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Targeting new ways for large-scale,high-speed surface functionalization using direct laser interference patterning in a roll-to-roll process

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International Journal of Extreme Manufacturing 2023年第3期5卷 569-583页

作者： Christoph Zwahr Nicolas Serey Lukas Nitschke Christian Bischoff Ulrich Radel Alexandra Meyer Penghui Zhu Wilhelm Pfleging Laser Precision Manufacturing Fraunhofer Institute for Material and Beam Technology(IWS)DresdenGermany Topag Lasertechnik GmbH DarmstadtGermany Institute of Manufacturing Science and Engineering Technical University DresdenDresdenGermany Institute for Applied Materials—Applied Materials Physics(IAM-AWP) Karlsruhe Institute of Technology(KIT)Eggenstein-LeopoldshafenGermany

Direct Laser Interference Patterning(DLIP)is used to texture current collector foils in a roll-to-roll process using a high-power picosecond pulsed laser system operating at either fundamental wavelength of 1064 nm or 2nd harmonic of 532 *** raw beam having a diameter of 3 mm@1/e^(2) is shaped into an elongated top-hat intensity profile using a diffractive so-called FBS■-L element and cylindrical *** shaped beam is split into its diffraction orders,where the two first orders are parallelized and guided into a galvanometer *** deflected beams inside the scan head are recombined with an F-theta objective on the working position generating the interference *** DLIP spot has a line-like interference pattern with about 15μm spatial *** fluences of up to 8 J cm^(-2) were achieved using a maximum pulse energy of 0.6 ***,an in-house built roll-to-roll machine was *** this setup,aluminum and copper foil of 20μm and 9μm thickness,respectively,could be *** to current collector structuring coating of composite electrode material took *** case of lithium nickel manganese cobalt oxide(NMC 622)cathode deposited onto textured aluminum current collector,an increased specific discharge capacity could be achieved at a C-rate of 1℃.For the silicon/graphite anode material deposited onto textured copper current collector,an improved rate capability at all C-rates between C/10 and 5℃ was *** rate capability was increased up to 100%compared to reference *** C-rates between C/2 and 2℃,the specific discharge capacity was increased to 200 mAh g^(-1),while the reference electrodes with untextured current collector foils provided a specific discharge capacity of 100 m Ah g^(-1),showing the potential of the DLIP technology for cost-effective production of battery cells with increased cycle lifetime.

关键词： DLIP lithium-ion battery surface texturing copper aluminum

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Tuning surface reactivity towards high-performance hard carbon in Li/Na/K-ion batteries

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Journal of Energy Chemistry 2025年第4期103卷 27-36页

作者： Wang Zhou Dan Wang Ying Mo Rui Tang Peng Gao Miaomiao Han Shi Chen Keigo Wakabayashi Takeharu Yoshii Hirotomo Nishihara Jilei Liu College of Materials Science and Engineering Hunan Joint International Laboratory of Advanced Materials and Technology of Clean EnergyHunan Province Key Laboratory for Advanced Carbon Materials and Applied TechnologyHunan UniversityChangsha 410082HunanChina The Key Laboratory of Micro-nano Energy Materials and Application Technologies University of Hunan Province&College of Physics and Electronic EngineeringHengyang Normal UniversityHengyang 421002HunanChina Joint Key Laboratory of the Ministry of Education Institute of Applied Physics and Materials EngineeringUniversity of MacaoMacao 999078China Institute of Multidisciplinary Research for Advanced Materials Tohoku University2-1-1 KatahiraAoba-kuSendaiMiyagi 980-8577Japan Advanced Institute for Materials Research(WPI-AIMR) Tohoku University2-1-1 KatahiraAoba-kuSendaiMiyagi 980-8577Japan

Controlling surface chemistry is critically important for improving the initial Coulombic efficiency(ICE)and adsorption capacity of hard carbon anode used in Li/Na/K-ion ***,accurately identifying the types and concentrations of hydrogen/oxygen terminated functional groups(HTFG/OTFGs)and distinguishing their functionalities remain ***,we quantitatively investigated the surface chemistry on hard carbon via ultra-high temperature programed desorption measurements,and uncovered the role of HTFG/OTFGs in influencing ICE and adsorption capacity in Li/Na/K-ions *** C-H group is found to be dominant species on the surface of hard carbon,and presents a positive correlation with ICE values and adsorption *** low reactivity of C-H group with both electrolyte salt and solvent results in the formation of thinner and highly conducive solid electrolyte interphase(SEI)layer,which benefit for the enhanced ICE and improved Li/Na/K-ions diffusion across SEI ***,the pimping trapping effect of C-H groups allows the adsorbed Li/Na/K-ions to migrate into graphitic interlayer quickly,enhancing the slope *** fabricating a C-H group-rich surface chemistry on hard carbon,a high ICE value and satisfactory specific capacity have been *** findings enrich our understanding of the surface chemistry-induced interfacial reaction,which effectively guides the rational design of high-performance hard carbon.

关键词： Hard carbon Surface chemistry C–H bond Initial coulombic efficiency Adsorption capacity

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Revealing the vertical structure of in-situ fabricated perovskite nanocrystals films toward efficient pure red light-emitting diodes

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Fundamental Research 2024年第2期4卷 362-368页

作者： Xian-gang Wu Shipei Sun Tinglu Song Xin Zhang Chenhui Wang Yingguo Yang Shuangpeng Wang Haizheng Zhong MIIT Key Laboratory for Low-Dimensional Quantum Structure and Devices School of Materials Science&EngineeringBeijing Institute of TechnologyBeijing 100081China Experimental Center of Advanced Materials School of Materials Science&EngineeringBeijing Institute of TechnologyBeijing 100081China Shanghai Synchrotron Radiation Facility(SSRF) Shanghai Institute of Applied PhysicsChinese Academy of SciencesShanghai 201204China Institute of Applied Physics and Materials Engineering University of MacaoMacao 999078China

The development of efficient perovskite light-emitting diodes(PeLEDs)relies strongly on the fabrication of perovskite films with rationally designed structures(grain size,composition,surface,etc.).Therefore,an understanding of structure-performance relationships is of vital importance for developing high-performance perovskite devices,particularly for devices with in-situ fabricated perovskite nanocrystal *** this study,we reveal the vertical structure of an in-situ fabricated quasi-two-dimensional perovskite *** combining time-of-flight secondary ion mass spectrometry,energy dispersive spectroscopy,grazing incidence wide-angle X-ray scattering(GIWAXS),and low-temperature photoluminescence spectra,we illustrate that the resulting in-situ fabricated DPPA_(2)Cs_(n-1)Pb_(n)(Br_(0.3)I_(0.7))_(3n+1)(DPPA^(+):3,3-diphenylpropylammonium)film has a gradient structure with a very thin layer of ligands on the surface,predominantly small-n domains at the top,and predominantly large-n domains at the bottom owing to the solubility difference of the *** addition,GIWAXS measurements show that the domain of n=2 on the top layer has an ordered in-plane *** on the understanding of the film structure,we developed an in-situ fabrication process with ligand exchange to achieve efficient pure red PeLEDs at 638 nm with an average external quantum efficiency(EQE)of 7.4%.The optimized device had a maximum luminance of 623 cd/m^(2) with a peak EQE of 9.7%.

关键词： Light-emitting diodes Perovskite TOF-SIMS Vertical structure in-situ fabrication

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Elaborating strengthen mechanism of Pt-Ir solid solution superalloy at finite temperature

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Rare Metals 2024年第3期43卷 1243-1256页

作者： Wei Yu Xiao-Yu Chong Yun-Xuan Zhou Meng-Di Gan Ying-Xue Liang Yan Wei Ai-Min Zhang Chang-Yi Hu Xing-Yu Gao Li Chen Hai-Feng Song Jing Feng Faculty of Materials Science and Engineering Kunming University of Science and TechnologyKunming650093China Yunnan Precious Metals Laboratory Co.LTD Kunming650106China Laboratory of Computational Physics Institute of Applied Physics and Computational MathematicsBeijing100088China

Pt-Ir alloy is potential superalloys used above 1300℃because of their high strength and creep ***,the ductility of Pt-Ir alloy has rapidly deteriorated with the increase of Ir,resulting in poor *** work quantitatively evaluated the solid solution strengthening(SSS)and grain refinement strengthening(GRS)of Pt-Ir alloy using first-principles calculations combined with experimental ***,the stretching force constants in the second nearest neighbor region(SFC^(2nd))of pure Ir(193.7 eV·nm^(-2))are 3.40 times that of pure Pt(57.0 eV·nm^(-2)),i.e.,the interatomic interaction is greatly enhanced with the increase of Ir content,which leads to the decrease of ductility,and modulus misfit plays a dominant role in ***,the physical mechanisms responsible for the hardness(H_(V))of Pt-Ir alloy,using the power-law-scaled function of electron work function coupled SSS and GRS,are attributed to the electron redistribution caused by different Ir ***,a thorough assessment of the thermodynamic characteristics of Pt-Ir binary alloy was conducted,culminating in development of a mapping model that effectively relates enmposition,temperature and *** results revealed that the compressive strength incrcases with the Ir content,and the highest strength was observed in Pt_(0.25)Ir_(0.75).This study provides valuable insights into the Pt-Ir alloy system.

关键词： Elastic properties Phonon Solid solution strengthen Force constants CALPHAD

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Practical GHz single-cavity all-fiber dual-comb laser for high-speed spectroscopy

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光：科学与应用（英文版） 2025年第5期14卷 1354-1363页

作者： Lin Ling Wei Lin Zhaoheng Liang Minjie Pan Chiyi Wei Xuewen Chen Yang Yang Zhijin Xiong Yuankai Guo Xiaoming Wei Zhongmin Yang School of Physics and Optoelectronics South China University of TechnologyGuangzhouChina School of Physics and Optoelectronics South China University of TechnologyGuangzhouChina School of Materials Science and Engineering Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques South China University of TechnologyGuangzhouChina School of Physics and Optoelectronics South China University of TechnologyGuangzhouChina School of Materials Science and Engineering Guangdong Engineering Technology Research and Development Center of Special Optical Fiber Materials and Devices Guangdong Provincial Key Laboratory of Fiber Laser Materials and Applied Techniques South China University of TechnologyGuangzhouChina Research Institute of Future Technology South China Normal UniversityGuangzhouChina

Dual-comb spectroscopy(DCS)with few-GHz tooth spacing that provides a better trade-off between spectral resolution and refresh rate is a powerful tool for measuring and analyzing rapidly evolving transient *** such an exciting opportunity,existing technologies compromise either the spectral resolution or refresh rate,leaving few-GHz DCS with robust design largely unmet for frontier *** this work,we demonstrate a novel GHz DCS by exploring the multimode interference-mediated spectral filtering effect in an all-fiber ultrashort cavity *** GHz single-cavity all-fiber dual-comb source is seeded by a dual-wavelength mode-locked fiber laser operating at fundamental repetition rates of about 1.0 GHz differing by 148 kHz,which has an excellent stability in the free-running state that the Allan deviation is only 101.7 mHz for an average time of 1 *** to the large repetition rate difference between the asynchronous dichromatic pulse trains,the GHz DCS enables a refresh time as short as 6.75 μs,making it promising for studying nonrepeatable transient phenomena in real *** this end,the practicality of the present GHz DCS is validated by successfully capturing the'shock waves'of balloon and firecracker explosions *** GHz single-cavity all-fiber dual-comb system promises a noteworthy improvement in acquisition speed and reliability without sacrificing measurement accuracy,anticipated as a practical tool for high-speed applications.

关键词： laser all-fiber dual-comb high-speed practical single-cavity spectroscopy

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Concerted Steric and Electronic Strategy in Thermostable Salicylaldiminato Nickel Catalysts for Ethylene(Co)polymerization

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Chinese Journal of Polymer Science 2024年第8期42卷 1085-1092页

作者： Hong-Yu Ji Hong-Liang Mu Chun-Feng Tang Yu-Xing Zhang Yue Chi Zhong-Bao Jian Key Laboratory of Advanced Structural Materials Ministry of EducationSchool of Materials Science and EngineeringChangchun University of TechnologyChangchun 130012China State Key Laboratory of Polymer Physics and Chemistry Changchun Institute of Applied ChemistryChinese Academy of SciencesChangchun 130022China

Olefin polymerization is one of the most im portant chemical reactions in *** work presents a strategy that emphasizes the synergistic meta/poro-steric hindrance of N-aryl groups and electronic effects in newly synthesized neutral salicylaldiminato nickel *** nickel(Ⅱ)catalysts exhibit exceptional thermostability,ranging from 30℃to 130℃,demonstrating enhanced catalytic activities and broadly regulated polyethylene molecular weights(3-341 kg·mol^(-1))and controlled polymer branch density(2-102 brs/1000C).The preferred catalyst Ni3 with concerted steric and electronic effects enables the production of solid-state semi-crystalline polyethylene materials at temperatures below 90℃.Notably,Ni3 exhibits an impressive tolerance of 110℃and can withstand even the challenging polymerization temperature of 130℃,leading to the production of polyethylene wax and ***,functionalized polyethylene is produced.

关键词： Polyolefin Salicylaldiminato ligand Nickel catalyst Oil Wax

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Inhibiting oxygen vacancies and twisting NbO_(6) octahedron in erbium modified KNN-based multifunctional ceramics

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Journal of Materiomics 2024年第1期10卷 179-189页

作者： Lulu Gao Zhiyong Liu Pengrong Ren Renhong Liang Ting Li Kun Guo Bing Xie Jinshan Lu Pu Mao Jun Tian Longlong Shu School of Materials Science and Engineering Nanchang Hangkong UniversityNanchang330063China School of Materials Science and Engineering Xi'an University of TechnologyXi'an710048China School of Physics and Materials Science Nanchang UniversityNanchang330031China Institute of Applied Chemistry Jiangxi Academy of SciencesNanchang330096China

It is a challenge to obtain highly tunable multifunctional performances in one ferroelectric system by a simple approach to meet the miniaturization,integration,and functionalization requirements of advanced electronic ***,rare earth erbium(Er)modulated 0.9K_(0.5)Na_(0.5)NbO_(3)-0.1Sr(1-x)Er_(x)Ti_((1-x/4))O_(3),(0.9KNN-0.1ST:xEr)transparent-photoluminescent-ferroelectric energy storage multifunctional ceramics are prepared to solve this *** effect of lattice distortion and oxygen vacancies by Er doping on the optical and electrical properties is systematically *** Er^(3+)ions can introduce a large distortion of the NbO_(6) octahedron by replacing the A-site in KNN-based *** to the higher c/a ratio and lower oxygen vacancy content are simultaneously obtained in 0.9KNN-0.1ST:0.1Er *** effective energy storage density(Wrec)of 0.86 J/cm^(3),excellent near-infrared transmittance of 51.7%(1100 nm)and strong green upconversion photoluminescence are achieved in this multifunctional *** study provides a solid basis for rare earth ions doped ferroelectric ceramics with tunable multifunctional properties and has significant potential for applications in optoelectronic devices.

关键词： KNN Upconversion photoluminescence Multifunctional ceramics Oxygen vacancy Octahedron

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Enhancing the Performance of Perovskite Light-Emitting Diodes via Synergistic Effect of Defect Passivation and Dielectric Screening

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Nano-Micro Letters 2024年第10期16卷 244-256页

作者： Xuanchi Yu Jia Guo Yulin Mao Chengwei Shan Fengshou Tian Bingheng Meng Zhaojin Wang Tianqi Zhang Aung Ko Ko Kyaw Shuming Chen Xiaowei Sun Kai Wang Rui Chen Guichuan Xing Institute of Applied Physics and Materials Engineering University of MacaoAvenida da UniversidadeTaipaMacao 999078People's Republic of China Department of Electrical and Electronic Engineering Southern University of Science and TechnologyShenzhen 518055People's Republic of China

Metal halide perovskites,particularly the quasi-two-dimensional perovskite subclass,have exhibited considerable potential for next-generation electroluminescent materials for lighting and ***,the presence of defects within these perovskites has a substantial influence on the emission efficiency and durability of the *** this study,we revealed a synergistic passivation mechanism on perovskite films by using a dual-functional compound of potassium *** dual functional potassium bromide on the one hand can passivate the defects of halide vacancies with bromine anions and,on the other hand,can screen the charged defects at the grain boundaries with potassium *** approach effectively reduces the probability of carriers quenching resulting from charged defects capture and consequently enhances the radiative recombination efficiency of perovskite thin films,leading to a significant enhancement of photoluminescence quantum yield to near-unity values(95%).Meanwhile,the potassium bromide treatment promoted the growth of homogeneous and smooth film,facilitating the charge carrier injection in the ***,the perovskite light-emitting diodes based on this strategy achieve a maximum external quantum efficiency of~21%and maximum luminance of~60,000 cd m^(-2).This work provides a deeper insight into the passivation mechanism of ionic compound additives in perovskite with the solution method.

关键词： Synergistic passivation strategy Defects passivation Dielectric screening Perovskite light-emitting diodes

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materials-oriented integrated design and construction of structures in civil engineering—A review

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Frontiers of Structural and Civil engineering 2022年第1期16卷 24-44页

作者： Xing MING John C.HUANG Zongjin LI Institute of Applied Physics and Materials Engineering University of MacaoMacao SAR 999078China CHC Engineering LLCFairfaxVA 20030USA

Design is a goal-oriented planning activity for creating products,processes,and systems with desired functions through *** is a decision-making exploration:the design outcome may vary greatly depending on the designer’s knowledge and *** design is one type of design philosophy that takes an interdisciplinary and holistic *** civil engineering,structural design is such an activity for creating buildings and ***,structural design in many countries has emphasized a performance-based philosophy that simultaneously considers a structure’s safety,durability,serviceability,and ***,integrated design in civil engineering has become more popular,useful,and ***-oriented integrated design and construction of structures(MIDCS)combine materials engineering and structural engineering in the design stage:it fully utilizes the strengths of materials by selecting the most suitable structural forms and construction *** paper will explore real-world examples of MIDCS,including the realization of MIDCS in timber seismic-resistant structures,masonry arch structures,long-span steel bridges,prefabricated/on-site extruded light-weight steel structures,fiber-reinforced cementitious composites structures,and fiber-reinforced polymer bridge ***,advanced material design methods such as bioinspired design and structure construction technology of additive manufacturing are briefly reviewed and discussed to demonstrate how MIDCS can combine materials and structures.A unified strengthdurability design theory is also introduced,which is a human-centric,interdisciplinary,and holistic approach to the description and development of any civil infrastructure and includes all processes directly involved in the life cycle of the ***,this paper lays out future research directions for further development in the field.

关键词： integrated design and construction fiber-reinforced concrete fiber-reinforced polymer light-weight steel structures digital fabrication composites

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Effect of succinic acid on morphology transformation of the anhydrous magnesium carbonate particles prepared by magnesium chloride hexahydrate and urea

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Particuology 2024年第7期90卷 209-217页

作者： Song Liu Guojun Cheng Zhongfeng Tang School of Materials Science and Engineering Anhui University of Science and TechnologyHuainan232001China Shanghai Institute of Applied Physics Chinese Academy of SciencesShanghai 201800China Anhui Province Key Laboratory of Environment-friendly Polymer Materials Anhui UniversityHefei230601China

The homogeneous and controllable morphology of anhydrous magnesium carbonate(MgCO_(3))particles with excellent properties is difficult to obtain because of a variety of synthetic *** effect of succinic acid as a crystal modifier on the particle morphology transformation of anhydrous MgCO_(3)was investigated by the hydrothermal *** effect of the addition of succinic acid on the particles was similar to that of temperature *** morphology of particles with a folded diamond-like shape was gradually uniform,and the particle size was between 3.3 and 7.5μ*** MgCO_(3)particles prepared at pH 9 could easily agglomerate,and the average particle size increased from diamond-like to cube-like as the reaction time *** interaction between succinic acid and magnesium ions at different concentrations was the main factor responsible for the morphological *** pH,temperature,and time affected the molecular motion rate and crystal growth.

关键词： MgCO_(3) MgCl_(2)·6H_(2)O Urea Succinic acid Morphology

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