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Win-Win:Anthropogenic circularity for metal criticality and carbon neutrality

Frontiers of environmental Science & Engineering 2023年第2期17卷 111-122页

作者： Xianlai Zeng State Key Joint Laboratory of Environment Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing 100084China

Resource depletion and environmental degradation have fueled a burgeoning discipline of anthropogenic circularity since the *** generally consists of waste reuse,remanufacturing,recycling,and *** economy and“zero-waste”cities are sweeping the globe in their current practices to address the world’s grand concerns linked to resources,the environment,and ***,metal criticality and carbon neutrality,which have become increasingly popular in recent years,denote the material's feature and state,*** goal of this article is to determine how circularity,criticality,and neutrality are *** anthropogenic circularity has the potential to expand the metal supply and,as a result,reduce metal *** barely accomplished 15%of its potential emission reduction by recycling iron,copper,and *** circularity has a lot of room to achieve a win-win objective,which is to reduce metal criticality while also achieving carbon neutrality in a near closed-loop *** barriers or challenges for conducting anthropogenic circularity are deriving from the inadequacy of life-cycle insight governance and the emergence of anthropogenic circularity *** flow analysis and life cycle assessment are the central methodologies to identify the hidden *** processing and smelting,as well as end-of-life management,are indicated as critical priority areas for enhancing anthropogenic circularity.

关键词： Anthropogenic circularity Material flow analysis Criticality Carbon neutrality Solid waste Circular economy

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Effects of surface fluoride modification on TiO_(2)for the photocatalytic oxidation of toluene

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Journal of environmental Sciences 2025年第1期147卷 561-570页

作者： Shaoyu Yuan Min Chen Xiaoxiao Qin Xueyan Chen Jianghao Zhang Changbin Zhang State Key Joint Laboratory of Environment Simulation and Pollution Control Research Center for Eco-Environmental SciencesChinese Academy of SciencesBeijing 100085China University of Chinese Academy of Sciences Beijing 100049China

In the present study,we investigated the influence of surface fluorine(F)on TiO_(2)for the photocatalytic oxidation(PCO)of ***_(2)modified with different F content was prepared and *** was found that with the increasing of F content,the toluene conversion rate first increased and then ***,CO_(2)mineralization efficiency showed the opposite *** on the characterizations,we revealed that F substitutes the surface hydroxyl of TiO_(2)to form the structure of≡*** presence of the appropriate amount of surface≡Ti-F on TiO_(2)greatly enhanced the separation of photogenerated carriers,which facilitated the generation of·OH and promoted the activity for the PCO of *** was further revealed that the increase of only·OH promoted the conversion of toluene to ring-containing intermediates,causing the accumulation of intermediates and then conversely inhibited the·OH generation,which led to the decrease of the CO_(2)mineralization *** above results could provide guidance for the rational design of photocatalysts for toluene oxidation.

关键词： Photocatalysis TiO_(2) Toluene Fluorine

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Single and combined effects of secondary polyethylene microplastic on the growth of Pak choi and the soil microbiome composition

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Frontiers of environmental Science & Engineering 2024年第5期18卷 1-12页

作者： Jiamin Hu Zhenwen Xie Jiane Zuo State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua UniversityBeijing100084China Tsinghua Shenzhen International Graduate School Tsinghua UniversityShenzhen518055China

It has been confirmed that microplastics(MPs)are present in the *** study simulated secondary PE-MPs via aging and mechanical processes to evaluate their effects on Pak choi(Brassica rapa L.)over 21 *** common pollutants,dichlorodiphenyltrichloroethane(DDT)and naphthalene,were used in the combined toxicity *** results indicated that the growth of Pak choi was significantly inhibited after exposure to secondary PE-MPs,and the combined effects were antagonistic,owing to the adsorption capacity of secondary PE-MPs to DDT and *** stress in Pak choi can be markedly affected,leading to oxidative damage to plant *** moisture content,soil bulk density,soil density,cation exchange capacity(CEC),and FDA hydrolase in the planted soils increased in the treated groups,and the TOC content changed *** also found that the microbial composition of the soil in the DDT and naphthalene groups showed more significant alterations than that in the other *** diversity analysis showed that species diversity increased in the combined groups but indicated a clear downward trend in the single MPs *** study suggests that secondary PE-MPs harm the growth of Pak choi and can change soil properties,revealing the harm to the ecosystem of MPs in the soil.

关键词： Secondary PE-MPs Combined effects Oxidative stress Soil properties Bacterial community

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Chemodiversity of soil dissolved organic matter affected by contrasting microplastics from different types of polymers

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Frontiers of environmental Science & Engineering 2023年第12期17卷 149-162页

作者： Hong Yu Beidou Xi Lingling Shi Wenbing Tan State Key Laboratory of Environmental Criteria and Risk Assessment and State Environmental Protection Key Laboratory of Simulation and Control of Groundwater PollutionChinese Research Academy of Environmental SciencesBeijing 100012China

Chemodiversity of dissolved organic matter(DOM)is a crucial factor controlling soil nutrient availability,greenhouse gas emissions,and pollutant ***(MPs)are widespread pollutants in terrestrial ecosystems in many ***,the effects of MPs on DOM chemodiversity are not sufficiently understood,particularly under different types of *** UV-Vis spectroscopy,3D fluorescence spectroscopy,and Fourier-transform ion cyclotron resonance mass spectrometry,the effects of three prevalent MPs[polyethylene,polystyrene,and polyvinyl chloride(PVC)]on the chemical properties and composition of soil DOM were investigated via a 310-d soil incubation *** results showed that MPs reduced the aromatic and hydrophobic soil DOM components by more than 20%,with PVC MPs having the greatest ***,as MP contents increase,the humification level of soil DOM significantly *** increased DOM molecules with no heteroatom by 8.3%-14.0%,but decreased DOM molecules with nitrogen content by 17.0%-47.8%.This may be because MPs cause positive“priming effect,”resulting in the breakdown of bioavailable components in soil *** is also related to MPs changing microbial richness and diversity and enriching microbial communities involved in lignin compositions *** the presence of MPs,soil DOM chemodiversity depended on soil pH,electrical conductivity,dissolved organic carbon,soil organic matter,bacterial Shannon,and fungal Chao ***,DOM in MP-contaminated soils featured more lipids and less condensed aromatics and proteins/amino sugars,thereby conferring a lower DOM aromaticity and higher lability.

关键词： Microplastics Dissolved organic matter FT-ICR MS Chemodiversity Molecular signature

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Thermodynamic-based ecological scaling theory in urban metabolic framework:a review

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Frontiers of environmental Science & Engineering 2025年第1期19卷 69-85页

作者： Gengyuan Liu Mingwan Wu State Key Joint Laboratory of Environmental Simulation and Pollution Control School of EnvironmentBeijing Normal UniversityBeijing 100875China Beijing Engineering Research Center for Watershed Environmental Restoration&Integrated Ecological Regulation Beijing 100875China

Prior research has consistently demonstrated that urban economic and social systems adhere to the empirical scaling ***,a plethora of evidence,including the scale-free networks of energy metabolism,the allometric growth patterns of species and populations,and the scaling law relationship between exergy and transformity in biosphere systems across various levels,indicates that urban ecosystems exhibit multi-level scaling law characteristics in energy metabolism under self-organization,alongside significant human activity *** study synthesizes these findings to hypothesize that urban ecological components are also aligned with system-level scaling theory within the urban metabolism *** encompasses:1)the existence of multistable coexistence and mutual transformation phenomena,mirroring the dynamic nature of scaling laws;and 2)a nuanced balance between the ecosystem and the socio-economic system,particularly in the realms of spatial competition and output *** ecosystem scaling theory hypotheses of urban metabolic processes offer a theoretical foundation for identifying ecological security tipping points,which are pivotal in the strategic decision-making for ecological planning and management in the future.

关键词： Ecosystem scaling theory Urban metabolism Complexity Critical review

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Synergistic promotion of particulate matter reduction and production performance via adjusting electrochemical reactions in the zinc electrolysis industry

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Frontiers of environmental Science & Engineering 2024年第1期18卷 23-33页

作者： Zizhen Ma Jingkun Jiang Lei Duan Jianguo Deng Fuyuan Xu Zehui Li Linhua Jiang Ning Duan School of Environmental and Municipal Engineering Qingdao University of TechnologyQingdao 266520China State Key Joint Laboratory of Environmental Simulation and Pollution Control School of the EnvironmentTsinghua UniversityBeijing 100084China State Key Laboratory of Pollution Control and Resources Reuse College of Environmental Science and EngineeringTongji UniversityShanghai 200092China School of Physics Peking UniversityBeijing 100871China

Heavy particulate matter (PM) pollution and high energy consumption are the bottlenecks of hydrometallurgy, especially in the electrolysis process. Therefore, an urgent need is to explore PM reduction methods with production performance co-benefits. This study presents three PM reduction methods based on controlling operating parameters, i.e., lowering electrolyte temperature, H2SO4 concentration, and current density of the cathode. The optimized conditions were also investigated using the response surface methodology to balance the PM reduction effect and Zn production. The results showed that lowering electrolyte temperature is the most efficient, with an 89.0% reduction in the PM generation flux (GFPM). Reducing H2SO4 concentration led to the minimum side effects on the current efficiency of Zn deposition (CEZn) or power consumption (PC). With the premise of non-deteriorating CEZn and PC, GFPM can be reduced by 86.3% at the optimal condition (electrolyte temperature = 295 K, H2SO4 = 110 g/L, current density = 373 A/m^(2)). In addition, the reduction mechanism was elucidated by comprehensively analyzing bubble characteristics, electrochemical reactions, and surface tension. Results showed that lower electrolyte temperature inhibited the oxygen evolution reaction (OER) and compressed gas volume. Lower H2SO4 concentration inhibited the hydrogen evolution reaction (HER) and reduced electrolyte surface tension. Lower current density inhibited both OER and HER by decreasing the reaction current. The inhibited gas evolutions reduced the microbubbles’ number and size, thereby reducing GFPM. These results may provide energy-efficient PM reduction methods and theoretical hints of exploring cleaner PM reduction approaches for industrial electrolysis.

关键词： Zinc electrolysis Particulate matter Energy consumption Operating parameters Bubble characteristic Electrochemical reaction

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Evolution of soil DOM during thermal remediation below 100℃:concentration,spectral characteristics and complexation ability

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Frontiers of environmental Science & Engineering 2024年第8期18卷 31-41页

作者： Wan Huang Ziren Wan Di Zheng Lifeng Cao Guanghe Li Fang Zhang State Key Joint Laboratory of Environment Simulation and Pollution Control State Environment Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China National Engineering Laboratory for Site Remediation Technologies Beijing 100015China

The impact of thermal remediation on soil function has drawn increasing *** far,as the most active fraction of soil organic matter,the evolution of dissolved organic matter(DOM)during the thermal remediation lacks in-depth investigation,especially for the temperatures value below 100℃.In this study,a series of soil thermal treatment experiments was conducted at 30,60,and 90℃ during a 90-d period,where soil DOM concentration increased with heating temperature and *** molecular weight,functional groups content and aromaticity of DOM all decreased during the thermal *** excitation-emission matrices(EEM)results suggested that humic acid-like substances transformed into fulvic acid-like substances(FIII/FV increased from 0.27 to 0.44)during the heating process,and five DOM components were further identified by *** change of DOM structures and components indicated the decline of DOM stability and hydrophilicity,and can potentially change the bioavailability and *** temperature also resulted in the decline of DOM complexation ability,which may be caused by the loss of binding sites due to the decrease of polar function groups,aromatic structures and hydrophilic *** study provides valuable information about the evolution of DOM during thermal remediation,which would potentially change the fate of metal ions and the effectiveness of the post-treatment technologies in the treated region.

关键词： Thermal remediation below 100℃ Heating temperature Soil DOM concentration DOM spectral characteristics Excitation-emission matrices(EEM) Complexation ability

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A global perspective on microbial risk factors in effluents of wastewater treatment plants

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Journal of environmental Sciences 2024年第4期138卷 227-235页

作者： Kejing Chen Jinsong Liang Yuhan Wang Yechen Tao Yun Lu Aijie Wang School of Civil and Environmental Engineering Harbin Institute of TechnologyShenzhen 518055China Shenzhen Guohuan Environmental Protection Technology Development Co. LTD.Shenzhen 518055China State Key Joint Laboratory of Environmental Simulation and Pollution Control State Environmental Protection Key Laboratory of Microorganism Application and Risk ControlSchool of EnvironmentTsinghua UniversityBeijing 100084China

Effective monitoring and management of microbial risk factors in wastewater treatment plants(WWTPs)effluents require a comprehensive investigation of these risks.A global survey on microbial risk factors in WWTP effluents could reveal important insights into their risk *** study aims to explore the abundance and types of antibiotic resistance genes(ARGs),virulence factor genes(VFGs),the vector of ARG/VFG,and dominant pathogens in global WWTP *** collected 113 metagenomes of WWTP effluents from the Sequence Read Archive of the National Center for Biotechnology Information and characterized the microbial risk *** results showed that multidrug resistance was the dominant ARG type,while offensive virulence factors were the most abundant type of *** most dominant types of ARGs in the vector of plasmid and phage were both aminoglycoside resistance,which is concerning as aminoglycosides are often a last resort for treating multi-resistant *** baumannii was the most dominant pathogen,rather than Escherichia coli,and a weak negative correlation between Escherichia coli and two other dominant pathogens(Acinetobacter baumannii and Bacteroides uniformis)suggests that using Escherichia coli as a biological indicator for all pathogens in WWTP effluents may not be *** Getah virus was the most dominant virus found in global WWTP *** study presents a comprehensive global-scale investigation of microbial risk factors in WWTP effluents,providing valuable insights into the potential risks associated with WWTP effluents and contributing to the monitoring and control of these risks.

关键词： Wastewater treatment plant Microbial risk factor Effluent Pathogen Antibiotic resistance gene Virulence factor gene

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Effects of exogenous acylated homoserine lactones on biofilms in biofilters for gaseous toluene treatment

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Frontiers of environmental Science & Engineering 2023年第2期17卷 29-38页

作者： Zhuqiu Sun Bairen Yang Marvin Yeung Jinying Xi Environmental Simulation and Pollution Control State Key Joint Laboratory School of EnvironmentTsinghua UniversityBeijing 100084China School of Environmental Science and Engineering Yancheng Institute of TechnologyYancheng 224051China

Biofilters are typical biofilm reactors, and they usually have poor biofilm formation resulting in limited reactor performance. Exogenous acylated homoserine lactones (AHLs) can enhance biofilm formation in many bioreactors based on quorum sensing regulation. However, their effect on biofilm in biofilters utilized for volatile organic compound (VOC) removal is unknown and needs to be investigated. In this study, the effects of the exogenous AHLs on biofilters for gaseous toluene removal were investigated. Analysis of biofilms in biofilters showed that the addition of exogenous AHLs considerably enhanced biofilm growth;the average biofilm concentration increased by 18%. Furthermore, the average biofilm coverage proportions in biofilters with and without exogenous AHLs were 17 % and 13 %, respectively, demonstrating the positive effect of exogenous AHLs on biofilm coverage. In particular, exogenous AHLs promoted the production of extracellular polymeric substances and the microbial adhesive strength of the biofilm. In addition, the exogenous AHLs showed no significant effect on the gaseous toluene removal efficiency of the biofilter. These results show that exogenous AHLs can enhance biofilm formation and can guide the application of exogenous AHLs in VOC biofilters.

关键词： Quorum sensing AHLs Biofilter Biofilm formation

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A probe into the acid deposition mitigation path in China over the last four decades and beyond

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National Science Review 2024年第4期11卷 84-92页

作者： Qian Yu Xiaodong Ge Haotian Zheng Jia Xing Lei Duan Dongwei Lv Dian Ding Zhaoxin Dong Yisheng Sun Posch Maximilian Danni Xie Yu Zhao Bin Zhao Shuxiao Wang Jan Mulder Thorj?rn Larssen Jiming Hao State Key Laboratory of Environmental Simulation and Pollution Control School of EnvironmentTsinghua University State Key Laboratory of Pollution Control &Resource Reuse and School of the Environment Nanjing University State Environmental Protection Key Laboratory of Sources and Control of Air Pollution Complex School of EnvironmentTsinghua University International Institute for Applied System Analysis(IIASA) School of Land Engineering Chang'an University Faculty of Environmental Sciences and Natural Resource Management Norwegian University of Life Sciences Norwegian Institute for Water Research

China currently has the highest acid deposition globally, yet research on its status, impacts, causes and controls is lacking. Here, we compiled data and calculated critical loads regarding acid deposition. The results showed that the abatement measures in China have achieved a sharp decline in the emissions of acidifying pollutants and a continuous recovery of precipitation p H, despite the drastic growth in the economy and energy consumption. However, the risk of ecological acidification and eutrophication showed no significant decrease. With similar emission reductions, the decline in areas at risk of acidification in China(7.0%) lags behind those in Europe(20%) or the USA(15%). This was because, unlike Europe and the USA, China's abatement strategies primarily target air quality improvement rather than mitigating ecological impacts. Given that the area with the risk of eutrophication induced by nitrogen deposition remained at 13%of the country even under the scenario of achieving the dual targets of air quality and carbon dioxide mitigation in 2035, we explored an enhanced ammonia abatement pathway. With a further 27% reduction in ammonia by 2035, China could largely eliminate the impacts of acid deposition. This research serves as a valuable reference for China's future acid deposition control and for other nations facing similar challenges.

关键词： acid deposition critical loads acidification eutrophication ammonia abatement

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