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Enhancing photocatalytic CO_(2)reduction with TiO_(2)-based materials:Strategies,mechanisms,challenges,and perspectives

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environmental science and Ecotechnology 2024年第4期20卷 18-33页

作者： Zhimin Yuan Xianglin Zhu Xianqiang Gao Changhua An Zheng Wang Cheng Zuo Dionysios D.Dionysiou Hong He Zaiyong Jiang School of Chemistry&Chemical Engineering and Environmental Engineering Weifang UniversityWeifang261061PR China State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing100085PR China Institute for Energy Research School of Chemistry and Chemical EngineeringJiangsu UniversityZhenjiang212013PR China Tianjin Key Laboratory of Organic Solar Cells and Photochemical Conversion School of Chemistry and Chemical EngineeringTianjin University of TechnologyTianjin300384PR China Environmental Engineering and Science Program Department of Chemical and Environmental Engineering(DChEE)University of CincinnatiCincinnatiOH45221-0012USA College of Forestry Shandong Agricultural UniversityTaian271018PR China

The concentration of atmospheric CO_(2)has exceeded 400 ppm,surpassing its natural variability and raising concerns about uncontrollable shifts in the carbon cycle,leading to significant climate and environmental impacts.A promising method to balance carbon levels and mitigate atmospheric CO_(2)rise is through photocatalytic CO_(2)*** dioxide(TiO_(2)),renowned for its affordability,stability,availability,and eco-friendliness,stands out as an exemplary catalyst in photocatalytic CO_(2)*** strategies have been proposed to modify TiO_(2)for photocatalytic CO_(2)reduction and improve catalytic activity and product ***,few studies have systematically summarized these strategies and analyzed their advantages,disadvantages,and current ***,we comprehensively review recent advancements in TiO_(2)engineering,focusing on crystal engineering,interface design,and reactive site construction to enhance photocatalytic efficiency and product *** discuss how modifications in TiO_(2)'s optical characteristics,carrier migration,and active site design have led to varied and selective CO_(2)reduction *** enhancements are thoroughly analyzed through experimental data and theoretical ***,we identify current challenges and suggest future research directions,emphasizing the role of TiO_(2)-based materials in understanding photocatalytic CO_(2)reduction mechanisms and in designing effective *** review is expected to contribute to the global pursuit of carbon neutrality by providing foundational insights into the mechanisms of photocatalytic CO_(2)reduction with TiO_(2)-based materials and guiding the development of efficient photocatalysts.

关键词： summarized dioxide neutral

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Dimensionality reduction and prediction of soil consolidation coefficient using random forest coupling with Relief algorithm

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Frontiers of Structural and Civil engineering 2022年第2期16卷 224-238页

作者： Hai-Bang LY Huong-Lan Thi VU Lanh Si HO Binh Thai PHAM Department of Civil Engineering University of Transport TechnologyHanoi100000Vietnam Civil and Environmental Engineering Program Hiroshima UniversityHiroshima739-8527Japan Department of Science Technology and International CooperationUniversity of Transport TechnologyHanoi100000Vietnam

The consolidation coefficient of soil(C_(v))is a crucial parameter used for the design of structures leaned on soft *** general,the C_(v) is determined experimentally in the ***,the experimental tests are time-consuming as well as ***,researchers tried several ways to determine C_(v) via other simple soil *** this study,we developed a hybrid model of Random Forest coupling with a Relief algorithm(RF-RL)to predict the C_(v) of *** conduct this study,a database of soil parameters collected from a case study region in Vietnam was used for *** performance of the proposed models was assessed via statistical indicators,namely Coefficient of determination(R^(2)),Root Mean Squared Error(RMSE),and Mean Absolute Error(MAE).The proposal models were constructed with four sets of soil variables,including 6,7,8,and 13 *** results revealed that all models performed well with a high performance(R^(2)>0.980).Although the RF-RL model with 13 variables has the highest prediction accuracy(R^(2)=0.9869),the difference compared with other models was negligible(i.e.,R^(2)=0.9824,0.9850,0.9825 for the cases with 6,7,8 inputs,respectively).Thus,it can be concluded that the hybrid model of RF-RL can be employed to predict C_(v) based on the basic soil parameters.

关键词： soil consolidation coefficient machine learning random forest Relief

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Effects of superhydrophobic sand mulching on evapotranspiration and phenotypic responses in tomato (Solanum lycopersicum) plants under normal and reduced irrigation

Plant-Environment Interactions

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Plant-Environment Interactions 2022年第2期3卷 74-88页

作者： Odokonyero, Kennedy Gallo, Adair Dos Santos, Vinicius Mishra, Himanshu Environmental Science and Engineering Program Biological and Environmental Sciences and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal Saudi Arabia Water Desalination and Reuse Center (WDRC) King Abdullah University of Science and Technology (KAUST) Thuwal Saudi Arabia Chemical Engineering Program Physical Science and Engineering Division King Abdullah University of Science and Technology (KAUST) Thuwal Saudi Arabia

Irrigated agriculture in arid and semi-arid regions is a vital contributor to the global food supply. However, these regions endure massive evaporative losses that are compensated by exploiting limited freshwater resources. To increase water-use efficiency in these giga-scale operations, plastic mulches are utilized;however, their non-biodegradability and eventual land-filling renders them unsustainable. In response, we have developed superhydrophobic sand (SHS) mulching technology that is comprised of sand grains or sandy soils with a nanoscale coating of paraffin wax. Here, we investigate the effects of 1 cm-thick SHS mulching on the evapotranspiration and phenotypic responses of tomato (Solanum lycopersicum) plants as a model system under normal and reduced irrigation inside controlled growth chambers. Experimental results reveal that under either irrigation scenario, SHS mulching suppresses evaporation and enhances transpiration by 78% and 17%, respectively relative to the unmulched soil. Comprehensive phenotyping revealed that SHS mulching enhanced root xylem vessel diameter, stomatal aperture, stomatal conductance, and chlorophyll content index by 21%, 25%, 28%, and 23%, respectively, in comparison with the unmulched soil. Consequently, total fruit yields, total dry mass, and harvest index increased in SHS-mulched plants by 33%, 20%, and 16%, respectively compared with the unmulched soil. We also provide mechanistic insights into the effects of SHS mulching on plant physiological processes. These results underscore the potential of SHS for realizing food–water security and greening initiatives in arid regions. © 2022 The Authors. Plant-Environment Interactions published by New Phytologist Foundation and John Wiley & Sons Ltd.

关键词： chlorophyll content index evapotranspiration food–water security mulching Solanum lycopersicum stomatal conductance superhydrophobic sand transpiration efficiency

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Machine learning in concrete science:applications,challenges,and best practices

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npj Computational Materials 2022年第1期8卷 1192-1208页

作者： Zhanzhao Li Jinyoung Yoon Rui Zhang Farshad Rajabipour Wil V.Srubar III Ismaila Dabo Aleksandra Radlińska Department of Civil and Environmental Engineering The Pennsylvania State UniversityUniversity ParkPA16802USA Department of Structural Engineering Research Korea Institute of Civil Engineering and Building Technology(KICT)Goyang-si10223Republic of Korea Department of Civil Environmentaland Architectural EngineeringUniversity of Colorado BoulderBoulderCO80309USA Materials Science and Engineering Program University of Colorado BoulderBoulderCO80309USA Department of Materials Science and Engineering The Pennsylvania State UniversityUniversity ParkPA16802USA

Concrete,as the most widely used construction material,is inextricably connected with human *** conceptual and methodological progress in concrete science,concrete formulation for target properties remains a challenging task due to the ever-increasing complexity of cementitious *** the ability to tackle complex tasks autonomously,machine learning(ML)has demonstrated its transformative potential in concrete *** the rapid adoption of ML for concrete mixture design,there is a need to understand methodological limitations and formulate best practices in this emerging computational ***,we review the areas in which ML has positively impacted concrete science,followed by a comprehensive discussion of the implementation,application,and interpretation of ML *** conclude by outlining future directions for the concrete community to fully exploit the capabilities of ML models.

关键词： concrete directions autonomous

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Regulation of regeneration in Arabidopsis thaliana

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aBIOTECH 2023年第4期4卷 332-351页

作者： Md Khairul Islam Sai Teja Mummadi Sanzhen Liu Hairong Wei Computational Science and Engineering Program Michigan Technological UniversityHoughtonMI 49931USA Computer Science Michigan Technological UniversityHoughtonMI 49931USA Department of Plant Pathology Kansas State UniversityManhattanKS 66506USA College of Forest Resources and Environmental Science Michigan Technological UniversityHoughtonMI 49931USA

We employed several algorithms with high efficacy to analyze the public transcriptomic data,aiming to identify key transcription factors(TFs)that regulate regeneration in Arabidopsis ***,we utilized CollaborativeNet,also known as TF-Cluster,to construct a collaborative network of all TFs,which was subsequently decomposed into many subnetworks using the Triple-Link and Compound Spring Embedder(CoSE)*** analysis of these subnetworks led to the identification of nine subnetworks closely associated with *** further applied principal component analysis and gene ontology(GO)enrichment analysis to reduce the subnetworks from nine to three,namely subnetworks 1,12,and *** for TF-binding sites in the promoters of the co-expressed and co-regulated(CCGs)genes of all TFs in these three subnetworks and Triple-Gene Mutual Interaction analysis of TFs in these three subnetworks with the CCGs involved in regeneration enabled us to rank the TFs in each ***,six potential candidate TFs-WOx9A,LEC2,PGA37,WIP5,PEI1,and AIL1 from subnetwork 1-were identified,and their roles in somatic embryogenesis(GO:0010262)and regeneration(GO:0031099)were discussed,so were the TFs in Subnetwork 12 and 17 associated with *** TFs identified were also assessed using the CIS-BP database and Expression *** analyses suggest some novel TFs that may have regulatory roles in regeneration and embryogenesis and provide valuable data and insights into the regulatory mechanisms related to *** tools and the procedures used here are instrumental for analyzing high-throughput transcriptomic data and advancing our understanding of the regulation of various biological processes of interest.

关键词： Regeneration Pluripotency Transcription factor Collaborative network

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Core/shell magnetite/copolymer composite nanoparticles enabling highly stable magnetorheological response

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International Journal of Mechanical System Dynamics 2022年第2期2卷 155-164页

作者： Wenjiao Han Shun Wang Xiaoting Rui Yuzhen Dong Hyoungjin Choi School of Energy and Power Engineering Nanjing University of Science and TechnologyNanjingChina School of Materials Science and Engineering Harbin Institute of Technology at WeihaiWeihaiChina Department of Polymer Science and Engineering Inha UniversityIncheonRepublic of Korea Program of Environmental and Polymer Engineering College of EngineeringInha UniversityIncheonRepublic of Korea

Magnetorheological fluids(MRFs)have been successfully used in a variety of smart control systems,but are still limited due to their relatively poor settling ***,a core/shell‐structured Fe_(3)O_(4)/copolymer composite nanoparticle is synthesized as a new candidate material for stimulus‐responsive MRFs to tackle the limitation of the long‐term dispersion ***‐co‐diphenylamine copolymers(PANI‐co‐PDPA)are loaded onto the surface of Fe_(3)O_(4) nanoparticles,providing a lighter density and sufficient active interface for the dispersion of magnetic particles in the carrier *** features of the Fe_(3)O_(4)/copolymer composite nanoparticles,including morphology,compositional,and crystalline properties,are *** MRF is prepared by suspending Fe_(3)O_(4)/copolymer composite nanoparticles in a nonmagnetic medium oil,and its rheological properties are assessed using a controlled shear rate test and dynamic oscillation tests using a rotational *** models including the Bingham model and the Herschel–Bulkley model are fitted to the flow curves of the *** obtained Fe_(3)O_(4)/copolymer composite shows soft‐magnetic properties,as well as greater density adaptability and higher stability,compared to Fe_(3)O_(4).Moreover,the sedimentation testing provides information about the dispersion stability characteristics of MRF and shows a good correlation with high‐stability magnetorheological(MR)*** Fe_(3)O_(4)/copolymer‐based MRF with a tunable and instantaneous MR response is considered a promising material for smart control applications.

关键词： magnetorheological fluids core/shell dispersion stability copolymer magnetite

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Effect of Molarity of Potassium Hydroxide Solution on Heat Resistance of Fly Ash-Slag Based Geopolymer 2nd

Effect of Molarity of Potassium Hydroxide Solution on Heat R...

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2nd International Conference on Sustainable Civil engineering and Architecture, ICSCEA 2021

作者： Saludung, Apriany Azeyanagi, Takumu Ogawa, Yuko Kawai, Kenji Department of Civil and Environmental Engineering Graduate School of Engineering Hiroshima University 1-4-1 Kagamiyama Higashihiroshima City Japan Civil and Environmental Engineering Program Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashihiroshima City Japan

ISBN: (纸本)9789811933028

Designing a building material with high fire resistance is crucial for minimizing the impact of catastrophic fire. Geopolymer, a new type of binder synthesized by the reaction of aluminosilicate sources with an alkaline solution, has been extensively studied as it offers comparable or even high durability when compared to ordinary Portland cement (OPC). The concentration of the alkaline solution is one of the important factors that affect the durability;however, there is very little data on the heat resistance of geopolymer activated with potassium hydroxide. Thus, this study aims to investigate the effect of molarity of potassium hydroxide on the heat resistance of fly ash-slag blended geopolymer paste. The potassium hydroxide (10, 12, and 14 M) and sodium silicate solutions were prepared as activator solutions. The initial heat curing at 70 ºC for 24 h was applied. In addition, an OPC specimen was also prepared for comparison. After curing for 28 days, some specimens were exposed to high temperatures (500, 750, and 950 ºC). The compressive strength of unexposed and exposed geopolymer and OPC paste specimens was measured. The results showed that the increase of molarity of potassium hydroxide solution increased the heat resistance of geopolymer in terms of retained compressive strength. Moreover, the geopolymer specimens could maintain higher compressive strength than that of OPC paste when exposed to high temperatures up to 950 ºC. This is attributed to the mineral composition of geopolymer, which is different from OPC paste, as studied by X-ray diffraction analysis. © 2023, The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd.

关键词： Potassium hydroxide

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Ag-decorated 3D flower-like Bi_(2)MoO_(6)/rGO with boosted photocatalytic performance for removal of organic pollutants

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Rare Metals 2021年第5期40卷 1086-1098页

作者： Xin Liu Wei-Ya Huang Qin Zhou Xi-Rong Chen Kai Yang Dan Li Dionysios D.Dionysiou Faculty of Materials Metallurgical and ChemistryJiangxi University of Science and TechnologyGanzhou 341000China Environmental Engineering and Science Program Department of Chemical and Environmental EngineeringUniversity of CincinnatiCincinnatiOH 45221-0012USA College of Science HealthEngineering and EducationMurdoch UniversityMurdoch 6150Australia

A series of unique 3D flower-like Bi_(2)MoO_(6)(BMO)/reduced graphene oxide(rGO)heterostructured composites decorated with varying amounts of Ag nanoparticles(NPs)were *** morphological characteristics,structural features,energy band structures and photoelectrochemical properties were systematically *** the Ag/BMO/rGO ternary composites(AgBGy;y=1%,2%and 3%)demonstrated greater photocatalytic activity towards efficient removal of our selected organic models[methyl orange(MO),rhodamine B(RhB)and phenol],as compared with the BMO/rGO binary composites(BG-x;x=0.25,2,4 and 5).Particularly,AgBG-2%,which was synthesized with the addition of 2 wt% rGO and 2 wt%Ag in BMO,possessed superior photocatalytic *** fitted rate constants(k)for the photocatalytic degradation of RhB,MO and phenol using AgBG-2% were estimated to be 0.0286,0.0301 and 0.0165 min^(-1),respectively,which were over one order of magnitude greater than those obtained using pure *** factors may contribute to the observed enhancement,including greater specific surface area,enhanced light absorption,promoted spatial separation of electronhole(e^(-)-h^(+))pairs and their suppressed recombination,especially benefiting from the synergistic effects among BMO,rGO and Ag *** work suggests that the rational design of BMO/rGO/Ag ternary composite was an effective strategy to boost the photocatalytic activity of the resulting catalyst towards the highly efficient removal of organic pollutants from water.

关键词： Bi_(2)MoO_(6) Reduced graphene oxide Ag nanoparticles 3D flower-like morphology Photocatalytic degradation

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The effect of Zn2+ ion substitution on nanoparticles of ZnxMn(1-X) Fe2O4 (X = 0.2, 0.4, 0.6, 0.8) towards signal surface plasmon resonance (SPR)

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Materials Research Innovations 2023年第6期27卷 420-428页

作者： Almi Putra, Rachmad Andi Fadlly, Teuku Asmara, Vina Monica, Desy Sartika Hijrahnisa Novia, Wina Yakob, Muhammad Indrayana, Ipt Geubrina Raszky, Rachmita Mujahid Hamdan, Abd Arfi, Febrina Rahwanto, Adi Jalil, Zulkarnain Physics Study Program Faculty of Engineering Universitas Samudra Langsa Indonesia Doctoral Study Program School of Engineering Universitas Syiah Kuala Banda Aceh Indonesia Department of Physics Education Faculty of Teaching and Education Universitas Samudra Langsa Indonesia Physics Study Program Faculty of Natural Science and Engineering Technology Universitas Udayana Denpasar Indonesia Department of Environmental Engineering Faculty of Science and Technology UIN Ar-Raniry Banda Aceh Indonesia Department of Chemistry Faculty of Science and Technology UIN Ar-Raniry Banda Aceh Indonesia Department of Physics Faculty of Mathematics and Natural Sciences Syiah Kuala University Banda Aceh Indonesia

This study examined the effect of Zn2+ ion substitution on ZnxMn(1-x) Fe2O4 nanoparticles (x = 0.2, 0.4, 0.6, 0.8) towards signal Surface Plasmon Resonance (SPR). The co-precipitation method synthesised the nanoparticles at a temperature of 90°C. The X-Ray Diffraction (XRD) results showed a polycrystalline structure with a crystallite size varied from 19.05 nm to 19.77 nm. In addition, as the Zn element increased in the ZnxMn(1-x)Fe2O4 nanoparticles, the degree of crystallinity increased by 21.72%, respectively. The optical properties of the nanoparticles ZnxMn(1-x) Fe2O4 indicate absorbance at wavelengths of 330.36–331.74 nm. The absorbance level increased as the Zn element decreased, resulting a direct optical gap of 3.47 eV and an indirect optical gap of 3.23 eV. The Attenuated Total Reflection (ATR) curve in the SPR biosensor indicated a shift in the reflective angle of the Prism/Au/Air configuration, which is 47.78° on Prisma/Au/nanoparticle of Zn0.8Mn0.2Fe2O4/air by 50.75°, and the prism/Au/nanoparticle of Zn0.2Mn0.8Fe2 O4/air by 51.04°. The substitution of Zn ions in the compound Zn x Mn(1-x)Fe2O4 affects the resulting ATR curve. The shift in the SPR angle is caused by changes in the refractive index in each layer which is influenced by the concentration of each material which has an impact on the absorbance ability and photon reflectance. This research has the potential to continue with the testing of dielectric and magnetic properties, as well as special testing for biological analytes compatible with ZnxMn(1-x)Fe2O4 nanoparticles. © 2023 Informa UK Limited, trading as Taylor & Francis Group.

关键词： Surface plasmon resonance

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Dry-season sources of riverine sediment from the tropical mixed urban-agricultural watershed of the Mun River Basin in northeastern Thailand

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International Journal of Sediment Research 2023年第2期38卷 240-252页

作者： Arika Bridhikitti Thayukorn Prabamroong Gaohuan Liu Environmental Engineering and Disaster Management Program School of Interdisciplinary Studies Mahidol University Kanchanaburi Campus Earth Science Research Center Mahidol University Kanchanaburi Campus Faculty of Environment and Resource Studies Mahasarakham University State Key Laboratory of Resources and Environmental Information System Institute of Geographic Sciences and Natural Resources Research Chinese Academy of Sciences

Northeastern(NE) Thailand is well recognized as the land for rice cropping and consequently, it is potentially contaminated with chemicals from soil fertilization, pest/weed control, and urban *** Mun River basin in NE Thailand principally is comprised of rice paddies and sedimentation in the river has been pronounced, but the studies on sediment source identification are limited. The current study aims to identify sediment sources in the Mun River basin and discuss possible impacts on ecosystems attributed to exposure to polluted sediment. The assessment relies upon physicochemical properties and heavy metal contents(iron(Fe), manganese(Mn), copper(Cu), chromium(Cr), nickel(Ni),and Zinc(Zn)) in the fine-grained sediment(<63 μm) taken from the Mun River basin and the Chi River in the dry season of 2020-2021. The findings revealed that the heavy metals in the sediment had not accumulated to levels of concern. Most sediment was from natural sources, including Fe-and Mn-rich sediment, Cr-dominant sediment, and Ni-and Cu-rich sediment. Fe-and Zn-rich sediment was, however, found in the urban watershed of Lam Ta Klong, and it could originate from mixed urban sources. Ferich sediment was predominant in the Mun River basin, which and could be a significant sink and source of toxic elements from agricultural and urban discharges. It is suggested that the toxic compounds in the sediment should be consistently monitored, whereas ecological and health risk assessment should be focused on the mobile forms.

关键词： Sediment Heavy metals Mun River Lower Mekong River Agriculture

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