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MXene:From synthesis to environment remediation

Chinese Journal of Chemical engineering 2023年第9期61卷 260-280页

作者： Ali Nikkhah Hasan Nikkhah Hadis langari Alireza Nouri Abdul Wahab Mohammad Ang Wei Lun Ng law Yong Rosiah Rohani Ebrahim Mahmoudi Department of Chemical and Process Engineering Faculty of Engineering and Built EnvironmentUniversiti Kebangsaan MalaysiaBangi 43600Malaysia Department of Mechanical and Aerospace Engineering University at BuffaloBuffaloUSA Department of Chemical and Biomolecular Engineering University of ConnecticutStorrsUSA Department of Chemistry and Medicinal Chemistry University at BuffaloBuffaloUSA Chemical and Water Desalination Engineering Program College of EngineeringUniversity of SharjahSharjah 27272United Arab Emirates Lee Kong Chian Faculty of Engineering and Science Universiti Tunku Abdul RahmanJalan Sungai LongBandar Sungai LongKajangSelangorMalaysia

A new burgeoning family of two-dimensional(2D)transition metal carbides/nitrides,better known as MXenes,have received extensive attention because of their distinct properties,such as metallic conductivity,good hydrophilicity,large surface area,good mechanical stability,and *** 40 different MXenes have been synthesized,and dozens more structures and properties have been theoretically ***,the recent progress in MXenes development is not well covered in chronological order based on different *** review article focuses on emerging synthesis methods,the properties of MXenes,and mainly the applications of MXenes and MXene-based material family in environmental remediation,a comprehensive review of gaseous and aqueous pollutants treatment.

关键词： MXene 2D materials Wastewater treatment CO_(2)capture Adsorption Photodegradation

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Photoplastic effect in organic–inorganic lead iodide perovskite thin films

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Journal of materials science: materials in Energy 2025年第1期1卷 1-6页

作者： Tunesi, Michele Liu, Yulin Lee, Jung-Kun Lucca, Don A. School of Mechanical and Aerospace Engineering Oklahoma State University Stillwater USA Department of Mechanical Engineering and Materials Science University of Pittsburgh Pittsburgh USA

The positive photoplastic effect (PPE) and photoinduced stiffening are the reversible increases of the flow stress and the elastic modulus of a material upon irradiation with light. Several material groups, including the II-VI compounds and alkali halides show some form of these effects. The dependence of mechanical properties on light illumination has not been reported for methylammonium lead iodide (CH3NH3PbI3 or MAPbI3) perovskites. In this study a positive PPE and photoinduced stiffening were found in MAPbI3 thin film perovskites. Thin films of 500 nm thickness were synthesized and then polished. The chemical formation of MAPbI3 was verified by x-ray diffraction. Atomic force microscopy and scanning electron microscopy were used to characterize the surface topography. Nanoindentation experiments were performed to investigate the elastic and plastic properties in darkness and under illumination. The elastic modulus and hardness were found to increase by 53% and 67% respectively when the perovskite was illuminated.

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Correction: materials laboratories of the future for alloys, amorphous, and composite materials (MRS Bulletin, (2025), 50, 2, (190-207), 10.1557/s43577-024-00846-y)

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MRS Bulletin 2025年 1-2页

作者： Banerjee, Sarbajit Meng, Y. Shirley Minor, Andrew M. Zhang, Minghao Zaluzec, Nestor J. Chan, Maria K.Y. Seidler, Gerald McComb, David W. Agar, Joshua Mukherjee, Partha P. Melot, Brent Chapman, Karena Guiton, Beth S. Klie, Robert F. McCue, Ian D. Voyles, Paul M. Robertson, Ian Li, Ling Chi, Miaofang Destino, Joel F. Devaraj, Arun Marquis, Emmanuelle A. Segre, Carlo U. Liu, Huinan H. Yang, Judith C. Momeni, Kasra Misra, Amit Abdolrahim, Niaz Medvedeva, Julia E. Cai, Wenjun Sehirlioglu, Alp Dizbay-Onat, Melike Mehta, Apurva Graham-Brady, Lori Maruyama, Benji Rajan, Krishna Warner, Jamie H. Taheri, Mitra L. Kalinin, Sergei V. Reeja-Jayan, B. Schwarz, Udo D. Simon, Sindee L. Brown, Craig M. Department of Chemistry and Department of Materials Science & Engineering Texas A & M University College Station United States Pritzker School of Molecular Engineering The University of Chicago Chicago United States Department of Materials Science & Engineering University of California Berkeley Berkeley United States National Center for Electron Microscopy Molecular Foundry Lawrence Berkeley National Laboratory Berkeley United States Center for Nanoscale Materials Argonne National Laboratory Lemont United States Department of Physics University of Washington Seattle United States Department of Materials Science & Engineering The Ohio State University Columbus United States Department of Mechanical Engineering and Mechanics Drexel University Philadelphia United States School of Mechanical Engineering Purdue University West Lafayette United States Department of Chemistry University of Southern California Los Angeles United States Department of Chemistry Stony Brook University The State University of New York Stony Brook United States Department of Chemistry University of Kentucky Lexington United States Department of Physics University of Illinois at Chicago Chicago United States Department of Materials Science & Engineering Northwestern University Evanston Bangladesh Department of Materials Science & Engineering University of Wisconsin–Madison Madison United States Department of Materials Science and Engineering University of Pennsylvania Philadelphia United States Department of Mechanical Engineering and Materials Science Duke University Durham United States Department of Chemistry Creighton University Omaha United States Physical and Computational Sciences Directorate Pacific Northwest National Laboratory Richland United States Department of Materials Science & Engineering University of Michigan–Ann Arbor Ann Arbor United States Department of Physics Illinois Institute of Technology Chicago United States Department of Bioengineering and the Mater

This article was updated to correct Minghao Zhang’s affiliation from "Pritzker School of Molecular engineering, The University of Chicago, Chicago, USA" to "Pritzker School of Molecular engineering, The University of Chicago, Chicago, USA;Argonne National Laboratory, Lemont, USA." Argonne National Laboratory was left off the original publication. © The Author(s) 2025.

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The Investigation of Microstructure and mechanical Property of Incorporation of Cerium Oxide to AA2219 Through Liquid Forging Technique

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Journal of The Institution of Engineers (India): Series D 2025年第1期106卷 9-17页

作者： Karthik, A. Karunanithi, R. Srinivasan, S.A. Kumareshbabu, S.P. Department of Mechanical Engineering B.S. Abdur Rahman Crescent Institute of Science and Technology Seethakathi Estate Vandalur Tamil Nadu Chennai600048 India Department of Aerospace Engineering B.S. Abdur Rahman Crescent Institute of Science and Technology Seethakathi Estate Vandalur Tamil Nadu Chennai600048 India Department of Metallurgical and Materials Engineering National Institute of Technology Tiruchirappalli Tanjore Main Road National Highway 67 Tamil Nadu Tiruchirappalli620015 India

In this study, an attempt is made to prepare aluminum metal matrix composites of AA2219 with varying reinforcement of weight percentages of cerium oxide (X = 0.5%, 1%, 1.5%, and 2%) by liquid metallurgy technique involving liquid forging operation. The incorporation of rare earth oxide to AA2219 through liquid forging technique offers excellent solubility of the solute atom along with near-net shape capability, higher materials property, and reduced porosity level when compared with conventional casting route. The reinforcement of cerium oxide improves mobility, casting microstructure, reduces shrinkage and hot tearing tendency of AA2219. The AA2219 composites sample were casted at the following process parameter such as the applied pressure load 350 MPa, the heating die temperature 200 °C, melt temperature 750 °C, and 60 s dwell time. The main objective was to determine the effect of CeO2 particles on the microstructure and mechanical properties of AA2219 composites through liquid forging technique. X-ray diffraction studies revealed the presence of intermetallic phase present in the composites and the presence of CeO2 confirmed by EDS analysis. Scanning electron microscopy images showed a homogeneous distribution of CeO2 particles within the matrix and the grain boundaries. The reinforcement of CeO2 increase hardness of the composites with a maximum hardness of 123 VHN observed for 2 wt% CeO2 with AA2219. The tensile test indicated the significant effect of the CeO2 particles with an ultimate tensile strength of 232 MPa and 87 MPa yield strength when compared to the unreinforced material was around 130 Mpa and 75 MPa, respectively. Fractography showed ductile fracture mode failure and the increase in CeO2 decrease the level of strain rate. © The Institution of Engineers (India) 2020.

关键词： Microstructure

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Na-22 for Safeguarding and Mass Accounting of Molten Salt Systems

Na-22 for Safeguarding and Mass Accounting of Molten Salt Sy...

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2023 Transactions of the American Nuclear Society Winter Conference and Expo, ANS 2023

作者： Zile, Matthew Van Kauffman, Andrew Herminghuysen, Kevin Li, Shelly Simpson, Michael Kandlakunta, Praneeth Cao, Guoping Cao, Lei R. Nuclear Engineering Program Department of Mechanical and Aerospace Engineering Ohio State University United States Nuclear Reactor Laboratory College of Engineering Ohio State University United States Department of Materials Science and Engineering University of Utah.Idaho National Laboratory United States

The Na-22based radioactive tracer dilution (RTD) technique has been previously demonstrated for mass accounting in small quantities of clean molten salt for bench top testing. While the concept of RTD has proven to be a promising method, it has lacked further validation in large-scale quantities and in fuel-bearing salt. Towards that end, two research initiatives are on-going at The Ohio State University (OSU) and Idaho National Laboratory (INL) to address these challenges. Current work at OSU is focused on evaluating the RTD using the full gamma-ray spectrum of fission products produced by irradiating fuel bearing salt, i.e., UCl3-MgCl2-KCl in a 500-kW research reactor. The INL team has successfully demonstrated the RTD for mass determination using an 8-kg LiCl-KCl-UCl3salt for uranium electrorefining and is currentlyseeking to validate the tracer method with large(about 60 kg)molten salt system(bearing fission products) in an oxide reduction (OR) facility for spent nuclear fuel (SNF) reprocessing. © 2023 American Nuclear Society. All rights reserved.

关键词： Fission products

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Thermomechanical Characterization of Hot Surface Ignition Device Using Phenomenological Heat Flux Model

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JOURNAL OF PROPULSION AND POWER 2022年第4期38卷 656-670页

作者： Kang, Sang-Guk Ryu, Je Ir Motily, Austen H. Numkiatsakul, Prapassorn Lee, Tonghun Kriven, Waltraud M. Kim, Kenneth S. Kweon, Chol-Bum M. U.S. Army Research Laboratory Aberdeen Proving Ground MD 21005 Aerospace Engineer Weapons and Materials Research Directorate Postdoctoral Fellow Computational and Information Sciences Directorate University of Illinois at Urbana-Champaign Urbana IL 61801 Graduate Student Department of Mechanical Science and Engineering. Student Member AIAA Graduate Student Department of Materials Science and Engineering Professor Department of Mechanical Science and Engineering. Associate Fellow AIAA Professor Department of Materials Science and Engineering Mechanical Engineer Computational and Information Sciences Directorate. Member AIAA Program Manager Computational and Information Sciences Directorate. Member AIAA.

Modern aircraft compression ignition engines that seek to achieve fuel-flexible operation require ignition-assisting devices to perform reliably. Many military propulsion systems, and unmanned aircraft in particular, can use hot surface energy addition to improve engine performance. An analysis of the thermomechanical stress behavior of hot surface ignition devices is therefore critical to ensure that they can satisfy new operational requirements. In this paper, a phenomenological heat-flux model is proposed to simulate heat generation inside a heating element. Two finite element analysis models are established using the proposed heat-flux model in order to characterize the transient thermomechanical behavior of an ignition assistant: a two-dimensional (2-D) axisymmetric model with an equivalent cylindrical heating element and a three-dimensional (3-D) solid model with realistic heating element geometry. The transient behavior of the ignition assistant is investigated at standard conditions by characterizing the temperature and thermal stress inside the device for various input voltages. The effect of the nonaxisymmetric heating element geometry on the temperature and thermal stress distribution is assessed. Furthermore, the 3-D ignition assistant model is used to analyze the thermomechanical behavior of an ignition device subjected to a combustion event inside a rapid compression machine. Multiple circumferential orientations of the heating element plane relative to the spray axis are investigated. Results demonstrate that the observed maximum principal stress depends significantly on heating element orientation.

关键词： Heat Flux Stress Distribution Heat Generation Unmanned Aerial Vehicle Propulsion System Surface Energy Adaptive Mesh Refinement Fuel Injection CFD Simulation Fracture Toughness

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Damage identification in 4D images of a nano-engineered composite via a deep-learning tool 23

Damage identification in 4D images of a nano-engineered comp...

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23rd International Conference on Composite materials, ICCM 2023

作者： Mehdikhani, Mahoor Upadhyay, Shailee Soete, Jeroen Swolfs, Yentl Smith, Abraham G. Ali Aravand, M. Liotta, Andrew H. Wicks, Sunny S. Wardle, Brian L. Lomov, Stepan V. Gorbatikh, Larissa Department of Materials Engineering KU Leuven Belgium Department of Computer Science University of Copenhagen Denmark School of Mechanical and Aerospace Engineering QUB UK Department of Aeronautics and Astronautics MIT US

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Data-driven modeling of dislocation mobility from atomistics using physicsinformed machine learning

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npj Computational materials 2024年第1期10卷 937-948页

作者： Yifeng Tian Soumendu Bagchi Liam Myhill GiacomoPo Enrique Martinez Yen Ting Lin Nithin Mathew Danny Perez Information Sciences Group ComputerComputational and Statistical Sciences Division(CCS-3)Los Alamos National LaboratoryLos Alamos87545 NMUSA Physics and Chemistry of Materials Theoretical Division(T-1)Los Alamos National LaboratoryLos Alamos87545 NMUSA Center for Nanophase Materials Sciences Oak Ridge National LaboratoryOak RidgeUSA Department of Materials Science and Engineering Clemson UniversityClemson29623 SCUSA Department of Mechanical and Aerospace Engineering University of MiamiMiami33146 FLUSA

Dislocationmobility,which dictates the response of dislocations to an applied stress,is a fundamental property of crystalline materials that governs the evolution of plastic *** approaches for deriving mobility laws rely on phenomenological models of the underlying physics,whose free parameters are in turn fitted to a small number of intuition-driven atomic scale simulations under varying conditions of temperature and *** tedious and time-consuming approach becomes particularly cumbersome for materials with complex dependencies on stress,temperature,and local environment,such as body-centered cubic crystals(BCC)metals and *** this paper,we present a novel,uncertainty quantification-driven active learning paradigm for learning dislocation mobility laws from automated high-throughput large-scale molecular dynamics simulations,using Graph Neural Networks(GNN)with a physics-informed *** demonstrate that this Physics-informed Graph Neural Network(PI-GNN)framework captures the underlying physics more accurately compared to existing phenomenological mobility laws in BCC metals.

关键词： stress dislocation consuming

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Bioinspired materials for droplet manipulation:Principles,methods and applications

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Droplet 2022年第1期1卷 11-37页

作者： Jinkai Xu Siyu Xiu Zhongxu Lian Huadong Yu Jiaji Cao Department of Mechanical Design Manufacturing and AutomationMinistry of Education Key Laboratory for Cross‐Scale Micro and Nano ManufacturingChangchun University of Science and TechnologyChangchunChina Department of Mechanical Materials and Process EngineeringSchool of EngineeringUniversity of WarwickCoventryUK Department of Mechanical and Electronic Engineering School of Mechanical and Aerospace EngineeringJilin UniversityChangchunChina

Droplet manipulation techniques such as transport and merging have been widely used in many fields including biology,chemistry,material and energy ***,droplet manipulation strategies have been extensively investigated and reviewed in terms of droplet placement on solid ***,less attention has been paid to the practice of droplet manipulation technology in other environments,limiting our understanding and the broadening of technology *** this article,we provided an overview of the recent progress in controlling droplets in various situations,including droplet manipulation on a surface mediated by the passive strategy(Laplace pressure and wettability gradients)and active strategy(electric field,magnetic field,light and heat).We also presented the principle of droplet manipulation and detailed the application of bionic surfaces in droplet manipulation,and the applications and prospects of droplet manipulation technology were summarized.

关键词： summarized limiting manipulation

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21-Component compositionally complex ceramics: Discovery of ultrahigh-entropy weberite and fergusonite phases and a pyrochlore–weberite transition

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Journal of Advanced Ceramics 2022年第4期11卷 641-655页

作者： Mingde QIN Heidy VEGA Dawei ZHANG Sarath ADAPA Andrew J.WRIGHT Renkun CHEN Jian LUO Department of Nano Engineering University of California San DiegoLa Jolla 92093USA Department of Chemistry and Biochemistry University of California San DiegoLa Jolla 92093USA Program of Materials Science and Engineering University of California San DiegoLa Jolla 92093USA Department of Mechanical and Aerospace Engineering University of California San DiegoLa Jolla 92093USA

Two new high-entropy ceramics(HECs)in the weberite and fergusonite structures,along with the unexpected formation of ordered pyrochlore phases with ultrahigh-entropy compositions and an abrupt pyrochlore–weberite transition,are discovered in a 21-component oxide *** the Gibbs phase rule allows 21 equilibrium phases,9 out of the 13 compositions examined possess single HEC phases(with ultrahigh ideal configurational entropies:~2.7kB per cation or higher on one sublattice in most cases).Notably,(15RE_(1/15))(Nb_(1/2)Ta_(1/2))O_(4) possess a single monoclinic fergusonite(C2/c)phase,and(15RE_(1/15))_(3)(Nb_(1/2)Ta_(1/2))_(1)O_(7) form a single orthorhombic(C222_(1))weberite phase,where 15RE_(1/15) represents Sc_(1/15)Y_(1/15)La_(1/15)Pr_(1/15)Nd_(1/15)Sm_(1/15)Eu_(1/15)Gd_(1/15)Tb_(1/15)Dy_(1/15)Ho_(1/15)Er_(1/15)Tm_(1/15) Yb_(1/15)Lu_(1/15).Moreover,a series of eight(15RE_(1/15))_(2+x)(Ti_(1/4)Zr_(1/4)Ce_(1/4)Hf_(1/4))_(2−2x)(Nb_(1/2)Ta_(1/2))_(x)O_(7) specimens all exhibit single phases,where a pyrochlore–weberite transition occurs within 0.75

关键词： compositionally complex ceramics high-entropy ceramics(HECs) weberite pyrochlore fergusonite ultrahigh-entropy ceramics many-component ceramics

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