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Anisotropic node distortions in amorphous MOFs: Low-valent Zr sites as catalytic hotspots

Chem 2025年

作者： Till Schertenleib Mehrdad Asgari Beatriz Mouriño Vikram V. Karve Timo M.O. Felder Dragos Stoian Volodymyr Bon Jian Hao Andres Ortega-Guerrero Emad Oveisi Kumar Varoon Agrawal Berend Smit Stefan Kaskel Simon J.L. Billinge Wendy L. Queen Laboratory for Functional Inorganic Materials (LFIM) Institut des Sciences et Ingénierie Chimiques École Polytechnique Fédérale de Lausanne (EPFL) Rue de l’Industrie 17 Sion 1950 Switzerland Departement of Chemical Engineering and Biotechnology University of Cambridge Cambridge CB3 0AS UK Lucy Cavendish College University of Cambridge Cambridge CB3 0BU United Kingdom Laboratory of Molecular Simulation (LSMO) Institut des Sciences et Ingénierie Chimiques École Polytechnique Fédérale de Lausanne (EPFL) Rue de l’Industrie 17 Sion 1950 Switzerland Swiss-Norwegian Beamlines European Synchrotron Research Facilities (ESRF) Grenoble BP 220 France Chair of Inorganic Chemistry I Technische Universität Dresden Dresden 01062 Germany Laboratory of Advanced Separations (LAS) Institut des Sciences et Ingénierie Chimiques École Polytechnique Fédérale de Lausanne (EPFL) Rue de l’Industrie 17 Sion 1950 Switzerland nanotech@surfaces Laboratory Empa–Swiss Federal Laboratories for Materials Science and Technology Dübendorf 8600 Switzerland Interdisciplinary Centre for Electron Microscopy (CIME) École Polytechnique Fédérale de Lausanne (EPFL) Lausanne 1015 Switzerland Fraunhofer Institute for Material and Beam Technology IWS Dresden 01277 Germany Department of Applied Physics and Applied Mathematics Columbia University New York NY 10027 USA

We introduce a new approach to defect engineering in Zr-based metal-organic frameworks (Zr-MOFs), aiming to reduce Zr site valency while preserving high node connectivity. Using a rapid heat treatment (RHT) in humid air, oxygen vacancies (O-vacancies) were created in Dresden University of Technology (DUT)-67 through cluster dehydration. Unlike conventional defect engineering, aimed at creating missing-linker defects, this method breaks intra-cluster Zr- μ 3 O–Zr bonds, generating coordinatively unsaturated Zr (Zr cus ) sites. Pair distribution function (PDF) analysis, X-ray absorption spectroscopy (XAS), and density functional theory (DFT) calculations reveal that the O-vacancies lead to symmetry breaking, irreversible node distortions, and framework amorphization. This treatment converts 50% of metal sites to Zr cus sites, nearly doubling the catalytic activity of DUT-67 in glyoxal conversion to glycolic acid. DFT modeling and in situ PDF analysis highlight the dynamic behavior of Zr clusters under reaction conditions, suggesting a new avenue for defect engineering in Zr-MOFs to enhance catalytic performance.

关键词： amorphous MOFs Zr-oxo clusters pair distribution function O-vacancies defects catalysis metal-organic frameworks catalyst dehydroxylation coordinatively unsaturated metal sites SDG12: Responsible consumption and production

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On collisions times of 'self-sorting' interacting particles in one-dimension with random initial positions and velocities

arXiv

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arXiv 2017年

作者： Lega, Joceline Sethuraman, Sunder Young, Alexander L. Department of Mathematics University of Arizona Program in Applied Mathematics University of Arizona

We investigate a one-dimensional system of N particles, initially distributed with random positions and velocities, interacting through binary collisions. The collision rule is such that there is a time after which the N particles do not interact and become sorted according to their velocities. When the collisions are elastic, we derive asymptotic distributions for the final collision time of a single particle and the final collision time of the system as the number of particles approaches infinity, under different assumptions for the initial distributions of the particles' positions and velocities. For comparison, a numerical investigation is carried out to determine how a non-elastic collision rule, which conserves neither momentum nor energy, affects the median collision time of a particle and the median final collision time of the *** Codes 82C22, 62G30 (Primary) 82C23, 62-04, 62E20 (Secondary) Copyright © 2017, The Authors. All rights reserved.

关键词： Velocity

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Review of Particle Physics*

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Physical Review D 2024年第3期110卷 030001-030001页

作者： S. Navas C. Amsler T. Gutsche C. Hanhart J. J. Hernández-Rey C. Lourenço A. Masoni M. Mikhasenko R. E. Mitchell C. Patrignani C. Schwanda S. Spanier G. Venanzoni C. Z. Yuan K. Agashe G. Aielli B. C. Allanach J. Alvarez-Muñiz M. Antonelli E. C. Aschenauer D. M. Asner K. Assamagan H. Baer Sw. Banerjee R. M. Barnett L. Baudis C. W. Bauer J. J. Beatty J. Beringer A. Bettini O. Biebel K. M. Black E. Blucher R. Bonventre R. A. Briere A. Buckley V. D. Burkert M. A. Bychkov R. N. Cahn Z. Cao M. Carena G. Casarosa A. Ceccucci A. Cerri R. S. Chivukula G. Cowan K. Cranmer V. Crede O. Cremonesi G. D’Ambrosio T. Damour D. de Florian A. de Gouvêa T. DeGrand S. Demers Z. Demiragli B. A. Dobrescu M. D’Onofrio M. Doser H. K. Dreiner P. Eerola U. Egede S. Eidelman A. X. El-Khadra J. Ellis S. C. Eno J. Erler V. V. Ezhela A. Fava W. Fetscher B. D. Fields A. Freitas H. Gallagher T. Gershon Y. Gershtein T. Gherghetta M. C. Gonzalez-Garcia M. Goodman C. Grab A. V. Gritsan C. Grojean D. E. Groom M. Grünewald A. Gurtu H. E. Haber M. Hamel S. Hashimoto Y. Hayato A. Hebecker S. Heinemeyer K. Hikasa J. Hisano A. Höcker J. Holder L. Hsu J. Huston T. Hyodo Al. Ianni M. Kado M. Karliner U. F. Katz M. Kenzie V. A. Khoze S. R. Klein F. Krauss M. Kreps P. Križan B. Krusche Y. Kwon O. Lahav L. P. Lellouch J. Lesgourgues A. R. Liddle Z. Ligeti C.-J. Lin C. Lippmann T. M. Liss A. Lister L. Littenberg K. S. Lugovsky S. B. Lugovsky A. Lusiani Y. Makida F. Maltoni A. V. Manohar W. J. Marciano J. Matthews U.-G. Meißner I.-A. Melzer-Pellmann P. Mertsch D. J. Miller D. Milstead K. Mönig P. Molaro F. Moortgat M. Moskovic N. Nagata K. Nakamura M. Narain P. Nason A. Nelles M. Neubert Y. Nir H. B. O’Connell C. A. J. O’Hare K. A. Olive J. A. Peacock E. Pianori A. Pich A. Piepke F. Pietropaolo A. Pomarol S. Pordes S. Profumo A. Quadt K. Rabbertz J. Rademacker G. Raffelt M. Ramsey-Musolf P. Richardson A. Ringwald D. J. Robinson S. Roesler S. Rolli A. Romaniouk L. J Rosenberg J. L. Rosner G. Rybka M. G. Ryskin R. A. Ryutin B. Safdi Y. Sakai S. Sarkar F. Sauli O. Universidad de Granada Dpto. de Física Teórica y del Cosmos & C.A.F.P.E. Granada Spain Stefan Meyer Institute for Subatomic Physics Austrian Academy of Sciences Vienna Austria Universität Tübingen Institut für Theoretische Physik Tübingen Germany Forschungszentrum Jülich Institute for Advanced Simulation Jülich Germany IFIC—Instituto de Física Corpuscular Universitat de València—C.S.I.C. Valencia Spain CERN European Organization for Nuclear Research Genève Switzerland INFN Sezione di Cagliari Monserrato Italy Institut für Experimentalphysik 1 Ruhr-Universität Bochum Bochum Germany Indiana University Department of Physics Bloomington IN United States of America Università di Bologna and INFN Dip. Scienze per la Qualità della Vita Rimini Italy HEPHY Vienna Austria University of Tennessee Department of Physics and Astronomy Knoxville TN United States of America University of Liverpool Department of Physics Liverpool United Kingdom INFN Sezione di Pisa Pisa Italy Institute of High Energy Physics Chinese Academy of Sciences Beijing China University of Maryland Department of Physics College Park MD United States of America Università degli Studi di Roma “Tor Vergata” Rome Italy Department of Applied Mathematics and Theoretical Physics University of Cambridge Cambridge United Kingdom Instituto Galego de Física de Altas Enerxías (IGFAE) & Dept. Física de Partículas Universidade de Santiago de Compostela Santiago de Compostela Spain Lab. Nazionali di Frascati dell’INFN Frascati Italy Brookhaven National Laboratory Nuclear and Particle Physics Directorate Upton NY United States of America University of Oklahoma Department of Physics and Astronomy Norman OK United States of America University of Louisville Louisville KY United States of America Physics Division Universität Zürich Physik-Institut Zürich Switzerland Ohio State University Department of Physics Columbus OH United States of America INFN and Dipartimento di Fisica e Astronomia Universit

The Review summarizes much of particle physics and cosmology. Using data from previous editions, plus 2,717 new measurements from 869 papers, we list, evaluate, and average measured properties of gauge bosons and the recently discovered Higgs boson, leptons, quarks, mesons, and baryons. We summarize searches for hypothetical particles such as supersymmetric particles, heavy bosons, axions, dark photons, etc. Particle properties and search limits are listed in Summary Tables. We give numerous tables, figures, formulae, and reviews of topics such as Higgs Boson Physics, Supersymmetry, Grand Unified Theories, Neutrino Mixing, Dark Energy, Dark Matter, Cosmology, Particle Detectors, Colliders, Probability and Statistics. Most of the 120 reviews are updated, including many that are heavily revised.

关键词： Particle phenomena Baryons Hypothetical particles Leptons Mesons Particle properties Particle data analysis

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Measurement of the inclusive tt¯ production cross section in the lepton+jets channel in pp collisions at s=7 TeV with the ATLAS detector using support vector machines

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Physical Review D 2023年第3期108卷 032014-032014页

作者： M. Aaboud G. Aad B. Abbott D. C. Abbott D. K. Abhayasinghe S. H. Abidi O. S. AbouZeid N. L. Abraham H. Abramowicz H. Abreu Y. Abulaiti B. S. Acharya S. Adachi L. Adam C. Adam Bourdarios L. Adamczyk L. Adamek J. Adelman M. Adersberger A. Adiguzel T. Adye A. A. Affolder Y. Afik C. Agapopoulou M. N. Agaras A. Aggarwal C. Agheorghiesei J. A. Aguilar-Saavedra F. Ahmadov G. Aielli S. Akatsuka T. P. A. Åkesson E. Akilli A. V. Akimov K. Al Khoury G. L. Alberghi J. Albert M. J. Alconada Verzini S. Alderweireldt M. Aleksa I. N. Aleksandrov C. Alexa D. Alexandre T. Alexopoulos M. Alhroob B. Ali G. Alimonti J. Alison S. P. Alkire C. Allaire B. M. M. Allbrooke B. W. Allen P. P. Allport A. Aloisio A. Alonso F. Alonso C. Alpigiani A. A. Alshehri M. I. Alstaty M. Alvarez Estevez B. Alvarez Gonzalez D. Álvarez Piqueras M. G. Alviggi Y. Amaral Coutinho A. Ambler L. Ambroz C. Amelung D. Amidei S. P. Amor Dos Santos S. Amoroso C. S. Amrouche F. An C. Anastopoulos N. Andari T. Andeen C. F. Anders J. K. Anders A. Andreazza V. Andrei C. R. Anelli S. Angelidakis I. Angelozzi A. Angerami A. V. Anisenkov A. Annovi C. Antel M. T. Anthony M. Antonelli D. J. A. Antrim F. Anulli M. Aoki J. A. Aparisi Pozo L. Aperio Bella G. Arabidze J. P. Araque V. Araujo Ferraz R. Araujo Pereira A. T. H. Arce F. A. Arduh J-F. Arguin S. Argyropoulos J.-H. Arling A. J. Armbruster L. J. Armitage A. Armstrong O. Arnaez H. Arnold G. Artoni S. Artz S. Asai N. A. Asbah E. M. Asimakopoulou L. Asquith K. Assamagan R. Astalos R. J. Atkin M. Atkinson N. B. Atlay H. Atmani K. Augsten G. Avolio R. Avramidou M. K. Ayoub A. M. Azoulay G. Azuelos A. E. Baas M. J. Baca H. Bachacou K. Bachas M. Backes F. Backman P. Bagnaia H. Bahrasemani A. J. Bailey V. R. Bailey J. T. Baines M. Bajic C. Bakalis O. K. Baker P. J. Bakker D. Bakshi Gupta S. Balaji E. M. Baldin P. Balek F. Balli W. K. Balunas J. Balz E. Banas A. Bandyopadhyay Sw. Banerjee A. A. E. Bannoura L. Barak W. M. Barbe E. L. Barberio D. Barberis M. Barbero T. Barillari M-S. Barisits J. Barkeloo T. Barklow R. Barnea S. L. LPMR Faculté des Sciences Université Mohamed Premier Oujda Morocco CPPM Aix-Marseille Université CNRS/IN2P3 Marseille France Homer L. Dodge Department of Physics and Astronomy University of Oklahoma Norman Oklahoma USA Department of Physics University of Massachusetts Amherst Massachusetts USA Department of Physics Royal Holloway University of London Egham United Kingdom Department of Physics University of Toronto Toronto ON Canada Niels Bohr Institute University of Copenhagen Copenhagen Denmark Department of Physics and Astronomy University of Sussex Brighton United Kingdom Raymond and Beverly Sackler School of Physics and Astronomy Tel Aviv University Tel Aviv Israel Department of Physics Technion Israel Institute of Technology Haifa Israel High Energy Physics Division Argonne National Laboratory Argonne Illinois USA INFN Gruppo Collegato di Udine Sezione di Trieste Udine Italy ICTP Trieste Italy International Center for Elementary Particle Physics and Department of Physics University of Tokyo Tokyo Japan Institut für Physik Universität Mainz Mainz Germany IJCLab Université Paris-Saclay CNRS/IN2P3 91405 Orsay France AGH University of Science and Technology Faculty of Physics and Applied Computer Science Krakow Poland Department of Physics Northern Illinois University DeKalb Illinois United States of America Fakultät für Physik Ludwig-Maximilians-Universität München München Germany Department of Physics Bogazici University Istanbul Türkiye Particle Physics Department Rutherford Appleton Laboratory Didcot United Kingdom Santa Cruz Institute for Particle Physics University of California Santa Cruz Santa Cruz California USA LPC Université Clermont Auvergne CNRS/IN2P3 Clermont-Ferrand France Institute for Mathematics Astrophysics and Particle Physics Radboud University/Nikhef Nijmegen Netherlands Department of Physics Alexandru Ioan Cuza University of Iasi Iasi Romania Departamento de Física Teórica y del Cosmos Universidad de Granada

A measurement of the top quark pair-production cross section in the lepton+jets decay channel is presented. It is based on 4.6 fb−1 of s=7 TeV pp collision data collected during 2011 by the ATLAS experiment at the CERN Large Hadron Collider. A three-class, multidimensional event classifier based on support vector machines is used to differentiate tt¯ events from backgrounds. The tt¯ production cross section is found to be σtt¯=168.5±0.7(stat) −5.9+6.2(syst) −3.2+3.4(lumi) pb. The result is consistent with the Standard Model prediction based on QCD calculations at next-to-next-to-leading order.

关键词： Particle production Top quark Hadron colliders

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Epidemic spreading in localized environments with recurrent mobility patterns

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Physical Review E 2018年第5期97卷 052302-052302页

作者： Clara Granell Peter J. Mucha Departament de Física de la Matèria Condensada Universitat de Barcelona Martí i Franquès 1 E-08028 Barcelona Spain Universitat de Barcelona Institute of Complex Systems (UBICS) Universitat de Barcelona E-08007 Barcelona Spain Carolina Center for Interdisciplinary Applied Mathematics Department of Mathematics University of North Carolina Chapel Hill North Carolina 27599-3250 USA

The spreading of epidemics is very much determined by the structure of the contact network, which may be impacted by the mobility dynamics of the individuals themselves. In confined scenarios where a small, closed population spends most of its time in localized environments and has easily identifiable mobility patterns—such as workplaces, university campuses, or schools—it is of critical importance to identify the factors controlling the rate of disease spread. Here, we present a discrete-time, metapopulation-based model to describe the transmission of susceptible-infected-susceptible-like diseases that take place in confined scenarios where the mobilities of the individuals are not random but, rather, follow clear recurrent travel patterns. This model allows analytical determination of the onset of epidemics, as well as the ability to discern which contact structures are most suited to prevent the infection to spread. It thereby determines whether common prevention mechanisms, as isolation, are worth implementing in such a scenario and their expected impact.

关键词： Epidemic Spreading Bipartite graphs Monte Carlo methods SIS model

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The repertoire of mutational signatures in human cancer (vol 578, pg 94, 2020)

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NATURE 2023年第7948期614卷 E41-E41页

作者： Alexandrov, Ludmil B. Kim, Jaegil Haradhvala, Nicholas J. Huang, Mi Ni Ng, Alvin Wei Tian Wu, Yang Boot, Arnoud Covington, Kyle R. Gordenin, Dmitry A. Bergstrom, Erik N. Islam, S. M. Ashiqul Lopez-Bigas, Nuria Klimczak, Leszek J. McPherson, John R. Morganella, Sandro Sabarinathan, Radhakrishnan Wheeler, David A. Mustonen, Ville Getz, Gad Rozen, Steven G. Stratton, Michael R. Department of Cellular and Molecular Medicine Department of Bioengineering Moores Cancer Center University of California San Diego CA USA Wellcome Sanger Institute Wellcome Genome Campus Hinxton UK Department of Cellular and Molecular Medicine and Department of Bioengineering University of California San Diego La Jolla CA USA UC San Diego Moores Cancer Center San Diego CA USA University of California San Diego San Diego CA USA Broad Institute of MIT and Harvard Cambridge MA USA Center for Cancer Research Massachusetts General Hospital Boston MA USA Massachusetts General Hospital Boston MA USA Department of Pathology Massachusetts General Hospital Boston MA USA Harvard Medical School Boston MA USA Laboratory for Medical Science Mathematics RIKEN Center for Integrative Medical Sciences Yokohama Japan Computational Biology Program Ontario Institute for Cancer Research Toronto ON Canada Programme in Cancer & Stem Cell Biology Duke-NUS Medical School Singapore Singapore Centre for Computational Biology Duke-NUS Medical School Singapore Singapore Programme in Cancer and Stem Cell Biology Duke-NUS Medical School Singapore Singapore Programme in Cancer and Stem Cell Biology Centre for Computational Biology Duke-NUS Medical School Singapore Singapore SingHealth Duke-NUS Institute of Precision Medicine National Heart Centre Singapore Singapore Singapore Cancer Science Institute of Singapore National University of Singapore Singapore Singapore Institute of Molecular and Cell Biology Singapore Singapore Laboratory of Cancer Epigenome Division of Medical Science National Cancer Centre Singapore Singapore Singapore Duke-NUS Medical School Singapore Singapore Human Genome Sequencing Center Baylor College of Medicine Houston TX USA Dan L. Duncan Cancer Center Baylor College of Medicine Houston TX USA Department of Molecular and Human Genetics Baylor College of Medicine Houston TX USA Genome Integrity and Structural Biology Laboratory National Ins

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Mid-Range Science Objectives for the Event Horizon Telescope

arXiv

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arXiv 2024年

作者： Akiyama, Kazunori Albentosa-Ruíz, Ezequiel Alberdi, Antxon Alef, Walter Algaba, Juan Carlos Anantua, Richard Asada, Keiichi Azulay, Rebecca Bach, Uwe Baczko, Anne-Kathrin Ball, David Balokovi, Mislav Bandyopadhyay, Bidisha Barrett, John Baubck, Michi Benson, Bradford A. Bintley, Dan Blackburn, Lindy Blundell, Raymond Bouman, Katherine L. Bower, Geoffrey C. Bremer, Michael Brissenden, Roger Britzen, Silke Broderick, Avery E. Broguiere, Dominique Bronzwaer, Thomas Bustamante, Sandra Carlstrom, John E. Chael, Andrew Chan, Chi-Kwan Chang, Dominic O. Chatterjee, Koushik Chatterjee, Shami Chen, Ming-Tang Chen, Yongjun Cheng, Xiaopeng Cho, Ilje Christian, Pierre Conroy, Nicholas S. Conway, John E. Crawford, Thomas M. Crew, Geoffrey B. Cruz-Osorio, Alejandro Cui, Yuzhu Curd, Brandon Dahale, Rohan Davelaar, Jordy De Laurentis, Mariafelicia Deane, Roger Dempsey, Jessica Desvignes, Gregory Dexter, Jason Dhruv, Vedant Dihingia, Indu K. Doeleman, Sheperd S. Dzib, Sergio A. Eatough, Ralph P. Emami, Razieh Falcke, Heino Farah, Joseph Fish, Vincent L. Fomalont, Edward Ford, H. Alyson Foschi, Marianna Fraga-Encinas, Raquel Freeman, William T. Friberg, Per Fromm, Christian M. Fuentes, Antonio Galison, Peter Gammie, Charles F. García, Roberto Gentaz, Olivier Georgiev, Boris Goddi, Ciriaco Gold, Roman Gómez-Ruiz, Arturo I. Gómez, JoséL Gu, Minfeng Gurwell, Mark Hada, Kazuhiro Haggard, Daryl Hesper, Ronald Heumann, Dirk Ho, Luis C. Ho, Paul Honma, Mareki Huang, Chih-Wei L. Huang, Lei Hughes, David H. Ikeda, Shiro Impellizzeri, C.M. Violette Inoue, Makoto Issaoun, Sara James, David J. Jannuzi, Buell T. Janssen, Michael Jeter, Britton Jiang, Wu Jiménez-Rosales, Alejandra Johnson, Michael D. Jorstad, Svetlana Jones, Adam C. Joshi, Abhishek V. Jung, Taehyun Karuppusamy, Ramesh Kawashima, Tomohisa Keating, Garrett K. Kettenis, Mark Kim, Dong-Jin Kim, Jae-Young Kim, Jongsoo Kim, Junhan Kino, Motoki Koay, Jun Yi Kocherlakota, Prashant Kofuji, Yutaro Koch, Patrick M. Koyama, Shoko Kramer, Carsten Kramer, Joana A. Kramer, Michael Krichbaum, T Massachusetts Institute of Technology Haystack Observatory 99 Millstone Road WestfordMA01886 United States National Astronomical Observatory of Japan 2-21-1 Osawa Mitaka Tokyo181-8588 Japan Black Hole Initiative Harvard University 20 Garden Street CambridgeMA02138 United States Departament d’Astronomia i Astrofísica Universitat de València C. Dr. Moliner 50 Burjassot ValènciaE-46100 Spain Instituto de Astrofísica de Andalucía-CSIC Glorieta de la Astronomía s/n GranadaE-18008 Spain Max-Planck-Institut für Radioastronomie Auf dem Hügel 69 BonnD-53121 Germany Department of Physics Faculty of Science Universiti Malaya Kuala Lumpur50603 Malaysia Center for Astrophysics Harvard & Smithsonian 60 Garden Street CambridgeMA02138 United States Department of Physics & Astronomy The University of Texas at San Antonio One UTSA Circle San AntonioTX78249 United States Institute of Astronomy and Astrophysics Academia Sinica 11F of Astronomy-Mathematics Building AS/NTU No. 1 Sec. 4 Roosevelt Rd. Taipei106216 Taiwan Observatori Astronòmic Universitat de València C. Catedrático JoséBeltrán 2 Paterna ValènciaE-46980 Spain Department of Space Earth and Environment Chalmers University of Technology Onsala Space Observatory OnsalaSE-43992 Sweden Steward Observatory Department of Astronomy University of Arizona 933 N. Cherry Ave. TucsonAZ85721 United States Yale Center for Astronomy & Astrophysics Yale University 52 Hillhouse Avenue New HavenCT06511 United States Astronomy Department Universidad de Concepción Casilla 160-C Concepción Chile Department of Physics University of Illinois 1110 West Green Street UrbanaIL61801 United States Fermi National Accelerator Laboratory MS209 P.O. Box 500 BataviaIL60510 United States Department of Astronomy and Astrophysics University of Chicago 5640 South Ellis Avenue ChicagoIL60637 United States East Asian Observatory 660 N. A’ohoku Place HiloHI96720 United States 660 N. A’ohoku Place HiloHI

The first images of the black holes in Sgr A∗ and M87∗ have created a wide range of new scientific opportunities in gravitational physics, compact objects, and relativistic astrophysics. We discuss here the scientific opportunities that arise from the rich data sets that have already been obtained and the new data sets that will be obtained, exploiting a wide range of technical advances, including observational agility, receiver upgrades, and the addition of new stations. This document provides a 5-year framework for Event Horizon Telescope (EHT) science structured around four fundamental questions that are used to prioritize the analysis of existing data, guide technical upgrades, and determine the optimal use of future observational opportunities with EHT, ALMA, and multi-wavelength facilities. Through enhancements over this period, the EHT will create the first movie of M87∗ connecting black hole and jet physics, provide detailed studies of the structure and dynamics of Sgr A∗, characterize the magnetospheres of both systems through polarimetric imaging, and explore the spacetime properties of black holes with greater precision and range. © 2024, CC BY.

关键词： Astrophysics

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FUTURE-AI: International consensus guideline for trustworthy and deployable artificial intelligence in healthcare

arXiv

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arXiv 2023年

作者： Lekadir, Karim Feragen, Aasa Fofanah, Abdul Joseph Frangi, Alejandro F. Buyx, Alena Emelie, Anais Lara, Andrea Porras, Antonio R. Chan, An-Wen Navarro, Arcadi Glocker, Ben Botwe, Benard O. Khanal, Bishesh Beger, Brigit Wu, Carol C. Cintas, Celia Langlotz, Curtis P. Rueckert, Daniel Mzurikwao, Deogratias Fotiadis, Dimitrios I. Zhussupov, Doszhan Ferrante, Enzo Meijering, Erik Weicken, Eva González, Fabio A. Asselbergs, Folkert W. Prior, Fred Krestin, Gabriel P. Collins, Gary S. Tegenaw, Geletaw S. Kaissis, Georgios Misuraca, Gianluca Tsakou, Gianna Dwivedi, Girish Kondylakis, Haridimos Jayakody, Harsha Woodruf, Henry C. Mayer, Horst Joachim Aerts, Hugo JWL Walsh, Ian Chouvarda, Ioanna Buvat, Irène Tributsch, Isabell Rekik, Islem Duncan, James Kalpathy-Cramer, Jayashree Zahir, Jihad Park, Jinah Mongan, John Gichoya, Judy W. Schnabel, Julia A. Kushibar, Kaisar Riklund, Katrine Mori, Kensaku Marias, Kostas Amugongo, Lameck M. Fromont, Lauren A. Maier-Hein, Lena Alberich, Leonor Cerdá Rittner, Leticia Phiri, Lighton Marrakchi-Kacem, Linda Donoso-Bach, Lluís Martí-Bonmatí, Luis Cardoso, M. Jorge Bobowicz, Maciej Shabani, Mahsa Tsiknakis, Manolis Zuluaga, Maria A. Bielikova, Maria Fritzsche, Marie-Christine Camacho, Marina Linguraru, Marius George Wenzel, Markus De Bruijne, Marleen Tolsgaard, Martin G. Ghassemi, Marzyeh Ashrafuzzaman, Md Goisauf, Melanie Yaqub, Mohammad Abadía, Mónica Cano Mahmoud, Mukhtar M.E. Elattar, Mustafa Rieke, Nicola Papanikolaou, Nikolaos Lazrak, Noussair Díaz, Oliver Salvado, Olivier Pujol, Oriol Sall, Ousmane Guevara, Pamela Gordebeke, Peter Lambin, Philippe Brown, Pieta Abolmaesumi, Purang Dou, Qi Lu, Qinghua Osuala, Richard Nakasi, Rose Zhou, S. Kevin Napel, Sandy Colantonio, Sara Albarqouni, Shadi Joshi, Smriti Carter, Stacy Klein, Stefan Petersen, Steffen E. Aussó, Susanna Awate, Suyash Raviv, Tammy Riklin Cook, Tessa Mutsvangwa, Tinashe E.M. Rogers, Wendy A. Niessen, Wiro J. Puig-Bosch, Xènia Zeng, Yi Mohammed, Yunusa G. Aquino, Yves Saint James Salahuddin, Zohaib Starmans, Martijn P.A. Department de Matemàtiques i Informàtica Universitat de Barcelona Barcelona Spain Barcelona Spain DTU Compute Technical University of Denmark Kgs Lyngby Denmark Department of Mathematics and Computer Science Faculty of Science and Technology Milton Margai Technical University Freetown Sierra Leone Center for Computational Imaging & Simulation Technologies in Biomedicine Schools of Computing and Medicine University of Leeds Leeds United Kingdom Cardiovascular Science and Electronic Engineering Departments KU Leuven Leuven Belgium Institute of History and Ethics in Medicine Technical University of Munich Munich Germany Faculty of Engineering of Systems Informatics and Sciences of Computing Galileo University Guatemala City Guatemala Department of Biostatistics and Informatics Colorado School of Public Health University of Colorado Anschutz Medical Campus AuroraCO United States Department of Medicine Women’s College Research Institute University of Toronto Toronto Canada Universitat Pompeu Fabra BarcelonaBeta Brain Research Center Barcelona Spain Department of Computing Imperial College London London United Kingdom School of Biomedical & Allied Health Sciences University of Ghana Accra Ghana Department of Midwifery & Radiography School of Health & Psychological Sciences City University of London United Kingdom Kathmandu Nepal European Heart Network Brussels Belgium Department of Thoracic Imaging University of Texas MD Anderson Cancer Center Houston United States IBM Research Africa Nairobi Kenya Departments of Radiology Medicine and Biomedical Data Science Stanford University School of Medicine Stanford United States Institute for AI and Informatics in Medicine Klinikum rechts der Isar Technical University Munich Munich Germany Department of Computing Imperial College London London United Kingdom Muhimbili University of Health and Allied Sciences Dar es Salaam Tanzania United Republic of Ioannina Greece Almaty AI Lab Almaty Kazakhstan

Background: Despite major advances in artificial intelligence (AI) research for healthcare, the deployment and adoption of AI technologies remain limited in clinical practice. In recent years, concerns have been raised about the clinical, technical, ethical and legal risks associated with healthcare AI. To increase adoption in the real world, it is essential that AI technologies are trusted and accepted by patients, clinicians, health organisations and authorities. This paper describes the FUTURE-AI framework as the first international consensus guideline for trustworthy AI in healthcare. Methods: The FUTURE-AI consortium was founded in 2021 and now comprises 117 interdisciplinary experts from 50 countries representing all continents, including AI scientists, clinical researchers, biomedical ethicists, and social scientists. Over a two-year period, the consortium established guiding principles and best practices for trustworthy and deployable AI through an iterative process comprising an in-depth literature review, a modified Delphi survey, and online consensus meetings. Findings: The FUTURE-AI framework was established based on six guiding principles for trustworthy AI in healthcare, i.e. Fairness, Universality, Traceability, Usability, Robustness and Explainability. Through consensus, a set of 30 best practices were defined, addressing technical, clinical, socio-ethical and legal dimensions of trustworthy AI. The recommendations cover the entire lifecycle of healthcare AI, from design, development and validation to regulation, deployment, and monitoring. Interpretation: FUTURE-AI is a structured, risk-informed framework which provides guidance for constructing healthcare AI tools that will be trusted, deployed and adopted in real-world clinical practice. Researchers are encouraged to take the recommendations into account in proof-of-concept stages to facilitate future translation towards clinical practice of healthcare AI. Copyright © 2023, The Authors. All rights

关键词： Clinical research

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A multi-frequency study of sub-parsec jets with the Event Horizon Telescope

arXiv

引用

arXiv 2025年

作者： Röder, Jan Wielgus, Maciek Lobanov, Andrei P. Krichbaum, Thomas P. Nair, Dhanya G. Lee, Sang-Sung Ros, Eduardo Fish, Vincent L. Blackburn, Lindy Chan, Chi-Kwan Issaoun, Sara Janssen, Michael Johnson, Michael D. Doeleman, Sheperd S. Bower, Geoffrey C. Crew, Geoffrey B. Tilanus, Remo P.J. Savolainen, Tuomas Impellizzeri, C.M. Violette Alberdi, Antxon Baczko, Anne-Kathrin Gómez, José L. Lu, Ru-Sen Paraschos, Georgios F. Traianou, Efthalia Goddi, Ciriaco Kim, Daewon Lisakov, Mikhail Kovalev, Yuri Y. Voitsik, Petr A. Sokolovsky, Kirill V. Akiyama, Kazunori Albentosa-Ruíz, Ezequiel Alef, Walter Algaba, Juan Carlos Anantua, Richard Asada, Keiichi Azulay, Rebecca Bach, Uwe Ball, David Baloković, Mislav Bandyopadhyay, Bidisha Barrett, John Bauböck, Michi Benson, Bradford A. Bintley, Dan Blundell, Raymond Bouman, Katherine L. Bremer, Michael Brinkerink, Christiaan D. Brissenden, Roger Britzen, Silke Broderick, Avery E. Broguiere, Dominique Bronzwaer, Thomas Bustamante, Sandra Byun, Do-Young Carlstrom, John E. Ceccobello, Chiara Chael, Andrew Chang, Dominic O. Chatterjee, Koushik Chatterjee, Shami Chen, Ming-Tang Chen, Yongjun Cheng, Xiaopeng Cho, Ilje Christian, Pierre Conroy, Nicholas S. Conway, John E. Cordes, James M. Crawford, Thomas M. Cruz-Osorio, Alejandro Cui, Yuzhu Curd, Brandon Dahale, Rohan Davelaar, Jordy De Laurentis, Mariafelicia Deane, Roger Dempsey, Jessica Desvignes, Gregory Dexter, Jason Dhruv, Vedant Dihingia, Indu K. Dougall, Sean Taylor Dzib, Sergio A. Eatough, Ralph P. Emami, Razieh Falcke, Heino Farah, Joseph Fomalont, Edward H. Ford, Alyson Foschi, Marianna Fraga-Encinas, Raquel Freeman, William T. Friberg, Per Fromm, Christian M. Fuentes, Antonio Galison, Peter Gammie, Charles F. García, Roberto Gentaz, Olivier Georgiev, Boris Gold, Roman Gómez-Ruiz, Arturo I. Gu, Minfeng Gurwell, Mark Hada, Kazuhiro Haggard, Daryl Haworth, Kari Hecht, Michael H. Hesper, Ronald Heumann, Dirk Ho, Luis C. Ho, Paul Honma, Mareki Huang, Chih-Wei L. Huang, Lei Hughes, David H. Ikeda, Shiro Inoue, Makoto James, David J. Max-Planck-Institut für Radioastronomie Auf dem Hügel 69 BonnD-53121 Germany Instituto de Astrofísica de Andalucía-CSIC Glorieta de la Astronomía s/n GranadaE-18008 Spain Astronomy Department Universidad de Concepción Casilla 160-C Concepción Chile Korea Astronomy and Space Science Institute Daedeok-daero 776 Yuseong-gu Daejeon34055 Korea Republic of Massachusetts Institute of Technology Haystack Observatory 99 Millstone Road WestfordMA01886 United States Black Hole Initiative Harvard University 20 Garden Street CambridgeMA02138 United States Center for Astrophysics Harvard & Smithsonian 60 Garden Street CambridgeMA02138 United States Steward Observatory Department of Astronomy University of Arizona 933 N. Cherry Ave. TucsonAZ85721 United States Data Science Institute University of Arizona 1230 N. Cherry Ave. TucsonAZ85721 United States Program in Applied Mathematics University of Arizona 617 N. Santa Rita TucsonAZ85721 United States NASA Hubble Fellowship Program United States Radboud University P.O. Box 9010 Nijmegen6500 GL Netherlands Institute of Astronomy and Astrophysics Academia Sinica 645 N. A’ohoku Place HiloHI96720 United States Department of Physics and Astronomy University of Hawaii at Manoa 2505 Correa Road HonoluluHI96822 United States Leiden Observatory Leiden University Postbus 2300 Leiden9513 RA Netherlands Postbus 93138 Den Haag2509 AC Netherlands Aalto University Department of Electronics and Nanoengineering PL 15500 AaltoFI-00076 Finland Aalto University Metsähovi Radio Observatory Metsähovintie 114 KylmäläFI-02540 Finland National Radio Astronomy Observatory 520 Edgemont Road CharlottesvilleVA22903 United States Department of Space Earth and Environment Chalmers University of Technology Onsala Space Observatory OnsalaSE-43992 Sweden Shanghai Astronomical Observatory Chinese Academy of Sciences 80 Nandan Road Shanghai200030 China Key Laboratory of Radio Astronomy Chinese Academy of Scien

Context. The 2017 observing campaign of the Event Horizon Telescope (EHT) delivered the first very long baseline interferometry (VLBI) images at the observing frequency of 230 GHz, leading to a number of unique studies on black holes and relativistic jets from active galactic nuclei (AGN). In total, eighteen sources were observed, including the main science targets, Sgr A* and M 87 and various calibrators. Sixteen sources were AGN. Aims. We investigated the morphology of the sixteen AGN in the EHT 2017 data set, focusing on the properties of the VLBI cores: size, flux density, and brightness temperature. We studied their dependence on the observing frequency in order to compare it with the Blandford-Königl (BK) jet model. In particular, we aimed to study the signatures of jet acceleration and magnetic energy conversion. Methods. We modeled the source structure of seven AGN in the EHT 2017 data set using linearly polarized circular Gaussian components (1749+096, 1055+018, BL Lac, J0132–1654, J0006–0623, CTA 102, 3C 454.3) and collected results for the other nine AGN from dedicated EHT publications, complemented by lower frequency data in the 2-86 GHz range. Combining these data into a multi-frequency EHT+ data set, we studied the dependences of the VLBI core component flux density, size, and brightness temperature on the frequency measured in the AGN host frame (and hence on the distance from the central black hole), characterizing them with power law fits. We compared the observations with the BK jet model and estimated the magnetic field strength dependence on the distance from the central black hole. Results. Our observations spanning event horizon- to parsec scales indicate a deviation from the standard BK model, particularly in the decrease of the brightness temperature with the observing frequency. Only some of the discrepancies may be alleviated by tweaking the model parameters or the jet collimation profile. Either bulk acceleration of the jet material, energ

关键词： Luminance

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Early Detection of Preeclampsia using a Rule-Based System Information System

引用

Journal of Physics: Conference Series 2019年第1期1179卷

作者： F N Aini M N Widyawati S Suryono Purwokerto Midwifery Program Poltekkes Kemenkes Semarang Indonesia Postgraduate Applied Science Midwifery Program Poltekkes Kemenkes Semarang Indonesia Department of Physics Faculty of Science and Mathematics University Diponegoro Semarang Indonesia

Preeclampsia is the highest cause of maternal death. One program to reduce Maternal Mortality Rate (MMR) is by early detection. The incomplete history of maternal history that has occurred has led to the determination of an incorrect diagnosis and has resulted in errors in decision making. The results of the survey in the detection of preeclampsia include midwives not conducting a history of past medical history, physical examination during the first antenatal care visit is incomplete. During this time the detection and diagnosis model is still done manually, so it was not effective and efficient. The inspection data obtained using the information system becomes more complete and faster. Data obtained with information systems can be seen anywhere and anytime. This study produced innovations for the detection of preeclampsia in pregnant women using a rule-based system information system. This study uses the Quasy experimental posttest-only design. The subjects of this study were 66 pregnant women. Data collection was carried out using questionnaires and checklists. The results showed that early detection of preeclampsia using a rule-based system information system could improve the completeness of data on pregnant women up to 35.66%, and speed up the detection time of preeclampsia up to 35.60%. This system also has an effectivenessvalue 84.8%.

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