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Designing carboxymethyl cellulose based hydrogel electrolyte membranes enhanced by inorganic nanoparticle toward stable zinc anode

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Green Energy & Environment 2025年第3期10卷 537-550页

作者： Xiangye Li Yuan Li Yu Jiang Dahui Wang Fen Ran State Key Laboratory of Advanced Processing and Recycling of Non-ferrous Metals Department of Polymeric Materials EngineeringSchool of Material Science and EngineeringLanzhou University of TechnologyLanzhou730050China

Aqueous zinc metal batteries have garnered substantial attention ascribing to affordability,intrinsic safety,and environmental benignity Nevertheless,zinc metal batteries yet are challenged with potential service life issues resulted from dendrites and side *** this paper,a strategy of nanoparticles doped hydrogel is proposed for constructing carboxymethyl cellulose/graphite oxide hybrid hydrogel electrolyte membranes with exceptional ionic conductivity,anti-swelling property,and simultaneously addressing the dendrites and parasitic *** pivotal functions of the carboxymethyl cellulose/graphite oxide hydrogel electrolyte in mitigating hydrogen evolution and fostering accelerated Zn deposition have been elucidated based on principles of thermodynamic and reaction *** carboxymethyl cellulose/graphite oxide hydrogel electrolyte endows exceptional cycling longevity (800 h at 1 mA cm^(-2)/1 mAh cm^(-2)) for Znjj Zn battery,as well as high Coulombic efficiency for Znjj Cu battery (averagely 99.14%within 439 cycles at 1 mA cm^(-2)/1 mAh cm^(-2)).The assembled Znjj NH_(4)V_(4)O_(10)battery delivers a high reversible specific capacity of 328.5 mAh g^(-1)at 0.1 A g^(-1).Moreover,the device of Znjj NH_(4)V_(4)O_(10)pouch battery remains operational under severe conditions like bending and *** work provides valuable reference in developing inorganic nanoparticle hybrid hydrogel electrolyte for realizing high-performance zinc metal batteries.

关键词： Carboxymethyl cellulose Graphite oxide Hydrogel electrolyte Anti-swelling

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Polymer composites designed with 3D fibrous CNT“tracks”achieving excellent thermal conductivity and electromagnetic interference shielding efficiency

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Nano Research 2023年第8期16卷 11411-11421页

作者： Gui Yang Liangchun Zhou Mingjie Wang Tiantian Xiang Duo Pan Jingzhan Zhu Fengmei Su Youxin Ji Chuntai Liu Changyu Shen National Engineering Research Center for Advanced Polymer Processing Technology The Key Laboratory of Material Processing and Mold of Ministry of EducationCollege of Materials Science and EngineeringZhengzhou UniversityZhengzhou 450002China

The rapid improvement in the running speed,transmission efficiency,and power density of miniaturized devices means that multifunctional flexible composites with excellent thermal management capability and high electromagnetic interference(EMI)shielding performance are urgently ***,inspired by the fibrous pathways of the human nervous system,a“core–sheath”fibers structured strategy was proposed to prepare thermoplastic polyurethane/polydopamine/carbon nanotube(TPU/PDA/CNT)composites film with thermal management capability and EMI shielding ***,TPU@PDA@CNT fibers with CNT shell were prepared by a facile polydopamine-assisted coating on electrospun TPU ***,TPU/PDA/CNT composites with three-dimensional(3D)fibrous CNT“tracks”are obtained by a hot-pressing process,where CNTs distributed on adjacent fibers are compactly *** fabricated TPU/PDA/CNT composites exhibit a high in-plane thermal conductivity(TC)of 9.6 W/(m·K)at low CNT loading of 7.6 wt.%.In addition,it also presents excellent mechanical properties and excellent EMI shielding effectiveness of 48.3 dB as well as multi-source driven thermal management ***,this study provides a simple yet scalable technique to prepare composites with advanced thermal management and EMI shielding performance to develop new-generation wireless communication technologies and portable intelligent electronic devices.

关键词： composites three-dimensional(3D)fibrous carbon nanotube(CNT)“tracks” in-plane thermal conductivity(TC) electromagnetic interference(EMI)shielding multi-source driven thermal management

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Phosphorus incorporation-induced adsorption behavior modulation for carbon cathodes enables ultrastable and high-energy aqueous Zn-ion hybrid capacitors

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science China Chemistry 2025年第3期68卷 900-907页

作者： Lai Yu Xiaoyue He Rong Liu Guanglin Wan Xinyi Ma Anqiang Pan Liang Shi Genqiang Zhang Hefei National Research Center for Physical Sciences at the Microscale CAS Key Laboratory of Material for Energy ConversionDepartment of Material Science and EngineeringUniversity of Science and Technology of ChinaHefei 230026China School of Materials and Engineering Xinjiang UniversityUrumqi 830046China

The aqueous zinc ions hybrid capacitors(ZHCs)have great potential for future energy storage devices by their high safety and low cost merits,more importantly,it could combine the advantages of batteries and supercapacitors with high energy density and power output,***,the development of reliable cathodes is still a challenge with the unsatisfactory cycling stability and limited reaction kinetic,severely restricting its further commercial ***,we present phosphorus functionalized nitrogen-doped hierarchical porous carbon nanosheets(PN-HPCNS),where the P incorporation could effectively enhance the electronic transfer kinetics and ion adsorption capability to achieve superior zinc-ion storage *** asprepared PN-HPCNS cathode-based ZHC exhibits a high energy and power density(169.1 Wh kg^(-1)/68 W kg^(-1),15,840 W kg^(-1)/30.8 Wh kg^(-1))and long cycling lifespans more than 20,000 cycles with 92.0%capacity *** characterizations coupled with kinetics studies indicate that phosphorus modification is crucial to superior zinc ion storage,enabling PN-HPCNS with favorable reaction kinetics,promoting ion adsorption by providing more active ***,the theoretical calculation reveals that the phosphorus modification could enhance the adsorption ability,contributing to the superior ZHCs performance of PN-HPCNS.

关键词： carbon zinc ion hybrid capacitors cathode nanosheet density function theory

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Microstructural evolution and properties of the Cu-Cr-Ti alloys after cold deformation and subsequent aging treatment

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Progress in Natural science:materials International 2024年第6期34卷 1258-1266页

作者： Xueqin Dai Shuguo Jia Yanjun Zhou Yingxuan Ma Zhenpeng Xiao Huiwen Guo Xiao Cao Yuduo Fu Kexing Song Zongye Ding School of Material Science and Engineering Henan University of Science and Technology Provincial and Ministerial Co-construction Collaborative Innovation Center of Nonferrous New Materials and Advanced Processing Technology Chinalco Luoyang Copper Processing Co Ltd School of Mechatronic Engineering and Automation Foshan University National United Engineering Laboratory for Advanced Bearing Tribology Henan University of Science and Technology

The increasingly desirable mechanical and physical properties limits the application of traditional Cu-Cr alloys,and deserves the compositional design and processing optimization of Cu-Cr-Ti alloys. The effects of cold deformation and aging treatment on the microstructures and properties of the Cu-0.2Cr-0.08Ti alloys were investigated. The shapes of precipitates and evolution of dislocations in the specimens with increasing deformation amounts and aging times was uncovered, and the strengthening mechanisms of Cu-Cr-Ti alloys were elucidated by using TEM and HRTEM analysis. When the deformation amount is not higher than 40 %, the increased deformation amounts increases the dislocation density in the Cu-0.2Cr-0.08Ti alloy, promoting the formation of dislocation cell and dislocation tangles with small size. The precipitation of fine Cr particles coherent with Cu matrix is accelerated, accompanied by the enhancement of microhardness and electrical *** Cu-0.2Cr-0.08Ti alloy with 40 % deformation amounts after aging at 480°C for 1 h has the optimal comprehensive properties, which is related to the increasing dislocation density, the refinement of Cu grains and the precipitation of Cr particles. The enhanced strength of Cu-0.2Cr-0.08Ti alloy with 40 % deformation amounts after aging at 480°C for 1 h is attributed to the solute strengthening of solute atoms, precipitate strengthening of fine Cr particles, dislocations strengthening and grain boundary strengthening mechanisms.

关键词： Cu-Cr-Ti alloy Cold deformation Aging treatment Microstructures Precipitates

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Metallized polymer current collector as“stress acceptor”for stable micron-sized silicon anodes

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Journal of Energy Chemistry 2025年第2期101卷 786-794,I0017页

作者： Ziyi Cao Haoteng Sun Yi Zhang Lixia Yuan Yaqi Liao Haijin Ji Shuaipeng Hao Zhen Li Long Qie Yunhui Huang State Key Laboratory of Material Processing and Die&Mold Technology School of Materials Science and EngineeringHuazhong University of Science and TechnologyWuhan 430074HubeiChina Department of Chemistry Brown UniversityProvidence RI 02912United States

Micron-sized silicon(μSi)is a promising anode material for next-generation lithium-ion batteries due to its high specific capacity,low cost,and abundant ***,the volume expansion that occurs during cycling leads to the accumulation of undesirable stresses,resulting in pulverization of silicon microparticles and shortened lifespan of the ***,a composite film of Cu-PET-Cu is proposed as the current collector(CC)forμSi anodes to replace the conventional Cu ***-PET-Cu CC is prepared by depositing Cu on both sides of a polyethylene terephthalate(PET)*** PET layer promises good ductility of the film,permitting the Cu-PET-Cu CC to accommodate the volumetric changes of silicon microparticles and facilitates the stress release through ductile *** a result,theμSi electrode with Cu-PET-Cu CC retains a high specific capacity of 2181 mA h g^(-1),whereas theμSi electrode with Cu CC(μSi/Cu)exhibits a specific capacity of 1285 mA h g^(-1)after 80 *** stress relieving effect of CuPET-Cu was demonstrated by in-situ fiber optic stress monitoring and multi-physics *** work proposes an effective stress relief strategy at the electrode level for the practical implementation ofμSi anodes.

关键词： Micron-sized Si anodes Metallized polymer current collector Stress relieving Electrode design

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Three-dimensional lightweight melamine foams modified by MXene sheets and CoNi alloys towards multifunctional microwave absorption

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Nano Research 2025年第2期18卷 377-389页

作者： Nannan Wu Zhengying Shen Yitao Ma Zhizheng Wu Chuanxin Hou Sijie Guo Jian Tian Jiurong Liu School of Material Science and Engineering Shandong University of Science and TechnologyQingdao 266590China School of Mathematics and Systems Science Shandong University of Science and TechnologyQingdao 266590China School of Environmental and Material Engineering Yantai UniversityYantai 264005China Department of Chemical&Biomolecular Engineering University of TennesseeKnoxvilleTN 37996USA Key Laboratory for Liquid-Solid Structural Evolution and Processing of Materials Ministry of Education and School of Materials Science and EngineeringShandong UniversityJinan 250061China

Taking the increasing issue of electromagnetic waves(EMW)pollution and the necessity for applications in extreme environments,there is a pressing requirement to create multifunctional microwave absorption materials(MAMs)to meet the current *** this work,we achieved the successful combination of MXene sheets and metal organic framework(MOFs)derived CoNi@C magnetic alloys onto the three dimensional(3D)melamine foam(MF)skeleton using vacuum impregnation and electrostatic self-assembly *** obtained MF@MXene/CoNi@C composite foams achieved outstanding MA performance,with an optimal reflection loss(RL)value of–24.1 dB and a maximum effective absorption bandwidth(EAB)of 6.88 GHz at a thickness of 1.68 mm,effectively covering the whole Ku *** superior MA performance is ascribed to the composite foams’multi-component architecture,distinctive 3D porous structure,and the synergistic impact of multiple loss ***,the MF@MXene/CoNi@C composite foams demonstrate exceptional photothermal conversion,thermal insulation,and infrared stealth capabilities,effectively coping with the demands of applications in extreme *** work serves as a valuable resource and source of inspiration for the development of lightweight broadband,multifunctional efficient MAMs.

关键词： multifunctional microwave absorption MXene thermal insulation infrared stealth

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State-of-art of in situ observations of inclusion agglomeration at steel/Ar and steel/slag interfaces:a review of recent development on experimental and theoretical studies

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Journal of Iron and Steel Research International 2025年第2期32卷 315-333页

作者： Yi Wang Jian-xun Fu Deepoo Kumar Qiang Wang Hong-liang Yang Wang-zhong Mu Center for Advanced Solidification Technology(CAST) School of Materials Science and EngineeringShanghai UniversityShanghai 200444China Department of Materials Science and Engineering KTH Royal Institute of TechnologyStockholm 10044Sweden Engineering Materials Division of Materials ScienceDepartment of Engineering Science and MathematicsLuleåUniversity of TechnologyLuleå 97187Sweden Department of Metallurgical Engineering and Materials Science IIT BombayPowaiMumbaiIndia Key Laboratory of Electromagnetic Processing of Materials(Ministry of Education) Northeastern UniversityShenyang 110819LiaoningChina ABB Metallurgy Västerås 72136Sweden

Cleanliness control of advanced steels is of vital importance for quality control of the *** order to understand and control the inclusion removal during refining process in molten steel,its motion behaviors at the multiple steel/gas/slag interfaces have attracted the attention much of metallurgical *** recent development of the agglomeration of non-metallic inclusions at the steel/Ar and steel/slag interfaces has been summarized,and both the experimental as well as theoretical works have been *** terms of in situ observation of high-temperature interfacial phenomena in the molten steel,researchers utilized high-temperature confocal laser scanning microscopy to observe the movement of more types of inclusions at the interface,i.e.,the investigated inclusion is no longer limited to Al_(2)O_(3)-based inclusions but moves forward to rare earth oxides,MgO-based oxides,*** terms of theoretical models,especially the model of inclusions at the steel/slag interface,the recent development has overcome the limitations of the assumptions of Kralchevsky-Paunov model and verified the possible errors caused by the model assumptions by combining the water model and the physical *** but not least,the future work in this topic has been suggested,which could be in combination of thermal physical properties of steels and slag,as well as utilize the artificial intelligence-based methodology to implement a comprehensive inclusion motion behaviors during a comprehensive metallurgical process.

关键词： Inclusion movement Steel/Ar interface Steel/slag interface In situ observation

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High micropore-utilization carbon aerogel with controlled nanostructures via adjusting aggregation state of polyacrylonitrile for energy storage systems

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SusMat 2024年第4期4卷 27-38页

作者： Yuanyou Peng Yihan Fu Meimei Yu Lei Zhao Huanzhong Zeng Shengtao Niu Jie Zhang Junlong Chen Guang Liu Youzhi Wu Fen Ran State Key Laboratory of Advanced Processing and Recycling of Non-Ferrous Metals Department of Polymeric Materials EngineeringSchool of Material Science and EngineeringLanzhou University of TechnologyLanzhouChina

Designing and optimizing the pore structure of porous carbon electrodes is essen-tial for diverse energy storage *** this study,an innovative approach spray phase-inversion strategy was developed for the rapid and efficient fabri-cation of controlled porous carbon ***,the aggregation structure of polyacrylonitrile is controlled by adjusting the Hansen’s solubility parameter,thereby regulating the electrode material ***,the theoretical analysis of the spray phase-inversion process revealed that this regulation pro-cess is jointly regulated by solvent hydrodynamic diameter and phase-inversion *** optimization,a novel porous carbon material was obtained that exhibited excellent performance as an electrode *** utilized in supercapacitors for energy storage,it demonstrated a high specific capacitance of 373.1 F g^(-1) in a 6 M KOH electrolyte ***,it has been observed that the preparation strategy for porous electrodes offers notable advan-tages in terms of excellent designability,broad universality,simplicity,and high efficiency,thereby holding promise for large-scale fabrication of diverse porous electrode materials and various types of electrodes for diverse energy storage applications.

关键词： aggregation structure electrode materials phase inversion porous carbon supercapacitors

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Distribution pattern of acoustic and streaming field during multi-source ultrasonic melt treatment process

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China Foundry 2023年第5期20卷 452-460页

作者： Xiao-gang Fang Qi Wei Tian-yang Zhang Ji-guang Liu You-wen Yang Shu-lin Lü Shu-sen Wu Yi-qing Chen School of Materials Science and Engineering Hefei University of TechnologyHefei 230009China Engineering Research Center of High-Performance Copper Alloy Materials and Processing Ministry of EducationHefei 230009China State Key Laboratory of Material Processing and Die&Mould Technology Huazhong University of Science and TechnologyWuhan 430074China

The ultrasonic melt treatment(UMT)is widely used in the fields of casting and ***,there are certain drawbacks associated with the conventional process of single-source ultrasonic(SSU)treatment,such as the fast attenuation of energy and limited range of *** this study,the propagation models of SSU and four-source ultrasonic(FSU)in Al melt were respectively established,and the distribution patterns of acoustic and streaming field during the ultrasonic treatment process were investigated by numerical simulation and physical *** simulated results show that the effective cavitation zone is mainly located in a small spherical region surrounding the end of ultrasonic horn during the SSU treatment *** the FSU is applied,the effective cavitation zone is obviously expanded in the *** increases at first and then decreases with increasing the vibration-source spacing(Lv)from 30 mm to 100 ***,when the Lv is 80 mm,the area of effective cavitation zone reaches the largest,indicating the best effect of ***,the acoustic streaming level and flow pattern in the melt also change with the increase of *** the Lv is 80 mm,both the average flow rate and maximum flow rate of the melt reach the highest,and the flow structure is more stable and uniform,with the typical morphological characteristics of angular vortex,thus significantly expanding the range of acoustic *** accuracy of the simulation results was verified by physical experiments of glycerol aqueous solution and tracer particles.

关键词： four-source ultrasound acoustic cavitation streaming field vibration-source spacing

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High‑Performance p‑Type Bi_(2)Te_(3)‑Based Thermoelectric materials with a Wide Temperature Range Obtained by Direct Sb Doping

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Acta Metallurgica Sinica(English Letters) 2025年第5期38卷 849-858页

作者： Xicheng Guan Zhiyuan Liu Ni Ma Zhou Li Juan Liu Huiyan Zhang Hailing Li Qian Ba Junjie Ma Chuangui Jin Ailin Xia Advanced Ceramics Research Center School of Materials Science and EngineeringAnhui University of TechnologyMaanshan 243002China Institute of Energy Hefei Comprehensive National Science Center(Anhui Energy Laboratory)Hefei 230051China School of Chemistry and Materials Science University of Science and Technology of ChinaHefei 230026China School of Materials Science and Engineering Anhui UniversityHefei 230601China Anhui Key Lab of Metal Material and Processing Anhui University of TechnologyMa’anshan 243002China

Doping modification is one of the most effective ways to optimize the thermoelectric properties of Bi_(2)Te_(3)-based alloys.P-type Bi_(2−x)Sb_(x)Te_(3) thermoelectric materials have been successfully prepared by direct Sb doping *** can be found that doping Sb into Bi_(2)Te_(3) lattice array for Bi-site replacement facilitates the generation of Sb′Te anti-site *** anti-site defects can increase the hole concentration and optimize electrical transport properties of Bi_(2−x)Sb_(x)Te_(3) *** addition,the point defects induced by mass and stress fluctuations and the Sb impurities produced during the sintering process can enhance the multi-scale phonon scattering and reduce the lattice thermal *** a result,the Bi_(0.47)Sb_(1.63)Te_(3) sample has a maximum thermoelectric figure of merit ZT of 1.04 at 350 *** is worth noting that the bipolar effect of Bi_(2)Te_(3)-based alloys can be weakened with the increase of Sb *** Bi_(0.44)Sb_(1.66)Te_(3) sample has a maximum average ZT value(0.93)in the temperature range of 300–500 K,indicating that direct doping of Sb can broaden the temperature range corresponding to the optimal ZT *** work provides an idea for developing high-performance near room temperature thermoelectric materials with a wide temperature range.

关键词： Bi2Te3-based materials Sb doping Wide temperature range Thermoelectric properties

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