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IEEE/ACM Symposium on Edge Computing (SEC)

作者： Sahil Gulania Zichang He Bo Peng Niranjan Govind Yuri Alexeev Mathematics and Computer Science Division Argonne National Laboratory Lemont Illinois United States Department of Electrical and Computer Engineering University of California Santa Barbara Santa Barbara California United States Physical and Computational Sciences Directorate Pacific Northwest National Laboratory Richland Washington United States Computational Science Division Argonne National Laboratory Lemont Illinois United States

ISBN: (数字)9781665486118

ISBN: (纸本)9781665486125

Qu YBE is an open-source algebraic compiler for the compression of quantum circuits. It has been applied for the efficient simulation of the Heisenberg Hamiltonian on quantum computers. Currently, it can simulate the time dynamics of one-dimensional chains. It includes modules to generate the quantum circuits for the above as well as produce the compressed circuits, which are independent of the time step. It utilizes the Yang-Baxter equation (YBE) to perform the compression. QuYBE enables users to seamlessly design, execute, and analyze the time dynamics of the Heisenberg Hamiltonian on quantum computers. QuYBE is the first step toward making the YBE technique available to a broader community of scientists from multiple domains. The QuYBE compiler is available at https://***/ZichangHe/QuYBE.

关键词： Computers Computational modeling Pipelines Mathematical models Integrated circuit modeling Quantum circuit Compression algorithms

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InP/ZnS core/shell quantum dots: Synthesis, characterization and their application in fullerene derivative based flexible solar cells

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Results in Physics 2025年 69卷

作者： Zhichu, Chen Tahir, Muhammad Muhammad, Fida Aziz, Fakhra Ayub, Ambreen Badshah, Fazal Refat, Moamen S. Cakmak, Sadiye M. Rehan, Shanza Adam, Abdel Majid A. Alsuhaibani, Amnah Mohammed Ayob, Afida Sarker, Mahidur R Khan, Adam School of Electrical and Information Engineering Hubei University of Automotive Technology Shiyan 442002 China Semiconductor Physics & Devices Laboratory Department of Physics Faculty of Physical and Numerical Sciences Abdul Wali Khan University Mardan 23200 Pakistan Department of Electronics University of Peshawar KP Pakistan Department of Physics Women University Mardan KP 23200 Pakistan Department of Chemistry College of Science Taif University P.O. Box 11099 Taif 21944 Saudi Arabia Program of Medical Monitoring Techniques Osmangazi University Eskisehir Eskisehir 26040 Turkey Faculty of Materials and Chemical Engineering GIK Institute of Engineering Sciences and Technology Topi 23640 Pakistan Department of Physical Sport Sciences College of Sport Sciences & Physical Activity Princess Nourah bint Abdulrahman University P.O. Box 84428 Riyadh 11671 Saudi Arabia Centre for Integrated Systems Engineering and Advanced Technologies (INTEGRA) Department of Electrical Electronic and Systems Engineering Universiti Kebangsaan Malaysia Bangi 43600 Malaysia Institute of Visual Informatics Universiti Kebangsaan Selangor Malaysia Bangi 43600 Malaysia Universidad de Diseno Innovacion y Tecnología UDIT Av. Alfonso XIII 97 Madrid 28016 Spain Department of Electronics Engineering University of Engineering & Technology Peshawar (Abbottabad Campus) Abbottabad Pakistan

Herein, we report on the synthesis and characterization of p-type semiconductor indium phosphide/zinc sulphide (InP/ZnS) core/shell quantum dots (QDs) prepared via a simple solvothermal method and their potential application in bulk heterojunction (BHJ) flexible solar cell (SC). The BHJ SC composed of donor–acceptor (D-A) configuration at nanoscale provides larger interfacial junction area throughout the bulk volume of the photo-absorber D-A blend that facilitates excitons to efficiently dissociate within the bulk layer at D-A interface. Hence, InP/ZnS core–shell QDs and a fullerene derivative – phenyl C61 butyric acid methyl ester (PCBM) – are used as hybrid inorganic–organic D-A materials, respectively, to fabricate Ag/LiF/InP/ZnS-PCBM/P3HT/ITO/PET BHJ flexible SC. Indium tin oxide (ITO) coated on polyethylene terephthalate (PET), poly(3-hexylthiophene) (P3HT), lithium fluoride (LiF) and silver (Ag) are employed as a flexible substrate, hole transport layer (HTL), electron transport layer (ETL) and counter electrode, respectively. Photovoltaic (PV) properties of the fabricated BHJ flexible SC are studied under standard testing conditions (STC) i.e., 25 ⁰C, 1.5 AM global and 100 mW/cm² irradiation, which exhibit fill factor (FF) of 59 ± 0.02 % and power conversion efficiency (PCE) of 4.22 ± 0.05 %. Also, the heterojunction characteristics are investigated in dark condition (0 lx) to find series resistance (R_s), ideality factor (n), and reverse saturation current (I₀). X-ray diffraction (XRD), atomic force microscopy (AFM), scanning electron microscopy (SEM) and ultraviolet–visible (UV–vis) spectroscopy are performed to further investigate the properties of InP/ZnS-PCBM thin films. Transmission electron microscopy (TEM) image of InP/ZnS core/shell QDs confirmed the successful synthesis of QDs having an average size of 5 ± 1 nm. The InP/ZnS-PCBM D-A photo-absorber layer reveals its potential as one of good candidates for hi

关键词： Flexible solar cell Hybrid bulk heterojunction (BHJ) InP/ZnS core/shell QDs Power conversion efficiency (PCE) Quantum dots (QDs) synthesis

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Evaluating the influence of functional unit on life cycle assessment (LCA) reliability of concrete

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Materials Today: Proceedings 2024年

作者： Glenda Terán-Cuadrado Sami Sbahieh Furqan Tahir Anissa Nurdiawati Mohammed A. Almarshoud Sami G. Al-Ghamdi Chemical Engineering Program Physical Sciences and Engineering King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia KAUST Climate and Livability Initiative King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Division of Sustainable Development College of Science and Engineering Hamad Bin Khalifa University Doha 34110 Qatar Environmental Science and Engineering Program Biological and Environmental Science and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Civil and Environmental Engineering Department College of Engineering University of Jeddah (UJ) Jeddah 23890-2871 Saudi Arabia

The linear lifecycle of concrete, from production through usage to disposal, highlights its status as one of the most carbon-, energy-, and resource-intensive processes in the industry. The development of life cycle assessment (LCA) models to quantify concrete’s embodied and buildings’ operational emissions is strongly influenced by the selection of the functional unit (FU) since it dictates the magnitude and significance of the environmental burdens from concrete and buildings' life span. The chosen FU should comprehensively capture the concrete's functionalities and construction parameters. Nonetheless, establishing a FU that encompasses spatial, temporal, and intensity aspects of cement/concrete and its applications remains a significant limitation in the practice of current LCA models. This study analyzed the FU influence on the environmental footprint of concrete samples with specific compressive strengths (material level) via LCA. The LCA was conducted in OneClick LCA using the environmental product declaration (EPD) provided by the software for each ready-mix concrete sample. From the LCA results, the C 30/37 concrete mix (lowest compressive strength) exhibited the lowest carbon footprint for all the environmental indicators when a volume-based FU was considered. In contrast, the results were more favorable for the C 65/70 concrete specimen when the compressive strength (28 curing days) was chosen because less cement is needed to achieve one MPa of strength. This behavior was also observed in the modeling of a column in a building, where the mixture with the highest compressive strength (C 65/70) showed the lowest environmental impact for all the indicators. However, this assessment does not represent the actual building system's footprint. Thus, regionally specific functional units need to be established, considering not just concrete functionalities but also national regulations, stakeholder needs, and local resource availability.

关键词： Buildings Concrete Functional unit Embodied carbon emissions LEED Life cycle assessment (LCA)

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Giant and Tunable Bosonic Quantum Interference Induced by Two-Dimensional Metals

arXiv

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arXiv 2024年

作者： Zhang, Kunyan Maniyara, Rinu Abraham Wang, Yuanxi Jain, Arpit Wetherington, Maxwell T. Mai, Thuc T. Dong, Chengye Bowen, Timothy Wang, Ke Rotkin, Slava V. Hight Walker, Angela R. Crespi, Vincent H. Robinson, Joshua Huang, Shengxi Department of Electrical Engineering The Pennsylvania State University University ParkPA16802 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and Engineering The Pennsylvania State University University ParkPA16802 United States Department of Physics University of North Texas DentonTX76203 United States Materials Research Institute The Pennsylvania State University University ParkPA16802 United States Quantum Measurements Division Physical Measurement Laboratory National Institute of Standards and Technology GaithersburgMD20899 United States Department of Engineering Science and Mechanics The Pennsylvania State University University ParkPA16802 United States Department of Physics The Pennsylvania State University University ParkPA16802 United States Two-Dimensional Crystal Consortium and Materials Research Institute The Pennsylvania State University University ParkPA16802 United States

Harnessing quantum interference among bosons provides significant opportunities as bosons often carry longer coherence time than fermions1. As an example of quantum interference, Fano resonance involving phonons or photons describes the coupling between discrete and continuous states, signified by an asymmetric spectral lineshape2. Utilizing photon-based Fano resonance, molecule sensing with ultra-high sensitivity and ultrafast optical switching has been realized3,4. However, phonon-based Fano resonance, which would expand the application space to a vaster regime, has been less exploited because of the weak coupling between discrete phonons with continuous states such as electronic continuum. In this work, we report the discovery of giant phonon-based Fano resonance in a graphene/2D Ag/SiC heterostructure. The Fano asymmetry, being proportional to the coupling strength, exceeds prior reports by two orders of magnitude5-7. This Fano asymmetry arises from simultaneous frequency and lifetime matching between discrete and continuous phonons of SiC. The introduction of 2D Ag layers restructures SiC at the interface and facilitates resonant scattering to further enhance the Fano asymmetry, which is not achievable with conventional Ag thin films. With these unique properties, we demonstrated that the phonon-based Fano resonance can be used for ultrasensitive molecule detection at the single-molecule level. Our work highlights strong Fano resonance in the phononic system, opening avenues for engineering quantum interference based on bosons. Further, our findings provide opportunities for advancing phonon-related applications, including biochemical sensing, quantum transduction, and superconductor-based quantum computing. Copyright © 2024, The Authors. All rights reserved.

关键词： Bosons

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Roadmap for Unconventional Computing with Nanotechnology

arXiv

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arXiv 2023年

作者： Finocchio, Giovanni Incorvia, Jean Anne C. Friedman, Joseph S. Yang, Qu Giordano, Anna Grollier, Julie Yang, Hyunsoo Ciubotaru, Florin Chumak, Andrii Naeemi, Azad J. Cotofana, Sorin D. Tomasello, Riccardo Panagopoulos, Christos Carpentieri, Mario Lin, Peng Pan, Gang Joshua Yang, J. Todri-Sanial, Aida Boschetto, Gabriele Makasheva, Kremena Sangwan, Vinod K. Trivedi, Amit Ranjan Hersam, Mark C. Camsari, Kerem Y. McMahon, Peter L. Datta, Supriyo Koiller, Belita Aguilar, Gabriel H. Temporão, Guilherme P. Rodrigues, Davi R. Sunada, Satoshi Everschor-Sitte, Karin Tatsumura, Kosuke Goto, Hayato Puliafito, Vito Åkerman, Johan Takesue, Hiroki Ventra, Massimiliano Di Pershin, Yuriy V. Mukhopadhyay, Saibal Roy, Kaushik Wang, I-Ting Kang, Wang Zhu, Yao Kaushik, Brajesh Kumar Hasler, Jennifer Ganguly, Samiran Ghosh, Avik W. Levy, William Roychowdhury, Vwani Bandyopadhyay, Supriyo Department of Mathematical and Computer Sciences Physical Sciences and Earth Sciences University of Messina Messina98166 Italy Chandra Family Department of Electrical and Computer Engineering University of Texas at Austin AustinTX78712 United States Department of Electrical and Computer Engineering University of Texas at Dallas RichardsonTX75080 United States Department of Electrical and Computer Engineering National University of Singapore Singapore117576 Singapore Department of Engineering University of Messina Messina98166 Italy Laboratoire Albert Fert CNRS Thales Université Paris-Saclay Palaiseau91767 France IMEC Leuven3001 Belgium Faculty of Physics University of Vienna Vienna1090 Austria School of Electrical & Computer Engineering Georgia Institute of Technology AtlantaGA30332 United States Quantum and Computer Engineering Department Delft University of Technology DelftCD 2628 Netherlands Department of Electrical and Information Engineering Politecnico di Bari Bari70125 Italy Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore639798 Singapore College of Computer Science and Technology Zhejiang University Hangzhou310013 China Department of Electrical and Computer Engineering University of Southern California Los AngelesCA90089 United States Electrical Engineering Department Eindhoven University of Technology AZ Eindhoven5612 Netherlands Microelectronics Department LIRMM Université de Montpellier Montpellier34095 France Laplace CNRS UT3 INPT University of Toulouse Toulouse31062 France Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Department of Electrical and Computer Engineering University of Illinois at Chicago ChicagoIL60607 United States Department of Electrical and Computer Engineering University of California at Santa Barbara Santa BarbaraCA93106 United States School of Applied and

In the "Beyond Moore's Law" era, with increasing edge intelligence, domain-specific computing embracing unconventional approaches will become increasingly prevalent. At the same time, adopting a variety of nanotechnologies will offer benefits in energy cost, computational speed, reduced footprint, cyber resilience, and processing power. The time is ripe for a roadmap for unconventional computing with nanotechnologies to guide future research, and this collection aims to fill that need. The authors provide a comprehensive roadmap for neuromorphic computing using electron spins, memristive devices, two-dimensional nanomaterials, nanomagnets, and various dynamical systems. They also address other paradigms such as Ising machines, Bayesian inference engines, probabilistic computing with p-bits, processing in memory, quantum memories and algorithms, computing with skyrmions and spin waves, and brain-inspired computing for incremental learning and problem-solving in severely resource-constrained environments. These approaches have advantages over traditional Boolean computing based on von Neumann architecture. As the computational requirements for artificial intelligence grow 50 times faster than Moore's Law for electronics, more unconventional approaches to computing and signal processing will appear on the horizon, and this roadmap will help identify future needs and challenges. In a very fertile field, experts in the field aim to present some of the dominant and most promising technologies for unconventional computing that will be around for some time to come. Within a holistic approach, the goal is to provide pathways for solidifying the field and guiding future impactful discoveries. © 2023, CC BY-NC-SA.

关键词： Nanotechnology

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Low-Velocity-Favored Transition Radiation

引用

physical Review Letters 2023年第11期131卷 113002-113002页

作者： Jialin Chen Ruoxi Chen Fuyang Tay Zheng Gong Hao Hu Yi Yang Xinyan Zhang Chan Wang Ido Kaminer Hongsheng Chen Baile Zhang Xiao Lin Interdisciplinary Center for Quantum Information State Key Laboratory of Extreme Photonics and Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center College of Information Science & Electronic Engineering Zhejiang University Hangzhou 310027 China International Joint Innovation Center the Electromagnetics Academy at Zhejiang University Zhejiang University Haining 314400 China Department of Electrical and Computer Engineering Technion-Israel Institute of Technology Haifa 32000 Israel Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas 77005 USA School of Electrical and Electronic Engineering Nanyang Technological University Singapore 639798 Singapore Department of Physics University of Hong Kong Hong Kong 999077 China Key Lab of Advanced Micro/Nano Electronic Devices & Smart Systems of Zhejiang Jinhua Institute of Zhejiang University Zhejiang University Jinhua 321099 China Shaoxing Institute of Zhejiang University Zhejiang University Shaoxing 312000 China Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore Centre for Disruptive Photonic Technologies Nanyang Technological University Singapore 637371 Singapore

When a charged particle penetrates through an optical interface, photon emissions emerge—a phenomenon known as transition radiation. Being paramount to fundamental physics, transition radiation has enabled many applications from high-energy particle identification to novel light sources. A rule of thumb in transition radiation is that the radiation intensity generally decreases with the decrease of particle velocity v; as a result, low-energy particles are not favored in practice. Here, we find that there exist situations where transition radiation from particles with extremely low velocities (e.g., v/c<10−3) exhibits comparable intensity as that from high-energy particles (e.g., v/c=0.999), where c is the light speed in free space. The comparable radiation intensity implies an extremely high photon extraction efficiency from low-energy particles, up to 8 orders of magnitude larger than that from high-energy particles. This exotic phenomenon of low-velocity-favored transition radiation originates from the interference of the excited Ferrell-Berreman modes in an ultrathin epsilon-near-zero slab. Our findings may provide a promising route toward the design of integrated light sources based on low-energy electrons and specialized detectors for beyond-standard-model particles.

关键词： Atom or molecule scattering from surfaces Atomic & molecular collisions Cherenkov radiation Crystal optics Electron beams & optics Light-matter interaction Optical sources & detectors Optical transient phenomena Plasmonics

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Janus faces of dipolar sources in directional near-field coupling with an oriented misalignment

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physical Review A 2024年第3期109卷 033505-033505页

作者： Chenxu Bian Yuhan Zhong Xuhuinan Chen Tony Low Hongsheng Chen Baile Zhang Xiao Lin State Key Laboratory of Extreme Photonics and Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center College of Information Science and Electronic Engineering Zhejiang University Hangzhou 310027 China and International Joint Innovation Center The Electromagnetics Academy at Zhejiang University Zhejiang University Haining 314400 China Department of Electrical and Computer Engineering University of Minnesota Minneapolis Minnesota 55455 USA Key Lab of Advanced Micro/Nano Electronic Devices & Smart Systems of Zhejiang Jinhua Institute of Zhejiang University Zhejiang University Jinhua 321099 China and Shaoxing Institute of Zhejiang University Zhejiang University Shaoxing 312000 China Division of Physics and Applied Physics School of Physical and Mathematical Sciences and Centre for Disruptive Photonic Technologies Nanyang Technological University Singapore 637371 Singapore

Directional near-field coupling can enable many applications, such as directional routing, on-chip information processing, and chiral quantum optics. This directional near-field coupling is generally face dependent, since the induced near-field radiation pattern is dependent on which face (e.g., the upper or lower face) of the dipolar source is facing toward the outcoupler. In other words, the dipolar sources in the directional near-field coupling intrinsically have two faces (e.g., Janus faces), whose corresponding near-field coupling strength and coupling directionality might be distinct. Here, we outline a general physical framework to control these Janus faces in the directional near-field coupling and find that they can have the feature of an oriented misalignment. To be specific, the upper and lower radiation patterns of excited surface waves can have the same shape but are misaligned with a twist angle. For example, the twist angle can be any acute angle if the source is composed of a Huygens dipole and an electric dipole, and it can be any obtuse angle if the source is constructed by a circular electric dipole and a magnetic dipole.

关键词： Classical optics Light-matter interaction Metamaterials Near-field optics Photonics Plasmonics

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Pioneering bone regeneration: A review of cutting-edge scaffolds in tissue engineering

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Bioprinting 2024年 43卷

作者： Alex, Y. Vincent, Sumi Divakaran, Nidhin Uthappa, U.T. Srinivasan, Parthasarathy Mubarak, Suhail Al-Harthi, Mamdouh Ahmed Dhamodharan, Duraisami School for Advanced Research in Petrochemicals: Laboratory for Advanced Research in Polymeric Materials (LARPM) Central Institute of Petrochemicals Engineering and Technology (CIPET) Bhubaneswar 751024 India Mechanical Engineering Program Physical Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Mechanics of Composites for Energy and Mobility Laboratory King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia College of Chemistry and Environmental Engineering Shenzhen University Shenzhen 518055 China Department of Electronics and Communication Engineering Amrita School of Engineering Amrita Vishwa Vidyapeetham Tamil Nadu Chennai 601103 India Research Institute of Humanities and Social Sciences University of Sharjah Sharjah 27272 United Arab Emirates Interdisciplinary Research Center for Refining and Advanced Chemicals King Fahd University of Petroleum and Minerals Dhahran 31261 Saudi Arabia Department of Chemical Engineering King Fahd University of Petroleum & Minerals Dhahran Saudi Arabia

Bone tissue engineering (BTE) is aims to develop advanced strategies to regenerate damaged or diseased bone, through the integration of principles from cellular biology, biomaterials science, and engineering. The vital aspect of these studies includes the design and fabrication of scaffolds that support cell adhesion, proliferation, and differentiation, ultimately promoting the formation of new bone tissue. Recent developments in scaffold materials have focused on organic, inorganic, and composite biomaterials. Each of these showcasing unique and distinct advantages in terms of biocompatibility, biodegradability, and mechanical strength. Polymers, such as poly (lactic-co-glycolic acid) (PLGA), provide flexibility and degradation profiles, which are conducive to tissue integration. While ceramics, including hydroxyapatite (HA) and β-tricalcium phosphate (β-TCP), offer mechanical properties similar to native bone. The fusion of organic and inorganic components in composites has yielded scaffolds with enhanced functionality, such as improved osteo-conductivity and controlled degradation rates. Advanced fabrication techniques, particularly electrospinning and 3D printing, have revolutionized scaffold design by enabling precise control over pore size, porosity, and surface architecture, critical parameters for mimicking the extracellular matrix (ECM) of bone. These structural characteristics directly influence cellular behaviors such as migration, proliferation, and differentiation, which are crucial for successful bone regeneration. This review critically evaluates the recent advances in biomaterials for scaffold fabrication, with a focus on optimizing the interplay between material properties and scaffold architecture to improve therapeutic outcomes in bone regeneration. The findings underscore the importance of material selection and scaffold design in BTE and provide actionable insights for both researchers and clinicians in the development of next-generation scaffol

关键词： Biomaterials Bone scaffold design Ideal scaffold Polymer Scaffold Tissue engineering

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Micromagnetic Neural Stimulation and Spintronic Neural Sensing

Micromagnetic Neural Stimulation and Spintronic Neural Sensi...

引用

Magnetic Conference - Short Papers (INTERMAG Short Papers), IEEE International

作者： Renata Saha Denis Tonini Matthew S. Hopper Abhinav Goyal Jason Yuen Yoonbae Oh Zachary Sanger Sadegh Faramarzi Maple Shiao Dusty Van Helden Robert P. Bloom Onri J. Benally Kai Wu Susan A. Keirstead Theoden I. Netoff Walter C. Low John Osborn Kevin E. Bennet Kendall H. Lee Hojin Shin Jian-Ping Wang Department of Electrical and Computer Engineering University of Minnesota Minneapolis MN United States Department of Neurologic Surgery Mayo Clinic Rochester MN United States Medical Scientist Training Program Mayo Clinic Rochester MN United States IMPACT - the Institute for Mental and Physical Health and Clinical Translation Barwon Health Deakin University School of Medicine Geelong VIC Australia Department of Biomedical Engineering Mayo Clinic Rochester MN United States Department of Biomedical Engineering University of Minnesota Minneapolis MN United States Stem Cell Institute University of Minnesota Minneapolis MN United States Department of Surgery University of Minnesota Minneapolis MN United States Department of Neurosurgery University of Minnesota Minneapolis MN United States Division of Engineering Mayo Clinic Rochester MN United States

ISBN: (数字)9798350362213

ISBN: (纸本)9798350362220

We report our team's recent magnetic biomedical brain-related research work: 1) micromagnetic neural stimulation $(\boldsymbol{\mu} \mathbf{MS})$ ; 2) calculation of magnetic field generated by neural cells and tissues and spintronic neural sensing. First, the designing, fabrication, and testing of two micromagnetic implants - the Magnetic Pen (MagPen), a solenoid-shaped single $\boldsymbol{\mu} \mathbf{coil}$ prototype, and the Magnetic Patch (MagPatch), a rectangular helix-shaped planar $\boldsymbol{\mu} \mathbf{coil}$ array prototype, is discussed. The efficacy of micromagnetic activation using MagPen has been successfully tested over many rodent models. The MagPen prototype had its caveat in terms of mm-size, lack of multidimensional spatial control and activation at the cellular-level. To bridge this research gap, the MagPatch array was designed and fabricated to study $\boldsymbol{\mu} \mathbf{MS}$ at the single-cell resolution. Second, we used FEM exemplary models and open-source computational libraries and calculated the magnetic fields generated by individual neurons and neuronal networks at micrometer distances. Our results show that the magnetic field generated by a single-neuron action potential can be detected by ultra-high sensitivity sub-pT magnetic field sensors, which opens the door to future in vivo decoding of neuronal activities through neural networks. Room temperature, high endurance, small volume and low power make spintronic sensors one of the promising candidates for neural sensing. On this aspect, the recent experimental progress for the spintronic sensors for neural sensing has been reviewed, with a specific discussion on our effort on spintronic stack design, device fabrication and detection.

关键词： Temperature sensors Fabrication Magnetic sensors Computational modeling Prototypes Micromagnetics Magnetic fields

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3D Crumpled Ultrathin 1T MoS2 for Inkjet Printing of Mg-Ion Asymmetric Micro-supercapacitors (vol 14, pg 7308, 2020)

引用

ACS NANO 2020年第10期14卷 14247-14247页

作者： Shao, Yuanlong Fu, Jui-Han Cao, Zhen Song, Kepeng Sun, Ruofan Wan, Yi Shamim, Atif Cavallo, Luigi Han, Yu Kaner, Richard B. Tung, Vincent C. College of Energy Soochow Institute for Energy and Materials Innovations (SIEMIS) Key Laboratory of Advanced Carbon Materials and Wearable Energy Technologies of Jiangsu Province Soochow University Suzhou 215006 People’s Republic of China Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Electrical Engineering Program Computer Electrical and Mathematical Sciences (CEMS) Division KAUST Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia Department of Chemistry and Biochemistry Department of Materials Science and Engineering California NanoSystems Institute (CNSI) University of California Los Angeles Los Angeles California 90095 United States Physical Science and Engineering (PSE) Division King Abdullah University of Science and Technology (KAUST) Thuwal 23955-6900 Saudi Arabia

Metallic molybdenum disulfide (MoS2), e.g., 1T phase, is touted as a highly promising material for energy storage that already displays a great capacitive performance. However, due to its tendency to aggregate and restack, it remains a formidable challenge to assemble a high-performance electrode without scrambling the intrinsic structure. Here, we report an electrohydrodynamic-assisted fabrication of 3D crumpled MoS2 (c-MoS2) and its formation of an additive-free stable ink for scalable inkjet printing. The 3D c-MoS2 powders exhibited a high concentration of metallic 1T phase and an ultrathin structure. The aggregation-resistant properties of the 3D crumpled particles endow the electrodes with open space for electrolyte ion transport. Importantly, we experimentally discovered and theoretically validated that 3D 1T c-MoS2 enables an extended electrochemical stable working potential range and enhanced capacitive performance in a bivalent magnesium-ion aqueous electrolyte. With reduced graphene oxide (rGO) as the positive electrode material, we inkjet-printed 96 rigid asymmetric micro-supercapacitors (AMSCs) on a 4-in. Si/SiO2 wafer and 100 flexible AMSCs on photo paper. These AMSCs exhibited a wide stable working voltage of 1.75 V and excellent capacitance retention of 96% over 20 000 cycles for a single device. Our work highlights the promise of 3D layered materials as well-dispersed functional materials for large-scale printed flexible energy storage devices.

关键词： supercapacitors MoS2 printing technique Mg-ion microdevice

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