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arXiv 2025年

作者： Calvat, Mathieu Bean, Chris Anjaria, Dhruv Park, Hyoungryul Wang, Haoren Vecchio, Kenneth Stinville, J.C. Materials Science and Engineering Department University of Illinois Urbana-Champaign UrbanaIL United States Department of NanoEngineering University of California San Diego La Jolla San DiegoCA United States

To leverage advancements in machine learning for metallic materials design and property prediction, it is crucial to develop a data-reduced representation of metal microstructures that surpasses the limitations of current physics-based discrete microstructure descriptors. This need is particularly relevant for metallic materials processed through additive manufacturing, which exhibit complex hierarchical microstructures that cannot be adequately described using the conventional metrics typically applied to wrought materials. Furthermore, capturing the spatial heterogeneity of microstructures at the different scales is necessary within such framework to accurately predict their properties. To address these challenges, we propose the physical spatial mapping of metal diffraction latent space features. This approach integrates (i) point diffraction data encoding via variational autoencoders or contrastive learning and (ii) the physical mapping of the encoded values. Together these steps offer a method offers a novel means to comprehensively describe metal microstructures. We demonstrate this approach on a wrought and additively manufactured alloy, showing that it effectively encodes microstructural information and enables direct identification of microstructural heterogeneity not directly possible by physics-based models. This data-reduced microstructure representation opens the application of machine learning models in accelerating metallic material design and accurately predicting their properties. © 2025, CC BY-NC-SA.

关键词： Mapping

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Design of Mixed-Dimensional QDs/MoS2/TiO2 Heterostructured Resistive Random-Access Memory with Interfacial Analog Switching Characteristics for Potential Neuromorphic Computing

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ACS Applied Electronic materials 2024年第3期6卷 1581-1589页

作者： Tang, Shin-Yi Shih, Yu-Chuan Shen, Ying-Chun Cyu, Ruei-Hong Chen, Chieh-Ting Yang, Tzu-Yi Chaudhary, Mayur Peng, Yu-Ren Kuo, Yao-Ren Miao, Wen-Chien Yu, Yi-Jen Lee, Ling Kuo, Hao-Chung Chueh, Yu-Lun Department of Materials Science and Engineering National Tsing Hua University Hsinchu30013 Taiwan College of Semiconductor Research National Tsing Hua University Hsinchu30013 Taiwan Semiconductor Research Center Hon Hai Research Institute Taipei11492 Taiwan Ph. D. Program in Prospective Functional Materials Industry National Tsing Hua University Hsinchu30013 Taiwan Department of Electrophysics College of Science National Yang Ming Chiao Tung University Hsinchu30010 Taiwan Instrument Center National Tsing Hua University Hsinchu30013 Taiwan Department of Photonics Institute of Electro-Optical Engineering National Yang-Ming Chiao Tung University Hsinchu30010 Taiwan Department of Physics National Sun Yat-Sen University Kaohsiung80424 Taiwan Department of Materials Science and Engineering Korea University Seoul02841 Korea Republic of

Resistive random-access memory (RRAM) is one of the most promising candidates for next-generation nanoscale nonvolatile memory devices and neuromorphic computing applications. In this study, we developed a novel mixed-dimensional design for RRAM devices, incorporating zero-dimensional quantum dots (QDs), two-dimensional MoS2, and a TiO2 switching layer to achieve prominent interfacial switching behaviors. Compared with typical filamentary RRAM devices, the proposed heterostructure featured a light-sensitive QDs/MoS2 layer that allowed for bias-controllable resistive changes during the set and reset processes without abrupt switching. This was endowed by effective electron-hole pair separations upon excitation and the generation of a thin molybdenum oxide (MoOx) layer due to the accumulation of oxygen ions at the interface between MoS2 and TiO2. The ITO/QDs/MoS2/TiO2/Pt RRAM device exhibited an on/off ratio of 10 with improved endurance under 515 nm laser illumination and wavelength-dependent resistive switching behavior, making it useful for multilevel storage. Furthermore, the heterostructured device demonstrated synaptic characteristics with enhanced potentiation and depression nonlinearities and asymmetry factors, revealing its potential for future neuromorphic applications. © 2024 American Chemical Society.

关键词： Titanium dioxide

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Uncovering In-Plane Domain Structures in Two-Dimensional Ferroelectric SnSe Using Machine-Learning Assisted 4D-STEM

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Microscopy and Microanalysis 2022年第S1期28卷 374-375页

作者： Shi, Chuqiao Mao, Nannan Kong, Jing Han, Yimo Department of Materials Science and NanoEngineering Rice University Houston TX Department of Electrical Engineering and Computer Science Massachusetts Institute of Technology Cambridge MA

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Enhancement of piezophototronic hydrogen evolution reaction through the polarization of ferroelectric Bi4Ti3O12 microplates

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International Journal of Hydrogen Energy 2024年 50卷 15-25页

作者： Chang, Shun Cheng Chen, Po-Han Chen, Yu-Ching Wu, Jyh Ming Department of Materials Science and Engineering National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan High Entropy Materials Center National Tsing Hua University Section 2 Kuang Fu Road 101 Hsinchu300 Taiwan Ph.D. Program in Prospective Functional Materials Industry National Tsing Hua University 101 Section 2 Kuang Fu Road Hsinchu300 Taiwan

In this study, we analyzed the properties of Bi4Ti3O12 microplates in the context of hydrogen evolution reaction. Piezoresponse force microscopy revealed a typical butterfly curve, indicating that as-synthesized Bi4Ti3O12 exhibits ferroelectric properties. Under ultrasonication, the amount of hydrogen produced by polarized (2000 V) Bi4Ti3O12 increased from 728 to 1349 μmol g−1, which was 1.85 times higher than that generated by unpolarized Bi4Ti3O12. The increase in hydrogen evolution rate may be attributed to the gradual alignment of polarization within the ferroelectric domains of Bi4Ti3O12. Moreover, with synergistic piezophototronic activity, the amount of hydrogen produced by Bi4Ti3O12 was further increased to 1478 μmol g−1, which was 200% higher than that generated by unpolarized Bi4Ti3O12. Theoretical calculations revealed that Bi4Ti3O12 microplates exhibit a high piezoelectric potential along the x-axis, which is consistent with the spontaneous polarization of the microplates. By applying an external polarization field, ferroelectric polarization was activated to effectively separate free charges and extend carrier lifetime (from 0.6 to 0.84 ns). The application of an external electric field to ferroelectric Bi4Ti3O12 appears to be a favorable strategy for enhancing its piezophototronic activity. Our findings may facilitate future studies in the fields of environmental science and renewable energy. © 2023 Hydrogen Energy Publications LLC

关键词： Bismuth compounds

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Preparation of LFP-based cathode materials for lithium-ion battery applications

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materials Today: Proceedings 2022年 65卷 2347-2350页

作者： Suttison, Suchanat Pengpat, Kamonpan Intatha, Uraiwan Fan, Jinchen Zhang, Wei Eitssayeam, Sukum Master's Degree Program in Materials Science Faculty of Science Chiang Mai University Chiang Mai 50200 Thailand Graduate School Chiang Mai University Chiang Mai Thailand Department of Physics and Materials Science Faculty of Science Chiang Mai University Thailand Center of Innovative Materials for Sustainability School of Science Mae Fah Luang University Chiang Rai 57100 Thailand School of Materials and Chemistry University of Shanghai for Science and Technology Shanghai 200093 China Department of Engineering Mechanics Dalian University of Technology Dalian 116024 China

Lithium-ion batteries (LIB) have developed into the mainstream power source of energy storage devices due to their advantages: high power density, high power, long service life, and less pollution. This materials development for LFP batteries was considered successful in synthesizing powder. Here we show that three synthesis conditions were performed. LFP doped NiO, NMC, and (NH4)2HPO4 were synthesized by the nitrogen gas flow method. LFP-doped NiO was burned at 600 °C and 700 °C for five h. NMC doped with LFP burned at 550 °C for five h, and NMC-doped LFP and (NH4)2HPO4 were burned at 550 °C and 600 °C for five h. The structure and morphology of the material were examined by X-ray diffraction (XRD) and scanning electron microscopy (SEM). © 2022

关键词： Lithium-ion batteries

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Correlating the Ambient Conditions and Performance Indicators of the LoRaWAN via Surrogate Gaussian Process-Based Bidirectional LSTM Stacked Autoencoder

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IEEE Transactions on Network and Service Management 2023年第3期20卷 3413-3427页

作者： Bhat, Showkat Ahmad Huang, Nen-Fu Hussain, Imtiyaz Sajjad, Uzair National Tsing Hua University College of Electrical and Computer Science Hsinchu1300044 Taiwan National Tsing Hua University Department of Computer Science Hsinchu1300044 Taiwan National Taipei University of Technology Graduate Program in Energy and Opto-Electronic Materials Taipei10608 Taiwan National Taipei University of Technology Department of Energy and Refrigerating Airconditioning Engineering Taipei10608 Taiwan

LoRa's biggest advantage is its flexibility, which is the ability to increase or decrease data rate and range while decreasing or increasing sensitivity. Whenever propagation conditions change frequently, this function allows the spreading factor to be modified accordingly. Despite their efficiency and scalability, adaptive data rate algorithms ignore and fail to factor in the complex correlation between ambient weather parameters influencing the communication channel design. In this research, a Bayesian surrogate Gaussian process-based bidirectional LSTM stacked autoencoder model (BSGP-BLSTM-SAE) is proposed to estimate the channel performance indicators such as received signal strength indicator (RSSI) and signal-to-noise ratio (SNR) and to determine the correlation between the ambient weather conditions and performance indicators for the LoRaWAN network. Bayesian optimization algorithm has been used to optimize the hyper-parameters of the developed model. A LoRaWAN experimental multivariate time series dataset has been used for the evaluation of the developed model, which upon testing and validation produces high accuracy in predicting the channel performance indicators and ambient conditions of the experimental LoRaWAN network. The mean absolute error of the developed model was around 0.45. Thus, the proposed model can predict the link performance indicators and thereby assist in real-time optimization of the transmission parameters to enhance the network performance in LoRaWAN-based systems at different ambient conditions. © 2004-2012 IEEE.

关键词： Internet of things

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Characterizing catalyst function and transformations in the plasma reduction of CO₂ on atomic layer deposition-synthesized catalysts

RSC Applied Interfaces

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RSC Applied Interfaces 2024年第3期1卷 552-563页

作者： Conlin, Samuel K. Mehrabi, Hamed Parette, David N. Nichols, Eva M. Coridan, Robert H. Department of Chemistry and Biochemistry University of Arkansas Fayetteville 72701 AR United States Materials Science and Engineering Program University of Arkansas Fayetteville 72701 AR United States Department of Chemistry University of British Columbia Vancouver V6T 1Z1 BC Canada

The enhancement of CO2 reduction in atmospheric-pressure, non-thermal plasma has been shown using a variety of catalyst systems with ranging composition, particle sizes, and morphologies. Improvements in CO2 conversio...

The enhancement of CO₂ reduction in atmospheric-pressure, non-thermal plasma has been shown using a variety of catalyst systems with ranging composition, particle sizes, and morphologies. Improvements in CO₂ conversion can be attained by choice of catalyst material. However, inhomogeneity in the material distribution arising from the synthesis affects the catalytically active surface area and dielectric environment that modulates the plasma properties near the catalyst. Atomic layer deposition (ALD) can be used to control the composition of ultra-thin layers on support materials. We used ALD to synthesize metal oxide catalyst coatings on high surface area supports. We found that TiO₂ achieved significantly higher yields of CO₂ conversion (to CO and O₂) at low reactor power compared to ZnO or Al₂O₃, materials commonly used as a support for other catalysts. We also observed an unexpected increase in the catalytic activity on ZnO with increasing power. The results here suggest that ALD can unambiguously isolate the catalytic effects of materials in plasma reactors. © 2024 RSC.

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Fully rubbery synaptic transistors made out of all-organic materials for elastic neurological electronic skin

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Nano Research 2022年第2期15卷 758-764页

作者： Hyunseok Shim Seonmin Jang Jae Gyu Jang Zhoulyu Rao Jong-ln Hong Kyoseung Sim Cunjiang Yu Materials Science and Engineering Program University of HoustonHoustonTX 77204 USA Department of Chemistry Seoul National UniversitySeoul 08826Republic of Korea Department of Chemistry Ulsan National Institute of Science and Technology(UNIST)Ulsan 44919Republic of Korea Department of Mechanical Engineering University of HoustonHoustonTX 77204 USA Department of Biomedical Engineering University of HoustonHoustonTX 77204USA Department of Electrical and Computer Engineering University of HoustonHoustonTX 77204 USA Texas Center for Superconductivity University of HoustonHoustonTX 77204USA

Neurologic function implemented soft organic electronic skin holds promise for wide range of applications,such as skin prosthetics,neurorobot,bioelectronics,human-robotic interaction(HRI),***,we report the development of a fully rubbery synaptic transistor which consists of all-organic materials,which shows unique synaptic characteristics existing in biological *** synaptic characteristics retained even under mechanical stretch by 30%.We further developed a neurological electronic skin in a fully rubbery format based on two mechanoreceptors(for synaptic potentiation or depression)of pressure-sensitive rubber and an all-organic synaptic *** converting tactile signals into Morse Code,potentiation and depression of excitatory postsynaptic current(EPSC)signals allow the neurological electronic skin on a human forearm to communicate with a robotic *** collective studies on the materials,devices,and their characteristics revealed the fundamental aspects and applicability of the all-organic synaptic transistor and the neurological electronic skin.

关键词： synaptic transistor stretchable electronic skin all-organic

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Thermal energy dependent transient permittivity of epsilon-near-zero material

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science China(Physics,Mechanics & Astronomy) 2022年第8期65卷 96-101页

作者： Heng Wang Lixun Sun Kang Du Wending Zhang SooJin Chua Guixin Li Ting Mei MOE Key Laboratory of Material Physics and Chemistry under Extraordinary Conditions and Shaanxi Key Laboratory of Optical Information TechnologySchool of Physical Science and TechnologyNorthwestern Polytechnical UniversityXi’an710129China Department of Materials Science and Engineering Southern University of Science and TechnologyShenzhen518055China Shenzhen Institute for Quantum Science and Engineering Southern University of Science and TechnologyShenzhen518055China Department of Electrical and Computer Engineering National University of SingaporeSingapore117583Singapore LEES Program Singapore-MIT Alliance for Research&Technology(SMART)Singapore138602Singapore

Transparent conductive oxides exhibit attractive optical nonlinearity with ultrafast response and giant refractive index change near the epsilon-near-zero(ENZ) wavelength, originating from the intraband dynamics of conduction electrons. The optical nonlinearity of ENZ materials has been explained by using the overall-effective-mass and the overall-scattering-time of electrons in the extended Drude model. However, their response to optical excitation is yet the last building block to complete the theory. In this paper, the concept of thermal energy is theoretically proposed to account for the total energy of conduction electrons exceeding their thermal equilibrium value. The time-varying thermal energy is adopted to describe the transient optical response of indium-tin-oxide(ITO), a typical ENZ material. A spectrally-resolved femtosecond pump-probe experiment was conducted to verify our theory. By correlating the thermal energy with the pumping density, both the giant change and the transient response of the permittivity of ITO can be predicted. The results in this work provide a new methodology to describe the transient permittivities of ENZ materials, which will benefit the design of ENZ-based nonlinear photonic devices.

关键词： epsilon-near-zero optical nonlinearity transient response thermal energy hot electron indium tin oxide

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The Feather Structure and Bioinspired Rachis Design

SSRN

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SSRN 2024年

作者： Velasco-Hogan, Audrey Tavares, Sheron S. Lazarus, Benjamin Mahrous, Mahmoud A. Jasiuk, Iwona Meyers, Marc Andre Materials Science and Engineering Program University of California San Diego United States Department of Civil and Environmental Engineering University of Illinois at Urbana-Champaign UrbanaIL United States Mechanical Science and Engineering Department University of Illinois at Urbana-Champaign United States Depts. Of Nanoengineering and Mechanical and Aerospace Engineering University of California San Diego United States

The feather structure is comprised of a central shaft, lateral barbs and a network of barbules connecting them. These three components act synergistically to provide lift and damage recovery. The feather shaft is the predominant load-bearing component of the feather and is composed of the calamus and the rachis. Both the shaft and barbs consist of an external hollow shell filled with cellular keratin. Quantitative measurements of core (medulla) density and viscoelastic parameters are made across several avian species. There is a notable decrease in both storage and loss moduli with the mass of the birds. The mechanics of the feather shaft are explored through 3D-printed bioinspired designs to investigate structure-property relationships with respect to flight. Sandwich structures inspired by the feather shaft are printed with and without a foam core to establish flexural properties. The flexural strength of the sandwich structure increases with the addition of a foam core, due to the increase in the resistance to buckling and a modest moment of inertia. However, the stiffness is not significantly altered with the addition of the core. It is primarily determined by the cortex since the foam provides negligible moment of inertia. Both experiments and analysis on synthetic systems demonstrate that the feather rachis uses a highly optimized design. © 2024, The Authors. All rights reserved.

关键词： Viscoelasticity

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