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Integration of Bio-Enzyme-Treated Super-Wood and AIE-Based Nonwoven Fabric for Efficient Evaporating the Wastewater with High Concentration of Ammonia Nitrogen

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Nano-Micro Letters 2025年第8期 9-24页

作者： Qian Ding Bingqi Jin Yinxia Zheng Huiru Zhao Jun Wang Haoxuan Li Dong Wang Ben Zhong Tang Engineering Research Center of Technical Textiles Ministry of EducationCollege of Materials Science and EngineeringDonghua University State Key Laboratory of Pollution Control and Resources Reuse School of Environmental Science and EngineeringTongji University Nonwoven Technology Laboratory College of Textile Science and EngineeringJiangnan University Centre for AIE Research Shenzhen Key Laboratory of Polymer Science and TechnologyGuangdong Research Center for Interfacial Engineering of Functional MaterialsCollege of Material Science and EngineeringShenzhen University School of Science and Engineering Shenzhen Institute of Aggregate Science and TechnologyThe Chinese University of Hong KongShenzhen (CUHK-Shenzhen)

The treatment of ammonia nitrogen wastewater（ANW） has garnered significant attention due to the ecology, and even biology is under increasing threat from over discharge ANW. Conventional ANW treatment methods often encounter challenges such as complex processes, high costs and secondary pollution. Considerable progress has been made in employing solar-induced evaporators for wastewater treatment. However, there remain notable barriers to transitioning from fundamental research to practical applications, including insufficient evaporation rates and inadequate resistance to biofouling. Herein, we propose a novel evaporator, which comprises a bio-enzyme-treated wood aerogel that serves as water pumping and storage layer, a cost-effective multi-walled carbon nanotubes coated hydrophobic/hydrophilic fibrous nonwoven mat functioning as photothermal evaporation layer,and aggregation-induced emission（AIE） molecules incorporated as anti-biofouling agent. The resultant bioinspired evaporator demonstrates a high evaporation rate of 12.83 kg m-2h-1when treating simulated ANW containing 30 wt% NH4Cl under 1.0 sun of illumination. AIE-doped evaporator exhibits remarkable photodynamic antibacterial activity against mildew and bacteria, ensuring outstanding resistance to biofouling over extended periods of wastewater treatment. When enhanced by natural wind under 1.0 sun irradiation, the evaporator achieves an impressive evaporation rate exceeding 20 kg m-2h-1. This advancement represents a promising and viable approach for the effective removal of ammonia nitrogen wastewater.

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Interface terminal group regulated organic phototransistors with tunable persistent and switchable photoconductivity

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Science China Chemistry 2022年第12期65卷 2567-2575页

作者： Di Xue Yingying Zhang Weijie Gong Yao Yin Zi Wang Lizhen Huang Lifeng Chi Institute of Functional Nano&Soft Materials(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials&DevicesSoochow UniversitySuzhou215123China Gusu Laboratory of Materials Suzhou215123China Macao Institute of Materials Science and Engineering(MIMSE) MUST-SUDA Joint Research Center for Advanced Functional MaterialsMacao University of Science and TechnologyTaipaMacao999078China

With both light detection and intrinsic amplification functions,organic phototransistors have demonstrated promising applications,including photodetection and *** achieve excellent photoresponse and superior photogain,a common and effective strategy is to modulate the trapping effect with the purpose of reducing recombination or prolonging the lifetime of the photogenerated charge ***,introducing trapping sites delicately is challenging and might sacrifice the response rate together with a typical persistent ***,we demonstrate a facile strategy for achieving high photo-responsive organic phototransistors with both persistent and switchable photoconductivity features via interface terminal group *** varying the terminate groups of self-assembled monolayer(SAMs)from the strong electron withdrawing group-F,neutral−CH_(3) to electron donating−NH_(2) on the dielectric surface,we realize both minority carrier trapping and majority carrier trapping in the organic phototransistor based on the C8-BTBT active *** electron withdrawing effect of F significantly enhances the minority carrier trapping process and yields a high photoresponsivity with a long-lasting persistent *** contrast,the electron donating group−NH_(2) with a distinct majority carrier trapping ability causes switchable photoconductivity so that the photocurrent can rise pronouncedly and fully decay along with light on/***,both cases can deliver high performance with photoresponsivities higher than 104 A W^(−1) together with a photosensitivity in the level of 107 and a detectivity of approximately 10^(15)–10^(16) *** a tunable,excellent photoresponse property enables the convenient exploration of organic phototransistors to satisfy different application requirements.

关键词： organic phototransistor surface modification trapping persistent photoconductivity

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CO electroreduction:What can we learn from its parent reaction,CO_(2) electroreduction?

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eScience 2023年第6期3卷 1-8页

作者： Xue Ding Jie Zhang Yanguang Li Institute of Functional Nano and Soft Materials(FUNSOM) Soochow UniversitySuzhou 215123China Jiangsu Key Laboratory for Advanced Negative Carbon Technologies Soochow UniversitySuzhou 215123China Macao Institute of Materials Science and Engineering(MIMSE) MUST-SUDA Joint Research Center for Advanced Functional MaterialsMacao University of Science and TechnologyMacao999078China

The CO electroreduction reaction(CORR)represents an important piece of the decarbonization puzzle and is heavily inspired by research on the CO_(2) electroreduction reaction(CO_(2)RR).Compared to its parent reaction,CORR circumvents the(bi)carbonate issue that plagues CO_(2)RR,potentially enabling greater stability and selectivity toward C2þproducts,particularly *** its unique potential,CORR still suffers from unsatisfactory *** this perspective article,we aim to provide a concise and informative overview of CORR and its close connection with CO_(2)*** start by briefly presenting the two reactions’similarities and differences,then discussing several catalyst design *** is followed by highlights of the latest results on device integration and ***,we offer our thoughts about possible future research opportunities that could render this technology a practical reality.

关键词： CO electroreduction CO_(2)electroreduction Catalysts Devices

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Lycium barbarum L.-Derived miR162a Functions on Osteoporosis Through Directly Promoting Osteoblast Formation

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engineering 2025年第3期46卷 162-171页

作者： Chunyan Gu Xichao Yu Xiaozhu Tang Leilei Gong Jingquan Tan Yuanjiao Zhang Huili Zheng Ze Wang Chenqian Zhang Yejin Zhu Zuojian Zhou Heming Yu Kai Xu Jinao Duan Xiaosong Gu Ye Yang Nanjing Hospital of Chinese Medicine Affiliated to Nanjing University of Chinese Medicine Nanjing 210022China School of Medicine&Holistic Integrative Medicine Nanjing University of Chinese MedicineNanjing 210023China Key Laboratory of Neuroregeneration of Jiangsu and Ministry of Education Nantong UniversityNantong 226001China Jiangsu Key Laboratory for Microbes and Functional Genomics Jiangsu Engineering and Technology Research Center for MicrobiologyCollege of Life SciencesNanjing Normal UniversityNanjing 210023China State Administration of Traditional Chinese Medicine Key Laboratory of Chinese Medicinal Resources Recycling Utilization Jiangsu Collaborative Innovation Center of Chinese Medicinal Resources IndustrializationNanjing University of Chinese MedicineNanjing 210023China School of Artificial Intelligence and Information Technology Nanjing University of Chinese MedicineNanjing 210023China

Traditional Chinese medicine(TCM)can help prevent or treat diseases;however,there are few studies on the active substances of *** example,Lycium barbarum *** been proven to be effective in treating osteoporosis for thousands of years,but its active substance remains to be *** by the efforts to modernize TCM,the present study focused on the novel active substance of Lycium barbarum *** reinforce kidney essence to produce bone *** deep sequencing analysis and stemloop polymerase chain reaction(PCR)assay revealed that miR162a,a Lycium barbarum L.-derived microRNA,can pass through the gastrointestinal tract to target the bone marrow in *** staining showed that miR162a was absorbed through systemic RNA interference defective transmembrane family member 1(SIDT1)in the *** prediction and luciferase reporter assay identified that miR162a targeted nuclear receptor corepressor(NcoR).Alizarin red staining and micro-computed tomography(microCT)confirmed that miR162a promoted osteogenic differentiation in bone marrow mesenchymal stem cells,zebrafish,and a mouse model of *** addition,transgenic Nicotiana benthamiana(***)leaves overexpressing miR162a were developed by agrobacterium infiltration *** and tartrate-resistant acid phosphatase staining confirmed that transgenic *** leaves effectively protected against osteoporosis in *** study mechanistically explains how Lycium barbarum *** osteoporosis and supports that Lycium barbarum *** kidney essence,thereby strengthening the ***162a expressed by transgenic plants may represent a novel and safe treatment for human osteoporosis.

关键词： Traditional Chinese medicine Lycium barbarum L. miR162a Osteoporosis Nuclear receptor corepressor Transgenic plants

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Stachyose modulates gut microbiota and alleviates DSS-induced ulcerative colitis in mice

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Food Science and Human Wellness 2023年第6期12卷 2211-2220页

作者： Chen Wang Junying Bai Botao Wang Leilei Yu Fengwei Tian Jianxin Zhao Hao Zhang Huayi Suo Wei Chen Qixiao Zhai College of Food Science Southwest UniversityChongqing 400715China State Key Laboratory of Food Science and Technology Jiangnan UniversityWuxi 214122China School of Food Science and Technology Jiangnan UniversityWuxi 214122China Bloomage Biotechnology Co. Ltd.Jinan 250000China National Engineering Research Center for Functional Food Jiangnan UniversityWuxi 214122China Wuxi Translational Medicine Research Center and Jiangsu Translational Medicine Research Institute Wuxi Branch Wuxi 214122China

Stachyose is a prebiotic that traditionally extracted from plants,such as *** has been demonstrated to alleviate intestinal inflammation by regulating gut microbiota,but the mechanism has been *** research aims to detect the potential mechanism of stachyose in alleviating the severity of ulcerative colitis(UC).The results indicated that the administration of stachyose could recover the body weight,protect against the colonic tissue damage,reduce the pro-inflammatory cytokines levels,and reverse the histological abnormalities in UC *** stachyose could restore dextran sulfate sodium(DSS)-induced disturbance in intestinal ***,the metabolome result of serum samples showed that stachyose treatment significantly altered serum metabolites against inflammatory responses in colitis ***,a significant correlation can be found between 23 metabolite biomarkers and 18 differential *** results provided a strong foundation for the future study of the protective role of stachyose in maintaining intestinal homeostasis.

关键词： Stachyose Prebiotic Colitis Metabonomics Gut microbiota

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Probiotics supplementation for management of type Ⅱ diabetes risk factors in adults with polycystic ovarian syndrome: a meta-analysis of randomized clinical trial

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Food Science and Human Wellness 2023年第4期12卷 1053-1063页

作者： Chengcheng Zhang Yingyue Sheng Jinchi Jiang Yuzheng Xue Leilei Yu Fengwei Tian Jianxin Zhao Hao Zhang Jian Jin Qixiao Zhai State Key Laboratory of Food Science and Technology Jiangnan UniversityWuxi 214122China School of Food Science and Technology Jiangnan UniversityWuxi 214122China Department of Gastroenterology Affiliated Hospital of Jiangnan UniversityWuxi 214122China National Engineering Research Center for Functional Food Jiangnan UniversityWuxi 214122China Wuxi Translational Medicine Research Center and Jiangsu Translational Medicine Research Institute Wuxi Branch Wuxi 214122China School of Pharmaceutical Sciences Jiangnan UniversityWuxi 214122China

This meta-analysis of randomized controlled trials aimed to evaluate the effects of probiotic supplementation on glucose homeostasis in patients with polycystic ovary syndrome(PCOS).The meta-analysis was performed in accordance with the Cochrane Handbook guidelines and relevant the preferred reporting items for systematic reviews and meta-analyses(PRISMA)statement *** 825 identified reports,11 randomized clinical trials were included in the *** analysis of pooled extracted data revealed that supplementation with probiotics significantly decreased fasting blood glucose(FBG,n=7;standardized mean difference(SMD)=−0.40;95%confidence interval(CI):−2.02,−0.02;P=0.04)and insulin levels(n=6;SMD=−0.57;95%CI:−0.89,−0.25;P=0.0004)and the homeostatic model assessment of insulin resistance(n=7;SMD=−0.64;95%CI:−0.96,−0.31;P=0.0001)while increasing the quantitative insulin sensitivity check index(QUICKI,n=5;SMD=0.58;95%CI:0.08,1.09;P=0.02)in patients with *** FBG-reducing effect decreased as the baseline body mass index(BMI)and mean age of the participants ***,a greater number of bacterial species and a higher bacterial dose were shown to reduce QUICKI *** systematic review indicated that probiotic supplementation may help to control glucose homeostasis in adults with polycystic ovarian syndrome.

关键词： Polycystic ovary syndrome Type 2 diabetes Glucose homeostasis Probiotic Meta-analysis Randomized clinical trial

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Physicochemical properties and antibacterial application of silver nanoparticles stabilized by whey protein isolate

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Food Bioscience 2022年第2期46卷 498-506页

作者： Aoqiong Zeng Beibei Wang Cheng Zhang Ruijin Yang Shuhuai Yu Wei Zhao State Key Laboratory of Food Science and Technology School of Food Science and TechnologyJiangnan University1800 Lihu AvenueWuxiJiangsu214122PR China National Engineering Research Center for Functional Food Jiangnan University1800 Lihu AvenueWuxiJiangsu214122PR China

Nano metal materials have been widely explored to be applied in medical,environmental,and material *** these nanoparticles,especially silver nanoparticles(AgNPs),have drawn increasing attention for antimicrobial *** researchers are keen on the development of the biologically friendly capping reagents for the synthesis of AgNPs,instead of unfriendly organic *** this study,the liquid chemical reduction method was used to synthesize AgNPs with edible whey protein isolate(WPI)as a capping *** WPI-AgNPs had a broad size distribution(average diameter of 138.6 nm),and their dimensions could be readily controlled in the range of 22.5-149.6 nm by introducing different concentrations of ***,it was confirmed that WPI-AgNPs were formed through two mechanisms,which were respectively reduced in situ(without the addition of NaCl)and ex situ(in presence of NaCl)to yield silver *** WPI-AgNPs synthesized in presence of 10 mM of NaCl as mediation reagent were stable at room temperature or 4℃ up to 3 ***,the synthesized WPI-AgNPs had a good antibacterial activity toward pathogens including Gram-negative *** and Gram-positive *** results shed light on method and capping reagent to stabilize silver nanoparticles,which highlighted the potential of WPI and chloride in metal nanoparticle synthesis.

关键词： Silver nanoparticles Whey protein isolate Chloride Liquid chemical reduction method

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Metal-Organic Framework-Derived Metallic Carbon with Record High Radon Gas Capture Performance

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CCS Chemistry 2024年第7期6卷 1789-1797页

作者： Shicheng Gong Yi Tao Lixi Chen Qiuting Xu Junhao Lu Fuyin Ma Xia Wang Guodong Li Jun Wan Guoxun Ji Linfeng He Xiaohui Yu Duo Zhang Xuhui Sun Zhifang Chai Shuao Wang State Key Laboratory of Radiation Medicine and Protection School for Radiological and Interdisciplinary Sciences(RAD-X)and Collaborative Innovation Center of Radiation Medicine of Jiangsu Higher Education InstitutionsSoochow UniversitySuzhou 215123 Institute of Functional Nano&Soft Materials Laboratory(FUNSOM) Jiangsu Key Laboratory for Carbon-Based Functional Materials and DevicesJiangsu Key Laboratory of Advanced Negative Carbon TechnologiesSoochow UniversitySuzhou 215123 School of Environment and Material Engineering Yantai UniversityYantai 264005 Xi’an Research Institute of Hi-Technology Hong Qing TownXi’an 710025 Shanghai Institute of Measurement and Testing Technology Shanghai 201203 Engineering Institute of Advanced Manufacturing and Modern Equipment Technology Jiangsu UniversityZhenjiang 212013

Developing efficient adsorbents for radon(Rn)capture from the ambient environment is of paramount importance for public ***,it poses a great challenge due to the chemical inertness and extremely low molar concentration of Rn in ***,we report a zeolite imidazolate frameworkderived metallic carbon adsorbent(Zn@NPC)with record high Rn removal performance under ambient *** one-step pyrolysis,the prepared Zn@NPC possesses pores with a preference for Rn and atomically dispersed Zn sites,achieving a high Rn removal efficiency that doubles in adsorption coefficient(9.47 L·g^(−1))and triples in adsorption kinetic coefficient(20.25 mL·g^(−1)·min^(−1))over the benchmark Rn adsorbent coconut activated *** functional theory calculations elucidate the important role of the metal polarization effect,which cooperates with the pore size confinement effect to boost the overall Rn adsorption *** work launches a promising alternative for practical Rn capture.

关键词： radon removal metal-organic frameworks microporous carbon synergistic effect dynamic adsorption

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Concentration of n-3 polyunsaturated fatty acid glycerides by Candida antarctica lipase A-catalyzed selective methanolysis

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Food Bioscience 2022年第2期46卷 423-429页

作者： Cong Jiang Ye Chen Yifan Wang Caiming Li Xiaosan Wang Zong Meng Xingguo Wang Collaborative Innovation Center of Food Safety and Quality Control in Jiangsu Province National Engineering Research Center for Functional FoodSchool of Food Science and TechnologyJiangnan University1800 Lihu RoadWuxiJiangsu214122PR China State Key Laboratory of Food Science and Technology School of Food Science and TechnologyJiangnan University1800 Lihu RoadWuxiJiangsu214122PR China

n-3 polyunsaturated fatty acids(n-3 PUFA)have biologically important functions in human beings,but their contents in natural oils are usually *** study investigated the concentration of n-3 PUFA-enriched glycerides by Candida antarctica lipase A(CAL-A)-catalyzed selective methanolysis of algal ***,lipases and acyl acceptors were ***,the methanolysis conditions including methanol concentration in aqueous solution,molar ratio of methanol to oil,reaction temperature,lipase loading and reaction time,were *** results indicated that CAL-A could effectively identify n-3 PUFA during *** fatty acids and monounsaturated fatty acids were released from algal oil by CAL-A-catalyzed methanolysis,causing the production of n-3 PUFA-enriched *** optimal conditions(3:1 of molar ratio of methanol to algal oil,20%methanol aqueous solution,6%CAL-A dosage,25℃,18 h),the n-3 PUFA content increased from the initial 45.96%to 73.96%,with an n-3 PUFA yield of 81.76%.The reusability of CAL-A demonstrated that under optimal conditions the lipase could be used for 8 ***,this enzymatic process is efficient for synthesis of n-3 PUFA-enriched glycerides.

关键词： n-3 PUFA concentrates Candida antarctica lipase A(CAL-A) Selective methanolysis Glycerides

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Effects of Bifidobacterium longum CCFM5871 as an adjunct starter culture on the production of fermented milk

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Food Bioscience 2022年第6期50卷 1949-1958页

作者： Ruocen Tian Zhiming Yu Leilei Yu Fengwei Tian Jianxin Zhao Hao Zhang Wei Chen Qixiao Zhai State Key Laboratory of Food Science and Technology Jiangnan UniversityWuxiJiangsu214122PR China School of Food Science and Technology Jiangnan UniversityWuxiJiangsu214122PR China Wuxi People's Hospital Afliated to Nanjing Medical University WuxiJiangsu214122PR China National Engineering Research Center for Functional Food Jiangnan UniversityWuxiJiangsu214122PR China Wuxi Translational Medicine Research Center and Jiangsu Translational Medicine Research Institute Wuxi Branch WuxiJiangsu214122PR China

Bifidobacterium has been widely studied for its probiotic properties. In our previous study, Bifidobacterium longum CCFM5871 (CCFM5871) showed potential to relieve inflammation and constipation. In current study, we investigated the application of CCFM5871 as an adjunct starter culture for the production of fermented milk. First, genome analysis indicated that CCFM5871 possess various carbohydrate metabolic pathways, including the Leloir pathway of galactose metabolism and galactose related genes GH2 and GH27. Comparative genomic analysis shows that similar functional gene were detected in other bifidobacteria strains applied in dairy fermentation. Then the sugar metabolism phenotype experiment verified the result of genomic analysis. Subsequently, we evaluated the effects of CCFM5871 supplementation on the production and storage of fermented milk by monitoring changes in multiple parameters over 14 days of storage at 4℃, including pH, titratable acidity, physical properties, volatile flavor compounds, and sensory quality. The bacterial level was significantly higher at the fermentation termination than the fermentation initiation, indicating that CCFM5871 can be regarded as a candidate for adjunct start culture. Compared to the control group, supplementation with CCFM5871 increased acidification and solidification of fermented milk. Moreover, we revealed that there was no other significant difference between the yogurt fermented with CCFM5871 and the yogurt with culture only in flavor and taste. In summary, our results identified that CCFM5871 may be an appropriate co-culture for fermented milk, and the genomic analysis may be instructive for future to filter the culture in fermented milk.

关键词： Bifidobacterium longum Fermented milk Storage stability Electronic nose Electronic tongue

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