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arXiv 2022年

作者： Aguila, Myrron Albert C. Esmenda, Joshoua C. Wang, Jyh-Yang Lee, Teik-Hui Chen, Yen-Chun Yang, Chi-Yuan Lin, Kung-Hsuan Chang-Liao, Kuei-Shu Kafanov, Sergey Pashkin, Yuri A. Chen, Chii-Dong Department of Engineering and System Science National Tsing Hua University Hsinchu30013 Taiwan Nano Science and Technology Program Taiwan International Graduate Program National Tsing Hua University Academia Sinica Taiwan Institute of Physics Academia Sinica Nankang Taipei11529 Taiwan Department of Physics Lancaster University LancasterLA1 4YB United Kingdom

nanomechanical resonators made from van der Waals materials (vdW NMRs) provide a new tool for sensing absorbed laser power. The photothermal response of vdW NMRs, quantified from the resonant frequency shifts induced by optical absorption, is enhanced when incorporated in a Fabry-Perot (FP) interferometer. Along with the enhancement comes the dependence of the photothermal response on NMR displacement, which lacks investigation. Here, we address the knowledge gap by studying electromotively driven niobium diselenide drumheads fabricated on highly reflective substrates. We use a FP-mediated absorptive heating model to explain the measured variations of the photothermal response. The model predicts a higher magnitude and tuning range of photothermal responses on few-layer and monolayer NbSe2 drumheads, which outperform other clamped vdW drum-type NMRs at a laser wavelength of 532 nm. Further analysis of the model shows that both the magnitude and tuning range of NbSe2 drumheads scale with thickness, establishing a displacement-based framework for building bolometers using FP-mediated vdW NMRs. © 2022, CC BY.

关键词： Van der Waals forces

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Photoluminescence of oxygen vacancy-rich nano-TiO2 photocatalyst for methylene blue color degradation

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Materials science and Engineering: B 2025年 320卷

作者： Simanjuntak, Mayer Made Joni, I. Faizal, Ferry Gultom, Noto Susanto Kuo, Dong-Hau Panatarani, Camellia Department of Physics Faculty of Mathematic and Natural Sciences Universitas Padjadjaran Jl. Raya Bandung-Sumedang KM 21 Jatinangor Sumedang45363 Indonesia Study Program of Biotechnology Faculty of Graduate School Universitas Padjadjaran Jl. Dipati Ukur No.35 Coblong Bandung40132 Indonesia Functional Nano Powder University Center of Excellence Universitas Padjadjaran Jl. Raya Bandung-Sumedang KM 21 Jatinangor Sumedang45363 Indonesia Department of Materials Science and Engineering National Taiwan University of Science and Technology No.43 Sec. 4 Keelung Road Taipei10607 Taiwan

Wastewater containing synthetic dyes poses a critical environmental hazard, necessitating the development of effective treatment techniques. Despite its promise as a photocatalyst, TiO2′s inability to efficiently absorb visible light limits its practical use. To overcome this limitation, oxygen vacancy (OV) engineering was carried out in TiO2 through solvothermal at temperatures of 150°C, 180°C, and 210°C. Comprehensive analyses confirmed a temperature-induced increase in crystallinity and OV concentration. Furthermore, photoluminescence analysis revealed mid-gap states that improve visible light absorption. Notably, the T150 sample achieved 93.43% degradation of methylene blue within 3 h under sunlight, outperforming commercial TiO2. The superior performance was attributed to a reduced bandgap energy, enhanced charge carrier separation, and increased generation of reactive oxygen species, all facilitated by an optimal concentration of OV. This study clarifies the interaction between photoluminescence and photocatalytic activity, highlighting OV engineering as a highly effective strategy for developing advanced TiO2-based materials for wastewater treatment. © 2025 Elsevier B.V.

关键词： Photocatalytic activity

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Optogenetic Neural Probes: Fiberless, High-Density, Artifact-Free Neuromodulation : (Invited)

Optogenetic Neural Probes: Fiberless, High-Density, Artifact...

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International Electron Devices Meeting (IEDM)

作者： Eunah Ko Kanghwan Kim Mihály Vöröslakos Sungjin Oh György Buzsáki Kensall D. Wise Euisk Yoon Department of Electrical Engineering and Computer Science University of Michigan Ann Arbor MI USA Center for BioMicrosystems Brain Science Institute Korea Institute of Science and Technology Seoul Korea Neuroscience Institute Langone Medical Center New York University New York NY USA Department of Biomedical Engineering University of Michigan Ann Arbor MI USA Center for Nanomedicine Institute for Basic Science (IBS) and Graduate Program of Nano Biomedical Engineering (Nano BME) Advanced Science Institute Yonsei University Seoul Korea

ISBN: (纸本)9781665489607

Evolution of “Michigan Probes” has enabled unraveling the connectivity of neurons at cellular resolution and their dynamic interaction within and across brain areas that underlie behavioral and cognitive functions. Recently, micro-LEDs were monolithically integrated for optogenetic neuromodulation at scale without requiring external optical fiber connection. The ‘hectoSTAR’ micro-LED optoelectrode features 256 recording electrodes and 128 stimulation micro-LEDs in four silicon micro-needle shanks, covering a large volume with 1.3-mm × 0.9-mm cross-sectional area located as deep as 6 mm inside the brain. Technical challenges to overcome in scaling of optogenetic probes will be discussed, followed by future direction.

关键词： Optical fibers Electrodes Brain Optogenetics Silicon Recording Optical fiber devices

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Structural, Morphological, Optical, and Antibacterial Activities of Zinc Oxide nanopowders: A Comparative Study of Green and Soft Chemical Synthesis

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Advances in Materials science and Engineering 2022年第0期2022卷

作者： Siriya Pushpa, K. Catherine Sakthivel, P. Saravanakumar, K. Anuradha, N. Sankaranarayanan, R.K. Paulraj, Mosae Selvakumar Post-Graduate and Research Department of Physics Bon Secours College for Women Tamil Nadu Thanjavur613006 India Centre for Materials Science Department of Physics Science and Humanities Faculty of Engineering Karpagam Academy of Higher Education Coimbatore641021 India Mallasamudram Tamil Nadu Namakkal637503 India Centre for Nano Science and Technology Department of Chemistry Chennai Institute of Technology Tamil Nadu Kundrathur600069 India AUW Chemistry Hub Science and Math Program Asian University for Women Chattogram Bangladesh

Zinc oxide, a well-known inorganic metal oxide in nanoparticle form, has outstanding antibacterial properties. In this work, the authors focus on determining ZnO nanoparticles’ structural, optical, and antibacterial activity. A simple soft chemical route synthesizes C-ZnO nanoparticles chemically, while the green synthesis method is used to prepare G-ZnO nanoparticles. Ocimum tenuiflorum leaf extract was used to prepare G-ZnO nanopowders. These samples are investigated and compared in terms of their structural, morphological, optical, and antibacterial properties. According to XRD investigations, the synthesized ZnO nanopowders possess a hexagonal structure. The particle size of G-ZnO is smaller than that of C-ZnO nanoparticles. The XPS result revealed the binding and interactions between molecules. The FTIR study confirmed the presence of molecules and their vibrations. UV-vis-DRS spectroscopy was used to investigate optical properties such as reflectance and band gap. The grain size of the G-ZnO nanopowders was decreased, and oxygen vacancy was produced. The antibacterial efficiency of plant extracts against two different bacterial strains, S. aureus (Gram-positive) and *** (Gram-negative), has been studied and reported. Copyright © 2022 K. Catherine Siriya Pushpa et al.

关键词： ZnO nanoparticles

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Solution-Processed and Room-Temperature Spin Light-Emitting Diode Based on Quantum Dots/Chiral Metal-Organic Framework Heterostructure

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Advanced Functional Materials 2023年第19期33卷

作者： Mustaqeem, Mujahid Chou, Pi-Tai Kamal, Saqib Ahmad, Naveed Lin, Jia-Yu Lu, Yu-Jung Lee, Xing-Hao Lin, Kung-Hsuan Lu, Kuang-Lieh Chen, Yang-Fang Nano-Science and Technology Program Taiwan International Graduate Program Institute of Physics Academia Sinica Taipei106 Taiwan Department of Physics National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Taiwan Department of Chemistry National Taiwan University No. 1 Section 4 Roosevelt Rd Taipei10617 Taiwan Institute of Chemistry Academia Sinica Taipei115 Taiwan Department of Materials Science and Engineering National Taiwan University of Science and Technology Taipei10607 Taiwan Research Center for Applied Sciences Academia Sinica Taipei115024 Taiwan Institute of Physics Academia Sinica Taipei11529 Taiwan

Spin optoelectronics is an indispensable key for the future development of spintronics. In conventional spin light emitting diodes (LEDs), spin-polarized carrier pairs are injected electrically into the light emitting layer and create circularly polarized light (CPL). Generally, spin-polarized carriers are accomplished using ferromagnetic contacts or applying an external magnetic field, which will produce several drawbacks, including low temperature operation, low spin-polarized carriers injection efficiency, etc. To circumvent the existing shortcomings, here, an alternative approach is proposed and achieves spin-polarized LEDs at room temperature based on quantum dots (QDs)/chiral metal-organic framework heterojunction without using ferromagnetic contacts or magnetic fields. The spin-polarized injected layer composed of self-assembled monolayer (SAM)/Chiral-MOF ([Sr(9,10-adc)(DMAc)2]n)) film, which produces spin-polarized holes with spin orientation, determining the polarization and strength of circularly polarized electroluminescence (CP-EL). The spin-QLED emits CP-EL at a rate of 12.24% efficiency, which provides an excellent alternative to generate new functionality for conventional QLEDs. The approach is anticipated to be very useful, enabling to offer a general methodology for generating not yet realized spin optoelectronic devices. © 2023 Wiley-VCH GmbH.

关键词： Room temperature

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A green recyclable Li3VO4-pectin electrode exhibiting pseudocapacitive effect as an advanced anode for lithium-ion battery

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Journal of Energy Storage 2023年 72卷

作者： Su, Yu-Hsuan Chung, Chin-Yi Chen, Yan-Ruei Wu, Feng-Yu Lin, Ya-Huei Chi, Po-Wei Wu, Phillip M. Paul, Tanmoy Lin, Hwai-En Chang-Liao, Kuei-Shu Wang, Sea-Fue Wu, Maw-Kuen Institute of Physics Academia Sinica 128 Section 2 Academia Road Taipei11529 Taiwan Nano Science and Technology Program Taiwan International Graduate Program Academia Sinica and National Tsing Hua University 128 Section 2 Academia Road Taipei11529 Taiwan Department of Engineering and System Science National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu300044 Taiwan 1 Section 3 Zhongxiao E. Rd. Taipei106 Taiwan 1 Section 3 Zhongxiao E. Road Taipei106 Taiwan Research Institute for Sustainable Energy TCG Centres for Research and Education in Science and Technology BIPL Building Salt Lake Kolkata700091 India

Battery system design and development is prioritizing environmentally friendly recycling processes to ensure a sustainable future for our planet. The reuse of active materials in Li-ion batteries is critical for this goal. Herein, we investigated the electrochemical performance of Li3VO4 (LVO) anode with pectin as a binder. Our Li-ion half-cells showed stable capacity of 230 mAh g−1 at a current density of 0.02 A g−1 after 100 cycles. In addition, we observed a novel enhanced specific capacity of 400 mAh g−1 during delithiation at a high current density of 1 A g−1, which did not occur during lithiation. This higher capacity was can be attributed to the pseudocapacitive lithium storage behavior in the LVO-pectin electrode, as identified by CV and EIS analyses. The heterostructure of LVO-pectin resulted in an interfacial surface charge that contributed to the capacity, as demonstrated by impedance spectroscopy in conjunction with the distribution of relaxation times. The utilization of pectin as an eco-friendly binder demonstrated nearly 90 % material recovery and 100 % capability for subsequent re-lithiation, indicating recyclability. Furthermore, the pseudocapacitive effect becomes increasingly dominant in regenerated LVO-pectin cells. These results exemplify a promising approach towards the development of environmentally friendly Li-ion batteries with high energy and power density. © 2023 Elsevier Ltd

关键词： Lithium-ion batteries

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Doping Engineered InSe Flakes for High Mobility Phototransistor

Doping Engineered InSe Flakes for High Mobility Phototransis...

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Novel Optical Materials and Applications, NOMA 2020

作者： Inbaraj, Christy Roshini Paul Mathew, Roshan Jesus Sankar, Raman Lee, Chih-Hao Chen, Yang-Fang Department of Engineering and System Science National Tsing Hua University Hsinchu Taiwan Nano-Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei Taiwan Center for Condensed Matter Sciences National Taiwan University Taipei Taiwan Department of Physics National Taiwan University Taipei Taiwan

Sn doped InSe crystal has a reduced oxide phase and enhanced electron mobility. Along with the substrate modification, the mobility enhances to 2560 240 cm2 V-1s-1. Moreover, it exhibits a piezo-phototronic effect use... 详细信息

ISBN: (纸本)9781943580798

关键词： Indium compounds

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Cementing the grain boundary defects in the strain relaxed mixed Sn-Pb perovskite solar cells

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Chemical Engineering Journal 2025年 516卷

作者： Kumar, Abhishek Ansari, Zeeshan Alam Hanmandlu, Chintam Banerjee, Soumallya Chen, Yu-Te Yang, Po-Yu Musa, Ahmed Fouad You, Yun-Wen Pao, Chun-Wei Wei, Tzu-Chien Shyue, Jing-Jong Lu, Yu-Jung Chu, Chih-Wei Department of Physics National Taiwan University Sec. 4 Roosevelt Road Taipei106 Taiwan Research Center for Applied Sciences Academia Sinica 128 Academia Road Section 2 Taipei Nangang11529 Taiwan Nano-Science and Technology Program Taiwan International Graduate Program Academia Sinica Taipei106 Taiwan Department of Materials Science and Engineering National Yang Ming Chiao Tung University Hsinchu300 Taiwan Department of Chemical Engineering National Tsing Hua University 101 Section 2 Kuang-Fu Road Hsinchu City300044 Taiwan College of Engineering Center for Green Technology Chang Gung University Taoyuan City333002 Taiwan Department of Photonics National Yang Ming Chiao Tung University Hsinchu City30010 Taiwan Institute of Applied Mechanics National Taiwan University Sec. 4 Roosevelt Road Taipei106 Taiwan

Mixed Tin-lead (Sn-Pb) perovskite solar cells (PSCs) offer a promising avenue for achieving high power conversion efficiencies (PCEs) due to their narrow bandgaps and substantial optical absorption in the visible–near-infrared region. However, the disparated reaction kinetics of PbI2 and SnI2 with organic salts, resulting in an uneven spatial distribution of Sn2+ and Pb2+ within the perovskite lattice, inducing micro-strain in the film and a Sn-rich surface vulnerable to oxidation-Sn2+ to Sn4+, thereby elevating nonradiative recombination. Here, we report the incorporation of 2,5-Dibromo-3,4-pyridinediamine (DBPDA) as an additive in the mixed Sn-Pb perovskite precursor solution, designed to mitigate micro-strain formation, reduce defect density by suppressing Sn4+ formation, and enhance the passivation of undercoordinated Sn/Pb species through synergistic bonding interaction. The best performing PSCs achieved an impressive PCE of 21.24 % with a high open circuit voltage (Voc) of 0.85 V, alongside significantly improved long-term stability, retaining near 80 % of their initial PCE after 1,008 h in a nitrogen-filled glovebox without encapsulation. In contrast, the control devices retained only 18 % of their initial efficiency under identical conditions. Additionally, an enhanced field effect hole mobility, increasing from 0.18 cm2/V-s in the control film to 1.43 cm2/V-s in the target film, was achieved in mixed Sn-Pb perovskite thin film transistors (TFTs) using these films as active layers. These findings present a viable strategy for strain-relieved perovskite films, enabling stable and high-performance mixed Sn-Pb PSCs and TFTs. © 2025 Elsevier B.V.

关键词： Crystallization kinetics

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Design of experiments as a strategy for modulating the colloidal stability, physico-chemical properties and drug-delivery potential of small mesoporous silica nanoparticles

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Advanced Powder technology 2023年第10期34卷

作者： Lestari, Windy Ayu Saputra, Ozi Adi Díaz-García, Diana Wahyuningsih, Sayekti Gómez-Ruiz, Santiago Wibowo, Fajar Rakhman Magister Program in Chemistry Faculty of Mathematics and Natural Sciences Universitas Sebelas Maret Surakarta57126 Indonesia Department of Chemistry Faculty of Mathematics and Natural Sciences Universitas Sebelas Maret Surakarta57126 Indonesia COMET-NANO Group Departamento de Biología y Geología Física y Química Inorgánica Universidad Rey Juan Carlos Calle Tulipán s/n Madrid MóstolesE-28933 Spain Institute of Chemistry Taiwan International Graduate Program Sustainable Chemical Science and Technology Academia Sinica Taipei115 China Department of Chemical Engineering National Taiwan University Taipei10617 China

The synthesis of highly stable small mesoporous silica nanoparticles (SMSN) in colloid dispersions is still challenging for biomedical applications. This study is focus on the successfully synthesis and formulation of porous, highly dispersed and colloidal stable SMSN via the soft–templating method. This study reports how the differences in synthesis variables, namely, temperature, amount of triethylamine (TEA) and/or cetyltrimethylammonium bromide (CTAB) influence the morphology and textural properties of SMSN. The analysis of the particle size, surface area, pore size, pore volume, zeta potential, and colloidal stability (represent by absorbance decreasing rate) show that temperature is the most influential factor governing the preparation of SMSN. The optimal conditions found for the synthesis of these nanoparticles were 50 °C, using a molar ratio between TEA and CTAB (3.5971: 1). Therefore, our study shows interesting insights on the effect of each variable to control the morphology and properties of small MSN for the design of this kind of nanoparticulated systems, therefore, giving valuable data to be considered for the future construction of tailor-made effective drug carrier materials. © 2023 The Society of Powder technology Japan

关键词： Synthesis (chemical)

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High-sensitivity of initial SrO growth on the residual resistivity in epitaxial thin films of SrRuO3 on SrTiO3(001)

arXiv

引用

arXiv 2021年

作者： Kar, Uddipta Singh, Akhilesh Kr. Yang, Song Lin, Chun-Yen Das, Bipul Hsu, Chia-Hung Lee, Wei-Li Institute of Physics Academia Sinica Nankang Taipei11529 Taiwan National Synchrotron Radiation Research Center Hsinchu30076 Taiwan Nano Science and Technology Taiwan International Graduate Program Academia Sinica National Taiwan University Taiwan

The growth of SrRuO3 (SRO) thin film with high-crystallinity and low residual resistivity (RR) is essential to explore its intrinsic properties. Here, utilizing the adsorption-controlled growth technique, the growth condition of initial SrO layer on TiO2-terminated SrTiO3 (STO) (001) substrate was found to be crucial for achieving a low RR in the resulting SRO film grown afterward. The optimized initial SrO layer shows a c(2 × 2) superstructure that was characterized by electron diffraction, and a series of SRO films with different thicknesses (ts) were then grown. The resulting SRO films exhibit excellent crystallinity with orthorhombic-phase down to t ≈ 4.3 nm, which was confirmed by high resolution X-ray measurements. From X-ray azimuthal scan across SRO orthorhombic (02±1) reflection, we uncover four structural domains with a dominant domain of orthorhombic SRO [001] along cubic STO [010] direction. The dominant domain population depends on t, STO miscut angle (α), and miscut direction (β), giving a volume fraction of about 92 % for t ≈ 26.6 nm and (α,β) ≈ (0.14o, 5o). On the other hand, metallic and ferromagnetic properties were well preserved down to t ≈ 1.2 nm. Residual resistivity ratio (RRR = ρ(300K)/ρ(5K)) reduces from 77.1 for t ≈ 28.5 nm to 2.5 for t ≈ 1.2 nm, while ρ(5K) increases from 2.5 µΩcm for t ≈ 28.5 nm to 131.0 µΩcm for t ≈ 1.2 nm. The ferromagnetic onset temperature (Tc′) of around 151 K remains nearly unchanged down to t ≈ 9.0 nm and decreases to 90 K for t ≈ 1.2 nm. Our finding thus provides a practical guideline to achieve high crystallinity and low RR in ultra-thin SRO films by simply adjusting the growth of initial SrO layer. Copyright © 2021, The Authors. All rights reserved.

关键词： Ferromagnetism

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