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37th International Cosmic Ray Conference, ICRC 2021

作者： Kobayshi, Yukiho Sanchez, David Abe, H. Aguasca, A. Agudo, I. Antonelli, L.A. Aramo, C. Armstrong, T. Artero, M. Asano, K. Ashkar, H. Aubert, P. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Becerra González, J. Bernardos, M.I. Berti, A. Biederbeck, N. Bigongiari, C. Blanch, O. Bonnoli, G. Bordas, P. Bose, D. Bulgarelli, A. Burelli, I. Buscemi, M. Cardillo, M. Caroff, S. Carosi, A. Cassol, F. Cerruti, M. Chai, Y. Cheng, K. Chikawa, M. Chytka, L. Contreras, J.L. Cortina, J. Costantini, H. Dalchenko, M. De Angelis, A. de Bony de Lavergne, M. Deleglise, G. Delgado, C. Delgado Mengual, J. della Volpe, D. Depaoli, D. Di Pierro, F. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Elsässer, D. Emery, G. Escudero, J. Fiasson, A. Foffano, L. Fonseca, M.V. Freixas Coromina, L. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Green, D. Grespan, P. Gunji, S. Hackfeld, J. Hadasch, D. Hahn, A. Hassan, T. Hayashi, K. Heckmann, L. Heller, M. Herrera Llorente, J. Hirotani, K. Hoffmann, D. Horns, D. Houles, J. Hrabovsky, M. Hrupec, D. Hui, D. Hütten, M. Inada, T. Inome, Y. Iori, M. Ishio, K. Iwamura, Y. Jacquemont, M. Jimenez Martinez, I. Jouvin, L. Jurysek, J. Kagaya, M. Karas, V. Katagiri, H. Kataoka, J. Kerszberg, D. Kobayashi, Y. Kong, A. Kubo, H. Kushida, J. Lamanna, G. Lamastra, A. Le Flour, T. Longo, F. López-Coto, R. López-Moya, M. López-Oramas, A. Luque-Escamilla, P.L. Majumdar, P. Makariev, M. Mandat, D. Manganaro, M. Mannheim, K. Mariotti, M. Marquez, P. Marsella, G. Martí, J. Martinez, O. Martínez, G. Martínez, M. Marusevec, P. Mas, A. Maurin, G. Mazin, D. Mestre Guillen, E. Micanovic, S. Miceli, D. Miener, T. Miranda, J.M. Miranda, L.D.M. Mirzoyan, R. Mizuno, T. Molina, E. Montaruli, T. Monteiro, I. Moralejo, A. Morcuende, D. Moretti, E. Morselli, A. Mrakovcic, K. Murase, K. Nagai, A. LAPP Université de Savoie Mont-Blanc CNRS/IN2P3 Annecy74941 France Institute for Cosmic Ray Research The University of Tokyo Kashiwa Japan Institute for Cosmic Ray Research University of Tokyo Japan Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain Instituto de Astrofísica de Andalucía CSIC INAF - Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy Aix Marseille Univ CNRS/IN2P3 CPPM France The Barcelona Institute of Science and Technology Spain IRFU CEA Université Paris-Saclay France LAPP Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS/IN2P3 Annecy France Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan EMFTEL department IPARCOS Universidad Complutense de Madrid Spain INAF - Osservatorio di Astrofisica Scienza dello Spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil INFN Sezione di Padova Università degli Studi di Padova Italy Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain Max-Planck-Institut für Physik Germany Department of Physics TU Dortmund University Germany Saha Institute of Nuclear Physics INFN Sezione di Trieste Università degli Studi di Udine Italy INFN Sezione di Catania Italy Italy University of Geneva Département de Physique Nucléaire et Corpusculaire Switzerland Palacky University Olomouc Faculty of Science Czech Republic CIEMAT Port d'Informació Científica INFN Sezione di Torino Italy Dipartimento di Fisica Universitá degli Studi di Torino Italy INFN Sezione di Bari Università di Bari Italy University of Rijeka Department of Physics Croatia Institute for Theoretical Physics and Astrophysics Universität Würzburg Germany Physics Program Graduate School of Advanced Science and Engineering Hiroshima University Japan INFN Sezione di Bari Politecnico di Bari Italy Faculty of Physics and Applied Informatics University of L

The recent detection of a very high energy (VHE) emission from Gamma-Ray Bursts (GRBs) above 100 GeV performed by the MAGIC and H.E.S.S. collaborations, has represented a significant, long-awaited result for the VHE astrophysics community. Although these results' scientific impact has not yet been fully exploited, the possibility to detect VHE gamma-ray signals from GRBs has always been considered crucial for clarifying the poorly known physics of these objects. Furthermore, the discovery of high-energy neutrinos and gravitational waves associated with astrophysical sources have definitively opened the era of multi-messenger astrophysics, providing unique insights into the physics of extreme cosmic accelerators. In the near future, the Cherenkov Telescope Array (CTA) will play a major role in these observations. Within this framework, the Large Size Telescopes (LSTs) will be the instruments best suited to significantly impact on short time-scale transients follow-up thanks to their fast slewing and large effective area. The observations of the early emission phase of a wide range of transient events with good sensitivity below 100 GeV will allow us to open new opportunities for time-domain astrophysics in an energy range not affected by selective absorption processes typical of other wavelengths. In this contribution, we will report about the observational program and first transients follow-up observations performed by the LST-1 telescope currently in its commissioning phase on La Palma, Canary Islands, the CTA northern hemisphere site. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Telescopes

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Tunable spin Hall and spin Nernst effects in Dirac line-node semimetals XCuYAs (X=Zr,Hf;Y=Si,Ge)

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Physical Review Materials 2020年第12期4卷 124205-124205页

作者： Babu Baijnath Prasad Guang-Yu Guo Department of Physics and Center for Theoretical Physics National Taiwan University Taipei 10617 Taiwan Republic of China Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei 11529 Taiwan Republic of China Physics Division National Center for Theoretical Sciences Taipei 10617 Taiwan Republic of China

The quaternary arsenide compounds XCuYAs (X=Zr,Hf; Y=Si,Ge) belong to the vast family of the 1111-type quaternary compounds, which possess outstanding physical properties ranging from p-type transparent semiconductors to high-temperature Fe-based superconductors. In this paper, we study the electronic structure topology, the spin Hall effect (SHE), and the spin Nernst effect (SNE) in these compounds based on density functional theory calculations. First we find that the four considered compounds are Dirac semimetals with the nonsymmorphic symmetry-protected Dirac line nodes along the Brillouin zone boundary A−M and X−R and low density of states near the Fermi level (EF). Second, the intrinsic SHE and SNE in some of these considered compounds are found to be large. In particular, the calculated spin Hall conductivity (SHC) of HfCuGeAs is as large as −514(ℏ/e)(S/cm). The spin Nernst conductivity (SNC) of HfCuGeAs at room temperature is also large, being −0.73 (ℏ/e) (A/m K). Moreover, both the magnitude and sign of the SHC and SNC in these compounds can be manipulated by varying either the applied electric field direction or the spin current direction. The SHE and SNE in these compounds can also be enhanced by tuning the Fermi level via chemical doping or electric gating. Finally, a detailed analysis of the band-decomposed and k-resolved spin Berry curvatures reveals that these large SHC and SNC as well as their notable tunabilities originate largely from the presence of a large number of spin-orbit coupling-gapped Dirac points near the Fermi level as well as the gapless Dirac line nodes, which give rise to large spin Berry curvatures. Our findings thus suggest that the four XCuYAs compounds not only provide a valuable platform for exploring the interplay between SHE, SNE, and band topology, but they also have promising applications in spintronics and spin caloritronics.

关键词： Electronic structure First-principles calculations Topological materials

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Status and results of the prototype LST of CTA 37

Status and results of the prototype LST of CTA

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37th International Cosmic Ray Conference, ICRC 2021

作者： Mazin, D. Abe, H. Aguasca, A. Agudo, I. Antonelli, L.A. Aramo, C. Armstrong, T. Artero, M. Asano, K. Ashkar, H. Aubert, P. Baktash, A. Bamba, A. Baquero Larriva, A. Baroncelli, L. Barres de Almeida, U. Barrio, J.A. Batkovic, I. Becerra González, J. Bernardos, M.I. Berti, A. Biederbeck, N. Bigongiari, C. Blanch, O. Bonnoli, G. Bordas, P. Bose, D. Bulgarelli, A. Burelli, I. Buscemi, M. Cardillo, M. Caroff, S. Carosi, A. Cassol, F. Cerruti, M. Chai, Y. Cheng, K. Chikawa, M. Chytka, L. Contreras, J.L. Cortina, J. Costantini, H. Dalchenko, M. De Angelis, A. de Bony de Lavergne, M. Deleglise, G. Delgado, C. Delgado Mengual, J. della Volpe, D. Depaoli, D. Di Pierro, F. Di Venere, L. Díaz, C. Dominik, R.M. Dominis Prester, D. Donini, A. Dorner, D. Doro, M. Elsässer, D. Emery, G. Escudero, J. Fiasson, A. Foffano, L. Fonseca, M.V. Freixas Coromina, L. Fukami, S. Fukazawa, Y. Garcia, E. Garcia López, R. Giglietto, N. Giordano, F. Gliwny, P. Godinovic, N. Green, D. Grespan, P. Gunji, S. Hackfeld, J. Hadasch, D. Hahn, A. Hassan, T. Hayashi, K. Heckmann, L. Heller, M. Herrera Llorente, J. Hirotani, K. Hoffmann, D. Horns, D. Houles, J. Hrabovsky, M. Hrupec, D. Hui, D. Hütten, M. Inada, T. Inome, Y. Iori, M. Ishio, K. Iwamura, Y. Jacquemont, M. Jimenez Martinez, I. Jouvin, L. Jurysek, J. Kagaya, M. Karas, V. Katagiri, H. Kataoka, J. Kerszberg, D. Kobayashi, Y. Kong, A. Kubo, H. Kushida, J. Lamanna, G. Lamastra, A. Le Flour, T. Longo, F. López-Coto, R. López-Moya, M. López-Oramas, A. Luque-Escamilla, P.L. Majumdar, P. Makariev, M. Mandat, D. Manganaro, M. Mannheim, K. Mariotti, M. Marquez, P. Marsella, G. Martí, J. Martinez, O. Martínez, G. Martínez, M. Marusevec, P. Mas, A. Maurin, G. Mestre Guillen, E. Micanovic, S. Miceli, D. Miener, T. Miranda, J.M. Miranda, L.D.M. Mirzoyan, R. Mizuno, T. Molina, E. Montaruli, T. Monteiro, I. Moralejo, A. Morcuende, D. Moretti, E. Morselli, A. Mrakovcic, K. Murase, K. Nagai, A. Nakamori, T. Nickel, L. Nieto, D. Institute for Cosmic Ray Research University of Tokyo 5-1-5 Kashiwa-no-ha Chiba Kashiwa277-8582 Japan Max-Planck-Institut für Physik München80805 Germany Departament de Física Quàntica i Astrofísica Institut de Ciències del Cosmos Universitat de Barcelona IEEC-UB Spain Instituto de Astrofísica de Andalucía-CSIC Spain INAF - Osservatorio Astronomico di Roma Italy INFN Sezione di Napoli Italy Aix Marseille Univ CNRS IN2P3 CPPM France The Barcelona Institute of Science and Technology Spain IRFU CEA Université Paris-Saclay France LAPP Univ. Grenoble Alpes Univ. Savoie Mont Blanc CNRS-IN2P3 Annecy France Universität Hamburg Institut für Experimentalphysik Germany Graduate School of Science University of Tokyo Japan EMFTEL department IPARCOS Universidad Complutense de Madrid Spain INAF - Osservatorio di Astrofisica e Scienza dello spazio di Bologna Italy Centro Brasileiro de Pesquisas Físicas Brazil INFN Sezione di Padova Università degli Studi di Padova Italy Instituto de Astrofísica de Canarias Departamento de Astrofísica Universidad de La Laguna Spain Department of Physics TU Dortmund University Germany Saha Institute of Nuclear Physics India INFN Sezione di Trieste Università degli Studi di Udine Italy INFN Sezione di Catania Italy Italy University of Geneva Département de Physique Nucléaire et Corpusculaire Switzerland Palacky University Olomouc Faculty of Science Czech Republic CIEMAT Port d'Informació Científica INFN Sezione di Torino Italy Dipartimento di Fisica Universitá degli Studi di Torino Italy INFN Sezione di Bari Università di Bari Italy University of Rijeka Department of Physics Croatia Institute for Theoretical Physics and Astrophysics Universität Würzburg Germany Physics Program Graduate School of Advanced Science and Engineering Hiroshima University Japan INFN Sezione di Bari Politecnico di Bari Italy Faculty of Physics and Applied Informatics University of Lodz Poland University of Split FESB Croatia Department of Physics

The Large-Sized Telescopes (LSTs) of Cherenkov Telescope Array (CTA) are designed for gamma-ray studies focusing on low energy threshold, high flux sensitivity, rapid telescope repositioning speed and a large field of view. Once the CTA array is complete, the LSTs will be dominating the CTA performance between 20 GeV and 150 GeV. During most of the CTA Observatory construction phase, however, the LSTs will be dominating the array performance until several TeVs. In this presentation we will report on the status of the LST-1 telescope inaugurated in La Palma, Canary islands, Spain in 2018. We will show the progress of the telescope commissioning, compare the expectations with the achieved performance, and give a glance of the first physics results. © Copyright owned by the author(s) under the terms of the Creative Commons.

关键词： Telescopes

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Benchmarking Diamond Surface Preparation and Fluorination Via Inductively Coupled Plasma-Reactive Ion Etching

SSRN

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SSRN 2024年

作者： Gray, Tia Zhang, Xiang Biswas, Abhijit Terlier, Tanguy Oliveira, Eliezer F. Puthirath, Anand B. Li, Chenxi Pieshkov, Tymofii S. Garratt, Elias J. Neupane, Mahesh R. Pate, Bradford B. Glen, A. Birdwell Ivanov, Tony G. Vajtai, Robert Ajayan, Pulickel M. Department of Materials Science and Nanoengineering Rice University HoustonTX77005 United States SIMS laboratory Shared Equipment Authority Rice University HoustonTX77005 United States SP Bauru17033-360 Brazil Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States DEVCOM Army Research Laboratory RF Devices and Circuits AdelphiMD20783 United States Chemistry Division U.S. Naval Research Laboratory WashingtonDC20375 United States

Diamond, renowned for its exceptional semiconducting properties, stands out as a promising material for high-performance power electronics, optics, quantum, and biosensing technologies. This study methodically investigates the optimization of polycrystalline diamond (PCD) substrate surfaces through Inductively Coupled Plasma Reactive Ion Etching (ICP-RIE). Various parameters, including gaseous species, flow rate, coil power, and bias power were tuned to understand their impact on surface morphology and chemistry. A thorough characterization, encompassing chemical, spectroscopic, and microscopic methods, shed light on the effects of different ICP-RIE conditions on surface properties. CF4/O2 plasma emerged as a viable treatment for achieving smooth PCD surfaces with minimal etch pit formation. Most notably, surface fluorination, a critical aspect of increasing chemical and thermal stability, was successfully accomplished using CF4, SF6, and other F-containing plasmas. The fluorine concentration and surface chemistry variations were studied, with high resolution X-ray Photoelectron Spectroscopy unveiling differences amongst the sp2 C phase, sp3 C phase, C-O, C=O, and C-F bonds. Time-of-flight secondary Ion Mass Spectrometry (ToF-SIMS) and depth-profile analysis unveiled a consistent surface fluorination pattern with CF4/O2 treatment. Furthermore, contact angle measurements showcased heightened hydrophobicity. This study provides valuable insights into precise diamond surface engineering, important for the development of future diamond-based semiconductor technologies. © 2024, The Authors. All rights reserved.

关键词： Surface morphology

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Unravelling the asphericities in the explosion and multi-faceted circumstellar matter of SN 2023ixf

arXiv

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arXiv 2024年

作者： Singh, Avinash Teja, Rishabh Singh Moriya, Takashi J. Maeda, Keiichi Kawabata, Koji S. Tanaka, Masaomi Imazawa, Ryo Nakaoka, Tatsuya Gangopadhyay, Anjasha Yamanaka, Masayuki Swain, Vishwajeet Sahu, D.K. Anupama, G.C. Kumar, Brajesh Anche, Ramya M. Sano, Yasuo Raj, A. Agnihotri, V.K. Bhalerao, Varun Bisht, D. Bisht, M.S. Belwal, K. Chakrabarti, S.K. Fujii, Mitsugu Nagayama, Takahiro Matsumoto, Katsura Hamada, Taisei Kawabata, Miho Kumar, Amit Kumar, Ravi Malkan, Brian K. Smith, Paul Sakagami, Yuta Taguchi, Kenta Tominaga, Nozomu Watanabe, Arata Hiroshima Astrophysical Science Centre Hiroshima University 1-3-1 Kagamiyama Higashi-Hiroshima Hiroshima739-8526 Japan Department of Astronomy The Oskar Klein Center Stockholm University AlbaNova University Center StockholmSE 106 91 Sweden Indian Institute of Astrophysics II Block Koramangala Karnataka Bengaluru560034 India Pondicherry University UT of Puducherry R.V. Nagar Kalapet Pondicherry605014 India National Astronomical Observatory of Japan National Institutes of Natural Sciences 2-21-1 Osawa Mitaka Tokyo181-8588 Japan Graduate Institute for Advanced Studies SOKENDAI 2-21-1 Osawa Mitaka Tokyo181-8588 Japan School of Physics and Astronomy Monash University ClaytonVIC3800 Australia Department of Astronomy Kyoto University Kitashirakawa-Oiwake-cho Sakyo-ku Kyoto606-8502 Japan Department of Physics Graduate School of Advanced Science and Engineering Hiroshima University 1-3-1 Kagamiyama Higashi-Hiroshima Hiroshima739-8526 Japan Astronomical Institute Tohoku University Aoba Sendai980-8578 Japan Department of Physics Graduate School of Advanced Science and Engineering Hiroshima Astrophysical Science Centre Hiroshima University 1-3-1 Kagamiyama Higashi-Hiroshima Hiroshima739-8526 Japan Graduate School of Science and Engineering Kagoshima University 1-21-35 Korimoto Kagoshima Kagoshima890-0065 Japan Department of Physics Indian Institute of Technology Bombay Powai Mumbai400076 India South-Western Institute for Astronomy Research Yunnan University Yunnan Kunming650504 China Steward Observatory University of Arizona 933N Cherry Avenue TucsonAZ85721 United States Observation and Data Center for Cosmosciences Faculty of Science Hokkaido University Kita-ku Sapporo-shi Hokkaido060-0810 Japan Nayoro Observatory 157-1 Nisshin Nayoro-shi Hokkaido096-0066 Japan Indian Centre for Space Physics 466 Barakhola Netai Nagar West Bengal Kolkata700099 India Cepheid Observatory India Fujii Kurosaki Observatory 4500 Kurosaki

We present a detailed investigation of photometric, spectroscopic, and polarimetric observations of the Type II SN 2023ixf. Earlier studies have provided compelling evidence for a delayed shock breakout from a confined dense circumstellar matter (CSM) enveloping the progenitor star. The temporal evolution of polarization in SN 2023ixf revealed three distinct peaks in polarization evolution at 1.4 d, 6.4 d, and 79.2 d, indicating an asymmetric dense CSM, an aspherical shock front and clumpiness in the low-density extended CSM, and an aspherical inner ejecta/He-core. SN 2023ixf displayed two dominant axes, one along the CSM-outer ejecta and the other along the inner ejecta/He-core, showcasing the independent origin of asymmetry in the early and late evolution. The argument for an aspherical shock front is further strengthened by the presence of a high-velocity broad absorption feature in the blue wing of the Balmer features in addition to the P-Cygni absorption post 16 d. Hydrodynamical light curve modeling indicated a progenitor mass of 10 M☉ with a radius of 470 R☉ and explosion energy of 2 × 1051 erg, along with 0.06 M☉ of 56 Ni, though these properties are not unique due to modeling degeneracies. The modeling also indicated a two-zone CSM: a confined dense CSM extending up to 5×1014 cm, with a mass-loss rate of 10−2 M☉ yr−1 and an extended CSM spanning from 5×1014 cm to at least 1016 cm with a mass-loss rate of 10−4 M☉ yr−1, both assuming a wind-velocity of 10 km s−1. The early nebular phase observations display an axisymmetric line profile of [O I], red-ward attenuation of the emission of Hα post 125 days and flattening in the Ks-band marking the onset of dust formation. Copyright © 2024, The Authors. All rights reserved.

关键词： Supernovae

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Smart photonic wristband for pulse wave monitoring

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Opto-Electronic science 2024年第12期3卷 12-27页

作者： Renfei Kuang Zhuo Wang Lin Ma Heng Wang Qingming Chen Arnaldo Leal Junior Santosh Kumar Xiaoli Li Carlos Marques Rui Min Center for Cognition and Neuroergonomics State Key Laboratory of Cognitive Neuroscience and LearningBeijing Normal UniversityZhuhai 519087China College of Science Shenyang Aerospace UniversityShenyang 110136China School of Microelectronics Science and Technology Guangdong Provincial Key Laboratory of Optoelectronic Information Processing Chips and SystemsSun Yat-Sen UniversityZhuhai 519082China Graduate Program in Electrical Engineering Federal University of Espírito SantoFernando Ferrari AvenueVitoria 29075-910Brazil Department of Electronics and Communication Engineering Koneru Lakshmaiah Education FoundationVaddeswaramAndhra Pradesh 522302India CICECO-Aveiro Institute of Materials Physics DepartmentUniversity of AveiroAveiro 3810-193Portugal

Real-time acquisition of human pulse signals in daily life is clinically important for cardiovascular disease monitoring and ***,we propose a smart photonic wristband for pulse signal monitoring based on speckle pattern analysis with a polymer optical fiber(POF)integrated into a sports *** different speckle pattern processing algorithms and POFs with different core diameters were *** results indicated that the smart photonic wristband had a high signal-to-noise ratio and low latency,with the measurement error controlled at approximately 3.7%.This optimized pulse signal could be used for further medical diagnosis and was capable of objectively monitoring subtle pulse signal changes,such as the pulse waveform at different positions of Cunkou and pulse waveforms before and after *** the assistance of artificial intelligence(AI),functions such as gesture recognition have been realized through the established prediction model by processing pulse signals,in which the recognition accuracy reaches 95%.Our AI-assisted smart photonic wristband has potential applications for clinical treatment of cardiovascular diseases and home monitoring,paving the way for medical Internet of Things-enabled smart systems.

关键词： smart healthcare specklegram pulse monitoring gesture recognition artificial intelligence wearable sensor

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Effects of chain-chain interaction on the configuration of short-chain alkanethiol self-assembled monolayers on a metal surface

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Journal of Chemical physics 2024年第21期160卷 214711-214711页

作者： Liao, Chia-Li Faizanuddin, Syed Mohammed Haruyama, Jun Liao, Wei-Ssu Wen, Yu-Chieh Department of Chemistry National Taiwan University Taipei 10617 Taiwan Institute of Physics Academia Sinica Taipei 11529 Taiwan Taiwan International Graduate Program Academia Sinica Taipei 11529 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu 300044 Taiwan Solid State Chemistry Laboratory Cluster for Pioneering Research RIKEN Wako 351-0198 Japan Center for Emerging Material and Advanced Devices National Taiwan University Taipei 10617 Taiwan

Surface-specific sum frequency generation vibrational spectroscopy is applied to study the molecular configuration of short-chain n-alkanethiol self-assembled monolayers (SAMs with n = 2-6) on the Au surface. For monolayers with n ≥ 3, the alkanethiols are upright-oriented, with the CH₃ tilt angle varying between ∼33° and ∼46° in clear even-odd dependency. The ethanethiol monolayer (n = 2) is, however, found to exhibit a distinct lying-down configuration with a larger methyl tilt angle (67°-79°) and a smaller CH₂ tilt angle (56°-68°). Such a unique configurational transition from n = 2 to n ≥ 3 discloses the steric effect owing to chain-chain interaction among neighboring molecules. Through density functional theory calculations, the transition is further confirmed to be energetically favorable for thiols on a defective reconstructed Au(111) surface but not on the pristine one. Our study highlights the roles of the chain-chain interaction and the substrate surface atomic structure when organizing SAMs, offering a strategic pathway for exploiting their applications. © 2024 Author(s).

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Angle-resolved photoemission spectroscopy with an in situ tunable magnetic field

arXiv

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arXiv 2023年

作者： Huang, Jianwei Yue, Ziqin Baydin, Andrey Zhu, Hanyu Nojiri, Hiroyuki Kono, Junichiro He, Yu Yi, Ming Department of Physics and Astronomy Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Smalley–Curl Institute Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Institute for Materials Research Tohoku University Katahira 2-1-1 Sendai980-8577 Japan Department of Applied Physics Yale University New HavenCT06511 United States

Angle-resolved photoemission spectroscopy (ARPES) is a powerful tool for probing the momentum-resolved single-particle spectral function of materials. Historically, in situ magnetic fields have been carefully avoided as they are detrimental to the control of photoelectron trajectory during the photoelectron detection process. However, magnetic field is an important experimental knob for both probing and tuning symmetry-breaking phases and electronic topology in quantum materials. In this paper, we introduce an easily implementable method for realizing an in situ tunable magnetic field at the sample position in an ARPES experiment and analyze magnetic field induced artifacts in ARPES data. Specifically, we identified and quantified three distinct extrinsic effects of a magnetic field: Constant energy contour rotation, emission angle contraction, and momentum broadening. We examined these effects in three prototypical quantum materials, i.e., a topological insulator (Bi2Se3), an iron-based superconductor (LiFeAs), and a cuprate superconductor (Pb-Bi2Sr2CuO6+x), and demonstrate the feasibility of ARPES measurements in the presence of a controllable magnetic field. Our studies lay the foundation for the future development of the technique and interpretation of ARPES measurements of field-tunable quantum phases. Copyright © 2023, The Authors. All rights reserved.

关键词： Photoelectrons

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Investigation of the Interface Between Pulse Laser Deposition Grown Cubic Boron Nitride and Nitrogen Functionalized Diamond

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Microscopy and Microanalysis 2024年第SUPPLEMENT_1期30卷

作者： Pieshkov, Tymofii S Biswas, Abhijit Hachtel, Jordan A Vajtai, Robert Ajayan, Pulickel M Department of Materials Science and Nanoengineering Rice University Houston TX USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston TX USA Center for Nanophase Materials Science Oak Ridge National Laboratory Oak Ridge TN USA

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Structural, Electronic, Optical, and Potassium Anodic Electrochemical Characteristics of 2-Dimensional Silicane: A Density Functional Theory Investigation

SSRN

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SSRN 2022年

作者： Peng, Qiong Rehman, Javed Aziz, Saadullah G. Laref, Amel Albaqami, Munirah D. Alotabi, Reham Ghazi Dinh, Van An Shibl, Mohamed F. Institution of Condensed Physics College of Physics and Electronics Engineering Hengyang Normal University Hengyang421002 China Department of Physics National University of Defense Technology Hunan Changsha410073 China Baluchistan Quetta87300 Pakistan Chemistry Department Faculty of Science King Abdulaziz University Jeddah21589 Saudi Arabia Department of Physics and Astronomy College of Science King Saud University Riyadh11451 Saudi Arabia Chemistry Department College of Science King Saud University Riyadh11451 Saudi Arabia Department of Precision Engineering Graduate School of Engineering Osaka University 2-1 Yamadaoka Osaka Suita565-0871 Japan Renewable Energy Program Center for Sustainable Development College of Arts and Sciences Qatar University Doha2713 Qatar

Two-dimensional (2D) graphene-like materials have attracted tremendous interest due to their remarkable properties in nanoelectronics. To understand and characterize the various physical properties of silicane relevant to optoelectronic and battery applications, various characteristics of 2D silicane Si2H2 are investigated using the density-functional theory. It is disclosed that the structure of 2D Si2H2 is stable, which corroborates its experimental feasibility based on the computational outcomes. With absorption coefficients of about 73.08 (104/cm) and 158.86 (104/cm) at 7.63 eV and 7.66 eV, respectively, it is pertinent to optoelectronic devices. 2D silicane is an exemplary K anodic material, owing to its lesser average open-circuit voltage (OCV) (0.23) and superior theoretical capacity (506 mAhg-1). Afterward, we procured the lowest activation barrier (40 meV) for K migration, which implies the swift charge/discharge mechanism for potassium ion batteries (PIBs). These concomitant findings reinforce the pertinence of silicane material in solar and K anodic utilizations. © 2022, The Authors. All rights reserved.

关键词： Open circuit voltage

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