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Macroscopically Self-Aligned and Chiralized Carbon Nanotubes: From Filtration to Innovation

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arXiv 2023年

作者： Doumani, Jacques Zahn, Keshav Yu, Shengjie Barrios, Gustavo Rodriguez Sasmal, Somesh Kikuchi, Rikuta Kritzell, T. Elijah Xu, Hongjing Baydin, Andrey Kono, Junichiro Department of Electrical and Computer Engineering Rice University 6100 Main Street HoustonTX77005 United States Applied Physics Graduate Program Smalley–Curl Institute Rice University 6100 Main Street HoustonTX77005 United States Carbon Hub Rice University 6100 Main Street HoustonTX77005 United States Smalley–Curl Institute Rice University 6100 Main Street HoustonTX77005 United States Department of Physics and Astronomy Rice University 6100 Main Street HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University 6100 Main Street HoustonTX77005 United States

Because of their natural one-dimensional (1D) structure combined with intricate chiral variations, carbon nanotubes (CNTs) exhibit various exceptional physical properties, such as ultrahigh electrical and thermal conductivity, exceptional mechanical strength, and chirality-dependent metallicity. These properties make CNTs highly promising for diverse applications, including field-effect transistors, sensors, photodetectors, and thermoelectric devices. While CNTs excel individually at the nanoscale, their 1D and chiral nature can be lost on a macroscopic scale when they are randomly assembled. Therefore, the alignment and organization of CNTs in macroscopic structures is crucial for harnessing their full potential. In this review, we explore recent advancements in understanding CNT alignment mechanisms, improving CNT aligning methods, and demonstrating macroscopically 1D properties of ordered CNT assemblies. We also focus on a newly discovered class of CNT architectures, combining CNT alignment and twisting mechanisms to create artificial radial and chiral CNT films at wafer scales. Finally, we summarize recent developments related to aligned and chiral CNT films in optoelectronics, highlighting their unique roles in solar cells, thermal emitters, and optical modulators. Copyright © 2023, The Authors. All rights reserved.

关键词： Carbon nanotubes

Effects of spatial uniformity of continuous and pulse laser irradiation on the microstructure and mechanical properties of Ti-6Al-4V in powder bed fusion

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materials Today Communications 2025年 46卷

作者： Seunghwan Moon Seungmuk Ji Yoonseok Ko Min-Su Lee Tea-Sung Jun Dong-Ik Kim Jong-Souk Yeo School of Integrated Technology College of Computing Yonsei University Seoul 03722 Republic of Korea BK21 Graduate Program in Intelligent Semiconductor Technology Yonsei University Seoul 03722 Republic of Korea Center for Energy Materials Research Korea Institute of Science and Technology Seoul 02792 Republic of Korea Department of Mechanical Engineering Incheon National University Incheon 22012 Republic of Korea

Powder bed fusion of metals with laser beam (PBF-LB/M) using Ti-6Al-4V (Ti64) has enabled delicate fabrication of biocompatible medical implants. This research focuses on how the spatial uniformity of laser irradiation affects material under continuous wave (CW) and pulse width modulated (PWM) laser conditions, using a self-developed PBF-LB/M system. The volumetric energy density (VED) was used as a reference parameter in order to accurately compare the effects of CW and PWM lasers, but limitations of VED, which does not include spatial and kinetic factors, which are reinforced in the PWM laser process, were also considered. Results revealed that the uniform distribution of energy irradiation across the entire region brought similar porosities and Vickers hardness tendencies for CW and PWM laser processes. In contrast, the spatially nonuniform energy transfer resulted in a significantly higher porosity in the specimen fabricated using the PWM laser than that produced using the CW laser at the same VED, reducing compressive yield strength. The electron backscattered diffraction analysis showed no significant differences in the average grain size, phase distribution, and misorientation angle of the samples produced using CW and PWM lasers under the same VED. However, sharper grains with an aspect ratio of less than 0.3 were 7 % higher in specimens produced using the PWM laser. This study highlights the possibility of controlling the microstructure and mechanical properties in a wider range when using the PWM laser with spatially nonuniform irradiation.

关键词： Vickers hardness

Regulating COOH Intermediate via Rationally Constructed Surface-Active Sites of Bi2WO6for Solar-Driven CO2-to-CO Production (Adv. Funct. Mater. 23/2025)

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Advanced Functional materials 2025年第23期35卷

作者： Nguyen Quoc Thang Amr Sabbah Raghunath Putikam Chih-Yang Huang Tsai-Yu Lin Mahmoud Kamal Hussien Heng-Liang Wu Ming-Chang Lin Chih-Hao Lee Kuei-Hsien Chen Li-Chyong Chen Institute of Atomic and Molecular Sciences Academia Sinica Taipei 10617 Taiwan Center for Condensed Matter Sciences National Taiwan University Taipei 10617 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei 11529 Taiwan Institute of Physics Academia Sinica Taipei 15201 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu 30013 Taiwan Center of Atomic Initiative for New Materials National Taiwan University Taipei 10617 Taiwan Tabbin Institute for Metallurgical Studies Tabbin Helwan 109 Cairo 11421 Egypt Department of Applied Chemistry National Yang-Ming Chiao Tung University Hsinchu 30010 Taiwan International Graduate Program of Molecular Science and Technology National Taiwan University (NTU-MST) Taipei 10617 Taiwan Molecular Science and Technology Program Taiwan International Graduate Program (TIGP) Academia Sincia Taipei 11529 Taiwan Department of Chemistry Faculty of Science Assiut University Assiut 71516 Egypt Department of Chemistry National Taiwan University Taipei 10617 Taiwan Department of Physics National Taiwan University Taipei 10617 Taiwan

Terahertz Cavity Phonon Polaritons in Lead Telluride in the Deep-Strong Coupling Regime

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arXiv 2025年

作者： Baydin, Andrey Manjappa, Manukumara Mishra, Sobhan Subhra Xu, Hongjing Doumani, Jacques Tay, Fuyang Kim, Dasom Rappl, Paulo H.O. Abramof, Eduardo Singh, Ranjan Hernandez, Felix G.G. Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley–Curl Institute Rice University HoustonTX77005 United States Rice Advanced Materials Institute Rice University HoustonTX77005 United States Instrumentation and Applied Physics Department Indian Institute of Science Bangalore560012 India Center for Disruptive Photonic Technologies The Photonics Institute Nanyang Technological University 639798 Singapore Department of Physics and Astronomy Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley–Curl Institute Rice University HoustonTX77005 United States Group of Research and Development in Materials and Plasma National Institute for Space Research São José dos Campos São Paulo12201-970 Brazil Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Instituto de Física Universidade de São Paulo São Paulo05508-090 Brazil Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

Lead telluride is an important thermoelectric material due to its large Seebeck coefficient combined with its unusually low thermal conductivity that is related to the strong anharmonicity of phonons in this material. Here, we have studied the resonant and nonperturbative coupling of transverse optical phonons in lead telluride with cavity photons inside small-mode-volume metallic metasurface cavities that have photonic modes with terahertz frequencies. We observed a giant vacuum Rabi splitting on the order of the bare phonon and cavity frequencies. Through terahertz time-domain spectroscopy experiments, we systematically studied the vacuum Rabi splitting as a function of sample thickness, temperature, and cavity length. Under the strongest light–matter coupling conditions, the strength of coupling exceeded the bare phonon and cavity frequencies, putting the system into the deep-strong coupling regime. These results demonstrate that this uniquely tunable platform is promising for realizing and understanding predicted cavity-vacuum-induced ferroelectric instabilities and exploring applications of light–matter coupling in the ultrastrong and deep-strong coupling regimes in quantum technology. Copyright © 2025, The Authors. All rights reserved.

关键词： Phonons

Bridging particle deformability and collective response in soft solids

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Physical Review materials 2021年第5期5卷 055605-055605页

作者： John D. Treado Dong Wang Arman Boromand Michael P. Murrell Mark D. Shattuck Corey S. O'Hern Department of Mechanical Engineering & Materials Science Yale University New Haven Connecticut 06520 USA Integrated Graduate Program in Physical and Engineering Biology Yale University New Haven Connecticut 06520 USA Department of Biomedical Engineering Yale University New Haven Connecticut 06520 USA Department of Physics Yale University New Haven Connecticut 06520 USA Systems Biology Institute Yale University West Haven Connecticut 06516 USA Benjamin Levich Institute and Physics Department The City College of New York New York New York 10031 USA Department of Applied Physics Yale University New Haven Connecticut 06520 USA

Soft, amorphous solids such as tissues, foams, and emulsions are composed of deformable particles. However, the effect of single-particle deformability on the collective behavior of soft solids is still poorly understood. We perform numerical simulations of two-dimensional jammed packings of explicitly deformable particles to study the mechanical response of model soft solids. We find that jammed packings of deformable particles with excess shape degrees of freedom possess low-frequency quartic vibrational modes that stabilize the packings even though they possess fewer interparticle contacts than the nominal isostatic value. Adding intraparticle constraints can rigidify the particles, but these particles undergo a buckling transition and gain an effective shape degree of freedom when their preferred perimeter is above a threshold value. We find that the mechanical response of jammed packings of deformable particles with shape degrees of freedom differs significantly from that of jammed packings of rigid-shape particles, which emphasizes the importance of particle deformability in modeling soft solids.

关键词： Collective behavior Jamming Emulsions Foams Tissues Molecular dynamics

Influence of Morphology on Fracture Propagation of PMMAe/PC Blend in Tensile Tests at High Strain Rate

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Macromolecular Symposia 2020年第1期394卷 2000153-2000153页

作者： Gomes, Felipe Pedro da Costa Reinaldo, Juciklécia da Silva Rodrigues, Antônio Henrique Venâncio de Macedo, Thatiana Cristina Pereira Silva, Bismarck Luiz Ito, Edson Noriyuki Graduate Program in Materials Science and Engineering Federal University of Rio Grande do Norte Avenida Senador Salgado Filho 3000 NatalRio Grande do Norte59078–970 Brazil Mechanical Engineering Department Federal University of Rio Grande do Norte Avenida Senador Salgado Filho 3000 NatalRio Grande do Norte59078–970 Brazil Graduate Program in Materials Science and Engineering Federal University of Sergipe Avenida Marechal Rondon s/n 49100-000 São CristóvãoSergipe Brazil Materials Engineering Department Federal University of Rio Grande do Norte Avenida Senador Salgado Filho 3000 NatalRio Grande do Norte59078–970 Brazil

The aim of this study is to evaluate toughness mechanism of elastomeric poly(methyl methacrylate) (PMMAe) and polycarbonate (PC) blend through crack propagation at high speed tensile tests. Samples are processed using two types of extruders, single and twin screw, in order to eliminate the influence of processing in the final product's properties. Pure polymers and polymer blend samples are cryo-ultramicrotomed and their morphology is characterized using atomic force microscopy (AFM). Fractured samples obtained from uniaxial tensile tests at high strain rate are inspected using optical microscopy (OM) and scanning electron microscopy (SEM). The results obtained for the PMMAe/PC blend in tests at high deformation rate showed that the shear rate during the mixing process influences the maximum strength of the polymer blend near its region of co-continuous morphology. The visual evaluation of the fracture surface and the fractographic analysis corroborated the results of this study of polymer toughening. © 2020 Wiley-VCH GmbH

关键词： Fracture

Terahertz cavity magnon polaritons

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arXiv 2023年

作者： Kritzell, T. Elijah Baydin, Andrey Tay, Fuyang Rodriguez, Rodolfo Nojiri, Hiroyuki Everitt, Henry O. Barsukov, Igor Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Physics and Astronomy University of California RiversideCA92521 United States Institute for Materials Research Tohoku University Sendai980-8577 Japan DEVCOM Army Research Laboratory-South HoustonTX77005 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

Hybrid light-matter coupled states, or polaritons, in magnetic materials have attracted significant attention due to their potential for enabling novel applications in spintronics and quantum information processing. However, most studies to date have been carried out for ferromagnetic materials with magnon excitations at gigahertz frequencies. Here, we have investigated strong resonant photon-magnon coupling at frequencies above 1 terahertz for the first time in a prototypical room-temperature antiferromagnetic insulator, NiO, inside a Fabry-Pérot cavity. The cavity was formed by the crystal itself when it was thinned down to an optimized thickness. By using terahertz time-domain spectroscopy in high magnetic fields up to 25 T, we swept the magnon frequency through Fabry-Pérot cavity modes and observed photon-magnon anticrossing behavior, demonstrating clear vacuum Rabi splittings exceeding the polariton linewidths. These results show that NiO is a promising platform for exploring antiferromagnetic spintronics and cavity magnonics in the terahertz frequency range. Copyright © 2023, The Authors. All rights reserved.

关键词： Polariton

Persistent flat band splitting and strong selective band renormalization in a kagome magnet thin film

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arXiv 2024年

作者： Ren, Zheng Huang, Jianwei Tan, Hengxin Biswas, Ananya Pulkkinen, Aki Zhang, Yichen Xie, Yaofeng Yue, Ziqin Chen, Lei Xie, Fang Allen, Kevin Wu, Han Ren, Qirui Rajapitamahuni, Anil Kundu, Asish K. Vescovo, Elio Kono, Junichiro Morosan, Emilia Dai, Pengcheng Zhu, Jian-Xin Si, Qimiao Minár, Ján Yan, Binghai Yi, Ming Department of Physics and Astronomy Rice University HoustonTX77005 United States Department of Condensed Matter Physics Weizmann Institute of Science Rehovot Israel New Technologies-Research Center University of West Bohemia Plzeň301 00 Czech Republic Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States National Synchrotron Light Source II Brookhaven National Lab UptonNY United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Chemistry Rice University HoustonTX77005 United States Theoretical Division Center for Integrated Nanotechnologies Los Alamos National Laboratory Los AlamosNM United States

Magnetic kagome materials provide a fascinating playground for exploring the interplay of magnetism, correlation and topology. Many magnetic kagome systems have been reported including the binary FemXn (X=Sn, Ge;m:n = 3:1, 3:2, 1:1) family and the rare earth RMn6Sn6 (R = rare earth) family, where their kagome flat bands are calculated to be near the Fermi level in the paramagnetic phase. While partially filling a kagome flat band is predicted to give rise to a Stoner-type ferromagnetism, experimental visualization of the magnetic splitting across the ordering temperature has not been reported for any of these systems due to the high ordering temperatures, hence leaving the nature of magnetism in kagome magnets an open question. Here, we probe the electronic structure with angle-resolved photoemission spectroscopy in a kagome magnet thin film FeSn synthesized using molecular beam epitaxy. We identify the exchange-split kagome flat bands, whose splitting persists above the magnetic ordering temperature, indicative of a local moment picture. Such local moments in the presence of the topological flat band are consistent with the compact molecular orbitals predicted in theory. We further observe a large spin-orbital selective band renormalization in the Fe dxy+dx2-y2spin majority channel reminiscent of the orbital selective correlation effects in the iron-based superconductors. Our discovery of the coexistence of local moments with topological flat bands in a kagome system echoes similar findings in magic-angle twisted bilayer graphene, and provides a basis for theoretical effort towards modeling correlation effects in magnetic flat band systems. © 2024, CC BY.

关键词： Iron-based Superconductors

Observation of current-induced switching in non-collinear antiferromagnetic IrMn3 by differential voltage measurements

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arXiv 2021年

作者： Arpaci, Sevdenur Lopez-Dominguez, Victor Shi, Jiacheng Sánchez-Tejerina, Luis Garesci, Francesca Wang, Chulin Yan, Xueting Sangwan, Vinod K. Grayson, Matthew Hersam, Mark C. Finocchio, Giovanni Amiri, Pedram Khalili Department of Electrical and Computer Engineering Northwestern University EvanstonIL60208 United States Graduate Program in Applied Physics Northwestern University EvanstonIL60208 United States Department of Mathematical and Computer Sciences Physical Sciences and Earth Sciences University of Messina Messina98166 Italy Department of Engineering University of Messina Messina98166 Italy Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States Department of Chemistry Northwestern University EvanstonIL60208 United States

There is accelerating interest in developing memory devices using antiferromagnetic (AFM) materials, motivated by the possibility for electrically controlling AFM order via spin-orbit torques, and its read-out via magnetoresistive effects. Recent studies have shown, however, that high current densities create non-magnetic contributions to resistive switching signals in AFM/heavy metal (AFM/HM) bilayers, complicating their interpretation. Here we introduce an experimental protocol to unambiguously distinguish current-induced magnetic and nonmagnetic switching signals in AFM/HM structures, and demonstrate it in IrMn3/Pt devices. A six-terminal double-cross device is constructed, with an IrMn3 pillar placed on one cross. The differential voltage is measured between the two crosses with and without IrMn3 after each switching attempt. For a wide range of current densities, reversible switching is observed only when write currents pass through the cross with the IrMn3 pillar, eliminating any possibility of non-magnetic switching artifacts. Micromagnetic simulations support our findings, indicating a complex domain-mediated switching process. © 2021, CC BY.

关键词： Binary alloys