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arXiv 2024年

作者： Mihm, Tina N. Trerayapiwat, Kasidet Jing Li, Xinxin Ma, Xuedan Sharifzadeh, Sahar Department of Electrical and Computer Engineering Boston University MA02215 United States Department of Chemistry Boston University MA02215 United States Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States Consortium for Advanced Science and Engineering University of Chicago ChicagoIL60637 United States Materials Science and NanoEngineering Rice University HoustonTX77251 United States Northwestern Argonne Institute of Science and Engineering EvanstonIL60208 United States Department of Chemistry Boston University BostonMA02215 United States Materials Science Division Boston University BostonMA02215 United States Department of Physics Boston University BostonMA02215 United States

Semiconducting single-walled carbon nanotubes (SWCNT) containing covalent defects are a promising class of optoelectronic materials, demonstrating single photon emission and long-lived spins. The defect introduces new optical transitions due to both symmetry breaking induced band splitting and introduction of in-gap electronic states. We investigate sulfur-oxide containing compounds as a new class of optically active dopants on (6,5) SWCNT. The SWCNT is exposed to sodium dithionite with the resulting compound displaying a red-shifted and bright photoluminescence peak that is characteristic of these covalent defects. Density functional theory calculations are then performed on the adsorbed compounds that may arise (S, SO, SO2 and SO3). These calculations indicate that the two smallest molecules strongly bind to the SWCNT with binding energies of ∼ 1.5−1.8 eV and 0.56 eV for S and SO, respectively. Moreover, these adsorbates introduce in-gap electronic states into the bandstructure of the tube consistent with the measured red-shift of (0.1 − 0.3) eV. Our study suggests that sulfur-based compounds are promising new dopants for (6,5) SWCNT with tunable electronic properties. © 2024, CC BY.

关键词： Sulfur dioxide

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Spectral evidence for local-moment ferromagnetism in the van der Waals metals Fe3GaTe2 and Fe3GeTe2

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Physical Review B 2024年第10期109卷 104410-104410页

作者： Han Wu Chaowei Hu Yaofeng Xie Bo Gyu Jang Jianwei Huang Yucheng Guo Shan Wu Cheng Hu Ziqin Yue Yue Shi Rourav Basak Zheng Ren T. Yilmaz Elio Vescovo Chris Jozwiak Aaron Bostwick Eli Rotenberg Alexei Fedorov Jonathan D. Denlinger Christoph Klewe Padraic Shafer Donghui Lu Makoto Hashimoto Junichiro Kono Alex Frano Robert J. Birgeneau Xiaodong Xu Jian-Xin Zhu Pengcheng Dai Jiun-Haw Chu Ming Yi Department of Physics and Astronomy and Rice Center for Quantum Materials Rice University Houston Texas 77005 USA Department of Physics University of Washington Seattle Washington 98195 USA Department of Materials Science and Engineering University of Washington Seattle Washington 98195 USA Theoretical Division and Center for Integrated Nanotechnologies Los Alamos National Laboratory Los Alamos New Mexico USA Department of Advanced Materials Engineering for Information and Electronics Kyung Hee University Yongin 17104 Republic of Korea Department of Physics University of California at Berkeley Berkeley California 94720 USA Advanced Light Source Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Physics University of California San Diego La Jolla California 92093USA National Synchrotron Light Source II Brookhaven National Lab Upton New York 11973 USA Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo Park California 94025 USA Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Department of Material Science and NanoEngineering Rice University Houston Texas 77005 USA Materials Sciences Division Lawrence Berkeley National Laboratory Berkeley California 94720 USA Department of Materials Science and Engineering University of California Berkeley CaliforniaUSA

Magnetism in two-dimensional (2D) materials has attracted considerable attention recently for both fundamental understanding of magnetism and its tunability towards device applications. The isostructural Fe3GeTe2 and Fe3GaTe2 are two members of the Fe-based van der Waals (vdW) ferromagnet family, but exhibit very different Curie temperatures (TC) of 210 and 360 K, respectively. Here, by using angle-resolved photoemission spectroscopy and density functional theory, we systematically compare the electronic structures of the two compounds. Qualitative similarities in the Fermi surface can be found between the two compounds, with expanded hole pockets in Fe3GaTe2 suggesting additional hole carriers compared to Fe3GeTe2. Interestingly, we observe almost no band shift in Fe3GaTe2 across its TC of 360 K, compared to a small shift in Fe3GeTe2 across its TC of 210 K. The weak temperature-dependent evolution strongly deviates from the expectations of an itinerant Stoner mechanism. Our results suggest that itinerant electrons have minimal contributions to the enhancement of TC in Fe3GaTe2 compared to Fe3GeTe2, and that the nature of ferromagnetism in these Fe-based vdW ferromagnets must be understood with considerations of the electron correlations.

关键词： Magnetism Van der Waals systems Angle-resolved photoemission spectroscopy

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engineering dimensionality of collective dipole-dipole interactions using a nanophotonic environment

Engineering dimensionality of collective dipole-dipole inter...

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Conference on Lasers and Electro-Optics (CLEO)

作者： Ashwin K. Boddeti Yi Wang Xitlali Juarez Alexandra Boltasseva Hadiseh Alaeian Teri W. Odom Zubin Jacob Elmore Family School of Electrical and Computer Engineering and Birck Nanotechnology Center Purdue University West Lafayette Indiana USA Graduate Program in Applied Physics Northwestern University Evanston IL USA Department of Materials Science and Engineering Northwestern University Evanston Illinois USA Department of Chemistry and Department of Materials Science and Engineering Northwestern University Evanston Illinois USA

We experimentally demonstrate reduced dimensionality in a interacting ensemble of emitters. The well-known stretched exponential decay dynamics, I(t)/I 0 = exp(−γ D t)exp(−αt β ) with β = 0.5 in 3D geometries, is... 详细信息

ISBN: (纸本)9781957171258

关键词： Energy transfer Fluorescence Molecules Spontaneous emission Titanium dioxide

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Optical Patterning of Two-Dimensional materials

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Research 2020年第1期2020卷 1064-1078页

作者： Pavana Siddhartha Kollipara Jingang Li Yuebing Zheng Walker Department of Mechanical Engineering The University of Texas at AustinAustinTX 78712USA Materials Science&Engineering Program and Texas Materials Institute The University of Texas at AustinAustinTX 78712USA

Recent advances in the field of two-dimensional(2D)materials have led to new electronic and photonic devices enabled by their unique properties at atomic *** 2D materials into desired patterns on substrates is often an essential and foremost step for the optimum performance of the functional *** this regard,optical patterning of 2D materials has received enormous interest due to its advantages of high-throughput,site-specific,and on-demand *** years have witnessed scientific reports of a variety of optical techniques applicable to patterning 2D *** this minireview,we present the state-of-the-art optical patterning of 2D materials,including laser thinning,doping,phase transition,oxidation,and *** applications based on optically patterned 2D materials will be discussed as *** further developments,optical patterning is expected to hold the key in pushing the frontiers of manufacturing and applications of 2D materials.

关键词： frontier doping optimum

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Continuous Collapse of the Spin Cycloid in BiFeO3 Thin Films under an Applied Magnetic Field probed by Neutron Scattering

arXiv

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arXiv 2024年

作者： Pervez, Md Firoz Zhang, Hongrui Huang, Yen-Lin Caretta, Lucas Ramesh, Ramamoorthy Ulrich, Clemens School of Physics The University of New South Wales NSW2052 Australia Materials Science Division Lawrence Berkeley National Laboratory BerkeleyCA94720 United States Ningbo Institute of Materials Technology & Engineering Chinese Academy of Sciences Ningbo315201 China Department of Materials Science and Engineering University of California BerkeleyCA94720 United States School of Engineering Brown University ProvidenceRI02912 United States Department of Physics University of California BerkeleyCA94720 United States Materials Science and NanoEngineering Rice University HoustonTX77005 United States Departments of Chemistry and Physics and Astronomy Rice University HoustonTX77005 United States Rice Advanced Materials Institute Rice University HoustonTX77005 United States

Bismuth ferrite (BiFeO3) is one of the rare materials that exhibits multiferroic properties already at room-temperature. Therefore, it offers tremendous potential for future technological applications, such as memory and logic. However, a weak magnetoelectric coupling together with the presence of a noncollinear cycloidal spin order restricts various practical applications of BiFeO3. Therefore, there is a large interest in the search for suitable methods for the modulation of the spin cycloid in BiFeO3. By performing neutron diffraction experiments using a triple-axis instrument we have determined that the spin cycloid can be systematically suppressed by applying a high magnetic field of 10 T in a BiFeO3 thin film of about 100 nm grown on a (110)-oriented SrTiO3 substrate. As predicted by previous theoretical calculations, we observed that the required critical magnetic field to suppress the spin cycloid in a BiFeO3 thin film was lower as compared to the previously reported critical magnetic field for bulk BiFeO3 single crystals. Our experiment reveals that the spin cycloid continuously expands with increasing magnetic field before the complete transformation into a G-type antiferromagnetic spin order. Such tuning of the length of the spin cycloid up to a complete suppression offers new functionalities for future technological applications as in spintronics or magnonics. Copyright © 2024, The Authors. All rights reserved.

关键词： Magnetic fields

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Stretchable Textile Bands for Ambulatory Electrocardiogram and Oximetry

IEEE Journal on Flexible Electronics

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IEEE Journal on Flexible Electronics 2022年第4期1卷 214-222页

作者： Liu, Jiaxi Le, Thy Sadatian, Ellie Yao, Lulu Garudadri, Harinath Dunphy, Stephen A. McClung, Christian Ng, Tse Nga University of California at San Diego Department of Electrical and Computer Engineering La Jolla CA92093 United States University of California at San Diego Materials Science and Engineering Program La Jolla CA92093 United States Qualcomm Institute University of California at San Diego La Jolla CA92093 United States Cb Innovations Llc Rancho Santa FeCA92067 United States

This work presents a vital sign monitoring interface combining electrocardiogram (ECG) and reflective photoplethysmography (PPG) acquisition on stretchable kinesiology tapes (KTs). The integrated textile bands are less prone to electrode misplacement and deliver high-quality diagnostic ECG signals with dry electrodes. The reflective PPG measured over the subclavian artery is used to track blood oxygen saturation, and in combination with ECG, enables the determination of pulse transit time and inference of blood pressure. This multimodal interface improves clinical workflows because it is easy to don, reduces motion artifacts, and facilitates more efficient and accurate diagnosis in emergency settings. © 2022 IEEE.

关键词： Electrocardiograms

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Giant Deep-Ultraviolet Circular Dichroism in Synthetic Architectures of Ordered Carbon Nanotubes

Giant Deep-Ultraviolet Circular Dichroism in Synthetic Archi...

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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Doumani, Jacques Lou, Minhan Dewey, Oliver Hong, Nina Fan, Jichao Baydin, Andrey Pasquali, Matteo Yomogida, Yohei Yanagi, Kazuhiro Saito, Riichiro Kono, Junichiro Gao, Weilu Department of Electrical and Computer Engineering Rice University HoustonTX United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX United States Department of Electrical and Computer Engineering The University of Utah Salt Lake CityUT United States Carbon Hub Rice University HoustonTX United States Department of Chemical and Biomolecular Engineering Rice University HoustonTX United States J.A. Woollam Co. LincolnNE United States The Smalley-Curl Institute Rice University HoustonTX United States Department of Chemistry Rice University HoustonTX United States Department of Materials Science and NanoEngineering Rice University HoustonTX United States Department of Physics and Astronomy Tokyo Metropolitan University Tokyo Japan Department Physics Tohoku University Sendai Japan Department Physics and Astronomy Rice University HoustonTX United States

We demonstrate tunable, giant, and structure-induced deep-ultraviolet circular dichroism in macroscopically chiral assemblies of racemic carbon nanotubes prepared using two approaches: mechanical-rotation-assisted vac... 详细信息

ISBN: (纸本)9781957171258

关键词： Dichroism

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Optical Imaging of Flavor Order in Flat Band Graphene

arXiv

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arXiv 2024年

作者： Xie, Tian Wolf, Tobias M. Xu, Siyuan Cui, Zhiyuan Xiong, Richen Ou, Yunbo Hays, Patrick Holleis, Ludwig F. Guo, Yi Sheekey, Owen I. Patterson, Caitlin Arp, Trevor Watanabe, Kenji Taniguchi, Takashi Tongay, Seth Ariel Young, Andrea F. MacDonald, Allan H. Jin, Chenhao Department of Physics University of California at Santa Barbara Santa BarbaraCA93116 United States Department of Physics University of Texas at Austin AustinTX78712 United States Materials Science and Engineering Program School of Engineering for Matter Transport and Energy Arizona State University TempeAZ85287 United States Research Center for Electronic and Optical Materials National Institute for Materials Science 1-1 Namiki Tsukuba305-0044 Japan Research Center for Materials Nanoarchitectonics National Institute for Materials Science 1-1 Namiki Tsukuba305-0044 Japan

Spin- and valley flavor polarization plays a central role in the many-body physics of flat band graphene1–21, with fermi surface reconstructions—often accompanied by quantized anomalous Hall1–8 and superconducting state9–14—observed in a variety of experimental systems. Here we describe an optical technique that sensitively and selectively detects flavor textures via the exciton response of a proximal transition metal dichalcogenide layer. Through a systematic study of rhombohedral and rotationally faulted graphene bilayers and trilayers, we show that when the semiconducting dichalcogenide is in direct contact with the graphene, the exciton response is most sensitive to the large momentum rearrangement of the Fermi surface, providing information that is distinct from and complementary to electrical compressibility measurements. The wide-field imaging capability of optical probes allows us to obtain spatial maps of flavor orders with high throughput, and with broad temperature and device compatibility. Our work paves the way for optical probing and imaging of flavor orders in flat band graphene systems. Copyright © 2024, The Authors. All rights reserved.

关键词： Graphene

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Recent Advancements in Nanophotonics for Optofluidics

arXiv

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arXiv 2024年

作者： Yang, Sen Hong, Chuchuan Zhu, Guodong Anyika, Theodore Hong, Ikjun Ndukaife, Justus C. Institute of Physics Chinese Academy of Sciences Beijing National Laboratory for Condensed Matter Physics Beijing100190 China Department of Chemistry Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Department of Electrical and Computer Engineering Vanderbilt University NashvilleTN37235 United States Department of Mechanical Engineering Vanderbilt University NashvilleTN37235 United States Interdisciplinary Materials Science Program Vanderbilt University NashvilleTN37240 United States

Optofluidics is dedicated to achieving integrated control of particle and fluid motion, particularly on the micrometer scale, by utilizing light to direct fluid flow and particle motion. The field has seen significant growth recently, driven by the concerted efforts of researchers across various scientific disciplines, notably for its successful applications in biomedical science. In this review, we explore a range of optofluidic architectures developed over the past decade, with a primary focus on mechanisms for precise control of micro and nanoscale biological objects and their applications in sensing. Regarding nanoparticle manipulation, we delve into mechanisms based on optical nanotweezers using nanolocalized light fields and light-based hybrid effects with dramatically improved performance and capabilities. In the context of sensing, we emphasize those works that used optofluidics to aggregate molecules or particles to promote sensing and detection. Additionally, we highlight emerging research directions, encompassing both fundamental principles and practical applications in the field. Copyright © 2024, The Authors. All rights reserved.

关键词： Flow of fluids

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Ultrastrong Spin-Photon Coupling in Gadolinium Gallium Garnet

Ultrastrong Spin-Photon Coupling in Gadolinium Gallium Garne...

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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Kritzell, T. Elijah Bao, Junzhe Doumani, Jacques Lee, Jae Joon Xu, Hongjing Tay, Fuyang Nojiri, Hiroyuki Bamba, Motoaki Baydin, Andrey Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Institute for Materials Research Tohoku University Sendai980-8577 Japan The Hakubi Center for Advanced Research Kyoto University Kyoto606-8502 Japan Department of Physics I Kyoto University Kyoto606-8502 Japan Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

We examine ultrastrong coupling of an ensemble of paramagnetic spins in Gd3Ga5O12 with terahertz photons in the presence of a high external magnetic field both in the bulk and thin-film limits. © 2023 The Author(s)

ISBN: (纸本)9781957171258

关键词： Photons

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