibit various exceptional physical properties, such as ultrahigh electrical and thermal conductivity, exceptional mechanical strength, and chirality-dependent metallicity. These properties make CNTs highly promising for diverse applications, including field-effect transistors, sensors, photodetectors, and thermoelectric devices. While CNTs excel individually at the nanoscale, their 1D and chiral nature can be lost on a macroscopic scale when they are randomly assembled. Therefore, the alignment and organization of CNTs in macroscopic structures is crucial for harnessing their full potential. In this review, we explore recent advancements in understanding CNT alignment mechanisms, improving CNT aligning methods, and demonstrating macroscopically 1D properties of ordered CNT assemblies. We also focus on a newly discovered class of CNT architectures, combining CNT alignment and twisting mechanisms to create artificial radial and chiral CNT films at wafer scales. Finally, we summarize recent developments related to aligned and chiral CNT films in optoelectronics, highlighting their unique roles in solar cells, thermal emitters, and optical modulators. Copyright © 2023, The Authors. All rights reserved.

关键词： Carbon nanotubes

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electrically driven programmable phase-change meta-switch reaching 80% efficiency

arXiv

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arXiv 2021年

作者： Abdollahramezani, Sajjad Hemmatyar, Omid Taghinejad, Mohammad Taghinejad, Hossein Krasnok, Alex Eftekhar, Ali A. Teichrib, Christian Deshmukh, Sanchit El-Sayed, Mostafa Pop, Eric Wuttig, Matthias Alù, Andrea Cai, Wenshan Adibi, Ali School of Electrical and Computer Engineering Georgia Institute of Technology 778 Atlantic Drive NW AtlantaGA30332-0250 United States Photonics Initiative Advanced Science Research Center City University of New York New YorkNY10031 United States Department of Electrical Engineering Precourt Institute for Energy Stanford University StanfordCA94305 United States Laser Dynamics Laboratory School of Chemistry and Biochemistry Georgia Institute of Technology AtlantaGA30332-0400 United States George W. Woodruff School of Mechanical Engineering Georgia Institute of Technology AtlantaGA30332-0405 United States Physikalisches Institut IA RWTH Aachen Sommerfeldstrasse 14 Aachen52074 Germany Physics Program Graduate Center City University of New York New YorkNY10016 United States School of Materials Science and Engineering Georgia Institute of Technology 801 Ferst Drive NW AtlantaGA30332-0295 United States

Despite recent advances in active metaoptics, efficient wide dynamic range combined with highspeed reconfigurable solutions is still elusive. Phase-change materials (PCMs) offer a compelling platform for metasurface optical elements, owing to the large index contrast and fast yet stable phase transition properties. Here, we experimentally demonstrate an in situ electrically driven reprogrammable metasurface by harnessing the unique properties of a phase-change chalcogenide alloy, Ge2Sb2Te5 (GST), in order to realize non-volatile, reversible, multilevel, fast, and pronounced optical modulation in the near-infrared spectral range. Co-optimized through a multiphysics analysis, we integrate an efficient heterostructure resistive microheater that indirectly heats and transforms the embedded GST film without compromising the optical performance of the metasurface even after several reversible phase transitions. A hybrid plasmonic-PCM meta-switch with a record eleven-fold change in the reectance (an absolute reectance contrast reaching 80%), unprecedented quasi-continuous spectral tuning over 250 nm, and operation speed that can potentially reach a few kHz is presented. Our work represents a significant step towards the development of fully integrable dynamic metasurfaces and their potential for beamforming applications. © 2021, CC BY.

关键词： Phase change materials

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Message

Message

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Conference on Advances in Signal Processing (CASP)

作者： Shri Promoad Gorhe Pradeep K. Sinha Madhuri A. Joshi M. B. Khambete Prachi Mukherji James L Garrison Pramod Kale Hemant A. Patil Aditya Abhyankar Arnab Das Maharshi Karve Stree Shikshan Samstha New Raipur University FIET (U.K.) FIE (I) FIETE (I) IET Pune Local Network College of Engineering Pune CCEW General Chair CASP-2016 (E&TC) CCEW Co Chair CASP-2016 Aeronautics and Astronautics Electrical and Computer Engineering (by courtesy) Ecological Sciences & Engineering Interdisciplinary Graduate Program Purdue University USA ICIT Pvt. Ltd. Pune Former Director ISRO DA-IICT Gandhinagar Gujarat State Faculty of Technology University of Pune Department of Technology University of Pune Acoustic Research Lab of the Tropical Marine Science Institute at the National University of Singapore Retd. Electrical Officer Indian Navy (1994 - 2015) Adjunct Faculty at IIT Delhi and DIAT Pune

Presents the introductory welcome message from the conference proceedings. May include the conference officers' congratulations to all involved with the conference event and publication of the proceedings record.

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Single-molecule localization microscopy reveals the ultrastructural constitution of distal appendages in expanded mammalian centrioles

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Nature communications 2023年第1期14卷 1688页

作者： Ting-Jui Ben Chang Jimmy Ching-Cheng Hsu T Tony Yang Department of Physics National Taiwan University Taipei Taiwan. Department of Electrical Engineering National Taiwan University Taipei Taiwan. Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Taiwan University Taipei Taiwan. Department of Electrical Engineering National Taiwan University Taipei Taiwan. tonyyang@ntu.edu.tw. Graduate Institute of Biomedical Electronics and Bioinformatics National Taiwan University Taipei Taiwan. tonyyang@ntu.edu.tw.

Distal appendages (DAPs) are vital in cilia formation, mediating vesicular and ciliary docking to the plasma membrane during early ciliogenesis. Although numerous DAP proteins arranging a nine-fold symmetry have been studied using superresolution microscopy analyses, the extensive ultrastructural understanding of the DAP structure developing from the centriole wall remains elusive owing to insufficient resolution. Here, we proposed a pragmatic imaging strategy for two-color single-molecule localization microscopy of expanded mammalian DAP. Importantly, our imaging workflow enables us to push the resolution limit of a light microscope well close to a molecular level, thus achieving an unprecedented mapping resolution inside intact cells. Upon this workflow, we unravel the ultra-resolved higher-order protein complexes of the DAP and its associated proteins. Intriguingly, our images show that C2CD3, microtubule triplet, MNR, CEP90, OFD1, and ODF2 jointly constitute a unique molecular configuration at the DAP base. Moreover, our finding suggests that ODF2 plays an auxiliary role in coordinating and maintaining DAP nine-fold symmetry. Together, we develop an organelle-based drift correction protocol and a two-color solution with minimum crosstalk, allowing a robust localization microscopy imaging of expanded DAP structures deep into the gel-specimen composites.

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Sensing the local magnetic environment through optically active defects in a layered magnetic semiconductor

arXiv

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arXiv 2022年

作者： Klein, Julian Song, Zhigang Pingault, Benjamin Dirnberger, Florian Chi, Hang Curtis, Jonathan B. Dana, Rami Bushati, Rezlind Quan, Jiamin Dekanovsky, Lukas Sofer, Zdenek Alù, Andrea Menon, Vinod M. Moodera, Jagadeesh S. Lončar, Marko Narang, Prineha Ross, Frances M. Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA02139 United States John A. Paulson School of Engineering and Applied Sciences Harvard University CambridgeMA United States College of Letters and Sciences UCLA Los AngelesCA90095 United States QuTech Delft University of Technology Delft2600 GA Netherlands Department of Physics City College of New York New YorkNY10031 United States Francis Bitter Magnet Laboratory Plasma Science and Fusion Center Massachusetts Institute of Technology CambridgeMA02139 United States U.S. Army CCDC Army Research Laboratory AdelphiMD20783 United States Department of Physics The Graduate Center City University of New York New YorkNY10016 United States Department of Electrical and Computer Engineering The University of Texas at Austin AustinTX78712 United States Photonics Initiative CUNY Advanced Science Research Center New YorkNY10031 United States Department of Electrical Engineering City College of the City University of New York New YorkNY10031 United States Physics Program Graduate Center City University of New York New YorkNY10026 United States Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 Prague 6166 28 Czech Republic Department of Physics Massachusetts Institute of Technology CambridgeMA02139 United States

Atomic-level defects in van der Waals (vdW) materials are essential building blocks for quantum technologies and quantum sensing applications. The layered magnetic semiconductor CrSBr is an outstanding candidate for exploring optically active defects owing to a direct gap in addition to a rich magnetic phase diagram including a recently hypothesized defect-induced magnetic order at low temperature. Here, we show optically active defects in CrSBr that are probes of the local magnetic environment. We observe spectrally narrow (1 meV) defect emission in CrSBr that is correlated with both the bulk magnetic order and an additional low temperature defect-induced magnetic order. We elucidate the origin of this magnetic order in the context of local and non-local exchange coupling effects. Our work establishes vdW magnets like CrSBr as an exceptional platform to optically study defects that are correlated with the magnetic lattice. We anticipate that controlled defect creation allows for tailor-made complex magnetic textures and phases with the unique ingredient of direct optical access. Copyright © 2022, The Authors. All rights reserved.

关键词： Magnetic semiconductors

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Corrigendum to "Target-specific near-IR induced drug release and photothermal therapy with accumulated Au/Ag hollow nanoshells on pulmonary cancer cell membranes" [Biomaterials 45 (2015) 81-92]

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Biomaterials 2015年 65卷 124-125页

作者： Mi Suk Noh Somin Lee Homan Kang Jin-Kyoung Yang Hyunmi Lee Doyk Hwang Jong Woo Lee Sinyoung Jeong Yoonjeong Jang Bong-Hyun Jun Dae Hong Jeong Seong Keun Kim Yoon-Sik Lee Myung-Haing Cho Laboratory of Toxicology College of Veterinary Medicine Seoul National University Seoul 151-742 Republic of Korea Program in Nano Science and Technology Graduate School of Convergence Science and Technology Seoul National University Seoul 151-742 Republic of Korea Medical Supplies Evaluation Center Korea Testing Certification Gunpo 435-862 Republic of Korea. Graduate Group of Tumor Biology Seoul National University Seoul 151-742 Republic of Korea. Interdisciplinary Program in Nano-Science and Technology Seoul National University Seoul 151-742 Republic of Korea School of Electrical Engineering and Computer Science Seoul National University Seoul 151-742 Republic of Korea. School of Chemical and Biological Engineering Seoul National University Seoul 151-742 Republic of Korea. Department of Biophysics and Chemical Biology and Department of Chemistry Seoul National University Seoul 151-742 Republic of Korea. Department of Chemistry Education Seoul National University Seoul 151-742 Republic of Korea. Laboratory of Toxicology College of Veterinary Medicine Seoul National University Seoul 151-742 Republic of Korea. Department of Bioscience and Biotechnology Konkuk University Seoul 143-701 Republic of Korea. Department of Chemistry Education Seoul National University Seoul 151-742 Republic of Korea. School of Chemical and Biological Engineering Seoul National University Seoul 151-742 Republic of Korea. Electronic address: yslee@snu.ac.kr. Graduate Group of Tumor Biology Seoul National University Seoul 151-742 Republic of Korea Advanced Institute of Convergence Technology Seoul National University Suwon 443-270 Republic of Korea. Electronic address: mchotox@snu.ac.kr.

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A web-based, hospital-wide health care-associated bloodstream infection surveillance and classification system: Development and evaluation

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JMIR Medical Informatics 2015年第3期3卷 e31页

作者： Tseng, Yi-Ju Wu, Jung-Hsuan Lin, Hui-Chi Chen, Ming-Yuan Ping, Xiao-Ou Sun, Chun-Chuan Shang, Rung-Ji Sheng, Wang-Huei Chen, Yee-Chun Lai, Feipei Chang, Shan-Chwen Graduate Institute of Biomedical Electronics and Bioinformatics National Taiwan University Taipei Taiwan Computational Health Informatics Program Boston Children's Hospital Boston MA United States Department of Electrical Engineering National Taiwan University Taipei Taiwan Center for Infection Control National Taiwan University Hospital Taipei Taiwan National Taiwan University Hospital Information Systems Office Taipei Taiwan Department of Computer Science and Information Engineering National Taiwan University Taipei Taiwan Department of Internal Medicine National Taiwan University Hospital and College of Medicine Taipei Taiwan National Health Research Institutes National Institute of Infectious Diseases and Vaccinology Miaoli Taiwan

Background: Surveillance of health care-associated infections is an essential component of infection prevention programs, but conventional systems are labor intensive and performance dependent. Objective: To develop an automatic surveillance and classification system for health care-associated bloodstream infection (HABSI), and to evaluate its performance by comparing it with a conventional infection control personnel (ICP)-based surveillance system. Methods: We developed a Web-based system that was integrated into the medical information system of a 2200-bed teaching hospital in Taiwan. The system automatically detects and classifies HABSIs. Results: In this study, the number of computer-detected HABSIs correlated closely with the number of HABSIs detected by ICP by department (n=20;r=.999 P<.001) and by time (n=14;r=.941;P<.001). Compared with reference standards, this system performed excellently with regard to sensitivity (98.16%), specificity (99.96%), positive predictive value (95.81%), and negative predictive value (99.98%). The system enabled decreasing the delay in confirmation of HABSI cases, on average, by 29 days. Conclusions: This system provides reliable and objective HABSI data for quality indicators, improving the delay caused by a conventional surveillance system. © 2020 JMIR Publications Inc. All rights reserved.

关键词： Health care-associated infection Infection control Information systems Surveillance Web-based services

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Ubiquitous Flat Bands in a Cr-based Kagome Superconductor

arXiv

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arXiv 2024年

作者： Guo, Yucheng Wang, Zehao Xie, Fang Huang, Yuefei Gao, Bin Oh, Ji Seop Wu, Han Liu, Zhaoyu Ren, Zheng Fang, Yuan Biswas, Ananya Zhang, Yichen Yue, Ziqin Hu, Cheng Jozwiak, Chris Bostwick, Aaron Rotenberg, Eli Hashimoto, Makoto Lu, Donghui Kono, Junichiro Chu, Jiun-Haw Yakobson, Boris I. Birgeneau, Robert J. Si, Qimiao Dai, Pengcheng Yi, Ming Department of Physics and Astronomy Rice University HoustonTX77005 United States Advanced Light Source Lawrence Berkeley National Laboratory BerkeleyCA94720 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Department of Physics University of California BerkeleyCA94720 United States Department of Physics University of Washington Washington98105 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo ParkCA94025 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States

In the quest for novel quantum states driven by topology and correlation, kagome lattice materials have garnered significant interest due to their distinctive electronic band structures, featuring flat bands (FBs) arising from the quantum destructive interference of the electronic wave function. The tuning of the FBs to the chemical potential would lead to the possibility of liberating electronic instabilities that lead to emergent electronic orders. Despite extensive studies, direct evidence of FBs tuned to the chemical potential and their participation in emergent electronic orders have been lacking in bulk quantum materials. Here using a combination of Angle-Resolved Photoemission Spectroscopy (ARPES) and Density Functional Theory (DFT), we reveal that the low-energy electronic structure of the recently discovered Cr-based kagome metal superconductor CsCr3Sb5 is dominated by a pervasive FB in close proximity to, and below the Fermi level. A comparative analysis with orbital-projected DFT and polarization dependence measurement uncovers that an orbital-selective renormalization mechanism is needed to reconcile the discrepancy with the DFT calculations, which predict the FB to appear 200 meV above the Fermi level. Furthermore, we observe the FB to shift away from the Fermi level by 20 meV in the low-temperature density wave-ordered phase, highlighting the role of the FB in the emergent electronic order. Our results reveal CsCr3Sb5 to stand out as a promising platform for further exploration into the effects of FBs near the Fermi level on kagome lattices, and their role in emergent orders in bulk quantum materials. © 2024, CC BY.

关键词： Density functional theory

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