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arXiv 2024年

作者： Cho, Minhyun Datta, Biswajit Han, Kwanghee Chand, Saroj B. Adak, Pratap Chandra Yu, Sichao Li, Fengping Watanabe, Kenji Taniguchi, Takashi Hone, James Jung, Jeil Grosso, Gabriele Kim, Young Duck Menon, Vinod M. Department of Physics Kyung Hee University 26 Kyungheedae-ro Seoul02447 Korea Republic of Department of Physics City College of New York New YorkNY10031 United States Photonics Initiative Advanced Science Research Center City University of New York New YorkNY10031 United States Department of Physics Department of Smart Cities University of Seoul Seoul02504 Korea Republic of Research Center for Electronic and Optical Materials National Institute for Materials Science 1-1 Namiki Tsukuba305-0044 Japan Research Center for Materials Nanoarchitectonics National Institute for Materials Science 1-1 Namiki Tsukuba305-0044 Japan Department of Mechanical Engineering Columbia University New YorkNY10027 United States Physics Program Graduate Center City University of New York New YorkNY10016 United States Department of Information Display Kyung Hee University Seoul02447 Korea Republic of

Twisted hexagonal boron nitride (thBN) exhibits emergent ferroelectricity due to the formation of moiré superlattices with alternating AB and BA domains. These domains possess electric dipoles, leading to a periodic electrostatic potential that can be imprinted onto other 2D materials placed in its proximity. Here we demonstrate the remote imprinting of moiré patterns from twisted hexagonal boron nitride (thBN) onto monolayer MoSe2 and investigate the resulting changes in the exciton properties. We confirm the imprinting of moiré patterns on monolayer MoSe2 via proximity using Kelvin probe force microscopy (KPFM) and hyperspectral photoluminescence (PL) mapping. By developing a technique to create large ferroelectric domain sizes ranging from 1 µm to 8.7 µm, we achieve unprecedented potential modulation of ∼ 387±52 meV. We observe the formation of exciton polarons due to charge redistribution caused by the antiferroelectric moiré domains and investigate the optical property changes induced by the moiré pattern in monolayer MoSe2 by varying the moiré pattern size down to ∼110 nm. Our findings highlight the potential of twisted hBN as a platform for controlling the optical and electronic properties of 2D materials for optoelectronic and valleytronic applications. © 2024, CC BY-NC-ND.

关键词： Boron nitride

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Solution-Processed and Room-Temperature Spin Light-Emitting Diode Based on Quantum Dots/Chiral Metal-Organic Framework Heterostructure

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Advanced Functional materials 2023年第19期33卷

作者： Mustaqeem, Mujahid Chou, Pi-Tai Kamal, Saqib Ahmad, Naveed Lin, Jia-Yu Lu, Yu-Jung Lee, Xing-Hao Lin, Kung-Hsuan Lu, Kuang-Lieh Chen, Yang-Fang Nano-Science and Technology Program Taiwan International Graduate Program Institute of Physics Academia Sinica Taipei106 Taiwan Department of Physics National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Taiwan Department of Chemistry National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Taiwan Institute of Chemistry Academia Sinica Taipei115 Taiwan Department of Materials Science and Engineering National Taiwan University of Science and Technology Taipei10607 Taiwan Research Center for Applied Sciences Academia Sinica Taipei115024 Taiwan Institute of Physics Academia Sinica Taipei11529 Taiwan

Spin optoelectronics is an indispensable key for the future development of spintronics. In conventional spin light emitting diodes (LEDs), spin-polarized carrier pairs are injected electrically into the light emitting layer and create circularly polarized light (CPL). Generally, spin-polarized carriers are accomplished using ferromagnetic contacts or applying an external magnetic field, which will produce several drawbacks, including low temperature operation, low spin-polarized carriers injection efficiency, etc. To circumvent the existing shortcomings, here, an alternative approach is proposed and achieves spin-polarized LEDs at room temperature based on quantum dots (QDs)/chiral metal-organic framework heterojunction without using ferromagnetic contacts or magnetic fields. The spin-polarized injected layer composed of self-assembled monolayer (SAM)/Chiral-MOF ([Sr(9,10-adc)(DMAc)2]n)) film, which produces spin-polarized holes with spin orientation, determining the polarization and strength of circularly polarized electroluminescence (CP-EL). The spin-QLED emits CP-EL at a rate of 12.24% efficiency, which provides an excellent alternative to generate new functionality for conventional QLEDs. The approach is anticipated to be very useful, enabling to offer a general methodology for generating not yet realized spin optoelectronic devices. © 2023 Wiley-VCH GmbH.

关键词： Room temperature

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Inside Back Cover: Reversible Handedness Inversion and Circularly Polarized Light Reflection Tuning in Self-Organized Helical Superstructures Using Visible-Light-Driven Macrocyclic Chiral Switches (Angew. Chem. Int. Ed. 8/2023)

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Angewandte Chemie International Edition 2023年第8期62卷

作者： Dr. Hao Wang Yuqi Tang Dr. Hari Krishna Bisoyi Prof. Quan Li Advanced Materials and Liquid Crystal Institute and Materials Science Graduate Program Kent State University Kent OH 44242 USA Institute of Advanced Materials and School of Chemistry and Chemical Engineering Southeast University Nanjing 211189 China

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Multi-Level Hierarchical Nanoporous Structure by Additive Manufacturing and Dealloying

SSRN

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SSRN 2023年

作者： Kvaratskheliya, Askar Bianchini, Bruno Filimonov, Aleksandr Gomes, Leonardo Fernandes Macedo dos Santos, Rafael Formenton Gargarella, Piter Mädler, Lutz Okulov, Ilya Faculty ofProduction Engineering University ofBremen Badgasteiner Straße 2 28359Bremen Germany Leibniz Institute for Materials Engineering IWT Badgasteiner Straße 3 28359Bremen Germany Graduate Program in Materials Science andEngineering FederalUniversity ofSão Carlos Rod. Washington Luis km 235 SP São Carlos13565-905 Brazil Rod. Washington Luis Km 235 SP São Carlos13565-905 Brazil Rod. Washington Luis Km 235 SP São Carlos13565-905 Brazil MAPEX- Center for Materials andProcesses University ofBremen Bremen28359 Germany

Hierarchical nanoporous materials feature a unique set of physical, mechanical, and chemical properties which make them promising in various technological applications. This paper presents a novel approach to synthesise bulk (centimetre size) hierarchical Cu structures featuring three levels of porosity: (i) design of lattice structures for the mm-scale porosity by additive manufacturing;(ii) design of phase composition for the µm-scale porosity;(iii) and chemical dealloying for the nm-scale porosity. During the first step, a lattice structure composed of the Cu50Al50 wt. % precursor material was manufactured by laser powder bed fusion. The precursor consists of Cu2Al and Al phases. Second, the Al phase was etched from the Cu50Al50 precursor by corrosion in the NaOH solution. Third, the nanoporous Cu was formed by dealloying of the Cu2Al phase in the NaOH solution. The current approach paves the way for advancing the functionality of nanoporous materials via their multi-level hierarchical organization. © 2023, The Authors. All rights reserved.

关键词： Additives

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Innenrücktitelbild: Reversible Handedness Inversion and Circularly Polarized Light Reflection Tuning in Self-Organized Helical Superstructures Using Visible-Light-Driven Macrocyclic Chiral Switches (Angew. Chem. 8/2023)

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Angewandte Chemie 2023年第8期135卷

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Maximum A-Posteriori Probability (MAP) Terahertz Parameter Extraction for Pancreatic Ductal Adenocarcinoma

Maximum A-Posteriori Probability (MAP) Terahertz Parameter E...

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International Conference on Infrared and Millimeter Waves

作者： Debamitra Chakraborty Bradley N. Mills Jing Cheng Scott A. Gerber Roman Sobolewski Materials Science Graduate Program University of Rochester Rochester New York USA Laboratory for Laser Energetics University of Rochester Rochester New York USA Department of Surgery University of Rochester Medical Center Rochester New York USA Department of Electrical and Computer Engineering University of Rochester Rochester New York USA

ISBN: (数字)9781728194271

ISBN: (纸本)9781728194288

We developed a maximum a-posteriori probability-based terahertz parameter extraction method to obtain tissue characteristics of paraffin-embedded murine pancreatic ductal adenocarcinoma samples. This estimation algorithm can produce conservative estimates of tissue parameters without resorting to frequency-domain analysis. We report well-resolved and statistically significant differences in tumor tissue regions as compared to their healthy counterparts using our parameters extraction algorithm. We propose to use the index of refraction and the absorption as imaging biomarker parameters for biological tissue characterization.

关键词： Maximum a posteriori estimation Absorption Frequency-domain analysis Biological tissues Refractive index Estimation Probability

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Emulating Complex Synapses Using Interlinked Proton Conductors

arXiv

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arXiv 2024年

作者： Zhang, Lifu Li, Ji-An Hu, Yang Jiang, Jie Lai, Rongjie Benna, Marcus K. Shi, Jian Department of Materials Science and Engineering Rensselaer Polytechnic Institute TroyNY12180 United States Neurosciences Graduate Program University of California San Diego La Jolla CA92093 United States Department of Mathematics Purdue University West LafayetteIN47907 United States Department of Neurobiology School of Biological Sciences University of California at San Diego La Jolla CA92093 United States Department of Physics Applied Physics and Astronomy Rensselaer Polytechnic Institute TroyNY12180 United States

In terms of energy efficiency and computational speed, neuromorphic electronics based on non-volatile memory devices is expected to be one of most promising hardware candidates for future artificial intelligence (AI). However, catastrophic forgetting, networks rapidly overwriting previously learned weights when learning new tasks, remains as a pivotal hurdle in either digital or analog AI chips for unleashing the true power of brain-like computing. To address catastrophic forgetting in the context of online memory storage, a complex synapse model (the Benna-Fusi model) has been proposed recently[1], whose synaptic weight and internal variables evolve following a diffusion dynamics. In this work, by designing a proton transistor with a series of charge-diffusion-controlled storage components, we have experimentally realized the Benna-Fusi artificial complex synapse. The memory consolidation from coupled storage components is revealed by both numerical simulations and experimental observations. Different memory timescales for the complex synapse are engineered by the diffusion length of charge carriers, the capacity and number of coupled storage components. The advantage of the demonstrated complex synapse in both memory capacity and memory consolidation is revealed by neural network simulations of face familiarity detection. Our experimental realization of the complex synapse suggests a promising approach to enhance memory capacity and to enable continual learning. Copyright © 2024, The Authors. All rights reserved.

关键词： Computational efficiency

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Outcoupling Hyperbolic Modes from Aligned Carbon Nanotube Films

Outcoupling Hyperbolic Modes from Aligned Carbon Nanotube Fi...

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CLEO: QELS_Fundamental science, QELS 2022

作者： Jerome, Bryant Prasad, Ciril S. Doumani, Jacques Dewey, Oliver S. Baydin, Andrey Pasquali, Matteo Kono, Junichiro Gao, Weilu Alabastri, Alessandro Naik, Gururaj V. Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Chemistry Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering University of Utah Salt Lake CityUT84112 United States

Aligned carbon nanotube films make an excellent hyperbolic material platform in the infrared. Here, we experimentally demonstrate the presence of high-k modes in aligned carbon nanotube films and outcouple them to fre... 详细信息

ISBN: (纸本)9781557528209

关键词： Carbon films

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Stokesian Dynamics with odd viscosity

arXiv

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arXiv 2022年

作者： Yuan, Hang de la Cruz, Monica Olvera Applied Physics Graduate Program Northwestern University EvanstonIL60208 United States Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Department of Chemistry Northwestern University EvanstonIL60208 United States Department of Physics and Astronomy Northwestern University EvanstonIL60208 United States

Stokesian Dynamics is a well-established computational method for simulating dynamics of many particles suspended in a conventional passive fluid medium. Active fluids composed of self-propelling particles with broken time reversal symmetry permit the emergence of a so-called odd viscosity. In this work, we extended the conventional Stokesian Dynamics formalism to incorporate the additional hydrodynamic effects due to odd viscosity, which enables simulating collective behaviors of many particles suspended in an active fluid medium with both even viscosity and odd viscosity. © 2022, CC BY.

关键词： Viscosity

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Effect of Temperature and Mischmetal Addition on the Microstructure, Mechanical Andcorrosion Behavior of Crn Hard Coatings Deposited Onto Zk60 Magnesium Alloys Using Hipims

SSRN

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SSRN 2023年

作者： Pereira da Silva, Erenilton Oliveira Junior, William Tavares Avila, Pedro Renato Lima Ribeiro, Josy Kelly Alves dos Santos, Marcos Junio Cortez Maciel, Natalia Mendes Rodrigues, Alisson Pinto, Haroldo Cavalcanti MG Janaúba39447-790 Brazil Department of Engineering Physics Polytechnique Montréal P.O. Box 6079 Station Centre-Ville MontréalQCH3C 3A7 Canada Graduate Program in Materials Science UnB Planaltina Faculty University of Brasilia DF Brasilia70904-910 Brazil SP São Carlos13566-590 Brazil

Magnesium alloys have recently gained popularity due to their low density and suitability for various applications requiring both lightweight and robust mechanical qualities. Nevertheless, their widespread utilization could be improved by their inadequate corrosion resistance. This study examines the deposition of ceramic films using chromium nitride (CrN) via High Power Impulse Magnetron Sputtering (HiPIMS) on ZK60 and ZK60 + 1.5 Mischmetal (MM) at 200°C and 300°C. The morphology and thickness of the CrN films was evaluated by Field Emission Gun-Scanning Electron Microscopy (FEG-SEM) and X-ray Diffraction (XRD), roughness by atomic force microscopy (AFM), and mechanical properties (hardness and elastic modulus) were measured by nanoindentation experiments. Furthermore, the electrochemical impedance spectroscopy (EIS) analysis was used to evaluate the corrosion resistance. Fractured cross-section SEM-FEG images of CrN coatings deposited at 200°C and 300°C revealed differences in thickness and morphology for all samples. ZK60 samples exhibited thicker coatings compared to ZK60+1.5MM, which can be attributed to the stability of intermetallic phases. Increasing temperature resulted in the formation of thinner coatings. Also, at 300°C samples presented different thickness. Surface roughness decreases with temperature, reflecting the formation of refined columnar structures. Hardness and elastic modulus increased with temperature, also presenting different behaviors at 300°C. Corrosion resistance also presented improvement at higher temperatures, with ZK60 outperforming ZK60+1.5MM, as EIS analysis confirmed the denser films enhance corrosion protection, while porous coatings exhibit lower resistance, as was observed for ZK60+1.5MM at 300°C. Results also showed the impact of the thermic stability of the samples on the coating formation, indicating that substrate temperature rises during deposition, leading to possible phase changes in the substrate and, consequently, affe

关键词： Corrosion resistance

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