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Mn single-atoms decorated CNT electrodes for high-performance supercapacitors

Nano Research 2024年第5期17卷 4039-4046页

作者： Qian Rong Chao Yuwen Yingkai Liu Yuanrong Liu Chunyang Wang Yang Wang Ding Zhang Zhen Wen Yunnan Key Laboratory of Opto-Electronic Information Technology Institute of Physics and Electronic InformationYunnan Normal UniversityKunming 650500China Faculty of Metallurgical and Energy Engineering Kunming University of Science and TechnologyKunming 650093China Department of Physics and Astronomy University of CaliforniaIrvineCA 92697USA School of Materials Science and Engineering National Institute for Advanced MaterialsSmart Sensing Interdisciplinary Science CenterNankai UniversityTianjin 300350China Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices Institute of Functional Nano and Soft Materials(FUNSOM)Soochow UniversitySuzhou 215123China

Developing highly robust and efficient electrode materials is of critical importance to promoting the energy density of current supercapacitors for ***,we report an efficient catalyst with monodispersed Mn single-atoms embedded in carbon nanotubes(Mn-CNTs)for enhancing the electrode performance of supercapacitors.A high specific capacitance(1523.6 F·g^(-1) at 1.0 A·g^(-1))can be achieved,which is about twice as high as the specific capacitance of the electrode material without the introduction of Mn ***,the asymmetric electrochemical capacitor created with Mn-CNT and activated carbon exhibits a high energy density of 180.8 Wh·kg^(-1) at a power density of 1.4 kW·kg^(-1),much higher than most reported *** study shows that the integration of Mn atoms into the CNT can enhance the charge transport capacity and the number of polar active sites of Mn-CNT and then facilitate chemical interactions between Mn-CNT and OH-.This work provides a novel strategy to enable high-energy storage in supercapacitors by introducing single-atoms into carbon nanotubes to improve electrodes’energy density and cycle life.

关键词： carbon nanotube(CNT) supercapacitor single-atoms power density energy density

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High-excited-state splitting and multimode vibrational coupling in Mn^(4+)-activated fluoride phosphor

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Science China(physics,Mechanics & Astronomy) 2024年第3期67卷 95-101页

作者： Debao Zhang Wanggui Ye Xuguang Cao Ji Zhou Fei Tang Changcheng Zheng Jiqiang Ning Shijie Xu Department of Optical Science and Engineering School of Information Science and TechnologyFudan University Shanghai 200438China Jiangsu Key Laboratory of Advanced Laser Materials and Devices Schoolof Physics and Electronic Engineering Jiangsu Normal UniversityXuzhou 221116China Division of Natural and Applied Sciences Duke Kunshan UniversityKunshan 215316China

Excited-states play a crucial role in the optical absorption and luminescence of solids and hence their accurate information is highly desired. Herein, we attempt to seize the excited-states information of Mn^(4+)ions in K_(2)SiF_(6) microcrystals via measuring and calculating their variable-temperature photoluminescence excitation(PLE) spectra. At cryogenic temperatures, an unpredicted splitting of the high-excited-state is observed. Moreover, the two-split high-excited-state levels are further revealed to primarily couple with the two hyperfine split modes of quasi-localized ν2 vibration in the distorted Mn-F_(6) octahedral configuration,whereas the coupling strengths are found to be substantially different from each other. The slightly split vibrational mode is firmly supported by the low-temperature Raman spectra. Jahn-Teller lattice distortion is believed to be responsible for the observed splitting of the electronic high-excited-state and the quasi-localized vibrational mode.

关键词： splitting of excited-state photoluminescence excitation spectrum electron-phonon coupling Jahn-Teller effect

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Anisotropic phonon dynamics in Dirac semimetal PtTe2 thin films enabled by helicity-dependent ultrafast light excitation

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Light(Science & Applications) 2024年第9期13卷 1888-1897页

作者： Ziyang Li Yequan Chen Anke Song Jinzhong Zhang Rong Zhang Zongzhi Zhang Xuefeng Wang Key Laboratory of Micro and Nano Photonic Structures(MOE) School of Information Science and TechnologyFudan UniversityShanghaiChina Jiangsu Provincial Key Laboratory of Advanced Photonic and Electronic Materials State Key Laboratory of Spintronics Devices and TechnologiesSchool of Electronic Science and EngineeringCollaborative Innovation Center of Advanced MicrostructuresNanjing UniversityNanjingChina Department of Physics School of Physics and Electronic ScienceEast China Normal UniversityShanghaiChina Department of Physics Xiamen UniversityXiamenChina

Coherent phonons have aroused considerable attention in condensed matter physics owing to their extraordinary capacity of reflecting and controlling the physical properties of ***,the investigation on the interaction between coherent phonons and other microscopic particles on the ultrafast timescale within topological systems continues to be an active and unresolved ***,we show the energy transfer of coherent optical phonons(COP)in Dirac semimetal PtTe2 thin films using ultrafast optical pump-probe ***,the helicitydependent light-driven anisotropic COP signals disclose their direct connection with the light-excited anisotropic spinpolarized electrons via an angular momentum ***,we observe the notable decreases in the COP oscillation frequency and the decay rate with increasing temperatures due to the anharmonic phonon-phonon scattering and electron-phonon scattering in the COP dissipation process,*** work paves the way for uncovering the coherent phonons in Dirac semimetals for the potential applications in optoelectronics and optospintronics.

关键词： spectroscopy phonon Dirac

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Rotational magnetoelectric switching in orthorhombic multiferroics

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npj Computational materials 2024年第1期10卷 2505-2511页

作者： Xu Li Hao Tian Lan Chen Hongjun Xiang Jun-Ming Liu L.Bellaiche Di Wu Yurong Yang National Laboratory of Solid State Microstructures and Collaborative Innovation Center of Advanced Microstructures Nanjing UniversityNanjing 210093China Jiangsu Key Laboratory of Artificial Functional Materials Department of Materials Science and EngineeringNanjing UniversityNanjing 210093China School of Physics and Electronic Engineering Zhengzhou Normal UniversityZhengzhou 450044China School of Science Nanjing University of Posts and TelecommunicationsNanjing 210023China Key Laboratory of Computational Physical Sciences(Ministry of Education) State Key Laboratory of Surface Physicsand Department of PhysicsFudan UniversityShanghai 200433China Physics Department and Institute for Nanoscience and Engineering University of ArkansasFayettevilleAR 72701USA

Controlling the direction of ferromagnetism and antiferromagnetism by an electric field in single-phase multiferroics will open the door to the next generation of devices for spintronics and *** typical magnetoelectric coupling such as the linear magnetoelectric effect is very weak in type-I multiferroics and therefore the magnetoelectric switching is rarely ***,using firstprinciples simulations,we propose a magnetoelectric switching mechanism to achieve such highly desired control in orthorhombic multiferroics.

关键词： orthorhombic magneto desired

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Highly active cobalt-doped nickel sulfide porous nanocones for high-performance quasi-solid-state zinc-ion batteries

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Journal of Energy Chemistry 2022年第3期31卷 237-249,I0008页

作者： Xin Tong Yun Li Ning Pang Yang Zhou Dajun Wu Dayuan Xiong Shaohui Xu Lianwei Wang Paul K.Chu Key Laboratory of Polar Materials and Devices(MOE) Department of ElectronicsEast China Normal UniversityShanghai 200241China Jiangsu Laboratory of Advanced Functional Materials School of Electronic and Information EngineeringChangshu Institute of TechnologyChangshu 215500JiangsuChina School of Physics and Electronic Engineering Hanshan Normal UniversityChaozhou 521041GuangdongChina Department of Physics Department of Materials Science and Engineeringand Department of Biomedical EngineeringCity University of Hong KongKowloon 999077Hong KongChina

Flexible quasi-solid zinc-ion batteries(ZIBs)have large potential in power applications due to the low price,wearable nature,safety,and high ***,the use of transition metal sulfide cathodes in ZIBs has not been studied extensively and the underlying mechanism and theoretical basis of this type of batteries are not well ***,a highly active cobalt-doped Ni_(3)S_(2) porous nanocone framework(C12NS)is designed and demonstrated as a zinc-ion battery ***-principles calculation and experiments reveal that the cobalt dopant improves the battery properties *** assembled flexible zinc-ion battery exhibits a high specific capacity of 453.3 mAh g^(−1)at a current density of 0.4 A g^(−1)in as well as excellent cycling stability as manifested by a capacity retention ratio of 89.5%at a current density of 4 A g^(−1)after 5000 *** peak energy density of 553.9 Wh kg^(−1)is also superior to those of most recently reported NiCo-based zinc-ion *** importantly,the flexible battery can be operated under severe mechanical bending and even continues to work after physical puncturing without showing *** exciting results not only reveal a novel design of cathode materials for zinc-based batteries,but also suggest their immense commercial potential in portable and wearable electronics.

关键词： Zn-ion battery Quasi-solid electrolyte Nanocone Doping Wearable electronic

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Self-Assembled Porous-Reinforcement Microstructure-Based Flexible Triboelectric Patch for Remote Healthcare

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Nano-Micro Letters 2023年第7期15卷 324-336页

作者： Hao Lei Haifeng Ji Xiaohan Liu Bohan Lu Linjie Xie Eng Gee Lim Xin Tu Yina Liu Peixuan Zhang Chun Zhao Xuhui Sun Zhen Wen Institute of Functional Nano and Soft Materials(FUNSOM) Joint International Research Laboratory of Carbon-Based Functional Materials and DevicesSoochow UniversitySuzhou 215123People’s Republic of China Department of Electrical and Electronic Engineering School of Advanced TechnologyXi’an Jiaotong-Liverpool UniversitySuzhou 215123People’s Republic of China Department of Applied Mathematics School of Mathematics and PhysicsXi’an Jiaotong-Liverpool UniversitySuzhou 215123People’s Republic of China Department of Electrical and Electronic Engineering University of LiverpoolLiverpool L693GJUK Jiangsu Key Laboratory for Carbon-Based Functional Materials and Devices Soochow UniversitySuzhou 215123JiangsuPeople’s Republic of China

Realizing real-time monitoring of physiological signals is vital for preventing and treating chronic diseases in elderly individuals. However,wearable sensors with low power consumption and high sensitivity to both weak physiological signals and large mechanical stimuli remain ***, a flexible triboelectric patch(FTEP) based on porous-reinforcement microstructures for remote health monitoring has been reported. The porousreinforcement microstructure is constructed by the self-assembly of silicone rubber adhering to the porous framework of the PU sponge. The mechanical properties of the FTEP can be regulated by the concentrations of silicone rubber dilution. For pressure sensing, its sensitivity can be effectively improved fivefold compared to the device with a solid dielectric layer, reaching 5.93 kPa^(-1) under a pressure range of 0–5 kPa. In addition, the FTEP has a wide detection range up to 50 kPa with a sensitivity of 0.21 kPa^(-1). The porous microstructure makes the FTEP ultra-sensitive to external pressure, and the reinforcements endow the device with a greater deformation limit in a wide detection range. Finally, a novel concept of the wearable Internet of Healthcare(Io H) system for real-time physiological signal monitoring has been proposed, which could provide real-time physiological information for ambulatory personalized healthcare monitoring.

关键词： Pressure sensor Triboelectric nanogenerator Porous dielectric layer Physiological signals Internet of Healthcare

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Insights into photocatalytic mechanism over a novel Cu_(2)WS_(4)/MoS_(2) S-scheme heterojunction

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Rare Metals 2024年第7期43卷 3118-3133页

作者： Wei Zhao Ji-Hui Cao Jun-Jie Liao Yun Liu Xiao-Jun Zeng Jun-Yu Shen Xue-Kun Hong Yang Guo He-Hua Zeng Ya-Zi Liu School of Materials Engineering Jiangsu Key Laboratory of Advanced Functional MaterialsSchool of Electronic and Information EngineeringChangshu Institute of TechnologyChangshu215500China School of Chemistry and Chemical Engineering Changji UniversityChangji 831100China State Environmental Protection Key Laboratory of Soil Environmental Management and Pollution Control Ministry of Ecology and EnvironmentNanjing Institute of Environmental SciencesNanjing 210023China School of Environment Jiangsu Engineering Lab of Water and Soil Eco-RemediationNanjing Normal UniversityNanjing 210023China Department of Chemical Engineering Curtin UniversityPerthWA6845Australia

A novel efficient Cu_(2)WS_(4)/MoS_(2) step-scheme(S-scheme)heterojunction photocatalyst was constructed for the first time and applied in the removal of environmental *** the as-prepared photocatalysts,the Cu_(2)WS_(4)/MoS_(2)-8%heterojunc tion photoc atalyst demonstrates the optimal photocatalytic performance,with the catalytic oxidation efficiency of tetracycline(TC)and the catalytic reduction efficiency of Cr^(6+)reaching 93.3%and 82.1%,*** excellent catalytic properties of Cu_(2)WS_(4)/MoS_(2) heterojunction photocatalysts are attributed to the effective separation pathways of charges and the presence of S-scheme heterojunctions,together with stronger redox *** is speculated that the photogenerated carrier migration path of the Cu_(2)WS_(4)/MoS_(2) catalyst follows the typical S-scheme photocatalytic mechanism,which is verified by the in-depth experimental study and simulated calculations including the electron paramagnetic resonance(EPR)analysis,free radical quenching experiments,charge density distribution,and simulated built-in electric field formation at the interface,which acts as driving force to promote the separation of photoinduced electrons and ***,the photocatalytic mechanism of S-scheme photogenerated carrier migration for the Cu_(2)WS_(4)/MoS_(2) catalyst is revealed based on the systematic experimental techniques and simulated calculations,accounting for its superior photocatalytic oxidation and reduction *** study provides inspiring implications to develop high-efficient S-scheme photocatalytic systems for versatile applications in solarenergy conversion.

关键词： Cu_(2)WS_(4)/MoS_(2) S-scheme Heterojunction Photocatalysis

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Space-confined vapor deposited molecular ferroelectric film for photovoltaic devices

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Nano Research 2025年第3期18卷 611-618页

作者： Chen Wang Shan Cong Lingbo Xiao Chao-ran Huang Ruonan Wang Ruijie Li Lutao Li Guifu Zou Qiang Zhang College of Mechanical and Electronic Engineering Shandong University of Science and TechnologyQingdao 266590China College of Energy Soochow Institute for Energy and Materials Innovationsand Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu ProvinceSoochow UniversitySuzhou 215000China Department of Applied Physics Zhejiang University of Science and TechnologyHangzhou 310023China School of Advanced Energy Sun Yat-sen UniversityShenzhen 518107China

Molecular ferroelectrics,characterized by outstanding photoelectric and unique ferroelectric properties,invigorate the field of ferroelectric ***,the performance of molecular ferroelectric devices is hindered by fine grains resulting from poor high-temperature *** this work,we successfully achieved micron-grained molecular ferroelectric films by using the space-confined vapor deposited *** optimized film exhibited a significant increase in grain size from the nanometer level(0.08μm)to the micrometer level(~2μm),leading to improved optoelectronic and ***,it optimizes the energy level and enhances the photovoltaic performance of vertical *** on the mechanism shows that high annealing temperature and inhibiting component loss play an important role in obtaining large grain *** work provides new research ideas for improving the quality of molecular ferroelectric films and provides valuable reference for the fabrication of high performance molecular ferroelectric photovoltaic devices.

关键词： molecular ferroelectric large grain space confinement photovoltaic devices

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Gate-tunable Berry curvature in van der Waals itinerant ferromagnetic Cr_(7)Te_(8)

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InfoMat 2024年第3期6卷 108-116页

作者： Kui Meng Zeya Li Zhansheng Gao Xiangyu Bi Peng Chen Feng Qin Caiyu Qiu Lingyun Xu Junwei Huang Jinxiong Wu Feng Luo Hongtao Yuan National Laboratory of Solid State Microstructures Collaborative Innovation Center of Advanced MicrostructuresCollege of Engineering and Applied SciencesJiangsu Key Laboratory of Artificial Functional MaterialsNanjing UniversityNanjingthe People's Republic of China Center for the Physics of Low-Dimensional Materials Henan Joint International Research Laboratory of New Energy Materials and DevicesSchool of Physics and ElectronicsHenan UniversityKaifengthe People's Republic of China Tianjin Key Lab for Rare Earth Materials and Applications Center for Rare Earth and Inorganic Functional MaterialsSmart Sensor Interdisciplinary Science CenterSchool of Materials Science and EngineeringNankai UniversityTianjinthe People's Republic of China

The anomalous Hall effect(AHE)that associated with the Berry curvature of occupied electronic states in momentum-space is one of the intriguing aspects in condensed matter physics,and provides an alternative for potential applications in topological *** experiments reported the tunable Berry curvature and the resulting magnetization switching process in the AHE based on strain engineering or chemical ***,the AHE modulation by these strategies are usually irreversible,making it difficult to realize switchable control of the AHE and the resultant spintronic ***,we demonstrated the switchable control of the Berry-curvature-related AHE by electrical gating in itinerant ferromagnetic Cr_(7)Te_(8)with excellent ambient *** gate-tunable sign reversal of the AHE can be attributed to the redistribution of the Berry curvature in the band structure of Cr_(7)Te_(8)due to the intercalation-induced change in the Fermi *** work facilitates the applications of magnetic switchable devices based on gate-tunable Berry curvature.

关键词： anomalous Hall effect Berry curvature van der Waals itinerant ferromagnetism

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Colossal magnetoresistance and Fermi surface topology in the layered Zintl-phase compound YbAl2Si2

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Physical Review B 2024年第17期110卷 174408页

作者： Fang Tang Yang Chen Xunqing Yin Weiyao Zhao Lei Zhang Zhida Han Renkui Zheng Xiaoming Zhang Yong Fang Jiangsu Laboratory of Advanced Functional Materials School of Electronic and information Engineering Jiangsu Key Laboratory of Thin Films School of Physical Science and Technology School of Physics and Astronomy and Tsung-Dao Lee Institute Department of Materials Science and Engineering School of Materials Science and Engineering School of Physics and Materials Science

Considerable attention has been devoted to CaAl2Si2-type Zintl-phase compounds for their intriguing physical properties, particularly the complex interplay between band structures and magnetism. Herein we grow high-quality single crystals of nonmagnetic YbAl2Si2 and examine the physical properties, including resistivity, magnetoresistance, angular magnetoresistance, Hall resistivity, and band structures. This compound shows metallic properties and Fermi-liquid behaviors. Its resistivity under magnetic fields increases as per Kohler rule, with normalized magnetoresistance curves merging into one, ruling out potential metal-insulator-like transitions. Colossal magnetoresistance is observed at low temperatures. Hall resistivity analysis categorizes this compound as an uncompensated semimetal. Its angle dependence of the magnetoresistance and quantum oscillation frequencies demonstrate an anisotropy ratio of ∼1.26 for the Fermi surface. Theoretical calculations corroborate these findings, mapping Fermi surfaces with three hole pockets and an electron pocket. Considering both the experimental and theoretical results, the colossal and angle-dependent magnetoresistance may be ascribed to unequal carrier densities coupled with large differences in carrier mobilities and Fermi-surface anisotropy, respectively. These results imply YbAl2Si2 is a promising candidate to study the crucial effect of electronic properties on its charge transport.

关键词： Colossal magnetoresistance Fermi surface Magnetotransport Semimetals Single crystal materials Topological materials Density functional calculations Fermi liquid theory Resistivity measurements

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