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High-performance non-Fermi-liquid metallic thermoelectric materials

npj Computational materials 2023年第1期9卷 1943-1949页

作者： Zirui Dong Yubo Zhang Jun Luo Ying Jiang Zhiyang Yu Nan Zhao Liusuo Wu Yurong Ruan Fang Zhang Kai Guo Jiye Zhang Wenqing Zhang School of Materials Science and Engineering Shanghai UniversityShanghai 200444China Department of Materials Science and Engineering Department of Physicsand Shenzhen Institute for Quantum Science and EngineeringSouthern University of Science and TechnologyShenzhen 518055China Shenzhen Municipal Key-Lab for Advanced Quantum Materials and Devices and Guangdong Provincial Key Lab for Computational Science and Materials DesignSouthern University of Science and TechnologyShenzhen 518055China Materials Genome Institute Shanghai UniversityShanghai 200444China State Key Laboratory of Photocatalysis on Energy and Environment College of ChemistryFuzhou UniversityFuzhou 350002China School of Physics and Materials Science Guangzhou UniversityGuangzhou 510006China

Searching for high-performance thermoelectric(TE)materials in the paradigm of narrow-bandgap semiconductors is hampered by a *** we report on the discovery of metallic compounds,TiFe_(x)Cu_(2x−1)Sb and TiFe1.33Sb,showing the thermopower exceeding many TE semiconductors and the dimensionless figure of merits zTs comparable with the state-of-the-art TE materials.A quasi-linear temperature(T)dependent electrical resistivity in 2–700 K and the logarithmic T-dependent electronic specific heat at low temperature coexist with the high thermopower,highlighting the strong intercoupling of the non-Fermi-liquid(NFL)quantum critical behavior of electrons with TE *** structure analysis reveals a competition between the antiferromagnetic(AFM)ordering and Kondo-like spin compensation as well as a parallel two-channel Kondo *** T-dependent magnetic susceptibility agrees with the quantum critical scenario of strong local *** work demonstrates the correlation among high TE performance,NFL quantum criticality,and magnetic fluctuation,which opens up directions for future research.

关键词： materials metallic Fermi

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Construction of dendritic Pt–Pd bimetallic nanotubular heterostructure for advanced oxygen reduction

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Interdisciplinary materials 2024年第6期3卷 907-918页

作者： Mingwei Wang Zhiyi Hu Jieheng Lv Zhiwen Yin Zhewei Xu Jingfeng Liu Shihao Feng Xiaoqian Wang Jiazhen He Sicheng Luo Dafu Zhao Hang Li Xuemin Luo Qi Liu Damin Liu Baolian Su Dongyuan Zhao Yong Liu International School of Materials Science and Engineering(ISMSE) State Key Laboratory of Advanced Technology for Materials Synthesis and ProcessingWuhan University of TechnologyWuhanChina Department of Chemistry Laboratory of Inorganic Materials ChemistryUniversity of NamurNamurBelgium Department of Chemistry Laboratory of Advanced MaterialsShanghai Key Lab of Molecular Catalysis and Innovative MaterialsState Key Laboratory of Molecular Engineering of PolymersFudan UniversityShanghaiChina

Compositions and morphologies of Pt-based electrocatalysts have great impact on the electrocatalytic activity and stability of oxygen reduction reaction(ORR).Herein,we report a novel design of one-dimensional(1D)Pt-Pd dendritic nanotubular heterostructures(DTHs)by controlling the degree of Pt 2+-Pt reduction reaction and Pd-Pt galvanic replacement reaction with uniform Pd nanowires as sacrificial *** obtained Pt-Pd bimetallic DTHs catalyst exhibited uniform and dense Pt dendritic nanobranches on the surface of 1D hollow Pt-Pd alloy nanotubes,possessing superior catalytic activity for ORR compared to state-of-the-art commercial Pt/C ***,the Pt_(4)Pd DTHs catalyst showed efficient mass activity(MA,1.05 A mg_(Pt)^(−1))and specific activity(SA,1.25 mA cm_(Pt)^(−2))at 0.9 V(***),and the catalyst exhibited high stability with 90.4%MA retention after 20000 potential *** Pt-Pd bimetallic DTHs configuration combines the advantages of 1D hollow nanostructures and dense Pt dendritic nanobranches,which results in rich electrochemical active surface sites,fast charge transport,and multiple dendritic anchoring points contact on carbon support,thus boosting its catalytic activity and stability towards electrocatalysis.

关键词： dendritic hollow heterostructures electrocatalysis one-dimensional nanowires oxygen reduction proton exchange membrane fuel cells

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Enhancing crystal integrity and structural rigidity of CsPbBr_(3) nanoplatelets to achieve a narrow colorsaturated blue emission

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Light(science & Applications) 2024年第5期13卷 985-997页

作者： Qianqian Huang Wenxu Yin Bo Gao Qingsen Zeng Dong Yao Hao Zhang Yinghe Zhao Weijia Zheng Jiaqi Zhang Xuyong Yang Xiaoyu Zhang Andrey L.Rogach Key Laboratory of Automobile Materials MOE School of Materials Science&Engineeringand Jilin Provincial International Cooperation Key Laboratory of High-Efficiency Clean Energy MaterialsJilin UniversityChangchunChina. State Key Laboratory of Supramolecular Structure and Materials College of ChemistryJilin UniversityChangchunChina. State Key Laboratory of Materials Processing and Die&Mould Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhanHubeiChina. Department of Chemistry University of VictoriaVictoriaBCCanada. Key Laboratory of Advanced Display and System Applications of Ministry of Education Shanghai UniversityShanghaiChina. Department of Materials Science and Engineering and Centre for Functional Photonics(CFP)City University of Hong KongHong Kong S.A.RChina

Quantum-confined CsPbBr_(3) perovskites are promising blue emitters for ultra-high-definition displays,but their soft lattice caused by highly ionic nature has a limited ***,we endow CsPbBr_(3) nanoplatelets(NPLs)with atomic crystal-like structural rigidity through proper surface engineering,by using strongly bound N-dodecylbenzene sulfonic acid(DBSA).A stable,rigid crystal structure,as well as uniform,orderly-arranged surface of these NPLs is achieved by optimizing intermediate reaction stage,by switching from molecular clusters to mono-octahedra,while interaction with DBSA resulted in formation of a Cs_(x)O monolayer shell capping the NPL *** a result,both structural and optical stability of the CsPbBr3 NPLs is enhanced by strong covalent bonding of DBSA,which inhibits undesired phase transitions and decomposition of the perovskite phase potentially caused by ligand ***,rather small amount of DBSA ligands at the NPL surface results in a short inter-NPL spacing in their closely-packed films,which facilitates efficient charge injection and *** photoluminescence of the produced CsPbBr_(3) NPLs is bright(nearly unity emission quantum yield)and peaks at 457 nm with an extremely narrow bandwidth of 3.7 nm at 80 K,while the bandwidth of the electroluminescence(peaked at 460 nm)also reaches a record-narrow value of 15 nm at room *** value corresponds to the CIE coordinates of(0.141,0.062),which meets Rec.2020 standards for ultra-high-definition displays.

关键词： temperature stability narrow

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Chlorine-rich lithium argyrodites enables superior performances for solid-state Li-Se batteries at wide temperature range

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Rare Metals 2022年第12期41卷 4065-4074页

作者： Jin-Yan Lin Shuai Chen Jia-Yang Li Dian Yu Xiang-Ling Xu Chuang Yu Shao-Qing Chen Xue-Fei Miao Lin-Feng Peng Chao-Chao Wei Chong-Xuan Liu Shi-Jie Cheng Jia Xie State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430074China School of Materials Huazhong University of Science and TechnologyWuhan 430074China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Key Laboratory of Advanced Metallic and Intermetallic Materials Technology School of Materials Science and EngineeringNanjing University of Science and TechnologyNanjing 210094China School of Environmental Science and Engineering Southern University of Science and TechnologyShenzhen 518055China

All-solid-state Li-Se battery shows great potential as a candidate for next-generation energy storage devices due to its high energy density and ***,the low ionic conductivity of the solid electrolytes and large volume changes of Se active materials are two of the major issues that limit its ***,a simple solid-state reaction method is applied to synthesize chlorine-rich argyrodite Li_(5.5)PS_(4.5)CI_(1.5)electrolyte with high conductivity of 6.25 mS·cm^(-1)at room *** nanotube(CNT)is introduced as the host for Se to obtain Se/CNT composite with both enhanced electronic conductivity and lower volume expansion during the electrochemical reaction ***-solid-state Li-Se battery using Li_(5.5)PS_(4.5)CI_(1.5)as solid electrolyte combined with Se/CNT cathode and Li-In anode shows a discharge capacity of 866 mAh·g-1for the 2nd cycle under0.433 mA·cm-2at room ***,the assembled battery delivers a high discharge capacity of1026 mAh·g^(-1)for the 2nd cycle when cycled at the same current density at 60℃and maintains a discharge capacity of 380 mAh·g^(-1)after 150 *** to the high Li-ion conductivity of Li_(5.5)PS_(4.5)CI_(1.5)electrolyte,the assembled battery displays a high discharge capacity of 344 mAh·g^(-1)under 0.113 mA·cm^(-2)at-20℃C and remains 66.1%after200 *** addition,this all-solid-state Li-Se battery shows ultralong cycling performances up to 1000 cycles under 0.433 mA·cm^(-2)at-20℃.This work offers the design clue to fabricate the all-solid-state Li-Se battery workable at different operating temperatures with an ultralong cycling life.

关键词： Lithium argyrodite Chlorine-rich All-solidstate Li-Se batteries Operating temperatures Long cycling performances

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Design and applications of carbon dots-based ratiometric fluorescent probes:A review

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Nano Research 2023年第1期16卷 1064-1083页

作者： Bin-Bin Chen Meng-Li Liu Ya-Ting Gao Shuai Chang Ruo-Can Qian Da-Wei Li Key Laboratory for Advanced Materials Shanghai Key Laboratory of Functional Materials ChemistryFrontiers Science Center for Materiobiology&Dynamic ChemistrySchool of Chemistry&Molecular EngineeringEast China University of Science and TechnologyShanghai 200237China School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhenShenzhen 518172China Department of Chemistry Laboratory of Advanced MaterialsShanghai Key Lab of Molecular Catalysis and Innovative Materials and State Key Laboratory of Molecular Engineering of PolymersCollege of Chemistry and MaterialsFudan UniversityShanghai 200433China

Ratiometric fluorescence(FL)probes can eliminate the background interference and provide more accurate detection results than single emission intensity-based ***,carbon dots(CDs)-based ratiometric FL probes have received extensive research attention due to their excellent biocompatibility,water solubility,and multi-emission *** this review,we firstly summarize the construction strategies of CDs-based ratiometric FL probes,including physical mixing,nanohybrid,and dual-emitting CDs ***,we classify the sensing types of CDs-based ratiometric FL probes into five categories according to the difference in spectral variation caused by analytes:“single-response-ON”,“single-response-OFF”,“doubleresponses-ON”,“double-responses-OFF”,and“double-responses-Reverse”***,a thorough overview of CDs-based ratiometric FL probe applications in ions,molecules,pH,and temperature sensing is *** believe this review can show the latest research progress of CDs-based ratiometric FL sensing fields and provide perspectives on future developments for the construction of CDs-based ratiometric FL probes and their potential applications.

关键词： carbon dots ratiometric fluorescent probes construction strategy sensing type a review

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Acoustical properties of a 3D printed honeycomb structure filled with nanofillers:Experimental analysis and optimization for emerging applications

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Defence technology（防务技术） 2024年第5期35卷 248-258页

作者： Jeyanthi Subramanian Vinoth kumar Selvaraj Rohan Singh Ilangovan S Naresh Kakur Ruban Whenish School of Mechanical Engineering Vellore Institute of TechnologyChennai600127Tamil NaduIndia Department of Mechanical Engineering SRM Institute of Science and TechnologyRamapuramChennai600089India Department of Chemical Engineering and Materials Science University of Southern CaliforniaLos Angeles90089USA Advanced Materials Research Centre Technology Innovation InstituteAbu Dhabi9639UAE Center for Biomaterials Cellular and Molecular TheranosticsVellore Institute of TechnologyVellore632014Tamil NaduIndia

The novelty of this research lies in the successful fabrication of a 3D-printed honeycomb structure filled with nanofillers for acoustic properties,utilizing an impedance tube setup in accordance with ASTM standard E *** Creality Ender-3,a 3D printer,was used for printing the honeycomb structures,and polylactic acid(PLA)material was employed for their *** organic,inorganic,and polymeric compounds within the composites were identified using fourier transformation infrared(FTIR)*** structure and homogeneity of the samples were examined using a field emission scanning electron microscope(FESEM).To determine the sound absorption coefficient of the 3D printed honeycomb structure,numerous samples were systematically developed using central composite design(CCD)and analysed using response surface methodology(RSM).The RSM mathematical model was established to predict the optimum values of each factor and noise reduction coefficient(NRC).The optimum values for an NRC of 0.377 were found to be 1.116 wt% carbon black,1.025 wt% aluminium powder,and 3.151 mm distance between parallel ***,the results demonstrate that a 3Dprinted honeycomb structure filled with nanofillers is an excellent material that can be utilized in various fields,including defence and aviation,where lightweight and acoustic properties are of great importance.

关键词： 3D printing Honeycomb structure Acoustics Field emission scanning electron microscope Response surface methodology

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Ultrastrong and ductile BCC high-entropy alloys with low-density via dislocation regulation and nanoprecipitates

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Journal of materials science & technology 2022年第15期110卷 109-116页

作者： Xuehui Yan Peter K.Liaw Yong Zhang Beijing Advanced Innovation Center of Materials Genome Engineering State Key Laboratory for Advanced Metals and MaterialsUniversity of Science and Technology BeijingBeijing 100083China Department of Materials Science and Engineering The University of TennesseeKnoxvilleTN 37996United States of America

The high strength is a typical advantage of body-centered-cubic high-entropy alloys(BCC–HEAs).However,brittleness and weak strain-hardening ability are still their Achilles'***,extraordinary strength together with good tensile ductility are achieved in(Zr_(0.5)Ti_(0.35)Nb_(0.15))_(100-x)Al_(x) alloys(at.%,x=10 and 20)at room *** low densities of less than 6 g/cm^(3)are exhibited in these *** nanoprecipitates and diversifying dislocation motions are the keys to achieving such salient *** is worth noting that the tensile strength of 1.8 GPa in(Zr_(0.5)Ti_(0.35)Nb_(0.15))_(80)Al_(20)alloy is a record-high value known in reported BCC–HEAs,as well as a tensile strain over 8%.Furthermore,the maximum strain of~25%in(Zr_(0.5)Ti_(0.35)Nb_(0.15))_(90)Al_(10)alloy can challenge existing limit value,and is accompanied with a tensile strength of 1.2 *** current work does not only provide novel ultra-strong and tough structural materials with low density,but also sheds new light on designing BCC–HEAs with attractive performances and strain-hardening ability.

关键词： High-entropy alloys Mechanical properties Dislocation Nanoprecipitates Strain hardening

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Boosting ultra-wide temperature dielectric stability of multilayer ceramic capacitor through tailoring the combination types of polar nanoregions

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Journal of Materiomics 2024年第4期10卷 751-761页

作者： Jiacheng Liu Kaibiao Xi Beibei Song Huarong Cheng Xiaole Yu Mupeng Zheng Mankang Zhu Yudong Hou College of Materias Science and Engineering Key Laborutory of Advanced Functional Materials Education Ministry of China Beijing University of TechnologyBeijing100124China Materials R&D Department Beijing Yuanliu Hongyuan Eletronic Technology CompanyLtdBeijing102600China

With the rapid development of space exploration and new energy vehicles,it is urgent to build ultra-wide temperature multilayer ceramic capacitors(UWT MLCCs)to match electronic circuits that can withstand harsh environmental *** ferroelectrics with diffuse phase transition feature are potential dielectrics for the construction of UWT ***,how to ensure high dielectric constant together with low dielectric loss in the wide temperature region is still a big ***,the above difficulties are addressed by tailoring the combination types of polar nanoregions(PNRs)in the(1-x)(0.8Na_(0.5)Bi_(0.5)TiO_(3)-0.2K_(0.5)Bi_(0.5)TiO_(3))-xNaTaO3(NBT-KBT-xNT)*** with PNRS types of P4bm+R3c and P4bm+Pbnm,the combination type of P4bm+Pbnm+R3c PNRs in NBT-KBT-0.31NT is the most beneficial to obtain comprehensive excellent dielectric performance because it can balance the relationship between high dielectric constant and temperature stability over a wide temperature ***,by optimizing the laminating pressure and co-firing temperature to realize a tight interfacial structure between the dielectric layer and the Pt inner electrode,a record-high dielectric constant(er=(907%±15%))together with low dielectric loss(tan δ≤0.025)is achieved over an ultra-wide range from-61℃ to 306℃ for NBT-KBT-0.31 NT MLCC,demonstrating that tailoring the combination types of PNRs is a powerful strategy in designing UWT MLCC dielectrics.

关键词： Lead-free dielectrics Ultra-wide temperature Multilayer ceramic capacitor Polar nanoregion

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Machine learning study on time-temperature-transformation diagram of carbon and low-alloy steel

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Journal of Iron and Steel Research International 2023年第5期30卷 1032-1041页

作者： Xiao-ya Huang Biao Zhang Qiang Tian Hong-hui Wu Bin Gan Zhong-nan Bi Wei-hua Xue Asad Ullah Hao Wang School of Materials Science and Engineering University of Science and Technology BeijingBeijing 100083China School of Materials Science and Engineering Beihang UniversityBeijing 100191China High Temperature Materials Research Division Central Iron and Steel Research InstituteBeijing 100081China Beijing Advanced Innovation Center for Materials Genome Engineering Collaborative Innovation Center of Steel TechnologyUniversity of Science and Technology BeijingBeijing 100083China Beijing Key Laboratory of Advanced High Temperature Materials Central Iron and Steel Research InstituteBeijing 100081China School of Materials Science and Engineering Liaoning Technical UniversityFuxin 123099LiaoningChina Department of Mathematical Sciences Karakoram International UniversityGilgit-Baltistan 15100Pakistan

Time-temperature-transformation(TTT)diagram plays a critical role in designing appropriate heat treatment process of steels by describing the relationship among holding time,temperature,and quantities of phase *** predictions for TTT diagrams of new steel rapidly and accurately is therefore of much practical importance,especially for costly and time-consuming experimental ***,TTT diagrams for carbon and low-alloy steels were predicted using machine learning *** commonly used machine learning(ML)algorithms,backpropagation artificial neural network(BP network),LibSVM,k-nearest neighbor,Bagging,and Random tree,were adopted to select appropriate models for the *** results illustrate that Bagging is the optimal model for the prediction of pearlite transformation and bainite transformation,and BP network is the optimal model for martensite ***,the ML framework composed of Bagging and BP network models was applied to predict the entire TTT ***,the ML models show superior performance on the prediction of testing samples than the commercial software JMatPro.

关键词： Time-temperature-transformation diagram Carbon steel Low-alloy steel Machine learning Prediction framework

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MOF-mediated synthesis of novel PtFeCoNiMn high-entropy nanoalloy as bifunctional oxygen electrocatalysts for zinc-air battery

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Nano Research 2024年第6期17卷 5288-5297页

作者： Mingkuan Xie Xin Xiao Duojie Wu Cheng Zhen Chunsheng Wu Wenjuan Wang Hao Nian Fayan Li Meng Danny Gu Qiang Xu Shenzhen Key Laboratory of Micro/Nano-Porous Functional Materials(SKLPM) Shenzhen 518055China Department of Chemistry Southern University of Science and TechnologyShenzhen 518055China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China SUSTech-Kyoto University Advanced Energy Materials Joint Innovation Laboratory(SKAEM-JIL) Shenzhen 518055China Key University Laboratory of Highly Efficient Utilization of Solar Energy and Sustainable Development of Guangdong Southern University of Science and TechnologyShenzhen 518055China Eastern Institute for Advanced Study Eastern Institute of TechnologyNingbo 315200China

High-entropy alloy(HEA)-based materials are expected to be promising oxygen electrocatalysts due to their exceptional *** electronic structure regulation of HEAs plays a pivotal role in enhancing their elctrocatalytic ***,PtFeCoNiMn nanoparticles(NPs)with subtle lattice distortions are constructed on metal-organic framework-derived nitrogen-doped carbon by an ultra-rapid Joule heating *** to the modulated electronic structure and the inherent cocktail effect of HEAs,the as-synthesized PtFeCoNiMn/NC exhibits superior bifunctional electrocatalytic performance with a positive half-wave potential of 0.863 V *** hydrogen electrode(RHE)for oxygen reduction reaction and a low overpotential of 357 mV at 10 mA·cm^(-2)for oxygen evolution *** assembled quasi-solid-state zinc-air battery using PtFeCoNiMn/NC as air electrode shows a high peak power density of 192.16 mW·cm^(-2),low charge−discharge voltage gap,and excellent durability over 500 cycles at 5 mA·cm^(-2).This work demonstrates an effective route for rational design of bifunctional nanostructured HEA electrocatalysts with favorable electronic structures,and opens up a fascinating directions for energy storage and conversion,and beyond.

关键词： oxygen reduction reaction oxygen evolution reaction high-entropy nano-alloy zinc-air battery

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