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2008 MRS Fall Meeting

作者： Gosnell, Jonathan D. Weiss, Sharon M. Interdisciplinary Graduate Program in Materials Science Vanderbilt University Station B 350106 Nashville TN 37235 United States Department of Electrical Engineering and Computer Science Vanderbilt University Station B 351824 Nashville TN 37235 United States

ISBN: (纸本)9781615677740

In order for solid state lighting technology to become a mainstream technology, one of the major challenges to overcome is increasing the efficiency of these devices while maintaining a proper color balance. A significant source of efficiency loss in commercial phosphor-based white light-emitting diodes (LEDs) is light scattering off large, micron-sized phosphor particles. The use of recently reported single-size CdSe white-light nanocrystals in place of traditional phosphors, such as YAG:Ce3+, could lead to lower scattering losses and higher device efficiencies as a result of the extremely small CdSe core diameter of approximately 1.5 nm. This work theoretically and experimentally investigates the absorption, scattering, and extinction coefficients and cross sections of CdSe white-light nanocrystals in comparison to YAG:Ce3+ phosphor particles. Calculations were performed based on the Rayleigh approximation and Mie theory of scattering. Experiments were carried out using thin films of encapsulated nanocrystals. By measuring the absorbance and thickness of the films, in addition to the concentration of the nanocrystals, extinction coefficients and cross sections were determined using the Beer-Lambert law. A reasonable agreement was obtained between theoretical and experimental data showing that the size of the particle has a significant impact on the extinction, absorption, and scattering properties of thin films. The considerably reduced scattering from the nanocrystals compared to traditional phosphors, along with their inherent high quality white light emission, makes them a promising candidate for future solid state lighting applications. © 2009 materials Research Society.

关键词： Cadmium compounds

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In situ characterization of Ti-peroxy gel during formation on titanium surfaces in hydrogen peroxide containing solutions

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materials science and engineering C 2006年第8期26卷 1408-1411页

作者： Muyco, Julie J. Gray, Jeremy J. Ratto, Timothy V. Orme, Christine A. McKittrick, Joanna Frangos, John Lawrence Livermore National Laboratory Chemistry and Materials Science 7000 East Ave. L-350 Livermore CA 94550 United States University of California Mechanical and Aerospace Engineering Materials Science and Engineering Graduate Program 9500 Gilman Dr La Jolla CA 92093 United States La Jolla Bioengineering Institute 505 Coast Blvd. S. Ste. #405 La Jolla CA 92037 United States

Three possible functions of Ti-peroxy gel are: reduction of the inflammatory response through the reduction of hydrogen peroxide and other reactive oxygen species;creation of a favorable surface for calcium phosphate nucleation;and as a transitional layer between the compliant surrounding tissue and the stiff titanium. Traditional surface characterization techniques operate in high vacuum environments that alter the actual sample-solution interface. Our studies used techniques that allowed samples to remain in solution and be observed over time. Atomic force microscopy (AFM) force-distance curves, electrochemical impedance spectroscopy (EIS), and Raman spectroscopy were each used in situ to define kinetic and mechanical properties of Ti-peroxy gel as it formed over time on titanium during exposure to hydrogen peroxide. Our studies enabled us to monitor real-time changes in the native oxide layer on titanium in hydrogen peroxide containing solution, including the formation of a Ti-peroxy gel layer above the native oxide. Peaks attributed to Ti-peroxy gel were seen to emerge over the course of several hours using in situ Raman spectroscopy. Force-distance curves suggest a layer that thickens with time on the titanium sample surface. EIS data showed that changes in the surface layers could be monitored in solution over time. © 2005 Elsevier B.V. All rights reserved.

关键词： Gels

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New high efficient red phosphor (Y,M)NbO4: Eu3++(M: Ga3+3+, Al3++) for X-ray and UV excitation

New high efficient red phosphor (Y,M)NbO4: Eu3++(M: Ga3+3+, ...

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2nd International Conference on Computer Research and Development, ICCRD 2010

作者： Nazarov, Mihail Kim, Young Jin Lee, Eun Young Min, Kyoung-In Jeong, Mun Seok Lee, Su Woong Noh, Do Young Department of Materials Science and Engineering Institute of Science and Technology Gwangju Korea Republic of Department of Materials Science and Engineering Kyonggi University Suwon Korea Republic of Advanced Photonics Research Institute 1 Oryong-dong Buk-gu Gwangju Korea Republic of Department of Physics Chonbuk National University Jeonju Korea Republic of Graduate Program of Photon Science and Technology Gwangju Institute of Science and Technology Korea Republic of

ISBN: (纸本)9780769540436

Efficient phosphors based on YNbO4 and doped by Eu3+, Ga3+, Al3+ were synthesized and investigated under UV, and X-ray excitation in luminescence and Raman spectroscopy. Monoclinic fergusonite crystal structure and excellent luminescent properties under X-ray excitation allow recommend these phosphors as good candidates for different applications. © 2010 IEEE.

关键词： Luminescence

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Spin-orbit-locked hyperbolic polariton vortices carrying reconfigurable topological charges

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eLight 2022年第1期2卷 143-153页

作者： Mingsong Wang Guangwei Hu Saroj Chand Michele Cotrufo Yohannes Abate Kenji Watanabe Takashi Taniguchi Gabriele Grosso Cheng‑Wei Qiu Andrea Alù Photonics Initiative Advanced Science Research CenterCity University of New YorkNew York CityNY 10031USA Department of Electrical and Computer Engineering National University of SingaporeSingapore 116083Singapore Department of Physics and Astronomy The University of GeorgiaAthensGA 30602USA Research Center for Functional Materials National Institute for Materials ScienceTsukubaIbaraki 305‑0044Japan International Center for Materials Nanoarchitectonics National Institute for Materials ScienceTsukubaIbaraki 305‑0044Japan Physics Program Graduate CenterCity University of New YorkNew YorkNY 10016USA

The topological features of optical vortices have been opening opportunities for free-space and on-chip photonic technologies,e.g.,for multiplexed optical communications and robust information *** a parallel but disjoint effort,polar anisotropic van der Waals nanomaterials supporting hyperbolic phonon polaritons(HP2s)have been leveraged to drastically boost light-matter *** far HP2 studies have been mainly focusing on the control of their amplitude and scale *** we report the generation and observation of mid-infrared hyperbolic polariton vortices(HP2Vs)associated with reconfigurable topological ***-shaped gold disks coated with a flake of hexagonal boron nitride are exploited to tailor spin-orbit interactions and realise deeply subwavelength *** complex interplay between excitation spin,spiral geometry and HP2 dispersion enables robust reconfigurability of the associated topological *** results reveal unique opportunities to extend the application of HP2s into topological photonics,quantum information processing by integrating these phenomena with single-photon emitters,robust on-chip optical applications,sensing and nanoparticle manipulation.

关键词： Hyperbolic polariton vortex Light-matter interactions Spin-orbit interaction Topological charge Reconfigurability

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Giant long-range dipole-dipole interactions in a plasmonic lattice

Giant long-range dipole-dipole interactions in a plasmonic l...

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Frontiers in Optics + Laser science 2021, FiO+LS 2021 - Part of Frontiers in Optics, FiO 2021

作者： Boddeti, Ashwin K. Guan, Jun Sentz, Tyler Juarez, Xitali Newman, Ward Cortes, Cristian Odom, Teri W. Jacob, Zubin School of Electrical and Computer Engineering Birck Nanotechnology Center Purdue University West LafayetteIN47907 United States Graduate Program in Applied Physics Northwestern University EvanstonIL60208 United States Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Intel Corporation BeavertonOR97007 United States Center for Nanoscale Materials Argonne National Laboratory LemontIL60439 United States Graduate Program in Applied Physics Department of Materials Science and Engineering Department of Chemistry Northwestern University EvanstonIL60208 United States

We observe long-range dipole-dipole interactions in a plasmonic lattice. Fluorescence lifetime measurements show density-dependent non-exponential decay dynamics over 800nm mean nearest-neighbour separation distances ... 详细信息

ISBN: (纸本)9781557528209

关键词： Plasmonics

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Transforming organic chemistry research paradigms:Moving from manual efforts to the intersection of automation and artificial intelligence

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National science Open 2024年第2期3卷 98-127页

作者： Chengchun Liu Yuntian Chen Fanyang Mo School of Materials Science and Engineering Peking UniversityBeijing 100871China Ningbo Institute of Digital Twin Eastern Institute of TechnologyNingbo 315000China AI for Science(AI4S)-Preferred Program Peking University Shenzhen Graduate SchoolShenzhen 518055China

Organic chemistry is undergoing a major paradigm shift,moving from a labor-intensive approach to a new era dominated by automation and artificial intelligence(AI).This transformative shift is being driven by technological advances,the ever-increasing demand for greater research efficiency and accuracy,and the burgeoning growth of interdisciplinary *** models,supported by computational power and algorithms,are drastically reshaping synthetic planning and introducing groundbreaking ways to tackle complex molecular *** addition,autonomous robotic systems are rapidly accelerating the pace of discovery by performing tedious tasks with unprecedented speed and *** article examines the multiple opportunities and challenges presented by this paradigm shift and explores its far-reaching *** provides valuable insights into the future trajectory of organic chemistry research,which is increasingly defined by the synergistic interaction of automation and AI.

关键词： organic chemistry automation platform artificial intelligence algorithms

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An Assessment of Patent Scoring Using Natural Language programming

An Assessment of Patent Scoring Using Natural Language Progr...

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2022 Portland International Conference on Management of engineering and Technology, PICMET 2022

作者： Khongamnuaisak, Lertchai Pentrakoon, Duanghathai Sinthupinyo, Sukree Suanpong, Kwanrat Chulalongkorn University Technopreneurship and Innovation Management Program Graduate School Bangkok Thailand Chulalongkorn University Faculty of Science Department of Materials Science Bangkok Thailand Faculty of Engineering Chulalongkorn University Department of Computer Engineering Bangkok Thailand Chulalongkorn Business School Commerce Department Bangkok Thailand

ISBN: (数字)9781890843410

ISBN: (纸本)9781890843410

Patent has been an increasingly important role in the world because it is not only significant to protect the invention of the company's business but also to generate revenue from the commercialization. WIPO (2018) reports that the repository has many patents so, to assess patent, it consumes time and requires various expertise. Generally, several models have been developed to address this matter, which to assess using a questionnaire tool for portfolios by human. Perhaps, there is not precise because it is assessed base on personal bias or previous experience of expertise. So that, occurs bias any limitation exists that our research will address by artificial intelligence. Thus, this research applies a Natural Language programming to assess for commercial of the patent. Then, the obtained data is used to assigned factors and calculate the model for assessing the commercialization of patent. This finding should deliver an alternative effective patent assessment, which is tool addresses, some current deficiency patent assessment for commercialization. © 2022 PICMET.

关键词： Patents and inventions

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The Effect of air carbon arc gouging on the mechanical and electrochemical properties of AISI 316L submerged arc welds 11

The Effect of air carbon arc gouging on the mechanical and e...

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11th European Stainless Steel Conference science and Market, ESSC 2022 and 7th European Duplex Stainless Steel Conference and Exhibition, DUPLEX 2022

作者： Campesan, Gabriel Roberto de Bribean Guerra, Ana Paula Koga, Guilherme Yuuki Bolfarini, Claudemiro Federal University of São Carlos Department of Materials Science and Engineering Rod. Washington Luis São Carlos SP CEP 13565-905 Brazil Federal University of São Carlos Graduate Program in Materials Science and Engineering Rod. Washington Luis São Carlos SP CEP 13565-905 Brazil

ISBN: (纸本)9788898990269

In the maintenance and manufacturing practices of equipment in the petrochemical industry, the air carbon arc gouging-ACG is used in the preparation of carbon steel joints to be repaired or joined by welding. However, the Standards impose several restrictions to the use of this cost-effective process to stainless steels. The main concern is the pick-up of carbon and sensitization of the steels against corrosion. Therefore, this paper aimed to evaluate the effect of ACG of AISI 316L steel on its electrochemical and mechanical properties. The repaired/welded joints were studied in three different situations, namely: i) any type of cleaning, ii) brushing and iii) machining after gouging. The 20-mm-thick plate was submerged arc welded. Different regions on cross-section of welds were inspected to assess the degree of sensitization by double-loop electrochemical potentiokinetic reactivation (DL-EPR) method, and the risk of intergranular corrosion by oxalic acid etching tests. The electrochemical techniques and mechanical tests (only welded joints) such as tensile, hardness and impact measurements showed no impairing of such properties with the use of ACG, irrespective to the cleaning method used. © ESSC and DUPLEX 2022. All rights reserved.

关键词： Welds

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Pressure, Temperature, and Thickness Dependence of CO2-Induced Devitrification of Polymer Films

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Physical Review Letters 2003年第17期91卷 175503-175503页

作者： Joseph Q. Pham Stephen M. Sirard Keith P. Johnston Peter F. Green Graduate Program in Materials Science and Engineering University of Texas at Austin Austin Texas 78712 USA Department of Chemical Engineering and Texas Materials Institute University of Texas at Austin Austin Texas 78712 USA

The glass transition temperature is known to increase with decreasing film thickness h for sufficiently thin poly(methyl methacrylate) films supported by silicon oxide substrates. We show that this system undergoes a CO2 pressure-induced devitrification transition, Pg, which is film thickness dependent, Pg(h)=ΔPg+Pgbulk. Pgbulk is the bulk glass transition and ΔPg can be positive or negative depending on T and P. The phenomenon of retrograde vitrification, wherein the polymer exhibits a rubbery-to-glassy-to-rubbery transition upon changing temperature isobarically, is also shown to occur in this system and it is film thickness dependent.

关键词： Polymethyl methacrylates

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Accuracy of DFT computed oxygen-vacancy formation energies and high-throughput search of solar thermochemical water-splitting compounds

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Physical Review materials 2023年第6期7卷 065403-065403页

作者： Bianca Baldassarri Jiangang He Xin Qian Emanuela Mastronardo Sean Griesemer Sossina M. Haile Christopher Wolverton Graduate Program in Applied Physics Northwestern University Evanston Illinois USA Department of Materials Science and Engineering Northwestern University Evanston Illinois USA

The enthalpy change involved in metal oxide reduction is a key quantity in various processes related to energy conversion and storage and is of particular interest for computational prediction. Often this prediction involves the simulation of a high-temperature reduction process with a 0-K methodology like density functional theory (DFT), and it is not infrequent for the high temperature and 0-K stable crystal structures to differ. This introduces a conundrum with regard to the choice of crystal structure to utilize in the computation, with approaches in the literature varying and experimental validation remaining scarce. In this work, we address both the crystal structure conundrum and the experimental validation, and then apply the insights we gain to guide a high-throughput search for new materials for solar thermochemical water-splitting applications. By computing the DFT+U oxygen-vacancy formation energy (ΔEvf) of a selection of ABO3 compounds and comparing different crystal structures for each composition, we highlight the issues that arise when the structure utilized in the computation is dynamically unstable at 0 K, namely the presence of an artificial lowering of ΔEvf, and the lack of convergence of ΔEvf with cell size. We solve these limitations by identifying and employing a suitable surrogate dynamically stable structure. We then validate the predictive power of our calculations against appositely generated experimental measurements of reduction enthalpy for a series of Hubbard U values, finding an accuracy ranging between 0.2–0.6 eV/O. In light of such conclusions, we revise and expand a previous a high-throughput DFT study on ABO3 perovskite oxides. We provide a list of candidate STCH materials, highlight trends with redox-active cation and structural distortion, and identify Mn4+, Mn3+, and Co3+ as the most promising redox-active cations.

关键词： Energy applications First-principles calculations Hydrogen energy

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