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Ion-Anchoring Dipole-Integrated Composite Elastomer Electrolyte and Cathode for High-Performance Lithium Metal Batteries via Multiple-Bridge engineering

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Advanced Energy Materials 2025年第0期

作者： Cho, A Hyeon Je, Ji Hyang Choi, U Hyeok Department of Polymer Science and Engineering and Program in Environmental and Polymer Engineering Inha University Incheon22212 Korea Republic of

Solid-state electrolytes (SSEs) hold significant potential for advancing lithium metal batteries (LMBs) by enhancing safety through the replacement of liquid electrolytes. However, challenges such as low ionic conductivity, limited electrochemical stability, and poor electrolyte/electrode interface compatibility hinder the development of high-energy-density LMBs. Herein, a strategy for designing SSEs is proposed using multiple-bridge engineered composite elastomer electrolytes (CEEs) that incorporate ion-rotating dipole interactions, ion-anchoring dipole interactions, and hydrogen bonding, along with a CEE-based composite elastomer cathode (CEC). This design combines a volume-adaptive elastomer matrix, a high-Li+ conducting deep eutectic electrolyte, and robust nanowires. The resultant CEE exhibits high ionic conductivity (1.7 × 10−3 S cm−1), a lithium transference number of 0.72, and a wide electrochemical stability window (up to 4.9 V) at 298 K. The engineered uniform Li+ flux also promotes stable Li plating/stripping for over 900 h at 0.1 mA cm−2. Furthermore, the LFP-based CEC|CEE|Li full cells deliver a reversible capacity of 133 mAh g−1 with 95% retention after 300 cycles in coin cells, and 129 mAh g−1 with 96% retention after 250 cycles in pouch cells at 1 C. This strategy presents a promising approach for designing solid-state polymer electrolytes to extend the lifespan of high-energy-density LMBs. © 2025 Wiley-VCH GmbH.

关键词： Elastomers

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MOF-Derived Bimetal-Embedded Carbon with Etched Morphologies as an Efficient Activator of Peroxymonosulfate for Eliminate Emerging Contaminants

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Korean Journal of Chemical engineering 2024年第6期41卷 1815-1831页

作者： Chen, Yi-Chun Jiang, Xin-Yu Lin, Jia-Yin Thanh, Bui Xuan Wang, Haitao Huang, Chao-Wei Ghotekar, Suresh Huang, Chih-Feng Lin, Kun-Yi Andrew Department of Biotechnology National Formosa University Yunlin63208 Taiwan Department of Environmental Engineering & amp Innovation and Development Center of Sustainable Agriculture National Chung Hsing University Taichung Taiwan Semiconductor and Green Technology Program National Chung Hsing University 250 Kuo-Kuang Road Taichung Taiwan Ho Chi Minh City Viet Nam Ho Chi Minh City700000 Viet Nam Key Laboratory of Pollution Processes and Environmental Criteria College of Environmental Science and Engineering Nankai University Tianjin300071 China Department of Engineering Science National Cheng Kung University Tainan70101 Taiwan Centre for Herbal Pharmacology and Environmental Sustainability Chettinad Hospital and Research Institute Chettinad Academy of Research and Education Kelambakkam Tamil Nadu Chennai603103 India Department of Chemical Engineering National Chung Hsing University Taichung Taiwan Institute of Analytical and Environmental Sciences National Tsing Hua University Hsinchu Taiwan Department of Civil Engineering National Taipei University of Technology Taipei City Taiwan

As bis(4-hydroxyphenyl)methanone (BHP) is one of the most common UV light stabilizers (UVLS), but exhibits endocrine disrupting toxicity, this study aims to develop useful sulfate radical-based techniques to eliminate BHP from water by activating peroxymonosulfate (PMS). Hence, while cobalt (Co) exhibits efficacy as a transition metal for the activation of PMS, the utilization of manganese/cobalt (Mn/Co) bimetallic oxides presents an even more encouraging prospect as heterogeneous catalysts for PMS activation. In this study, we have successfully produced N-doped carbon-supported Mn/Co nanoparticles (NCMC) with a distinctive hollow-engineered nanostructure. The synthesis involved the utilization of Co-MOF as a precursor, followed by easy etching and Mn doping to achieve the desired composition of Mn/Co bimetallic oxide nanoparticles. The inclusion of Mn dopant facilitates the integration of Mn/Co nanoparticles into the hollow-structured N-doped carbon matrix. NCMC demonstrates much higher activity compared to NCC and the benchmark catalyst, Co3O4 NP, in terms of PMS activation for the degradation of BHP. The findings of the eco-toxicity study indicate that the degradation of BHP by NCMC + PMS does not yield hazardous or extremely toxic byproducts, so establishing NCMC as a potentially effective heterogeneous catalyst for activating PMS in the degradation of BHP. © The Author(s), under exclusive licence to Korean Institute of Chemical Engineers, Seoul, Korea 2024.

关键词： Transition metals

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Identification of Extreme Precipitation Changes Due to Climate Change in Indonesia 3rd

Identification of Extreme Precipitation Changes Due to Clima...

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3rd International Conference on Radioscience, Equatorial Atmospheric science and Environment, INCREASE 2023

作者： Aminah, Siti Riawan, Edi Syahputra, Muhammad Ridho Kuntoro, Arno Adi Master Program in Water Resource Management Faculty of Civil and Environmental Engineering Bandung Institute of Technology Bandung Indonesia Atmospheric Sciences Research Group Faculty of Earth Science and Technology Bandung Institute of Technology Bandung Indonesia Water Resources Engineering Research Group Faculty of Civil and Environmental Engineering Bandung Institute of Technology Bandung Indonesia

ISBN: (纸本)9789819707393

This study uses Global Precipitation Measurement (GPM) and Coupled Model Intercomparison Project Phase 6 (CMIP6) precipitation data to identify extreme precipitation intensity and frequency changes in Indonesia. Extreme precipitation calculations were performed using the Gumbel distribution and return period fitted to annual maxima data. Extreme precipitation and frequency of extreme events were compared between the historical period and the near-future period (2026–2055) and the far-future period (2070–2099) to identify changes. The results showed that there were changes in extreme precipitation in Indonesia both in intensity and frequency of occurrence. Extreme precipitation with a 5-year return period in Indonesia generally has a change value in the range of − 5 to + 25% with most areas likely to increase. The increased value reaches + 20% in the near-future period and + 40% in the far-future period. For the frequency of extreme precipitation above the 5-year return period in Indonesia, the change value is generally in the range of − 40 to + 120% with most areas likely to increase. The increased value reaches + 160% in the near-future period and + 200% in the far-future period. In the higher emission scenario (SSP5-8.5), the areas with higher values of increase will expand both in the change in intensity and frequency of occurrence. © The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd. 2024.

关键词： Climate change

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Effect of Molarity of Potassium Hydroxide Solution on Heat Resistance of Fly Ash-Slag Based Geopolymer 2nd

Effect of Molarity of Potassium Hydroxide Solution on Heat R...

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2nd International Conference on Sustainable Civil engineering and Architecture, ICSCEA 2021

作者： Saludung, Apriany Azeyanagi, Takumu Ogawa, Yuko Kawai, Kenji Department of Civil and Environmental Engineering Graduate School of Engineering Hiroshima University 1-4-1 Kagamiyama Higashihiroshima City Japan Civil and Environmental Engineering Program Graduate School of Advanced Science and Engineering Hiroshima University 1-4-1 Kagamiyama Higashihiroshima City Japan

ISBN: (纸本)9789811933028

Designing a building material with high fire resistance is crucial for minimizing the impact of catastrophic fire. Geopolymer, a new type of binder synthesized by the reaction of aluminosilicate sources with an alkaline solution, has been extensively studied as it offers comparable or even high durability when compared to ordinary Portland cement (OPC). The concentration of the alkaline solution is one of the important factors that affect the durability;however, there is very little data on the heat resistance of geopolymer activated with potassium hydroxide. Thus, this study aims to investigate the effect of molarity of potassium hydroxide on the heat resistance of fly ash-slag blended geopolymer paste. The potassium hydroxide (10, 12, and 14 M) and sodium silicate solutions were prepared as activator solutions. The initial heat curing at 70 ºC for 24 h was applied. In addition, an OPC specimen was also prepared for comparison. After curing for 28 days, some specimens were exposed to high temperatures (500, 750, and 950 ºC). The compressive strength of unexposed and exposed geopolymer and OPC paste specimens was measured. The results showed that the increase of molarity of potassium hydroxide solution increased the heat resistance of geopolymer in terms of retained compressive strength. Moreover, the geopolymer specimens could maintain higher compressive strength than that of OPC paste when exposed to high temperatures up to 950 ºC. This is attributed to the mineral composition of geopolymer, which is different from OPC paste, as studied by X-ray diffraction analysis. © 2023, The Author(s), under exclusive license to Springer Nature Singapore Pte Ltd.

关键词： Potassium hydroxide

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Seagrass Meadows under the Changing Climate:A Review of the Impacts of Climate Stressors

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Research in Ecology 2022年第1期4卷 27-36页

作者： Kuok Ho Daniel Tang Tony Hadibarata Environmental Science Program Division of Science and TechnologyBeijing Normal University-Hong Kong Baptist University United International CollegeZhuhaiGuangdong519087China Environmental Engineering Program Faculty of Engineering and ScienceCurtin University MalaysiaCDT 250MiriSarawak98009Malaysia

Seagrass meadows provide important ecological functions,particularly by serving as carbon sinks and breeding grounds for marine *** change has threatened seagrass communities,causing their replacement,loss and increased *** review examined scholarly articles published between 2010-2021 to comprehensively present the impacts of climate change on seagrass *** shows that ocean warming negatively affects seagrass communities by favouring communities of lower structuring capacities,thus reducing the effectiveness of their ecological *** warming also promotes the propagation and spread of invasive species,and changes the trophic structures leading to further loss of seagrasses of *** seawater temperature is associated with shoot mortality and retarded growth of certain *** level rise causes more wave energy to be received by coastal seagrass communities,thus,creating more damage to the *** sea limits light penetration and alters distribution of seagrass *** dioxide enrichment of seawater increases photosynthetic rate of seagrasses but ocean warming and acidification counteract this beneficial *** dioxide enrichment affects different seagrass species and different parts of a seagrass species differently,and,where beneficial to seagrass communities,could enhance their ecological *** extremes could kill seagrasses while marine heatwaves and flooding could act synergistically to increase carbon demand of certain seagrasses and unfavourably change their *** impacts are often aggravated by anthropogenic *** review calls for more studies and conservation efforts to understand the impacts of climate change on seagrass communities and future-proof them against the changing climate.

关键词： Climate change Extreme weather Seagrass Ocean warming Ocean acidification Vulnerability

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Navigating Legal Frameworks for National Resilience: A Comparative Analysis of Key Disaster Management Laws in Thailand and Japan 4

Navigating Legal Frameworks for National Resilience: A Compa...

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4th International Symposium on Instrumentation, Control, Artificial Intelligence, and Robotics, ICA-SYMP 2025

作者： Laosunthara, Ampan Thongthip, Ratchaneekorn Krutphong, Kodchakorn School of Environment and Society Institute of Science Tokyo Tokyo Japan Disaster Preparedness Mitigation and Management Department of Civil & Infrastructure Engineering Pathumthani Thailand Environmental Engineering and Disaster Management Program Mahidol University Kanchanaburi Thailand

ISBN: (纸本)9798331505400

This study compares the disaster management laws of Thailand and Japan. The research reveals significant differences in legislative approaches, reflecting each country's unique historical, and governance contexts. Japan's law demonstrates a more comprehensive approach to the disaster management cycle and stakeholder involvement, with integrated financial provisions. Thailand's law emphasizes organizational aspects. Both prioritize response measures but show potential gaps in addressing preparedness and mitigation phases. The study identifies areas for further investigation, including financial measures, and international cooperation approaches. This comparative analysis offers valuable insights into both countries' ongoing development of disaster management systems and highlights potential areas for mutual learning and improvement in disaster risk reduction strategies. Creating resilience in the society through the core of the government working and stakeholders' given authorities. © 2025 IEEE.

关键词： Disaster prevention

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Advancing Understanding of Urgent Gaps and Needs in Atmospheric science Key Insights from the Climate, Weather, and Water Forum

Advancing Understanding of Urgent Gaps and Needs in Atmosphe...

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作者： Zhang, Lujia Song, Yurong Cheng, Tat Fan Lu, Mengqian Interdisciplinary Program Office Hong Kong University of Science and Technology Hong Kong Department of Civil and Environmental Engineering Hong Kong University of Science and Technology Hong Kong

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ANALYSIS OF NITROGEN FLOW IN FOOD WASTE: A CASE STUDY OF THE UNIVERSITY RESTAURANT-UNB 32nd

ANALYSIS OF NITROGEN FLOW IN FOOD WASTE: A CASE STUDY OF THE...

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32nd European Biomass Conference and Exhibition, EUBCE 2024

作者： Ramos, Arthur Augusto Frasson De Brites, Eneida Campos Felipe Soares, Raquel Moraes Silveira, Edgar A. Contreras, Francisco University of Brasilia Department of Civil and Environmental Engineering DF Brasilia70910-900 Brazil University of Brasilia Graduate Program on Environmental Technology and Water Resources Department of Civil and Environmental Engineering DF Brasilia70910-900 Brazil Federal Institute of Education Science and Technology of Brasília Estrutural Campus DF Brasília71250-000 Brazil University of Brasília Mechanical Sciences Graduate Program Laboratory of Energy and Environment DF Brasilia70910-900 Brazil

With the projected global population reaching 9.7 billion by 2050, the production and consumption of food continue to escalate. Nitrogen is pivotal in this landscape due to its significance in living organisms and the environmental repercussions associated with nutrient-rich waste. Inappropriate disposal of such residues contributes to nitrogen release into the environment, impacting aquatic ecosystems and precipitating the generation of greenhouse gases. This study tackles the global challenge of effectively managing nitrogen in food waste by utilizing Material Flow Analysis (MFA) as a tool to comprehend this cycle. The analysis uncovered that vegetables, legumes, and fruits constitute the primary sources of waste generation, while meats, despite their lower mass, account for a substantial proportion of total nitrogen depletion. In the surveyed month of October 2023, 174,834 meals were served, resulting in an average food consumption N-footprint of 0.003 kg of nitrogen discarded per individual meal within the restaurant’s organic waste. These findings indicate that 65% of nitrogen is consumed in meal form, while 35% is discarded as organic solid waste. However, 53% of the nitrogen in the residues originates from food preparation processes, with food preparation responsible for over half of this figure. A deeper process analysis reveals that vegetables have low nitrogen concentrations, although they significantly contribute to waste at all stages. In contrast, meats and eggs, with higher nitrogen concentrations, emerge as noteworthy contributors to the overall nitrogen content in waste. Vegetables and meats contribute about 50% and 45% of the total nitrogen, respectively. These outcomes substantially enhance our comprehension of waste generation dynamics and nutrient utilization at the university restaurant, assisting with waste management, design of sustainable menus, reduction of food waste, and optimized resource utilization, contributing to sustainability and re

关键词： Effluent treatment

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Machine learning in concrete science:applications,challenges,and best practices

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npj Computational Materials 2022年第1期8卷 1192-1208页

作者： Zhanzhao Li Jinyoung Yoon Rui Zhang Farshad Rajabipour Wil V.Srubar III Ismaila Dabo Aleksandra Radlińska Department of Civil and Environmental Engineering The Pennsylvania State UniversityUniversity ParkPA16802USA Department of Structural Engineering Research Korea Institute of Civil Engineering and Building Technology(KICT)Goyang-si10223Republic of Korea Department of Civil Environmentaland Architectural EngineeringUniversity of Colorado BoulderBoulderCO80309USA Materials Science and Engineering Program University of Colorado BoulderBoulderCO80309USA Department of Materials Science and Engineering The Pennsylvania State UniversityUniversity ParkPA16802USA

Concrete,as the most widely used construction material,is inextricably connected with human *** conceptual and methodological progress in concrete science,concrete formulation for target properties remains a challenging task due to the ever-increasing complexity of cementitious *** the ability to tackle complex tasks autonomously,machine learning(ML)has demonstrated its transformative potential in concrete *** the rapid adoption of ML for concrete mixture design,there is a need to understand methodological limitations and formulate best practices in this emerging computational ***,we review the areas in which ML has positively impacted concrete science,followed by a comprehensive discussion of the implementation,application,and interpretation of ML *** conclude by outlining future directions for the concrete community to fully exploit the capabilities of ML models.

关键词： concrete directions autonomous

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Dimensionality reduction and prediction of soil consolidation coefficient using random forest coupling with Relief algorithm

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Frontiers of Structural and Civil engineering 2022年第2期16卷 224-238页

作者： Hai-Bang LY Huong-Lan Thi VU Lanh Si HO Binh Thai PHAM Department of Civil Engineering University of Transport TechnologyHanoi100000Vietnam Civil and Environmental Engineering Program Hiroshima UniversityHiroshima739-8527Japan Department of Science Technology and International CooperationUniversity of Transport TechnologyHanoi100000Vietnam

The consolidation coefficient of soil(C_(v))is a crucial parameter used for the design of structures leaned on soft *** general,the C_(v) is determined experimentally in the ***,the experimental tests are time-consuming as well as ***,researchers tried several ways to determine C_(v) via other simple soil *** this study,we developed a hybrid model of Random Forest coupling with a Relief algorithm(RF-RL)to predict the C_(v) of *** conduct this study,a database of soil parameters collected from a case study region in Vietnam was used for *** performance of the proposed models was assessed via statistical indicators,namely Coefficient of determination(R^(2)),Root Mean Squared Error(RMSE),and Mean Absolute Error(MAE).The proposal models were constructed with four sets of soil variables,including 6,7,8,and 13 *** results revealed that all models performed well with a high performance(R^(2)>0.980).Although the RF-RL model with 13 variables has the highest prediction accuracy(R^(2)=0.9869),the difference compared with other models was negligible(i.e.,R^(2)=0.9824,0.9850,0.9825 for the cases with 6,7,8 inputs,respectively).Thus,it can be concluded that the hybrid model of RF-RL can be employed to predict C_(v) based on the basic soil parameters.

关键词： soil consolidation coefficient machine learning random forest Relief

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