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Photocatalytic degradation of perfluorooctane sulfonic acid and perfluorooctanoic acid using titanium dioxide/graphene oxide nanocomposite immobilized on polyvinyl alcohol film

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Case Studies in Chemical and Environmental engineering 2024年 10卷

作者： Boonchata, Putthicha Boontanon, Narin Jindal, Vinod Aung, Humm Kham Zan Zan Visvanathan, Chettiyappan Fujii, Shigeo Boontanon, Suwanna Kitpati Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Research Center and Technology Development for Environmental Innovation Faculty of Environment and Resource Studies Mahidol University Department of Chemical Engineering Faculty of Engineering Mahidol University Graduate School of Global Environmental Studies Kyoto University

In full-scale units, the real application of nanoparticles photocatalytic degradation is still challenging due to the requirement of post separation for recovery of fine particles. This work investigated the removal efficiencies of perfluorooctane sulfonic acid (PFOS) and perfluorooctanoic acid (PFOA) using titanium dioxide (TiO₂) nanoparticles coupling with graphene oxide (GO) sheets immobilized in polyvinyl alcohol (PVA) matrix via solution-casting and a heat-treatment process to achieve the TiO₂/GO/PVA nanocomposite film as a photocatalyst. The operative parameters were focused on initial solution pH value, GO concentration, and heat-treatment time, which subsequently determined the optimal indices for the catalyst film. The structure characterization of the Ti–O–C bond indicated that a strong interaction between GO and TiO₂ had been formed at the hydrolysis process while TiO₂/GO nanoparticles were chemically embedded in PVA matrix by the heat-treatment method. The photocatalytic degradation of PFOS and PFOA produced a nanocomposite film with 25 wt% TiO₂/GO that was treated at 120 °C for 3 h and exhibited a remarkable removal activity in acidic solution with a pH of 3. This condition efficiently degraded PFOS and PFOA by approximately 95.99 % and 96.89 %, respectively, through a photocatalytic reaction. This research presents a straightforward method to synthesize TiO₂/GO/PVA catalyst that influences persistent organic pollutants (POPs) under ultraviolet irradiation, which is of practical significance for environmental applications. © 2024 The Authors

关键词： Graphene oxide PFOA PFOS Photocatalytic Polyvinyl alcohol Titanium dioxide

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A Multi-Scale Approach to Assess water Quality and Evaporation in Agricultural Irrigation Canals

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SSRN 2024年

作者： Fender, Chloe L. Good, Stephen Garcia-Jaramillo, Manuel Department of Environmental and Molecular Toxicology Oregon State University CorvallisOR United States Department of Biological and Ecological Engineering Oregon State University CorvallisOR United States Water Resources Graduate Program Oregon State University CorvallisOR United States

Irrigation networks play a crucial role in water distribution and food production in agricultural systems and contribute to the overall economy. While studies have examined the effects of organic chemical pollutants, including pesticides, on crop and soil health, there is a lack of research on the overall composition and occurrence of organic chemical contaminants in irrigation water. To this point, there are currently no standardized methods for monitoring contaminants and assessing the transformation and potential toxicity of these compounds in irrigation water distribution systems. In this study, we used liquid chromatography high-resolution mass spectrometry to analyze the organic chemical composition of water samples from an irrigation canal and a river that serves as the source of water for the canal. We estimated the relative evaporation rate in the canal as a proxy for residence time by measuring the isotopic ratio of hydrogen and oxygen in the canal water with cavity ring-down spectroscopy. We assessed adverse effects of chemical contaminants in our samples by evaluating the collected water with a high-throughput zebrafish embryonic platform. We evaluated the hazard of annotated chemicals with an assessment tool developed by the US EPA. The canal showed a greater decrease in the abundance of organic contaminants relative to the river as we moved further from the source. Evaporation, a proxy for residence time, was evaluated in the canal and increased after a holding reservoir due to its higher surface area relative to the rest of the canal. This study improves our understanding of the occurrence and degradation of organic chemicals in irrigation networks compared with rivers, and how they may correlate with evaporation and distance. The approach implemented in this study can help build a standardized methodology for monitoring water quality and assessing the potential toxicity of organic contaminants in agricultural irrigation systems. © 2024, The Authors.

关键词： Organic chemicals

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A Multi-Scale Approach to Assess water Quality and Evaporation in Agricultural Irrigation Canals

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SSRN 2023年

作者： Fender, Chloe L. Good, Stephen P. Garcia-Jaramillo, Manuel Department of Environmental and Molecular Toxicology Oregon State University CorvallisOR United States Department of Biological and Ecological Engineering Oregon State University CorvallisOR United States Water Resources Graduate Program Oregon State University CorvallisOR United States

关键词： Organic chemicals

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Spatially differentiated life cycle assessment of Thailand's transport: The implications from country-specific factors and alternative technologies

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Sustainable Production and Consumption 2025年 57卷 319-340页

作者： Vitoon Chotanapund Shabbir H. Gheewala Vladimir Strezov Nazmul Huda Jitti Mungkalasiri Trakarn Prapaspongsa Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Nakhon Pathom Thailand School of Natural Sciences Faculty of Science and Engineering Macquarie University NSW 2109 Australia The Joint Graduate School of Energy and Environment (JGSEE) King Mongkut's University of Technology Thonburi Bangkok Thailand Center of Excellence on Energy Technology and Environment Ministry of Higher Education Science Research and Innovation Ministry of Education Bangkok Thailand School of Engineering Faculty of Science and Engineering Macquarie University NSW 2109 Australia Technology and Informatics Institute for Sustainability (TIIS) National Metal and Materials Technology Center (MTEC) National Science and Technology Development Agency (NSTDA) Pathum Thani Thailand

This study proposed country-specific characterisation factors (CFs) for Thailand by modifying the Thai Spatially Differentiated Life Cycle Impact Assessment (ThaiSD) method and introducing monetary conversion factors to express environmental impacts in Thai Baht. Five impact categories were fully parameterised, including fine particulate matter formation (PMF), human toxicity (both cancer and non-cancer) (HT c and HT nc ), freshwater ecotoxicity (FET), and water scarcity (WS). Other spatialised CFs were selected from regionalisation models in ReCiPe2016 and IMPACT World+. When comparing the use of country-specific CFs with global average, the impact scores for PMF, HT c , HT nc , FET, photochemical ozone formation and terrestrial acidification demonstrated notably different levels, ranging from ±25 to ±50 %. The developed method was then applied to assess environmental impacts and costs of Thailand's transport sector, encompassing freight and passenger transport across roadway, railway, waterway, and aviation. Climate change (CC) was significantly attributed to human health and ecosystem quality impacts, while the major contributor to resource scarcity impact was fossil resource scarcity (FS). In some scenarios, non-exhaust emissions, particularly from freight trucks, accounted for 40–60 % of the total PMF impacts. Environmental costs of freight and passenger transport in Thailand were 0.08–3.64 Thai Baht per tonne-kilometre and 0.01–0.81 Thai Baht per passenger-kilometre, respectively. Among transport modes, trains were found to be the most environmentally favourable option for both passenger and freight transport, while aviation had the highest environmental impact for freight transport. In contrast, passenger aviation had a comparable environmental burden to passenger cars due to optimised occupancy rates. Despite the efficiency of modern internal combustion engine vehicles (ICEVs), particularly Euro 5 and 6, employing blended biodiesel was less effective in comp

关键词： Life cycle assessment Thai Spatially Differentiated Life Cycle Impact Assessment Freight transport Passenger transport Transport technologies

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Rainfall frequency analysis using event-maximum rainfalls – An event-based mixture distribution modeling approach

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Weather and Climate Extremes 2024年 43卷

作者： Cheng, Ke-Sheng Chen, Bo-Yu Lin, Teng-Wei Nakamura, Kimihito Ruangrassamee, Piyatida Chikamori, Hidetaka Department of Bioenvironmental Systems Engineering National Taiwan University Taipei Taiwan Master Program in Statistics National Taiwan University Taipei Taiwan Graduate School of Agriculture Kyoto University Kyoto Japan Department of Water Resources Engineering Faculty of Engineering Chulalongkorn University Bangkok Thailand Department of Environmental Management Engineering Okayama University Okayama Japan

Rainfall frequency analysis, an essential work for water resources management, is often conducted by using the annual maximum rainfall series. For rainfall stations with short record lengths and outliers presence, the use of annual maximum series for rainfall frequency analysis may yield design rainfall estimates of higher uncertainties. Moreover, for regions with cyclostationary climate patterns, the annual maximum rainfalls may be caused by different prevalent storm types, which differ in terms of their occurrence frequency and storm rainfall characteristics. In this study, we propose a novel event-maximum-rainfall-based mixture distribution modeling approach for rainfall frequency analysis. By considering the event-maximum rainfalls of individual storm events, the sample size for parameter estimation increases, and the uncertainty of design rainfall estimates reduces. Mixture distribution modeling enables a thorough investigation of the contributing probabilities of different storm types to the annual maximum rainfall. Through rigorous stochastic simulation, we demonstrated the superiority of the proposed approach over the conventional annual maximum rainfall approach. The proposed approach was applied to four representative rainfall stations in Taiwan, and the results revealed that the proposed approach is more robust than the conventional annual maximum rainfall approach. The results provide insights into the contributions of individual storm types to the annual maximum rainfall. © 2023 The Authors

关键词： Annual maxima Event-maximum rainfalls Frequency analysis Mixture distribution Negative binomial distribution Poisson distribution

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Rainfall Frequency Analysis Using Event-Maximum Rainfalls – an Event-Based Mixture Distribution Modeling Approach

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SSRN 2023年

作者： Cheng, Ke-Sheng Chen, Bo-Yu Lin, Teng-Wei Nakamura, Kimihito Ruangrasamee, Piyatida Chikamori, Hidetaka Department of Bioenvironmental Systems Engineering National Taiwan University Taipei Taiwan Master Program in Statistics National Taiwan University Taipei Taiwan Graduate School of Agriculture Kyoto University Kyoto Japan Department of Water Resources Engineering Faculty of Engineering Chulalongkorn University Bangkok Thailand Department of Environmental Management Engineering Okayama University Okayama Japan

Rainfall frequency analysis, an essential work for water resources management, is often conducted by using the annual maximum rainfall series. For rainfall stations with short record lengths and outliers presence, the use of annual maximum series for rainfall frequency analysis may yield design rainfall estimates of higher uncertainties. Moreover, for regions with cyclostationary climate patterns, the annual maximum rainfalls may be caused by different prevalent storm types, which differ in terms of their occurrence frequency and storm rainfall characteristics. In this study, we propose an event-maximum-rainfall-based mixture distribution modeling approach for rainfall frequency analysis. By considering the event-maximum rainfalls of individual storm events, the sample size for parameter estimation increases, and the uncertainty of design rainfall estimates reduces. Mixture distribution modeling enables a thorough investigation of the contributing probabilities of different storm types to the annual maximum rainfall. Through rigorous stochastic simulation, we demonstrated the superiority of the proposed approach over the conventional annual-maximum-rainfall approach. The proposed approach was applied to four representative rainfall stations in Taiwan, and the results revealed that the proposed approach is more robust than the conventional annual-maximum-rainfall approach. The results provide insights into the contributions of individual storm types to the annual maximum rainfall. © 2023, The Authors. All rights reserved.

关键词： Poisson distribution

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Climate Change Projections of Soil Erosion in South America in the Xxi Century

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SSRN 2023年

作者： Riquetti, Nelva B. Mello, Carlos Rogerio Leandro, Diuliana Guzman, Jorge A. Water Resources Graduate Program Federal University of Pelotas Campus Porto Rua Gomes Carneiro 1 RS Pelotas96010-610 Brazil Water Resources Department Federal University of Lavras Campus Universitário CP 3037 MG Lavras37200-900 Brazil Department of Agricultural and Biological Engineering College of ACES University of Illinois at Urbana‐Champaign UrbanaIL61801 United States

Global climate projections indicate that continental South America (S.A.) can experience significant changes in soil erosion caused by water in the coming years due to changes in the precipitation spatial and temporal patterns, threatening food security and biodiversity, and impairing agroecosystems to provide services. This study aims to quantify future impacts on soil erosion in the S.A. provoked by changes in precipitation from climate change scenarios using the Revised Universal Soil Loss Equation (RUSLE). A 20 km spatial resolution of annual precipitation projected from the ensemble of four global climate models (BESM, CanESM2, HadGEM2-ES, and MIROC5 models) was used to assess impacts between 2010 and 2099, sliced every 30 years. The datasets were dynamically regionalized by the Eta/CPTEC model, and the RCPs 4.5 and 8.5 scenarios were selected to quantify rainfall erosivity and soil erosion rates. The projected average soil erosion was 37% above the present estimation (3.8 Mg ha-1 year-1) for S.A., reaching 5.2 Mg ha-1 year-1 over the 21st century. The projections indicate an increase in soil losses across the Andes Cordillera with less severe impacts on lowlands commonly used for crops and livestock. Contrastingly, soil erosion rates telatternd to decrease by the end of the century in northern S.A. due to the reduced precipitation projected by most of the climate models. Overall, the most significant projected erosion impacts of climate change were found for the last time slice (2071-2099) in the RCP 8.5 scenario. © 2023, The Authors. All rights reserved.

关键词： Erosion

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An Efficient Three-Factor Authenticated Key Agreement Technique Using FCM Under HC-IoT Architectures

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Computers, Materials & Continua 2022年第7期72卷 1373-1389页

作者： Chandrashekhar Meshram Agbotiname Lucky Imoize Sajjad Shaukat Jamal Parkash Tambare Adel R.Alharbi Iqtadar Hussain Department of Post Graduate Studies and Research in Mathematics Jayawanti Haksar Government Post-Graduation CollegeCollege of Chhindwara UniversityBetul460001M.P.India Department of Electrical and Electronics Engineering Faculty of EngineeringUniversity of LagosAkokaLagos100213Nigeria Department of Electrical Engineering and Information Technology Institute of Digital CommunicationRuhr University44801BochumGermany Department of Mathematics College of ScienceKing Khalid UniversityAbhaSaudi Arabia Water Resources&Applied Mathematics Research Lab Nagpur440027India College of Computing and Information Technology University of TabukTabuk71491Saudi Arabia Mathematics Program Department of MathematicsStatistics and PhysicsCollege of Arts and SciencesQatar University2713DohaQatar

The Human-Centered Internet of Things(HC-IoT)is fast becoming a hotbed of security and privacy *** users can establish a common session key through a trusted server over an open communication channel using a three-party authenticated key *** of the early authenticated key agreement systems relied on pairing,hashing,or modular exponentiation processes that are computationally intensive and *** order to address this problem,this paper offers a new three-party authenticated key agreement technique based on fractional chaotic *** new scheme uses fractional chaotic maps and supports the dynamic sensing of HC-IoT devices in the network architecture without a password *** projected security scheme utilized a hash function,which works well for the resource-limited HC-IoT *** results show that our new technique is resistant to password guessing attacks since it does not use a ***,our approach provides users with comprehensive privacy protection,ensuring that a user forgery attack causes no ***,our new technique offers better security features than the techniques currently available in the literature.

关键词： Three-party authenticated key agreement anonymity fractional chaotic maps Chebyshev polynomial password table human-centered internet of things(HC-IoT)

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Comparison of Taylor Galerkin and FTCS models for dam-break simulation 5

Comparison of Taylor Galerkin and FTCS models for dam-break ...

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5th International Seminar on Sustainable Urban Development, ISoSUD 2020

作者： Hafiyyan, Q. Adityawan, M.B. Harlan, D. Natakusumah, D.K. Magdalena, I. Graduate School of Civil Engineering Bandung Institute of Technology Jawa Barat Bandung Indonesia Center for Coastal and Marine Development Bandung Institute of Technology Jawa Barat Bandung Indonesia Study Program of Water Resouces Engineering and Management Bandung Institute of Technology Jawa Barat Bandung Indonesia Study Program of Water Resources Engineering Bandung Institute of Technology Jawa Barat Bandung Indonesia Industrial and Financial Mathematics Research Group Bandung Institute of Technology Jawa Barat Bandung Indonesia

The aim of this paper is to compare the ability of two numerical models to simulate two-dimensional dam-break flows. Dam-break modelling is important in reducing the high-risk of dam failure by determining the water flow movement and its effect on buildings downstream. In this study, the Taylor Galerkin and Forward Time Central Space method is presented to simulate 2-D dam-break flow. The Hansen filter is applied to both methods to reduce numerical instability oscillations in the model. The filters were used for each time step at each computing point. The model is verified by comparing the result simulation with numerical results from previous studies. The result show that Taylor Galerkin numerical scheme with Hansen filter is successful to simulate the problem of 2-D dam-break. Also, the Taylor Galerkin model has better results than the FTCS model. Studies like this are needed for mitigation efforts in the event of dam failure. © Published under licence by IOP Publishing Ltd.

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Health risk assessment of soil contamination with heavy metals in a child care center co-located in vicinity to small scale industrial area: Case study of Thailand

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Case Studies in Chemical and Environmental engineering 2024年 9卷

作者： Simatupang, Cathleen Ariella Santhaweesuk, Kanitthika Strezov, Vladimir Pongkiatkul, Prapat Boontanon, Narin Jindal, Ranjna Boontanon, Suwanna Kitpati Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Nakhon Pathom 73170 Thailand School of Natural Sciences Faculty of Science and Engineering Macquarie University 2109 NSW Australia Department of Environmental Engineering King Mongkut's University of Technology Thonburi Bangkok 10800 Thailand Faculty of Environment and Resource Studies Mahidol University Nakhon Pathom 73170 Thailand Environmental Engineering and Management Program Department of Energy Environment and Climate Change School of Environment and Resources Development Asian Institute of Technology Pathumthani 12120 Thailand Graduate School of Global Environmental Studies Kyoto University Yoshida Sakyo-Ku Kyoto 606-8501 Japan

Environmental impacts of small scale industries are still not well investigated, especially for estates where multiple small scale industries are clustered causing cumulative effects potentially impacting most vulnerable groups. This study aimed to investigate the concentrations of heavy metals (Mn, Fe, Ni, Cu, Pb, Al, Zn, and Cr) and the metalloid (As) in surface soils near the intensely active small-scale industrial area in Thailand, assess the contamination levels in the co-located child care center, and estimate potential human health risks from exposure to the heavy metals. Surface soil heavy metal(loid) elements were evaluated across a background area, area near main roads, a small-scale industrial area, and a child care centre. The concentrations of Al were found be the highest at all investigation sites, with the most elevated concentrations observed in the small-scale industrial area. The concentration of Pb in the industrial area reached 1176 mg/kg, exceeding the national standard and acceptable limit. Moreover, the contamination level for Cu, Pb, and Zn in the industrial area imply a considerable risk with enrichment factor EF > 40, and geo-accumulation index Igeo ≥5. Heavy metal levels (Ni, Cu, Pb) in the soil near the road and the child care center were similar, suggesting shared contamination sources. Conversely, Al, Zn, As, and Cr in the child care center had slightly higher concentrations than near the road but lower than the small-scale industrial area, indicating potential industrial influence on metal levels within the child care center. The principal component analysis showed Mn and Fe distributed in the background, while As, Pb, Ni, Cu, Al, Zn, and Cr accumulated in the small-scale industrial area. The findings indicate that small-scale industrial activities contribute to elevated levels of heavy metals in the soil, particularly within the child care center, posing significant ingestion risks, especially for children (HI > 1). Implementing conta

关键词： Children Contamination sources Environmental impact PCA Surface soil

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