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2023 Conference on Lasers and Electro-Optics, CLEO 2023

作者： Overvig, Adam C. Kasahara, Y. Alu, Andrea Photonics Initiative Advanced Science Research Center City University of New York New YorkNY10031 United States Department of Electrical and Computer Engineering The University of Texas at Austin AustinTX78712 United States Physics Program Graduate Center of the City University of New York New YorkNY10016 United States

We theoretically propose and experimentally demonstrate nonlocal metasurfaces rationally designed using symmetry-breaking principles to manipulate the optical wavefront with a geometric phase selective to custom ellip...

ISBN: (纸本)9781957171258

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Advanced TiO2/Al2O3 Bilayer ALD Coatings for Improved Lithium-Rich Layered Oxide Electrodes

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ACS Applied Materials and Interfaces 2024年第10期16卷 13029-13040页

作者： Chen, Wei-Ming Hsieh, Hsin-Yu Wu, Dong-Ze Tang, Horng-Yi Chang-Liao, Kuei-Shu Chi, Po-Wei Wu, Phillip M. Wu, Maw-Kuen Institute of Physics Academia Sinica 128 Section 2 Academia Road Taipei11529 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University 128 Section 2 Academia Road Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu300044 Taiwan Graduate Institute of Energy and Sustainability Technology National Taiwan University of Science and Technology 43 Keelung Road Sec 4 Taipei10607 Taiwan Department of Applied Chemistry National Chi Nan University 1 University Road Puli Nantou545301 Taiwan College of Science National Chung Hsing University 145 Xingda Rd. South Dist. Taichung City402 Taiwan

Surface modification is a highly effective strategy for addressing issues in lithium-rich layered oxide (LLO) cathodes, including phase transformation, particle cracking, oxygen gas release, and transition-metal ion dissolution. Existing single-/double-layer coating strategies face drawbacks such as poor component contact and complexity. Herein, we present the results of a low-temperature atomic layer deposition (ALD) process for creating a TiO2/Al2O3 bilayer on composite cathodes made of AS200 (Li1.08Ni0.34Co0.08Mn0.5O2). Electrochemical analysis demonstrates that TiO2/Al2O3-coated LLO electrodes exhibit improved discharge capacities and enhanced capacity retention compared with uncoated samples. The TAA-5/AS200 bilayer-coated electrode, in particular, demonstrates exceptional capacity retention (∼90.4%) and a specific discharge capacity of 146 mAh g-1 after 100 cycles at 1C within the voltage range of 2.2 to 4.6 V. The coated electrodes also show reduced voltage decay, lower surface film resistance, and improved interfacial charge transfer resistances, contributing to enhanced stability. The ALD-deposited TiO2/Al2O3 bilayer coatings exhibit promising potential for advancing the electrochemical performance of lithium-rich layered oxide cathodes in lithium-ion batteries. © 2024 The Authors. Published by American Chemical Society.

关键词： Cathodes

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Backcasting Perspectives on Services of Future Quantum Internet

Backcasting Perspectives on Services of Future Quantum Inter...

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Quantum Software (QSW), IEEE International Conference on

作者： Shota Nagayama Toshihiko Sasaki Akihito Soeda Mercari R4D Mercari Inc Tokyo Japan Graduate School of Media and Governance Keio University Fujisawa Japan Department of Applied Physics Graduate School of Engineering The University of Tokyo Tokyo Japan Principles of Informatics Research Division National Institute of Informatics Tokyo Japan Informatics Program SOKENDAI (The Graduate University for Advanced Studies) Tokyo Japan Department of Physics Graduate School of Science The University of Tokyo Tokyo Japan

ISBN: (数字)9798350368475

ISBN: (纸本)9798350368482

A quantum internet is an emerging quantum information technology, possibly becoming a pinnacle of wide-area distributed system allowed under the laws of physics. The current expansion of quantum technologies would lead to innumerable types of quantum systems, composed of various kinds of quantum devices connected by a dedicated quantum network. However, the (inter)connectivity offered by a quantum internet should ideally be agnostic of the technologies used by each component system. Furthermore, concurrent progresses of the quantum technologies complicate the task of defining what a quantum internet is. In this paper, we adopt a backcasting approach to elucidate what a quantum internet should be. We begin by discussing what we believe to be the requirements of an ultimate distributed quantum system, from which we explain what role a quantum internet would play in achieving this ultimate system. We then lead to more practical requirements on a quantum internet, considering the known and expected constraints in designing a quantum internet. We also organize and categorize the relationship among known quantum network technologies and services relevant to a quantum internet. We hope this document to lay a common ground for all the key stakeholders of a quantum internet, including researchers, industrial enterprises, and policy makers and regulators.

关键词： Quantum system Protocols Quantum mechanics Transportation Logic gates Internet Quantum networks

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Nanoslot-Induced Ultrastrong Phonon-Photon and Phonon-Phonon Coupling in Hybrid Organic-Inorganic Perovskites 16

Nanoslot-Induced Ultrastrong Phonon-Photon and Phonon-Phonon...

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16th Pacific Rim Conference on Lasers and Electro-Optics, CLEO-PR 2024

作者： Kim, Dasom Hou, Jin Lee, Geon Agrawal, Ayush Kim, Sunghwan Zhang, Hao Bao, Di Baydin, Andrey Wu, Wenjing Tay, Fuyang Huang, Shengxi Hagenmüller, Daivd Chia, Elbert E. M. Kim, Dai-Sik Seo, Minah Mohite, Aditya D. Kono, Junichiro Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Electrical and Computer Engineering Rice University HoustonTX77005 United States Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Sensor System Research Center Korea Institute of Science and Technology Seoul02792 Korea Republic of Department of Physics and Astronomy Seoul National University Seoul08826 Korea Republic of Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Ulsan44919 Korea Republic of Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University 637371 Singapore Smalley-Curl Institute Rice University HoustonTX77005 United States Université de Strasbourg Cnrs Strasbourg67000 France KU-KIST Graduate School of Converging Science and Technology Korea University Seoul02841 Korea Republic of Department of Physics and Astronomy Rice University HoustonTX77005 United States

Methods for harnessing vibrational states are desired for phonon-based technologies. We realized ultrastrong coupling of two phonon modes in perovskite materials induced by ultrastrong coupling with a common photonic ... 详细信息

ISBN: (纸本)9798350372076

关键词： Organic-inorganic materials

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Physically consistent gravitational waveform for capturing beyond general relativity effects in the compact object merger phase

arXiv

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arXiv 2023年

作者： Watarai, Daiki Nishizawa, Atsushi Cannon, Kipp Graduate School of Science The University of Tokyo Tokyo113-0033 Japan Graduate School of Science The University of Tokyo Tokyo113-0033 Japan Physics Program Graduate School of Advanced Science and Engineering Hiroshima University Higashi-Hiroshima Hiroshima739-8526 Japan

The merger phase of compact binary coalescences is the strongest gravity regime that can be observed. To test the validity of general relativity (GR) in strong gravitational fields, we propose a gravitational waveform parameterized for deviations from GR in the dynamical and nonlinear regime of gravity. Our fundamental idea is that perturbative modifications to a GR waveform can capture possible deviations in the merger phase that are difficult to model in a specific theory of gravity. One of notable points is that our waveform is physically consistent in the sense that the additional radiative losses of energy and angular momentum associated with beyond-GR modifications are included. Our prescription to ensure physical consistency in the whole coalescence process is expected to be applicable to any deviation from the standard model of compact binary coalescence, such as the extended models of gravity or the environmental effects of compact objects, as long as perturbative modifications are considered. Based on the Fisher analysis and the compatibility with Einstein-dilaton Gauss-Bonnet waveforms, we show that our parameterization is a physically-consistent minimal one that captures the deviations in the nonlinear regime. Copyright © 2023, The Authors. All rights reserved.

关键词： Merging

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Origin of nonlinear photocurrents in chiral multifold semimetal CoSi unveiled by terahertz emission spectroscopy

arXiv

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arXiv 2024年

作者： Chan, Yao-Jui Faizanuddin, Syed Mohammed Kalaivanan, Raju Raman, Sankar Lin, Hsin Kar, Uddipta Singh, Akhilesh Kr. Lee, Wei-Li Vankayala, Ranganayakulu K. Ou, Min-Nan Wen, Yu-Chieh Institute of Physics Academia Sinica Taipei11529 Taiwan Taiwan International Graduate Program Academia Sinica Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu300044 Taiwan

Spectroscopic identification of distinct nonlinear photocurrents unveils quantum geometric properties of electron wavefunctions and the momentum-space topological structures. This is especially interesting, but still puzzling, for chiral topological semimetals with possibilities of hosting giant quantized circular photogalvanic effect. Here we report a comprehensive terahertz (THz) emission spectroscopic analysis of nonlinear photoconductivity of chiral multifold CoSi at 0.26 ~ 1 eV. We find a large linear shift conductivity (17 μA/V2), and confirm a giant injection conductivity (167 μA/V2) as a consequence of strongly interfered non-quantized contributions from the vicinity of multifold nodes with opposite chiralities. The bulk injection current excited by the pump field with a complex wavevector is shown to carry both longitudinal and transverse components. Symmetry analyses further unveil weak nonlocal photon drag effect in addition to the photogalvanic effect. This work not only highlights chiral transition metal monosilicides for mid-infrared photovoltaic applications via various nonlinear optical channels, but also consolidates the THz spectroscopy for quantitative photovoltaic research. Copyright © 2024, The Authors. All rights reserved.

关键词： Terahertz spectroscopy

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Observation of Photonic Chiral Flatbands

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Physical Review Letters 2025年第10期134卷 103801-103801页

作者： Minho Choi Andrea Alù Arka Majumdar Department of Electrical and Computer Engineering University of Washington Seattle Washington 98195 USA Photonics Initiative Advanced Science Research Center City University of New York New York New York 10031 USA and Physics Program Graduate Center City University of New York New York New York 10031 USA Department of Electrical and Computer Engineering University of Washington Seattle Washington 98195 USA and Department of Physics University of Washington Seattle Washington 98195 USA

Distinct selectivity to the spin angular momenta of photons has garnered significant attention in recent years, for its relevance in basic science and for imaging and sensing applications. While nonlocal metasurfaces with strong chiral responses to the incident light have been reported, these responses are typically limited to a narrow range of incident angles. In this study, we demonstrate a nonlocal metasurface that showcases strong chirality, characterized by circular dichroism (∼0.6), over a wide range of incident angles ±5°. Its quality factor, circular dichroism and resonant frequency can be optimized by design. These findings pave the way to further advance the development of valley-selective optical cavities and augmented reality applications.

关键词： Natural frequencies

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Third-Order Optical Properties of Ag Nanocubes and Ag-Au Hollow Nanostructures Investigated by Femtosecond Z-Scan Measurements

SSRN

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SSRN 2024年

作者： Sousa, Claudevan A. Melo, Antonio F.A.A. Silva, Nefe J.B. Silva, Tânia Patrícia Silva E. Viana, Bartolomeu C. Santos, Francisco Eroni P. Garcia, Hans Department of Physics UFPI - Universidade Federal do Piauí PI Teresina64049-550 Brazil Materials Engineering Graduate Program Federal Institute of Education Science and Technology of Piauí Central Campus PI Teresina64000-040 Brazil Interdisciplinary Laboratory for Advanced Materials BioMatLab group Materials Science & Engineering Graduate Program UFPI - Universidade Federal do Piauí PI Teresina64049-550 Brazil

In this work, we reported experimental investigations on third-order optical properties of aqueous colloidal dispersions of silver nanocubes (Ag-NCs) and Ag-Au hollow nanostructures. The hollow bimetallic are nanoboxes, that were synthesized by galvanic substitution using silver nanocubes as templates, inserting silver with gold in molar ratios of 1.5 and 3.0 mL. This process adjusted tuning the Surface Plasmon Resonance (SPR) compared to the original Ag-NCs nanocubes. Femtosecond Z-scan measurements performed at 1040 nm, 350fs and laser intensities from 99.7 - 279 GW/cm2 shows negative nonlinear refraction for both nanocube and nanoboxes colloids, attributed to hot electron generation. Solvent effects are simultaneously suppressed of the nanostructures. On the other hand, the non-linear absorption observed for bimetallic nanoboxes shows the presence of saturated absorption (SA), but the Ag-NCs do not show a non-linear absorption signal. Therefore, our experimental results provide a reliable reference for the application of these bimetallic nanostructures as active media in nonlinear photonic devices. © 2024, The Authors. All rights reserved.

关键词： Surface plasmon resonance

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Cofilin-Mediated Filament Softening and Crosslinking Counterbalance to Enhance Actin Network Flexibility

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Physical Review Letters 2024年第21期133卷 218402-218402页

作者： Zachary Gao Sun Michael Murrell Department of Physics Yale University 217 Prospect Street New Haven Connecticut 06511 USA Systems Biology Institute Yale University West Haven Connecticut 06516 USA Integrated Graduate Program in Physical and Engineering Biology Yale University New Haven Connecticut 06520 USA Department of Biomedical Engineering Yale University New Haven Connecticut 06511 USA

Filamentous-actin (F-actin) crosslinking within the cell cytoskeleton mediates the transmission of mechanical forces, enabling changes in cell shape, as occurs during cell division and cell migration. Crosslinking by actin binding proteins (ABPs) generally increases the connectivity of the F-actin network, but also increases network rigidity. As a result, there is a narrow range in the concentration of crosslinker protein at which F-actin networks are both connected and labile. Another ABP, cofilin, severs F-actin filaments at high pH through increasing their bending flexibility and concentrating mechanical stress, inducing fragmentation. By contrast, at lower pH, cofilin increases filament flexibility yet does not sever. Instead, it forms disulfide bonds, which crosslink F-actin into bundles, and bundles into networks. Here, we combine light microscopy and rheology to determine the impact of two potentially opposing effects on the mechanics of F-actin networks—increased flexibility at the filament level, and increased connectivity at the network level. Indeed, by linear rheology, we find that these mechanisms are counterbalanced, such that cofilactin network moduli are only weakly dependent on cofilin concentration over a broad range, in contrast to the dramatic stiffening that occurs with F-actin crosslinking protein. Further, by nonlinear rheology, the network stiffens at a higher stress than crosslinking protein, indicative of a broader range in which the material remains flexible. These results may enable F-actin networks to increase connectivity without heavy penalties to rigidity, and thus provide a new route to modulating active polymer mechanics unseen using traditional F-actin accessory proteins.

关键词： Biomimetic & bio-inspired materials Biomolecular self-assembly Living matter & active matter Persistence length Polymer entanglement Rheological properties Rheology Shear deformation Strain

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In vivo Detection of NO using Photonic Microring Resonators

In vivo Detection of NO using Photonic Microring Resonators

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CLEO: Science and Innovations, S and I 2022

作者： Hassan, Sakib Zhao, Xuan Schreib, Christian C. Duret, Guillaume Veiseh, Omid Robinson, Jacob T. Electrical & Computer Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley-Curl Institute Rice University HoustonTX77005 United States Department of Bioengineering Rice University HoustonTX77005 United States

Here we show how photonic microring resonators enable real-time detection of Nitric Oxide (NO) in vivo, which is critical for physiological monitoring particularly during the wound healing process. © Optica Publi... 详细信息

ISBN: (纸本)9781557528209

关键词： Nitric oxide

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