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arXiv 2023年

作者： Abbasi, Mahdiyeh Liao, Shusen Zhu, Yunxuan Natelson, Douglas Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics and Astronomy Engineering Rice University HoustonTX77005 United States Department of Materials Science and Nanoengineering Rice University HoustonTX77005 United States

Tunneling metal-insulator-metal (MIM) junctions can exhibit an open-circuit photovoltage (OCPV) response under illumination that may be useful for photodetection. One mechanism for photovoltage generation is hot carrier tunneling, in which photoexcited carriers generate a net photocurrent that must be balanced by a drift current in the open-circuit configuration. We present experiments in electromigrated planar MIM structures, designed with asymmetric plasmonic properties using Au and Pt electrodes. Decay of optically excited local plasmonic modes preferentially creates hot carriers on the Au side of the junction, leading to a clear preferred directionality of the hot electron photocurrent and hence a preferred polarity of the resulting OCPV. In contrast, in an ensemble of symmetric devices constructed from only one Au, polarity of the OCPV has no preferred direction. Copyright © 2023, The Authors. All rights reserved.

关键词： Plasmonics

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Self-templated formation of cobalt-embedded hollow N-doped carbon spheres for efficient oxygen reduction

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Nano Research 2021年第8期14卷 2819-2825页

作者： Ayaz Mahsud Jianian Chen Xiaolei Yuan Fenglei Lyu Qixuan Zhong Jinxing Chen Yadong Yin Qiao Zhang Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesJoint International Research Laboratory of Carbon-Based Functional Materials and DevicesSoochow University199 Ren’ai RoadSuzhou 215123China School of Chemistry and Chemical Engineering Nantong UniversityNantong9 Seyuan RoadNantong226019China Department of Chemistry Materials Science and Engineering programand UCR Center for CatalysisUniversity of CaliforniaRiversideCA 92521USA

The slow kinetics at the cathode of oxygen reduction reaction(ORR)seriously limits the efficiencies of fuel cells and metal-air ***,the state-of-the-art ORR electrocatalyst,suffers from high cost,low earth abundance,and poor *** a self-templated strategy based on metal-organic frameworks(MOFs)is proposed for the fabrication of hollow nitrogen-doped carbon spheres that are embedded with cobalt nanoparticles(Co/HNC).The Co/HNC manifests better ORR activities,methanol tolerance,and stability than commercial Pt/*** high ORR performance of Co/NHC can be attributed to the hollow structure which provides enlarged electrochemically active surface area,the formation of more Co-N species,and the introduction of *** work highlights the significance of rational engineering of MOFs for enhanced ORR activity and stability and offers new routes to the design and synthesis of high-performance electrocatalysts.

关键词： cobalt self-templated metal organic framework hollow sphere oxygen reduction reaction

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Characterization of Nanocomposite Membrane Based Bacterial Cellulose Made of Pineapple Waste Reinforced by Graphite Nanoplatelets

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Journal of Renewable materials 2022年第9期10卷 2465-2475页

作者： Heru Suryanto Bili Darnanto Susilo Jibril Maulana Aminnudin Uun Yanuhar Surjani Wonorahardjo Husni Wahyu Wijaya Abu Saad Ansari Center of Excellence for Cellulose Composite(CECCom) Department of Mechanical EngineeringUniversitas Negeri MalangMalang65145Indonesia Centre of Advanced Material for Renewable Energy(CAMRY) Universitas Negeri MalangMalang65145Indonesia Master Program of Mechanical Engineering Faculty of EngineeringUniversitas Negeri MalangMalang65145Indonesia Department of Aquatic Resources Management Faculty of Fisheries and Marine SciencesBrawijaya UniversityMalang65145Indonesia Department of Chemistry Faculty of Mathematics and Natural SciencesUniversitas Negeri MalangMalang65145Indonesia Department of Materials Science&Engineering Incheon National UniversityIncheon464-742South Korea

Waste is the main problem for the *** waste for various useful applications has a benefit for the *** work has been studied for handling pineapple peel waste to make composite film bacterial cellulose nanocomposite membrane(BCNM)with addition graphite nanoplatelet(GNP).The concentration of GNP in the membrane influence the membrane *** bacterial cellulose(BC)pellicle was synthesized by using media from pineapple peel waste *** pellicle is cleaned with water and NaOH solution to be free from *** is synthesized through the mechanical disintegration *** results of disintegration using high pressure homogenizer at 150 bar and five ***/GNP is synthesized with varying addition of GNP of 2.5,5.0,10 and 100 wt%of dry bacterial nanocellulose(BNC).The BC and GNP solution were dried in an oven for 14 h at 80℃.BCNM morphology was observed using *** is dispersed and distributed in the BC matrix as *** analysis shows many peaks of BNC less pronounced with increasing of *** higher concentration of GNP,the rougher of *** optimum tensile strength of BCNM was achieved after addition GNP of 2.5 wt%.

关键词： Bacterial nanocellulose graphite nanoplatelet membrane nanocomposite pineapple waste

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Epilayer on NEAT Grown GaN Schottky Diodes for Radiation Detection

Epilayer on NEAT Grown GaN Schottky Diodes for Radiation Det...

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2023 Transactions of the American Nuclear Society Annual Meeting and Technology Expo, ANS 2023

作者： Remy, Jarod Zhang, Yuxuan Talesara, Vishank Zhao, Hongping Lu, Wu Hashimoto, Tadao Cao, Lei R. Nuclear Engineering Program Department of Mechanical and Aerospace Engineering 281 W. Lane Ave. ColumbusOH43210 United States Department of Electrical and Computer Engineering 281 W. Lane Ave ColumbusOH43210 United States Department of Material Science and Engineering The Ohio State University 281 W. Lane Ave ColumbusOH43210 United States SixPoint Materials Inc 37 Industrial Way STE 106 BuelltonCA United States

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Non-Hermitian selective thermal emitter for thermophotovoltaics

Non-Hermitian selective thermal emitter for thermophotovolta...

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Conference on Lasers and Electro-Optics (CLEO)

作者： Ciril S. Prasad Samuel C. Raphaelson Gururaj V. Naik Department of Electrical and Computer Engineering Rice University Houston TX USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston TX USA Department of Material Science and NanoEngineering Rice University Houston TX USA

Selective thermal emitters can boost the efficiency of heat-to-electricity conversion in thermophotovoltaic systems only if their spectral selectivity is high. We demonstrate a non-Hermitian metasurface-based selectiv... 详细信息

ISBN: (纸本)9781957171258

关键词： Emissivity Light intensity Optical constants Silicon Temperature Thermal emission

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Computational inverse design of acoustoplasmonic metasurfaces

arXiv

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arXiv 2025年

作者： Holland, Julia E. Boechler, Nicholas Poulikakos, Lisa V. Department of Mechanical & Aerospace Engineering UC La Jolla San DiegoCA92093-0021 United States Program in Materials Science & Engineering UC La Jolla San DiegoCA92093-0021 United States

Optical and acoustic metasurfaces are two-dimensional arrays of subwavelength elements that locally modulate or phase shift incident waves. Acoustoplasmonic metasurfaces combine the physics of light and sound, producing acoustic wavefronts in response to optical stimuli. Herein, we present a computational inverse acoustoplasmonic metasurface design algorithm for desired optically-generated acoustic wave fields. We consider gold nanoparticles producing spherical acoustic waves in water, and the resulting acoustic wave propagation along the plane containing the nanoparticle array. We demonstrate how our algorithm can be used to design metasurfaces that can be used to achieve complex acoustic wave fields. This includes the design of a single metasurface that produces acoustic wave fields mimicking two different Morse code patterns upon stimulation with two orthogonal polarization states of light. This work provides a new tool for the design of complex optically generated acoustic wavefronts, enabling functionality beyond what would be achievable with off-optical-resonance optoacoustic excitation. Copyright © 2025, The Authors. All rights reserved.

关键词： Acoustic wave propagation

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New insight into pyrrolic-N site effect towards the first NIR window absorption of pyrrolic-N-rich carbon dots

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Nano Research 2023年第4期16卷 6001-6009页

作者： Fitri Aulia Permatasari Reza Umami Citra Deliana Dewi Sundari Tirta Rona Mayangsari Atthar Luqman Ivansyah Fahdzi Muttaqien Takashi Ogi Ferry Iskandar Department of Physics Faculty Mathematics and Natural SciencesInstitut Teknologi BandungJalan Ganesha 10BandungWest Java 40132Indonesia Collaboration Research Center for Advanced Energy Materials National Research and Innovation Agency-Institut Teknologi BandungJalan Ganesha 10BandungWest Java 40132Indonesia Department of Chemistry Faculty of Mathematics and Natural SciencesInstitut Teknologi BandungJl.Ganesha 10BandungWest Java 40132Indonesia Department of Chemistry Education UIN Sunan Gunung Djati BandungJl.CimincrangBandungWest Java 40292Indonesia Department of Chemistry Universitas PertaminaJakarta 12220Indonesia Master Program in Computational Science Faculty of Mathematics and Natural SciencesInstitut Teknologi BandungJl.Ganesha 10BandungWest Java 40132Indonesia Instrumentation and Computational Physics Research Group Faculty of Mathematics and Natural SciencesInstitut Teknologi BandungJl.Ganesha 10Bandung 40132Indonesia Research Center for Nanoscience and Nanotechnology Institut Teknologi BandungJalan Ganesha 10BandungWest Java 40132Indonesia Chemical Engineering Program Department of Advanced Science and EngineeringGraduate School of Advanced Science and EngineeringHiroshima UniversityHigashi-Hiroshima 739-8527Japan

Controlled C-N configurations,i.e.,pyrrolic-N,pyridinic-N,and graphitic-N,are promising strategies to tailor the carbon dots’(CDs)optical properties into the first near infrared(NIR)window(650-900 nm),a responsive range for biomedical ***,a deep understanding of the role of the C-N configuration in the CDs’properties is still challenging and thoughtprovoking owing to their complex ***,an underlying pyrrolic-N concentration and position effect on the pyrrolic-N-rich CDs’absorption was comprehensively elucidated based on the integrated experimental and computational *** assynthesized pyrrolic-N-rich CDs exhibit a first NIR window absorption centered at 650 nm with high photothermal ***-N concentrations from 1.4%to 11.3%and positions(edge and mid-site)were systematically investigated.A mid-site pyrrolic-N was subsequently generated after the pyrrolic-N concentration more than 10%.Edge-site pyrrolic-N induces a frontier orbital hybridization,reducing bandgap energy,while mid-site pyrrolic-N plays a critical role in inducing a first NIR window absorption owing to their high charge ***,pyrrolic-N-rich CDs inherit a bowl-like topological feature,elevating the CDs’layer thickness as much as 0.71 *** study shed light on the design and optimization of pyrrolic-N on CDs for the first NIR window responsive materials in any biomedical application.

关键词： absorption carbon dots charge transfer first near infrared(NIR)window frontier orbital hybridization mid-site pyrrolic-N

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Alternative photothermal/electrothermal hierarchical membrane for hypersaline water treatment

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SusMat 2022年第6期2卷 679-688页

作者： Miao Wang Wen He Yuhui Hua Xinwen Xie Shiyan Chen Lei Zhou Yunmao Zhang Yaqi Hou Shihong Lin Haiping Xia Jing Zheng Xu Hou State Key Laboratory of Physical Chemistry of Solid Surfaces Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenChina College of Materials Xiamen UniversityXiamenChina Research Institute for Biomimetics and Soft Matter Fujian Provincial Key Laboratory for Soft Functional Materials ResearchJiujiang Research InstituteCollege of Physical Science and TechnologyXiamen UniversityXiamenChina Shenzhen Grubbs Institute and Guangdong Provincial Key Laboratory of Catalysis Department of ChemistrySouthern University of Science and TechnologyShenzhenChina Collaborative Innovation Center of Chemistry for Energy Materials(iChEM) Xiamen UniversityXiamenChina Department of Civil and Environmental Engineering Vanderbilt UniversityNashvilleTennesseeUSA Interdisciplinary Material Science Program Vanderbilt UniversityNashvilleTennesseeUSA Tan Kah Kee Innovation Laboratory Xiamen UniversityXiamenChina Engineering Research Center of Electrochemical Technologies of Ministry of Education Department of ChemistryCollege of Chemistry and Chemical EngineeringXiamen UniversityXiamenChina

Over the last decades,the treatment of the large quantities of hypersaline wastewater generated by conventional industries,inland desalination,and fossil-fueled power plants has been an important economic issue and also an inescapable green ***,we developed a versatile interfacial heating membrane with alternating utilization of electricity or solar energy for hypersaline water *** hierarchical membrane functions both as a separation membrane and an interface heater,which can quickly(<0.1 s)convert electricity or solar energy into heat to evaporate the outermost layer of hypersaline *** 10wt% hyper-saline water,the freshwater production rate can reach 16.8kg/m^(2)⋅h by applying a voltage of 10 V and 1.36 kg/m^(2)⋅h under 1-sun ***,it exhibits high electrochemical resistance to corrosion and therefore remains stable tack-ling hypersaline water(>5 wt%),with a high salt rejection rate of 99.99%.This system shows an efficient desalination strategy that can provide fresh water from brines for agriculture and industry,and even for daily life.

关键词： carbon nanotubes electrothermal hypersaline water treatment interface evaporate pho-tothermal

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Rational effect of CuSe2phase with octadecyl amine modified reduced graphene composite for dual-mode sensing of environmental hazardous anthelminthic drug in aquatic and biological samples

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Journal of Environmental Chemical engineering 2023年第1期11卷

作者： Hwa, Kuo-Yuan Ganguly, Anindita Santhan, Aravindan Department of Molecular Science and Engineering National Taipei University of Technology Taipei Taiwan International Graduate Program in Energy and Optoelectronic Materials National Taipei University of Technology Taipei Taiwan

The increasing usage of antihelminthic drug mebendazole (MEB) in humans and livestock poses serious threat and is considered a significant environmental pollutant. Hence, monitoring the MEB residues in environmental samples, and human fluids is essential to decrease the ecological risk and improve the health of humans. In this work, copper selenide (CuSe2) nano/microspheres were hydrothermally synthesized and ultrasonically treated with rGO surface modified with ODA alkyl amine (rGO-ODA). The optical, structural, morphological, and functional analysis were performed which revealed the CuSe2 in marcasite phase, orthorhombic pattern with Pnnm space group, and substantial composite formation. The morphological studies revealed sphere structure of the CuSe2 and wrinkled sheets of rGO-ODA. A sensor that detects MEB using the cyclic voltammetry (CV), differential pulse voltammetry (DPV) and UV-Vis absorbance techniques was developed. For DPV analysis, the sensor exhibited a very low value for limit of detection 13.55 nM and a sensitivity of 9.4871 μA M-1cm-2. For UV-Vis, the sensor demonstrated a very low limit of detection 22.3 nM. The use of this sensor was validated in real-time analysis with aquatic and biological real samples. The results suggested > 90% of analyte recovery and enhanced efficiency for MEB detection with a potential for commercialization in future. © 2022 Elsevier Ltd.

关键词： Copper compounds

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Photon avalanche-driven multicolor emission: yttrium vanadate upconversion phosphors for optical thermometry, forensics, and healing light applications

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Chemical engineering Journal 2025年 516卷

作者： Pavitra, Eluri Antony, Lintymol Park, Jin Young Hwang, Seung Kyu Lee, Jeong-Hwan Chandra, Gogineni Rajesh Basaveswara Rao, M.V. Raju, Ganji Seeta Rama Han, Young-Kyu Huh, Yun Suk NanoBio High-Tech Materials Research Center Department of Biological Sciences and Bioengineering Inha University Incheon22212 Korea Republic of 3D Convergence Center Inha University Incheon22212 Korea Republic of Department of Energy and Materials Engineering Dongguk University-Seoul Seoul04620 Korea Republic of Department of Electrical Electronics and Software Engineering Pukyong National University Yongdang Campus Busan48547 Korea Republic of Department of Materials Science and Engineering Inha University Incheon22212 Korea Republic of Program in Semiconductor Convergence Inha University Incheon22212 Korea Republic of Department of Computer Science and Engineering Vignan's Lara Institute of Technology & Science Andhra Pradesh Guntur India Department of Chemistry Krishna University Andhra Pradesh Machillipatnam521001 India

The exploration of photon upconversion has led to the development of multifunctional lanthanide-based materials, particularly through the mechanism of photon avalanche, marking a transformative advancement in material science. In this study, yttrium vanadate upconversion nanocrystalline phosphors (UCNCPs) activated by Ho3+/Er3+/Tm3+/Yb3+ ions are reported. These UCNCPs demonstrate a remarkable ability in the photon avalanche, offering highly intense and tunable emissions across the visible spectrum at room temperature under low excitation power of 980 nm laser. The average number of photons involved in the UC process at threshold pump power, highlighting the intricate interplay of cross-relaxation and energy transfer loops in avalanche mechanism. Notably, these UCNCPs have shown exceptional temperature sensing capabilities, where non-thermally coupled levels of the Ho3+ and Tm3+ ions provide higher relative sensitivity and accuracy than thermally coupled levels of Er3+ ions. The versatility of these UCNCPs is further established by their application in solid-state lighting, where they can produce vibrant red, green, blue, and warm-white light, and in security, serving as multi-level anti-counterfeiting inks that respond to 980 nm laser illumination. These developments not only pave the way for more energy-efficient lighting solutions but also offer new avenues for enhancing the security of valuable items. The temperature sensing capabilities of these phosphors add another layer of functionality, making them ideal for high-tech applications ranging from medical diagnostics to environmental monitoring. © 2025 Elsevier B.V.

关键词： Phosphors

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