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arXiv 2024年

作者： Zhang, Bo-Wen Qiu, Xi-Yang Ma, Yicheng Hu, Qingmei Fitó-Parera, Aina Kohata, Ikuma Feng, Ya Zheng, Yongjia Zhang, Chiyu Matsuo, Yutaka Wang, YuHuang Chiashi, Shohei Otsuka, Keigo Xiang, Rong Levshov, Dmitry I. Cambré, Sofie Wenseleers, Wim Rotkin, Slava V. Maruyama, Shigeo Department of Mechanical Engineering The University of Tokyo Tokyo113-8656 Japan State Key Laboratory of Fluid Power and Mechatronic Systems School of Mechanical Engineering Zhejiang University Hangzhou310027 China Theory and Spectroscopy of Molecules and Materials Department of Physics University of Antwerp Antwerp2610 Belgium Key Laboratory of Ocean Energy Utilization and Energy Conservation of Ministry of Education School of Energy and Power Engineering Dalian University of Technology Liaoning 116024 China Department of Chemistry and Biochemistry Chemical Physics Program Maryland Nano Center University of Maryland College ParkMD20742 United States Department of Chemical Systems Engineering Graduate School of Engineering Nagoya University Nagoya464-8603 Japan Institute of Materials Innovation Institutes for Future Society Nagoya University Nagoya464-8603 Japan Theory and Spectroscopy of Molecules and Materials Department of Chemistry University of Antwerp Antwerp2610 Belgium Nanostructured and Organic Optical and Electronic Materials Department of Physics University of Antwerp Antwerp2610 Belgium Materials Research Institute Department of Engineering Science & Mechanics The Pennsylvania State University University ParkPA16802 United States

Carbyne, a one-dimensional (1D) carbon allotrope with alternating triple and single bonds, has the highest known mechanical strength but is unstable to bending, limiting synthesis to short linear chains. Encapsulation within carbon nanotubes (CNTs) stabilizes carbyne, forming confined carbyne (CC), thus enabling further research concerning attractive 1D physics and materials properties of carbyne. While CC has been synthesized in multi-walled CNTs (MWCNTs) using the arc-discharge method and in double-walled CNTs (DWCNTs) via high-temperature high-vacuum (HTHV) method, synthesis in single-walled CNTs (SWCNTs) has been challenging due to their fragility under such conditions. In this work, we report a low-temperature method to synthesize CC inside SWCNTs (CC@SWCNT). By annealing SWCNTs containing ammonium deoxycholate (ADC) at 400°C, ADC is converted into CC without damaging the SWCNTs. Raman spectroscopy revealed a strong CC phonon (CC-mode) peak at 1860–1870 cm-1, much stronger than the SWCNT G-band peak, confirming a high fraction of CC in the resulting material. The Raman mapping result showed the uniformity of the CC-mode signal across the entire film sample, proving the high efficiency of this method in synthesizing CC in every SWCNT of appropriate size. Notably, the CC-mode peaks of CC@SWCNT (above 1860 cm-1) are higher than those reported in previous CC@CNT samples (mostly -1). This is attributed to larger SWCNT diameters (>0.95 nm) used in this study, compared to the typical 0.6–0.8 nm range. Larger diameters result in reduced confinement, allowing carbyne to closely resemble free-standing carbyne while remaining stabilized. This low-temperature synthesis of long-chain, nearly freestanding carbyne within large-diameter SWCNTs offers new opportunities for exploring 1D physics and the unique properties of carbyne for potential applications. © 2024, CC BY-NC-ND.

关键词： Single-walled carbon nanotubes (SWCN)

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Low-Velocity-Favored Transition Radiation

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Physical Review Letters 2023年第11期131卷 113002-113002页

作者： Jialin Chen Ruoxi Chen Fuyang Tay Zheng Gong Hao Hu Yi Yang Xinyan Zhang Chan Wang Ido Kaminer Hongsheng Chen Baile Zhang Xiao Lin Interdisciplinary Center for Quantum Information State Key Laboratory of Extreme Photonics and Instrumentation ZJU-Hangzhou Global Scientific and Technological Innovation Center College of Information Science & Electronic Engineering Zhejiang University Hangzhou 310027 China International Joint Innovation Center the Electromagnetics Academy at Zhejiang University Zhejiang University Haining 314400 China Department of Electrical and Computer Engineering Technion-Israel Institute of Technology Haifa 32000 Israel Department of Electrical and Computer Engineering Rice University Houston Texas 77005 USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston Texas 77005 USA School of Electrical and Electronic Engineering Nanyang Technological University Singapore 639798 Singapore Department of Physics University of Hong Kong Hong Kong 999077 China Key Lab of Advanced Micro/Nano Electronic Devices & Smart Systems of Zhejiang Jinhua Institute of Zhejiang University Zhejiang University Jinhua 321099 China Shaoxing Institute of Zhejiang University Zhejiang University Shaoxing 312000 China Division of Physics and Applied Physics School of Physical and Mathematical Sciences Nanyang Technological University Singapore 637371 Singapore Centre for Disruptive Photonic Technologies Nanyang Technological University Singapore 637371 Singapore

When a charged particle penetrates through an optical interface, photon emissions emerge—a phenomenon known as transition radiation. Being paramount to fundamental physics, transition radiation has enabled many applications from high-energy particle identification to novel light sources. A rule of thumb in transition radiation is that the radiation intensity generally decreases with the decrease of particle velocity v; as a result, low-energy particles are not favored in practice. Here, we find that there exist situations where transition radiation from particles with extremely low velocities (e.g., v/c<10−3) exhibits comparable intensity as that from high-energy particles (e.g., v/c=0.999), where c is the light speed in free space. The comparable radiation intensity implies an extremely high photon extraction efficiency from low-energy particles, up to 8 orders of magnitude larger than that from high-energy particles. This exotic phenomenon of low-velocity-favored transition radiation originates from the interference of the excited Ferrell-Berreman modes in an ultrathin epsilon-near-zero slab. Our findings may provide a promising route toward the design of integrated light sources based on low-energy electrons and specialized detectors for beyond-standard-model particles.

关键词： Atom or molecule scattering from surfaces Atomic & molecular collisions Cherenkov radiation Crystal optics Electron beams & optics Light-matter interaction Optical sources & detectors Optical transient phenomena Plasmonics

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Protein and lipid expansion microscopy with trypsin and tyramide signal amplification for 3D imaging

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Scientific reports 2023年第1期13卷 21922页

作者： Ueh-Ting Tim Wang Xuejiao Tian Yae-Huei Liou Sue-Ping Lee Hsiao-Tang Hu Chieh-Han Lu Po-Ting Lin Ya-Jen Cheng Peilin Chen Bi-Chang Chen Affiliated Senior High School of National Taiwan Normal University Taipei 106348 Taiwan. Research Center for Applied Sciences Academia Sinica Taipei 11529 Taiwan. Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University Taipei 11529 Taiwan. Department of Engineering and System Science National Tsing Hua University Hsinchu 300 Taiwan. Institute of Molecular Biology Academia Sinica Taipei 11529 Taiwan. Institute and Undergraduate Program of Electro-Optical Engineering National Taiwan Normal University Taipei 116 Taiwan. Neuroscience Program NPAS Academia Sinica Taipei 11529 Taiwan ROC. Research Center for Applied Sciences Academia Sinica Taipei 11529 Taiwan. chenb10@gate.sinica.edu.tw.

Expansion microscopy, whereby the relative positions of biomolecules are physically increased via hydrogel expansion, can be used to reveal ultrafine structures of cells under a conventional microscope. Despite its utility for achieving super-resolution imaging, expansion microscopy suffers a major drawback, namely reduced fluorescence signals caused by excessive proteolysis and swelling effects. This caveat results in a lower photon budget and disfavors fluorescence imaging over a large field of view that can cover an entire expanded cell, especially in 3D. In addition, the complex procedures and specialized reagents of expansion microscopy hinder its popularization. Here, we modify expansion microscopy by deploying trypsin digestion to reduce protein loss and tyramide signal amplification to enhance fluorescence signal for point-scanning-based imaging. We name our new methodology TT-ExM to indicate dual trypsin and tyramide treatments. TT-ExM may be applied for both antibody and lipid staining. TT-ExM displayed enhanced protein retention for endoplasmic reticulum and mitochondrial markers in COS-7 cell cultures. Importantly, TT-ExM-based lipid staining clearly revealed the complex 3D membrane structures in entire expanded cells. Through combined lipid and DNA staining, our TT-ExM methodology highlighted mitochondria by revealing their DNA and membrane structures in cytoplasm, as well as the lipid-rich structures formed via phase separation in nuclei at interphase. We also observed lipid-rich chromosome matrices in the mitotic cells. These high-quality 3D images demonstrate the practicality of TT-ExM. Thus, readily available reagents can be deployed in TT-ExM to significantly enhance fluorescence signals and generate high-quality and ultrafine-resolution images under confocal microscopy.

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The thickness dependence of quantum oscillations in ferromagnetic Weyl metal SrRuO3

arXiv

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arXiv 2021年

作者： Kar, Uddipta Singh, Akhilesh Kr. Hsu, Yu-Te Lin, Chih-Yu Das, Bipul Cheng, Cheng-Tung Berben, M. Yang, Song Lin, Chun-Yen Hsu, Chia-Hung Wiedmann, S. Lee, Wei-Cheng Lee, Wei-Li Institute of Physics Academia Sinica Nankang Taipei11529 Taiwan Radboud University Toernooiveld 7 Nijmegen6525 ED Netherlands Department of Physics Applied Physics and Astronomy Binghamton University BinghamtonNY13902 United States Scientific Research Division National Synchrotron Radiation Research Center Hsinchu30076 Taiwan Nano Science and Technology Taiwan International Graduate Program Academia Sinica National Taiwan University Taiwan Radboud University Institute for Molecules and Materials Heyendaalseweg 135 Nijmegen6525 AJ Netherlands Department of Physics National Taiwan University Taipei10617 Taiwan

Quantum oscillations in resistivity and magnetization at high magnetic fields are a macroscopic fingerprint of the energy quantization due to the cyclotron motion of quasiparticles. In a thin Weyl semimetal, a unique thickness dependent Weyl-orbit quantum oscillation was proposed to exist, originating from a nonlocal cyclotron orbit via the electron tunneling between the top and bottom Fermi-arc surface states. Here, untwinned and high crystalline Weyl metal SrRuO3 thin films with different thicknesses were grown on miscut SrTiO3 (001) substrates. Magneto-transport measurements were carried out in magnetic fields up to 35 T, and quantum oscillations with different frequencies were observed and compared to the calculated band structure. In particular, we discovered a frequency F ≈ 30 T at low temperatures and above 3 T that corresponds to a small Fermi pocket with a light effective mass. Its oscillation amplitude appears to be at maximum for film thicknesses in a range of 10 to 20 nm, and the phase of the oscillation exhibits a systematic change with the film thickness. After isolating the well separated frequencies, the constructed Landau fan diagram shows an unusual concave downward curvature in the 1/µ0Hn-n curve, where n is the Landau level index. Based on the rigorous analysis of the thickness and field-orientation dependence of the quantum oscillations, the oscillation with F ≈ 30 T is attributed to be of surface origin, which is related to the Fermi-arc surface state originating from non-overlapping Weyl nodes projected on the film’s surface plane. Those findings can be understood within the framework of the Weyl-orbit quantum oscillation effect with non-adiabatic corrections. © 2021, CC BY-NC-ND.

关键词： Strontium titanates

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Transformative and sustainable insights of agricultural waste-based adsorbents for water defluoridation: Biosorption dynamics, economic viability, and spent adsorbent management

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Heliyon 2024年第8期10卷 e29747页

作者： Das, Koyeli Sukul, Uttara Chen, Jung-Sheng Sharma, Raju Kumar Banerjee, Pritam Dey, Gobinda Taharia, Md. Wijaya, Christian J. Lee, Cheng-I Wang, Shan-Li Nuong, Nguyen Hoang Kim Chen, Chien-Yen Department of Biomedical Sciences Graduate Institute of Molecular Biology National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Doctoral Program in Science Technology Environment and Mathematics Department of Earth and Environmental Sciences National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Department of Medical Research E-Da Hospital Kaohsiung 82445 Taiwan Department of Chemistry and Biochemistry National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Department of Chemical Engineering Widya Mandala Surabaya Catholic University Kalijudan 37 Surbaya 60114 Indonesia Collaborative Research Center for Zero Waste and Sustainability Kalijudan 37 Surabaya 60114 Indonesia Center for Nano Bio-Detection Center for Innovative Research on Aging Society AIM-HI National Chung Cheng University 168 University Road Min-Hsiung Chiayi County 62102 Taiwan Department of Agricultural Chemistry National Taiwan University Taipei 106319 Taiwan

With the progression of civilization, the harmony within nature has been disrupted, giving rise to various ecocidal activities that are evident in every spheres of the earth. These activities have had a profound and far-reaching impact on global health. One significant example of this is the presence of fluoride in groundwater exceeding acceptable limits, resulting in the widespread occurrence of “Fluorosis” worldwide. It is imperative to mitigate the concentration of fluoride in drinking water to meet safety standards. While various defluoridation techniques exist, they often have drawbacks. Biosorption, being a simple, affordable and eco-friendly method, has gained preference for defluoridation. However, its limited commercialization underscores the pressing need for further research in this domain. This comprehensive review article offers a thorough examination of the defluoridation potential of agro-based adsorbents, encompassing their specific chemical compositions and preparation methods. The review presents an in-depth discussion of the factors influencing fluoride biosorption and conducts a detailed exploration of adsorption isotherm and adsorption kinetic models to gain a comprehensive understanding of the nature of the adsorption process. Furthermore, it evaluates the commercial viability through an assessment of regeneration potential and a cost analysis of these agro-adsorbents, with the aim of facilitating the scalability of the defluoridation process. The elucidation of the adsorption mechanism and recommendations for overcoming challenges in large-scale implementation offer a comprehensive outlook on this eco-friendly and sustainable approach to fluoride removal. In summary, this review article equips readers with a lucid understanding of agro-adsorbents, elucidates their ideal conditions for improved performance, offers a more profound insight into the fluoride biosorption mechanism, and introduces the concept of effective spent adsorbent management.

关键词： Adsorption mechanism Agricultural waste Bio-sorption Cost analysis Defluoridation Regeneration Spent adsorbent management

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Density functional study on the oxygen evolution reaction mechanism of transition metal doped bimetallic NiCu phosphate surface

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Computational and Theoretical Chemistry 2025年 1250卷

作者： Hamdi Ikhwan Dzaki Ahmad Syaifullah Muhammad Arkan Nuruzzahran Nadhratun Naiim Mobarak Sasfan Arman Wella Fadjar Fathurrahman Ni Luh Wulan Septiani Adhitya Gandaryus Saputro Graduate Program of Engineering Physics Faculty of Industrial Technology Institut Teknologi Bandung Bandung West Java 40132 Indonesia PT. PLN (Persero) Indonesia Department of Chemical Sciences Faculty of Science and Technology Universiti Kebangsaan Malaysia 43600 UKM Bangi Selangor Darul Ehsan Malaysia Research Center for Quantum Physics National Research and Innovation Agency (BRIN) South Tangerang 15314 Indonesia Collaboration Research Center for Advanced Energy Materials BRIN - Institut Teknologi Bandung Bandung 40132 Indonesia Quantum and Nano Technology Research Group Bandung Institute of Technology Bandung 40132 Indonesia Research Centre for Nanoscience and Nanotechnology Institut Teknologi Bandung Bandung West Java 40132 Indonesia Research Center for Electronics National Research and Innovation Agency KST Samaun Samadikun Bandung 40135 Indonesia

We have explored the oxygen evolution reaction (OER) activity of both undoped nickel copper phosphate (NiCuPO) and transition metal-doped NiCuPO-M (M = Mn, Fe, Co) surfaces using periodic density functional theory (DFT)-based calculations. Our findings highlight that while the undoped NiCuPO surface exhibits a high overpotential of 0.98 V, the introduction of transition metal doping remarkably enhances the OER performance, reducing the overpotential to as low as 0.41 V in the Mn-doped case, outperforming the widely used IrO 2 catalyst. This enhancement is primarily due to a favorable shift in the d -band center, which increases O* adsorption strength and decreases the OER overpotential. Among the doped systems, Mn and Fe doping demonstrate the most substantial reductions in overpotential, underscoring their potential as efficient catalysts for OER applications.

关键词： DFT NiCu phosphate Oxygen evolution reaction Transition metal doping Water electrolysis

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Observing off-resonance motion of nanomechanical resonators as modal superposition

arXiv

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arXiv 2020年

作者： Esmenda, Joshoua Condicion Aguila, Myrron Albert Callera Wang, Jyh-Yang Lee, Teik-Hui Yang, Chi-Yuan Lin, Kung-Hsuan Chang-Liao, Kuei-Shu Katz, Nadav Kafanov, Sergey Pashkin, Yuri Chen, Chii-Dong Department of Engineering and System Science National Tsing Hua University Hsinchu30013 Taiwan Nano-Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei11529 Taiwan Institute of Physics Academia Sinica Taipei11529 Taiwan Department of Physics National Taiwan University Taipei10617 Taiwan Racah Institute of Physics Hebrew University Jerusalem91904 Israel Department of Physics Lancaster University LancasterLA1 4YB United Kingdom

Observation of resonance modes is the most straightforward way of studying mechanical oscillations because these modes have maximum response to stimuli. However, a deeper understanding of mechanical motion could be obtained by also looking at modal responses at frequencies in between resonances. In this paper, we present visualisation of the modal response shapes for a mechanical drum driven off-resonance. Furthermore, we describe these transitions through superposition of resonance modes. Copyright © 2020, The Authors. All rights reserved.

关键词： Modal analysis

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Mechanistic Insights into Enhanced Reactivation of Organophosphate-Inhibited Enzymes by Methyl-Substituted 2-Pralidoxime Analogs

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The journal of physical chemistry. B 2025年第23期129卷 2025 May 27页

作者： Phiphob Naweephattana Nalinee Kongkaew Panida Surawatanawong Nawee Kungwan Yin Fang Peter Wolschann Phornphimon Maitarad Kowit Hengphasatporn Yasuteru Shigeta Thanyada Rungrotmongkol Alisa S Vangnai Center of Excellence in Biocatalyst and Sustainable Biotechnology Department of Biochemistry Faculty of Science Chulalongkorn University Bangkok 10330 Thailand. Program in Bioinformatics and Computational Biology Graduate School Chulalongkorn University Bangkok 10330 Thailand. Department of Chemistry and Center of Excellence for Innovation in Chemistry Faculty of Science Mahidol University Bangkok 10400 Thailand. Department of Chemistry Faculty of Science Chiang Mai University Chiang Mai 50200 Thailand. Research Center for Translational Medicine Shanghai East Hospital Affiliated to Tongji University Shanghai 200120 China. Institute of Theoretical Chemistry University of Vienna Vienna 1010 Austria. Research Center of Nano Science and Technology Department of chemistry College of Science Shanghai University Shanghai 200444 China. Center for Computational Sciences University of Tsukuba 1-1-1 Tennodai Ibaraki Tsukuba 305-8577 Japan.

Organophosphate (OP) compounds, such as paraoxon (POX), inhibit enzymes critical for neurotransmission, causing severe neurotoxic effects. Pralidoxime (2-pyridine aldoxime methyl chloride) or 2-PAM is commonly employed to reverse this inhibition, but its reactivation efficiency is limited. This study computationally explores the reactivation mechanisms of 2-PAM and its methyl-substituted analogs, 4-methyl-2-PAM (4-Met-2-PAM), and 4,6-dimethyl-2-PAM (4,6-Dimet-2-PAM). The reactivation process involves several key steps, such as hydrogen transfer and nucleophilic substitution (). Introducing methyl groups at positions 4 and 6 increases the negative charge on the oxime oxygen, improving nucleophilicity and reactivity. Both 4-Met-2-PAM and 4,6-Dimet-2-PAM show better reactivity than 2-PAM, with 4,6-Dimet-2-PAM demonstrating the greatest improvement. This enhanced reactivity shifts the rate-determining step from nucleophilic substitution to the initial hydrogen transfer. These findings offer valuable insights for designing more effective oxime-based antidotes for organophosphate poisoning.

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The bulk van der Waals layered magnet CrSBr is a quasi-1D material

arXiv

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arXiv 2022年

作者： Klein, Julian Pingault, Benjamin Florian, Matthias Heißenbüttel, Marie-Christin Steinhoff, Alexander Song, Zhigang Torres, Kierstin Dirnberger, Florian Curtis, Jonathan B. Weile, Mads Penn, Aubrey Deilmann, Thorsten Dana, Rami Bushati, Rezlind Quan, Jiamin Luxa, Jan Sofer, Zdenek Alù, Andrea Menon, Vinod M. Wurstbauer, Ursula Rohlfing, Michael Narang, Prineha Lončar, Marko Ross, Frances M. Department of Materials Science and Engineering Massachusetts Institute of Technology CambridgeMA02139 United States John A. Paulson School of Engineering and Applied Sciences Harvard University CambridgeMA02138 United States QuTech Delft University of Technology Delft2600 GA Netherlands Department of Electrical and Computer Engineering Department of Physics University of Michigan Ann ArborMI48109 United States Institut für Festkörpertheorie Westfälische Wilhelms-Universität Münster Münster48149 Germany Institut für Theoretische Physik Universität Bremen P.O. Box 330 440 Bremen28334 Germany Bremen Center for Computational Materials Science University of Bremen Bremen28359 Germany Department of Physics City College of New York New YorkNY10031 United States College of Letters and Science UCLA Los AngelesCA90095 United States Department of Physics Technical University of Denmark Kgs. LyngbyDK-2800 Denmark MIT.nano Massachusetts Institute of Technology CambridgeMA02139 United States Department of Physics The Graduate Center City University of New York New YorkNY10016 United States Photonics Initiative CUNY Advanced Science Research Center New YorkNY10031 United States Physics Program Graduate Center City University of New York New YorkNY10026 United States Department of Inorganic Chemistry University of Chemistry and Technology Prague Technická 5 Prague 6166 28 Czech Republic Institute of Physics Center for Nanotechnology University of Münster Münster48149 Germany

Correlated quantum phenomena in one-dimensional (1D) systems that exhibit competing electronic and magnetic order are of strong interest for studying fundamental interactions and excitations, such as Tomonaga-Luttinger liquids and topological orders and defects with properties completely different from the quasiparticles expected in their higher-dimensional counterparts. However, clean 1D electronic systems are difficult to realize experimentally, particularly magnetically ordered systems. Here, we show that the van der Waals layered magnetic semiconductor CrSBr behaves like a quasi-1D material embedded in a magnetically ordered environment. The strong 1D electronic character originates from the Cr-S chains and the combination of weak interlayer hybridization and anisotropy in effective mass and dielectric screening with an effective electron mass ratio of meX/meY ∼ 50. This extreme anisotropy experimentally manifests in strong electron-phonon and exciton-phonon interactions, a Peierls-like structural instability and a Fano resonance from a van Hove singularity of similar strength of metallic carbon nanotubes. Moreover, due to the reduced dimensionality and interlayer coupling, CrSBr hosts spectrally narrow (1 meV) excitons of high binding energy and oscillator strength that inherit the 1D character. Overall, CrSBr is best understood as a stack of weakly hybridized monolayers and appears to be an experimentally attractive candidate for the study of exotic exciton and 1D correlated many-body physics in the presence of magnetic order. Copyright © 2022, The Authors. All rights reserved.

关键词： Excitons

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Ultralow schottky barriers in h-BN encapsulated monolayer wse2 tunnel field-effect transistors

arXiv

引用

arXiv 2020年

作者： Pande, Gaurav Siao, Jyun-Yan Chen, Wei-Liang Lee, Chien-Ju Sankar, Raman Chang, Yu-Ming Chen, Chii-Dong Chang, Wen-Hao Chou, Fang-Cheng Lin, Minn-Tsong Department of Physics National Taiwan University Taipei Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica Taiwan Center for Condensed Matter Sciences National Taiwan University Taipei Taiwan Department of Electrophysics National Chiao Tung University Hsinchu Taiwan Institute of Physics Academia Sinica Taiwan MOST Taiwan Institute of Atomic and Molecular Sciences Academia Sinica Taiwan Research Center for Applied Sciences Academia Sinica Taiwan

To explore the potential of field-effect transistors (FETs) based on monolayers of the two-dimensional semiconducting channel(SC) for spintronics, the two most important issues are to ensure the formation of variable low resistive tunnel ferromagnetic contacts(FC), and to preserve intrinsic properties of the SC during fabrication. Large Schottky barriers lead to the formation of high resistive contacts and methods adopted to control the barriers often alter the intrinsic properties of the SC. This work aims at addressing both issues in fully encapsulated monolayer WSe2 FETs by using bi-layer h-BN as a tunnel barrier at the FC/SC interface. We investigate the electrical transport in monolayer WSe2 FETs with current-in-plane geometry that yields hole mobilities ∼ 38.3 cm2V −1s−1 at 240 K and On/Off ratios of the order of 107, limited by the contact regions. We have achieved ultralow effective Schottky barrier (∼ 5.34 meV) with encapsulated tunneling device as opposed to a non-encapsulated device in which the barrier heights are considerably higher. These observations provide an insight into the electrical behavior of the FC/h-BN/SC/h-BN heterostructures and such control over the barrier heights opens up the possibilities for WSe2-based spintronic devices. Copyright © 2020, The Authors. All rights reserved.

关键词： Monolayers

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