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Al-F co-doping towards enhanced electrolyte-electrodes interface properties for halide and sulfide solid electrolytes

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Chinese Chemical Letters 2025年第1期36卷 610-617页

作者： Han Yan Jingming Yao Zhangran Ye Qiaoquan Lin Ziqi Zhang Shulin Li Dawei Song Zhenyu Wang Chuang Yu Long Zhang College of Physics and Energy Fujian Normal UniversityFuzhou 350117China Clean Nano Energy Center State Key Laboratory of Metastable Materials Science and TechnologyYanshan UniversityQinhuangdao 066004China Tianjin Key Laboratory for Photoelectric Materials and Devices School of Materials Science and EngineeringTianjin University of TechnologyTianjin 300384China Guilin Electrical Equipment Scientific Research Institute Co. Ltd.Guilin 541004China State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430000China

All-solid-state Li batteries(ASSLBs)using solid electrolytes(SEs)have gained significant attention in recent years considering the safety issue and their high energy *** these advantages,the commercialization of ASSLBs still faces challenges regarding the electrolyte/electrodes interfaces and growth of Li *** doping is an effective and direct method to enhance the performance of ***,we report an Al-F co-doping strategy to improve the overall properties including ion conductivity,high voltage stability,and cathode and anode ***,the Al-F co-doping enables the formation of a thin Li-Al alloy layer and fluoride interphases,thereby constructing a relatively stable interface and promoting uniform Li *** similar merits of Al-F co-doping are also revealed in the Li-argyrodite *** assembled with these optimized electrolytes gain good electrochemical performance,demonstrating the universality of Al-F co-doping towards advanced SEs.

关键词： Solid electrolytes Li halides Li_(2)ZrCl_(6) Li argyrodites Fluorine doping

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Byzantine-robust distributed support vector machine

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Science China Mathematics 2025年第3期68卷 707-728页

作者： Xiaozhou Wang Weidong Liu Xiaojun Mao School of Statistics East China Normal UniversityShanghai 200062China Key Laboratory of Advanced Theory and Application in Statistics and Data Science(Ministry of Education) East China Normal UniversityShanghai 200062China School of Mathematical Sciences Shanghai Jiao Tong UniversityShanghai 200240China Key Laboratory of Artificial Intelligence(Ministry of Education) Shanghai Jiao Tong UniversityShanghai 200240China Key Laboratory of Scientific and Engineering Computing(Ministry of Education) Shanghai Jiao Tong UniversityShanghai 200240China

The development of information technology brings diversification of data sources and large-scale data sets and calls for the exploration of distributed learning algorithms. In distributed systems, some local machines may behave abnormally and send arbitrary information to the central machine(known as Byzantine failures), which can invalidate the distributed algorithms based on the assumption of faultless systems. This paper studies Byzantine-robust distributed algorithms for support vector machines(SVMs) in the context of binary classification. Despite a vast literature on Byzantine problems, much less is known about the theoretical properties of Byzantine-robust SVMs due to their unique challenges. In this paper, we propose two distributed gradient descent algorithms for SVMs. The median and trimmed mean operations in aggregation can effectively defend against Byzantine failures. Theoretically, we show the convergence of the proposed estimators and provide the statistical error rates. After a certain number of iterations, our estimators achieve near-optimal rates. Simulation studies and real data analysis are conducted to demonstrate the performance of the proposed Byzantine-robust distributed algorithms.

关键词： Byzantine robustness convergence distributed learning support vector machine

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SSP IMEX Runge-Kutta WENO Scheme for Generalized Rosenau-KdV-RLW Equation

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数学研究 2022年第1期55卷 1-21页

作者： Muyassar Ahmat Jianxian Qiu School of Mathematical Sciences and Fujian Provincial Key Laboratory of Mathematical Modeling and High-Performance Scientific Computing Xiamen UniversityXiamen 361005China

In this article,we present a third-order weighted essentially non-oscillatory(WENO)method for generalized Rosenau-KdV-RLW *** third order finite difference WENO reconstruction and central finite differences are applied to discrete advection terms and other terms,respectively,in spatial *** order to achieve the third order accuracy both in space and time,four stage third-order L-stable SSP Implicit-Explicit Runge-Kutta method(Third-order SSP EXRK method and third-order DIRK method)is applied to temporal *** high order accuracy and essentially non-oscillatory property of finite difference WENO reconstruction are shown for solitary wave and shock wave for Rosenau-KdV and Rosenau-KdV-RLW *** efficiency,reliability and excellent SSP property of the numerical scheme are demonstrated by several numerical experiments with large CFL number.

关键词： Rosenau-KdV-RLW equation WENO reconstruction finite difference method SSP implicit-explicit Runge-Kutta method

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A Derivative-free Trust-region Method for Optimization on the Ellipsoid

A Derivative-free Trust-region Method for Optimization on th...

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2023 International Conference on Advances in Computer Science and engineering Technology, ACSE 2023

作者： Xie, Pengcheng State Key Laboratory of Scientific and Engineering Computing Institute of Computational Mathematics and Scientific/Engineering Computing Academy of Mathematics and Systems Science Chinese Academy of Sciences University of Chinese Academy of Sciences ZhongGuanCun East Road No. 55 Beijing China

Optimization methods play a crucial role in various fields and applications. In some optimization problems, the derivative information of the objective function is unavailable. Such black-box optimization problems need to be solved by derivative-free optimization methods. At the same time, optimization problems with ellipsoidal constraints are important and have widespread applications in various fields as well. Following the development of the late professor M. J. D. Powell's efficient derivative-free trust-region optimization methods, this paper considers solving derivative-free optimization problems on the ellipsoid. Our new optimization solver EC-NEWUOA for problems on the ellipsoid in ., n is designed based on Powell's derivative-free software NEWUOA for unconstrained optimization problems. The proposed techniques for our new method mainly include using the Courant penalty function, the augmented Lagrangian method, and the projection technique. Details about the method and theoretical analysis are included in this paper. We also compare our new method with other algorithms by solving test problems and then show the numerical advantages of our new method. © Published under licence by IOP Publishing Ltd.

关键词： Lagrange multipliers

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A High Order Bound Preserving Finite Difference Linear Scheme for Incompressible Flows

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Communications in Computational Physics 2022年第6期32卷 126-155页

作者： Guoliang Zhang Tao Xiong School of Mathematical Sciences Xiamen UniversityXiamenFujian 361005P.R.China School of Mathematical Sciences and Fujian Provincial Key Laboratory of Mathematical Modeling and High-Performance Scientific Computing Xiamen UniversityXiamenFujian 361005P.R.China

We propose a high order finite difference linear scheme combined with ahigh order bound preserving maximum-principle-preserving (MPP) flux limiter tosolve the incompressible flow system. For such problem with highly oscillatory structure but not strong shocks, our approach seems to be less dissipative and much lesscostly than a WENO type scheme, and has high resolution due to a Hermite reconstruction. Spurious numerical oscillations can be controlled by the weak MPP fluxlimiter. Numerical tests are performed for the Vlasov-Poisson system, the 2D guidingcenter model and the incompressible Euler system. The comparison between the linearand WENO type schemes, with and without the MPP flux limiter, will demonstrate thegood performance of our proposed approach.

关键词： Finite difference scheme high order Hermite reconstruction MPP flux limiter incompressible flow Vlasov-Poisson

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High Order Conservative Finite Difference/Fourier Spectral Methods for Inviscid Surface Quasi-Geostrophic Flows

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Communications in Computational Physics 2022年第10期32卷 1474-1509页

作者： Nan Zhang Zhiping Mao Tao Xiong School of Mathematical Sciences Xiamen UniversityXiamenFujian361005P.R.China School of Mathematical Sciences Fujian Provincial Key Laboratory of Mathematical Modeling and High-Performance Scientific ComputingXiamen UniversityXiamenFujian361005P.R.China

In this paper,we develop an effective conservative high order finite difference scheme with a Fourier spectral method for solving the inviscid surface quasigeostrophic equations,which include a spectral fractional Laplacian determining the vorticity for the transport velocity of the potential *** fractional Laplacian is approximated by a Fourier-Galerkin spectral method,while the time evolution of the potential temperature is discretized by a high order conservative finite difference *** essentially non-oscillatory(WENO)reconstructions are also considered for *** to a low regularity of problems involving such a fractional Laplacian,especially in the critical or supercritical regime,directly applying the Fourier spectral method leads to a very oscillatory transport velocity associated with the gradient of the vorticity,*** smooth *** of using an artificial filter,we propose to reconstruct the velocity from the vorticity with central difference *** results are performed to demonstrate the good performance of our proposed approach.

关键词： Finite difference WENO Fourier spectral fractional Laplacian surface quasigeostrophic flow

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Two-step Runge–Kutta methods for Volterra integro-differential equations

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International Journal of Computer Mathematics 2024年第1期101卷 37-55页

作者： Wen, Jiao Huang, Chengming Guan, Hongbo College of Mathematics and Information Science Zhengzhou University of Light Industry Zhengzhou China School of Mathematics and Statistics Huazhong University of Science and Technology Wuhan China Hubei Key Laboratory of Engineering Modeling and Scientific Computing Huazhong University of Science and Technology Wuhan China

In this paper, we investigate two-step Runge–Kutta methods to solve Volterra integro-differential equations. Two-step Runge–Kutta methods increase the order of convergence in comparing the classical Runge–Kutta method without extra computational cost. First, the local order conditions and convergence theorem are derived. Then, stability properties of two-step Runge–Kutta methods corresponding to the basic and convolution test equations are analysed. Furthermore, one-stage method with order four and two-stage method with order six are constructed and we plot the stability regions. Numerical examples are presented to confirm the theoretical analyses. © 2024 Informa UK Limited, trading as Taylor & Francis Group.

关键词： Stability

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Synergy of I-Cl co-occupation on halogen-rich argyrodites and resultant dual-layer interface for advanced all-solid-state Li metal batteries

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Journal of Energy Chemistry 2023年第11期86卷 499-509,I0011页

作者： Han Yan Ruifeng Song Ruonan Xu Shulin Li Qiaoquan Lin Xinlin Yan Zhenyu Wang Chuang Yu Long Zhang Clean Nano Energy Center State Key Laboratory of Metastable Materials Science and TechnologyYanshan UniversityQinhuangdao 066004HebeiChina Fujian Provincial Key Laboratory of Quantum Manipulation and New Energy Materials College of Physics and EnergyFujian Normal UniversityFuzhou 350117FujianChina Institute of Solid State Physics Vienna University of TechnologyWiedner Hauptstr.8–101040 ViennaAustria Guilin Electrical Equipment Scientific Research Institute Co.Ltd. Guilin 541004GuangxiChina State Key Laboratory of Advanced Electromagnetic Engineering and Technology School of Electrical and Electronic EngineeringHuazhong University of Science and TechnologyWuhan 430000HubeiChina

The(electro)chemical stability and Li dendrite suppression capability of sulfide solid electrolytes(SEs)need further improvement for developing all-solid-state Li batteries(ASSLBs).Here,we report advanced halogen-rich argyrodites via I and Cl co-occupation on the crystal ***,a proper I content forms a single phase,whereas an excessive I causes precipitation of two argyrodite phases like a superlattice *** resultant synergistic effect of the optimized composition allows to gain high ionic conductivities at room temperature and-20℃,and enhances the(electro)chemical stability against Li and Li dendrite suppression *** Li|argyrodite interface is very sensitive to the ratio of I and Cl.A LiCl-and LiI-rich double-layer interface is observed from the cell using the SE with optimized composition,whereas too high I content forms only a single interface layer with a mixture of Lil and *** double-layer interface is found to effectively mitigate the Li/SE *** proper designed argyrodite enables ASSLBs to achieve good electrochemical properties at a broad temperature range regardless of the electrode *** co-occupation strategy provides a novel exploration for advanced halogen-rich argyrodite system.

关键词： Sulfide solid electrolytes Argyrodites Dual doping Li metal anode Solid-state batteries

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Conservative Discontinuous Galerkin/Hermite Spectral Method for the Vlasov-Poisson System

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Communications on Applied Mathematics and Computation 2022年第1期4卷 34-59页

作者： Francis Filbet Tao Xiong Institut de Mathématiques de Toulouse UniversitéPaul SabatierToulouse 31062France School of Mathematical Sciences and Fujian Provincial Key Laboratory of Mathematical Modeling and High-Performance Scientific Computing Xiamen UniversityXiamen 361005Fujian ProvinceChina

We propose a class of conservative discontinuous Galerkin methods for the Vlasov-Pois-son system written as a hyperbolic system using Hermite polynomials in the velocity *** schemes are designed to be systematically as accurate as one wants with prov-able conservation of mass and possibly total *** properties in general are hard to achieve within other numerical method frameworks for simulating the Vlasov-Poisson *** proposed scheme employs the discontinuous Galerkin discretization for both the Vlasov and the Poisson equations,resulting in a consistent description of the distribu-tion function and the electric *** simulations are performed to verify the order of the accuracy and conservation properties.

关键词： Energy conserving Discontinuous Galerkin method Hermite spectral method Vlasov-Poisson

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Learning to Reconnect Interrupted Trajectories for Weakly Supervised Multi-Object Tracking 48

Learning to Reconnect Interrupted Trajectories for Weakly Su...

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48th IEEE International Conference on Acoustics, Speech and Signal Processing, ICASSP 2023

作者： Li, Yu-Lei Lu, Yang Li, Jie Wang, Hanzi Xiamen University Fujian Key Laboratory of Sensing and Computing for Smart City School of Informatics China Xidian University Video and Image Processing System Laboratory School of Electronic Engineering China

ISBN: (纸本)9781728163277

Recently, some weakly supervised multi-object tracking (MOT) methods learn identity embedding features with pseudo identity labels rather than the high-cost manual ones. However, these pseudo identity labels may contain many false or missing identities, which adversely affect the optimization of tracking networks, resulting in interrupted trajectories of occluded targets. To effectively reconnect the interrupted trajectories caused by noisy pseudo labels, we propose a novel weakly supervised MOT method based on a Trajectory-Reconnecting Transformer (TRTMOT). TRT-MOT performs feature decoupling to extract discriminative embedding features for reconnecting trajectories of occluded targets. Experimental results show that TRTMOT outperforms previous weakly supervised MOT methods by at least +3.6 and +5.6 on MOTA for the MOT17 and MOT20 datasets, respectively. © 2023 IEEE.

关键词： Feature Decoupling Pseudo Identity Labels Trajectory-Reconnecting Transformer Weakly Supervised Multi-Object Tracking

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