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A review of biosensor for environmental monitoring: principle, application, and corresponding achievement of sustainable development goals

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Bioengineered 2023年第1期14卷 58-80页

作者： Chi-Wei Huang Chitsan Lin Minh Ky Nguyen Adnan Hussain Xuan-Thanh Bui Huu Hao Ngo Department of Marine Environmental Engineering National Kaohsiung University of Science and Technology Kaohsiung Taiwan. Ph.D. Program in Maritime Science and Technology College of Maritime National Kaohsiung University of Science and TechnologyPh.D. Program in Maritime Science and Technology Kaohsiung Taiwan. Ph. D. Program of Aquatic Science and Technology College of Hydrosphere Science National Kaohsiung University of Science and Technology Kaohsiung Taiwan. Department Water Science & Technology Key Laboratory of Advanced Waste Treatment Technology Ho Chi Minh City University of Technology (HCMUT) Vietnam National University Ho Chi Minh (VNU-HCM) Ho Chi Minh City Vietnam. Department Water Science & Technology Faculty of Environment & Natural Resources Ho Chi Minh City University of Technology (HCMUT) Ho Chi Minh City Vietnam. Department Water Science & Technology Centre for Technology in Water and Wastewater School of Civil and Environmental Engineering Faculty of Engineering and Information Technology University of Technology Sydney Sydney NSW Australia.

Human health/socioeconomic development is closely correlated to environmental pollution, highlighting the need to monitor contaminants in the real environment with reliable devices such as biosensors. Recently, variety of biosensors gained high attention and employed as application, in real-time, and cost-effective analytical tools for healthy environment. For continuous environmental monitoring, it is necessary for portable, cost-effective, quick, and flexible biosensing devices. These benefits of the biosensor strategy are related to the Sustainable Development Goals (SDGs) established by the United Nations (UN), especially with reference to clean water and sources of energy. However, the relationship between SDGs and biosensor application for environmental monitoring is not well understood. In addition, some limitations and challenges might hinder the biosensor application on environmental monitoring. Herein, we reviewed the different types of biosensors, principle and applications, and their correlation with SDG 6, 12, 13, 14, and 15 as a reference for related authorities and administrators to consider. In this review, biosensors for different pollutants such as heavy metals and organics were documented. The present study highlights the application of biosensor for achieving SDGs. Current advantages and future research aspects are summarized in this paper. ATP: Adenosine triphosphate; BOD: Biological oxygen demand; COD: Chemical oxygen demand; Cu-TCPP: Cu-porphyrin; DNA: Deoxyribonucleic acid; EDCs: Endocrine disrupting chemicals; EPA: U.S. environmental Protection Agency; Fc-HPNs: Ferrocene (Fc)-based hollow polymeric nanospheres; FeO@3D-GO: FeO@three-dimensional graphene oxide; GC: Gas chromatography; GCE: Glassy carbon electrode; GFP: Green fluorescent protein; GHGs: Greenhouse gases; HPLC: High performance liquid chromatography; ICP-MS: Inductively coupled plasma mass spectrometry; ITO: Indium tin oxide; LAS: Linear alkylbenzene sulfonate; : Laser-induced g

关键词： Biosensor bioavailability heavy metals organic pollutants sustainable development goals (SDGs)

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Peroxymonosulfate Activation by Ni-Fe (Hydr)Oxides Through Radical and Nonradical Pathways for Efficient Organic Pollutant Degradation

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SSRN 2022年

作者： Deng, Jia Chen, Weiguo Wu, Feng Dai, Yitao Dionysiou, Dionysios D. Huang, Li-Zhi School of Civil Engineering Wuhan University No. 8 East Lake South Road Wuhan430072 China State Key Laboratory of Water Resources and Hydropower Engineering Science Wuhan University 430072 China School of Resources and Environmental Science Wuhan University Wuhan China Department of Applied Chemistry University of Science and Technology of China Hefei230026 China Environmental Engineering and Science Program Department of Chemical and Environmental Engineering University of Cincinnati CincinnatiOH45221-0012 United States

Peroxymonosulfate (PMS)-based advanced oxidation processes have become promising water treatment technologies in recent years due to the generation ability of powerful oxidative radicals. The redox cycle between transitional metals in heterogeneous catalysis is essential for the continuous activation of PMS, which determines the removal efficiency of organic pollutants. In this work, we first prepared Fe3O4 using precipitation method under alkaline anoxic conditions and subsequently added Ni2+ aqueous solution to synthesize Ni-Fe (hydr)oxide catalysts. Ni-Fe (hydr)oxide catalysts show efficient PMS activation ability, causing the degradation of organic pollutants including trichloroethylene, perchloroethylene, bisphenol A, phenol, and tribromophenol. In Ni-Fe (hydr)oxides/PMS system, nonradical pathway is dominant at the initial stage of the reaction which generates SO5•− and indirectly produces 1O2. In this system, 1O2 and dissolved O2 together participate in the O2 cycling, •OH generation, and electron transfer involving the reduction of Ni(III). The formed Ni(II) reacted with PMS to generate strong oxidative •OH and SO4•− through radical pathway for pollutant degradation. The optimum Ni/Fe ratio of Ni-Fe (hydr)oxide catalysts under the studied conditions was 0.50. Ni-Fe (hydr)oxides show high reactivity and stability in real water matrices, demonstrating Ni-Fe (hydr)oxides are promising catalysts for PMS activation to degrade organic pollutants in contaminated water. © 2022, The Authors. All rights reserved.

关键词： Organic pollutants

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Unleashing the Power of Nature: Eco-Friendly Mussel-Byssus-Inspired Pbs/Pbat Fishing Gear for Biodegradation by Marine Microbes

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SSRN 2023年

作者： Hong, Yuri Yang, Ho-Sung Lee, Min Hee Kim, Sinyang Park, Sung Bae Hwang, Sung Yeon Park, Jeyoung Koo, Jun Mo Oh, Dongyeop Hwang, Dong Soo Gyeongsangbuk-do Pohang37673 Korea Republic of Ulsan44429 Korea Republic of Department of Plant & Environmental New Resources Graduate School of Biotechnology Kyung Hee University Gyeonggi-do 17104 Korea Republic of Department of Chemical and Biomolecular Engineering Sogang University Seoul04107 Korea Republic of Department of Organic Materials Engineering Chungnam National University Daejeon34134 Korea Republic of Department of Polymer Science and Engineering and Program in Environmental and Polymer Engineering Inha University Incheon22212 Korea Republic of

Abstract Abandoned, lost, and discarded fishing gear (ALDFG) poses global challenges for marine ecosystems as they destroy algal forests, the largest oceanic carbon dioxide sinks. Biodegradable polybutylene succinate (PBS), which has a tensile toughness similar to that of nylon, has been suggested as a potential fishing-gear material. However, its slow degradation in the marine environment and limited draping characteristics need to be addressed before it can be used in environmentally friendly fishing gear. Inspired by the mussel byssus, a mussel-thread-like holdfast known for its stiff yet extensible mechanical properties, we developed fishing gear using a mussel-byssus-mimetic fiber (artificial byssus, AB) structure. The AB was composed of poly(butylene adipate-co-butylene terephthalate) (PBAT) fibers with favorable draping characteristics coated with mechanically resilient and PBS, which demonstrated sufficient toughness and draping properties for use in fishing gear. The AB may serve as fishing-gear material capable of mitigating ALDFG issues, given its marine degradability by microbial strains that degrade PBS and PBAT. Furthermore, it could serve as a substrate for ocean afforestation, given the improved settlement and growth of seaweed spores (Pyropia yezoensis) on AB. Overall, AB-based fishing gear is expected to enhance macroalgal forest conservation and expansion, and facilitate marine carbon capture through marine afforestation. © 2023, The Authors. All rights reserved.

关键词： Butenes

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Relationship between nitrate, heavy metal, and sterols contents in Japanese agricultural soils with risk of groundwater pollution

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Chemosphere 2024年 361卷 142335页

作者： Nakagawa, Kei Islam, M. Shahidul Shah, Syed Shabbar Hussain Li, Zhuolin Takao, Yuji Berndtsson, Ronny Institute of Integrated Science and Technology Nagasaki University 1-14 Bunkyo-machi Nagasaki852-8521 Japan Graduate School of Fisheries and Environmental Sciences Nagasaki University 1-14 Bunkyo-machi Nagasaki852-8521 Japan Department of Chemistry Jashore University of Science and Technology Jashore7408 Bangladesh Division of Water Resources Engineering & Centre for Advanced Middle Eastern Studies Lund University Box 118 LundSE-221 00 Sweden

In Japanese agricultural lands, nitrate-nitrogen contamination of soil and groundwater often occurs due to the application of livestock excrements and compost. Therefore, rural soils in Japan were sampled and analyzed for nitrate-nitrogen leaching, heavy metal content, and sterols associated with livestock excrement and compost to calculate contamination risk indicators. The results were analyzed using self-organizing maps and cluster analysis. Nitrate-nitrogen content using water extraction was detected in most of the sampled soils. In addition, many samples from areas that were already severely contaminated with nitrate-nitrogen showed particularly high concentrations. Coprostanol, an indicator of fecal contamination, was detected in more than half of the samples. The main source of nitrate-nitrogen contamination in these areas is livestock excrement and compost. Self-organization maps showed that areas with high nitrate-nitrogen contamination also corresponded to areas with high copper and zinc soil contents. The self-organization maps and cluster analysis resulted in five clusters: a nitrate-contaminated group mainly originating from livestock excrement and compost, a heavy metal-contaminated group, a general group, a nitrate-contaminated group mainly originating from chemical fertilizers, and a contaminated group with potentially hazardous substances requiring attention. Authorities and decision-makers can use the results to prioritize areas requiring remediation. © 2024 The Authors

关键词： Soils

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Microwave-assisted hydrothermal synthesis of carbonated apatite with calcium and phosphate resources derived from green mussel shell and bovine bone wastes

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environmental Advances 2024年 17卷

作者： Muryanto, Stefanus Prihanto, Antonius Pusparizkita, Yustina M. Ismail, Rifky Jamari, J. Bayuseno, Athanasius P. Show, Pau Loke Department of Mechanical Engineering Diponegoro University Semarang Indonesia Department of Mechanical Engineering Universitas Negeri Surabaya Indonesia Department of Chemical Engineering UNTAG University in Semarang Indonesia Vocational Chemical Engineering Program Catholic Polytechnic Mangunwijaya Semarang Indonesia Department of Environmental Engineering Diponegoro University Semarang Indonesia Department of Chemical Engineering Khalifa University Abu Dhabi United Arab Emirates Zhejiang Provincial Key Laboratory for Subtropical Water Environment and Marine Biological Resources Protection Wenzhou University Wenzhou China Department of Chemical and Environmental Engineering Faculty of Science and Engineering University of Nottingham Malaysia Semenyih Malaysia Department of Sustainable Engineering Saveetha School of Engineering SIMATS Chennai India

resources recovery of calcium and phosphates from respective green mussel shells and bovine bones by calcination and chemically extracting are viable precursors for carbonate-rich apatite biomedical material applications. Because of their high osteoconductivity, carbonate-rich apatite bioceramics are being studied intensively for synthetic bone transplants. In the study, powder processing routes of calcination and following chemical dissolution in MgCl₂ and H₂SO₄ were each for recovering calcium of mussel shells and phosphate of bovine bones yielding a crystal-forming solution feedstock for use in microwave-irradiated synthesis. FTIR spectra and XRD patterns validated the crystallinity and phase identification for as-synthesized powders. As a result, the presence of CO₃, PO₄^3-, and OH- bands in carbonate-calcium phosphate complexes were present in FTIR spectra. According to the XRD Rietveld method, the as-synthesized powder product contained brushite, carbonated hydroxyapatite (CHA), calcite, and gypsum. The recoverable CHA crystallites' size was 40 nm. This present study demonstrated that microwave irradiation synthesis of CHA powder with calcium and phosphates derived from mussel shells and bovine bones is the potential to yield a large amount of CHA for bioceramics and would aid in the design of a powder processing step for preparing the CHA powder precursor in biomedical applications. © 2024

关键词： Calcination Carbonate-rich apatite Chemical dissolution Hydroxyapatite Microwave-irradiated synthesis

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Remediation of soil and groundwater contaminated with organic chemicals using stabilized nanoparticles: Lessons from the past two decades

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Frontiers of environmental Science & engineering 2020年第5期14卷 83-102页

作者： Zhengqing Cai Xiao Zhao Jun Duan Dongye Zhao Zhi Dang Zhang Lin National Engineering Lab for High-concentration Refractory Organic Wastewater East China University of Science and TechnologyShanghai 200237China Shanghai Institute of Pollution Control and Ecological Security Shanghai 200092China College of Water Resources&Civil Engineering China Agricultural UniversityBeijing 100083China Environmental Engineering Program Department of Civil EngineeringAuburn UniversityAuburnAL 36849USA School of Environment and Energy South China University of TechnologyGuangzhou 510006China

Due to improved soil deliverability and high reactivity,stabilized nanoparticles have been studied for nearly two decades for in situ remediation of soil and groundwater contaminated with organic *** large amounts of bench-and field-scale experimental data have demonstrated the potential of the innovative technology,extensive research results have also unveiled various merits and constraints associated different soil characteristics,types of nanoparticles and particle stabilization ***,this work aims to critically overview the fundamental principles on particle stabilization,and the evolution and some recent developments of stabilized nanoparticles for degradation of organic contaminants in soil and *** specific objectives are to:1)overview fundamental mechanisms in nanoparticle stabilization;2)summarize key applications of stabilized nanoparticles for in situ remediation of soil and groundwater contaminated by legacy and emerging organic chemicals;3)update the latest knowledge on the transport and fate of stabilized nanoparticles;4)examine the merits and constraints of stabilized nanoparticles in environmental remediation applications;and 5)identify the knowledge gaps and furore research needs pertaining to stabilized nanoparticles for remediation of contaminated soil and *** instructions of this invited special issue,this review is focused on contributions from our group(one of the pioneers in the subject field),which,however,is supplemented by important relevant works by *** knowledge gained is expected to further advance the science and technology in the environmental applications of stabilized nanoparticles.

关键词： Stabilized nanoparticle In-situ remediation Organic contaminant Soil remediation Groundwater Fate and transport

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Implications of technological improvement and circular agriculture on environmental sustainability of sugarcane production

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Cleaner environmental Systems 2025年 18卷

作者： Aakriti Deuja Min Hein Khant Thapat Silalertruksa Shabbir H. Gheewala Trakarn Prapaspongsa Graduate Program in Environmental and Water Resources Engineering Department of Civil and Environmental Engineering Faculty of Engineering Mahidol University Nakhon Pathom Thailand Department of Environmental Engineering Faculty of Engineering King Mongkut's University of Technology Thonburi Bangkok Thailand The Joint Graduate School of Energy and Environment King Mongkut's University of Technology Thonburi Bangkok Thailand Centre of Excellence on Energy Technology and Environment Ministry of Higher Education Science Research and Innovation Bangkok Thailand

The spatially differentiated environmental impacts and associated costs of technological improvement and circular agricultural practices in sugarcane production were assessed. Analysis of the cause-effect relationship between the key processes and substances each helped develop alternative scenarios for impact reduction. PM 2.5 emissions contributed to 92 % of the total human health impacts from open burning of field residues. Freshwater ecotoxicity, mainly due to ametryn emissions from pesticide application, contributed to 47 % of the total damage to the ecosystem. The environmental costs were 116 % higher than the value of sugarcane production, signifying the critical importance of adopting alternative pathways that provide economic benefits from environmental cost reduction compared to the production value. Scenarios considering green cane harvesting and waste management approaches demonstrated high potential for total impact reduction of 99 % and 97 %, respectively, and economic gains of 202 and 225 billion THB, respectively (5.76 and 6.42 billion USD, respectively). The economic benefits of waste utilization were 137 % higher than the value of sugarcane production, demonstrating the potential benefits of product substitution to help mitigate impacts. The core findings highlight the significance of the PM 2.5 impact-related external costs and underscore the benefits of adopting green cane harvesting in conjunction with on-field waste utilization to mitigate the impact of open burning and produce value-added products. Technological improvement and circular agricultural practices coupled with valuation of spatially differentiated impacts can provide useful and more accurate information to policymakers, to prioritize the implementation of mitigation strategies for enhancing the environmental sustainability of sugarcane production.

关键词： Life cycle assessment On-site and supply chain emissions Human health Ecosystem environmental cost environmental sustainability

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Adsorption of organic and inorganic pollutants onto biochars: Challenges, operating conditions, and mechanisms

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Bioresource Technology Reports 2021年 15卷

作者： Barquilha, Carlos E.R. Braga, Maria C.B. Postgraduate Program in Water Resources and Environmental Engineering Parana Federal University Av. Cel. Francisco H. dos Santos 100 CuritibaPR CEP81530-000 Brazil

The presence of toxic substances in the environment has increased due to population growth, urbanization, industrialization, as well as changes in people's lifestyles. Among many technologies, adsorption has proven to be an effective and inexpensive technique for water and wastewater treatment. Biochar has been identified as a promising and low-cost material, which can be produced from various carbonaceous materials with different origins, compositions, and processing methods. Consequently, the interaction between biochars and adsorbate species is not simple and may involve different adsorption mechanisms, such as van der Waals forces, electrostatic interactions, surface complexation, ion-exchange, hydrophobic interactions, π-interactions, co-precipitation, partition, and pore-filling. In addition, many operating conditions can affect the performance of adsorption processes. However, the development of biochars as competitive adsorbent materials depends on standardization, continuous-supply, application, and regulation. Thus, this paper discusses the challenges, the operating conditions, and the adsorption mechanisms to remove organic and inorganic micropollutants using biochar. © 2021 Elsevier Ltd

关键词： Adsorption

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Removal of RNA Viruses from Swine Wastewater Using Anaerobic Membrane Bioreactor: Performance and Mechanisms

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SSRN 2023年

作者： Li, Yu Wu, Baolei Zhai, Xuanyu Li, Qian Fan, Chenlong Li, Yu-You Sano, Daisuke Chen, Rong Key Lab of Environmental Engineering Shaanxi Province Xi'an University of Architecture and Technology No.13 Yanta Road Xi’an710055 China International S&T Cooperation Center for Urban Alternative Water Resources Development Key Laboratory of Northwest Water Resource Environment and Ecology MOE Xi'an University of Architecture and Technology No.13 Yanta Road Xi’an710055 China Vanke School of Public Health Tsinghua University Beijing100008 China Department of Civil and Environmental Engineering Graduate School of Engineering Tohoku University 6-6-06 Aza-Aoba Aramaki Aoba-ku Miyagi Sendai980-8579 Japan

The effective removal of viruses from swine wastewater using anaerobic membrane bioreactor (AnMBR) is vital to ecological safety. However, most studies have focused only on disinfectants, whereas the capabilities of the treatment process have not been investigated. In this study, the performance and mechanism of an AnMBR in the removal of porcine hepatitis E virus (HEV), porcine kobuvirus (PKoV), porcine epidemic diarrhea virus (PEDV), and transmissible gastroenteritis coronavirus (TGEV) are systematically investigated. The results show that the AnMBR effectively removes the four viruses, with average removal efficiencies of 1.62, 3.05, 2.41, and 1.34 log for HEV, PKoV, PEDV and TGEV, respectively. Biomass adsorption contributes primarily to the total virus removal in the initial stage of reactor operation, with contributions to HEV and PKoV removal exceeding 71.7% and 68.2%, respectively. When the membrane is fouled, membrane rejection dominated virus removal. The membrane rejection contribution test shows the significant contribution of membrane pore foulants (23%–76%). Correlation analysis shows that the surface characteristics and size differences of the four viruses contribute primarily to their different effects on biomass adsorption and membrane rejection. This study provides technical guidance for viral removal during the treatment of high-concentration swine wastewater using an AnMBR. © 2023, The Authors. All rights reserved.

关键词： Adsorption

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Effectiveness of different biochars in remediating a salt-affected Luvisol in Northeast Brazil

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Biochar 2021年第2期3卷 149-159页

作者： Wallace Melo dos Santos Maria Isidoria Silva Gonzaga JoséAiron da Silva AndréQuintão de Almeida JoséCarlos de Jesus Santos Thomas Antonio Silva Gonzaga Idamar da Silva Lima EloáMoura Araújo Water Resources Graduate Program Federal University of SergipeSão CristóvãoSE 49100‑000Brazil Agronomy Department Federal University of SergipeSão CristóvãoSE 49100‑000Brazil Agriculture Engineering Department Federal University of SergipeSão CristóvãoSE 49100‑000Brazil University of Notre Dame Notre DameIN 46556USA Soils and Agricultural Engineering Department Federal University of ParanáCuritibaPR 80060‑000Brazil

Biochar has been proposed as a soil amendment to reclaim salt-affected ***,the evaluation of the different biochar types in these soils is essential due to the significant variation among biochar *** this study,biochars from sugarcane bagasse(SB),orange bagasse(OB),and corncob(CB)were applied alone and in the presence of gypsum(G)to test their potential to remediate a highly degraded saline-sodic soil in Brazil´s Northeast *** that,we conducted a laboratory column-leaching experiment and a greenhouse *** the column-leaching test,we analyzed the sodium adsorption ratio(SAR),the electrical conductivity of the saturation extract(ECe),the concentrations of major ions,and the exchangeable sodium percentage(ESP).Maize plants were grown in the leached soil in a ***-and corncob-derived biochars were more efficient than gypsum in reducing the soil salinity,bringing the indicators below threshold values,and optimizing soil reclamation *** ECe,SAR,and ESP were reduced to 3.42 dS m−1,1.64(mmolc dm−3)0.5 and 4.86%,respectively,in the SB treatment;and to 3.19 dS m−1,0.88(mmolc dm−3)0.5 and 2.53%,respectively,in the CB *** bagasse biochar did not effectively reduce the salinity *** biochar treatments improved seed germination and plant *** SB,CB,SBG,and CBG treatments increased plant height(478–558%),shoot mass(783–983%),and root mass(386–500%),***,the application of SB and CB is an effective alternative to remediate saline-sodic soils and to reduce the impact of soil salinity in the environment.

关键词： Biochar Soil remediation Soil salinity Corn growth

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