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Temperature-dependent synergistic evolution mechanism of rhenium and irradiation defects in tungsten-rhenium alloys

Journal of materials science & Technology 2023年第14期145卷 221-234页

作者： Yu-Hao Li Fang-Ya Yue Zhong-Zhu Li Peng-Wei Hou Yu-Ze Niu Hui-Zhi Ma Ying Zhang Xun-Xiang Hu Hui-Qiu Deng Hong-Bo Zhou Fei Gao Guang-Hong Lu Department of Physics Beihang UniversityBeijing 100191China Beijing Key Laboratory of Advanced Nuclear Materials and Physics Beihang UniversityBeijing 100191China College of Physics Sichuan UniversityChengdu 610065China School of Physics and Electronics Hunan UniversityChangsha 410082China Department of Nuclear Engineering and Radiological Science University of MichiganAnn ArborMI 48109USA

We have systemically investigated the synergistic evolution of rhenium(Re)and irradiation defects in tungsten(W)-Re alloys under different temperatures and irradiation doses using object Kinetic Monte Carlo *** results revealed the underlying mechanism for the transition of Re effect on W from beneficial to harmful during the Re-defects evolution with the increase of irradiation dose,in which tem-perature always plays a critical *** the one hand,Re will significantly promote the defect annihila-tion at low irradiation doses and high temperatures,thereby effectively reducing their sizes and number *** is due to the formation of stable Re-SIAs complexes that can be eliminated by the mobile vacancy-type defects,whereas the transition of the migration pattern of SIAs only plays a weak role in the defect recombination in W-Re *** the other hand,with the increase of irradiation dose,Re will aggregate to form Re-rich clusters or even ***,the formation mechanism of Re-rich clusters is also dependent on *** low temperatures,the interstitial-mediated mech-anism plays a crucial role in the Re-rich cluster formation,while at high temperatures,both SIA-type and vacancy-type defects will act as the transport carriers of Re to promote their ***,the critical conditions for the transition of Re from beneficial to harmful and the formation of Re-rich clusters at different tem peratures and irradiation doses are given with the help of the phase *** work presents the temperature dependence of the synergy of Re and irradiation defects in W-Re in fusion-relevant environment,which provides a good reference for the development of radiation-resistant materials and the prediction of W performance in fusion reactors.

关键词： Synergistic evolution Irradiation defects Defects recombination Rhenium-rich clusters Tungsten-rhenium alloys

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Tilted Perpendicular Anisotropy-Induced Spin-Orbit Ratchet Effects

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Chinese physics Letters 2024年第7期41卷 181-186,I0001,I0002,I0003页

作者：陈彬龙垣图聂宇林凌姿瑀马天平张瑞轩吴义政骆泳铭王宁宁 School of Electronics and Information Engineering Hangzhou Dianzi UniversityHangzhou 310018China State Key Laboratory of Surface Physics and Department of Physics Fudan UniversityShanghai 200433China Research Center for Intelligent Computing Platforms Zhejiang LaboratoryHangzhou 311121China Wenzhou Institute of Hangzhou Dianzi University Wenzhou 325038China Anhui Key Laboratory of Magnetic Functional Materials and Devices School of Materials Science and EngineeringAnhui UniversityHefei 230601China

Using micromagnetic simulations, we demonstrate the tilted perpendicular anisotropy-induced spin-orbit ratchet effect. In spin-orbit torque(SOT)-induced magnetization switching, the critical currents required to switch between the two magnetization states(upward and downward magnetization) are asymmetric. In addition, in the nanowire structure, tilted anisotropy induces formation of tilted domain walls(DWs). The tilted DWs exhibit a ratchet behavior during motion. The ratchet effect during switching and DW motions can be tuned by changing the current direction with respect to the tilting direction of anisotropy. The ratchet motion of the DWs can be used to mimic the leaky-integrate-fire function of a biological neuron, especially the asymmetric property of the “potential” and “reset” processes. Our results provide a full understanding of the influence of tilted perpendicular anisotropy on SOT-induced magnetization switching and DW motion, and are beneficial for designs of further SOT-based devices.

关键词： motion effect magnetization

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Chiral Pair Density Waves with Residual Fermi Arcs in RbV_(3)Sb_(5)

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Chinese physics Letters 2024年第9期41卷 88-92页

作者： Xiao-Yu Yan Hanbin Deng Tianyu Yang Guowei Liu Wei Song Hu Miao Zhijun Tu Hechang Lei Shuo Wang Ben-Chuan Lin Hailang Qin Jia-Xin Yin Department of Physics Southern University of Science and TechnologyShenzhen 518055China Materials Science and Technology Division Oak Ridge National LaboratoryOak RidgeTennessee 37831USA Beijing Key Laboratory of Optoelectronic Functional Materials MicroNano Devices Department of PhysicsRenmin University of ChinaBeijing 100872China Key Laboratory of Quantum State Construction and Manipulation(Ministry of Education) Renmin University of ChinaBeijing 100872China Shenzhen Institute for Quantum Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Guangdong Provincial Key Laboratory of Quantum Science and Engineering Southern University of Science and TechnologyShenzhen 518055China Quantum Science Center of Guangdong-Hong Kong-Macao Greater Bay Area Shenzhen 518055China

The chiral 2×2 charge order has been reported and confirmed in the kagome superconductor RbV_(3)Sb_(5),while its interplay with superconductivity remains elusive owing to its lowest superconducting transition temperature Tc of about 0.85K in the AV_(3)Sb_(5) family(A=K,Rb,Cs)that severely challenges electronic spectroscopic ***,utilizing dilution-refrigerator-based scanning tunneling microscopy down to 30 mK,we observe chiral 2×2 pair density waves with residual Fermi arcs in RbV_(3)Sb_(5).We find a superconducting gap of 150 μeV with substantial residual in-gap *** spatial distribution of this gap exhibits chiral 2×2 modulations,signaling a chiral pair density wave(PDW).Our quasi-particle interference imaging of the zero-energy residual states further reveals arc-like *** discuss the relation of the gap modulations with the residual Fermi arcs under the space-momentum correspondence between PDW and Bogoliubov Fermi states.

关键词： Fermi chiral utilizing

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Magnetic properties and microstructures of multi-component Sm-Co-based films prepared by high-throughput experiments

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稀有金属（英文版） 2025年第2期44卷 1284-1293页

作者： Xin-Rui Zheng Si-Zhe Liang Zhao-Guo Qiu Yan-Song Gong Hong-Xia Meng Gang Wang Zhi-Gang Zheng Wei-Xing Xia De-Chang Zeng Ping Liu School of Materials Science and Engineering South China University of TechnologyGuangzhou 510640China Zhongshan R&D Center for Materials Surface and Thin Films Technology of the South China University of Technology Gent Materials Surface Technology(Guangdong)Co.Ltd.Zhongshan 528437China Laboratory of Rare-Earth Magnetic Functional Materials Ningbo Institute of Material Technology and EngineeringChinese Academy of SciencesNingbo 315201China Department of Physics University of Texas at ArlingtonArlington TX76019USA

Sm-Co-based films play an irreplaceable role in special applications due to their high curie temperature and magnetocrystalline anisotropic energy,especially in heat-assisted magnetic recording(HAMR),but the complex composition of Sm-Co phase and unclear synergistic coupling mechanisms of multi-elemental doping become the challenges to enhance the *** this work,a novel strategy combining magnetron sputtering and a high-throughput experiment method is applied to solve the above-mentioned ***/Cu co-doping highly increases the remanence while maintaining a coercivity larger than 26 kOe,leading to an enhancement of the magnetic energy product to 18.1 MGOe.X-ray diffraction(XRD)and high-resolution transmission electron micro-scope(HRTEM)reveals that SmCo5 phase occupies the major fraction,with Co atoms partially substituted by Fe and Cu *** situ Lorentz transmission electron microscopy(LTEM)observations show that the Sm(Co,Cu)5 phase effectively prohibits domain wall motions,leading to an increase of coercivity(Hc).Fe doping increases the low saturation magnetization(Ms)and low remanence(Mr)due to the Fe atom having a higher satu-ration magnetic *** magnetization reversal behaviors are further verified by micromagnetic *** results suggest that Sm-Co-based films prepared via Fe/Cu co-doping could be a promising candidate for high-performed HAMR in the future.

关键词： Magnetron sputtering High-throughput experiments Sm-Co Fe/Cu co-doping Magnetic properties Magnetic domain

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Two-step superconductor-insulator transitions in iron chalcogenide superconductors

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Physical Review B 2025年第6期111卷 L060506-L060506页

作者： Li Xu Zefeng Lin Wenxin Cheng Xuewei Wang Mingyang Qin Xingyu Jiang Liping Zhang Juan Xu Peiyu Xiong Beijing National Laboratory for Condensed Matter Physics Institute of Physics Chinese Academy of Sciences Beijing 100190 China School of Physical Sciences University of Chinese Academy of Sciences Beijing 100049 China Department of Materials Science and Engineering Southern University of Science and Technology Shenzhen 518055 China Beijing Academy of Quantum Information Sciences Beijing 100193 China School of Physics and Technology Wuhan University Wuhan 430072 China

The superconductor-insulator transition is an archetypal example of a quantum phase transition that plays a crucial role in physics and statistical mechanics. Belonging to different universality classes, the classical and quantum percolative transitions usually manifest in different systems and are studied separately. Here, we fabricate thickness-gradient FeyTe1−xSex (FTS) films and observe the existence of these two transitions. Variation in the film thickness, which controls substrate misfit and leads to a modification of Fe concentration, results in a superconducting quantum percolative transition. By exposing FTS films to air, we observe a shift in electrical resistivity behavior and a superconducting classical percolative transition. FTS films subjected to the two treatments exhibit very similar phase diagrams, except for different critical exponents. Remarkably, we identify a two-step superconductor-insulator transition at low temperature, where the appearance of superconductive zero resistivity coincides with a sign change in the temperature derivative of electrical resistivity in the normal state. Our analysis can provide a universal scheme to categorize the superconductor-insulator transition in various copper-oxide and iron-based superconductors.

关键词： Iron-based Superconductors

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Influence of extended interactions on spin dynamics in one-dimensional cuprates

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Physical Review B 2024年第16期110卷 165118页

作者： Ta Tang Daniel Jost Brian Moritz Thomas P. Devereaux Stanford Institute for Materials and Energy Sciences Department of Applied Physics Department of Materials Science and Engineering Geballe Laboratory for Advanced Materials

Quasi-one-dimensional (1D) materials provide a unique platform for understanding the importance and influence of extended interactions on the physics of strongly correlated systems due to their relative structural simplicity and the existence of powerful theoretical tools well adapted to one spatial dimension. Recently, this was highlighted by anomalous observations in the single-particle spectral function A(q,ω) of 1D cuprate chain compounds, measured by angle-resolved photoemission spectroscopy (ARPES), which were explained by the presence of a long-range attractive interaction. Such an extended interaction should leave its fingerprints on other observables, notably the dynamical spin structure factor S(q,ω), measured by neutron scattering or resonant inelastic x-ray scattering. Starting from a simple Hubbard Hamiltonian in 1D and using time-dependent density matrix renormalization group methods, we show that the presence of long-range attractive coupling, directly through an instantaneous Coulomb interaction V or retarded electron-phonon (el-ph) coupling, can introduce significant spectral weight redistribution in S(q,ω) across a wide range of doping. This underscores the significant impact that extended interactions can have on dynamical correlations among particles, and the importance of properly incorporating this influence in modeling. Our results demonstrate that S(q,ω) can provide a sensitive experimental constraint, which complements ARPES measurements, in identifying key interactions in 1D cuprates, beyond the standard Hubbard model.

关键词： Density matrix renormalization group Spin dynamics Cuprates

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Giant phonon-skyrmion coupling in ferromagnet/heavy metal heterostructures

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Physical Review B 2024年第6期110卷 064423-064423页

作者： Egor Savostin Vitaliy Lomakin Program in Materials Science and Engineering Center for Memory and Recording Research Department of Electrical and Computer Engineering

The strong impact of the strain-induced Dzyaloshinskii-Moriya interaction (SIDMI) on the magnetization dynamics of skyrmions in nanomagnetic structures is demonstrated. The effects of SIDMI are characterized by skyrmion equations (SEs) of motion and magnetoelastic (ME) equations. The study is performed on a model system of MgO/CoFe/Pt stacked on a piezoelectric substrate. The results demonstrate a major nonlinear amplification in both the first- and higher-harmonic magnitudes of the skyrmion breathing mode due to SIDMI. Remarkably, this enhancement can trigger a skyrmion collapse, enabling its deletion with ultraweak strain-induced excitations. The SIDMI effect is shown to be much more significant than the conventional ME effect. These findings open different avenues for the efficient manipulation of nanomagnetic structures through strain.

关键词： Exchange interaction Magnetic interactions Magnetization dynamics Magnetoacoustic effect Micromagnetism Spin dynamics

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Electronic structure and optical spectra of MSi2N4 (M = Mo, Ta, V) materials with single-atom decoration: a first-principles study

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Journal of materials Chemistry C 2023年第43期11卷 15097-15105页

作者： Wu, Tzu-Cheng Liao, Yin-Song Kao, Jui-Cheng Chou, Jyh-Pin Department of Physics National Tsing Hua University Hsinchu300044 Taiwan The Affiliated Senior High School of National Taiwan Normal University Taipei10658 Taiwan Tsing Hua Interdisciplinary Program National Tsing Hua University Hsinchu300044 Taiwan Department of Materials Science and Engineering National Tsing Hua University Hsinchu300044 Taiwan Department of Materials Science and Engineering National Yang Ming Chiao Tung University Hsinchu30010 Taiwan Department of Physics National Changhua University of Education Changhua50007 Taiwan

MoSi2N4 has outstanding potential for applications in electronics, spintronics, and semiconducting fabrication. This attractive scenario can be attributed to its remarkable electronic properties. In this study, we investigate the electronic structure and optical spectra of the MSi2N4 (M = Mo, Ta, and V) materials with single atom (H, N, and O) decoration using first-principles calculations. Pristine MoSi2N4 and VSi2N4 are semiconductors, and TaSi2N4 shows the half-metal properties. Decorating MoSi2N4 with single hydrogen and nitrogen atoms induces a magnetic moment. Single oxygen decorated TaSi2N4 does not change its intrinsic electronic properties, which is suitable for spintronic applications. On top of that, the semiconductor VSi2N4 can be turned into a half-metal via single hydrogen atom decoration. The absorption spectra demonstrate an enhancement in optical absorption for VSi2N4 after the decoration with a single nitrogen atom. Single atom decoration is one of the effective methods of tailoring the electronic properties of the two-dimensional MoSi2N4 family. Our findings can accelerate the development of the advanced electronic devices. © 2023 The Royal Society of Chemistry.

关键词： Silicon compounds

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Structural,magnetic and antibacterial properties of manganese-substituted magnetite ferrofluids

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International Journal of Minerals,Metallurgy and materials 2023年第7期30卷 1417-1426页

作者： Blessy Babukutty Deepalekshmi Ponnamma Swapna S.Nair Jiya Jose Saritha G.Bhat Sabu Thomas Department of Physics Central University of KeralaKasargod 671314India Materials Science and Technology Program College of Arts and SciencesQatar UniversityP.O.Box 2713DohaQatar Department of Biotechnology Cochin University of Science and TechnologyKalamasseryKeralaIndia Department of Chemistry Mahatma Gandhi UniversityKottayam 686560KeralaIndia

Manganese-substituted magnetite ferrofluids(FFs)Mnx Fe_(1-x)Fe_(2)O_(4)(x=0–0.8)were prepared in this work through a chemical coprecipitation *** controlled growth of FF nanomaterials for antibacterial activities is challenging,and therefore,very few reports are available on the *** research focuses on stabilizing aqueous FFs with the tetramethylammonium hydroxide surfactant to achieve high *** characterization reveals nanoparticles of 5–11 nm formed by the chemical reaction and nanocrystalline nature,as evident from structural ***-substituted magnetic FFs are analyzed for their structural,functional,and antibacterial performance according to the Mn-substituent *** studies show a high blue shift for Mn^(2+)-substituted Mnx Fe_(1-x)Fe_(2)O_(4)with the theoretical correlation of optical band gaps with the Mn *** superparamagnetic nature of substituted FFs causes zero coercivity and remanence,which consequently influence the particle size,cation distribution,and spin *** structural and functional performance of the FFs is correlated with the antibacterial activity,finally demonstrating the highest inhibition zone formation for Mnx Fe_(1-x)Fe_(2)O_(4)FFs.

关键词： manganese ferrofluids homogeneity antibacterial stability

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Flexible artificial synapse based on single-crystalline BiFeO_(3) thin film

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Nano Research 2022年第3期15卷 2682-2688页

作者： Zhen Zhao Amr Abdelsamie Rui Guo Shu Shi Jianhui Zhao Weinan Lin Kaixuan Sun Jingjuan Wang Junling Wang Xiaobing Yan Jingsheng Chen Key Laboratory of Brain-like Neuromorphic Devices and Systems of Hebei Province College of Electron and Information EngineeringHebei UniversityBaoding 071002China Department of Materials Science and Engineering Nanyang Technological UniversitySingapore 639798Singapore Department of Materials Science and Engineering National University of SingaporeSingapore 117576Singapore Department of Physics Southern University of Science and TechnologyShenzhen 518055China

Realization of functional flexible artificial synapse is a significant step toward neuromorphic ***,a flexible artificial synapse based on ferroelectric tunnel junctions(FTJs)is demonstrated,using BiFeO_(3)(BFO)thin film as the functional *** inorganic single crystalline FTJs grown on rigid perovskite substrates at high temperatures are integrated with the flexible plastic substrates,by using the water-soluble Sr_(3)Al_(2)O_(6)(SAO)as the sacrificial layer and the following *** transferred freestanding BFO thin film exhibits excellent ferroelectric ***,the memristive properties and the brain-like synaptic learning performance of the flexible FTJs are *** results show that multilevel resistance states were maintained well of the flexible artificial synapse,together with their stable synaptic learning *** work indicates the promising opportunity of ferroelectric thin film based flexible synapse used in the future neuromorphic computing system.

关键词： flexible ferroelectricity memristor artificial synapse

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