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Terahertz spin dynamics in rare-earth orthoferrites

Photonics Insights 2022年第2期1卷 1-56页

作者： Xinwei Li Dasom Kim Yincheng Liu Junichiro Kono Department of Physics California Institute of TechnologyPasadenaUSA Department of Electrical and Computer Engineering Rice UniversityHoustonUSA Applied Physics Graduate Program Smalley-Curl InstituteRice UniversityHoustonUSA Department of Physics and Astronomy Rice UniversityHoustonUSA Department of Materials Science and NanoEngineering Rice UniversityHoustonUSA

Recent interest in developing fast spintronic devices and laser-controllable magnetic solids has sparked tremendous experimental and theoretical efforts to understand and manipulate ultrafast dynamics in *** of spin dynamics in the terahertz(THz)frequency range are particularly important for elucidating microscopic pathways toward novel device ***,we review THz phenomena related to spin dynamics in rare-earth orthoferrites,a class of materials promising for antiferromagnetic *** expand this topic into a description of four key elements.(1)We start by describing THz spectroscopy of spin excitations for probing magnetic phase transitions in thermal *** acoustic magnons are useful indicators of spin reorientation transitions,electromagnons that arise from dynamic magnetoelectric couplings serve as a signature of inversion-symmetry-breaking phases at low temperatures.(2)We then review the strong laser driving scenario,where the system is excited far from equilibrium and thereby subject to modifications to the free-energy *** pathways for ultrafast laser manipulation of magnetic order are discussed.(3)Furthermore,we review a variety of protocols to manipulate coherent THz magnons in time and space,which are useful capabilities for antiferromagnetic spintronic applications.(4)Finally,new insights into the connection between dynamic magnetic coupling in condensed matter and the Dicke superradiant phase transition in quantum optics are *** presenting a review on an array of THz spin phenomena occurring in a single class of materials,we hope to trigger interdisciplinary efforts that actively seek connections between subfields of spintronics,which will facilitate the invention of new protocols of active spin control and quantum phase engineering.

关键词： terahertz spin dynamics magnetism orthoferrite ultrafast spectroscopy magneto-optics

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Novel drying additives and their evaluation for self-flowing refractory castables

arXiv

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arXiv 2021年

作者： Bezerra, B.P. Luz, A.P. Pandolfelli, V.C. Federal University of Sao Carlos Graduate Program in Materials Science and Engineering Rod. Washington Luis km 235 São Carlos - SPCEP:13565-905 Brazil

The drying step of dense refractory castables containing hydraulic binders is a critical process, which usually requires using slow heating rates due to the high explosion trend of such materials during their first thermal treatment. Thus, this work investigated the performance of alternative additives to induce faster and safer drying of self-flowing high-alumina refractory castables bonded with calcium aluminate cement (CAC) or hydratable alumina (HA). The following materials were analyzed for this purpose: polymeric fibers, a permeability enhancing compound (RefPac MIPORE 20) and an organic additive (aluminum salt of 2-hydroxypropanoic acid). The drying behavior and explosion resistance of the cured samples were evaluated when subjecting the prepared castables to heating rates of 2, 5 or 20°C/min and the obtained data were then correlated to the potential of the drying agents to improve the permeability and mechanical strength level of the refractories at different temperatures. The collected results attested that the selected additives were more efficient in optimizing the drying behavior of the CAC-bonded compositions, whereas the HA-containing castables performed better when the aluminum-based salt was blended with a small amount of CAC (0.5 wt.%), which changed the binders hydration reaction sequence and optimized the permeability level of the resulting microstructure. Consequently, some of the designed compositions evaluated in this work showed improved drying behavior and no explosion was observed even during the tests carried out under a high heating rate (20°C/min). © 2021, CC BY-NC-ND.

关键词： Aluminum oxide

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Exploring the magnetic properties of individual barcode nanowires using wide-field diamond microscopy

arXiv

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arXiv 2023年

作者： Yoon, Jungbae Moon, Jun Hwan Jeong, Jugyeong Kim, Yu Jin Kim, Kihwan Kang, Hee Seong Jeon, Yoo Sang Oh, Eunsoo Lee, Sun Hwa Han, Kihoon Lee, Dongmin Lee, Chul-Ho Kim, Young Keun Lee, Donghun Department of Physics Korea University Seoul Korea Republic of Department of Materials Science and Engineering Korea University Seoul Korea Republic of Institute for High Technology Materials and Devices Korea University Seoul Korea Republic of KU-KIST Graduate School of Converging Science and Technology Korea University Seoul Korea Republic of Center for Hydrogen∙Fuel Cell Research Korea Institute of Science and Technology Seoul Korea Republic of Ulsan44919 Korea Republic of BK21 Graduate Program Department of Biomedical Sciences Korea University College of Medicine Seoul Korea Republic of Department of Neuroscience Korea University College of Medicine Seoul Korea Republic of Department of Anatomy Korea University College of Medicine Seoul Korea Republic of

Barcode magnetic nanowires typically comprise a multilayer magnetic structure in a single body with more than one segment type. Interestingly, owing to selective functionalization and novel interactions between the layers, barcode magnetic nanowires have attracted significant attention, particularly in the field of bioengineering. However, an analysis of their magnetic properties at the individual nanowire level remains challenging. With this background, herein, we investigated the characterization of magnetic nanowires at room temperature under ambient conditions based on magnetic images obtained via wide-field quantum microscopy with nitrogen-vacancy centers in diamond. Consequently, we could extract critical magnetic properties, such as the saturation magnetization and coercivity, of single nanowires by comparing the experimental results with those of micromagnetic simulations. This study opens up the possibility for a versatile characterization method suited to individual magnetic nanowires. © 2023, CC BY.

关键词： Diamonds

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The connection between polymer collapse and the onset of jamming

arXiv

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arXiv 2023年

作者： Grigas, Alex T. Fisher, Aliza Shattuck, Mark D. O’Hern, Corey S. Graduate Program in Computational Biology and Bioinformatics Yale University New HavenCT06520 United States Integrated Graduate Program in Physical and Engineering Biology Yale University New HavenCT06520 United States Department of Mechanical Engineering and Materials Science Yale University New HavenCT06520 United States Benjamin Levich Institute and Physics Department The City College of New York New YorkNY10031 United States Department of Physics Yale University New HavenCT06520 United States Department of Applied Physics Yale University New HavenCT06520 United States

Previous studies have shown that the interiors of proteins are densely packed, reaching packing fractions that are as large as those found for static packings of individual amino-acid-shaped particles. How can the interiors of proteins take on such high packing fractions given that amino acids are connected by peptide bonds and many amino acids are hydrophobic with attractive interactions? We investigate this question by comparing the structural and mechanical properties of collapsed attractive disk-shaped bead-spring polymers to those of three reference systems: static packings of repulsive disks, of attractive disks, and of repulsive disk-shaped bead-spring polymers. We show that attractive systems quenched to temperatures below the glass transition T Tg and static packings of both repulsive disks and bead-spring polymers possess similar interior packing fractions. Previous studies have shown that static packings of repulsive disks are isostatic at jamming onset, i.e. the number of contacts Nc matches the number of degrees of freedom, which strongly influences their mechanical properties. We find that repulsive polymers are hypostatic at jamming onset, but effectively isostatic when including quartic modes. While attractive disk and polymer packings are hyperstatic, we identify a definition for interparticle contacts for which they can also be considered as effectively isostatic. As a result, we show that the mechanical properties (e.g. scaling of the potential energy with excess contact number and low-frequency contribution to the density of vibrational modes) of weakly attractive disk and polymer packings are similar to those of isostatic repulsive disk and polymer packings. Our results demonstrate that static packings generated via attractive collapse or compression of repulsive particles possess similar structural and mechanical properties. © 2023, CC BY.

关键词： Amino acids

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Gallium Oxide as Photonic Integrated Platforms in the UV–Visible Spectra

Gallium Oxide as Photonic Integrated Platforms in the UV–Vi...

引用

Conference on Lasers and Electro-Optics (CLEO)

作者： Jingan Zhou Xuan Zhao Rui Xu Xiang Zhang Kai Fu Tao Li Mingfei Xu Shisong Luo Ziyi He Jacob T. Robinson Hanyu Zhu Pulickel M. Ajayan Xiaodong Zhang Yuji Zhao Department of Electrical and Computer Engineering Rice University Houston TX USA Applied Physics Graduate Program Smalley-Curl Institute Rice University Houston TX USA Department of Materials Science and NanoEngineering Rice University Houston TX USA School of Electrical Computer and Energy Engineering Arizona State University Tempe Arizona USA Nanofabrication Facility Suzhou Institute of Nano-Tech and Nano-Bionics Chinese Academy of Sciences Suzhou China

We report the Ga 2 O 3 as photonic integrated platforms and its nonlinear optical effects in the UV–visible spectra. A low propagation loss of 3.7 dB/cm and second-order susceptibility of χ (2) =4.89×10 -3 pm... 详细信息

ISBN: (纸本)9781957171258

关键词： Material properties Nonlinear effects Nonlinear susceptibility Optical components Thin films Visible light communications

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Deterministic synthesis of phase pure 2D perovskites via progressive transformation of layer thickness

arXiv

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arXiv 2022年

作者： Hou, Jin Li, Wenbin Zhang, Hao Sidhik, Siraj Blancon, Jean-Christophe Even, Jacky Kanatzidis, Mercouri G. Mohite, Aditya D. Department of Materials Science and NanoEngineering Rice University HoustonTX77005 United States Department of Chemical and Biomolecular Engineering Rice University HoustonTX77005 United States Applied Physics Graduate Program Smalley‐Curl Institute Rice University HoustonTX77005 United States INSA de Rennes CNRS UMR 6082 Rennes35708 France Department of Chemistry Department of Materials Science and Engineering Northwestern University EvanstonIL60208 United States

Two-dimensional (2D) halide perovskites have emerged as semiconductor platforms for realizing efficient and durable optoelectronic devices. However, the reproducible synthesis of 2D perovskite crystals with desired layer thickness (or n value) greater than 2, has been an enduring challenge due to the lack of kinetic control (temperature, time, stoichiometry) for each layer thickness. Here, we demonstrate a novel method term as the kinetically controlled space confinement (KCSC) for the deterministic growth of phase pure Ruddlesden-Popper (RP) and Dion-Jacobson (DJ) 2D perovskites. The phase-pure growth was achieved by progressively increasing the temperature (fixed time) or the crystallization time (fixed temperature), which allowed for an acute control of the crystallization kinetics. We also observe a systematic transformation from a lower n-value to n=3, 4, 5, 6 in 2D perovskites. In-situ photoluminescence spectroscopy and imaging suggest that the progressive transformation from lower to higher n-value occurs via intercalation of excess precursor ions. These experiments enabled the development of a machine learning assisted multi-parameter phase diagram, which predicts the growth of 2D phase with a specific n-value. © 2022, CC BY.

关键词： Perovskite

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Chiral anomaly and Weyl orbit in three-dimensional Dirac semimetal Cd3As2 grown on Si

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Nanotechnology 2024年第16期35卷 165002-165002页

作者： Lin, Wei-Chen Tsai, Peng-Ying Zou, Jia-Zhu Lee, Jie-Ying Kuo, Chun-Wei Lee, Hsin-Hsuan Pan, Ching-Yang Yang, Cheng-Hsueh Chen, Sheng-Zong Wang, Jyh-Shyang Jiang, Pei-Hsun Liang, Chi-Te Chuang, Chiashain Taiwan International Graduate Program Academia Sinica Taipei115 Taiwan Department of Engineering and System Science National Tsing Hua University Hsinchu300 Taiwan Graduate Institute of Applied Physics National Taiwan University Taipei106 Taiwan National Taiwan University Taipei106 Taiwan Department of Electronic Engineering Chung Yuan Christian University Taoyuan320 Taiwan Department of Physics Chung Yuan Christian University Taoyuan320 Taiwan Department of Physics National Taiwan Normal University 106 Taiwan Research Center for Semiconductor Materials and Advanced Optics Chung Yuan Christian University Taoyuan320 Taiwan

Preparing Cd3As2, which is a three-dimensional (3D) Dirac semimetal in certain crystal orientation, on Si is highly desirable as such a sample may well be fully compatible with existing Si CMOS technology. However, there is a dearth of such a study regarding Cd3As2 films grown on Si showing the chiral anomaly. Here, for the first time, we report the novel preparation and fabrication technique of a Cd3As2 (112) film on a Si (111) substrate with a ZnTe (111) buffer layer which explicitly shows the chiral anomaly with a nontrivial Berry’s phase of π. Despite the Hall carrier density ( n 3 D ≈ 9.42 × 10 17 cm−3) of our Cd3As2 film, which is almost beyond the limit for the portents of a 3D Dirac semimetal to emerge, we observe large linear magnetoresistance in a perpendicular magnetic field and negative magnetoresistance in a parallel magnetic field. These results clearly demonstrate the chiral magnetic effect and 3D Dirac semimetallic behavior in our silicon-based Cd3As2 film. Our tailoring growth of Cd3As2 on a conventional substrate such as Si keeps the sample quality, while also achieving a low carrier concentration. © 2024 IOP Publishing Ltd.

关键词： II-VI semiconductors

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Development of high on/off current ratio in p-type copper oxide thin-film transistors with a back-end-of-line compatible process

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Journal of Vacuum science and Technology A: Vacuum, Surfaces and Films 2024年第5期42卷

作者： Kuo, Chi-Yuan Lin, Wei-Chen Lo, Tsung-Tien Shen, Ching-Hsuan Shen, Ming-Yu Lee, Chia-Chan Lin, Chi-Ping Lin, Yuang-Ming Huang, Haw-Tyng Yeh, Po-Chun Chen, Hsin-Chu Wu, Chih-I Graduate Institute of Photonics and Optoelectronic Department of Electrical Engineering National Taiwan University Taipei106 Taiwan Program of Quantum Technology and Advanced Material College of Science National Tsing Hua University Hsinchu300 Taiwan Institute of Innovative Semiconductor Manufacturing National Sun Yat-sen University Kaohsiung804 Taiwan Institute of Advanced Semiconductor Packaging and Testing National Sun Yat-sen University Kaohsiung804 Taiwan Department of Materials Science and Engineering National Taiwan University Taipei106 Taiwan Electronic and Optoelectronic System Research Laboratories Industrial Technology Research Institute Hsinchu300 Taiwan

The objective of this study is to develop an efficient process to synthesize wafer scale p-type cuprous oxide (Cu2O) with the back-end-of-line (BEOL) compatible process (2/Si substrates followed by rapid thermal oxidation to oxidize it into large-area, uniform Cu2O. Bottom-gate Cu2O thin-film transistors (TFTs) were fabricated as gate dielectric on 100 nm thermal oxide. The results of the ID-VG curve demonstrate that we have successfully fabricated BEOL-compatible p-type Cu2O TFTs. The drain-off current can be achieved to 0.1 pA, with the highest on/off ratio reaching up to 6 orders. Significantly, the TFT with an on/off ratio of 106 is sufficient to meet the requirements for digital circuit applications, including logic circuits, and the BEOL-compatible process (2O TFTs. © 2024 Author(s).

关键词： Thin film transistors

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Injectable cross-linked hyaluronic acid hydrogels with epigallocatechin gallate loading as vitreous substitutes

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International Journal of Biological Macromolecules 2024年第Part1期275卷 133467页

作者： Chen, Huai-An Tai, Yi-Ning Hsieh, Erh-Hsuan Thacker, Minal Lin, I-Chan Tseng, Ching-Li Lin, Feng-Huei Graduate Institute of Biomedical Materials and Tissue Engineering College of Biomedical Engineering Taipei Medical University Shuang-Ho Campus New Taipei City Taiwan Institute of Biomedical Engineering College of Medicine & College of Engineering National Taiwan University Taipei City Taiwan 17W Hong Kong Science Park Hong Kong Department of Ophthalmology Wan Fang Hospital Taipei Medical University Taipei City Taiwan Department of Ophthalmology School of Medicine College of Medicine Taipei Medical University Taipei City Taiwan International Ph. D. Program in Biomedical Engineering College of Biomedical Engineering Taipei Medical University Shuang-Ho Campus New Taipei City Taiwan Research Center of Biomedical Device College of Biomedical Engineering Taipei Medical University Taipei City Taiwan International Ph. D. Program in Cell Therapy and Regenerative Medicine College of Medicine Taipei Medical University Taipei City Taiwan National Health Research Institutes Miaoli County Taiwan

Hyaluronic acid (HA) serves as a vitreous substitute owing to its ability to mimic the physical functions of native vitreous humor. However, pure HA hydrogels alone do not provide sufficient protection against potential inflammatory risks following vitrectomy. In this study, HA was crosslinked with 1,4-butanediol diglycidyl ether (BDDE) to form HA hydrogels (HB). Subsequently, the anti-inflammatory agent epigallocatechin gallate (EGCG) was added to the hydrogel (HBE) for ophthalmic applications as a vitreous substitute. The characterization results indicated the successful preparation of HB with transparency, refractive index, and osmolality similar to those of native vitreous humor, and with good injectability. The anti-inflammatory ability of HBE was also confirmed by the reduced expression of inflammatory genes in retinal pigment epithelial cells treated with HBE compared with those treated with HB. In a New Zealand white rabbit model undergoing vitreous substitution treatment, HBE 50 (EGCG 50 μM addition) exhibited positive results at 28 days post-surgery. These outcomes included restored intraocular pressure, improved electroretinogram responses, minimal increase in corneal thickness, and no inflammation during histological examination. This study demonstrated the potential of an injectable HA-BDDE cross-linked hydrogel containing EGCG as a vitreous substitute for vitrectomy applications, offering prolonged degradation time and anti-inflammatory effects postoperatively. © 2024 The Authors

关键词： Hyaluronic acid

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High‑Performance Thick Cathode Based on Polyhydroxyalkanoate Binder for Li Metal Batteries

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Advanced Fiber materials 2024年第1期6卷 214-228页

作者： Dong Hyuk Kang Minhyuck Park Jeonghun Lee Chan Yeol Kim Jimin Park Youn‑Ki Lee Jong Chan Hyun Son Ha Jin Hwan Kwak Juhee Yoon Hyemin Kim Hyun Soo Kim Do Hyun Kim Sangmin Kim Ji Yong Park Robin Jang Seung Jae Yang Hee‑Dae Lim Se Youn Cho Hyoung‑Joon Jin Seungjin Lee Yunil Hwang Young Soo Yun KU‑KIST Graduate School of Converging Science and Technology Korea University145 Anam‑roSeongbuk‑guSeoul 02841South Korea Carbon Composite Materials Research Center Korea Institute of Science and Technology(KIST)92 Chundong‑roBongdong‑eupWanju‑gunJeollabuk‑do 55324South Korea Energy Storage Research Center Korea Institute of Science and Technology(KIST)514‑gil Hwaraong‑roSeoul 02792South Korea Program in Environmental and Polymer Engineering Inha University100 Inha‑ro Michuhol‑guIncheon 22212South Korea Advanced Analysis Data Center Korea Institute of Science and Technology(KIST)514‑gil Hwaraong‑roSeoul 02792South Korea Advanced Nanohybrids Laboratory Department of Chemistry and Chemical EngineeringInha University100 Inha‑roMichuhol‑guIncheon 22212South Korea CJ CheilJedang Corporation 55 Gwanggyo‑ro 42Beon‑gilYeongtong‑guSuwon 16495South Korea Department of Chemical Engineering Hanyang University222 Wangsimni‑roSeongdong‑guSeoul 04763South Korea Department of Integrative Energy Engineering Korea University145 Anam‑roSeongbuk‑guSeoul 02841South Korea

Thick cathodes can overcome the low capacity issues,which mostly hamper the performance of the conventional active cathode materials,used in rechargeable Li ***,the typical slurry-based method induces cracking and flaking during the fabrication of thick *** addition,a significant increase in the charge-transfer resistance and local cur-rent overload results in poor rate capabilities and cycling stabilities,thereby limiting electrode *** this study,a synergistic dual-network combination strategy based on a conductive nanofibrillar network(CNN)and a nano-bridging amor-phous polyhydroxyalkanoate(aPHA)binder is used to demonstrate the feasibility of constructing a high-performance thick *** CNN and aPHA dual network facilitates the fabrication of a thick cathode(≥250μm thickness and≥90 wt%active cathode material)by a mass-producible slurry *** thick cathode exhibited a high rate capability and excel-lent cycling *** addition,the thick cathode and thin Li metal anode pair(Li//t-NCM)exhibited an optimal energy performance,affording high-performance Li metal batteries with a high areal energy of~25.3 mW h cm^(-2),a high volumetric power density of~1720 W L^(-1),and an outstanding specific energy of~470 W h kg^(-1)at only 6 mA h cm^(-2).

关键词： Thick cathode Polyhydroxyalkanoate binder Nano-bridging Conductive nano-fibrillar network Lithium metal battery

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