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44th IEEE Photovoltaic Specialist Conference, PVSC 2017

作者： Chen, Qiong Liu, Henan Kim, Hui-Seon Liu, Yucheng Yang, Mengjin Yue, Naili Ren, Gang Zhu, Kai Liu, Shengzhong Frank Park, Nam-Gyu Zhang, Yong Department of Electrical and Computer Engineering Korea Republic of Optical Science and Engineering Graduate Program University of North Carolina at Charlotte CharlotteNC28223 United States School of Chemical Engineering and Department of Energy Science Sungkyunkwan University Suwon440-746 Korea Republic of Key Laboratory of Applied Surface and Colloid Chemistry National Ministry of EducationInstitute for Advanced Energy Materials School of Materials Science and Engineering Shaanxi Normal University Xi'an710062 China Chemical and Materials Science Center National Renewable Energy Laboratory GoldenCO80401 United States Molecular Foundry Lawrence Berkeley National Laboratory BerkeleyCA94720 United States

ISBN: (纸本)9781509056057

By performing spatially resolved Raman and photoluminescence spectroscopy with different illumination conditions, we have achieved a unified understanding towards the spectroscopy signatures of the organic-inorganic hybrid perovskite, transforming from the pristine state (CH3NH3PbI3 or MAPbI3) to fully degraded state (i.e., PbI2), for samples with varying crystalline domain size from mesoscopic scale to macroscopic size, synthesized by three different techniques. © 2017 IEEE.

关键词： Perovskite

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Resonant plasmon-exciton coupling in zinc oxide quantum well-aluminum nanodisc heterostructure arrays

Resonant plasmon-exciton coupling in zinc oxide quantum well...

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作者： Lawrie, Benjamin Kim, Kyeong-Won Norton, David Mu, Richard Haglund, Richard Interdisciplinary Graduate Program in Materials Science Vanderbilt University Nashville TN 37235 United States Department of Materials Science and Engineering University of Florida Gainesville FL 32611 United States Department of Physics Fisk University Nashville TN 37208 United States Department of Physics and Astronomy Vanderbilt University Nashville TN 37235 United States

The emergence of Fano resonances in the extinction spectra of arrays of aluminum nanodiscs 30-200 nm in diameter deposited on [Zn, Mg]O quantum wells provide the first evidence of strong coupling in zinc oxide heteros... 详细信息

ISBN: (纸本)9781557529107

关键词： Semiconductor quantum wells

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Revisiting the Assessment of Magnetic Texture of Magnets: The Role of Coercivity

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SSRN 2024年

作者： Quispe, Luis T. Antunes, Leonardo F. Baldárrago-Alcántara, Apuniano A. Macedo, Wagner C. Rosa, Marcelo Augusto Rebelo, Querem H.F. Lopes, Leonardo U. Souza, Sérgio Michielon Wendhausen, Paulo Antônio Pereira Magnetic Materials Laboratory MAGMA Federal University of Santa Catarina Florianopolis88040-900 Brazil Graduate Program in Materials Science and Engineering PGMAT Federal University of Santa Catarina Florianopolis88040-900 Brazil Institute of Engineering and Geosciences Federal University of Western Pará Pará Santarém68035-110 Brazil Department of Materials Physics Federal University of Manaus Manaus69077-000 Brazil

A crucial figure of merit of magnets is their magnetic texture, because it is closely related to the maximum remanence a magnet can achieve, hence assessing the magnetic texture is pivotal in terms of magnet’s performance. Fernengel et al. (1996) developed a methodology based on magnetometry, which allows for a quick determination of the texture by calculating the degree of alignment 〈cosθ〉 from the remanent magnetization in directions parallel and perpendicular to the texture axis of the magnet. Although this method provided reliable values, its application was limited to magnets with high degrees of alignment (〈cosθ〉 > 95%), a restriction that was corrected by Quispe et al. (2020). Nevertheless, recent experiments have indicated that the magnetometry technique can introduce errors in texture assessment when the magnet presents high levels of coercivity. This work presents an approach that incorporates a correction factor into the magnetometry technique, accounting for the effect of the coercivity and circumventing this error source in texture assessment. The proposed methodology has been successfully applied to magnets with varying levels of coercivity. © 2024, The Authors. All rights reserved.

关键词： Coercive force

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Heteromorphic Hematite Pigments Obtained from Steel Scrap and Encapsulated in Amorphous Silica for Porcelainized Stoneware

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材料科学与工程（中英文版） 2010年第5期4卷 1-13页

作者： Viviana Possamai Della Janaina Accordi Junkes Antonio Pedro Novaes de Oliveira Dachamir Hotza Federal Institute of Espirito Santo-IFES Graduate Program on Metallurgical and Materials Engineering-PROPEMM Vitoria29040-780 ES Brazil Federal University of Santa Catarina-UFSC Gradttate Program on Materials Science and Engineering-PGMA T Florian6polis88040-900 SC Brazil

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Molecular recognition by stable dispersion of gold nanoparticles modified with heterobifunctional poly (ethylene glycol)

Molecular recognition by stable dispersion of gold nanoparti...

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Transactions - 7th World Biomaterials Congress

作者： Aboshi, F. Takahashi, T. Ishii, T. Nagasaki, Y. Otsuka, Hidenori Kataoka, K. Pre-venture Program JST 4-1-8 Hon-machi Kawaguchi Saitama 332-0012 Japan Department of Materials Science Tokyo University of Science 2641 Yamazaki Noda Chiba 278-8510 Japan Department of Matereals Science Graduate School of Engineering University of Tokyo 7-3-1 Hongo Bunkyo-ku Tokyo 113-8656 Japan

ISBN: (纸本)1877040193

The stability of gold nanoparticles modified with heterobifunctional poly (ethylene glycol) (PEG) were investigated. An effective method for preparing hetero-bifunctional PEG by anionic ring-opening polymerization was also developed. Streptavidin-PEG gold nanoparticle showed extremely high response with biotinylated surface plasmon resonance (SPR) sensors. PEG-modified gold nanoparticles showed remarkable stability in physiological conditions, such as the solution of high ionic strength.

关键词： Nanostructured materials

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PH dependence of polypseudorotaxane formation between cationic linear polyethylenimine and cyclodextrins

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Macromolecules 2004年第18期37卷 6705-6710页

作者： Choi, Hak Soo Ooya, Tooru Lee, Sang Cheon Sasaki, Shintaro Kurisawa, Motoichi Uyama, Hiroshi Yui, Nobuhiko School of Materials Science Japan Adv. Inst. Sci. and Technol. 1-1 Asahidai Tatsunokuchi Ishikawa 923-1292 Japan Inst. of Bioeng. and Nanotechnology Singapore Science Park II #01-01/10 The Aries 117586 Singapore Department of Materials Chemistry Graduate School of Engineering Osaka University Suita Osaka 565-0871 Japan 21st Century COE Program Japan Adv. Inst. Sci. and Technol. 1-1 Asahidai Tatsunokuchi Ishikawa 923-1292 Japan

A series of linear polyethylenimines (LPEIs) with various molecular weights were synthesized and used for pH-dependent polypseudorotaxane formation with α- or γ-cyclodextrins (α-, γ-CDs). The polypseudorotaxane formation was significantly dependent on the pH of the aqueous media. The maximum yield of the recovered polypseudorotaxane precipitates was observed at pH 11.0, whereas no complexation was observed in the pH range below 8.0 due to the protonation of secondary amine groups in LPEI backbones. This suggests that the ionization of the secondary amine groups leads to dethreading of CD molecules because PEI chains with cationic nature disfavor the hydrophobic cavities of CDs. The solid-state 13C CP/MAS NMR and X-ray diffraction measurements verified the successful formation of crystalline polypseudorotaxanes through the inclusion complexation. In addition, 1H NMR analysis showed that LPEI formed a 2:1 inclusion complex with α-CD ([EI]:[α-CD] = 2:1) and a 4:1 complex with γ-CD ([EI]:[γ-CD] = 4:1) as reported in the poly(ethylene glycol)-based polypseudorotaxane system. Such unique pH-controllable polypseudorotaxane formation may be useful in designing many building blocks for stimuli-responsive polyrotaxanes.

关键词： Polyethylenes

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Ultrahigh zT from strong electron-phonon interactions and a low-dimensional Fermi surface

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Energy and Environmental science 2024年第5期17卷 1904-1915页

作者： Ranganayakulu, V.K. Wang, Te-Hsien Chen, Cheng-Lung Huang, Angus Ma, Ma-Hsuan Wu, Chun-Min Tsai, Wei-Han Hung, Tsu-Lien Ou, Min-Nan Jeng, Horng-Tay Lee, Chih-Hao Chen, Kuei-Hsien Li, Wen-Hsien Brod, Madison K. Snyder, G. Jeffrey Chen, Yang-Yuan Institute of Physics Academia Sinica Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu30013 Taiwan Taiwan International Graduate Program Taipei11529 Taiwan Department of Physics National Chung Hsing University Taichung City40227 Taiwan Graduate School of Materials Science National Yunlin University of Science and Technology Yunlin64002 Taiwan Bachelor Program in Semiconductor Materials and Fabrication Ming Chi University of Technology New Taipei City243303 Taiwan Department of Physics National Tsing Hua University Hsinchu30013 Taiwan Center for Theory and Computation National Tsing Hua University Hsinchu30013 Taiwan Physics Division National Center for Theoretical Sciences Taipei10617 Taiwan Department of Physics National Central University Jhongli32001 Taiwan National Synchrotron Radiation Research Center Hsinchu Science Park Hsinchu30076 Taiwan Institute of Atomic and Molecular Sciences Academia Sinica Taipei10617 Taiwan Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Graduate Institute of Applied Physics National Chengchi University Taipei11605 Taiwan

The outstanding thermoelectric performance of GeTe has attracted significant attention in the research community in recent years. However, many of the underlying physical mechanisms that contribute to GeTe's exceptionally high figure of merit (zT) remain not fully understood. In this study, an Sb-Bi codoped GeTe single crystal (Ge0.86Sb0.08Bi0.06)Te with an ultrahigh zT of 2.7 at 700 K and a record high device zT of 1.41 in the temperature range of 300-773 K was synthesized and investigated. The ultrahigh zT is attributed to the extremely low lattice thermal conductivity induced by strong electron-phonon (EP) interactions as revealed by the experimentally observed Kohn anomaly, through inelastic neutron scattering (INS) measurements. First-principles calculations further demonstrate that the remarkable EP interaction arises from the Fermi surface nesting featured in a one-dimensional (double-walled) topology. Our finding unravels the ultrahigh-zT mechanism in GeTe-based materials, serving as an inspiring guide toward high thermoelectric performance. © 2024 The Royal Society of Chemistry.

关键词： Neutron scattering

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Photoluminescence of oxygen vacancy-rich nano-TiO 2 photocatalyst for methylene blue color degradation

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materials science and engineering: B 2025年 320卷

作者： Mayer Simanjuntak I Made Joni Ferry Faizal Noto Susanto Gultom Dong-Hau Kuo Camellia Panatarani Department of Physics Faculty of Mathematic and Natural Sciences Universitas Padjadjaran Jl. Raya Bandung-Sumedang KM 21 Jatinangor Sumedang 45363 Indonesia Study Program of Biotechnology Faculty of Graduate School Universitas Padjadjaran Jl. Dipati Ukur No.35 Coblong Bandung 40132 Indonesia Functional Nano Powder University Center of Excellence Universitas Padjadjaran Jl. Raya Bandung-Sumedang KM 21 Jatinangor Sumedang 45363 Indonesia Department of Materials Science and Engineering National Taiwan University of Science and Technology No.43 Sec. 4 Keelung Road Taipei 10607 Taiwan

Wastewater containing synthetic dyes poses a critical environmental hazard, necessitating the development of effective treatment techniques. Despite its promise as a photocatalyst, TiO 2 ′s inability to efficiently absorb visible light limits its practical use. To overcome this limitation, oxygen vacancy (OV) engineering was carried out in TiO 2 through solvothermal at temperatures of 150°C, 180°C, and 210°C. Comprehensive analyses confirmed a temperature-induced increase in crystallinity and OV concentration. Furthermore, photoluminescence analysis revealed mid-gap states that improve visible light absorption. Notably, the T150 sample achieved 93.43% degradation of methylene blue within 3 h under sunlight, outperforming commercial TiO 2 . The superior performance was attributed to a reduced bandgap energy, enhanced charge carrier separation, and increased generation of reactive oxygen species, all facilitated by an optimal concentration of OV. This study clarifies the interaction between photoluminescence and photocatalytic activity, highlighting OV engineering as a highly effective strategy for developing advanced TiO 2 -based materials for wastewater treatment.

关键词： Photocatalytic activity

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Magnetoelastic coupling driven magnon gap in a honeycomb antiferromagnet

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Physical Review B 2024年第10期110卷 104419页

作者： Jeongheon Choe Andrey Baydin Gaihua Ye Bowen Ma Cynthia Nnokwe Martin Rodriguez-Vega David Lujan Swati Chaudhary Fuyang Tay Jiaming He Hiroyuki Nojiri Jianshi Zhou Gregory A. Fiete Junichiro Kono Rui He Xiaoqin Li Department of Physics Center of Complex Quantum Systems Center for Dynamics and Control of Materials Department of Electrical and Computer Engineering Smalley–Curl Institute Department of Physics Applied Physics Graduate Program Smalley–Curl Institute Department of Mechanical Engineering Institute for Materials Research Department of Physics and Astronomy Department of Materials Science and NanoEngineering

Cobalt titanate, CoTiO3, is a honeycomb antiferromagnet recently confirmed experimentally to host Dirac magnons, topological spin-orbit excitons, and chiral phonons. Here, we investigate a magnon gap at the zone center which calls for a refined spin Hamiltonian. We propose a microscopic model for the magnon gap and attribute it to a lattice-distortion (phonon)-induced higher-order spin interaction. Strong magnetoelastic coupling in CoTiO3 is also evident in Raman spectra, in which the magnetic order exerts a stronger influence on phonons corresponding to in-plane ionic motions than those with out-of-plane motions. We further examine the evolution of the zone-center magnons in a high magnetic field up to 18.5 T via THz absorption spectroscopy measurements. Based on this field dependence, we propose a spin Hamiltonian that not only agrees with magnon dispersion measured by inelastic neutron scattering but also includes fewer exchange constants and a realistic anisotropy term. Our work highlights the broad implications of magnetoelastic coupling in the study of topologically protected bosonic excitations.

关键词： Magnetism Magnons Topological materials Raman spectroscopy Terahertz spectroscopy

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Temperature Dependent Fluorescence of Nanocrystalline Ce-doped Garnets For Use as Thermographic Phosphors

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MRS Online Proceedings Library 2008年第1期1076卷 1-6页

作者： Hansel, Rachael Allison, Steve Walker, Greg Interdisciplinary Graduate Program in Materials Science Vanderbilt University Nashville USA Oak Ridge National Laboratory Oak Ridge USA Department of Mechanical Engineering Vanderbilt University Nashville USA

Four samples of (Y1−xCex)3(Al1−y Gay)5O12 (where x=0.01, 0.02 and y=0, 0.5) were synthesized via the simple, efficient combustion synthesis method in order to determine the effect of substituting Ga3+ for Al3+ on the temperature-dependent fluorescent lifetime. X-ray diffraction shows that the Ga-doped samples have longer lattice constants and transmission electron microscopy data show that each sample consists of nanocrystallites which have agglomerated in micron-sized particles. Photoluminescence data reveal that the addition of gallium into the YAG:Ce matrix induces a red shift in the absorption spectra and a blue-shift in the emission spectra. The laser-induced fluorescent lifetime was determined as a function of temperature over the range of 0-125°C using two different emission filters. Increasing the amount of dopant ultimately results in a decrease of the fluorescent lifetime. The quenching temperatures for the Ga-doped samples were lower than the samples without gallium. The results of this work show that combustion synthesis is viable method for making highly luminescent, nanocrystalline TGPs. In addition, these results show that the quenching temperature of YAG:Ce can be altered by substituting ions which alter the location of the charge transfer state and by changing the morphology of the sample.

关键词： crystalline sensor dopant

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