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Optimizing waste pre-collection model in Indonesian communities: comparing drop-off and door-to-door models through social cost–benefit analysis

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Journal of Material Cycles and Waste Management 2025年 1-17页

作者： Miftahadi, Machmuddin Fitra Hibino, Kohei Rachman, Indriyani Matsumoto, Toru Graduate Program in Environmental System Graduate School of Environmental Engineering The University of Kitakyushu Kitakyushu808-0135 Japan Kitakyushu Urban Centre Institute for Global Environmental Strategies Kitakyushu805-0062 Japan Department of Natural Science Education School of Postgraduate Studies Universitas Pakuan Kota Bogor16143 Indonesia Research Center for Urban Energy Management Institute of Environmental Science and Technology The University of Kitakyushu Kitakyushu808-0135 Japan

Indonesia lacks an established waste pre-collection system resulting 90% waste ending up in open-dumping site. This study identifies a 35-m radius per drop-off points as the most optimal model. The City of South Tangerang, on 21 residential areas with a population of 63,157, being examine. Utilizing ArcGIS Pro and Python scripting, 12 scenarios were developed, model drop-off radii of 15–45 m and household limits of 4–32 per drop-off point, including combined models. Spatial clustering KD-Tree algorithm and Proximity-based Routing were employed to determine collection placements and walking distances. Heatmap and ANOVA tests evaluated conformity with residential characteristics. Model then organized into eight frequency schemes, utilizing motorcart and handcart systems with 4-day and 2-day pickup schedules for waste bank and in-house compost programs. This optimized model reduces collection time by up to 81% and costs by 50% compared to traditional door-to-door systems, achieving cost reductions of $30–$38 USD per ton and lowering CO₂ emissions. The discussion covers opportunity costs and occupational risk. This approach supports Indonesia’s waste reduction targets and offers policy alignment for urban waste management. © The Author(s), under exclusive licence to Springer Nature Japan KK, part of Springer Nature 2025.

关键词： Python

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The fate of antibiotics during phosphate recovery processes - A critical review

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science of the Total Environment 2025年 968卷 178829页

作者： Bolujoko, Nathaniel Duling, Addison Shashvatt, Utsav Mangalgiri, Kiranmayi Environmental Science Graduate Program Oklahoma State University 202 Whitehurst StillwaterOK74078 United States Department of Biosystems and Agricultural Engineering Oklahoma State University 215A Agricultural Hall StillwaterOK74078 United States Department of Civil and Environmental Engineering University of California Berkeley 760 Davis Hall BerkeleyCA94720 United States

The principles of circular economy encourage the recovery of phosphorus from nutrient-rich waste streams such as animal manure, domestic wastewater, and urine to supplement existing sources of raw phosphorus. However, these waste streams also contain a wide variety of contaminants of emerging concern including antibiotics, and the recovery of phosphorus from these waste streams results in the co-occurrence of antibiotics with the recovered phosphorus products. This paper provides a comprehensive overview of the fate of environmentally relevant antibiotics in three major existing and upcoming phosphorus recovery processes: precipitation-, membrane-, and adsorption-based treatment. In general, the co-occurrence of antibiotics in recovered phosphorus increases with the presence of dissolved organic matter (DOM) and cations due to π-π interaction and cationic bridge formation, respectively. Additionally, antibiotics display pH-based speciation resulting in electrostatic interactions with recovered phosphorus at pH > 7.0. Furthermore, this critical review establishes a new metric, the relative antibiotic-to‑phosphorus (RAP), defined as the ratio of the concentration of antibiotics to phosphorus in recovered phosphorus to that of the phosphorus-rich waste. Precipitation-based methods, particularly struvite, demonstrated the lowest RAP, while the RAP in carbon-based adsorbents was 1.8 × 108 times higher than in membrane-based processes. In reviewing literature on the fate of antibiotics in phosphorus recovery processes, several research needs are also highlighted: the fate of non-tetracycline antibiotics, simultaneous investigation of phosphorus and antibiotic fate in membrane- and adsorption-based methods, treatment methods to mitigate the co-occurrence of antibiotics in recovered phosphorus product, and the release of antibiotics from recovered phosphate products. © 2024

关键词： Rivers

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Cytocompatible and antibacterial Fe-, Cu- and Zn-substituted calcium hydroxyapatite materials for skin applications

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Ceramics International 2025年第9期51卷 11286-11296页

作者： Lukaviciute, L. Lukowiak, A. Stankeviciute, Z. Junka, A. Mortimer, M. Zarkov, A. Yang, J.-C. Ganceviciene, R. Kareiva, A. Faculty of Chemistry and Geosciences Vilnius University Naugarduko st. 24 Vilnius03225 Lithuania Institute of Low Temperature and Structure Research Polish Academy of Sciences Okolna 2 Wroclaw50422 Poland Department of Pharmaceutical Microbiology and Parasitology Wroclaw Medical University Borowska 211A Wroclaw50556 Poland Laboratory of Environmental Toxicology National Institute of Chemical Physics and Biophysics Akadeemia tee 23 Tallinn12618 Estonia Graduate Institute of Nanomedicine and Medical Engineering International Ph.D. Program in Biomedical Engineering College of Biomedical Engineering Research Center of Biomedical Device Research Center of Digital Oral Science and Technology Taipei Medical University Taiwan Faculty of Medicine Vilnius University M.K. Ciurlionio st. 21 Vilnius03101 Lithuania

Calcium hydroxyapatite (C10(PO4)6(OH)2;CHAp) and metal-substituted samples (Fe:CHAp, Cu:CHAp, and Zn:CHAp) were synthesized using a recently developed method. This method involved the wet precipitation of amorphous calcium phosphate (ACP), followed by solid-state reaction synthesis of α-tricalcium phosphate (α-TCP), and finally hydrothermal synthesis of CHAp. The effect of Fe3+, Cu2+, and Zn2+ substitution on the phase purity and antimicrobial properties of CHAp are summarized in this study. Notably, it highlights the phase purity of CHAp and Zn:CHAp (in the presence of Fe3+ and Cu2+ ions, the α- and β-TCP phases have formed) as well as the antimicrobial activity of Zn:CHAp and Cu:CHAp against Staphylococcus aureus and Candida albicans. The synthesized nanosized CHAp, Fe:CHAp, Cu:CHAp, and Zn:CHAp samples were used as additives in the preparation of skin creams. In vitro biological studies of the resulting skin creams demonstrated their antimicrobial activity against Pseudomonas aeruginosa, and showed a reduction in osteoblasts cells viability of in the range of 20–40 %. The addition of zinc enhances antimicrobial efficacy but reduces biocompatibility, while copper maintains both high antimicrobial activity and biocompatibility, making it more suitable for the development of medical or cosmetic materials. Dermal creams containing CHAp with copper and iron ions also show significant antimicrobial activity while preserving good cell viability. These results highlight the importance of optimizing the balance between antimicrobial effectiveness and biocompatibility in these materials. © 2024

关键词： Biocompatibility

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Mo-terminated edges in two-dimensional molybdenum disulfide for site-specific hydrolysis and DNA cleavage

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Materials Today 2025年 86卷 162-171页

作者： Wang, Cong Wu, Menghan Li, Muqing Zhao, Yingcan Zhao, Mingchuang Zhang, Yunhao Bai, Yichao Gao, Jianxiang Wang, Xiaoxia Tian, Xilin Zhang, Han Chang, Liang Zou, Xiaolong Liu, Bilu Kang, Feiyu Terrones, Mauricio Lei, Yu Institute of Materials Research Shenzhen Key Laboratory of Advanced Layered Materials for Value-added Applications Guangdong Provincial Key Laboratory of Thermal Management Engineering and Materials & Center of Double Helix Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen518055 China Institute of Materials Research & Shenzhen Geim Graphene Center Shenzhen Key Laboratory of Advanced Layered Materials for Value-added Applications Tsinghua-Berkeley Shenzhen Institute and Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen518055 China Environmental Science Program Department of Life Sciences Beijing Normal University-Hong Kong Baptist University United International College Guangdong519087 China Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen518055 China Department of Physics Department of Chemistry Department of Materials Sciences Center for 2-Dimensional and Layered Materials The Pennsylvania State University University ParkPA16802 United States International Collaborative Laboratory of 2D Materials for Optoelectronics Science and Technology of Ministry of Education Institute of Microscale Optoelectronics Shenzhen University Shenzhen518060 China

The hydrolysis of DNA serves as the foundational principle for gene engineering that enable precise gene cleavage at the molecular level. This process typically occurs in biological nucleases, which exhibit nucleobase-selective and catalytic hydrolysis capabilities rarely replicated in abiotic nanomaterials. Here, we demonstrate that molybdenum-terminated (Mo-terminated) edges of molybdenum disulfide (MoS2) possess the unique ability to abstract a proton (H+) from water molecules, thereby facilitating catalytic hydrolysis reactions that cleave the phosphodiester bonds in DNA through the action of hydroxide ions. The enhanced proton absorption at Mo-terminated edges of MoS2 significantly reduces the activation energy required for the DNA hydrolysis reaction. Furthermore, the favorable interaction between the Mo-terminated edges and thymine nucleobases promotes both charge transfer and P-O bond cleavage, enabling targeted DNA hydrolysis at 'TTTTTTT' sequences under dark conditions. This discovery underscores the potential of MoS2 as a stable, efficient nanosystem for precise genetic editing, heralding advanced applications in the field of gene engineering. © 2025 The Author(s)

关键词： Activation energy

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Effect of double coating on microencapsulation of levofloxacin using the particles from gas-saturated solutions process as a controlled-release system

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Discover Chemistry 2025年第1期2卷 1-13页

作者： Sharmin, Tanjina Takeshita, Toshihiro Ouchi, Mikio Yoshida, Koji Znad, Hussein Saptoro, Agus Sarker, Zaidul Islam Irie, Keiichi Satho, Tomomitsu Nioh, Atsushi Masuda, Takaaki Muneyoshi, Yuuki Terayama, Suzuko Mishima, Kenji Department of Chemical Engineering Faculty of Engineering Fukuoka University Fukuoka Japan Research Institute of Composite Materials Fukuoka University Fukuoka Japan Resource Circulation Faculty of Environmental Engineering Fukuoka University Fukuoka Japan Faculty of Sciences Fukuoka University Fukuoka Japan Western Australian School of Mines: Minerals Energy and Chemical Engineering Faculty of Science and Engineering Curtin University Perth Australia Department of Chemical Engineering Faculty of Engineering Curtin Malaysia Graduate School Miri Sarawak Malaysia Department of State Program and Food Science Northern Marianas College Saipan USA Faculty of Pharmaceutical Sciences Fukuoka University Fukuoka Japan Yokohama Research Center Pola Chemical Industries Yokohama Japan

A novel double-coating technique was employed to encapsulate levofloxacin (LVF), a potent antibacterial drug, using the particles from gas-saturated solutions (PGSS) process to achieve extended release. The primary coating utilized glyceryl tristearate (GT), a lipid with a high melting point (72 °C), followed by a secondary coating with trimyristin (TM), a lipid with a lower melting point (52 °C). For comparison, a single-coating approach was also explored, using the biocompatible polymer poly-(ε-caprolactone) (PCL). The resulting particles were characterized for their shape, size, and LVF encapsulation efficiency, with confirmation of LVF entrapment provided by Fourier transform infrared (FTIR) spectroscopy, and X‐ray powder diffraction (XRD) analysis. The particles, with an average diameter of 95.3 ± 16.5 μm, exhibited an encapsulation efficiency of up to 92.1 ± 2.5%. Furthermore, in vitro release studies revealed that the double-coated microcapsules effectively suppressed the initial burst release and provided controlled, extended release of LVF (t30D = 36.3%), demonstrating the efficiency of this encapsulation method for prolonged drug delivery.

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Antioxidant system alterations and oxidative stress caused by polyfluoroalkyl substances (PFAS) in exposed biota: a review

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science of the Total Environment 2025年 977卷 179395页

作者： Soares, Lorena Oliveira Souza de Araujo, Gabriel Farias Gomes, Thais Braga Júnior, Sidney Fernandes Sales Cuprys, Agnieszka Katarzyna Soares, Raquel Moraes Saggioro, Enrico Mendes Laboratory of Environmental Health Assessment and Promotion Oswaldo Cruz Institute Oswaldo Cruz Foundation Av. Brasil 4365 RJ Rio de Janeiro21045-900 Brazil Post-Graduate Program in Public Health and Environment Sergio Arouca National School of Public Health Oswaldo Cruz Foundation Av. Leopoldo Bulhões 1480 RJ Rio de Janeiro21041-210 Brazil Faculty of Science and Technology Norwegian University of Life Sciences P.O. Box 5003 Ås1432 Norway Post-Graduate Program in Environmental Technology and Water Resources Department of Civil and Environmental Engineering – FT University of Brasília Darcy Ribeiro Campus Via L3 Norte DF Brasília70910-900 Brazil

Contamination of aquatic and terrestrial organisms by Perfluoroalkyl substances (PFAS), emerging contaminants, is widespread, as these compounds are present in water, soil, air, and food, owing to their environmental persistence. PFAS exposure induces biochemical process alterations associated with the disruption of the antioxidant defense system in several species. This review aims to discuss how PFAS-induced antioxidant system alterations lead to changes in biochemical processes in different organisms exposed to these pollutants. This disruption, then leads to an imbalance in antioxidant defense systems, contributing to the formation of reactive oxidative species (ROS), which, in turn, can be exacerbate oxidative stress, induce cellular damage, enhance lipid peroxidation, destabilize lysosomal membranes, and cause genotoxic effects, ultimately compromising DNA integrity. In acute tests, PFAS have led to mortality, growth inhibition, diminished behavioral and locomotor abilities, and reproductive impairment. PFAS-induced effects differ with varying species or types of substances, and further bioaccumulation through food chains exacerbates environmental contamination, carrying considerable risks. These findings demonstrate the complex and enduring impact of PFAS on environmental health, emphasizing the importance of this review in corroborating studies on sub-lethal toxicity in exposed organisms and how these effects reflect on the environment. © 2025 Elsevier B.V.

关键词： Biotic

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Investigation of Cyanobacteria-Hosted Antibiotic Resistance Genes in Cyanohab-Impacted Drinking Water Sources

SSRN

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SSRN 2025年

作者： Volk, Abigail Mills, Molly Chae, Soryong Lee, Jiyoung Division of Environmental Health Sciences College of Public Health The Ohio State University ColumbusOH United States Environmental Sciences Graduate Program The Ohio State University ColumbusOH United States Department of Chemical and Environmental Engineering University of Cincinnati CincinnatiOH United States Department of Food Science and Technology The Ohio State University ColumbusOH United States Infectious Diseases Institute The Ohio State University ColumbusOH United States

Freshwater cyanobacterial blooms (cyanoHABs) produce cyanotoxins that cause human and animal illness. cyanoHABs are also hypothesized to play a role in the antibiotic resistome, but whether Cyanobacteria host clinically-relevant antibiotic resistant genes (ARGs) in the environment is largely unknown. To investigate this emerging issue, we looked for the presence of Cyanobacteria-hosted ARGs using shotgun metagenomic sequencing of drinking water source samples collected during the 2022 bloom season from Lake Erie and Grand Lake St. Marys (GLSM). . ARGs were annotated using DeepARG and Resistance Gene Identifier (RGI). Cyanobacteria were annotated to host genes conferring possible antibiotic resistance. Two of these genes were rpoB2 and arlR, but these genes were likely spurious hits on housekeeping genes. qac and OXA genes were also annotated. While those hits suggest potential resistance to clinical antibiotics, overall Cyanobacteria did not host appreciable clinically-relevant ARGs. Because the two drinking water sources historically have high cyanotoxin concentrations, selected cyanotoxins, Cyanobacteria, and ARGs were chosen for quantification. We found high levels of Microcystis in Lake Erie and Planktothrix in GLSM, and high microcystin concentrations in GLSM, supporting previous trends in these water bodies. This study takes a novel approach pairing the issues of cyanoHABs and ARGs together in two drinking water sources. In a changing climate, drinking water treatment strategies should consider the treatment and public health implications of multiple contaminants. © 2025, The Authors. All rights reserved.

关键词： Lakes

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Development of ceramic membranes from sugarcane bagasse ash for microfiltration of biodiesel production effluents

Open Ceramics

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Open Ceramics 2025年 22卷

作者： Pin, Clarissa Ferreira Brandler, Danieli Flores, Gabriela Cristina Perusin Kubiaki Levandoski, William Mateus Bruschi, Giovani Jordi Pelissaro, Deise Trevizan Dervanoski, Adriana Korf, Eduardo Pavan Pasquali, Gean Delise Leal Graduate Program in Enviromental Science and Technology Federal University of Fronteira Sul Erechim/RS 99700-970 Brazil Departament of Civil Engineering Integrated Regional University of Alto Uruguai and Missões – Erechim/RS 99709-910 Brazil Departament of Environmental and Sanitary Engineering Federal University of Fronteira Sul Erechim/RS 99700-970 Brazil

Ceramic membranes have emerged as a promising solution for microfiltration processes, offering advantages such as cost-effectiveness, environmental benefits, and the utilization of abundant raw materials derived from agro-industrial solid waste. This study investigates the fabrication and performance of ceramic membranes composed of kaolin the varying proportions of sugarcane bagasse ash (SCBA - 40 wt % and 60 wt %), with focus on efficiency in treating biodiesel wastewater. The membranes were characterized (porosity, average pore diameter, and mechanical strength). The membrane containing 40 wt % SCBA - employed without any pre-treatment- exhibited the best overall performance, achieving porosity of 38.5 %, an pore diameter of 0.9 µm, and mechanical strength of 27 MPa, indicating a favorable balance between permeability and structural integrity. The best-performing membrane achieved removal efficiencies of color 83 % and turbidity 67 %. Microstructural analysis revealed a network of interconnected mesopores, which are particularly effective for the retention of colloidal and suspended contaminants. © 2025 The Authors

关键词： Agro-industrial solid waste Industrial effluent Membrane filtration

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Magnetically separable silica-chitosan hybrids for efficient phosphate adsorption in aqueous solution

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Case Studies in Chemical and environmental engineering 2025年 11卷

作者： Nuryono, Nuryono Sukamto, Sukamto Kunarti, Eko Sri Krisbiantoro, Philip Anggo Wan Abdullah, Wan Nazwanie Kamiya, Yuichi Department of Chemistry Faculty of Mathematics and Natural Sciences Universitas Gadjah Mada Bulaksumur Yogyakarta 55281 Indonesia of Life Science Hokkaido University Kita 10 Nishi 8 Kita-ku Sapporo 060-0810 Japan International Graduate Program of Molecular Science and Technology National Taiwan University No. 1 Sec. 4 Roosevelt Road Taipei 10617 Taiwan Molecular Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei 11529 Taiwan Department of Chemical Engineering College of Engineering National Taiwan University Taipei 10617 Taiwan School of Chemical Science Universiti Sains Malaysia Gelugor Penang 11800 Malaysia Faculty of Environmental Earth Science Hokkaido University Nishi 5 Kita 10 Kita-ku Sapporo 060-0810 Japan

In the present study, magnetic silica-chitosan hybrid (NMP@SiO2/CPTMS/Chi) was synthesized via a convenient and green sol-gel technique under room temperature, and the material was used as a highly efficient magnetic ... 详细信息

In the present study, magnetic silica-chitosan hybrid (NMP@SiO₂/CPTMS/Chi) was synthesized via a convenient and green sol-gel technique under room temperature, and the material was used as a highly efficient magnetic adsorbent for the removal of phosphate ions in water. While the magnetic properties of NMP from iron enable the material to be quickly separated via magnetic separation, the abundant active sites from the chitosan made the hybrid exhibit high adsorption capacity for phosphate ions. At pH 6, the removal of phosphate ions followed the pseudo-second-order (PSO) kinetic model with the adsorption rate constant (k₂) of 5.9 × 10^-3 mg g⁻¹ min⁻¹ and obeyed the Langmuir isotherm model with a maximum adsorption capacity (q_max) of 15.06 mg g⁻¹, outperforming most of the previously reported adsorbents. Stability tests and derivative thermogravimetry (DTG) analysis demonstrated that NMP@SiO₂/CPTMS/Chi remained stable even under strongly acidic conditions and possessed high thermal stability, respectively. The synergistic combination of high adsorption capacity, acid stability, thermal stability, and facile magnetic separation renders NMP@SiO₂/CPTMS/Chi a promising adsorbent for wastewater treatment and environmental remediation. Overall, this innovative material represents a significant advancement in phosphate removal, offering a sustainable and effective solution to address the global challenge of water pollution and protect aquatic ecosystems. © 2025 The Authors

关键词： Adsorption Chitosan Magnetic material Phosphate Silica Sol-gel

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Nitrite impairs bioreactor performance due to decreased replication of Candidatus Brocadia sapporoensis by unbalanced energy allocation

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Water Research 2025年 283卷 123806页

作者： Qiao, Xuejiao Zhang, Liyu Qiu, Zhiguang Wu, Yang Deng, Chunfang Geng, Yanni Zhang, Yichi Yan, Yan Li, Bing Zhang, Lijuan Zhuang, Wei-Qin Yu, Ke Eco-environment and Resource Efficiency Research Laboratory School of Environment and Energy Peking University Shenzhen Graduate School Guangdong Shenzhen518055 China -Preferred Program Peking University Shenzhen518055 China State Key Laboratory of Isotope Geochemistry CAS Center for Excellence in Deep Earth Science Guangzhou Institute of Geochemistry Chinese Academy of Sciences Guangdong Guangzhou510000 China Shenzhen Engineering Research Laboratory for Sludge and Food Waste Treatment and Resource Recovery Tsinghua Shenzhen International Graduate School Tsinghua University Shenzhen518055 China Department of Civil and Environmental Engineering The University of Auckland Auckland New Zealand

The effects of nitrite on anammox activities have been extensively studied. However, the molecular mechanisms of specific microorganisms responding to nitrite in anammox systems remain unexplored. This study investigates how excessive nitrite affects the core metabolisms of AnAOB and symbiotic bacteria, further elucidating the mechanisms by which it regulates microbial growth and nitrogen removal performance. Specifically, the nitrogen removal process in a continuous-flow anammox membrane bioreactor collapsed when the nitrite concentration reached 243 mg N/L. Integrated meta-omics analyses demonstrated that excessive nitrite disrupted the energy metabolism of Ca. Brocadia sapporoensis (AMXB1), reducing the energy available for developing tolerance. Subsequently, it disrupted cell replication by impairing the biosynthesis process of AMXB1, particularly DNA replication and the formation of vital cell structures such as the cell membrane and cell wall, as well as the cellular protection system, leading to the collapse of the anammox system. Additionally, the cross-feeding of amino acids and cofactors between AMXB1 and symbiotic bacteria plays an important role in the recovery of nitrogen removal performance of anammox consortia after nitrite inhibition. The findings provide a novel strategy and direction for improving the tolerance and resilience of anammox consortia in engineered ecosystems. © 2025

关键词： Listeria

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