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Structural, magnetic, and electronic properties of a GdAsSe single crystal: Experimental and theoretical studies

Physical Review B 2024年第18期109卷 184420-184420页

作者： R. Kalaivanan Balaji Venkatesan B. Dundi Sri Chandana Rajesh Kumar Ulaganathan G. Senthil Murugan K. Moovendaran Joydev Khatua Li-Hsin Su W. Zhou Xiaofeng Xu Chia-Seng Chang Tien-Ming Chuang Yoshiyuki Iizuka I. Panneer Muthuselvam Horng-Tay Jeng Kwang-Yong Choi Raman Sankar Institute of Physics Academia Sinica Taipei 10617 Taiwan Department of Physics National Taiwan University Taipei 10617 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Taiwan University Taipei 11529 Taiwan Department of Physics School of Basic and Applied Sciences Central University of Tamil Nadu Neelakudi Thiruvarur 610005 Tamil Nadu India Department of Physics Sungkyunkwan University Suwon 16419 Republic of Korea Department of Physics National Tsing Hua University Hsinchu 30013 Taiwan Department of Electro Physics National Yang Ming Chiao Tung University Hsinchu 300093 Taiwan School of Electronic and Information Engineering Changshu Institute of Technology Changshu 215500 China Department of Applied Physics Zhejiang University of Technology Hangzhou 310023 China Institute of Earth Sciences Academia Sinica Taipei 10617 Taiwan Department of Physics (MMV) Banaras Hindu University Varanasi 221005 Uttar Pradesh India Physics Division National Center for Theoretical Sciences Taipei 10617 Taiwan

We report high-quality single-crystal growth, x-ray diffraction, magnetic susceptibility [χ(T,H)], magnetization [M(H)], heat capacity [CP(T,H)], electrical resistivity [ρ(T,H)], and electron spin resonance (ESR) measurements of GdAsSe as functions of temperature and magnetic field. We identify an antiferromagnetic phase transition at TN∼11.9±0.2 K and construct magnetic phase diagrams for H||ab and H||c axes based on the χ(T,H) and CP(T,H) data. Isothermal M(H) curves along the H||ab direction at 3 K exhibit a field-induced spin orientation at HC∼3.78T. Both M(H) and χ(T,H) indicate an easy-plane-type anisotropy. The Curie-Weiss analysis of the high-temperature paramagnetic χ(T) yields a negative Weiss temperature, suggesting dominant antiferromagnetic interactions between the Gd ions. Magnetic entropy reaches 83% of R ln8 at TN. The presence of residual entropy above TN and the persistence of ESR critical broadening up to ∼3TN alludes to a degree of magnetic frustration in the studied material. The ρ(T) data above TN is well fitted to the Bloch-Grüneisen theory for metals. Further, density functional theory calculations reveal an antiferromagnetic ground state where the Gd atoms are coupled ferromagnetically in the ab plane and antiferromagnetically along the c axis.

关键词： Magnetic anisotropy Magnetic coupling Magnetic interactions Magnetic order Magnetism

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All-optical nonreciprocal response in a ring resonator integrating transition metal dichalcogenides

All-optical nonreciprocal response in a ring resonator integ...

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CLEO: science and Innovations, S and I 2022

作者： Kawaguchi, Yuma Guddala, Sriram Komissarenko, Filipp Kiriushechkina, Svetlana Vakulenko, Anton Chen, Kai Alù, Andrea Menon, Vinod M. Khanikaev, Alexander B. Department of Electrical Engineering Grove School of Engineering City College of the City University of New York New YorkNY United States Physics Program Graduate Center of the City University of New York New YorkNY United States Photonics Initiative Advanced Science Research Center City University of New York New YorkNY United States Department of Physics City College of New York New YorkNY United States

The photoinduced nonreciprocity was experimentally observed in WS2 monolayer pumped by circularly polarized light. Based on this, we propose a theoretical model of nonreciprocal optical ring resonator integrating vall... 详细信息

ISBN: (纸本)9781557528209

关键词： Monolayers

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Funneling of Lattice Vibrations Through Topological Phathways in Mid-Infrared Metasurfaces

Funneling of Lattice Vibrations Through Topological Phathway...

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CLEO: science and Innovations, S and I 2022

作者： Guddala, S. Komissarenko, F. Kiriushechkina, S. Vakulenko, A. Li, M. Menon, V.M. Alù, A. Khanikaev, A.B. Department of Electrical Engineering City College of the City University of New York New YorkNY10031 United States Department of Physics City College of New York New YorkNY10031 United States Physics Program Graduate Center of the City University of New York New YorkNY10016 United States Photonics Initiative Advanced Science Research Center City University of New York New YorkNY10031 United States

We demonstrate novel hybrid states of strongly-coupled photon and lattice vibrations in hexagonal boron nitride (hBN) integrated with mid-infrared metasurface and show their unconventional helical nature and resilient... 详细信息

ISBN: (纸本)9781557528209

关键词： Infrared devices

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Chiral metal-organic framework based spin-polarized flexible photodetector with ultrahigh sensitivity

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Materials Today Nano 2023年 21卷

作者： Mustaqeem, M. Kamal, S. Ahmad, N. Chou, P.-T. Lin, K.-H. Huang, Y.-C. Guo, G.-Y. Paul Inbaraj, C.R. Li, W.-K. Yao, H.-C. Lu, K.-L. Chen, Y.-F. Department of Chemistry National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Department of Physics National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Nano-Science and Technology Program Taiwan International Graduate Program Institute of Physics Academia Sinica Taipei106 Taiwan Institute of Chemistry Academia Sinica Taipei115 Taiwan Department of Materials Science and Engineering National Taiwan University of Science and Technology Taipei10607 Taiwan Institute of Physics Academia Sinica Taipei11529 Taiwan Department of Materials Engineering Ming Chi University of Technology

Spin-optoelectronics plays a key role in developing next-generation technologies with potential applications covering from pharmaceutical synthesis and quantum computing to optical communication. One of the most feasible ways to achieve high-performance spin optoelectronic devices is based on chiral materials. Chiral metal-organic frameworks (CMOFs), an emerging class of chiral hybrid materials, have sparked interest due to their structural variety and flexibility, order nanopores, cost-effectiveness, and unique chirality features. Herein, we have developed CMOF [Sr (9,10-adc) (DMAc)2]n based on achiral building blocks [(9,10-adc)] to detect circularly polarized light (CPL) with ultrahigh sensitivity. Their application in spin-polarized flexible detectors gives a detectivity (D∗) as high as 1.83 × 1012 jones, superior to all reported heterochiral MOF-based detectors. Meanwhile, the anisotropy factor (gIph) is up to 0.38 for CPL detection. The maximum photoresponsivity (Rph) and photogain (η) values of CMOFs reach up to 6.0 × 105 (A/W) and 1.8 × 106, respectively, which are also the record values among reported chiral MOFs. Additionally, the photodetector is mechanically flexible and durable, manifesting an important feature for wearable devices. Therefore, our study shown here is significant and timely to open a route for advancing spin-optoelectronics based on CMOF. © 2023 Elsevier Ltd

关键词： Photodetectors

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Ultrastrong Spin-Photon Coupling in Gadolinium Gallium Garnet

Ultrastrong Spin-Photon Coupling in Gadolinium Gallium Garne...

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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Kritzell, T. Elijah Bao, Junzhe Doumani, Jacques Lee, Jae Joon Xu, Hongjing Tay, Fuyang Nojiri, Hiroyuki Bamba, Motoaki Baydin, Andrey Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Physics and Astronomy Rice University HoustonTX77005 United States Institute for Materials Research Tohoku University Sendai980-8577 Japan The Hakubi Center for Advanced Research Kyoto University Kyoto606-8502 Japan Department of Physics I Kyoto University Kyoto606-8502 Japan Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

We examine ultrastrong coupling of an ensemble of paramagnetic spins in Gd3Ga5O12 with terahertz photons in the presence of a high external magnetic field both in the bulk and thin-film limits. © 2023 The Author(s)

ISBN: (纸本)9781957171258

关键词： Photons

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Anharmonic effects on lattice dynamics and thermal transport of two-dimensional InTe Monolayer

arXiv

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arXiv 2022年

作者： Alqurashi, Hind Pandit, Abhiyan Hamad, Bothina Materials Science and Engineering Graduate Program University of Arkansas FayettevilleAR72701 United States Physics Department The College of Science Al Baha University Al Baha65527 Saudi Arabia Department of Physics University of Arkansas FayettevilleAR72701 United States Physics Department The University of Jordan Amman11942 Jordan

The lattice thermal conductivity (kl) plays a key role in the performance of thermoelectric (TE) materials, where the lower values lead to higher figure of merit values. Two-dimensional (2D) group III-VI monolayers such as InTe are promising materials for TE energy generation owing to their low kl that lead to high TE figure of merit values. In this work, we investigate the influence of the lattice anharmonicity on the lattice thermal conductivity of InTe monolayer. The thermodynamic parameters are calculated by using the self-consistent phonon (SCP) theory. The kl value of the InTe monolayer is obtained to be 0.30 Wm−1 K−1 by using the standard Boltzmann transport equation (BTE) approach, while it is 3.58 Wm−1 K−1 by using SCP + BTE approach. These results confirm the importance of the anharmonic effects on the kl value, where it was found to be significantly higher (91%) using the SCP + BTE approach than that obtained using the standard BTE approach. © 2022, CC BY.

关键词： Monolayers

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Deep-Strong Coupling between Cavity Photons and Terahertz TO Phonons in PbTe

Deep-Strong Coupling between Cavity Photons and Terahertz TO...

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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Baydin, Andrey Manjappa, Manukumara Mishra, Sobhan Subhra Xu, Hongjing Tay, Fuyang Kim, Dasom Hernandez, Felix G.G. Rappl, Paulo H.O. Abramof, Eduardo Singh, Ranjan Kono, Junichiro Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley-Curl Institute Rice University HoustonTX77005 United States Instrumentation and Applied Physics Department Indian Institute of Science Bangalore560012 India Center for Disruptive Photonic Technologies The Photonics Institute Nanyang Technological University 639798 Singapore Department of Physics and Astronomy Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Instituto de Física Universidade de Sao Paulo SP Sao Paulo05508-090 Brazil Laboratorio Associado de Sensores e Materiais Instituto Nacional de Pesquisas Espaciais SP Sao Jose dos Campos12201-970 Brazil Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Department of Material Science and NanoEngineering Rice University HoustonTX77005 United States

We have investigated the resonant coupling of photons with TO phonons in lead telluride in small-mode-volume terahertz cavities, observing a giant vacuum Rabi splitting on the order of the bare cavity-phonon frequency... 详细信息

ISBN: (纸本)9781957171258

关键词： Photons

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Space-Time Nonlocal Metasurfaces for Event-Based Image Processing

arXiv

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arXiv 2024年

作者： Esfahani, Sedigheh Cotrufo, Michele Alù, Andrea Photonics Initiative Advanced Science Research Center City University of New York New YorkNY10031 United States Physics Program Graduate Center of the City University of New York New YorkNY10016 United States The Institute of Optics University of Rochester RochesterNY14627 United States

Analog computation with passive optical components can enhance processing speeds and reduce power consumption, recently attracting renewed interest thanks to the opportunities enabled by metasurfaces. Basic image processing tasks, such as spatial differentiation, have been recently demonstrated based on engineered nonlocalities in metasurfaces, but next-generation computational schemes require more advanced capabilities. Here, we tailor nonlocalities in space and time to design a metasurface that can perform mixed spatio-temporal differentiation of an input image, realizing event-based edge detection with a passive ultrathin silicon-based structured film compatible with standard fabrication techniques. The metasurface detects the object edges only when the object moves, and its design can be tailored to selectively enhance objects moving at desired speeds. Our results point towards fully-passive processing of spatio-temporal signals, for highly compact neuromorphic cameras. © 2024, CC BY.

关键词： Object detection

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Maxwell’s Demon Walks into Wall Street: Stochastic Thermodynamics Meets Expected Utility Theory

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Physical Review Letters 2023年第19期131卷 197103-197103页

作者： Andrés F. Ducuara Paul Skrzypczyk Francesco Buscemi Peter Sidajaya Valerio Scarani Yukawa Institute for Theoretical Physics Kyoto University Kitashirakawa Oiwakecho Sakyo-ku Kyoto 606-8502 Japan Center for Gravitational Physics and Quantum Information Yukawa Institute for Theoretical Physics Kyoto University H.H. Wills Physics Laboratory University of Bristol Tyndall Avenue Bristol BS8 1TL United Kingdom CIFAR Azrieli Global Scholars program CIFAR Toronto Canada Graduate School of Informatics Nagoya University Chikusa-Ku Nagoya 464-8601 Japan Centre for Quantum Technologies National University of Singapore 3 Science Drive 2 Singapore 117543 Singapore Department of Physics National University of Singapore 2 Science Drive 3 Singapore 117542 Singapore

The interplay between thermodynamics and information theory has a long history, but its quantitative manifestations are still being explored. We import tools from expected utility theory from economics into stochastic thermodynamics. We prove that, in a process obeying Crooks’s fluctuation relations, every α Rényi divergence between the forward process and its reverse has the operational meaning of the “certainty equivalent” of dissipated work (or, more generally, of entropy production) for a player with risk aversion r=α−1. The two known cases α=1 and α=∞ are recovered and receive the new interpretation of being associated with a risk-neutral and an extreme risk-averse player, respectively. Among the new results, the condition for α=0 describes the behavior of a risk-seeking player willing to bet on the transient violations of the second law. Our approach further leads to a generalized Jarzynski equality, and generalizes to a broader class of statistical divergences.

关键词： Econophysics Fluctuation theorems Information & communication theory Stochastic processes Stochastic thermodynamics Thermodynamics

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Topological Surface State Evolution in Bi2Se3 via Surface Etching

arXiv

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arXiv 2024年

作者： Yue, Ziqin Huang, Jianwei Wang, Ruohan Li, Jia-Wan Rong, Hongtao Guo, Yucheng Wu, Han Zhang, Yichen Kono, Junichiro Zhou, Xingjiang Hou, Yusheng Wu, Ruqian Yi, Ming Department of Physics and Astronomy Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Guangdong Provincial Key Laboratory of Magnetoelectric Physics and Devices Center for Neutron Science and Technology School of Physics Sun Yat-Sen University Guangzhou510275 China Institute of Physics Chinese Academy of Sciences Beijing100190 China Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Department of Physics and Astronomy University of California Irvine IrvineCA92697 United States

Topological insulators are materials with an insulating bulk interior while maintaining gapless boundary states against back scattering. Bi2Se3 is a prototypical topological insulator with a Dirac-cone surface state around Γ. Here, we present a controlled methodology to gradually remove Se atoms from the surface Se-Bi-Se-Bi-Se quintuple layers, eventually forming bilayer-Bi on top of the quintuple bulk. Our method allows us to track the topological surface state and confirm its robustness throughout the surface modification. Importantly, we report a relocation of the topological Dirac cone in both real space and momentum space, as the top surface layer transitions from quintuple Se-Bi-Se-Bi-Se to bilayer-Bi. Additionally, charge transfer among different surface layers is identified. Our study provides a precise method to manipulate surface configurations, allowing for the fine-tuning of the topological surface states in Bi2Se3, which represents a significant advancement towards nano-engineering of topological states. Copyright © 2024, The Authors. All rights reserved.

关键词： Topological insulators

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