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SSRN 2025年

作者： Ren, Jinglin Chen, Yulin Gu, Jiawei Zhang, Peng Chen, Chen Zhang, Jian Jiangsu Key Laboratory of Advanced Food Manufacturing Equipment and Technology School of Intelligent Manufacturing Jiangnan University Wuxi214122 China

Shape memory effect (SME) in shape memory alloys (SMAs) results from deformation below Af, accompanying pre-strain effect (PSE) which was usually implicated by dislocations. We systematically investigate the effects o... 详细信息

关键词： Titanium alloys

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基于预连接镍链的高应变敏感度动态可调电磁干扰屏蔽弹性体

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Science China Materials 2024年第2期67卷 629-641页

作者：卞敬周兴成周翔马林峰朱先军李建民刘淑娟赵强 College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology) National and Local Joint Engineering Laboratory of RF Integration and Micro-Assembly TechnologyNanjing University of Posts and TelecommunicationsNanjing 210023China State Key Laboratory of Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced Materials(IAM)Nanjing University of Posts&TelecommunicationsNanjing 210023China

具有动态可调电磁屏蔽性能的电磁干扰屏蔽材料备受关注,但其目前仍然存在制备复杂、厚度大、触发方式不便、调节范围窄等缺点.我们通过将尖刺镍微粒精确地分散到聚二甲基硅氧烷基体中形成预连接的链状结构,制备出了具有可开关电磁屏蔽... 详细信息

具有动态可调电磁屏蔽性能的电磁干扰屏蔽材料备受关注,但其目前仍然存在制备复杂、厚度大、触发方式不便、调节范围窄等缺点.我们通过将尖刺镍微粒精确地分散到聚二甲基硅氧烷基体中形成预连接的链状结构,制备出了具有可开关电磁屏蔽性能的弹性体材料.弹性体在机械拉伸和释放过程中表现出连续和可逆的电磁干扰屏蔽性能.原始弹性体具有良好的阻抗匹配和低介电损耗,允许大部分电磁波通过.拉伸使预连接的短链彼此接触,在内部形成大量的微尺度导电网络,显著增强了电导损耗能力,实现了较强的电磁干扰屏蔽能力.此外,我们通过无线应变传感系统验证了智能电磁干扰屏蔽弹性体的应用潜力,证明了可穿戴智能电磁干扰屏蔽精确监测人体运动的可能性.

关键词： adjustable electromagnetic interference shielding conductive elastomer electromagnetic sensing negative piezoresistivity

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Rapid Access to Polysubstituted Tetrahydrocarbazol-4-ones via Sequential Selective C—H Functionalization from N-Nitrosoanilines

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Chinese Journal of Chemistry 2023年第16期41卷 1957-1962页

作者： Chan Li Yanchen Yang Feifei Fang Chaoyi Liu Chunpu Li Dechuan Wang Hong Liu School of Science China Pharmaceutical UniversityNanjingJiangsu 211198China State Key Laboratory of Drug Research Shanghai Institute of Materia MedicaChinese Academy of Sciences555 Zu Chong Zhi Road Shanghai 201203 China School of PharmacyChina Pharmaceutical UniversityNanjingJiangsu 211198China Lingang Laboratory Shanghai 200031China School of Pharmaceutical Science and Technology Hangzhou Institute for Advanced StudyUCASHangzhouZhejiang 310024China University of Chinese Academy of Sciences Beijing 100049China

Comprehensive Summary Herein,we have developed a strategy of Rh(III)-catalyzed C—H activation of N-nitrosoanilines and iodonium ylides to construct novel tetralydrocarbzol-4-one scaffolds,which provided valuable templates for sequential C—H functionalization such as alkylation,alkenylation,amidation and(hetero)arylation at C^(5)-position of tetralydrocarbzol-4-one with different coupling ***-scale synthesis and further transformations of tetralydrocarbzol-4-one derivatives to Ondansetron and its analogues demonstrated the utility of this protocol,which enabled the concise and diverse construction of biologically active molecules.

关键词： C-H activation Cross dehydrogenative coupling Rhodium catalysis Iridium catalysis Alkenylation Amaidiation Heteroarylation

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Tailoring activation sites of metastable distorted 1T′-phase MoS_(2) by Ni doping for enhanced hydrogen evolution

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Nano Research 2022年第7期15卷 5946-5952页

作者： Mingming Liu Hengxu Li Shijie Liu Longlu Wang Lingbin Xie Zechao Zhuang Chun Sun Jin Wang Meng Tang Shujiang Sun Shujuan Liu Qiang Zhao College of Electronic and Optical Engineering&College of Flexible Electronics(Future Technology) Nanjing University of Posts&TelecommunicationsNanjing 210023China State Key Laboratory of Organic Electronics and Information Displays&Jiangsu Key Laboratory for Biosensors Institute of Advanced Materials(IAM)&Institute of Flexible Electronics(Future Technology)Nanjing University of Posts&TelecommunicationsNanjing 210023China Department of Chemistry Tsinghua UniversityBeijing 100084China

Heteroatom doping is a promising approach to enhance catalytic activity by modulating physical properties,electronic structure,and reaction ***,we demonstrate that appropriate Ni-doping could trigger a preferential transition of the basal plane from 2H(trigonal prismatic)to 1T′(clustered Mo)by inducing lattice distortion and S vacancy(SV)and thus dramatically facilitate its catalytic hydrogen evolution *** is noteworthy that the unique catalysts did possess superior catalytic performance of hydrogen evolution reaction(HER).The rate of photocatalytic hydrogen evolution could reach 20.45 mmol·g^(−1)·h^(−1) and reduced only slightly in the long period of the photocatalytic ***-principles calculations reveal that the distorted Ni-1T′-MoS_(2) with SV could generate favorable water adsorption energy(Ead(H_(2)O))and Gibbs free energy of hydrogen adsorption(∆GH).This work exhibits a facile and promising pathway for synergistically regulating physical properties,electronic structure,or wettability based on the doping strategy for designing HER electrocatalysts.

关键词： Ni doping S vacancy phase transformation electronic structure hydrogen evolution

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Balancing Energy-Level Difference for Efficient n-i-p Perovskite Solar Cells with Cu Electrode

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Energy Material Advances 2022年第1期2022卷 157-164页

作者： Ziqi Xu Nengxu Li Xiuxiu Niu Huifen Liu Guilin Liu Qi Chen Huanping Zhou Beijing Key Laboratory for Theory and Technology of Advanced Battery Materials Key Laboratory of Polymer Chemistry and Physics of Ministry of EducationBIC-ESATSchool of Materials Science and EngineeringPeking UniversityBeijing 100871China China Automotive Technology and Research Center Co. Ltd.TianjinChina Experimental Centre for Advanced Materials School of Materials Science and EngineeringBeijing Institute of TechnologyBeijing 100081China School of Science Jiangnan UniversityWuxiJiangsu 214122China

Developing low cost and stable metal electrode is crucial for mass production of perovskite solar cells(PSCs).As an earthabundant element,Cu becomes an alternative candidate to replace noble metal electrodes such as Au and Ag,due to its comparable physiochemical properties with simultaneously good stability and low ***,the undesirable band alignment associated with the device architecture impedes the exploration of efficient Cu-based n-i-p ***,we demonstrated the ability of tuning the Fermi level(E_(F))of hole transport layer(HTL)to reduce the energy level difference(Schottky barrier)between HTLs and ***,we identified that the balance of energy level difference between HTL and adjacent layers(including perovskite and Cu)is crucial to efficient carrier transportation and photovoltaic performance improvement in the *** the optimized condition,we achieve a device power conversion efficiency(PCE)of 20.10%,which is the highest on the planar n-i-p PSCs with Cu ***,the Cu-based PSCs can maintain 92%of their initial efficiency after 1000 h storage,which is comparable with Au-based *** present work not only extends the understanding on the band alignment of neighboring semiconductor functional layer in the device architecture to improve the resulting performance but also suggests great potential of Cu electrode for application in PSCs community.

关键词： perovskite alignment electrode

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All-weather,natural silent speech recognition via machine-learning-assisted tattoo-like electronics

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npj Flexible Electronics 2021年第1期5卷 183-191页

作者： Youhua Wang Tianyi Tang Yin Xu Yunzhao Bai Lang Yin Guang Li Hongmiao Zhang Huicong Liu YongAn Huang State Key Laboratory of Digital Manufacturing Equipment and Technology Huazhong University of Science and TechnologyWuhanChina Flexible Electronics Research Center Huazhong University of Science and TechnologyWuhanChina School of Mechanical and Electric Engineering Jiangsu Provincial Key Laboratory of Advanced RoboticsSoochow UniversitySuzhouChina State Key Laboratory of Industrial Control Technologyg Institute of Cyber Systems and ControlZhejiang UniversityHangzhouChina

The internal availability of silent speech serves as a translator for people with aphasia and keeps human–machine/human interactions working under various *** paper develops a silent speech strategy to achieve all-weather,natural *** strategy requires few usage specialized skills like sign language but accurately transfers high-capacity information in complicated and changeable daily *** the strategy,the tattoo-like electronics imperceptibly attached on facial skin record high-quality bio-data of various silent speech,and the machine-learning algorithm deployed on the cloud recognizes accurately the silent speech and reduces the weight of the wireless acquisition module.A series of experiments show that the silent speech recognition system(SSRS)can enduringly comply with large deformation(~45%)of faces by virtue of the electricitypreferred tattoo-like electrodes and recognize up to 110 words covering daily vocabularies with a high average accuracy of 92.64%simply by use of small-sample machine *** successfully apply the SSRS to 1-day routine life,including daily greeting,running,dining,manipulating industrial robots in deafening noise,and expressing in darkness,which shows great promotion in real-world applications.

关键词： translator weather silent

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Polarization-controlled dual resonant lattice Kerker effects

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Nano Research 2023年第2期16卷 3195-3200页

作者： Lei Xiong Xueqian Zhao Xiang Du Shuai Chen Yuanfu Lu Hongwei Ding Guangyuan Li School of Information Science and Engineering Yunnan UniversityKunming 650500China CAS Key Laboratory of Human-Machine Intelligence-Synergy Systems Shenzhen Institute of Advanced TechnologyChinese Academy of SciencesShenzhen 518055China School of Computer Electronic and InformationGuangxi UniversityNanning 530004China College of Physics and Electronic Technology Anhui Normal UniversityWuhu 241000China Tianjin H-Chip Technology Group Corporation Tianjin 300467China SIAT Branch Shenzhen Institute of Artificial Intelligence and Robotics for SocietyShenzhen 518055China

The generalized Kerker effects have attracted increasing interests in recent years due to their abilities to manipulate the far-field properties of ***,the dual-polarized generalized Kerker effect enabling different tailoring of orthogonally-polarized electromagnetic waves has not yet been ***,we demonstrate polarization-controlled dual resonant lattice Kerker effects in periodic silicon *** varying the incident angle,the electric dipole and magnetic dipole surface lattice resonances can spectrally overlap,causing zero reflectance and unitary transmittance,i.e.,the resonant lattice Kerker *** incident angle for achieving this effect can be tuned differently for s-and p-polarizations over large regions by varying the nanodisk size or the lattice *** proposed dual-polarized resonant lattice Kerker effects open up avenues for polarization-controlled manipulation of the phase and wavefront of light with metasurfaces.

关键词： Kerker effect surface lattice resonances dual-polarized silicon metasurface

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Novel Cellulosic Fiber Composites with Integrated Multi-Band Electromagnetic Interference Shielding and Energy Storage Functionalities

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Nano-Micro Letters 2025年第5期17卷 508-524页

作者： Xuewen Han Cheng Hao Yukang Peng Han Yu Tao Zhang Haonan Zhang Kaiwen Chen Heyu Chen Zhenxing Wang Ning Yan Junwen Pu Beijing Key Laboratory of Lignocellulosic Chemistry College of Materials Science and TechnologyBeijing Forestry UniversityBeijing 100083People’s Republic of China Department of Chemical Engineering and Applied Chemistry University of TorontoTorontoON M5S3E5Canada Key Laboratory of Advanced Marine Materials Ningbo Institute of Materials Technology and EngineeringChinese Academy of SciencesNingbo 315201People’s Republic of China College of Mechanical and Electronic Engineering Northwest A&F UniversityYangling 712100ShaanxiPeople’s Republic of China Jiangsu Provincial Key Lab of Sustainable Pulp and Paper Technology and Biomass Materials Nanjing Forestry UniversityNanjing 210037People’s Republic of China Co-Innovation Center of Efficient Processing and Utilization of Forest Resources Nanjing Forestry UniversityNanjing 210037People’s Republic of China

In an era where technological advancement and sustainability converge,developing renewable materials with multifunctional integration is increasingly in *** study filled a crucial gap by integrating energy storage,multi-band electromagnetic interference(EMI)shielding,and structural design into bio-based ***,conductive polymer layers were formed within the 2,2,6,6-tetramethylpiperidine-1-oxide(TEMPO)-oxidized cellulose fiber skeleton,where a mild TEMPO-mediated oxidation system was applied to endow it with abundant macropores that could be utilized as active sites(specific surface area of 105.6 m2 g-1).Benefiting from the special hierarchical porous structure of the material,the constructed cellulose fiber-derived composites can realize high areal-specific capacitance of 12.44 F cm^(-2)at 5 m A cm^(-2)and areal energy density of 3.99 m Wh cm^(-2)(2005 m W cm^(-2))with an excellent stability of maintaining 90.23%after 10,000 cycles at 50 m A cm^(-2).Meanwhile,the composites showed a high electrical conductivity of 877.19 S m-1 and excellent EMI efficiency(>99.99%)in multiple wavelength *** composite material’s EMI values exceed 100 d B across the L,S,C,and X bands,effectively shielding electromagnetic waves in daily *** proposed strategy paves the way for utilizing bio-based materials in applications like energy storage and EMI shielding,contributing to a more sustainable future.

关键词： Cellulose fiber skeleton TEMPO mediated oxidation In-situ polymerization Multi-band EMI shielding Energy storage

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Target Defense with Multiple Defenders and an Agile Attacker via Residual Policy Learning

arXiv

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arXiv 2025年

作者： Tao, Jiyue Shen, Tongsheng Zhao, Dexin Zhang, Feitian Robotics and Control Laboratory Department of Advanced Manufacturing and Robotics College of Engineering and the State Key Laboratory of Turbulence and Complex Systems Peking University Beijing100871 China National Innovation Institute of Defense Technology Beijing100071 China

The target defense problem involves intercepting an attacker before it reaches a designated target region using one or more defenders. This letter focuses on a particularly challenging scenario in which the attacker is more agile than the defenders, significantly increasing the difficulty of effective interception. To address this challenge, we propose a novel residual policy framework that integrates deep reinforcement learning (DRL) with the force-based Boids model. In this framework, the Boids model serves as a baseline policy, while DRL learns a residual policy to refine and optimize the defenders’ actions. Simulation experiments demonstrate that the proposed method consistently outperforms traditional interception policies, whether learned via vanilla DRL or fine-tuned from force-based methods. Moreover, the learned policy exhibits strong scalability and adaptability, effectively handling scenarios with varying numbers of defenders and attackers with different agility levels. Copyright © 2025, The Authors. All rights reserved.

关键词： Adversarial machine learning

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Direct ink writing of conductive materials for emerging energy storage systems

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Nano Research 2022年第7期15卷 6091-6111页

作者： Ting Huang Wenfeng Liu Chenliang Su Ya-yun Li Jingyu Sun College of Materials Science and Engineering Shenzhen Key Laboratory of Special Functional Materials&Shenzhen Engineering Laboratory for Advance Technology of CeramicsShenzhen UniversityShenzhen 518060China College of Energy Soochow Institute for Energy and Materials InnovationsJiangsu Provincial Key Laboratory for Advanced Carbon Materials and Wearable Energy TechnologiesSoochow UniversitySuzhou 215006China Institute of Microscale Optoelectronics International Collaborative Laboratory of 2D Materials for Optoelectronic Science&Technology of Ministry of EducationShenzhen UniversityShenzhen 518060China

Direct ink writing(DIW)has recently emerged as an appealing method for designing and fabricating three-dimensional(3D)*** 3D structures can be built layer-by-layer via digitally controlled extrusion and deposition of aqueous-based colloidal *** formulation of well-dispersed suspensions with specific rheological behaviors is a prerequisite for the use of this *** this review article,the fundamental concepts of DIW are presented,including the operation principles and basic *** strategies used for ink formulation are discussed with a focus on the most widely used electrode materials,including graphene,Mxenes,and carbon *** recent progress in printing design of emerging energy storage systems,encompassing rechargeable batteries,supercapacitors,and hybrid capacitors,is *** and future perspectives are also covered to provide guidance for the future development of DIW.

关键词： direct ink writing energy storage ink formulation conductive materials structure-performance relationship

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