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Ultra-flexible graphene/nylon/PDMS coaxial fiber-shaped multifunctional sensor

Nano Research 2023年第4期16卷 5541-5547页

作者： Peddathimula Puneetha Siva Pratap Reddy Mallem Sung Cheol Park Seoha Kim Dong Hun Heo Cheol Min Kim Jaesool Shim Sung Jin An Dong-Yeon Lee Kwi-Il Park Department of Robotics and Intelligent Machine Engineering/College of Mechanical and IT Engineering Yeungnam UniversityGyeongsan 38541Republic of Korea School of Materials Science and Engineering Kyungpook National UniversityDaegu 41566Republic of Korea Advanced Material Research Center Kumoh National Institute of TechnologyGumi 39177Republic of Korea School of Mechanical Engineering Yeungnam UniversityGyeongsan 38541Republic of Korea Department of Materials Science and Engineering Kumoh National Institute of TechnologyGumi 39177Republic of Korea

The development of flexible and wearable devices is mainly required for tactile sensing;as such devices can adapt to complicated nonuniform surfaces,they can be applied to the human ***,it remains necessary to simultaneously achieve small-scale,portable,and stable developments in such ***,this work aims at fabricating a novel,lightweight,ultra-flexible,and fiber-shaped coaxial structure with a diameter of 0.51 mm using polydimethylsiloxane/graphene/nylon material,based on piezoresistive and triboelectric *** piezoresistive-based robotic-hand-controlled sensor thus realized exhibits a response time of 120 ms and a fast recovery time of 55 ***,the piezoresistive-based sensors effectively feature whisker/joystick-guided behaviors and also sense the human finger *** to the triboelectric-based selfpowered nanogenerator behavior,the resulting sensor can convert mechanical motion into electrical energy,without adversely affecting human ***,this triboelectric-based human finger sensor can be operated under different bending modes at specific ***,this multifunctional sensor is cost-effective and suitable for various applications,including robotichand-controlled operations in medical surgery,whisker/joystick motions in lightweight drone technology,and navigation with highsensitivity components.

关键词： extremely lightweight ultra-flexible piezoresistive/triboelectric sensor human-machine whisker

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Polar materials for photocatalytic applications:A critical review

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Interdisciplinary materials 2024年第4期3卷 530-564页

作者： Xiaoqing Liu Yu Zhang Cong Wang Lei Shen Department of Mechanical Engineering National University of SingaporeSingaporeSingapore School of Physics Harbin Institute of TechnologyHarbinPR China School of Materials Science and Engineering Engineering Research Center of Optoelectronic Functional MaterialsMinistry of EducationChangchun University of Science and TechnologyChangchunPR China

The critical challenges of the energy crisis and environmental degradation promote innovative approaches for energy ***-based photocatalytic technology,which transforms solar energy into chemical energy,emerges as a promising ***,the practical application of this technology faces several challenges,such as the rapid recombination of photogenerated electrons and holes,significantly limiting photocatalytic *** this review,we provide a detailed discussion,an insightful perspective,and a critical evaluation of recent advances,challenges,and opportunities in the field of photocatalysis using polar *** present a comprehensive examination of the photocatalytic mechanisms,activity,and diverse applications of photocatalysts based on polar *** also briefly discuss the engineering design of polar photocatalysis in experiments and its scalability in the *** review outlines future trends and potential breakthroughs in the photocatalytic field using polar materials,projecting their transformative impact on environmental chemistry and energy engineering.

关键词： 2D Janus structures ferroelectric materials heterostructures photocatalysts polar materials

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Tailoring properties of directed energy deposited Al-Mg alloy by balancing laser shock peening and heat treatment

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Journal of materials science & Technology 2024年第36期203卷 78-96页

作者： Wei Dai Wei Guo Jun Xiao Ying Zhu Zewu Qi Jiaxin Shi Changhao Yin Dongsheng He Jiaxuan Chi Zhandong Wan Baoqiang Cong Minggao Li Hongqiang Zhang School of Mechanical Engineering and Automation Beihang UniversityBeijing100191China School of Materials Science and Engineering Beihang UniversityBeijing100191China Faculty of Materials and Manufacturing Beijing University of TechnologyBeijing100124China Technology Research Department CRRC InstituteBeijing100070China

Wire arc-directed energy deposition(WADED)has shown great advantages and potential in fabricating large-scale aluminum(Al)alloy ***,WADED Al alloys typically exhibit low strength and reliability due to pore defects and lack of work hardening or precipitation *** study utilized a combination of laser shock peening(LSP)and annealing to regulate the microstructure of WADED Al-Mg4.5Mn alloy and enhance mechanical *** effects of LSP and annealing on phase composition,pore distribution,and microstructures at multiple scales were systematically investigated to reveal the mechanical property improving *** results demonstrated that LSP-induced plastic deformation formed a defect-free zone by closing near-surface pore *** created the hardened layer with gradient mechanical properties by inducing gradient changes in grain size,the number of low-angle grain boundaries(LAGBs),and dislocation density along the depth *** annealing process promoted grain coarsening and reduced excessive dislocations and LAGBs,weakening the work harden-ing effect caused by ***,the high-density dislocations and high stored energy generated by LSP accelerated the recrystallization,facilitating growth of near-surface *** defect-free zone,dislocation strengthening,and LAGBs strengthening were responsible for the increase in strength,while the synergistic deformation between hardened layers and soft core facilitated maintaining excellent *** strength and elongation of WADED Al alloy can be synergistically improved by balancing the effects of LSP and heat treatment.

关键词： Wire arc-directed energy deposition Aluminum alloy Laser shock peening Pore distribution Tensile property

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Electronic structure prediction of multimillion atom systems through uncertainty quantification enabled transfer learning

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npj Computational materials 2024年第1期10卷 1423-1437页

作者： Shashank Pathrudkar Ponkrshnan Thiagarajan Shivang Agarwal Amartya S.Banerjee Susanta Ghosh Department of Mechanical Engineering-Engineering Mechanics Michigan Technological UniversityHoughtonMIUSA Department of Electrical and Computer Engineering University of CaliforniaLos AngelesCA90095USA Department of Materials Science and Engineering University of CaliforniaLos AngelesCA90095USA Faculty member of the Center for Data Sciences Michigan Technological UniversityHoughtonMIUSA

The ground state electron density—obtainable using Kohn-Sham Density Functional Theory(KSDFT)simulations—contains a wealth of material information,making its prediction via machine learning(ML)models ***,the computational expense of KS-DFT scales cubically with system size which tends to stymie training data generation,making it difficult to develop quantifiably accurate ML models that are applicable across many scales and system ***,we address this fundamental challenge by employing transfer learning to leverage the multi-scale nature of the training data,while comprehensively sampling systemconfigurations using *** ML models are less reliant on heuristics,and being based on Bayesian neural networks,enable uncertainty *** show that our models incur significantly lower data generation costs while allowing confident—and when verifiable,accurate—predictions for a wide variety of bulk systems well beyond training,including systems with defects,different alloy compositions,and at multi-million-atom ***,such predictions can be carried out using only modest computational resources.

关键词： alloy prediction transfer

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Towards atom-level understanding of metal oxide catalysts for the oxygen evolution reaction with machine learning

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npj Computational materials 2024年第1期10卷 2430-2440页

作者： Jaclyn R.Lunger Jessica Karaguesian Hoje Chun Jiayu Peng Yitong Tseo Chung Hsuan Shan Byungchan Han Yang Shao-Horn Rafael Gómez-Bombarelli Department of Materials Science and Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA Center for Computational Science and Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA Department of Chemical and Biomolecular Engineering Yonsei UniversitySeoul 03722Republic of Korea Department of Computational and Systems Biology Massachusetts Institute of TechnologyCambridgeMA 02139USA Department of Materials Science and Engineering University of TorontoTorontoON M5SCanada Department of Mechanical Engineering Massachusetts Institute of TechnologyCambridgeMA 02139USA Research Laboratory of Electronics Massachusetts Institute of TechnologyCambridgeMA 02139USA

Green hydrogen production is crucial for a sustainable future,but current catalysts for the oxygen evolution reaction(OER)suffer from slow kinetics,despite many efforts to produce optimal designs,particularly through the calculation of descriptors for *** this study,we develop a dataset of density functional theory calculations of bulk and surface perovskite oxides,and adsorption energies of OER intermediates,which includes compositions up to quaternary and facets up to(555).We demonstrate that per-site properties of perovskite oxides such as Bader charge or band center can be tuned through element substitution and faceting,and develop a machine learning model that accurately predicts these properties directly from the local chemical *** leverage these per-site properties to identify promising perovskites with high theoretical OER *** identified design principles and promising materials provide a roadmap for closing the gap between current artificial catalysts and biological enzymes such as photosystem II.

关键词： perovskite oxides kinetics

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Physics through the microscope

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Chinese Physics B 2024年第11期33卷 1-11页

作者： Stephen J.Pennycook Ryo Ishikawa Haijun Wu Xiaoxu Zhao Changjian Li Duane Loh Jiadong Dan Wu Zhou School of Physical Sciences and CAS Key Laboratory of Vacuum Physics University of Chinese Academy of SciencesBeijing 100049China Department of Materials Science and Engineering University of TennesseeKnoxvilleTN37996USA Institute of Engineering Innovation University of TokyoTokyo 113-8656Japan State Key Laboratory for Mechanical Behavior of Materials Xi'an Jiaotong UniversityXi'an 710049China School of Materials Science and Engineering Peking UniversityBeijing 100871China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Department of Physics National University of SingaporeSingapore 117551Singapore Department of Biological Sciences National University of SingaporeSingapore 117558Singapore

The electron microscope provides numerous insights into physics, from demonstrations of fundamental quantummechanical principles to the physics of imaging and materials. It reveals the atomic and electronic structure of key regionssuch as defects and interfaces. We can learn the underlying physics governing properties, and gain insight into how tosynthesize new materials with improved properties. Some recent advances and possible future directions are discussed.

关键词： scanning transmission electron microscopy materials science point defects artificial intelligence

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Polarization pinning at antiphase boundaries in multiferroic YbFeO_(3)

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Chinese Physics B 2024年第11期33卷 39-45页

作者： Guodong Ren Pravan Omprakash Xin Li Yu Yun Arashdeep S.Thind Xiaoshan Xu Rohan Mishra Institute of Materials Science and Engineering Washington University in St.LouisSt.LouisMO 63130USA Department of Physics and Astronomy University of NebraskaLincolnNE 68588USA Department of Mechanical Engineering & Mechanics Drexel UniversityPhiladelphiaPA 19104-2875USA Nebraska Center for Materials and Nanoscience University of NebraskaLincolnNE 68588USA Department of Mechanical Engineering and Material Science Washington University in St.LouisSt.LouisMO 63130USA

The switching characteristics of ferroelectrics and multiferroics are influenced by the interaction of topological defects with domain *** report on the pinning of polarization due to antiphase boundaries in thin films of the multiferroic hexagonal YbFeO_(3).We have directly resolved the atomic structure of a sharp antiphase boundary(APB)in YbFeO_(3) thin films using a combination of aberration-corrected scanning transmission electron microscopy(STEM)and total energy calculations based on density-functional theory(DFT).We find the presence of a layer of FeO_(6) octahedra at the APB that bridges the adjacent *** imaging shows a reversal in the direction of polarization on moving across the APB,which DFT calculations confirm is structural in nature as the polarization reversal reduces the distortion of the FeO_(6) octahedral layer at the *** APBs in hexagonal perovskites are expected to serve as domain-wall pinning sites and hinder ferroelectric switching of the domains.

关键词： hexagonal ferrites ferroelectric multiferroic topological defect STEM

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Mechanism of solute hardening and dislocation debris-me diate d ductilization in Nb-Si alloy

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Journal of materials science & Technology 2024年第36期203卷 167-179页

作者： Bo-Qing Li Irene J.Beyerlein Shuhei Shinzato Shigenobu Ogata Wei-Zhong Han Center for Advancing Materials Performance from the Nanoscale State Key Laboratory for Mechanical Behavior of MaterialsXi’an Jiaotong UniversityXi’an 710049China Materials Department University of CaliforniaSanta BarbaraCA 93106-5070USA Department of Mechanical Engineering University of CaliforniaSanta BarbaraCA 93106-5070USA Department of Mechanical Science and Bioengineering Osaka UniversityOsaka 560-8531Japan

Niobium(Nb)is sensitive to even minute quantities of silicon(Si)solutes,which are known to induce pronounced ***,the underlying mechanism for hardening remains elusive since the ef-fect of Si solutes on dislocation behavior is ***,using tensile testing,in-situ microscopy and nanomechanical testing,the behavior of dislocations in dilute Nb-Si alloys,containing from 0 at.%to 0.8 at.%Si,is *** show that the hardness,strength and strain hardening rate increase from two to four times,while the uniform elongation in tension only reduces 50%as the Si content *** evolve from complex entangled patterns in Nb to parallel long-straight screw dislocation-dominated structures in Nb-Si ***-situ indentation reveals that the origins of the marked harden-ing in Nb-Si alloy are the reduction of dislocation mobility and cross-slip *** densities of dislocation debris-superjogs and loops introduced throughout the sample during warm rolling and an-nealing are found to provide active internal dislocation sources,which explain the minimal ductility loss seen in these Nb-Si *** findings can help guide the alloy design of high-performance refractory materials for extreme temperature applications.

关键词： Niobium Si solute Hardening Ductilization Dislocation

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Magnetic properties and magnetocaloric effects in Eu(Ti,Nb,Mn)O_(3) perovskites

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Journal of Rare Earths 2024年第8期42卷 1560-1567,I0006页

作者： Junfeng Wang Huicai Xie Quanyi Liu Zhihong Hao Zhaojun Mo Qi Fu Xinqiang Gao Jun Shen Ganjiang Innovation Academy Chinese Academy of SciencesGanzhou341119China Faculty of Materials Metallurgy and Chemistry Jiangxi University of Science and TechnologyGanzhou341000China School of Rare Earth and New Materials Engineering Gannan University of Science and TechnologyGanzhou341000China Department of Energy and Power Engineering School of Mechanical EngineeringBeijing Institute of TechnologyBeijing100081China

In perovskite EuTiO_(3),the magnetic characteristics and magnetocaloric effect(MCE) can be flexibly regulated by converting the magnetism from antiferromagnetic to *** the present work,a series of Eu(Ti,Nb,Mn)O_(3) compounds,abbreviated as ETNMO for convenience of description,was fabricated and their crystallography,magnetism together with cryogenic magnetocaloric effects were systematically *** crystallographic results demonstrate the cubic perovskite structure for all the compounds,with the space group of *** magnetic phase transitions are observed in these second-order phase transition(SOPT) *** joint substitution of elements Mn and Nb can considerably manipulate the magnetic phase transition process and magnetocaloric performance of the ETNMO *** the Mn content increases,gradually widened-ΔS_(M)-T curves are obtained,and two peaks with a broad shoulder are observed in the-ΔS_(M)-T curves for Δμ_(0)H≤0-1 *** a field change of 0-5 T,the values of maximum magnetic entropy change(-ΔS_(M)^(max)) and refrigeration capacity(RC) are evaluated to be 34.7 J/(kg·K) and 364.9 J/kg for EuTi_(0.8625)Nb_(0.0625)Mn_(0.075)O_(3), 27.8 J/(kg·K) and367.6 J/kg for EuTi_(0.8375)Nb_(0.0625)Mn_(0.1)O_(3),23.2 J/(kg·K) and 369.2 J/kg for EuTi_(0.8125)Nb_(0.0625)Mn_(0.125)O_(3),17.1 J/(kg·K) and 357.6 J/kg for EuTi_(0.7875)Nb_(0.0625)Mn_(0.15)O_(3),*** co nsiderable MCE parameters make the ETNMO compounds potential candidates for cryogenic magnetic refrigeration.

关键词： ETNMO perovskites Cryogenic refrigeration Magnetic phase transition Magnetocaloric effect Rare earths

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Understanding the Thermal Impedance of Silicone Rubber/Hexagonal Boron Nitride Composites as Thermal Interface materials

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Chinese Journal of Polymer science 2024年第3期42卷 352-363,I0008页

作者： Yuan Ji Shi-Da Han Hong Wu Shao-Yun Guo Feng-Shun Zhang Jian-Hui Qiu The State Key Laboratory of Polymer Materials Engineering Sichuan Provincial Engineering Laboratory of Plastic/Rubber Complex Processing TechnologyPolymer Research InstituteSichuan UniversityChengdu 610065China Institute of Chemical Materials China Academy of Engineering PhysicsMianyang 621900China Department of Mechanical Engineering Faculty of Systems Science and TechnologyAkita Prefectural UniversityAkita 015-0055Japan

Silicone rubber(SR) composites are most widely used as thermal interface materials(TIMs) for electronics heat dissipation. Thermal impedance as the main bottleneck limiting the performance of TIMs is usually neglected. Herein, the thermal impedance of SR composites loaded with different levels of hexagonal boron nitride(h-BN) as TIMs was elaborated for the first time by the ASTM D 5470 standard test and finite element analysis. It was found that elastic modulus and surface roughness of SR composites increased with the increase of h-BN content, indicating that the conformity was reduced. When the assembly pressure was 0.69 MPa, there existed an optimal h-BN content at which the contact resistance was minimum(0.39 K·cm^(2)·W^(-1)). Although the decreased bond line thickness(BLT) by increasing the assembly pressure was beneficial to reduce the thermal impedance, the proper assembly pressure should be selected to prevent the warpage of the contact surfaces and the increase in contact resistance, according to the compression properties of the SR composites. This study provides valuable insights into fabrication of high-performance TIMs for modern electronic device applications.

关键词： Thermal interface materials Hexagonal boron nitride Thermal impedance Surfaces

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