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arXiv 2022年

作者： Jia, Xun Haldar, Anubhab Kim, Jungho Wang, Yilin Fabbris, Gilberto Ludwig, Karl Kourtis, Stefanos Upton, Mary Liu, Yu Lu, Wenjian Luo, Xuan Sun, Yu-Ping Casa, Diego Sharifzadeh, Sahar Darancet, Pierre T. Cao, Yue Materials Science Division Argonne National Laboratory LemontIL60439 United States Department of Electrical and Computer Engineering Boston University BostonMA United States Advanced Photon Source Argonne National Laboratory LemontIL60439 United States Hefei National Laboratory for Physical Science at Microscale University of Science and Technology of China Hefei230026 China Department of Physics Boston University BostonMA02215 United States Division of Materials Science and Engineering Boston University BostonMA United States Institut quantique & Departement de physique Universite de Sherbrooke QCJ1K 2R1 Canada Key Laboratory of Materials Physics Institute of Solid State Physics HFIPS Chinese Academy of Sciences Hefei230031 China High Magnetic Laboratory HFIPS Chinese Academy of Sciences Hefei230031 China Collaborative Innovation Centre of Advanced Microstructures Nanjing University Nanjing210093 China Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States Pritzker School of Molecular Engineering University of Chicago ChicagoIL60637 United States

Coexistence of localized and extended excitations is central to the macroscopic properties of correlated materials. For 5d transition metal compounds, electron correlations alone generally do not lead to a metal-insulator (Mott) transition, with insulating behavior usually resulting from their coupling with magnetic ordering and/or structural distortions. 1T-TaS2 is a prototypical example of such correlated insulating behavior, with a high-symmetry metallic phase transforming into a distorted, charge density wave (CDW) insulating state at low temperatures. The relevance of the localized electron physics at play in 3d compounds to these 5d transition metal compounds remains an open question. We resolved this standing controversy in 1T-TaS2 combining resonant inelastic X-ray spectroscopy and first-principles calculations. We observed five electronic excitations arising from the interband transitions of the Ta 5d orbitals and the S 3p ligand state, with none of the excitations on the order of the Mott gap. These excitations cannot be explained within the framework of standard multiplet calculations that assume a localized wavefunction, but instead, are captured by a band theory framework accounting for the low symmetry of the crystal field in the CDW state. Our findings suggest that the electronic property of 1T-TaS2 is dominated by both plasmonic quasiparticles and inter-band transitions associated with a Drude-type response, with no resonance associated with a putative Mott transition. Our discovery provides new insights into the electron localization and the onset of insulating behavior in 5d transition metal materials. © 2022, CC BY.

关键词： Electronic properties

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Light-driven C-H activation mediated by 2D transition metal dichalcogenides

arXiv

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arXiv 2022年

作者： Li, Jingang Zhang, Di Guo, Zhongyuan Jiang, Xi Larson, Jonathan M. Zhu, Haoyue Zhang, Tianyi Gu, Yuqian Blankenship, Brian Chen, Min Wu, Zilong Huang, Suichu Kostecki, Robert Minor, Andrew M. Grigoropoulos, Costas P. Akinwande, Deji Terrones, Mauricio Redwing, Joan M. Li, Hao Zheng, Yuebing Materials Science & Engineering Program Texas Materials Institute Walker Department of Mechanical Engineering The University of Texas at Austin AustinTX78712 United States Laser Thermal Laboratory Department of Mechanical Engineering University of California BerkeleyCA94720 United States Tohoku University Sendai980-8577 Japan Materials Sciences Division Lawrence Berkeley National Laboratory BerkeleyCA94720 United States Department of Chemistry and Biochemistry Baylor University WacoTX76798 United States Department of Materials Science and Engineering The Pennsylvania State University University ParkPA16802 United States Chandra Family Department of Electrical & Computer Engineering The University of Texas at Austin AustinTX78712 United States Department of Materials Science and Engineering University of California BerkeleyCA94720 United States Energy Storage and Distributed Resources Division Lawrence Berkeley National Laboratory BerkeleyCA94720 United States National Center for Electron Microscopy Molecular Foundry Lawrence Berkeley National Laboratory BerkeleyCA94720 United States Center for Two-Dimensional and Layered Materials The Pennsylvania State University University ParkPA16802 United States Department of Physics Department of Chemistry The Pennsylvania State University University ParkPA16802 United States 2D Crystal Consortium Materials Research Institute The Pennsylvania State University University ParkPA16802 United States

C-H bond activation enables the facile synthesis of new chemicals. While C-H activation in short-chain alkanes has been widely investigated, it remains largely unexplored for long-chain organic molecules. Here, we report light-driven C-H activation in complex organic materials mediated by 2D transition metal dichalcogenides (TMDCs) and the resultant solid-state synthesis of luminescent carbon dots in a spatially-resolved fashion. We unravel the efficient H adsorption and a lowered energy barrier of C-C coupling mediated by 2D TMDCs to promote C-H activation. Our results shed light on 2D materials for C-H activation in organic compounds for applications in organic chemistry, environmental remediation, and photonic materials. © 2022, CC BY-NC-SA.

关键词： Chemical activation

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Terahertz Cavity Phonon Polaritons in Lead Telluride in the Deep-Strong Coupling Regime

arXiv

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arXiv 2025年

作者： Baydin, Andrey Manjappa, Manukumara Mishra, Sobhan Subhra Xu, Hongjing Doumani, Jacques Tay, Fuyang Kim, Dasom Rappl, Paulo H.O. Abramof, Eduardo Singh, Ranjan Hernandez, Felix G.G. Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley–Curl Institute Rice University HoustonTX77005 United States Rice Advanced Materials Institute Rice University HoustonTX77005 United States Instrumentation and Applied Physics Department Indian Institute of Science Bangalore560012 India Center for Disruptive Photonic Technologies The Photonics Institute Nanyang Technological University 639798 Singapore Department of Physics and Astronomy Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley–Curl Institute Rice University HoustonTX77005 United States Group of Research and Development in Materials and Plasma National Institute for Space Research São José dos Campos São Paulo12201-970 Brazil Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Instituto de Física Universidade de São Paulo São Paulo05508-090 Brazil Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

Lead telluride is an important thermoelectric material due to its large Seebeck coefficient combined with its unusually low thermal conductivity that is related to the strong anharmonicity of phonons in this material. Here, we have studied the resonant and nonperturbative coupling of transverse optical phonons in lead telluride with cavity photons inside small-mode-volume metallic metasurface cavities that have photonic modes with terahertz frequencies. We observed a giant vacuum Rabi splitting on the order of the bare phonon and cavity frequencies. Through terahertz time-domain spectroscopy experiments, we systematically studied the vacuum Rabi splitting as a function of sample thickness, temperature, and cavity length. Under the strongest light–matter coupling conditions, the strength of coupling exceeded the bare phonon and cavity frequencies, putting the system into the deep-strong coupling regime. These results demonstrate that this uniquely tunable platform is promising for realizing and understanding predicted cavity-vacuum-induced ferroelectric instabilities and exploring applications of light–matter coupling in the ultrastrong and deep-strong coupling regimes in quantum technology. Copyright © 2025, The Authors. All rights reserved.

关键词： Phonons

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Acoustic conditions of clinic rooms for sound field audiometry 23

Acoustic conditions of clinic rooms for sound field audiomet...

引用

23rd International Congress on Acoustics: Integrating 4th EAA Euroregio, ICA 2019

作者： Zapata-Rodriguez, Valentina Jeong, Cheol-Ho Hoffmann, Ida Cho, Wan-Ho Beldam, Mai-Britt Harte, James Michael Interacoustics Research Unit Denmark Acoustic Technology Department of Electrical Engineering Technical University of Denmark Denmark Department of Civil Engineering Technical University of Denmark Denmark Division of Physical Metrology Korea Research Institute of Standards and Science Daejeon Korea Republic of Saint-Gobain Ecophon Sweden

ISBN: (纸本)9783939296157

The British Society of Audiology (BSA) recommends a maximum reverberation time of 0.25 s for sound field audiometry in clinic rooms. The present study measured room impulse responses from 36 rooms where sound field audiometry is conducted in Denmark, Germany and the Republic of Korea. The volumes of the rooms measured ranged from 4 m3 to 60 m3, and the reverberation times ranged from 0.04 s to 0.65 s. Office type rooms where other medical tasks also take place generally lack sound absorption particularly at low frequencies. © 2019 Proceedings of the International Congress on Acoustics. All rights reserved.

关键词： Modulation power Reverberation time Sound field audiometry

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Lattice Misorientation Evolution and Grain Refinement in Al-Si Alloys under High-Strain Shear Deformation

SSRN

引用

SSRN 2021年

作者： Gwalani, Bharat Fu, Wenkai Olszta, Mathew Silverstein, Joshua Yadav, Digvijay R. Manimunda, Praveena Guzman, Anthony Xie, Kelvin Rohatgi, Aashish Mathaudhu, Suveen Powell, Cynthia A. Sushko, Peter V. Li, Yulan Devaraj, Arun Physical and Computational Sciences Directorate Pacific Northwest National Laboratory RichlandWA99354 United States Energy and Environment Directorate Pacific Northwest National Laboratory RichlandWA99354 United States Applied Process Engineering Laboratory Pacific Northwest National Laboratory RichlandWA99354 United States Department of Materials Science and Engineering Texas A&M University College StationTX77843 United States Bruker Nano Surfaces Division 9625 West 76th Street Eden PrairieMN55344 United States Material Science and Engineering Program University of California Riverside RiversideCA United States

The starting alloy microstructure can be tailored to achieve varying degrees of grain refinement and enhance mechanical properties through severe plastic shear deformation during solid-phase processing. Crystal plasticity-based grain misorientation modeling, coupled with systematic pin-on-disk tribometry-based subsurface shear deformation experiments on as-cast Al-xSi alloys (x = 0, 1, 4 at %), was conducted. The post-deformation microstructural analysis, through a combined computational and experimental approach, conclusively shows that the initial volume fraction of the hard Si phase enhances the evolution of local lattice misorientation, leading to efficient grain refinement during severe plastic shear deformation. The shear-deformation–induced nanostructure resulted in more than double the nanoindentation hardness in the processed alloy. © 2021, The Authors. All rights reserved.

关键词： Aluminum alloys

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Action2Motion: Conditioned Generation of 3D Human Motions

arXiv

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arXiv 2020年

作者： Guo, Chuan Zuo, Xinxin Wang, Sen Zou, Shihao Sun, Qingyao Deng, Annan Gong, Minglun Cheng, Li Department of Electrical and Computer Engineering University of Alberta Canada Physical Sciences Division University of Chicago United States Graduate School of Arts and Sciences Yale University United States School of Computer Science University of Guelph Canada

Action recognition is a relatively established task, where given an input sequence of human motion, the goal is to predict its action category. This paper, on the other hand, considers a relatively new problem, which could be thought of as an inverse of action recognition: given a prescribed action type, we aim to generate plausible human motion sequences in 3D. Importantly, the set of generated motions are expected to maintain its diversity to be able to explore the entire action-conditioned motion space;meanwhile, each sampled sequence faithfully resembles a natural human body articulation dynamics. Motivated by these objectives, we follow the physics law of human kinematics by adopting the Lie Algebra theory to represent the natural human motions;we also propose a temporal Variational Auto-Encoder (VAE) that encourages a diverse sampling of the motion space. A new 3D human motion dataset Copyright © 2020, The Authors. All rights reserved.

关键词： Algebra

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Acoustic Supercoupling in a Zero-Compressibility Waveguide

引用

Research 2019年第1期2019卷 1086-1095页

作者： H.Esfahlani M.S.Byrne M.McDermott A.Alù Photonics Initiative Advanced Science Research CenterCity University of New YorkNew York CityNY 10031USA Department of Electrical and Computer Engineering Te University of Texas at AustinAustinTX 78712USA Electrical Engineering Institute Ecole Polytechnique Fed´erale de Lausanne(EPFL)CH-1015 LausanneSwitzerland Naval Surface Warfare Center Carderock Division West BethesdaMD 20817USA Physics Program Graduate CenterCity University of New YorkNew York CityNY 10026USA Department of Electrical Engineering City College of New YorkNew York CityNY 10031USA

Funneling acoustic waves through largely mismatched channels is of fundamental importance to tailor and transmit sound for a variety of *** electromagnetics,zero-permittivity metamaterials have been used to enhance the coupling of energy in and out of ultranarrow channels,based on a phenomenon known as *** metamaterial channels can support total transmission and complete phase uniformity,independent of the channel length,despite being geometrically mismatched with their input and output *** the feld of acoustics,this phenomenon is challenging to achieve,since it requires zero-density metamaterials,typically realized with waveguides periodically loaded with membranes or *** to electromagnetics,the additional challenge is due to the fact that conventional acoustic waveguides do not support a cut-of for the dominant mode of propagation,and therefore zero-index can be achieved only based on a collective resonance of the loading *** we propose and experimentally realize acoustic supercoupling in a dual regime,using a compressibility-nearzero acoustic *** than engineering the channel with subwavelength inclusions,we operate at the cut-of of a higherorder acoustic mode,demonstrating the realization and efcient excitation of a zero-compressibility waveguide with efective sof *** experimentally verify strong transmission through a largely mismatched channel and uniform phase distribution,independent of the channel *** results open interesting pathways towards the realization of extreme acoustic parameters and their implementation in relevant applications,such as ultrasound imaging,acoustic transduction and sensing,nondestructive evaluation,and sound communications.

关键词： waveguide coupling realization

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Strain-tunable Berry curvature in quasi-two-dimensional chromium telluride

arXiv

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arXiv 2022年

作者： Chi, Hang Ou, Yunbo Eldred, Tim B. Gao, Wenpei Kwon, Sohee Murray, Joseph Dreyer, Michael Butera, Robert E. Foucher, Alexandre C. Ambaye, Haile Keum, Jong Greenberg, Alice T. Liu, Yuhang Neupane, Mahesh R. de Coster, George J. Vail, Owen A. Taylor, Patrick J. Folkes, Patrick A. Rong, Charles Yin, Gen Lake, Roger K. Ross, Frances M. Lauter, Valeria Heiman, Don Moodera, Jagadeesh S. Francis Bitter Magnet Laboratory Plasma Science and Fusion Center Massachusetts Institute of Technology CambridgeMA02139 United States U.S. Army CCDC Army Research Laboratory AdelphiMD20783 United States Department of Materials Science and Engineering North Carolina State University RaleighNC27695 United States Department of Electrical and Computer Engineering University of California RiversideCA92521 United States Department of Physics University of Maryland College ParkMD20742 United States Laboratory for Physical Sciences College ParkMD20740 United States Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA02139 United States Neutron Scattering Division Neutron Sciences Directorate Oak Ridge National Laboratory Oak RidgeTN37831 United States Center for Nanophase Materials Sciences Physical Science Directorate Oak Ridge National Laboratory Oak RidgeTN37831 United States Department of Physics Georgetown University WashingtonDC20057 United States Department of Physics Northeastern University BostonMA02115 United States Department of Physics Massachusetts Institute of Technology CambridgeMA02139 United States

Magnetic transition metal chalcogenides form an emerging platform for exploring spin-orbit driven Berry phase phenomena owing to the nontrivial interplay between topology and magnetism. Here we show that the anomalous Hall effect in pristine Cr2Te3 thin films manifests a unique temperature-dependent sign reversal at nonzero magnetization, resulting from the momentum-space Berry curvature as established by first-principles simulations. The sign change is strain tunable, enabled by the sharp and well-defined substrate/film interface in the quasi-two-dimensional Cr2Te3 epitaxial films, revealed by scanning transmission electron microscopy and depth-sensitive polarized neutron reflectometry. This Berry phase effect further introduces hump-shaped Hall peaks in pristine Cr2Te3 near the coercive field during the magnetization switching process, owing to the presence of strain-modulated magnetic domains. The versatile interface tunability of Berry curvature in Cr2Te3 thin films offers new opportunities for topological electronics. Copyright © 2022, The Authors. All rights reserved.

关键词： High resolution transmission electron microscopy

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Wide-angle giant photonic spin Hall effect

arXiv

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arXiv 2022年

作者： Chen, Zhihao Chen, Yu Wu, Yaodong Zhou, Xinxing Sun, Handong Low, Tony Chen, Hongsheng Lin, Xiao Key Laboratory of Low-Dimensional Quantum Structures and Quantum Control Ministry of Education Synergetic Innovation Center for Quantum Effects and Applications School of Physics and Electronics Hunan Normal University Changsha410081 China International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology Engineering Technology Research Center for 2D Material Information Function Devices and Systems of Guangdong Province Institute of Microscale Optoelectronics Shenzhen University Shenzhen518060 China Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Department of Electrical and Computer Engineering University of Minnesota MinneapolisMN55455 United States Interdisciplinary Center for Quantum Information State Key Laboratory of Modern Optical Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center College of Information Science and Electronic Engineering Zhejiang University Hangzhou310027 China International Joint Innovation Center ZJU-UIUC Institute The Electromagnetics Academy at Zhejiang University Zhejiang University Haining314400 China

Photonic spin Hall effect is a manifestation of spin-orbit interaction of light and can be measured by a transverse shift δ of photons with opposite spins. The precise measurement of transverse shifts can enable many spin-related applications, such as precise metrology and optical sensing. However, this transverse shift is generally small (i.e. δ/λ -1, λ is the wavelength), which impedes its precise measurement. To-date proposals to generate giant spin Hall effect (namely with δ/λ > 102) have severe limitations, particularly its occurrence only over a narrow angular cone (with a width of ∆0 70◦ by exploiting the interface between free space and uniaxial epsilon-near-zero media. The underlying mechanism is ascribed to the almost-perfect polarization splitting between s and p polarized waves at the designed interface. Remarkably, this almost-perfect polarization splitting does not resort to the interference effect and is insensitive to the incident angle, which then gives rise to the wide-angle giant photonic spin Hall effect. Copyright © 2022, The Authors. All rights reserved.

关键词： Polarization

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Two-Step Electronic Response to Magnetic Ordering in a van der Waals Ferromagnet

arXiv

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arXiv 2023年

作者： Wu, Han Zhu, Jian-Xin Chen, Lebing Butcher, Matthew W. Yue, Ziqin Yuan, Dongsheng He, Yu Oh, Ji Seop Huang, Jianwei Wu, Shan Gong, Cheng Guo, Yucheng Mo, Sung-Kwan Denlinger, Jonathan D. Lu, Donghui Hashimoto, Makoto Stone, Matthew B. Kolesnikov, Alexander I. Chi, Songxue Kono, Junichiro Nevidomskyy, Andriy H. Birgeneau, Robert J. Dai, Pengcheng Yi, Ming Department of Physics and Astronomy Rice Center for Quantum Materials Rice University HoustonTX77005 United States Theoretical Division Los Alamos National Laboratory Los AlamosNM87545 United States Center for Integrated Nanotechnologies Los Alamos National Laboratory Los AlamosNM87545 United States Department of Physics University of California at Berkeley BerkeleyCA94720 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Materials Sciences Division Lawrence Berkeley National Laboratory BerkeleyCA94720 United States 1-1 Namiki Ibaraki Tsukuba305-0044 Japan Department of Applied Physics Yale University New HavenCT06511 United States Department of Electrical and Computer Engineering Quantum Technology Center University of Maryland College ParkMD20742 United States Advanced Light Source Lawrence Berkeley National Laboratory BerkeleyCA94720 United States Stanford Synchrotron Radiation Lightsource SLAC National Accelerator Laboratory Menlo ParkCA94025 United States Neutron Scattering Division Oak Ridge National Laboratory Oak RidgeTN37831 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States Department of Materials Science and Engineering University of California Berkeley United States

The two-dimensional (2D) material Cr2Ge2Te6 is a member of the class of insulating van der Waals magnets. Here, using high resolution angle-resolved photoemission spectroscopy in a detailed temperature dependence study, we identify a clear response of the electronic structure to a dimensional crossover in the form of two distinct temperature scales marking onsets of modifications in the electronic structure. Specifically, we observe Te p-orbital-dominated bands to undergo changes at the Curie transition temperature TC while the Cr d-orbital-dominated bands begin evolving at a higher temperature scale. Combined with neutron scattering, density functional theory calculations, and Monte Carlo simulations, we find that the electronic system can be consistently understood to respond sequentially to the distinct temperatures at which in-plane and out-of-plane spin correlations exceed a characteristic length scale. Our findings reveal the sensitivity of the orbital-selective electronic structure for probing the dynamical evolution of local moment correlations in vdW insulating magnets. © 2023, CC BY.

关键词： Electronic structure

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