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Environmental Functional Materials 2024年第1期3卷 72-93页

作者： Xinchun Lu Liguo Shen Cheng Chen Wei Yu Boya Wang Ning Kong Qianqian Zeng Siyuan Chen Xuezheng Huang Ying Wang Hongjun Lin College of Geography and Environmental Sciences Zhejiang Normal University Jinhua 321004 PR China Henan Province Key Laboratory of Water Pollution Control and Rehabilitation Technology Henan University of Urban Construction Pingdingshan 467000 PR China State Key Laboratory of Pollution Control and Resources Reuse (Tongji University) College of Environmental Science and Engineering Tongji University Shanghai 200092 PR China

The formidable challenge of membrane fouling by high-viscosity oils remains a primary impediment to the sustainable application of separation membranes in treating oil-contaminated wastewater. Consequently, there is an imperative for the development of oil-contaminated wastewater treatment membranes endowed with self-cleansing capabilities. The current review aims to delineate the landscape of self-cleansing membranes tailored for the treatment of oil-contaminated wastewater. Embarking from the foundational theories and benchmarks of self-cleansing, the self-cleansing functionalities were classified into active and passive modalities. We encapsulate the strides made in research, encompassing domains such as super-wettable surfaces, synchronously filtered self-cleansing, and post-filtration high-efficiency self-cleansing, while concurrently identifying extant constraints and prospective trajectories. By meticulously categorizing and dissecting self-cleansing functionalities, the aim of this work is delving into the fundamental tenets of self-cleansing within membranes intended for treating oil-contaminated wastewater, and furnishing guidance for the design and advancement of self-cleansing functionalities in oil-water separation membranes.

关键词： Membrane fouling Oil/water separation Self-cleaning Superwetting surfaces Functional material

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Comprehensive review of ecological risks and toxicity mechanisms of microplastics in freshwater: Focus on zebrafish as a model organism

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Aquatic Toxicology 2025年 284卷 107397页

作者： Sha, Haichao Li, Xi Li, Qi Zhang, Jingwei Gao, Ji Ge, Lukun Wang, Weinan Zeng, Taotao Xi'an Key Laboratory of Environmental Simulation and Ecological Health in the Yellow River Basin College of Urban and Environmental Sciences Northwest University Xi'an 710127 China Hunan Province Key Laboratory of Pollution Control and Resources Reuse Technology University of South China Hunan Hengyang 421001 China

Zebrafish, as a model organism, exhibit high sensitivity to environmental pollutants and has been widely used in microplastics (MPs) toxicology studies. However, the mechanisms underlying MPs’ effects on zebrafish have yet to be comprehensively summarized. This review systematically explores the sources, pollution status of freshwater MPs and their biological toxicity mechanisms using zebrafish as a model organism. This analysis reveals that the primary sources of MPs include sediment release, natural degradation of plastic products, and precipitation-mediated transport. Freshwater MPs predominantly comprise of polyethylene (PE), polypropylene (PP), polyethylene terephthalate (PET), polystyrene (PS), and polyvinyl chloride (PVC). These MPs typically appear transparent, white, black, or blue, and predominantly exist as fibers, films, fragments, foams, and particles. The concentration, size, shape, type, aging status, and loading capacity of MPs can induce developmental malformations in zebrafish embryos, including pericardial and yolk sac edema. In adult zebrafish, MPs cause intestinal injuries characterized by increased permeability, impaired barrier function, and microbiota dysbiosis. MPs exposure also induces behavioral abnormalities such as reduced locomotion and anxiety-like responses, while simultaneously provoking oxidative stress and immune-inflammatory reactions. The physical mechanism of MPs-induced toxicity in zebrafish involves particle accumulation and tissue abrasion. In contrast, physiological and molecular mechanisms encompass interactions between MPs’ surface functional groups and biological tissues, alterations in oxidative stress markers, enzymatic activity and cytokine profiles, and modulation of gene expression patterns. This review synthesizes current knowledge on the ecological risks of freshwater MP pollution and its toxicological impacts on zebrafish, thereby providing a comprehensive framework for understanding MP toxicity mechanisms. © 2025

关键词： Danio rerio Molecular actions Physical action Physiological pollution status Sources

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Screening legacy and emerging organic pollutants in the contaminated soil of Dhaka,Bangladesh

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Emerging Contaminants 2024年第3期10卷 343-353页

作者： Refayat Nigar Shizhen Zhao Xin Liu Huanfang Huang Lele Tian Yuwei Xiao Ahsan Habib Gan Zhang State Key Laboratory of Organic Geochemistry Guangzhou Institute of GeochemistryChinese Academy of SciencesGuangzhou510640China Guangdong-Hong Kong-Macao Joint Laboratory for Environmental Pollution and Control and Guangdong Provincial Key Laboratory of Environmental Protection and Resources Utilization Guangzhou510640China Anti-Drug Technology Center of Guangdong Province and National Anti-Drug Laboratory Guangdong Regional Center Guangzhou510230China State Environmental Protection Key Laboratory of Water Environmental Simulation and Pollution Control South China Institute of Environmental SciencesMinistry of Ecology and EnvironmentGuangzhou510530China Department of Chemistry University of DhakaDhaka1000Bangladesh University of Chinese Academy of Sciences Beijing100049China

The current understanding of the legacy and emerging organic pollutants in the soil of Bangladesh remains *** disposal practices,particularly in e-waste,landfills,and industrial operations,may lead to the pervasive presence of persistent organic pollutants(POPs)and polycyclic aromatic hydrocarbons(PAHs)in the *** study aimed to systematically investigate the concentrations,sources,and risk assessment of halogenated flame retardants(HFRs),polychlorinated biphenyls(PCBs),polychlorinated naphthalenes(PCNs),organochlorine pesticides(OCPs),chlorinated paraffins(CPs),and PAHs in the contaminated soil of Dhaka's dumpsites,e-waste,and industrial areas collected in *** total concentration of investigated pollutants averaged at 4790±4040 ng g^(-1)dw,with the following order:P44CPs(4110±4140 ng g^(-1)dw)>P16PAHs(422±491 ng g^(-1)dw)>P16HFRs(190±538 ng g^(-1)dw)>P209PCBs(43.5±73.5 ng g^(-1)dw)>P50PCNs(17.7±21.0 ng g^(-1)dw)>P27OCPs(9.41±9.61 ng g^(-1)dw).The e-waste site exhibited the highest total concentration of the target pollutants,reaching 12,700 ng g1 *** were the predominant contributors,accounting for averages of 81.8%,70.5%,and 68.5%to waste landfills,e-waste,and industrial sites,respectively.A comprehensive analysis of 209 PCB congeners revealed their primary origin from Aroclor PCBs,with minor contributions from unintentionally produced *** highest incremental lifetime carcinogenic risk(ILCR)occurred in e-waste sites,contributed by dioxin-like PCBs,with a maximum value of 5.9×10^(-5)for adults,exceeding the limit 1.0×10^(-6)set by the *** non-carcinogenic hazard quotients(HQs)were much lower,suggesting no significant risk from the investigated *** findings highlight the importance of proper waste management and regulated e-waste recycling to mitigate potential hazardous risks to the Bangladeshi population.

关键词： Persistent organic pollutants Polycyclic aromatic hydrocarbons Chlorinated paraffins Polychlorinated biphenyls Risk assessment Contaminated soil Bangladesh

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Facet-controlled LiMn_(2)O_(4)/C as Deionization Electrode with Enhanced Stability and High Desalination Performance

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Nano-Micro Letters 2022年第11期14卷 75-86页

作者： Yuxin Jiang Liyuan Chai Dehe Zhang Fangping Ouyang Xiangyuan Zhou Sikpaam IAlhassan Sailin Liu Yingjie He Lvji Yan Haiying Wang Wenchao Zhang School of Metallurgy and Environment Central South UniversityChangsha 410083People’s Republic of China Chinese National Engineering Research Center for Control and Treatment of Heavy Metal Pollution Changsha 410083People’s Republic of China Water Pollution Control Technology Key Lab of Hunan Province Changsha 410083People’s Republic of China School of Physics and Electronics Hunan Key Laboratory for Super-Microstructure and Ultrafast Processand Hunan Key Laboratory of Nanophotonics and DevicesCentral South UniversityChangsha 410083People’s Republic of China State Key Laboratory of Powder Metallurgy and Powder Metallurgy Research InstituteCentral South UniversityChangsha 410083People’s Republic of China School of Chemical Engineering and Advanced Materials Faculty of SciencesEngineering and TechnologyThe University of AdelaideAdelaide 5005Australia

Battery materials as emerging capacitive deionization electrodes for desalination have better salt removal capacities than traditional carbon-based ***_(2)O_(4),a widely used cathode mate-rial,is difficult to utilize as a deionization electrode due to its structural instability upon cycling and Mn dissolution in aqueous-based ***,a facile and low-cost ball-milling routine was proposed to prepare a LiMn_(2)O_(4)material with highly exposed(111)*** prepared electrode exhibited relatively low dissolution of Mn during cycling,which shows its long cycle *** the hybrid capacitive deionization system,the LiMn_(2)O_(4)/C electrode delivered a high desalination capacity of 117.3 mg g^(−1) without obvious capacity decay at a voltage of 1.0 V with a 20 mM initial salt *** addition,the exposed(111)facets significantly alleviated Mn ion dissolution,which also enhanced the structural steadiness.

关键词： Deionization electrode Desalination Lithium-ion battery

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Study on Coconut Shell Activated Carbon Temperature Swing Adsorption of Benzene and Formaldehyde

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Journal of Renewable Materials 2022年第12期10卷 3573-3585页

作者： Zhiguang Yang Gaojun Yan Xueping Liu Zhengyuan Feng Xinfeng Zhu Yanli Mao Songtao Chen Zhisheng Yu Ruimei Fan Linlin Shan Henan Province Key Laboratory of Water Pollution Control and Rehabilitation Technology Henan University of Urban ConstructionPingdingshan467036China College of Resources and Environment University of Chinese Academy of SciencesBeijing100085China College of Basic Medical Sciences Xinxiang Medical UniversityXinxiang 453003China

Adsorption can be used to recover effectively the volatile organic gases(VOCs)in the exhaust gas from factories through using an appropriate adsorption *** to form a physical or chemical bond,adsorption occurs between the porous solid medium and the liquid or gas multi component fluid *** regeneration capa-city of the adsorbent is as important as the adsorption capacity and it determines the economics of the adsorption *** regeneration of adsorbent can be realized through changing the pressure or temperature of the ***,activated carbon samples from coconut shell were prepared and *** or formal-dehyde in the mixed air was used as the adsorption object,and the adsorption experiment was carried out in a U-shaped *** how adsorption was affected by activated carbon type,adsorbate and *** results show that oxidation modifed activated carbon can increase the adsorption effect of form aldehyde,but will reduce the ad sorption effect of benzene,because their ad sorption mechanism is *** 30℃,the saturated adsorption apacity of AC-0 for benzene is 437.0 mg/*** that of AC-1 for formaldehyde is 670.5 mg/*** the experimental range,it is found that the adsorption capacity increases with the decrease of temperature,and their changes are very consistent with the ftted ExpDecay1 function.

关键词： Activated carbon adsorption benzene formaldehyde oxidation modification

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Comparison of the meat quality and fatty acid profile of muscles in finishing Xiangcun Black pigs fed varied dietary energy levels

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Animal Nutrition 2022年第4期11卷 15-24页

作者： Can Yang Wenlong Wang Xiaowu Tang Ruilin Huang Fengna Li Wenxuan Su Yulong Yin Chaoyue Wen Jian Liu College of Life Sciences and Environment Hunan Provincial Key Laboratory of Biological Resources Protection and Utilization in Nanyue Mountain AreaHengyang Normal UniversityHengyangHunan 421008China Key Laboratory of Agro-ecological Processes in Subtropical Region National Engineering Laboratory for Pollution Control and Waste Utilization in Livestock and Poultry ProductionInstitute of Subtropical AgricultureChinese Academy of ScienceChangsh1Hunan 410125China Hunan International Joint Laboratory of Animal Intestinal Ecology and Health Hunan Normal UniversityChangshaHunan 410081China College of Bioengineering Hunan Vocational Technical College of Environment and BiologyHengyangHunan 421005China Key Laboratory of Animal Feed and Nutrition of Zhejiang Province College of Animal SciencesZhejiang UniversityHangzhou 310058China Xiangcun High-technology Agricultural Co.LTD LoudiHunan 417000China

To study the effects of dietary energy level on the meat quality of different muscles in finishing pigs,400Xiangcun Black pigs(BW=79.55±4.77 kg)were randomly assigned to 5 treatments with varied calculated digestive energy(DE)at 3,050,3,100,3,150,3,200 and 3,250 kcal/kg,*** treatment had 8replicates with 10 pigs per *** quality,amino acid and fatty acid composition were tested in this *** differences in average daily gain,average daily feed intake or feed-to-gain ratio(P>0.05)were observed among dietary *** concentrations of longissimus dorsi(LD)muscle in DE3150was higher than those in other groups(P<0.05).The crude fat concentration of biceps femoris(BF)muscle in DE3250 tended to be higher than that in DE3150 and DE3100 groups(P<0.05).Pigs in DE3250 and DE3200 had higher fiber density and smaller cross-sectional area of BF muscle than those in DE3150(P<0.05).Pigs in DE3150 had the highest Cu concentration in LD muscle compared with those in DE3200,DE3250(P<0.05).The C16:1 proportion of LD muscle was lower(P<0.01)and C20:1 was higher(P<0.05)in DE3050 than that in the other dietary *** C18:3n6 and C20:3n6 proportions of BF muscle in DE3150 were higher than those in DE 3050,DE3200 and DE3250(P<0.05).For LD muscle,m RNA expressions of type I and IIa MyHC in group DE3150 were higher than other treatments(P<0.01).The LD muscle in DE3150 expressed higher PPARd than in other groups(P<0.01).Pigs in DE3100 expressed higher FOX1 than in DE3200 and DE3250(P<0.05).Sterol-regulatory element binding proteins(SREBPa)mRNA expression decreased linearly when dietary energy level increased in BF muscle(P<0.01).In conclusion,a200 kcal/kg decrease in digestible energy for 4 consecutive weeks did not affect growth performance of Xiangcun Black ***,LD and BF muscle respond differently to dietary energy level,and meat quality was improved by the medium energy level during the finishing phase.

关键词： Energy Growth performance Fatty acid Myofibrillar morphology Muscle

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The combined metabolism and transcriptome of tail muscles reveal the effects of antimony pulse exposure on swimming behavior of Pelophylax nigromaculatus tadpoles

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Science of the Total Environment 2025年 958卷 177929页

作者： Huang, Minyi Cao, Songle Huang, Ying Tan, Zikang Duan, Renyan College of Agriculture and Biotechnology Hunan University of Humanities Science and Technology Hunan Loudi417000 China Key Laboratory of Development Utilization Quality and Safety Control of Characteristic Agricultural Resources in Central Hunan Province Hunan Loudi417000 China

Due to the periodic emission of pollutants, the exposure mode of contaminants in water bodies is mostly pulse exposure, and the toxic effects of fluctuating exposure on aquatic animals are not consistent with traditional toxicological experiments of constant exposure. The toxic effects of heavy metal antimony (Sb) on the swimming behavior of Pelophylax nigromaculatus tadpoles after pulse exposure (PESb) and continuous exposure (CESb) for 28 days were explored. The mechanisms were analyzed from the perspectives of tail muscle metabolism and transcriptomics. Compared to the control group, PESb and CESb decreased the average speed of P. nigromaculatus tadpoles by 25.72 % and 18.08 %, respectively. PESb and CESb led to changes in 70 and 24 metabolites of tail muscle, respectively. PESb led to alterations in metabolic pathways related to pyrimidine metabolism, arginine biosynthesis, and glycerophospholipid metabolism. In contrast, CESb altered metabolic pathways such as alanine, aspartate, and glutamate metabolism. Compared to the control, 1225 and 1139 DEGs were identified for PESb and CESb, respectively. These DEGs were mainly associated with functions such as immune response, DNA replication, protein digestion, and absorption. It can be seen that PESb and CESb can alter the metabolism and transcriptome of the tail muscle of P. nigromaculatus tadpoles, leading to differential expression of individual movements. © 2024 Elsevier B.V.

关键词： Invertebrates

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Development of Methylene Bis-Benzotriazolyl Tetramethylbutylphenol-grafted lignin sub-microspheres loaded with TiO_(2) for sunscreen applications

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Journal of Bioresources and Bioproducts 2024年第4期9卷 534-547页

作者： Yarong Li Zhiguang Tang Xiaohan Zhou Junhua Zhang Xueping Song Kai Li Wei Liu Zhanying Zhang College of Light Industry and Food Engineering Guangxi UniversityNanning530004China Province and Ministry Co-Sponsored Collaborative Innovation Center of Cane Sugar Industry Nanning530004China Jiangsu Co-Innovation Center of Efficient Processing and Utilization of Forest Resources College of Chemical EngineeringNanjing Forestry UniversityNanjing210037China Guangxi Key Laboratory of Clean Pulp&Papermaking and Pollution Control Nanning530004China Tianjin Key Laboratory of Pulp&Paper Tianjin University of Science&TechnologyTianjin300457China School of Mechanical Medical and Process EngineeringCentre for Agriculture and the BioeconomyQueensland University of TechnologyQueensland4000Australia

Lignin serves as a promising Ultraviolet(UV)absorber within sunscreen ***,the commercial development of lignin-containing sunscreens faces challenges due to their low sun protection factor(SPF)and dark color in cosmetics *** this study,dual modifications on the chemical and physical structures of lignin were conducted to address these ***,methylene bis-benzotriazolyl tetramethylbutylphenol(MBBT)was grafted onto alkali lignin(AL)through an atom transfer radical polymerization reaction,resulting in a polymer of AL-graft-MBBT_(3)(AL-g-MBBT_(3)).The sunscreen prepared with 10%AL-g-MBBT_(3) displays outstand-ing sun protection performance with a SPF of 42.93 and a light color with a color difference value(ΔE)of 45.6,in contrast to 10%AL with a SPF of 4.74 and aΔE value of ***,AL-g-MBBT_(3) was transformed into normal submicron spheres(AL-g-MBBT_(3) N)and TiO_(2)-loading submicron spheres(AL-g-MBBT_(3)/TiO_(2)).The sun protection performances of 10%AL-g-MBBT_(3) N@C and AL-g-MBBT_(3)/TiO_(2)@C sunscreens obviously surpass that of AL-g-MBBT_(3)@C sunscreen,achieving SPFs of 60.38 and 66.20,***,there is a considerable improve-ment in the color of these sunscreens,withΔE values of 41.8 and 36.3,*** results provide valuable insights into exploring lignin’s high-value applications in sunscreen.

关键词： Lignin Graft Submicron sphere TiO_(2) Anti-UV performance Color

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Localized heating coupling with radical oxidation eliminating antibiotic resistance genes (ARGs) in interfacial photothermal Fenton-like disinfection process

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Science of the Total Environment 2024年 955卷 176779页

作者： Hou, Haozheng Zou, Dingli Shi, Weiye Wang, Yingying Ma, Defang Wang, Yan Li, Qian Gao, Yue Gao, Baoyu Shandong Key Laboratory of Water Pollution Control and Resource Reuse School of Environmental Science and Engineering Shandong University Qingdao266237 China No.1 Institute of Geology and Mineral Resources of Shandong Province Jinan250014 China

Conventional oxidative disinfection processes are inefficient in eliminating intracellular antibiotic resistance genes (iARGs) due to the barrier of the cell membrane and the competitive reaction of cellular constituents within antibiotic-resistant bacteria (ARB), resulting in the widespread prevalence of ARGs in recycled water. This study presented the first application of localized heating coupling with advanced oxidation to destroy the resistant Escherichia coli cells and improved subsequent iARGs (blaTEM-1) degradation in a novel photothermal Fenton-like disinfection process. The Fe-Mn@CNT microfiltration membrane, comprising carbon nanotubes wrapped with Fe and Mn nanoparticles (Fe-Mn@CNT), was employed as a nanomaterial for photothermal conversion and H2O2 activation. The highly efficient absorption of full-spectrum photons by CNTs enabled the Fe-Mn@CNT membrane to concentrate light to generate localized intense heat, resulting in the destruction of ARB nearby, and the subsequent release of iARGs. Interfacial heat favored Fe-Mn-induced H2O2 activation, leading to the production of more ·OH, which in turn promoted the oxidation for ARG degradation and ARB cell damage. The results of the acetylcysteine quenching experiments indicated that interfacial heating and radical oxidation-induced accumulation of intracellular reactive oxygen species contributed to the elimination of about 1-log iARGs through direct attack. The integrity of the cell membrane, the morphology of ARB and the variation of i/e ARG copy numbers were observed to reveal that the introduction of interfacial heating aggravated the cell lysis and accelerated the iARGs release, resulting in the inactivation of 7.27-log ARB and the elimination of 4.64-log iARGs and 2.23-log eARGs. Localized heating coupling with ·OH oxidation achieved a 143 % increase in iARGs removal compared to the conventional Fenton-like oxidation. The interfacial photothermal Fenton-like disinfection process exhibited remarkable

关键词： Escherichia coli

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Metal-center effect induced efficient charge transfer of metal-organic framework for strengthening Sb(Ⅴ)capture performance

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Nano Research 2022年第9期15卷 8516-8523页

作者： Deng You Hui Shi Mingming Peng Liming Yang Penghui Shao Kai Yin Haozhi Wang Shenglian Luo Xubiao Luo State Key Laboratory of Chemo/Biosensing and Chemometrics Hunan UniversityChangsha 410082China Key Laboratory of Jiangxi Province for Persistent Pollutants Control and Resources Recycle Nanchang Hangkong UniversityNanchang 330063China National-Local Joint Engineering Research Center of Heavy Metals Pollutants Control and Resource utilization Nanchang Hangkong UniversityNanchang 330063China Key Laboratory of Advanced Ceramics and Machining Technology(Ministry of Education) School of Materials Science and EngineeringTianjin UniversityTianjin 300072China

The adsorbents–adsorbates interaction is critical for resourcelization in heavy metal wastewater ***,it is still indistinct to depict the impact of metal center effect on heavy metals removal performance in metal-organic frameworks(MOFs)-based ***,a series of MOFs with different metal centers of Mg(II),La(III),and Zr(IV)are rationally designed,and the effect of electronic structure on the Sb(V)removal performance is systematically *** obtained La-MGs achieve Sb(V)adsorption capacity of 897.6 mg/g,which is about 1.2 and 4.5 times above average than those of Zr-MGs and Mg-MGs,*** account of more edge adsorption sites achieve,the sites utilization efficiency of La-MGs(92.1%)is much better than Zr-MGs(75.0%)and Mg-MGs(20.4%).Furthermore,density functional theory(DFT)calculations reveal that La-MGs are more active than Mg-MGs and Zr-MGs,owing to the lower adsorption energy,higher charge transfer,and stronger bonding interaction,which will promote the Sb(V)removal *** experimental results in practical water indicate that La-MGs effectively capture antimony at low concentration,reaching drinking water standard in samples from Ganjiang *** study opens an avenue for atomic-level insight into high-efficient absorbents design for water treatment from electronic structuremodification of active centers.

关键词： metal-organic frameworks metal center effect electronic structure theoretical calculation Sb(V)removal

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