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Technology Roadmap for Flexible Sensors

ACS NANO 2023年第6期17卷 5211-5295页

作者： Luo, Yifei Abidian, Mohammad Reza Ahn, Jong-Hyun Akinwande, Deji Andrews, Anne M. Antonietti, Markus Bao, Zhenan Berggren, Magnus Berkey, Christopher A. Bettinger, Christopher John Chen, Jun Chen, Peng Cheng, Wenlong Cheng, Xu Choi, Seon-Jin Chortos, Alex Dagdeviren, Canan Dauskardt, Reinhold H. Di, Chong-an Dickey, Michael D. Duan, Xiangfeng Facchetti, Antonio Fan, Zhiyong Fang, Yin Feng, Jianyou Feng, Xue Gao, Huajian Gao, Wei Gong, Xiwen Guo, Chuan Fei Guo, Xiaojun Hartel, Martin C. He, Zihan Ho, John S. Hu, Youfan Huang, Qiyao Huang, Yu Huo, Fengwei Hussain, Muhammad M. Javey, Ali Jeong, Unyong Jiang, Chen Jiang, Xingyu Kang, Jiheong Karnaushenko, Daniil Khademhosseini, Ali Kim, Dae-Hyeong Kim, Il-Doo Kireev, Dmitry Kong, Lingxuan Lee, Chengkuo Lee, Nae-Eung Lee, Pooi See Lee, Tae-Woo Li, Fengyu Li, Jinxing Liang, Cuiyuan Lim, Chwee Teck Lin, Yuanjing Lipomi, Darren J. Liu, Jia Liu, Kai Liu, Nan Liu, Ren Liu, Yuxin Liu, Yuxuan Liu, Zhiyuan Liu, Zhuangjian Loh, Xian Jun Lu, Nanshu Lv, Zhisheng Magdassi, Shlomo Malliaras, George G. Matsuhisa, Naoji Nathan, Arokia Niu, Simiao Pan, Jieming Pang, Changhyun Pei, Qibing Peng, Huisheng Qi, Dianpeng Ren, Huaying Rogers, John A. Rowe, Aaron Schmidt, Oliver G. Sekitani, Tsuyoshi Seo, Dae-Gyo Shen, Guozhen Sheng, Xing Shi, Qiongfeng Someya, Takao Song, Yanlin Stavrinidou, Eleni Su, Meng Sun, Xuemei Takei, Kuniharu Tao, Xiao-Ming Tee, Benjamin C. K. Thean, Aaron Voon-Yew Trung, Tran Quang Wan, Changjin Wang, Huiliang Wang, Joseph Wang, Ming Wang, Sihong Wang, Ting Wang, Zhong Lin Weiss, Paul S. Wen, Hanqi Xu, Sheng Xu, Tailin Yan, Hongping Yan, Xuzhou Yang, Hui Yang, Le Yang, Shuaijian Yin, Lan Yu, Cunjiang Yu, Guihua Yu, Jing Yu, Shu-Hong Yu, Xinge Zamburg, Evgeny Zhang, Haixia Zhang, Xiangyu Zhang, Xiaosheng Zhang, Xueji Zhang, Yihui Zhang, Yu Zhao, Siyuan Zhao, Xuanhe Zheng, Yuanjin Zheng, Yu-Qing Zheng, Zijian Zhou, Tao Zhu, Bowen Zhu, Ming Zhu, Rong Zhu, Yangzhi Zhu, Yong Zou, Guijin Chen, Xiaodong 08-03 Innovis Singapore 138634 Republic of Singapore Innovative Centre for Flexible Devices (iFLEX) School of Materials Science and Engineering Nanyang Technological University Singapore 639798 Singapore Department of Biomedical Engineering University of Houston Houston Texas 77024 United States School of Electrical and Electronic Engineering Yonsei University Seoul 03722 Republic of Korea Department of Electrical and Computer Engineering The University of Texas at Austin Austin Texas 78712 United States Microelectronics Research Center The University of Texas at Austin Austin Texas 78758 United States Department of Chemistry and Biochemistry California NanoSystems Institute and Department of Psychiatry and Biobehavioral Sciences Semel Institute for Neuroscience and Human Behavior and Hatos Center for Neuropharmacology University of California Los Angeles Los Angeles California 90095 United States Colloid Chemistry Department Max Planck Institute of Colloids and Interfaces 14476 Potsdam Germany Department of Chemical Engineering Stanford University Stanford California 94305 United States Laboratory of Organic Electronics Department of Science and Technology Campus Norrköping Linköping University 83 Linköping Sweden Wallenberg Initiative Materials Science for Sustainability (WISE) and Wallenberg Wood Science Center (WWSC) SE-100 44 Stockholm Sweden Department of Materials Science and Engineering Stanford University Stanford California 94301 United States Department of Biomedical Engineering and Department of Materials Science and Engineering Carnegie Mellon University Pittsburgh Pennsylvania 15213 United States Department of Bioengineering University of California Los Angeles Los Angeles California 90095 United States School of Chemistry Chemical Engineering and Biotechnology Nanyang Technological University Singapore 637457 Singapore Nanobionics Group Department of Chemical and Biological Engineering Monash University Clayton Australia 3800 Monash

Humans rely increasingly on sensors to address grand challenges and to improve quality of life in the era of digitalization and big data. For ubiquitous sensing, flexible sensors are developed to overcome the limitations of conventional rigid counterparts. Despite rapid advancement in bench-side research over the last decade, the market adoption of flexible sensors remains limited. To ease and to expedite their deployment, here, we identify bottlenecks hindering the maturation of flexible sensors and propose promising solutions. We first analyze continued...challenges in achieving satisfactory sensing performance for real-world applications and then summarize issues in compatible sensor-biology interfaces, followed by brief discussions on powering and connecting sensor networks. Issues en route to commercialization and for sustainable growth of the sector are also analyzed, highlighting environmental concerns and emphasizing nontechnical issues such as business, regulatory, and ethical considerations. Additionally, we look at future intelligent flexible sensors. In proposing a comprehensive roadmap, we hope to steer research efforts towards common goals and to guide coordinated development strategies from disparate communities. Through such collaborative

关键词： soft materials mechanics engineering flexible electronics conformable sensors bioelectronics human-machine interfaces body area sensor networks technology translation sustainable electronics

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Outcoupling Hyperbolic Modes from Aligned Carbon Nanotube Films

Outcoupling Hyperbolic Modes from Aligned Carbon Nanotube Fi...

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CLEO: QELS_Fundamental Science, QELS 2022

作者： Jerome, Bryant Prasad, Ciril S. Doumani, Jacques Dewey, Oliver S. Baydin, Andrey Pasquali, Matteo Kono, Junichiro Gao, Weilu Alabastri, Alessandro Naik, Gururaj V. Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Chemistry Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering University of Utah Salt Lake CityUT84112 United States

Aligned carbon nanotube films make an excellent hyperbolic material platform in the infrared. Here, we experimentally demonstrate the presence of high-k modes in aligned carbon nanotube films and outcouple them to fre... 详细信息

ISBN: (纸本)9781557528209

关键词： Carbon films

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Characterization of Water-Soluble Inorganic Ions and Carbonaceous Aerosols in the Urban Atmosphere in Amman, Jordan

SSRN

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SSRN 2024年

作者： Al-Hunaiti, Afnan Bakri, Zaid Li, Xinyang Duan, Lian Al-Abdallat, Asal Alastuey, Andres Viana, Mar Arar, Sharif Petäjä, Tuukka Hussein, Tareq Department of Chemistry School of Science University of Jordan Amman11942 Jordan Department of Chemistry and Materials Science School of Chemical Engineering Nanochemistry and Nanoengineering Aalto University Aalto00076 Finland Department of Physics and Atmospheric Sciences Program Michigan Technological University HoughtonMI49931 United States UHELFI- Helsinki00014 Finland Shanghai Key Laboratory of Atmospheric Particle Pollution and Prevention Department of Environmental Science & Engineering Fudan University Shanghai200438 China Department of Physics School of Science University of Jordan Amman11942 Jordan Barcelona08034 Spain

The Eastern Mediterranean is a unique region for air pollution because it is the crossroads between three continents exchanging air pollution. Here, we investigated urban particulate matter (PM) carbonaceous and water-soluble ions in Amman, Jordan. The PM2.5 total carbon (TC) annual mean was 7.6±3.6 µg/m3 (organic carbon (OC) 5.9±2.8 µg/m3 and elemental carbon (EC) 1.7±1.1 µg/m3), which was about 16.3% of the PM2.5. The PM10 TC annual mean was 8.4±3.9 µg/m3 (OC 6.5 ± 3.1 µg/m3 and elemental carbon (EC) 11.9±1.1µg/m3), about 13.3% of the PM10. The PM2.5 total water-soluble ions annual mean was 7.9±1.9 µg/m3 (about 16.9%), and that of the PM10 was 10.1±2.8 µg/m3 (about 16.0%). The minor ions (F-, NO2-, Br-, and PO43-) constituted less than 1% in the PM fractions. The significant fraction was for SO42- (PM2.5 4.7±1.6 µg/m3 (10.0%) and PM10 5.3±1.9 µg/m3 (8.3%)). The NH4+ had higher amounts of PM2.5 (1.3±0.6 µg/m3;2.7%) than that PM10 (0.9±0.4 µg/m3;1.4%). During sand and dust storm (SDS) events, TC, Cl-, and NO3- were doubled in PM, SO42- did not increase significantly, and NH4+ slightly decreased. Regression analysis revealed: (1) carbonaceous aerosols come equally from primary and secondary sources, (2) about 50% of the OC came from non-combustion sources, (3) traffic emissions dominate the PM, (4) agricultural sources have a negligible effect, (5) SO42- is completely neutralized by NH4+ in the PM2.5 but there could be additional reactions involved in the PM10, and (6) (NH4)2SO4, was the major species formed by SO42-and NH4+ instead of NH4HSO4. © 2024, The Authors. All rights reserved.

关键词： Ions

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Nanoslot-Induced Ultrastrong Phonon-Photon and Phonon-Phonon Coupling in Hybrid Organic-Inorganic Perovskites 16

Nanoslot-Induced Ultrastrong Phonon-Photon and Phonon-Phonon...

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16th Pacific Rim Conference on Lasers and Electro-Optics, CLEO-PR 2024

作者： Kim, Dasom Hou, Jin Lee, Geon Agrawal, Ayush Kim, Sunghwan Zhang, Hao Bao, Di Baydin, Andrey Wu, Wenjing Tay, Fuyang Huang, Shengxi Hagenmüller, Daivd Chia, Elbert E. M. Kim, Dai-Sik Seo, Minah Mohite, Aditya D. Kono, Junichiro Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Sensor System Research Center Korea Institute of Science and Technology Seoul02792 Korea Republic of Department of Physics and Astronomy Seoul National University Seoul08826 Korea Republic of Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Ulsan44919 Korea Republic of Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Smalley-Curl Institute Rice University HoustonTX77005 United States Université de Strasbourg Cnrs Strasbourg67000 France KU-KIST Graduate School of Converging Science and Technology Korea University Seoul02841 Korea Republic of Department of Physics and Astronomy Rice University HoustonTX77005 United States

Methods for harnessing vibrational states are desired for phonon-based technologies. We realized ultrastrong coupling of two phonon modes in perovskite materials induced by ultrastrong coupling with a common photonic ... 详细信息

ISBN: (纸本)9798350372076

关键词： Organic-inorganic materials

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Frontispiz: Synthesis of Erythrocyte Nanodiscs for Bacterial Toxin Neutralization

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Angewandte Chemie 2023年第21期135卷

作者： Dr. Lei Sun Dan Wang Dr. Ilkoo Noh Dr. Ronnie H. Fang Dr. Weiwei Gao Prof. Liangfang Zhang Department of NanoEngineering Chemical Engineering Program and Moores Cancer Center University of California San Diego La Jolla CA-92093 USA

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Frontispiece: Synthesis of Erythrocyte Nanodiscs for Bacterial Toxin Neutralization

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Angewandte Chemie International Edition 2023年第21期62卷

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Synthesis of Erythrocyte Nanodiscs for Bacterial Toxin Neutralization

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Angewandte Chemie 2023年第21期135卷

Nanodiscs are a compelling nanomedicine platform due to their ultrasmall size and distinct disc shape. Current nanodisc formulations are made primarily with synthetic lipid bilayers and proteins. Here, we report a cellular nanodisc made with human red blood cell (RBC) membrane (denoted “RBC-ND”) and show its effective neutralization against bacterial toxins. In vitro, RBC-ND neutralizes the hemolytic activity and cytotoxicity caused by purified α-toxin or complex whole secreted proteins (wSP) from methicillin-resistant Staphylococcus aureus bacteria. In vivo, RBC-ND confers significant survival benefits for mice intoxicated with α-toxin or wSP in both therapeutic and prevention regimens. Moreover, RBC-ND shows good biocompatibility and biosafety in vivo. Overall, RBC-ND distinguishes itself by inheriting the biological functions of the source cell membrane for bioactivity. The design strategy of RBC-ND can be generalized to other types of cell membranes for broad applications.

关键词： Bacterial Toxin Cell Membrane Cellular Nanodisc Detoxification Nanomedicine

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Suppressing chemical Corrosions of Lithium Metal Anodes

arXiv

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arXiv 2022年

作者： Lu, Bingyu Li, Weikang Cheng, Diyi Ceja, Miguel Bao, Wurigumula Fang, Chengcheng Meng, Ying Shirley Department of NanoEngineering University of California La Jolla San DiegoCA92093 United States Materials Science and Engineering Program University of California La Jolla San DiegoCA92093 United States Department of Chemical Engineering and Materials Science Michigan State University East LansingMI48824 United States Pritzker School of Molecular Engineering University of Chicago ChicagoIL60637 United States

The lithium (Li) metal anode is essential for next generation high energy density rechargeable Li metal batteries. Although extensive studies have been performed to prolong the cycle life of Li metal batteries, the calendar life, which associates with chemical corrosion of Li metal in liquid electrolytes, has not been quantitatively understood. Here, by combing the Titration Gas Chromatography (TGC) method and Cryogenic Focused Ion Beam (Cryo-FIB), we established a quantitative relationship between the chemical corrosion rate and electrochemically deposited Li morphology in various liquid electrolyte systems. We identified that the corrosion rate is dominated by the porosity of the deposited Li. The larger the porosity of deposited Li has, the faster the corrosion rate will be. We further proposed strategies to mitigate the chemical corrosion on Li thus to extend the calendar life of Li metal batteries. By strictly controlling the stacking pressure during Li plating, Li deposits with ultra-low porosity can be achieved, suppressing the corrosion rate to 0.08 ± 0.16%/day compared with 1.71 ± 0.19%/day of the high-porosity Li. Copyright © 2022, The Authors. All rights reserved.

关键词： Electrolytes

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Challenges for and Pathways toward Li-MetalBased All-Solid-State Batteries

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ACS ENERGY LETTERS 2021年第4期6卷 1399-1404页

作者： Albertus, Paul Anandan, Venkataramani Ban, Chunmei Balsara, Nitash Belharouak, Ilias Buettner-Garrett, Josh Chen, Zonghai Daniel, Claus Doeff, Marca Dudney, Nancy J. Dunn, Bruce Harris, Stephen J. Herle, Subramanya Herbert, Eric Kalnaus, Sergiy Libera, Joesph A. Lu, Dongping Martin, Steve McCloskey, Bryan D. McDowell, Matthew T. Meng, Y. Shirley Nanda, Jagjit Sakamoto, Jeff Self, Ethan C. Tepavcevic, Sanja Wachsman, Eric Wang, Chunsheng Westover, Andrew S. Xiao, Jie Yersak, Thomas Department of Chemical and Biomolecular Engineering University of Maryland College Park Maryland 20742 United States Ford Motor Company Dearborn Michigan 48121 United States Mechanical Engineering Department University of Colorado Boulder Colorado 80309 United States Department of Chemical and Biomolecular Engineering and Lawrence Berkeley National Laboratory Materials Sciences Division University of California Berkeley California 94720 United States Energy and Transportation Science Division Oak Ridge National Laboratory Oak Ridge Tennessee 37831 United States Solid Power Inc. Louisville Colorado 80027 United States Chemical Sciences and Engineering Division Argonne National Laboratory 9700 South Cass Avenue Argonne Illinois 60439 United States Lawrence Berkeley National Laboratory Energy Storage and Distributed Resources Division University of California Berkeley California 94720 United States Department of Materials Science and Engineering University of California Los Angeles California 90095 United States Applied Materials Inc. 3225 Oakmead Village Drive B12_2F6 Santa Clara California 95054 United States Department of Materials Science and Engineering Michigan Technological University Houghton Michigan 49931 United States Energy and Environmental Directorate Pacific Northwest National Laboratory Richland Washington 99352 United States Department of Materials Science & Engineering Iowa State University of Science & Technology Ames Iowa 50011 United States Woodruff School of Mechanical Engineering and School of Materials Science and Engineering Georgia Institute of Technology Atlanta Georgia 30332 United States Department of NanoEngineering and Materials Science and Engineering Program University of California San Diego La Jolla California 92093 United States Department of Materials Science and Engineering and Department of Mechanical Engineering University of Michigan Ann Arbor Michigan 48109 United States Chemical and Materials Systems Laborat

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A Biomimetic Nanoparticle to "Lure and Kill" Phospholipase A2

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Advanced Materials 2020年第26期132卷 10547-10551页

作者： Zhang, Qiangzhe Fang, Ronnie H. Gao, Weiwei Zhang, Liangfang Department of NanoEngineering Chemical Engineering Program and Moores Cancer Center University of California San Diego La Jolla CA92093 United States

Inhibition of phospholipase A2 (PLA2) has long been considered for treating various diseases associated with an elevated PLA2 activity. However, safe and effective PLA2 inhibitors remain unavailable. Herein, we report a biomimetic nanoparticle design that enables a "lure and kill" mechanism designed for PLA2 inhibition (denoted "L&K-NP"). The L&K-NPs are made of polymeric cores wrapped with modified red blood cell membrane with two inserted key components: melittin and oleyloxyethyl phosphorylcholine (OOPC). Melittin acts as a PLA2 attractant that works together with the membrane lipids to "lure" in-coming PLA2 for attack. Meanwhile, OOPC acts as inhibitor that "kills" PLA2 upon enzymatic attack. Both compounds are integrated into the L&K-NP structure, which voids toxicity associated with free molecules. In the study, L&K-NPs effectively inhibit PLA2-induced hemolysis. In mice administered with a lethal dose of venomous PLA2, L&K-NPs also inhibit hemolysis and confer a significant survival benefit. Furthermore, L&KNPs show no obvious toxicity in mice. and the design provides a platform technology for a safe and effective anti-PLA2 approach. © 2020 Wiley-VCH Verlag GmbH & Co. KGaA, Weinheim.

关键词： Toxicity

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