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Specular inverse Faraday effect in transition metals

Physical Review materials 2023年第12期7卷 125202-125202页

作者： Victor H. Ortiz Shashi B. Mishra Luat Vuong Sinisa Coh Richard B. Wilson Department of Mechanical Engineering and Materials Science and Engineering Program University of California Riverside 92521 CA United States

The inverse Faraday effect is an optomagnetic phenomenon that describes the ability of circularly polarized light to induce magnetism in solids. The capability of light to control magnetic order in solid state materials and devices is of interest for a variety of applications, such as magnetic recording, quantum computation, and spintronic technologies. However, significant gaps in understanding about the effect persist, such as what material properties govern the magnitude of the effect in metals. In this work, we report time-resolved measurements of the specular inverse Faraday effect in nonmagnetic metals, i.e., the magneto-optic Kerr effect induced by circularly polarized light. We measure this specular inverse Faraday effect in Cu, Pd, Pt, W, Ta, and Au at a laser wavelength of 783 nm. For Ta and W, we investigate both α and β phases. We observe that excitation of these metals with circularly polarized light induces significant circular dichroism. This nonlinear magneto-optical response to circularly polarized light is an order of magnitude larger in α-W than other metals, e.g., Pt or Au, and is greater than nearly all other reported values for the inverse Faraday effect in other materials. Our results benchmark the range of the inverse Faraday effect that can be observed in nonmagnetic metals and provide insight into what material properties govern the inverse Faraday effect in metals.

关键词： Light-induced magnetic effects Magneto-optics Ultrafast optics Magneto-optical Kerr effect Sputtering Ultrafast femtosecond pump probe

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Preface to Crystalline Porous materials

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Chinese Journal of Structural Chemistry 2022年第11期41卷 1-2页

作者： Jiandong Pang Ning Huang Shuai Yuan Jun-Sheng Qin School of Materials Science and Engineering National Institute for Advanced MaterialsTKL of Metal and Molecule-Based Material ChemistryNankai UniversityTianjin300350China MOE Key Laboratory of Macromolecular Synthesis and Functionalization State Key Laboratory of Silicon MaterialsDepartment of Polymer Science and EngineeringZhejiang UniversityHangzhou 310027China State Key Laboratory of Coordination Chemistry School of Chemistry and Chemical EngineeringNanjing UniversityNanjing 210023China State Key Laboratory of Inorganic Synthesis and Preparative Chemistry College of Chemistry and International Center of Future ScienceJilin UniversityChangchun130012China

Novel crystalline porous materials refer to porous materials constructed by linking organic molecule units with coordination bonds, covalent bonds, or supramolecular interactions, mainly including metal-organic frameworks(MOFs), covalent organic frameworks(COFs), metal organic cages(MOCs), and so on. Due to their predictable and designable long-range ordered structures.

关键词： porous Porous linking

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Vibrational EELS for Solid-State Li-Ion Batteries: Mapping Li Distributions and Beyond

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Microscopy and microanalysis : the official journal of Microscopy Society of America, Microbeam Analysis Society, Microscopical Society of Canada 2023年第1期29卷 633-635页

作者： Gadre, Chaitanya A. Lee, Tom Qi, Ji Ong, Shyue Ping Pan, Xiaoqing Department of Physics and Astronomy University of California Irvine CA United States Department of Materials Science and Engineering University of California Irvine CA United States Materials Science and Engineering Program University of California San Diego La Jolla CA United States Department of NanoEngineering University of California San Diego La Jolla CA United States Irvine Materials Research Institute University of California Irvine CA United States

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Characterization of Spicule Structure 152nd

Characterization of Spicule Structure

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152nd Annual Meeting and Exhibition of The Minerals, Metals and materials Society, TMS 2023

作者： Tavangarian, Fariborz Gray, Jennifer L. Clark, Trevor Gao, Chao Mechanical Engineering Program School of Science Engineering and Technology Pennsylvania State University Harrisburg MiddletownPA17057 United States Materials Research Institute The Pennsylvania State University University Park PA16802 United States Department of Mechanical and Industrial Engineering Norwegian University of Science and Technology Trondheim7034 Norway

ISBN: (纸本)9783031225239

Nature has been a great source of inspiration for engineers and scientists for centuries. It provides unique ideas to overcome the unmet needs of human beings. Spicules are structural elements of Euplectella Aspergillum sponges that reside in the deep ocean. They have an exceptional microstructure that provides excellent mechanical properties. Although spicules are composed of a brittle material, silica (SiO2), they behave differently under load compared to other ceramics. This behavior is due to their concentric cylindrical structure. To produce a similar structure with potential engineering and biomedical applications, one needs to investigate its microstructure in depth. In this study, we examined the microstructure of spicules to understand their architecture as a foundation to better design biomedical implants for tissue engineering applications. © 2023, The Minerals, Metals & materials Society.

关键词： Microstructure

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An ultraefficient surface functionalized Ti3C2Tx MXene piezocatalyst: synchronous hydrogen evolution and wastewater treatment

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Journal of materials Chemistry A 2023年第6期12卷 3340-3351页

作者： Lai, Sz-Nian Chen, Winston Yenyu Yen, Chao-Chun Liao, Yin-Song Chen, Po-Han Stanciu, Lia Wu, Jyh Ming Department of Materials Science and Engineering National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan PhD Program in Prospective Functional Materials Industry National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan High Entropy Materials Center National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan Tsing Hua Interdisciplinary Program National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan School of Materials Engineering Purdue University 610 Purdue Mall West LafayetteIN47907 United States Department of Materials Science and Engineering National Chung Hsing University 145 Xingda Road Taichung402 Taiwan

The Ti3C2Tx surface contains hydroxyl groups that can be modified through self-assembled monolayers by using (3-chloropropyl) trimethoxysilane (CPTMS) and fluoroalkylsilane (FOTS). This study demonstrates that an ultrahigh level of piezoelectricity can be achieved by modifying the Si-O bond of organo-silane headgroups in Ti3C2Tx. The theoretical calculation of surface functionalized Ti3C2Tx-FOTS reveals that its Si-O bond causes localized lattice distortion and enhances the noncentrosymmetric structure on the Ti3C2Tx surface. Ti3C2Tx-FOTS exhibits significantly higher butterfly loops than pristine Ti3C2Tx. The calculated rate constant of Ti3C2Tx-FOTS for dye degradation was 0.9 min−1, 15-fold higher than that of Ti3C2Tx-CPTMS and 111-fold higher than that of pristine Ti3C2Tx. The hydrogen evolution rate of Ti3C2Tx-FOTS is 900.46 μmo1 g−1 h−1, three times higher than that of Ti3C2Tx. The bifunctional surface functionalized Ti3C2Tx-FOTS can simultaneously catalyse the hydrogen evolution reaction (HER) and decomposition of wastewater, demonstrating that Ti3C2Tx-FOTS, obtained through the surface engineering of Ti3C2Tx, is a superior piezocatalyst. © 2024 The Royal Society of Chemistry.

关键词： Rate constants

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Investigation of oxygen-related defect engineering in nonstoichiometric vanadium oxides for electrochromic zinc-ion batteries with superior electrochromic-electrochemical performance

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Chemical engineering Journal 2025年 515卷

作者： Kim, Yonghan kim, Ilgyu Lee, Hye Kang Na, Hyunmin Jung, Ji-Won Yun, Tae Gwang Department of of Molecular Science and Technology Ajou University Gyeonggi Suwon16499 Korea Republic of Department of Materials Science and Engineering Konkuk University Seoul05029 Korea Republic of Advanced Materials Program Department of Materials Science and Engineering Konkuk University Seoul05029 Korea Republic of

Electrochromic-energy storage systems (e-ESS), which visualize the electrochemical charge–discharge process, are experiencing a rapid increase in demand for advanced applications. Electrochromic aqueous zinc-ion batteries (e-AZiBs) systems have emerged as a promising alternative due to their environmental friendliness, enhanced stability, and high volumetric energy density. In this study, we developed a non-stoichiometric vanadium oxide cathode that optimizes both electrochemical and electrochromic performance by controlling the oxygen defect concentration. By optimizing the annealing temperature, we effectively controlled the concentration of oxygen defects, which enhanced Zn2+ diffusion kinetics within the layered structure of V2O5 and promoted more reversible energy storage reactions. In particular, Ec-VO 350 sample, with the most favorable level of oxygen defects, exhibited a specific capacity of 383 mAh/g, representing a 160 % improvement in electrochemical performance compared to pristine V2O5. Additionally, the structural modifications induced by oxygen defects significantly improved electrochemical stability, achieving 98.27 % capacity retention after 500 cycles at 2 A/g, demonstrating excellent reversibility. Meanwhile, although the defect states generated by oxygen vacancies can affect the electronic structure and negatively influence electrochromic properties such as coloration efficiency and ΔT, Ec-VO 350 sample successfully achieved a coloration efficiency of 46.8 cm2/C and a ΔT of 65 %, owing to its enhanced Zn2+ diffusion kinetics despite a reduced optical bandgap. The methodology for developing the non-stoichiometric vanadium oxide cathode presented in this study offers an innovative strategy to enhance the potential for electrochromic energy storage systems (e-ESS) in advanced applications. © 2025

关键词： Virtual storage

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Biomass-Based Discrete Furan Oligomers as materials for Electrochromic Devices

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ACS Sustainable Chemistry and engineering 2024年第1期12卷 459-469页

作者： Atayde, Eduardo C. Fong, Guan-Lun Yeh, Jyun-Yi Matsagar, Babasaheb M. Wang, Yu-Cheng Chen, De-Chian Peng, Chi-How Li, Yi-Pei Yamauchi, Yusuke Ho, Kuo-Chuan Wu, Kevin C.-W. Molecular Science and Technology Program Taiwan International Graduate Program (TIGP-MST) Academia Sinica No. 128 Sec. 2 Academia Road Taipei 11529 Taiwan Department of Chemistry National Tsing Hua University No. 101 Sec. 2 Kuang-Fu Road Hsinchu 30013 Taiwan Department of Chemical Engineering National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Sustainable Chemical Science and Technology Program Taiwan International Graduate Program (TIGP-SCST) Academia Sinica No. 128 Sec. 2 Academia Road Taipei 11529 Taiwan School of Chemical Engineering and Australian Institute for Bioengineering and Nanotechnology (AIBN) The University of Queensl Brisbane 4072 QLD Australia Department of Materials Process Engineering Graduate School of Engineering Nagoya University Nagoya 464-8603 Japan Institute of Polymer Science and Engineering National Taiwan University No.1 Sec. 4 Roosevelt Rd. Taipei 10617 Taiwan Department of Chemical Engineering and Materials Science Yuan Ze University No. 135 Yuandong Rd. Taoyuan 320 Taiwan

Electrochromic devices (ECDs) are materials that can undergo reversible changes in transmittance when exposed to different applied potentials. While many conjugated heterocyclic oligomers, such as oligothiophenes, have been developed for this purpose, there is no reported study on the use of discrete oligomeric furans as ECD materials. In this work, we introduce a furan trimer that can be utilized as a discrete electrochromic material, which transitions from light yellow to red and has a very high coloration efficiency of 1940 cm²/C at 507 nm. We propose that the reversible π-stack formation of the oligomer radical cations is behind this phenomenon, as evidenced by both experimental and computational results. The derivability of this oligomer from biomass and its facile synthesis make it an interesting alternative for other existing organic electrochromic materials. © 2023 American Chemical Society

关键词： electrochromism furan oligomer hydroxyalkylation−alkylation reaction solvatochromism π-stacks

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Two-dimensional MXenes:New frontier of wearable and flexible electronics

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InfoMat 2022年第4期4卷 1-28页

作者： Abbas Ahmed Sudeep Sharma Bapan Adak Md Milon Hossain Anna Marie LaChance Samrat Mukhopadhyay Luyi Sun Polymer Program Institute of Materials ScienceUniversity of ConnecticutStorrsConnecticutUSA Advanced Sensor and Energy Research(ASER)Lab Department of Electronic EngineeringKwangwoon UniversitySeoulSouth Korea Department of Textile and Fiber Engineering Indian Institute of TechnologyNew DelhiIndia Department of Textile Engineering Chemistry and ScienceNorth Carolina State UniversityRaleighNorth CarolinaUSA Department of Textile Engineering Khulna University of Engineering&TechnologyKhulnaBangladesh Department of Chemical and Biomolecular Engineering University of ConnecticutStorrsConnecticutUSA

Wearable electronics offer incredible benefits in mobile healthcare monitoring,sensing,portable energy harvesting and storage,human-machine interactions,etc.,due to the evolution of rigid electronics structure to flexible and stretchable ***,transition metal carbides and nitrides(MXenes)are highly regarded as a group of thriving two-dimensional nanomaterials and extraordinary building blocks for emerging flexible electronics platforms because of their excellent electrical conductivity,enriched surface functionalities,and large surface *** article reviews the most recent developments in MXene-enabled flexible electronics for wearable *** MXeneenabled electronic devices designed on a nanometric scale are highlighted by drawing attention to widely developed nonstructural attributes,including 3D configured devices,textile and planer substrates,bioinspired structures,and printed ***,the unique progress of these nanodevices is highlighted by representative applications in healthcare,energy,electromagnetic interference(EMI)shielding,and humanoid control of *** emerging prospects of MXene nanomaterials as a key frontier in nextgeneration wearable electronics are envisioned and the design challenges of these electronic systems are also discussed,followed by proposed solutions.

关键词： flexible electronics MXene nanostructures wearable electronics

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An expandable chamber for safe brain retraction: new technologies in the field of transcranial endoscopic surgery

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Journal of Zhejiang University-science B(Biomedicine & Biotechnology) 2023年第4期24卷 326-335页

作者： Elena ROCA Anna GOBETTI Giovanna CORNACCHIA Oscar VIVALDI Barbara BUFFOLI Giorgio RAMORINO Head and Neck Department NeurosurgeryIstituto Ospedaliero Fondazione Poliambulanza25124 BresciaItaly Technology for Health PhD Program University of Brescia25124 BresciaItaly Materials Science and Technology at Department of Mechanical and Industrial Engineering University of Brescia25123 BresciaItaly Metallurgy at Department of Mechanical and Industrial Engineering University of Brescia25123 BresciaItaly Anatomy and Physiopathology Division Department of Clinical and Experimental SciencesUniversity of Brescia25123 BresciaItaly

Neurosurgery is a highly specialized field:it often involves surgical manipulation of noble structures and cerebral retraction is frequently necessary to reach deep-seated brain *** are still no reliable methods preventing possible retraction *** objective of this study was to design work chambers well suited for transcranial endoscopic surgery while providing safe retraction of the surrounding brain *** chamber is designed to be inserted close to the intracranial point of interest;once it is best placed it can be *** should guarantee an appreciable workspace similar to that of current neurosurgical *** experimental aspect of this study involved the use of a force sensor to evaluate the pressures exerted on the brain tissue during the retraction *** pterional craniotomy,pressure measurements were made during retraction with the use of a conventional metal spatula with different *** that,although the force values necessary for retraction and exerted on the spatula by the neurosurgeon are the same,the local pressure exerted on the parenchyma at the edge of the spatula at different inclinations varied greatly.A new method of cerebral retraction using a chamber retractor(CR)has been designed to avoid any type of complication due to spatula edge overpressures and to maintain acceptable pressure values exerted on the parenchyma.

关键词： Brain retraction Spatula Brain retractor design Brain retraction injury Retraction complication Transcranial endoscopic surgery

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Highly electrically conductive graphene papers via catalytic graphitization

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Nano Research 2022年第6期15卷 4902-4908页

作者： Huanqin Peng Xin Ming Kai Pang Yanru Chen Ji Zhou Zhen Xu Yingjun Liu Chao Gao MOE Key Laboratory of Macromolecular Synthesis and Functionalization Department of Polymer Science and EngineeringKey Laboratory of Adsorption and Separation Materials&Technologies of Zhejiang ProvinceZhejiang University38 Zheda RoadHangzhou 310027China Beijing Institute of Space Mechanics&Electricity Haidian DistrictBeijing Friendship Road 104Beijing 100094China Shanxi-Zheda Institute of Advanced Materials and Chemical Engineering Taiyuan 030032China

The highly electrically conductive graphene papers prepared from graphene oxide have shown promising perspectives in flexible electronics,electromagnetic interference(EMI)shielding,and *** achieve high electrical conductivity,the graphene oxide precursor usually needs to be graphitized at extremely high temperature(~2,800°C),which severely increases the energy consumption and production ***,we report an efficient catalytic graphitization approach to fabricate highly conductive graphene papers at lower annealing *** graphene papers with boron catalyst annealed at 2,000°C show a high conductivity of~3,400 S·cm^(-1),about 47%higher than pure graphene *** catalyst facilitates the recovery of structural defects and improves the degree of graphitization by 80%.We further study the catalytic effect of boron on the graphitization behavior of graphene *** results show that the activation energy of the catalytic graphitization process is as low as 80.1 kJ·mol^(–1)in the temperature ranges *** effective strategy of catalytic graphitization should also be helpful in the fabrication of other kinds of highly conductive graphene macroscopic materials.

关键词： graphene papers catalytic graphitization boron catalyst catalytic kinetics

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