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Broad-Learning-System-Based Model-Free Adaptive Predictive control for Nonlinear MASs Under DoS Attacks

IEEE/CAA Journal of Automatica Sinica 2025年第2期12卷 381-393页

作者： Hongxing Xiong Guangdeng Chen Hongru Ren Hongyi Li the School of Automation Guangdong-Hong Kong Joint Laboratory for Intelligent Decision and Cooperative Control Guangdong University of Technology Guangdong Provincial Key Laboratory for Intelligent Decision and Cooperative Control Guangdong University of Technology the College of Electronic and Information Engineering Southwest University IEEE

In this paper, the containment control problem in nonlinear multi-agent systems(NMASs) under denial-of-service(DoS) attacks is addressed. Firstly, a prediction model is obtained using the broad learning technique to train historical data generated by the system offline without DoS attacks. Secondly, the dynamic linearization method is used to obtain the equivalent linearization model of NMASs. Then, a novel model-free adaptive predictive control(MFAPC) framework based on historical and online data generated by the system is proposed, which combines the trained prediction model with the model-free adaptive control method. The development of the MFAPC method motivates a much simpler robust predictive control solution that is convenient to use in the case of DoS attacks. Meanwhile, the MFAPC algorithm provides a unified predictive framework for solving consensus tracking and containment control problems. The boundedness of the containment error can be proven by using the contraction mapping principle and the mathematical induction method. Finally, the proposed MFAPC is assessed through comparative experiments.

关键词： Broad learning technique denial-of-service (DoS) model-free adaptive predictive control (MFAPC) nonlinear multi-agent systems (NMASs)

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Green disposal of waste smartphone protective film:Efficiency,mechanism,bench-scale test and secondary waste reutilization

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Journal of Environmental Sciences 2025年第5期151卷 692-702页

作者： Jiangyao Chen Shunyu Ding Chenxu Gao Canhui Chen Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

The manufacture and obsolescence of smartphones produce numerous waste plastic accessories(e.g.,waste smartphone protective film(WSPF)),possessing immense potential for ***,available recycling technologies have limitations such as substrate damage and secondary pollutant *** present study aimed to develop a green disposal method that not only recycled polyethylene terephthalate(PET)from WSPF,but also reused the stripped polyacrylate(PAA)adhesive as an adsorbent to reduce solid waste *** the WSPF was treated in 1 mol/L NaOH solution at 90°C,the PAA hydrolyzed to two main by-products of 1-butanol and 2-ethylhexanol,weakening the binding strength between PAA and PET and then efficient separation of *** bench-scale test revealed that over 97.2%of detachment efficiency toward PAA was achieved during continuous treatment of 17 batches of WSPF(200 g for each)without supplement of NaOH and generation of ***,the economic evaluation indicated that the recycling method would generate a net profit margin of 647%for the second year without considering the incurrence of new cost and ***,the pyrolysis of waste PAA enabled its conversion into potential adsorbent,which showed 2 to 4 times enhanced adsorption capacity toward styrene and ethyl acetate after modification with NaOH *** study provides a green method for recycling waste plastics and inspires a referable solution for solid waste treatment in the smartphone industry.

关键词： Smartphone accessory Waste protective film Green recycle Polyethylene terephthalate Polyacrylate Adsorbent

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Research progress on secondary formation,photosensitive reaction mechanism and human health effects of chromophoric brown carbon

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Journal of Environmental Sciences 2025年第5期151卷 310-330页

作者： Baihang Chen Jiangyao Chen Guiying Li Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment Engineering Guangzhou Key Laboratory of Environmental Catalysis and Pollution ControlSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Brown carbon(BrC)has attracted widespread attention because of its strong absorption of solar radiation in the ultraviolet-visible wavelength range,which causes adverse impacts on human ***,BrC was a physically defined class of ***,current research has gradually shifted towards the identification of its chemical groups,because its light-absorbing capability,chemical properties and health effects mainly depend on the chemical composition of its ***,this review mainly focuses on the chemical understanding of BrC based on chromophores,and the secondary formation mechanism of chromophores,photosensitized reactions,and human health effects of BrC were detailly ***,BrC chromophores are divided into five categories:nitrogen-heterocycles,nitrogen-chain,aromatic species,oligomers and sulfur-containing organic *** chromophore precursor species exhibit variations,and their formation mechanisms are also ***,BrC can trigger the production of secondary organic aerosol(SOA)precursors or cause SOA growth because BrC is an important component of light-absorbing particles formed during incomplete combustion of biomass and fossil fuels,potentially exerting adverse effects on human ***,developing sufficiently separated methods for BrC and refining algorithms and machine learning can lead to a more effective understanding of the chemical composition of chromophores,thus enabling better evaluation of the atmospheric effects and health impacts of *** all,this review provides new insights into the categories of BrC chromophores and new advance in secondary formation mechanisms,photosensitized reactions,and human health effects on the basis of chemical structures.

关键词： Brown carbon Constituent characteristics Secondary formation mechanism Photosensitive Human health effects

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Carbonyl-amine condensation coupled ozonolysis of dipropylamine and styrene:Decay kinetics,reaction mechanism,secondary organic aerosol formation and cytotoxicity

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Journal of Environmental Sciences 2025年第3期149卷 444-455页

作者： Wanying Li Jiangyao Chen Qinhao Lin Yuemeng Ji Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Oxidation of organic amines(OAs)or aromatic hydrocarbons(AHs)produces carbonyls,which further react with OAs to form carbonyl-amine condensation products,threatening environmental quality and human ***,there is still a lack of systematic understanding of the carbonyl-amine condensation reaction processes of OAs or between OAs and AHs,and subsequent environmental health *** work systematically investigated the carbonyl-amine condensation coupled ozonolysis kinetics,reaction mechanism,secondary organic aerosol(SOA)formation and cytotoxicity fromthe mixture of dipropylamine(DPA)and styrene(STY)by a combined method of productmass spectrometry identification,particle property analysis and cell exposure *** results from ozonolysis of DPA and STY mixture revealed that STY inhibited the ozonolysis of DPA to different degrees to accelerate its own decay *** barycenter of carbonyl-amine condensation reactionswas shifted from inside of DPA to between DPA and STY,which accelerated STY ozonolysis,but slowed down DPA *** the first time,ozonolysis of DPA and STY mixture to complex carbonyl-amine condensation products through the reactions of DPA with its carbonyl products,DPA with STY’s carbonyl products and DPA’s bond breakage product with STY’s carbonyl products was *** condensation products significantly contributed to the formation and growth of *** SOA containing particulate carbonyl-amine condensation products showed definite *** findings are helpful to deeply and comprehensively understand the transformation,fate and environmental health effects of mixed organics in atmospheric environment.

关键词： Organic amines(OAs) Aromatic hydrocarbons(AHs) Coupled ozonolysis Carbonyl-amine condensation Secondary pollution Toxicity assessment

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Assessment of internal exposure risk from metals pollution of occupational and non-occupational populations around a non-ferrous metal smelting plant

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Journal of Environmental Sciences 2025年第1期147卷 62-73页

作者： Yingjun Wu Mengdie Qi Hang Yu Guiying Li Taicheng An Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and Health Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Key Laboratory for City Cluster Environmental Safety and Green DevelopmentSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Non-ferrous metal smelting poses significant risks to public ***,the copper smelting process releases arsenic,a semi-volatile metalloid,which poses an emerging exposure risk to both workers and nearby *** comprehensively understand the internal exposure risks of metal(loid)s from copper smelting,we explored eighteen metal(loid)s and arsenic metabolites in the urine of both occupational and non-occupational populations using inductively coupled plasma mass spectrometry with high-performance liquid chromatography and compared their health *** showed that zinc and copper(485.38 and 14.00μg/L),and arsenic,lead,cadmium,vanadium,tin and antimony(46.80,6.82,2.17,0.40,0.44 and 0.23μg/L,respectively)in workers(n=179)were significantly higher compared to controls(n=168),while Zinc,tin and antimony(412.10,0.51 and 0.15μg/L,respectively)of residents were significantly higher than ***,workers had a higher monomethyl arsenic percentage(MMA%),showing lower arsenic methylation *** appointment analysis identified arsenic,lead,cadmium,antimony,tin and thallium as co-exposure metal(loid)s from copper smelting,positively relating to the age of *** hazard index(HI)of workers exceeded 1.0,while residents and control were approximately at ***,all three populations had accumulated cancer risks exceeding 1.0×10^(-4),and arsenite(AsIII)was the main contributor to the variation of workers and ***,residents living closer to the smelting plant had higher health *** study reveals arsenic exposure metabolites and multiple metals as emerging contaminants for copper smelting exposure populations,providing valuable insights for pollution control in non-ferrous metal smelting.

关键词： Arsenic metabolites Metal(loid)s Non-ferrous metal smelting Human biomonitoring Exposure Urine

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Impact of coking plant to heavy metal characteristics in groundwater of surrounding areas:Spatial distribution,source apportionment and risk assessments

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Journal of Environmental Sciences 2025年第3期149卷 688-698页

作者： Congqing Wang Wanjun Wang ChaoWang Shixing Ren Yingjun Wu Meicheng Wen Guiying Li Taicheng An Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory Environmental Catalysis and Pollution Control Key Laboratory of City Cluster Environmental Safety and Green developmentSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Coking industry is a potential source of heavy metals(HMs)***,its impacts to the groundwater of surrounding residential areas have not been well *** study investigated the pollution characteristics and health risks of HMs in groundwater nearby a typical coking *** HMs including Fe,Zn,Mo,As,Cu,Ni,Cr,Pb and Cd were *** average concentration of total HMswas higher in the nearby area(244.27μg/L)than that of remote area away the coking plant(89.15μg/L).The spatial distribution of pollution indices including heavy metal pollution index(HPI),Nemerow index(NI)and contamination degree(CD),all demonstrated higher values at the nearby residential areas,suggesting coking activity could significantly impact the HMs distribution *** sources of HMs were identified by Positive Matrix Factorization(PMF)model,which indicated coal washing and coking emission were the dominant sources,accounted for 40.4%,and 31.0%,*** ingestionwas found to be the dominant exposure pathway with higher exposure dose to children than *** quotient(HQ)values were below 1.0,suggesting negligible non-carcinogenic health risks,while potential carcinogenic risks were from Pb and Ni with cancer risk(CR)values>10−*** Carlo simulation matched well with the calculated results with HMs concentrations to be the most sensitive *** study provides insights into understanding how the industrial coking activities can impact the HMs pollution characteristics in groundwater,thus facilitating the implement of HMs regulation in coking industries.

关键词： Coking industry Heavy metal Groundwater Spatial distribution Source apportionment Monte Carlo simulation

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Effects of triclosan adsorption on intestinal toxicity and resistance gene expression in Xenopus tropicalis with different particle sizes of polystyrene

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Journal of Environmental Sciences 2024年第12期146卷 176-185页

作者： Zhuo Dai Zikai Wang Xinying Pan Li Zheng Yanbin Xu Qingxia Qiao Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangzhou Key Laboratory Environmental Catalysis and Pollution ControlInstitute of Environmental Health and Pollution ControlCollege of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Microplastics(MPs)are commonly found with hydrophobic contaminants in the water column and pose a serious threat to aquatic *** effects of polystyrene microplastics of different particle sizes on the accumulation of triclosan in the gut of Xenopus tropicalis,its toxic effects,and the transmission of resistance genes were *** results showed that co-exposure to polystyrene(PS-MPs)adsorbed with triclosan(TCS)caused the accumulation of triclosan in the intestine with the following accumulation capacity:TCS+5μm PS group>TCS group>TCS+20μm PS group>TCS+0.1μm PS *** experimental groups showed increased intestinal inflammation and antioxidant enzyme activity after 28 days of exposure to PS-MPs and TCS of different particle *** TCS+20μm PS group exhibited the highest upregulated expression of pro-inflammatory factors(IL-10,IL-1β).The TCS+20μm group showed the highest increase in enzyme activity compared to the control ***-MPs and TCS,either alone or together,altered the composition of the intestinal microbial *** addition,the presence of more antibiotic resistance genes than triclosan resistance genes significantly increased the expression of tetracycline resistance and sulfonamide resistance genes,which may be associated with the development of intestinal inflammation and oxidative *** study refines the aquatic ecotoxicity assessment of TCS adsorbed by MPs and provides informative information for the management and control of microplastics and non-antibiotic bacterial inhibitors.

关键词： Polystyrene Triclosan Xenopus-tropicalis Resistance genes Gut community

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Photodegradation of xylene isomers:Kinetics,mechanism,secondary pollutant formation potential and health risk evaluation

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Journal of Environmental Sciences 2024年第2期136卷 658-669页

作者： Xiaoyan Chen Weikun Zhu Sufen Feng Jiangyao Chen Guangdong Key Laboratory of Environmental Catalysis and Health Risk Control Guangdong Technology Research Center for Photocatalytic Technology Integration and Equipment EngineeringInstitute of Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and HealthSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Photodegradation technology has been widely applied in the purification of industrial aromatic ***,whether this technology efficiently removes the pollutants to prevent secondary pollution and health risk is still ***,the photodegradation processes of three xylenes were compared under designed reaction atmospheres and light *** lamp showed poor photodegradation ability toward xylenes,no matter in N_(2) or N_(2)+O_(2)system,while much higher photodegradation performance of xylenes were obtained under ultraviolet(UV)and vacuum ultraviolet(VUV)irradiation,especially in N_(2)+O_(2)+VUV system,where 97.9%of m-xylene,99.0%of o-xylene or 87.5%of p-xylene with the initial concentration of 860 mg/m^(3) was removed within 240 *** xylenes underwent three processes of photo-isomerization,photodecomposition and photo-oxidation to produce intermediates of aromatics,alkanes and *** them,the photo-isomerization products showed the highest concentration percentage(e.g.,≥50%in o-xylene system),confirming that photo-isomerization reaction was the dominated photodegradation process of ***,these isomerized products not only contributed about 97%and91%to the formation potential of O3(OFP)and secondary organic aerosols(SOAFP),but also displayed obvious non-carcinogenic risk,although one of photodecomposition product—benzene showed the highest occupational exposure ***,the secondary pollution and health risks of photodegradation products of xylenes were non-ignorable,although the OFP,SOAFP and health risks of the generated products reduced at least 4.5 times in comparison with that of the degraded *** findings are helpful for the appropriate application of this technology in the purification of industrial organic waste gas.

关键词： Isomer aromatics Photodegradation Ozone formation Secondary organic aerosols Health risk

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Mechanisms of isomerization and hydration reactions of typicalβ-diketone at the air-droplet interface

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Journal of Environmental Sciences 2024年第7期141卷 225-234页

作者： Yuemeng Ji Weiyong Luo Qiuju Shi Xiaohui Ma Ziqi Wu Weina Zhang Yanpeng Gao Taicheng An Guangdong-Hong Kong-Macao Joint Laboratory for Contaminants Exposure and Health Guangdong Key Laboratory of Environmental Catalysis and Health Risk ControlInstitute Environmental Health and Pollution ControlGuangdong University of TechnologyGuangzhou 510006China Guangzhou Key Laboratory of Environmental Catalysis and Pollution Control Key Laboratory for City Cluster Environmental Safety and Green Development of the Ministry of EducationSchool of Environmental Science and EngineeringGuangdong University of TechnologyGuangzhou 510006China

Acetylacetone(AcAc)is a typical class ofβ-diketones with broad industrial applications due to the property of the keto-enol isomers,but its isomerization and chemical reactions at the air-droplet interface are still ***,using combined molecular dynamics and quantum chemistry methods,the heterogeneous chemistry of AcAc at the air-droplet interface was investigated,including the attraction of AcAc isomers by the droplets,the distribution of isomers at the air-droplet interface,and the hydration reactions of isomers at the air-droplet *** results reveal that the preferential orientation of two AcAc isomers(keto-and enol-AcAc)to accumulate and accommodate at the acidic air-droplet *** isomerization of two AcAc isomers at the acidic air-droplet interface is more favorable than that at the neutral air-droplet interface because the“water bridge”structure is destroyed by H_(3)O^(+),especially for the isomerization from keto-Ac Ac to *** the acidic air-droplet interface,the carbonyl or hydroxyl O-atoms of two AcAc isomers display an energetical preference to ***-diol is the dominant products to accumulate at the air-droplet interface,and excessive keto-diol can enter the droplet interior to engage in the *** photooxidation reaction of AcAc will increase the acidity of the air-droplet interface,which indirectly facilitate the uptake and formation of more *** results provide an insight into the heterogeneous chemistry ofβ-diketones and their influence on the environment.

关键词： Acetylacetone Air-droplet interface Theoretical simulation Isomerization Hydration reaction mechanism

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Neural-based prescribed-time consensus control for multiagent systems via dynamic memory event-triggered mechanism

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Science China(Technological Sciences) 2025年第3期68卷 217-227页

作者： Xiaohong ZHENG Hui MA Qi ZHOU Hongyi LI School of Automation Guangdong-Hong Kong Joint Laboratory for Intelligent Decision and Cooperative Controland Guangdong Provincial Key Laboratory for Intelligent Decision and Cooperative ControlGuangdong University of TechnologyGuangzhou510006China School of Mathematics and Statistics Guangdong University of TechnologyGuangzhou510006China College of Electronic and Information Engineering and the Chongqing Key Laboratory of Generic Technology and System of Service Robots Southwest UniversityChongqing400715China

This work investigates the implementation of distributed prescribed-time neural network(NN)control for nonlinear multiagent systems(MASs)using a dynamic memory event-triggered mechanism(DMETM).First,it introduces a composite learning technique in NN *** method leverages the prediction error within the NN update law to enhance the accuracy of the unknown nonlinearity ***,by introducing a time-varying transformation,the study establishes a distributed prescribed-time control *** notable feature of this algorithm is its ability to predetermine the convergence time independently of initial conditions or control ***,the DMETM is established to reduce the actuation frequency of the *** the conventional memoryless dynamic event-triggered mechanism,the DMETM incorporates a memory term to further increase triggering *** a distributed estimator for the leader,the DMETM-based NN prescribed-time controller is designed in a fully distributed manner,which guarantees that all signals in the closed-loop system remain bounded within the prescribed ***,simulation results are presented to validate the effectiveness of the proposed algorithm.

关键词： consensus control composite learning control dynamic memory event-triggered control prescribed-time control multiagent systems(MASs)

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