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Correction: Parallel water photo-oxidation reaction pathways in hematite photoanodes: implications for solar fuel production

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Energy & environmental science 2022年第7期15卷 3098-3098页

作者： Anton Tsyganok Paulino Monroy-Castillero Yifat Piekner Arik Yochelis Avner Rothschild Department of Materials Science and Engineering Technion – Israel Institute of Technology Haifa 3200002 Israel Department of Solar Energy and Environmental Physics Blaustein Institutes for Desert Research Ben-Gurion University of the Negev Sede Boqer Campus Midreshet Ben-Gurion 8499000 Israel Department of Physics Ben-Gurion University of the Negev Be’er Sheva 8410501 Israel The Nancy & Stephen Grand Technion Energy Program (GTEP) Technion – Israel Institute of Technology Haifa 3200002 Israel

Correction for ‘Parallel water photo-oxidation reaction pathways in hematite photoanodes: implications for solar fuel production’ by Anton Tsyganok et al., Energy Environ. Sci., 2022, https://***/10.1039/d1ee03953a.

Correction for ‘Parallel water photo-oxidation reaction pathways in hematite photoanodes: implications for solar fuel production’ by Anton Tsyganok et al., Energy Environ. Sci., 2022, https://***/10.1039/d1ee03953a.

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Is there any linkage between interstellar aldehyde and alcohol?

arXiv

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arXiv 2021年

作者： Mondal, Suman Kumar Gorai, Prasanta Sil, Milan Ghosh, Rana Etim, Emmanuel E. Chakrabarti, Sandip K. Shimonishi, Takashi Nakatani, Naoki Furuya, Kenji Tan, Jonathan C. Das, Ankan Indian Centre for Space Physics 43 Chalantika Garia Station Road Kolkata700084 India Department of Space Earth and Environment Chalmers University of Technology GothenburgSE-412 96 Sweden Department of Chemical Sciences Federal University Wukari Katsina-Ala Road P.M.B. 1020 Taraba State Wukari Nigeria Center for Transdisciplinary Research Niigata University Nishi-ku Niigata950-2181 Japan Environmental Science Program Department of Science Faculty of Science Niigata University Nishi-ku Niigata950-2181 Japan Institute for Catalysis Hokkaido University N21W10 Kita-ku Hokkaido Sapporo001-0021 Japan Center for Computational Sciences University of Tsukuba Tsukuba305-8577 Japan Department of Astronomy University of Virginia CharlottesvilleVA22904 United States Department of Chemistry Graduate School of Science and Engineering Tokyo Metropolitan University 1-1 Minami-Osawa Hachioji Tokyo192-0397 Japan National Astronomical Observatory of Japan Tokyo181-8588 Japan

It is speculated that there might be some linkage between interstellar aldehydes and their corresponding alcohols. Here, an observational study and astrochemical modeling are coupled together to illustrate the connection between them. The ALMA cycle 4 data of a hot molecular core, G10.47+0.03 is utilized for this study. Various aldehydes (acetaldehyde, propanal, and glycolaldehyde), alcohols (methanol and ethylene glycol), and a ketone (acetone) are identified in this source. The excitation temperatures and the column densities of these species were derived via the rotation diagram method assuming LTE conditions. An extensive investigation is carried out to understand the formation of these species. Six pairs of aldehyde-alcohol: i) methanal and methanol;ii) ethanal and ethanol;iii) propanal and 1-propanol;iv) propenal and allyl alcohol;v) propynal and propar gyl alcohol;vi) glycolaldehyde and ethylene glycol;vii) along with one pair of ketone-alcohol (acetone and isopropanol) and viii) ketene-alcohol (ethenone and vinyl alcohol) are considered for this study. Two succes sive hydrogenation reactions in the ice phase are examined to form these alcohols from aldehydes, ketone, and ketene, respectively. Quantum chemical methods are extensively executed to review the ice phase formation route and the kinetics of these species. Based on the obtained kinetic data, astrochemical modeling is employed to derive the abundances of these aldehydes, alcohols, ketone, and ketene in this source. It is seen that our model could successfully explain the observed abundances of various species in this hot molecular core. Copyright © 2021, The Authors. All rights reserved.

关键词： Acetone

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Correction: Thiazole-fused androstenone and ethisterone derivatives: potent β- and γ-actin cytoskeleton inhibitors to treat melanoma tumors

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RSC medicinal chemistry 2025年第4期16卷 2025 Apr 3页

作者： Sanjay Adhikary Subrata Roy Shailesh Budhathoki Siam Chowdhury Abbey Stillwell Alexei G Basnakian Alan Tackett Nathan Avaritt Mohamed Milad Mohammad Abrar Alam Department of Chemistry and Physics College of Sciences and Mathematics Arkansas State University Jonesboro Arkansas 72467 USA malam@astate.edu. Environmental Sciences Program College of Sciences and Mathematics Arkansas State University Jonesboro AR 72467 USA. Molecular Biosciences Program College of Sciences and Mathematics Arkansas State University Jonesboro AR 72467 USA. Computer Science The College of Engineering and Computer Science Arkansas State University Jonesboro AR 72468 USA. Department of Pharmacology and Toxicology University of Arkansas for Medical Sciences 4301 W. Markham St Little Rock AR 72205 USA. Central Arkansas Veterans Healthcare System W. 7th St Little Rock AR 72205 USA. Department of Biochemistry and Molecular Biology University of Arkansas for Medical Sciences Little Rock AR 72205 USA. The Department of Mathematics and Statistics Arkansas State University Jonesboro AR 72467 USA. Arkansas Biosciences Institute Arkansas State University Jonesboro AR 72467 USA.

[This corrects the article DOI: 10.1039/D4MD00719K.].

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Mediation analysis for TNF-α as a mediator between multiple metal exposure and kidney function

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Ecotoxicology and environmental safety 2024年 283卷 116837页

作者： Kuei-Hau Luo Hung-Pin Tu Huang-Chih Chang Chen-Cheng Yang Wei-Chun Weng Tzu-Hua Chen Cheng-Hong Yang Hung-Yi Chuang Graduate Institute of Medicine College of Medicine Kaohsiung Medicine University Kaohsiung City 807 Taiwan. Department of Public Health and Environmental Medicine School of Medicine College of Medicine Kaohsiung Medical University Kaohsiung 807 Taiwan. Divisions of Pulmonary & Critical Care Medicine Department of Internal Medicine Kaohsiung Chang Gung Memorial Hospital Chang Gung University College of Medicine Kaohsiung Taiwan. Graduate Institute of Medicine College of Medicine Kaohsiung Medicine University Kaohsiung City 807 Taiwan Department of Occupational Medicine Kaohsiung Municipal Siaogang Hospital Kaohsiung Medical University Kaohsiung 812 Taiwan. Division of Gastroenterology Department of Internal Medicine Kaohsiung Armed Forces General Hospital Kaohsiung 802 Taiwan. Department of Family Medicine Kaohsiung Municipal Ta-Tung Hospital Kaohsiung 801 Taiwan. Department of Information Management Tainan University of Technology Tainan 71002 Taiwan Department of Electronic Engineering National Kaohsiung University of Science and Technology Kaohsiung 80778 Taiwan. Department of Public Health and Environmental Medicine School of Medicine College of Medicine Kaohsiung Medical University Kaohsiung 807 Taiwan Department of Occupational and Environmental Medicine Kaohsiung Medicine University Hospital Kaohsiung Medicine University Kaohsiung 807 Taiwan Ph.D. Program in Environmental and Occupational Medicine College of Medicine and Research Center for Precision Environmental Medicine Kaohsiung Medical University Kaohsiung 807 Taiwan. Electronic address: ericch@kmu.edu.tw.

The association between metal mixtures and kidney function has been reported. However, reports on the mechanism of metal toxicity were limited. Oxidative stress was reported as a possible cause. This study aimed to determine the association between of kidney function and metals, such as arsenic (As), cadmium (Cd), cobalt (Co), copper (Cu), lead (Pb), selenium (Se), and zinc (Zn), and to explore the possible mediating role of tumor necrosis factor alpha (TNF-α) between metal toxicity and kidney function. In this study, we recruited 421 adults from a health examination. The concentration of blood metals was analyzed using inductively coupled plasma mass spectrometry. We used linear regression models to assess the association between metals and TNF-α. Then, mediation analysis was applied to investigate the relationship between metal exposure, TNF-α, and kidney function. In univariate linear regression, blood As, Cd, Co, Cu, Pb, and Zn levels significantly increased TNF-α and decreased kidney function. Higher blood As and Pb levels significantly increased TNF-α in multivariable linear regressions after adjusting for covariates. We found that blood levels of As (coefficients = -0.021, p = 0.011), Pb (coefficients = -0.060, p < 0.001), and Zn (coefficients = -0.230, p < 0.001) showed a significant negative association with eGFR in the multiple-metal model. Furthermore, mediation analysis showed that TNF-α mediated 41.7 %, 38.8 %, and 20.8 % of blood Cd, As and Pb, respectively. Among the essential elements, TNF-α mediated 24.5 %, 21.5 % and 19.9 % in the effects of blood Co, Cu, and Zn on kidney function, respectively. TNF-α, acting as a mediator, accounted for 20.1 % of the contribution between the WQS score of metal mixtures and the eGFR (p < 0.001). This study suggested that TNF-α may be a persuasive pathway mediating the association between metals and kidney function. Inflammation and kidney injury could be the underlying mechanisms of metal exposure. However, there i

关键词： Kidney function Mediation analysis Metals Pb TNF-α

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Effect of adoption of electric vehicles on public health and air pollution in China: a modelling study

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The Lancet Planetary Health 2021年 5卷 S8-S8页

作者： Daniel E Horton Jordan L Schnell Daniel R Peters David C Wong Xi Lu Hao Gao Hongliang Zhang Patrick L Kinney Department of Earth and Planetary Sciences and Institute for Sustainability and Energy Northwestern University Evanston IL USA Cooperative Institute for Research in Environmental Sciences at the University of Colorado Boulder National Oceanic and Atmospheric Administration Global Systems Laboratory Boulder CO USA Program in Environmental Sciences Northwestern University Evanston IL USA Environmental Defense Fund Austin TX USA US Environmental Protection Agency Research Triangle Park NC USA School of Environment State Key Joint Laboratory of Environment Simulation and Pollution Control Tsinghua University Beijing China Beijing China Department of Earth System Science University of California Irvine Irvine CA USA Department of Environmental Science and Engineering Fudan University Shanghai China Department of Environmental Health Boston University School of Public Health Boston MA USA

Background Adoption of electric vehicles has the potential to reduce air pollutant and greenhouse gas emissions, hence China has implemented policies incentivising use of electric vehicles. However, much is unknown about the potential air quality and public health benefits of electric vehicles, including optimal vehicle type prioritisation and the vehicles' ability to reduce acute health impacts due to extreme air quality events. We aimed to assess the potential climate and acute public health benefits of use of electric vehicles during an extreme winter air pollution event. Methods In this modelling study, we used the Weather Research Forecast and Community Multiscale Air Quality Modeling System air quality model to simulate the interplay between weather and atmospheric chemistry. We used this model to examine potential co-benefits of electric vehicle adoption during an extreme pollution episode in China. We simulated heavy-duty and light-duty electric vehicle adoption scenarios, in which 40% of the population adopted a heavy-duty or light-duty passenger electric vehicle, re-mapped battery power needs to energy generation facilities, and characterised differences in public health outcomes using China-specific concentration-response functions. Findings We found that widespread adoption of heavy-duty electric vehicles would reduces nitric oxide and fine particulate matter resulting in 562 (95% CI 410–723) fewer premature acute deaths than the non-electrified baseline scenario. However, widespread adoption of heavy-duty electric vehicles does not reduce carbon dioxide emissions without the addition of emission-free electricity generation. By contrast, widespread adoption of light-duty electric vehicles robustly reduces greenhouse gas emissions, but results in lesser air quality improvements and fewer premature deaths avoided (145 [95% CI 38–333]) than the heavy-duty scenario. Economic effects of human health endpoints and carbon dioxide reductions for adoption of ligh

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Analysis of Urban Forest Needs as Anthropogenic (CO2) Gas Absorbent in Semarang City 2

Analysis of Urban Forest Needs as Anthropogenic (CO2) Gas Ab...

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2nd International Conference on Energy, environmental and Information System, ICENIS 2017

作者： Febriani, Anisa Putri Soeprobowati, Tri Retnaningsih Maryono, Maryono Master Program of Environmental Science School of Postg. Stu. Diponegoro University Semarang Indonesia Departemen Biology Faculty of Science and Mathematic Diponegoro University Semarang Indonesia Department Urban and Regional Planning Faculty Engineering Diponegoro University Semarang Indonesia

Green open space in cities in significant needs to maintenance environment quality. On of the critical function is to absorb increasing number of gas CO2. Therefore, developing urban forest in cities is very importance. The objective of the study is to determine the area of urban forest as CO2 gas anthropogenic absorb which is formed from fuel, diesel fuel, liquid petroleum gas. The study consists of (1) Analyzing the number of CO2 gas emission by calculating the needs of petroleum and gas based on the number of population, (2) Analyzing the power of gas absorption, (3) Measuring the air concentration of CO2 gas ambient based on daily traffic activities. This study shown that from year 2013 to year 2017, the increasing of urban forest is not so significant. For year 2013 the green open space in Semarang City are 373.67 hectares (7.5 percent from Semarang City area), consists of 239 parks, 11 public cemeteries, production forests, community forests, and urban forests, however the area of urban forest is not increase. The study assess that Antidesmabunius is one of the green species which high absorb capacity planted for Semarang. This trees produce 31,31 ton annually. This study proposed to fostering Antidesmabunius as one principle threes in Semarang urban forest. © 2018 The Authors, published by EDP sciences.

关键词： Carbon dioxide

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Biologically-induced synthetic manganese carbonate precipitate (BISMCP) for potential applications in heavy metal removal

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Heliyon 2023年第5期9卷

作者： Dewi, Anggraeni Kumala Sharma, Raju Kumar Das, Koyeli Sukul, Uttara Lin, Pin-Yun Huang, Yi-Hsun Lu, Chung Ming Lu, Cheng-Kang Chen, Tsung-Hsien Chen, Chien-Yen Department of Physics National Chung Cheng University University Road Minhsiung Chiayi County 62102 Taiwan Doctoral Program in Science Technology Environment and Mathematics Department of Earth and Environmental Sciences National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Department of Chemistry and Biochemistry National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Department of Biomedical Sciences Graduate Institute of Molecular Biology National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Department of Chemical Engineering National Chung Cheng University University Road Minhsiung Chiayi County 62102 Taiwan Department of Chest Division Internal Medicine Ditmanson Medical Foundation Chiayi Christian Hospital 600566 Taiwan Department of Internal Medicine Ditmanson Medical Foundation Chiayi Christian Hospital 600566 Taiwan Center for Nano Bio-Detection Center for Innovative Research on Aging Society AIM-HI National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan

Heavy metal pollution of water is a burning issue of today's world. Among several strategies involved for heavy metal remediation purpose, biomineralization has shown great potential. Of late, research has been focused on developing effective mineral adsorbents with reduced time and cost consumption. In this present paper, the Biologically-Induced Synthetic Manganese Carbonate Precipitate (BISMCP) was produced based on the biologically-induced mineralization method, employing Sporosarcina pasteurii in aqueous solutions containing urea and MnCl₂. The prepared adsorbent was characterized using Fourier transform infrared spectroscopy (FTIR), scanning electron microscopy (SEM), SEM-energy dispersive X-ray spectroscopy (SEM-EDX), X-ray diffraction (XRD) and BET surface area analyzer. EDX analysis showed the elements in the crystal BISMCP were Mn, C, and O. XRD result of BISMCP determined the crystal structure, which is close to rhodochrosite (MnCO₃). Spectral peaks of FTIR at 1641.79 cm⁻¹ confirmed the appearance of C[dbnd]O binding, with strong stretching of CO₃²⁻ in Amide I. From the six kinds of BISMCP produced, sample MCP-6 has the higher specific surface area by BET analysis at 109.01 m²/g, with pore size at 8.76 nm and higher pore volume at 0.178 cm³/g. These specifications will be suitable as an adsorbent for heavy metal removal by adsorption process. This study presents a preliminary analysis of the possibility of BISMCP for heavy metals adsorption using ICP multi-element standard solution XIII (As, Cr, Cd, Cu, Ni, and Zn). BISMCP formed from 0.1 MnCl₂ and 30 ml of bacteria volume (MCP-6) produced a better adsorbent material than others concentrations, with the adsorption efficiency of total As at 98.9%, Cr at 97.0%, Cu at 94.7%, Cd at 88.3%, Zn at 48.6%, and Ni at 29.5%. Future work could be examined its efficiency adsorbing individual heavy metals. © 2023

关键词： Adsorbent material Biologically induced mineralization Biomineralization Heavy metal removal Manganese carbonate (MnCO3) Sporosarcina pasteurii

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Comparison of online group discussion and class discussion learning for a soil mechanics class

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IOP Conference Series: Materials science and engineering 2020年第3期830卷

作者： T S N Rachmawati C R Priadi F H Sagitaningrum B Swantika A Q Mairizal A Abdillah H B Santoso K Junus Civil Engineering Program Department of Civil Engineering Universitas Indonesia Depok 16424 Indonesia Engineering Education Working Group Faculty of Engineering Universitas Indonesia Depok 16424 Indonesia Environmental Engineering Program Department of Civil Engineering Universitas Indonesia Depok 16424 Indonesia Digital Library and Distance Learning Lab Faculty of Computer Science Universitas Indonesia Depok 16424 Indonesia

Soil Mechanics had been a fundamental science material that needs a great understanding of the concept. Many attempts had been done in varying the study method for this course. An attempt to utilize online discussion learning will be discussed in this paper. To analyze the online learning experience, the Community of Inquiry (CoI) model was utilized. The CoI model divides the dynamic online learning process as social presence, teaching presence, and cognitive presence. This study aims to compare the application of CoI in the Soil Mechanics course between two different types of discussion under the Civil engineering Department at a large public university in Indonesia. The students of the Soil Mechanics course were given two types of problem-based online discussions for two learning topics. The first one was a case study of Consolidation Settlement in a Group Discussion, while the second one was a case study of Seepage in a Class Discussion, which was done in one single discussion forum. Through quantitative analysis of the students' discussion transcripts, it was found that cognitive presence was dominantly higher than teaching presence and social presence in both types of discussion. Finally, through an interview with students, it was found that students with active participation gain several benefits, among others, the better ability of systematic and critical thinking of interpreting a problem and growing sense of engineering compare to passive students.

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Evaluation of dynamics of capillary rise of water in various papers

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Palpu Chongi Gisul/Journal of Korea Technical Association of the Pulp and Paper Industry 2018年第2期50卷 20-28页

作者： Yang, Han-Nwi Cho, Byoung-Uk Program of Paper Science and Engineering College of Forest and Environmental Sciences Kangwon National University Chuncheon24341 Korea Republic of

This study was conducted to elucidate and to model the dynamics of capillary rise of water in various papers using the Klemm method. Dynamics of water absorption by capillary rise in various papers such as fine paper, newsprint, tissues, and color paper were measured and the relationships between the Klemm method and other sizing test methods were evaluated. It was found that the dynamics of water absorption in paper by capillary rise can be modelled using the first order process model and thus the first order transfer function. The Klemm sizing degree had a high positive correlation (r=0.98) with the process gain K of the water absorption model while it has a negative correlation (r=-0.67) with the time constant x, meaning that the transfer rate of water was faster when the height of water absorption was higher. Klemm sizing degree was highly influenced by bulk and ash content of paper, and contact angle of water on paper. Correlation coefficients between each sizing test methods were not so high, meaning that any sizing degree test method can not represent all methods and a proper testing method shall be selected considering the purpose of usage. © 2018 Korean Technical Assoc. of the Pulp and Paper Industry. All rights reserved.

关键词： Dynamics

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An effect of humid climate on micro structure and chemical component of natural composite (Boehmeria nivea-Albizia falcata) based wind turbine blade 2

An effect of humid climate on micro structure and chemical c...

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2nd International Conference on Energy, environmental and Information System, ICENIS 2017

作者： Sudarsono, S. Purwanto, P. Sudarsono, Johny W. Department of Mechanical Engineering Institut Sains Dan Teknoogi AKPRIND Yogyakarta Indonesia Department of Chemical Engineering Faculty of Engineering Universitas Diponegoro Indonesia Doctoral Program of Environmental Science School of Postgraduate Studies Universitas Diponogero Semarang Indonesia Depart. of Material and Metallurgy Faculty of Engineering Universitas Indonesia Jakarta Indonesia

In this work, wind turbine blade NACA 4415 is fabricated from natural composite of Boehmeria nivea and Albizia falcate. The composite fabrication method used is hand lay up method. The aim of the work is to investigate an effect of humid climate of coastal area on micro structure and chemical composition of composite material of the blade. The wind turbine is tested at Pantai Baru, Bantul, Yogyakarta for 5.5 months. The micro structure scanning is performed with Scanning Electron Microscope (SEM) and material component is measured with Energy Dispersive X-ray spectrometer (EDS). The samples are tested before and after the use within 5.5 month at the location. The results show that composite material inexperienced interface degradation and insignificant change of micro structure. From EDS test, it is observed that Na filtration reduces C and increases O in composite material after 5.5 months. © 2018 The Authors, published by EDP sciences.

关键词： Microstructure

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